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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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NASA NTRS1994

Oxygen in the heliosphere

Oxygen within the heliosphere, whether neutral or ionized, comes from both the external source in the local interstellar medium (LISM) and internal sources. If transient cometary sources are neglected, Jupiter is the strongest of the internal sources by virtue of its corotation and charge exchange driven neutral wind. O(+) pickup ions are born where the penetrating neutrals lose an electron as a result of photoionization, charge exchange with solar wind protons, or solar wind electron impact ionization. The region of the heliosphere from which these pickup ions arise depends on the phase of the solar cycle as well as on the velocities of the neutrals. The present model of neutral O populations and their ionization suggests that Jovian pickup ions can dominate the inner heliospheric O(+) population if the LISM neutrals are strongly filtered at the heliopause, or are excluded by strong ionizing fluxes from the Sun. Other heliospheric species such as sulfur and nitrogen may have similar origins. These planetary sources need to be taken into account in the interpretation of interplanetary gas and ion composition observations.

Luhmann, J. G.↗
NASA NTRS1985

In-situ detection of micron-sized dust particles in near-Earth space

In situ detectors for micron sized dust particles based on the measurement of impact ionization have been flown on several space missions (Pioneer 8/9, HEOS-2 and Helios 1/2). Previous measurements of small dust particles in near-Earth space are reviewed. An instrument is proposed for the measurement of micron sized meteoroids and space debris such as solid rocket exhaust particles from on board an Earth orbiting satellite. The instrument will measure the mass, speed, flight direction and electrical charge of individually impacting debris and meteoritic particles. It is a multicoincidence detector of 1000 sq cm sensitive area and measures particle masses in the range from 10 to the -14th power g to 10 to the -8th power g at an impact speed of 10 km/s. The instrument is lightweight (5 kg), consumes little power (4 watts), and requires a data sampling rate of about 100 bits per second.

Gruen, E.↗
NASA NTRS1978

Balloon-borne photoionization mass spectrometer for measurement of stratospheric gases

A balloon-borne photoionization mass spectrometer used to measure stratospheric trace gases is described. Ions are created with photons from high-intensity krypton discharge lamps and a quadrupole mass analyzer is employed for ion identification. Differential pumping is achieved with liquid helium cryopumping. To insure measurement of unperturbed stratospheric air, the entire system is contained in a sealed gondola and the atmospheric sample is taken some distance away during descent. The photoionization technique allows the detection of a low ionization potential constituent, such as nitric oxide, at less than a part in one billion in the presence of the major atmospheric gases and their isotopes. Operation of the mass spectrometer system was demonstrated during a daytime flight from Palestine, Texas on 26 April 1977. The sensitivity achieved and the unique selectivity afforded by this technique offer a capability for trace constituent measurement not possible with the more conventional electron impact ionization approach.

Aikin, A. C.↗
NASA NTRS2003

Dissociative Ionization of Aromatic and Heterocyclic Molecules

Space radiation poses a major health hazard to humans in space flight. The high-energy charged particles in space radiation ranging from protons to high atomic number, high-energy (HZE) particles, and the secondary species they produce, attack DNA, cells, and tissues. Of the potential hazards, long-term health effects such as carcinogenesis are likely linked to the DNA lesions caused by secondary electrons in the 1 - 30 eV range. Dissociative ionization (DI) is one of the electron collision processes that can damage the DNA, either directly by causing a DNA lesion, or indirectly by producing radicals and cations that attack the DNA. To understand this process, we have developed a theoretical model for DI. Our model makes use of the fact that electron motion is much faster than nuclear motion and assumes DI proceeds through a two-step process. The first step is electron-impact ionization resulting in a particular state of the molecular ion in the geometry of the neutral molecule. In the second step the ion undergoes unimolecular dissociation. Thus the DI cross section sigma(sup DI)(sub a) for channel a is given by sigma(sup DI)(sub a) = sigma(sup I)(sub a) P(sub D) with sigma(sup I)(sub a) the ionization cross section of channel a and P(sub D) the dissociation probability. This model has been applied to study the DI of H2O, NH3, and CH4, with results in good agreement with experiment. The ionization cross section sigma(sup I)(sub a) was calculated using the improved binary encounter-dipole model and the unimolecular dissociation probability P(sub D) obtained by following the minimum energy path determined by the gradients and Hessians of the electronic energy with respect to the nuclear coordinates of the ion. This model is used to study the DI from the low-lying channels of benzene and pyridine to understand the different product formation in aromatic and heterocyclic molecules. DI study of the DNA base thymine is underway. Solvent effects will also be discussed.

Huo, Winifred M.↗
NASA NTRS1990

Direct simulation Monte Carlo with ionization and radiation

Improvements in the modeling of radiation in low density shock waves with Direct Simulation Monte Carlo (DSMC) are the subject of this study. The physical processes which determine the amount of radiation in a shock wave were investigated and the way in which they were modeled with DSMC was evaluated. Three physical processes were identified for which an improvement in the modeling technique could result in improved radiation predictions. New physical modeling schemes are introduced in this report for the three processes. First a method for determining the electric field and its effect on the flow is introduced. Second, a two step reaction process for electron impact ionization reactions is evaluated. Finally, a new scheme to determine the relaxation collision numbers for excitation of electronic states is proposed. Each new scheme attempts to move the DSMC method toward more accurate physics or more reliance on experimental data. The new schemes are all compared to the current modeling techniques and the differences in the results are evaluated. In all cases the results agree with the available data as well as, or better than the results from earlier schemes.

Carlson, Ann B.↗
NASA NTRS1990

An assessment of the conditions for critical velocity ionization at the weakly magnetized planets

It has been proposed that critical velocity ionization (CVI) may occur in the magnetosheaths of weakly magnetized planets where the solar wind flows through the planets' upper atmospheres. One can examine this possibility for Venus and Mars by using magnetosheath flow and exosphere models to determine whether the criteria for CVI are met. These criteria include Brenning's empirical condition on the cross-field flow velocity (it must not exceed the local magnetosonic velocity) and the 'Townsend condition' requiring that the integrated probability of impact ionization by a hot electron be greater than 1 along a streamline past the planet. Application of the Spreiter-Stahara gas dynamic flow model and the Nagy and coworkers' models for the exospheres lead to the conclusion that the conditions can be met in a limited region near Venus. However, evidence for CVI has not been identified in in-situ data. Since key details of the planet-solar wind interaction can be explained in terms of photoionization alone, other signatures of the process must be sought in the observations if the presence of CVI is to be positively inferred.

Luhmann, J. G.↗
NASA NTRS1975

Shock tube study of ionization rates of NaCl-contaminated argon

Electron density, electron temperature, and concentration of excited sodium atoms are measured in the weakly ionized regime behind a shock wave in impure argon in a shock tube using microwave techniques and spectrally resolved radiometry. Evidence is presented to show that an apparent increase in the rate of ionization is due to electron detachment of negative chlorine ions produced from sodium chloride vapor contained as an impurity. To be consistent with this chemical model, rate coefficients are found in the temperature range between 5500 and 8600 K for the dissociation of NaCl into an ion pair, dissociation of NaCl into a neutral pair, and electron detachment of a negative chlorine ion. Electron temperature is lower than heavy-particle temperature by roughly 1000 K. The electron-argon impact-ionization rate coefficient is a weak function of electron temperature in contradiction to expectation.

Schneider, K.-P.↗
NASA NTRS2006

Collisional Ionization Equilibrium for Optically Thin Plasmas

Reliably interpreting spectra from electron-ionized cosmic plasmas requires accurate ionization balance calculations for the plasma in question. However, much of the atomic data needed for these calculations have not been generated using modern theoretical methods and their reliability are often highly suspect. We have utilized state-of-the-art calculations of dielectronic recombination (DR) rate coefficients for the hydrogenic through Na-like ions of all elements from He to Zn. We have also utilized state-of-the-art radiative recombination (RR) rate coefficient calculations for the bare through Na-like ions of all elements from H to Zn. Using our data and the recommended electron impact ionization data of Mazzotta et al. (1998), we have calculated improved collisional ionization equilibrium calculations. We compare our calculated fractional ionic abundances using these data with those presented by Mazzotta et al. (1998) for all elements from H to Ni, and with the fractional abundances derived from the modern DR and RR calculations of Gu (2003a,b, 2004) for Mg, Si, S, Ar, Ca, Fe, and Ni.

Bryans, P.↗
NASA NTRS1994

First measurement of helium on Mars: Implications for the problem of radiogenic gases on the terrestrial planets

The 108 photons of the Martian He 584 A airglow detected by the Extreme Ultraviolet Explorer satellite during a two-day exposure (22-23 Jan. 1993) correspond to the effective disk average intensity of 43 (+/-) 10 Rayleigh. Radiative transfer calculations, using a model atmosphere appropriate to the conditions of the observation and having an exospheric temperature of 210 (+/-) 20 K, result in an He mixing ratio of 1.1 (+/-) 0.4 ppm in the lower atmosphere. Nonthermal escape of helium is due to the following: electron impact ionization and pickup of He(+) by the solar wind; collisions with hot oxygen atoms; and charge exchange with molecular species with corresponding column loss rates of 1.4 x 10(exp 5), 3 x 10(exp 4), and 7 x 10(exp 3) cm(exp -2)s(exp -1), respectively. The lifetime of helium on Mars is 5 x 10(exp 4) yr. The He outgassing rate, coupled with the Ar-40 atmospheric abundance and with the K:U:Th ratio measured in the surface rocks, is used as input to a simple two-reservoir degassing model which presumes the loss of all argon accumulated in the atmosphere during the first Byr by large-scale impacts. The model results in total planet mass ratios of 10(exp -5) g/g for K, 2.3 x 10(exp -9) g/g for U, 8.5 x 10(exp -9) g/g for Th, 4 x 10(exp -10) g/g for He, and 1.5 x 10(exp -9) g/g for Ar-40. The predicted radiogenic heat flux is 2 erg cm(exp -2)s(exp -1). Similar modeling for Venus results in total plant mass ratios of 4.7 x 10(exp -5) g/g for K, 6.7 x 10(exp -9) g/g for U, 2.2 x 10(exp -8) g/g for Th, 1.3 x 10(exp -9) for He, 6.7 x 10(exp -9) g/g for Ar-40, and a radiogenic heat flux of 15 erg cm(exp -2)s(exp -1). The implications of these results are discussed. The modeling shows that the radioactive elements were not distributed uniformly in the protoplanetary nebula, and their relative abundances differ very much in the terrestrial planets.

Bowyer, S.↗
NASA NTRS1994

First measurement of helium on Mars: Implications for the problem of radiogenic gases on the terrestrial planets

108 +/- 11 photons of the martian He 584-A airglow detected by the Extreme Ultraviolet Explorer (EUVE) satellite during a 2-day exposure (January 22-23, 1993) correspond to the effective disk average intensity of 43 +/- 10 Rayleigh (Ra). Radiative transfer calculations, using a model atmosphere appropriate to the conditions of the observation and having an exospheric temperature of 210 +/- 20 K, result in a He mixing ratio of 1.1 +/- 0.4 ppm in the lower atmosphere. Nonthermal escape of helium is due to electron impact ionization and pickup of He(+) by the solar wind, to collisions with hot oxygen atoms, and to charge exchange with molecular species with corresponding column loss rates of 1.4 x 10(exp 5), 3 x 10(exp 4), and 7 x 10(exp 3)/sq cm/s, respectively. The lifetime of helium on Mars is 5 x 10(exp 4) years. the He outgassing rate, coupled with the Ar-40 atmospheric abundance and with the K:U:Th ratio measured in the surface rocks, is used as input to a single two-reservoir degassing model which is applied to Mars and then to Venus. A similar model with known abundances if K, U, and Th is applied to Earth. The models for Earth and Mars presume loss of all argon accumulated in the atmospheres during the first billion years by large-scale meteorite and planetesimal impacts. The models show that the degassing coefficients for all three planets may be approximated by function delta = delta(sub 0) x (t(sub 0)/t)(exp 1/2) with delta(sub 0) = 0.1, 0.04, and 0.0125 Byr for Earth, Venus, and Mars, respectively. After a R(exp 2) correction this means that outgassing processes on Venus and Mars are weaker than on Earth by factors of 3 and 30, respectively. Mass ratios of U and Th are almost the same for all three planets, while potassiumis depleted by a factor of 2 in Venus and Mars. Mass ratio of helium and argon are close to 5 x 10(exp -9) and 2 x 10(exp -8) g/g in the interiors of all three planets. The implications of these results are discussed.

Krasnopolsky, V. A.↗
NASA NTRS1972

Investigation of high speed phenomena

Experimental research is reported for laboratory simulation of meteors and meteoroid impacts on solid surfaces. Two types of mass measurements are discussed: impact ionization risetime effect, and luminous efficiency measurements.

Becker, D. G.↗
NASA NTRS1974

Physics of sub-micron cosmic dust particles

Laboratory tests with simulated micrometeoroids to measure the heat transfer coefficient are discussed. Equations for ablation path length for electrically accelerated micrometeoroids entering a gas target are developed which yield guidelines for the laboratory measurement of the heat transfer coefficient. Test results are presented for lanthanum hexaboride (LaB sub 6) microparticles in air, argon, and oxygen targets. The tests indicate the heat transfer coefficient has a value of approximately 0.9 at 30 km/sec, and that it increases to approximately unity at 50 km/sec and above. Test results extend to over 100 km/sec. Results are also given for two types of small particle detectors. A solid state capacitor type detector was tested from 0.61 km/sec to 50 km/sec. An impact ionization type detector was tested from 1.0 to 150 km/sec using LaB sub 6 microparticles.

Roy, N. L.↗
NASA NTRS1976

Io's atmosphere and ionosphere - New limits on surface pressure from plasma models

The paper studies charge particle impact as a mechanism for the production of Io's ionosphere. Pioneer 10 thermal plasma measurements and magnetospheric plasma models which explain the observed spatial distribution of neutral hydrogen and sodium atoms in the vicinity of Jupiter's satellite Io imply electron fluxes of about 10 to the 10th/sq cm/s. The fluxes and the temperature (about 100 eV) of this plasma suggest that electron impact ionization is the dominant process in forming the ionosphere of Io. It is found that the surface number density of the neutral species required to match the observed electron density profiles is about 10 to the 9th/cu cm or less. This value is two orders of magnitude lower than previous estimates.

Johnson, T. V.↗
NASA NTRS1977

Some optical and kinetic properties of the nearby interstellar gas

A model for resonant scattering of sunlight by the nearby interstellar gas is developed which takes into account the modification of a Maxwell-Boltzmann velocity distribution by a central force. While the formalism applies to both hydrogen and helium, the latter is emphasized. Theoretical line profiles and integrated emission rates for helium are compared with those of approximate models and with existing observations. As a result of this analysis, an upward revision of the bulk flow velocity of interstellar helium relative to the solar system, previously deduced from He 584-A observations, is required. Velocities of 15-20 km/s, temperatures of the order of 5000-10,000 K, and densities of the order of 0.008-0.02 per cu cm are sufficient to explain the (helium) observations. However, higher-precision measurements are required in order to place more stringent limits on the gas parameters. Calculations of the flux of interstellar helium atoms impinging on earth's upper atmosphere show that the resulting impact ionization is small compared with terrestrial processes.

Meier, R. R.↗
NASA NTRS1977

Periodic variations in Io's sodium and potassium clouds

Spectra of Io's sodium cloud taken 7.5 to 45 sec north and south of Io at a variety of magnetic latitudes of Io obtained during 17 nights of the 1975 apparition of Jupiter confirm the weakening of the cloud in the neighborhood of Jupiter's magnetic equator. The time scale for these changes is 1.5 hours or less. For impact ionization to cause these changes, a minimum flux of 100 billion/sq cm/sec 15 eV electrons or 40 billion/sq cm/sec 8 keV protons is required. Sodium velocities near 10 km/sec are required to explain the replenishment of ionized regions of the cloud. We also obtained spectra of Io's potassium cloud on eight nights during the 1975 apparition. This cloud appears to behave like the sodium cloud as Io's magnetic latitude varies. The potassium, however, may become much weaker as Io passes through the magnetic equator. The brightest intensity measured for the 7665 A resonance line was about 1 kR at a point 7.5 sec east of Io.

Trafton, L.↗
NASA NTRS1978

Europa - Ultraviolet emissions and the possibility of atomic oxygen and hydrogen clouds

Emission signals from Europa with wavelength below 800 A were detected by the Pioneer 10 ultraviolet photometer. In the present paper, improved procedures for data reduction are used to determine the spatial region as well as the intensity of the suggested emission sources. The observations indicate a cloud with a radius of about 1.5 Jupiter radii and an apparent brightness of approximately 10 rayleighs for a wavelength of 500 A. It is argued that neutral oxygen atoms, along with neutral hydrogen, are produced through dissociation of water ice on the surface of Europa by particle impact. Electron impact ionization excitation of oxygen atoms in the resulting cloud then gives rise to the observed emission. The present source brightness and cloud radius results are used to estimate an oxygen column density of the order of 10 trillion per sq cm, while the density of atomic hydrogen is at most 100 billion per sq cm and 1 trillion per sq cm for molecular hydrogen.

Wu, F.-M.↗
NASA NTRS1978

Mass spectrometry

A review of mass spectrometry in organic chemistry is given, dealing with advances in instrumentation and computer techniques, selected topics in gas-phase ion chemistry, and applications in such fields as biomedicine, natural-product studies, and environmental pollution analysis. Innovative techniques and instrumentation are discussed, along with chromatographic-mass spectrometric on-line computer techniques, mass spectral interpretation and management techniques, and such topics in gas-phase ion chemistry as electron-impact ionization and decomposition, photoionization, field ionization and desorption, high-pressure mass spectrometry, ion cyclotron resonance, and isomerization reactions of organic ions. Applications of mass spectrometry are examined with respect to bio-oligomers and their constituents, biomedically important substances, microbiology, environmental organic analysis, and organic geochemistry.

Burlingame, A. L.↗