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DOE OSTI2021

Time-resolved particle image velocimetry

Time-resolved particle image velocimetry (TR-PIV) has become widespread in fluid dynamics. Essentially a velocity field movie, the dynamic content provides temporal as well as spatial information, in contrast to conventional PIV offering only statistical ensembles of flow quantities. From these time series arise further analyses such as accelerometry, space-time correlations, frequency spectra of turbulence including spatial variability, and derivation of pressure fields and forces. The historical development of TR-PIV is chronicled, culminating in an assessment of the current state of technology in high-repetition-rate lasers and high-speed cameras. Commercialization of pulse-burst lasers has expanded TR-PIV into more flows, including the compressible regime, and has achieved MHz rates. Particle response times and peak locking during image interrogation require attention but generally are not impediments to success. Accuracy considerations are discussed, including the risks of noise and aliasing in spectral content. Oversampled TR-PIV measurements allow use of multi-frame image interrogation methods, which improve the precision of the correlation and raise the velocity dynamic range of PIV. In combination with volumetric methods and data assimilation, a full four-dimensional description of a flow is not only achievable but becoming standardized. Lastly, a survey of exemplary applications is followed by a few predictions concerning the future of TR-PIV.

47 OTHER INSTRUMENTATION↗

DOE OSTI2024

Collaborative Research: Enhancing Laser-Based Ion Sources with High Data Rate Techniques

This collaborative research project focuses on leveraging advanced machine learning techniques to analyze and optimize data from high-repetition-rate laser experiments. The main goal is to apply modern computing hardware, customized data acquisition firmware/software, and machine learning approaches to improve data analysis and experimental control. The project also explores how methodology can be developed on smaller-scale experimental setups and then translated to larger facilities within DOE's LaserNetUS network. With extensive data collection and modeling, the research aims to predict and optimize experimental parameters to enhance performance and efficiency.

47 OTHER INSTRUMENTATION↗

DOE OSTI2025

A hybrid neural architecture: Online attosecond x-ray characterization

The emergence of high-repetition-rate x-ray free-electron lasers (XFELs), such as SLAC’s LCLS-II, serves as our canonical example for autonomous controls that necessitate high-throughput diagnostics paired with streaming computational pipelines capable of single-shot analysis with extremely low latency. We present the deterministic characterization with an integrated parallelizable hybrid resolver architecture, a hybrid machine learning framework designed for fast, accurate analysis of XFEL diagnostics using angular streaking-based sinogram images. This architecture integrates convolutional neural networks and bidirectional long short-term memory models to denoise input, identify x-ray sub-spike features, and extract sub-spike relative delays with sub-30 attosecond temporal resolution. Deployed on low-latency hardware, it achieves over 10 kHz throughput with 168.3 μs inference latency, indicating scalability to 14 kHz with field-programmable gate array integration. By transforming regression tasks into classification problems and leveraging optimized error encoding, we achieve high precision with low-latency performance that is critical for real-time streaming event selection and experimental control feedback signals. This represents a key development in real-time control pipelines for next-generation autonomous science, generally, and high repetition-rate x-ray experiments in particular.

Accelerator Physics (physics.acc-ph)↗

DOE OSTI2023

Ultra-short pulse laser acceleration of protons to 80 MeV from cryogenic hydrogen jets tailored to near-critical density

Laser plasma-based particle accelerators attract great interest in fields where conventional accelerators reach limits based on size, cost or beam parameters. Despite the fact that particle in cell simulations have predicted several advantageous ion acceleration schemes, laser accelerators have not yet reached their full potential in producing simultaneous high-radiation doses at high particle energies. The most stringent limitation is the lack of a suitable high-repetition rate target that also provides a high degree of control of the plasma conditions required to access these advanced regimes. Here, we demonstrate that the interaction of petawatt-class laser pulses with a pre-formed micrometer-sized cryogenic hydrogen jet plasma overcomes these limitations enabling tailored density scans from the solid to the underdense regime. Our proof-of-concept experiment demonstrates that the near-critical plasma density profile produces proton energies of up to 80 MeV. Based on hydrodynamic and three-dimensional particle in cell simulations, transition between different acceleration schemes are shown, suggesting enhanced proton acceleration at the relativistic transparency front for the optimal case.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2024

Plasma-based particle sources

High-brightness particle beams generated by advanced accelerator concepts have the potential to become an essential part of future accelerator technology. In particular, high-gradient accelerators can generate and rapidly accelerate particle beams to relativistic energies. The rapid acceleration and strong confining fields can minimize irreversible detrimental effects to the beam brightness that occur at low beam energies, such as emittance growth or pulse elongation caused by space charge forces. Due to the high accelerating gradients, these novel accelerators are also significantly more compact than conventional technology. Advanced accelerators can be extremely variable and are capable of generating particle beams with vastly different properties using the same driver and setup with only modest changes to the interaction parameters. So far, efforts have mainly been focused on the generation of electron beams, but there are concepts to extend the sources to generate spin-polarized electron beams or positron beams. The beam parameters of these particle sources are largely determined by the injection and subsequent acceleration processes. Although, over the last decade there has been significant progress, the sources are still lacking a sufficiently high 6-dimensional (D) phase-space density that includes small transverse emittance, small energy spread and high charge, and operation at high repetition rate. This is required for future particle colliders with a sufficiently high luminosity or for more near-term applications, such as enabling the operation of free-electron lasers (FELs) in the X-ray regime. Major research and development efforts are required to address these limitations in order to realize these approaches for a front-end injector for a future collider or next-generation light sources. In particular, this includes methods to control and manipulate the phase-space and spin degrees-of-freedom of ultrashort plasma-based electron bunches with high accuracy, and methods that increase efficiency and repetition rate. These efforts also include the development of high-resolution diagnostics, such as full 6D phase-space measurements, beam polarimetry and high-fidelity simulation tools. A further increase in beam luminosity can be achieve through emittance damping. Emittance cooling via the emission of synchrotron radiation using current technology requires kilometer-scale damping rings. For future colliders, the damping rings might be replaced by a substantially more compact plasma-based approach. Here, plasma wigglers with significantly stronger magnetic fields are used instead of permanent-magnet based wigglers to achieve similar damping performance but over a two orders of magnitude reduced length.

43 PARTICLE ACCELERATORS↗

NASA NTRS2003

Review of Laser Ablation Process for Single Wall Carbon Nanotube Production

Different types of lasers are now routinely used to prepare single wall carbon nanotubes (SWCNTs). The original method developed by researchers at Rice University utilized a "double pulse laser oven" process. A graphite target containing about 1 atomic percent of metal catalysts is ablated inside a 1473K oven using laser pulses (10 ns pulse width) in slow flowing argon. Two YAG lasers with a green pulse (532 nm) followed by an IR pulse (1064 nm) with a 50 ns delay are used for ablation. This set up produced single wall carbon nanotube material with about 70% purity having a diameter distribution peaked around 1.4 nm. The impurities consist of fullerenes, metal catalyst clusters (10 to 100 nm diameter) and amorphous carbon. The rate of production with the initial set up was about 60 mg per hour with 10Hz laser systems. Several researchers have used variations of the lasers to improve the rate, consistency and study effects of different process parameters on the quality and quantity of SWCNTs. These variations include one to three YAG laser systems (Green, Green and IR), different pulse widths (nano to microseconds as well as continuous) and different laser wavelengths (Alexandrite, CO, CO2, free electron lasers in the near to far infrared). It is noted that yield from the single laser (Green or IR) systems is only a fraction of the two laser systems. The yield seemed to scale up with the repetition rate of the laser systems (10 to 60 Hz) and depended on the beam uniformity and quality of the laser pulses. The shift to longer wavelength lasers (free electron, CO and CO2) did not improve the quality, but increased the rate of production because these lasers are either continuous (CW) or high repetition rate pulses (kHz to MHz). The average power and the peak power of the lasers seem to influence the yields. Very high peak powers (MegaWatts per square centimeter) are noted to increase ablation of bigger particles with reduced yields of SWCNTs. Increased average powers seem to help the conversion of the carbon from target into vapor phase to improve formation of nanotubes. The use of CW far infrared lasers reduced the need for the oven, at the expense of controlled ablation. Some of these variations are tried with different combinations and concentrations of metal catalysts (Nickel with Cobalt, Iron, Palladium and Platinum) different buffer gases (e.g. Helium); with different oven temperatures (Room temperature to 1473K); under different flow conditions (1 to 1000 kPa) and even different porosities of the graphite targets. It is to be noted that the original Cobalt and Nickel combination worked best, possibly because of improved carbonization with stable crystalline phases. The mean diameter and yield seemed to increase with increasing oven temperatures. Thermal conductivity of the buffer gas and flow conditions dictate the quality as well as quantity of the SWCNTs. Faster flows, lower pressures and heavier gases seem to increase the yields. This review will attempt to cover all these variations and their relative merits. Possible growth mechanisms under these different conditions will also be discussed.

Arepalli, Sivaram↗

DOE OSTI2022

Towards a Counting Point Detector for Nanosecond Coherent X-ray Science

We present the technical realization of a high-speed hard X-ray single-photon counting-detection scheme based on a commercial avalanche silicon photodiode and high-speed oscilloscope. The development is motivated by the need to perform pulse-resolved photon-correlation and pump-probe studies at synchrotron sources with densely packed pulse patterns that result in high repetition rate pulses on the order of hundreds of MHz. Commissioning experiments are performed at the 1C PAL-KRISS beamline at PLS-II of South Korea operating at a burst mode maximum repetition rate of 500 MHz. In such a high count-rate measurement, detector dead-time can lead to a distortion of counting statistics. We are able to model the counting behavior of our detector under these conditions with a detector dead-time comparable to time between X-ray pulses, implying that nanosecond X-ray photon correlation spectroscopy should be possible at diffraction-limited light sources.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Manufacturing Supply Chain Development for Modular Solar-Thermochemical Conversion Platform [Abstract]

We will develop a tunable pulsed electron source capable of generating variable intensity highly-focused electron pulses at high repetition rates. Specifically, we need to demonstrate a high-speed variable electron gun capable of generating a variable intensity electron pulse containing between 102 and 105 electrons with an accelerating voltage of 1kV focused into a spot size <100nm in diameter at with a pulse rate >10MHz (with path to 300MHz). This combined performance cannot be achieved by commercially available electron sources. The primary technology path selected for this work will be to use a photocathode approach, where an easily modulated UV laser is used to stimulate electron emission. The approach utilizes the advances made in the development of the Dynamic TEM (DTEM), though this project will be simpler in that the pulse intensity is lower and there is no requirement for coherency. Alternate paths, including using a traditional electron beam modulated using a v-shaped slit and electrostatically deflecting the beam to adjust intensity; will also be considered for future capabilities. The electron source will then be used generate optically stimulated luminescence (OSL) in lithium fluoride (LiF) substrates to demonstrate the potential for OSL to serve as a basis technology for next generation data storage systems.

42 ENGINEERING↗

DOE OSTI2024

Optically Stimulated Luminescence Data Storage (Abstract)

42 ENGINEERING↗

DOE OSTI2026

Air attenuation of high power XFEL beams

The Linac Coherent Light Source-II, a high-repetition-rate x-ray free electron laser, produces high average power as well as high peak power. Air is a key radiation safety element, helping to contain the FEL beams from reaching accessible areas. At high average power, air absorption can produce a high temperature and low-density channel along the x-ray beam path. In this case, the x-ray attenuation no longer follows the Beer-Lambert equation, e-μx . Air attenuation measurements were performed with x-rays focused into a gas cell at the LCLS Time-resolved AMO instrument. The air transmission was observed to significantly increase with x-ray power. Simulations were also performed, which include the thermal processes related to the high average power. In comparison to the measurements, the calculated air transmission is higher, confirming that the simulations are conservative and suitable for radiation safety analyses.

42 ENGINEERING↗

DOE OSTI2024

Machine learning based unfolding of x-ray spectra from filter stack spectrometer data

We demonstrate the application of neural networks to perform x-ray spectra unfolding from data collected by filter stack spectrometers. A filter stack spectrometer consists of a series of filter-detector pairs, where the detectors behind each filter measure the energy deposition through each layer as photo-stimulated luminescence (PSL). The network is trained on synthetic data, assuming x-rays of energies < 1 MeV and of two different distribution functions (Maxwellian and Gaussian) and the corresponding measured PSL values obtained from five different filter stack spectrometer designs. Predicted unfolds of single distributions are near identical reproductions of the ground truth spectra, with differences in the values lower than 20% at the higher energy end in some cases. The neural network has also demonstrated robustness to experimental measurement errors of < 5% and some capability of performing unfolds for linear combinations of the two distributions without previous training. The network can perform unfolds at rates > 1 Hz, ideal for application to some high-repetition-rate systems.

47 OTHER INSTRUMENTATION↗

DOE OSTI2022

Towards optimal gas cooling with minimal aero-optical distortion for a laser amplifier head

Next-generation lasers combining high-peak-power, ultrashort pulses with high repetition rates have the potential to efficiently deliver the high-average-power outputs required by many emerging technologies and areas of research. This work introduces a three-stage workflow consisting of low- and high-fidelity fluid simulations, in addition to aero-optical analyses. The final goal is to optimize gas cooling within a laser amplifier head while maintaining minimal aero-optical distortions. Low-fidelity RANS simulations are used to obtain mean flow solutions and transition locations. High-fidelity LES simulations, informed by their RANS counterparts, provide solutions containing density fluctuations, which are then passed on to the aero-optical analysis. The aero-optical analysis provides insight into the optical quality of the laser beam passing through the flow found in the LES results.

42 ENGINEERING↗

DOE OSTI2023

Optimal gas cooling with minimal aero-opticaldistortion for next generation high-average-power lasers (Progress report, Year 2)

Next-generation lasers that combine high-peak-power ultrashort pulses with high repetition rates have the potential to efficiently deliver the high-average-power outputs required for inertial fusion energy generation, laser-based particle acceleration, and to generate compact secondary x- and 𝛾-ray radiation sources, among others. The combination of long gain length with high surface-to-volume ratio to remove residual heat makes gas-cooled multi-slab amplifier heads an inherently aperture- and average power scalable technology that enables this new class of solid-state lasers, and their thermal management becomes the most pressing technical challenge. As the index-of refraction depends on the gas density, heat removal from the slab surfaces unavoidably entails scattering of propagated light from regions of high temperature fluctuations. The requirement to maximize convective heat extraction from the gain medium under the constraint of minimum optical aberration of the beam renders amplifier slab cooling a technological challenge at the intersection of aero-optics, fluid-mechanics and heat transfer. The goal of this research is to leverage computational fluid dynamics and aero optics simulations of different levels of fidelity to devise a numerical modeling and optimization framework for gas-cooled multi-slab amplifiers. The project will be conducted in close collaboration with the Advanced Photon Technologies Group at Lawrence Livermore National Laboratory, where a gas-cooled test stand for laser materials and thermal management structures will be developed and installed. The final goal of the collaborative effort is to manufacture and benchmark a physical prototype of an numerically optimized amplifier head design. Measurement data on solid-state and thermo-optical distortions will be used for the validation of the numerical models. The key technical challenge in this multi-objective design problem is that of balancing optimal heat removal with minimal optical distortion. To facilitate computationally efficient design optimization and, at the same time, deepen our basic understanding of the interaction of light with turbulence, a complementary study that combines high and low-fidelity flow simulations and aero-optical models is proposed. Along the lines of these two objectives and solution strategies, the project is organized into two thrusts.

42 ENGINEERING↗

DOE OSTI2025

Solving the Pulsed-Power Driven Inertial Fusion Energy Standoff Problem (Abbreviated Final Report)

The standoff problem in pulsed-power driven IFE (Inertial Fusion Energy) refers to the problem of electrically connecting a fusion target with the driver in a way that preserves the driver/target interface in the presence of a large fusion energy release (100’s of megajoules to 1000 megajoules). High yield fusion drivers for stockpile stewardship applications have similar concerns, but without the complication of the high repetition rate needed for energy production. All proposed IFE or high yield systems have the challenge of protecting the reactor vessel and driver from the energy release, but pulsed power drivers have the additional challenge of establishing an electrical connection in a way that does not create excessive debris or require costly/massive structures that must be expendable. Fortunately, there are conceptual solutions in the form of very low mass transmission lines, usually in the form of wires or foils, since very little mass is needed to overcome the magnetic forces driving the transmission lines apart or provide a low resistance pathway given the short pulse duration of the driver. Several important aspects of the standoff problem were analyzed in the course of this LDRD project. Conceptual means of introducing the low mass transmission lines into the reactor chamber were proposed, including analysis of methods to retain the power flow gap between the electrodes in the presence of the chamber environment. The energy losses due to ohmic dissipation and magnetic acceleration of the low mass transmission lines were evaluated for candidate driver pulses and different transmission line masses, and the fluence of x-ray and neutron energy on the persistent power flow structures that must survive the pulse of energy were evaluated. Finally, means of rapidly pumping down the chamber were explored as a way to return the system to low pressure following the multi-atmosphere post-pulse pressure rise. The overall conclusion from the analysis is that, while the reactor environment creates stressful conditions for a low mass transmission line standoff system, there are concepts expending 10 kg or less of electrode mass each pulse with the potential to mitigate the stresses and successfully drive fusion targets. Whether such a system could lead to a practical and economical fusion reactor would require extensive research and development beyond the scope of the feasibility study.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2023

Automated control and optimization of laser-driven ion acceleration

The interaction of relativistically intense lasers with opaque targets represents a highly non-linear, multi-dimensional parameter space. This limits the utility of sequential 1D scanning of experimental parameters for the optimization of secondary radiation, although to-date this has been the accepted methodology due to low data acquisition rates. High repetition-rate (HRR) lasers augmented by machine learning present a valuable opportunity for efficient source optimization. Here, an automated, HRR-compatible system produced high-fidelity parameter scans, revealing the influence of laser intensity on target pre-heating and proton generation. A closed-loop Bayesian optimization of maximum proton energy, through control of the laser wavefront and target position, produced proton beams with equivalent maximum energy to manually optimized laser pulses but using only 60% of the laser energy. This demonstration of automated optimization of laser-driven proton beams is a crucial step towards deeper physical insight and the construction of future radiation sources.

47 OTHER INSTRUMENTATION↗

DOE OSTI2022

FAST-GREENS: A High Efficiency Free Electron Laser Driven by Superconducting RF Accelerator

In this paper we’ll describe the FAST-GREENS experimental program where a 4 m-long strongly tapered helical undulator with a seeded prebuncher is used in the high gain TESSA regime to convert a significant fraction (up to 10 %) of energy from the 240 MeV electron beam from the FAST linac to coherent 515 nm radiation. We’ll also discuss the longer term plans for the setup where by embedding the undulator in an optical cavity matched with the high repetition rate from the superconducting accelerator (3,9 MHz), a very high average power laser source can be obtained. Eventually, the laser pulses can be redirected onto the relativistic electrons to generate by inverse compton scattering a very high flux of circularly polarized gamma rays for polarized positron production.

43 PARTICLE ACCELERATORS↗

DOE OSTI2021

Picosecond laser generated plasma as a source of singly charged ions for external injection into an EBIS

The focus of this paper is on practical aspects of ion generation by picosecond lasers as a source of low charge state ions for external injection of ions into an electron beam ion source (EBIS). For a ps-laser, compared to a ns-laser currently used at Relativistic Heavy Ion Collier Electron Beam Ion Source (RHIC EBIS), the influence of heat conductivity in the solid target is almost negligible, which results in a lower target consumption rate and less vacuum pressure rise. By using a laser with high repetition rate, it is possible to produce quasi continuous 1+ ion beams for periods of tens of milliseconds, making it possible to take advantage of the ability of the EBIS to accumulate ions in the “slow” injection capture mode. Producing such an ion pulse train is now feasible since ps-lasers with pulse energy up to 10 mJ and rep-rate up to 10 kHz have recently become commercially available. The advantages of this lower current accumulation scheme include: (1) easier beam transport due to lower space charge of lower beam currents required compared to the present single pulse fast injection scheme, (2) better EBIS pulse to pulse ion output stability since pulse to pulse ion variations of the laser source are averaged over a long train of laser pulses, and (3) the possible addition of an isotope separator in which rare beams could be produced and selected at run time from less expensive (unenriched) targets. We studied the properties of plasmas generated by a ps-laser with 1.27 mJ energy within an 8 ps pulse and a repetition rate up to 400 Hz at Argonne National Laboratory to investigate feasibility and specify parameters for a laser ion source for RHIC EBIS using a “slow” injection mode. Al, Ti, Cu, Nb, and Ta targets were tested with various target translation speeds. Here, we demonstrated that a both “slow” and “fast” injection modes are accessible with a single ion source geometry and single injection line, providing the most attractive option for an ion source for external injection into RHIC EBIS trap based on a ps-laser.

43 PARTICLE ACCELERATORS↗

DOE OSTI2025

Tailoring coherent beam combined laser pulse trains for high peak and average power applications

Laser systems based on coherent beam combination (CBC) that rely on tiled pupil architecture intrinsically carry digital capabilities independently applicable to all three essential characteristics of a laser pulse: amplitude, phase and polarization. Those capabilities allow the far-field energy distribution to be flexibly tailored in real time. Operation in the femtosecond regime at high repetition rates gives access to a wide range of applications requiring both high peak and average powers. We address the task of independent peak versus average power adjustment needed for applications seeking to decouple nonlinear phenomena associated with GW peak power from the thermal load inherent to kW average power operation. The technical solutions proposed are presented in the framework of the Ecole Polytechnique XCAN CBC laser platform (61 independent channels) with an emphasis on thermal management measures implemented to ensure its nominal operation.

47 OTHER INSTRUMENTATION↗