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DOE OSTI2023

Constraining the Equation of State of Dense Neutron-rich Matter (Final Report)

Using a new Time Projection Chamber (TPC), called the SpiRIT (SAMURAI pion Reconstruction Ion Tracker) constructed and funded by DOE office of science (award # DE-SC0004835), we performed two experiments with the SAMURAI spectrometer at RIKEN, Japan to study the equation of state of neutron rich matter. As a result of the project, the SpiRIT collaboration, an international collaboration consisting of groups from US, Japan, Korea, Poland, China and Germany, has been formed to pursue the science opportunities provided by the SpiRIT TPC. After the experiments, we developed the software to analyze the SpiRIT experiments and extract constraints of symmetry energy at supra-saturation densities. As a result 270 TB of data have been obtained. Over 10 technical papers on the TPC and 4 science papers on the nuclear equation of state have been published. A total of six (2 US, 1 Japanese and 1 Korean) PhD students have graduated based on their research on the EOS research using the SpiRIT data. In addition, the data also stimulated theorists on transport models to form the “Transport Model Evaluation Project” collaboration to improve the transport model to compare calculations with the data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2023

Constraining the Equation of State of Dense Neutron-rich Matter (Final Technical Report)

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2025

Precision Measurement of the Neutron Magnetic Form Factor via the Ratio Method at Jefferson Lab Hall A

Protons and neutrons, collectively known as nucleons, are composed of quarks and gluons. The Sachs electromagnetic form factors encode information about the spatial distributions of charge and magnetization in the nucleon, particularly at low momentum transfer. In particular, the neutron magnetic form factor (GMn) provides crucial information about the distribution of magnetization inside the neutron and helps constrain theoretical models of nucleon structure. Quasi-elastic electron scattering from deuterium was measured up to Q^2=13.5 GeV^2 using the Super BigBite Spectrometer in Hall A at Jefferson Lab. In this work, the neutron magnetic form factor GMn was extracted at Q^2 = 3.0 GeV^2 and Q^2=4.5 GeV^2 using the Ratio Method. These results represent a subset of the full dataset collected in this experiment, which extended to significantly higher Q^2. The extracted GMn values agree with the existing global fit within approximately two standard deviations at Q^2=3.0 and show excellent agreement at Q^2=4.5. The measurements achieved systematic uncertainties of about 2% and statistical uncertainties below 0.5%, among the most precise determinations of GMn at these kinematics. These results demonstrate the robustness of the experimental technique and provide an important validation point for future extractions at higher Q^2, where data remain scarce. In addition, the GRINCH heavy gas Cherenkov detector—a key component of the experimental apparatus—was commissioned and achieved an electron detection efficiency of approximately 97%, supporting reliable particle identification. Together, the analysis presented here advances both our understanding of nucleon structure and the validation of the experimental methods and instrumentation used to access it.

Satnik, Maria [College of William and Mary, Willia↗

DOE OSTI2023

Advancements of the nSpec system

For this study, a new characterization of the detector response for the EJ301 liquid scintillator based nSpec system has been conducted at the Los Alamos Neutron Science Center. The new characterization was accomplished in two orders of magnitude less time and with better statistics than the previous characterization. The new and old characterization methods were compared by conducting both types of characterization on two detectors (one EJ301 and one EJ301D). The two methods show consistent results and compare well to results previously published in the literature; however, the results from the characterization of the original nSpec detector show discrepancies that have been identified as being caused by oxygen being absorbed into the detector due to a leak. The new characterized detector response shows improved spectrum unfolding performance than the previous characterization. The cross talk of the detector system was also characterized as a function of incident neutron energy and found to have a negligible impact on spectrum unfolding results. Alternative materials (EJ301D and stilbene) were also characterized in a first step towards an upgraded system. The different materials show little difference in unfolding performance, but the comparison is ongoing. A SiPM based stilbene detector was used to evaluate the use of SiPMs in a future system upgrade. The SiPM provides adequate performance, but the custom SiPM readout results in a much longer pulse width than PMT based systems. The measured light output of the SiPM based stilbene compares well with the results in literature. Future work will look at additional materials (deuterated stilbene and organic glass) and optimizing the SiPM readout to decrease the pulse width.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2023

Quantification of the light output anistropy in deuterated stilbene

Deuterated stilbene is an organic scintillator that is a desirable material for fast neutron spectroscopy using spectrum unfolding techniques without requiring time-of-flight information. Due to the crystal structure of the material, some anisotropy of the light output exists, which is dependent on the direction of heavy charged particle recoil relative to the crystal structure. The anisotropy of trans-stilbene (hereafter referred to as stilbene) has been well characterized in previous work, but for deuterated stilbene, the anisotropy has only been partially characterized along the a and b crystal axes, while the artificial c' axis, which shows the largest anisotropy in stilbene, has not been characterized until this publication. Here, in this work, two deuterated stilbene crystals were characterized with neutron energies up to 35 MeV at the Los Alamos Neutron Science Center. For one of the crystals, the response is characterized along the a, b, and c' axes. This characterization shows a distinct anisotropy along the axes in deuterated stilbene, which is very similar to that found in regular stilbene, such that the a axis is the brightest, while the b' and c' axes are approximately 3% and 20%–35% lower relative to the a axis.

36 MATERIALS SCIENCE↗

DOE OSTI2026

Identifying neutron sources using recoil and time-of-flight spectroscopy

Identification of neutron sources is central to nuclear physics and its applications, from planetary science to nuclear security, yet direct source discrimination from measured neutron spectra remains fundamentally elusive. Here, we introduce a Bayesian protocol that directly infers source ensembles from measured neutron spectra by combining full-spectrum template matching with probabilistic evidence evaluation. Applying this protocol to recoil and time-of-flight spectroscopy, we recover single- and two-source configurations with strong statistical significance (beyond 4⁢𝜎) at event counts as low as ∼10 3 . These results demonstrate that neutron spectral signatures can be leveraged for robust source identification, opening a new observational window for both fundamental research and operationally driven applications.

neutron physics↗

DOE OSTI2020

β Decay of 61 V and its Role in Cooling Accreted Neutron Star Crusts

The interpretation of observations of cooling neutron star crusts in quasipersistent x-ray transients is affected by predictions of the strength of neutrino cooling via crust Urca processes. The strength of crust Urca neutrino cooling depends sensitively on the electron-capture and β -decay ground-state-to-ground-state transition strengths of neutron-rich rare isotopes. Nuclei with a mass number of A = 61 are predicted to be among the most abundant in accreted crusts, and the last remaining experimentally undetermined ground-state-to-ground-state transition strength was the β decay of 61 V. This Letter reports the first experimental determination of this transition strength, a ground-state branching of $8.1^{+4.0}_{- 3.1}%$, corresponding to a log ft value of $5.5^{+0.2}_{-0.2}$. This result was achieved through the measurement of the β -delayed γ rays using the total absorption spectrometer SuN and the measurement of the β -delayed neutron branch using the neutron long counter system NERO at the National Superconducting Cyclotron Laboratory at Michigan State University. This method helps to mitigate the impact of the pandemonium effect in extremely neutron-rich nuclei on experimental results. The result implies that A = 61 nuclei do not provide the strongest cooling in accreted neutron star crusts as expected by some predictions, but that their cooling is still larger compared to most other mass numbers. Finally, only nuclei with mass numbers 31, 33, and 55 are predicted to be cooling more strongly. However, the theoretical predictions for the transition strengths of these nuclei are not consistently accurate enough to draw conclusions on crust cooling. With the experimental approach developed in this work, all relevant transitions are within reach to be studied in the future.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2023

J/ψ Near-Threshold Photoproduction off the Proton and Neutron with CLAS12

In recent years, J/? photoproduction in the near-threshold region has seen a renewed theoretical interest due to the wealth of information it has to offer. Near-threshold J/? photopro-duction proceeds through the exchange of gluons in the t-channel and is expected to provide unique insight about the nucleon gluonic gravitational form factors (GFFs). Previous studies at the Thomas Jefferson National Accelerator Facility (JLab) in Virginia, USA, have already measured the total and differential cross section of J/? near-threshold photoproduction on the free proton. This thesis presents the first measurements of J/? near-threshold photoproduction on the bound proton and bound neutron in a deuteron target. The CEBAF Large Acceptance Spectrometer at 12 GeV (CLAS12) based at JLab?s Hall B uses a 11 GeV electron beam impinging on a fixed liquid deuteron target. J/? is then produced via the exchange of a quasi-real photon and decays to a lepton pair which is detected along-side the recoil nucleon by CLAS12. Analysis procedures and in particular machine learning based techniques were developed in order to correctly identify final state particles and select J/? photoproduction events. The total and differential cross section of J/? near-threshold photoproduction on the bound proton and bound neutron were then measured from the detected J/? photoproduction events. The measurements of the cross sections on the bound proton and bound neutron agree well within their statistical uncertainty. This is consistent with the assumed two-gluon exchange production mechanism which is isospin invariant. Overall a first measurement of the J/? near-threshold photoproduction cross sections on the bound proton and bound neutron was achieved. A better understanding of the mechanical properties of the nucleon, such as pressure and mass distributions, can be obtained by relating J/? production to the nucleon GFFs. This opens the way for exciting new insights into the internal structure of the nucleon, and in particular of the nucleon?s gluonic content. An upcoming overhaul of the CLAS12 reconstruction will increase the reconstruction efficiency and the statis- tical precision of the preliminary measurements described in this thesis, with an expected gain in statistics of at least 50%. Future upgrades at JLab will allow to test some of the theoretical assumptions made in relating J/? near-threshold photoproduction to the nucleon GFFs

Tyson, Richard↗

DOE OSTI2025

Measurement of the Neutron Electromagnetic Form Factors at High Momentum Transfer Using a Polarized 3He Target at Jefferson Lab

Ever since the composite structure of nucleons was uncovered, many experiments have been commissioned with the purpose of extracting parameters that shape our understanding of this structure. Form factors are powerful tools that rest at the forefront of the nucleon structure study. In the non-relativistic limit, they describe the magnetic and charge distributions inside the nucleon. The GEn-II experiment, which ran in Hall A of Jefferson Lab as a part of the SuperBigbite Spectrometer (SBS) program, aimed to extract the ratio of the neutron’s electric to magnetic Sachs form factors (GnE/GnM. This was accomplished using the double polarization technique: scattering polarized electrons with initial energies up to 8.45 GeV off high-density polarized 3He targets. The experiment was a coincidence measurement, with the scattered electrons detected in the BigBite Spectrometer and the recoil nucleons in a hadron calorimeter, a part of the SuperBigbite Spectrometer. The convection-style target cells used in this experiment have a 60cm long target chamber, an increase from the 40 cm cell used in the most recent polarized 3He target experiment. In addition, the cells were optically pumped from two sides of the pumping chamber. These improvements in design and functionality introduced world-record-breaking luminosity. This thesis presents preliminary results of the GEn-II experiment for the following 4-momentum transfer (Q2) values: 2.93, 6.76, and 9.78 GeV2, in addition to target performance and preliminary polarimetry results.

Presley, Hunter [Univ. of Virginia, Charlottesvill↗

DOE OSTI2025

ARCS White Beam Vanadium Normalization Data for SNS Cycle 2022B

Neutron scattering Data from a Vanadium cylinder. Acquired on the ARCS spectrometer in white beam mode to normalize the detector efficiencies. During Cycle 2022B

MATERIALS SCIENCE↗

DOE OSTI2025

Phase-Imaging Ion-Cyclotron-Resonance mass spectrometry with the Canadian Penning Trap at CARIBU

The Canadian Penning Trap mass spectrometer (CPT) has conducted precision mass measurements of neutron-rich nuclides from the CAlifornium Rare Isotope Breeder Upgrade (CARIBU) of the Argonne Tandem Linac Accelerator System (ATLAS) facility at Argonne National Laboratory using the Phase-Imaging Ion-Cyclotron-Resonance (PI-ICR) technique for over half a decade. Here, in this study, we discuss the CPT system, and methods to improve accuracy and precision in mass measurement using PI-ICR including some optimization techniques and recently studied systematic effects.

Penning trap mass spectrometry↗

DOE OSTI2020

Cross section measurements of deuteron electro-disintegration at very high recoil momenta and large 4-momentum transfers (Q^2)

The 2H(e,e'p)n cross sections have been measured at negative 4-momentum transfers of Q^2 = 4.5 +/- 0.5 (GeV/c)^2 and Q^2 = 3.5 +/- 0.5 (GeV/c)^2 reaching neutron recoil (missing) momenta up to p_r ?1.0 GeV/c. The data have been obtained at fixed neutron recoil angles 5 <= theta_nq <= 95 degrees with respect to the 3-momentum transfer q. The new data agree well with the previous data which reached p_r ?550 MeV/c. At theta_nq = 35 and 45 degrees, final state interactions (FSI), meson exchange currents (MEC) and isobar configurations (IC) are suppressed and the plane wave impulse approximation (PWIA) provides the dominant cross section contribution. The new data are compared to recent theoretical calculations, and a significant disagreement for recoil momenta p_r > 700 MeV/c is observed. The experiment was carried out in experimental Hall C at the Thomas Jefferson National Accelerator Facility (TJNAF) and formed part of a group of four experiments that were used to commission the new Super High Momentum Spectrometer (SHMS). The experiment consisted of a 10.6 GeV electron beam incident on a liquid deuterium target which resulted in the break-up of the deuteron into a proton and neutron. The scattered electrons were detected by the SHMS in coincidence with the knocked-out protons detected in the previously existing High Momentum Spectrometer (HMS) and the recoiling neutrons were reconstructed from energy-momentum conservation laws. To ensure that the 2H(e,e'p)n reaction channel was selected, we required the missing energy of the system to be the binding energy of the deuteron (?2.22 MeV). The spectrometers? central angles and momenta were set to measure three central missing momentum settings of the neutron corresponding to p_r = 80, 580 and 750 MeV/c, which required the SHMS central angle and momentum to be fixed and the HMS to be rotated from smaller to larger angles corresponding to the lower and higher missing momentum settings, respectively. The experiment was carried out in a time period of six days with typical electron beam currents of 45-60 uA at about 50% beam efficiency.

Yero, Carlos↗

DOE OSTI2021

Reconstructing 3D asymmetries in laser-direct-drive implosions on OMEGA

Three-dimensional reconstruction algorithms have been developed which determine the hot-spot velocity, hot-spot apparent ion temperature distribution, and fuel areal density distribution present in laser-direct-drive inertial con finement fusion implosions on the OMEGA laser. These reconstructions rely on multiple independent measurements of the neutron energy spectrum emitted from the fusing plasma. Measurements of the neutron energy spectrum on OMEGA are made using a suite of quasi-orthogonal neutron time-of-flight detectors and a magnetic recoil spectrometer. These spectrometers are positioned strategically around the OMEGA target chamber to provide unique 3-D measurements of the conditions of the fusing hot spot and compressed fuel near peak compression. Here, the uncertainties involved in these 3-D reconstructions are discussed and are used to identify a new nTOF diagnostic line of sight which when built will reduce the uncertainty in the hot-spot apparent ion temperature distribution from 0.7 to < 0.4 keV.

47 OTHER INSTRUMENTATION↗

DOE OSTI2020

Effect of an electric field on liquid helium scintillation produced by fast electrons

The dependence on applied electric field (0–40 kV/cm) of the scintillation light produced by fast electrons and α particles stopped in liquid helium in the temperature range of 0.44 K to 3.12 K is reported. For both types of particles, the reduction in the intensity of the scintillation signal due to the applied field exhibits an apparent temperature dependence. Using an approximate solution of the Debye-Smoluchowski equation, we show that the apparent temperature dependence for electrons can be explained by the time required for geminate pairs to recombine relative to the detector signal integration time. This finding indicates that the spatial distribution of secondary electrons with respect to their geminate partners possesses a heavy, non-Gaussian tail at larger separations and has a dependence on the energy of the primary ionization electron. Here, we discuss the potential application of this result to pulse shape analysis for particle detection and discrimination.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2021

Reconstructing 3-D Asymmetries in Laser-Direct-Drive Implosions on OMEGA

Three-dimensional reconstruction algorithms have been developed which determine the hot-spot velocity, hot-spot apparent ion temperature distribution, and fuel areal-density distribution present in laser-direct- drive inertial confinement fusion implosions on the OMEGA laser. These reconstructions rely on multiple independent measurements of the neutron energy spectrum emitted from the fusing plasma. Measurements of the neutron energy spectrum on OMEGA are made using a suite of quasi-orthogonal neutron time-of-flight detectors and a magnetic recoil spectrometer. These spectrometers are positioned strategically around the OMEGA target chamber to provide unique 3-D measurements of the conditions of the fusing hot spot and compressed fuel near peak compression. The uncertainties involved in these 3-D reconstructions are discussed and are used to identify a new nTOF diagnostic line of sight which when built will reduce the uncertainty in the hot-spot apparent ion temperature distribution from 700 to <400 eV.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2024

Quest for Cooper Pair Transfer in Heavy-Ion Reactions: The 206 Pb + 118 Sn Case

In this Letter we report on effects of nucleon-nucleon correlations probed in nucleon transfer reactions with heavy ions. We measured with high efficiency and resolution a complete set of observables for neutron transfer channels in the ²⁰⁶Pb + ¹¹⁸Sn system employing a large solid angle magnetic spectrometer, which allowed us to study a wide range of internuclear distances via a detailed excitation function. The coupled channel theory, based on an independent particle transfer mechanism, follows the experimental transfer probabilities for one- and two-neutron pick-up and stripping channels. The experimental two-neutron transfer cross sections indicate that in reactions between pair-vibrational (closed shell) and pair-rotational (open shell) nuclei, correlations manifest via pair-addition and pair-removal modes, which constitute one of the elementary modes of excitations in nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2022

Discrimination of phosgene from cyanogen chloride in recovered chemical munitions using tagged neutron interrogation with high-resolution gamma-ray spectroscopy

The Associated Particle technique has recently been utilized with a germanium-based high-resolution $\gamma$-ray spectrometer and assessed for its capability to improve field identification of recovered chemical warfare (CW) materiel through prompt gamma-ray neutron activation analysis (PGNAA) measurements. An accurate chemical identification is necessary for the safe handling, destruction, and disposal of such hazardous items. A particularly challenging pair of CW agents commonly found in recovered munitions are phosgene (CG) and cyanogen chloride (CK), which have two of three elements in common, i.e. chlorine and carbon, but differ in the third being either oxygen or nitrogen. The detection of both latter elements is complicated by high oxygen concentration in the field environment which interferes with the small signal produced from the chemical agents. The matter is further complicated by the precautionary field practice of overpacking recovered munitions with vermiculite in larger steel multiple round containers (MRCs), which places additional oxygen-rich material around the munition while further attenuating an already weak signal emitted from the munition center. Here, this work reports quantitative results from realistic field measurements of CG and CK simulants in mock 4.2-inch mortar rounds overpacked with vermiculite in a large MRC. Results obtained with the AP technique are compared to those obtained with the traditional PGNAA approach for both overpacked- and bare-munition measurements. The AP technique is shown to provide a much more confident discrimination between the two chemicals, particularly for the more challenging field-relevant overpacked measurements, where a significant gain in sensitivity to all the key elements chlorine, carbon, nitrogen and oxygen is achieved.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2020

A Replacement Cold Neutron Guide System for HFIR (Conceptual Design Report)

The design of a replacement cold neutron guide system for the High Flux Isotope Reactor (HFIR) is presented. The proposed six-channel design uses the latest technologies and is optimally designed to account for operational and site constraints. These include the design of the cold source and the beam tube, the size and shape of the penetrations in the reactor confinement boundary, and the shape and orientation of the guide hall. The existing user instruments are a macromolecular diffractometer (IMAGINE), an IMAGING station, two small-angle neutron scattering (SANS) instruments (Bio-SANS and GP-SANS), and a cold triple-axis spectrometer (C-TAX). These instruments will all be reinstalled at end-of-guide positions with improved performance, and a position for a new high-performance neutron spin echo instrument will be created. The proposed guide design requires an extension to the guide hall toward the south. The calculated flux gain for a typical experiment is between a factor of 1.3 and 3 for all instruments, with the exception of the C-TAX instrument, which stands to gain a factor of >30 in flux at the sample. The new guide system will also offer additional performance gains, such as an increase in Q-range on Bio-SANS. The stated performance gains do not take into account any potential performance gains resulting from renewal and realignment of the guide system. The design of the guide system in the common sections up to about 25 m from the source is considered to be complete and ready for engineering design, while the designs of the instrument-specific guides are in some cases still a work in progress. The present report describes the current status of those designs.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗