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TPSAS-NF1676L-11678-DND

Cloud vertical profiles retrieved from CALIPSO and CloudSat data provide additional information that greatly improves the estimate of atmospheric radiative heating rates and potentially improves the estimate of the global surface radiation budget. To utilize CALIPSO and CloudSat cloud vertical profiles, we combined their profiles and generated merged profiles. Weused the merged cloud profiles and MODIS derived cloud profiles by the CERES cloud algorithm in irradiance computations. In this study, the improvement of the irradiance by CALIPSO and CloudSat derived merged cloud vertical profiles is evaluated by comparing modeled irradiances with and without merged cloud profiles. Because of lower cloud base heights provided by the merged profiles compared with cloud base heights derived from an empirical formula using the MODIS derived cloud top height and optical thickness, the global annual mean surface longwave downward irradiance increases approximately by 7 Wm-2. While CALIPSO version 3 data have not been incorporated in the irradiance computation and the effect of the new CALIPSO data needs to be assessed, a comparison with surface observations suggests an improvement of surface downward longwave irradiance computations. The surface downward longwave irradiance computed with CALIPSO and CloudSat merged clouds agrees better with surface observations than the irradiance computed with MODIS only does. The bias difference over ARM SGP sites with 2 years of data decreases from -5 W m-2to -2 Wm-2, and it decreases from -9 Wm-2to no bias over polar validation sites. The result suggests that CALIPSO CloudSat derived merged clouds significantly improve surface longwave irradiance estimates once they are combined with MODIS derived cloud properties and with temperature and humidity profiles from reanalysis.

Seiji Kato↗
NASA NTRS2004

Aerosol Optical Properties Measured Onboard the Ronald H. Brown During ACE Asia as a Function of Aerosol Chemical Composition and Source Region

During the ACE Asia intensive field campaign conducted in the spring of 2001 aerosol properties were measured onboard the R/V Ronald H. Brown to study the effects of the Asian aerosol on atmospheric chemistry and climate in downwind regions. Aerosol properties measured in the marine boundary layer included chemical composition; number size distribution; and light scattering, hemispheric backscattering, and absorption coefficients. In addition, optical depth and vertical profiles of aerosol 180 deg backscatter were measured. Aerosol within the ACE Asia study region was found to be a complex mixture resulting from marine, pollution, volcanic, and dust sources. Presented here as a function of air mass source region are the mass fractions of the dominant aerosol chemical components, the fraction of the scattering measured at the surface due to each component, mass scattering efficiencies of the individual components, aerosol scattering and absorption coefficients, single scattering albedo, Angstrom exponents, optical depth, and vertical profiles of aerosol extinction. All results except aerosol optical depth and the vertical profiles of aerosol extinction are reported at a relative humidity of 55 +/- 5%. An over-determined data set was collected so that measured and calculated aerosol properties could be compared, internal consistency in the data set could be assessed, and sources of uncertainty could be identified. By taking into account non-sphericity of the dust aerosol, calculated and measured aerosol mass and scattering coefficients agreed within overall experimental uncertainties. Differences between measured and calculated aerosol absorption coefficients were not within reasonable uncertainty limits, however, and may indicate the inability of Mie theory and the assumption of internally mixed homogeneous spheres to predict absorption by the ACE Asia aerosol. Mass scattering efficiencies of non-sea salt sulfate aerosol, sea salt, submicron particulate organic matter, and dust found for the ACE Asia aerosol are comparable to values estimated for ACE 1, Aerosols99, and INDOEX. Unique to the ACE Asia aerosol was the large mass fractions of dust, the dominance of dust in controlling the aerosol optical properties, and the interaction of dust with soot aerosol.

Quinn, P. K.↗
NASA NTRS1973

Effect of shear on aircraft landing

A simulation study was conducted to determine the effect of wind shear on aircraft landings. The landing of various type of commercial and military aircraft was digitally simulated starting from an initial altitude of 300 feet. Assuming no pilot feedback during descent, the deviation in touchdown point due to vertical profiles of wind shear was determined. The vertical profiles of wind shear are defined in terms of surface roughness, Z sub 0, and stability, L, parameters. The effects on touchdown due to Z sub 0 and L have been calculated for the different type aircraft. Comparisons were made between the following types of aircraft: (1) C-130E, (2) C-135A, (3) C-141, (4) DC-8, (5) Boeing 747, and (6) an augmentor-wing STOL. In addition, the wind shear effect on touchdown resulting from different locations of the center of gravity and gross weights was also analyzed.

Luers, J. K.↗
NASA NTRS1999

Origin and Variability of Upper Tropospheric Nitrogen Oxides and Ozone at Northern Mid-Latitudes

Measurements of NO(x) and ozone performed during the NOXAR project are compared with results from the coupled chemistry-climate models ECHAM4.L39(DLR)/CHEM and GISS-model. The measurements are based on flights between Europe and the East coast of America and between Europe and the Far East in the latitude range 40 deg N to 65 deg N. The comparison concentrates on tropopause altitudes and reveals strong longitudinal variations of seasonal mean NO,, of 200 pptv. Either model reproduced strong variations 3 km below but not at the tropopause, indicating a strong missing NO(x) or NO(y) sink over remote areas, e.g. NO(x) to HNO3 conversion by OH from additional OH sources or HNO3 wash-out. Vertical profiles show maximum NO(x) values 2-3 km below the tropopause with a strong seasonal cycle. ECHAM4.L39(DLR)/CHEM reproduces a maximum, although located at the tropopause with a less pronounced seasonal cycle, whereas the GISS model reproduces the seasonal cycle but not the profile's shape due to its coarser vertical resolution. A comparison of NO(x) frequency distributions reveals that both models are capable of reproducing the observed variability, except that ECHAM4.L39(DLR)/CHEM shows no very high NO(x) mixing ratios. Ozone mean values, vertical profiles and frequency distributions are much better reproduced in either model, indicating that the NO(x) frequency distribution, namely the most frequent NO(x) mixing ratio, is more important for the tropospheric photochemical ozone production than its mean value. Both models show that among all sources, NO(x) from lightning contributes most to the seasonal cycle of NO(x) at tropopause altitudes. The impact of lightning in the upper troposphere on NO(x) does not vary strongly with altitude, whereas the impact of surface emissions decreases with altitude. However, the models show significant differences in lightning induced NO(x) concentrations, especially in winter, which may be related to the different treatment of the lower stratospheric coupling between dynamics and chemistry.

Grewe, V.↗
NASA NTRS2016

Multistatic Aerosol Cloud Lidar in Space: A Theoretical Perspective

Accurate aerosol and cloud retrievals from space remain quite challenging and typically involve solving a severely ill-posed inverse scattering problem. In this Perspective, we formulate in general terms an aerosol and aerosol-cloud interaction space mission concept intended to provide detailed horizontal and vertical profiles of aerosol physical characteristics as well as identify mutually induced changes in the properties of aerosols and clouds. We argue that a natural and feasible way of addressing the ill-posedness of the inverse scattering problem while having an exquisite vertical-profiling capability is to fly a multistatic (including bistatic) lidar system. We analyze theoretically the capabilities of a formation-flying constellation of a primary satellite equipped with a conventional monostatic (backscattering) lidar and one or more additional platforms each hosting a receiver of the scattered laser light. If successfully implemented, this concept would combine the measurement capabilities of a passive multi-angle multi-spectral polarimeter with the vertical profiling capability of a lidar; address the ill-posedness of the inverse problem caused by the highly limited information content of monostatic lidar measurements; address the ill-posedness of the inverse problem caused by vertical integration and surface reflection in passive photopolarimetric measurements; relax polarization accuracy requirements; eliminate the need for exquisite radiative-transfer modeling of the atmosphere-surface system in data analyses; yield the day-and-night observation capability; provide direct characterization of ground-level aerosols as atmospheric pollutants; and yield direct measurements of polarized bidirectional surface reflectance. We demonstrate, in particular, that supplementing the conventional backscattering lidar with just one additional receiver flown in formation at a scattering angle close to 170deg can dramatically increase the information content of the measurements. Although the specific subject of this Perspective is the multistatic lidar concept, all our conclusions equally apply to a multistatic radar system intended to study from space the global distribution of cloud and precipitation characteristics.

aerosols↗
NASA NTRS2017

TPSAS-NF1676L-28149-DND

An Optimal Estimation (OE) inversion method has been developed to retrieve vertical profiles of aerosol size distributions, volume/surface concentrations, complex refractive indices, and single scattering albedos using the High Spectral Resolution Lidar (HSRL) and polarimeter measurements. By combining the active and passive remote sensing data, we can take advantages of the high vertical resolution of the lidar measurements and the high information content of the combined observations. There are three components to the new retrieval system: 1) simultaneous aerosol vertical profile retrieval using HSRL data, 2) standalone aerosol retrieval using Research Scanning Polarimeter (RSP), and 3) combined HSRL and RSP optimal estimation retrieval. For the LIDAR retrieval, we solve for number concentrations, mode fractions, aerosol size distributions, and real and imaginary part of refractive indices simultaneously. Based on this information, other parameters such as effective particle radius, surface and volume concentration, single scattering albedo can be derived. The combined HSRL-polarimeter algorithm will provide improved single scattering albedo and refractive index retrievals. The newly developed retrieval algorithm is very fast, and it provides an optimal estimation solution with associated error estimates. By solving for the aerosol vertical profiles using HSRL extinctions and backscattering coefficients from different layers, the new OE method can effectively reduce the impact of measurement noise on the retrieved aerosol microphysical properties. It also enables us to effectively combing HSRL and RSP data in the single OE retrieval system since the passive polarimeter instruments measure path-integrated intensity and polarizations. We have performed sensitivity studies using simulated data and applied the OE algorithms to NASA airborne field data measured by the HSRL-2 and the RSP instruments.

Xu Liu↗
NASA NTRS2001

TRMM Precipitation Radar and Microwave Imager Observations of Convective and Stratiform Rain Over Land and Their Theoretical Implications

Observations of brightness temperature, Tb made over land regions by the Tropical Rainfall Measuring Mission (TRMM) Microwave Imager (TMI) radiometer have been analyzed along with the nearly simultaneous measurements of the vertical profiles of reflectivity factor, Z, made by the Precipitation Radar (PR) onboard the TRMM satellite. This analysis is performed to explore the interrelationship between the TMI and PR data in areas that are covered predominantly by convective or stratiform rain. In particular, we have compared on a scale of 20 km, average vertical profiles of Z with the averages of Tbs in the 19, 37 and 85 GHz channels. Generally, we find from these data that as Z increases, Tbs in the three channels decrease due to extinction. In order to explain physically the relationship between the Tb and Z observations, we have performed radiative transfer simulations utilizing vertical profiles of hydrometeors applicable to convective and stratiform rain regions. These profiles are constructed taking guidance from the Z observations of PR and recent LDR and ZDR measurements made by land-based polarimetric radars.

Prabhakara, C.↗
NASA NTRS1998

Atmos/Atlas 3 Infrared Profile Measurements of Clouds in the Tropical and Subtropical Upper Troposphere

Vertical profiles of infrared cirrus extinction have been derived from tropical and subtropical upper tropospheric solar occultation spectra. The measurements were recorded by the Atmospheric Trace Molecule Spectroscopy (ATMOS) Fourier transform spectrometer during the Atmospheric Laboratory for Applications and Sciences (ATLAS) 3 shuttle flight in November 1994. The presence of large numbers of small ice crystals is inferred from the appearance of broad extinction features in the 8-12 micron region. These features were observed near the tropopause and at lower altitudes. Vertical profiles of the ice extinction (/km) in microwindows at 831, 957, and 1204/cm have been retrieved from the spectra and analyzed with a model for randomly oriented spheroidal ice crystals. An area-equivalent spherical radius of 6 gm is estimated from the smallest ice crystals observed in the 8-12 micron region. Direct penetration of clouds into the lower stratosphere is inferred from observations of cloud extinction extending from the upper troposphere to 50 mbar (20 km altitude). Cloud extinction between 3 and 5 micron shows very little wavelength dependence, at least for the cases observed by the ATMOS instrument in the tropics and subtropics during ATLAS 3.

Rinsland, C. P.↗
NASA NTRS1998

ATMOS/ATLAS 3 Infrared Profile Measurements of Clouds in the Tropical and Subtropical Upper Troposphere

Vertical profiles of infrared cirrus extinction have been derived from tropical and subtropical upper tropospheric solar occultation spectra. The measurements were recorded by the Atmospheric Trace Molecule Spectroscopy (ATMOS) Fourier transform spectrometer during the Atmospheric Laboratory for Applications and Sciences (ATLAS) 3 shuttle flight in November 1994. The presence of large numbers of small ice crystals is inferred from the appearance of broad extinction features in the 8-12 micron region. These features were observed near the tropopause and at lower altitudes. Vertical profiles of the ice extinction (/km) in microwindows at 831, 957, and 1204/cm have been retrieved from the spectra and analyzed with a model for randomly oriented spheroidal ice crystals. An area-equivalent spherical radius of 6 microns is estimated from the smallest ice crystals observed in the 8-12 gm region. Direct penetration of clouds into the lower stratosphere is inferred from observations of cloud extinction extending from the upper troposphere to 50 mbar (20 km altitude). Cloud extinction between 3 and 5 microns shows very little wavelength dependence, at least for the cases observed by the ATMOS instrument in the tropics and subtropics during ATLAS 3.

Rinsland, C. P.↗
NASA NTRS2012

Multi-Scale Three-Dimensional Variational Data Assimilation System for Coastal Ocean Prediction

A multi-scale three-dimensional variational data assimilation system (MS-3DVAR) has been formulated and the associated software system has been developed for improving high-resolution coastal ocean prediction. This system helps improve coastal ocean prediction skill, and has been used in support of operational coastal ocean forecasting systems and field experiments. The system has been developed to improve the capability of data assimilation for assimilating, simultaneously and effectively, sparse vertical profiles and high-resolution remote sensing surface measurements into coastal ocean models, as well as constraining model biases. In this system, the cost function is decomposed into two separate units for the large- and small-scale components, respectively. As such, data assimilation is implemented sequentially from large to small scales, the background error covariance is constructed to be scale-dependent, and a scale-dependent dynamic balance is incorporated. This scheme then allows effective constraining large scales and model bias through assimilating sparse vertical profiles, and small scales through assimilating high-resolution surface measurements. This MS-3DVAR enhances the capability of the traditional 3DVAR for assimilating highly heterogeneously distributed observations, such as along-track satellite altimetry data, and particularly maximizing the extraction of information from limited numbers of vertical profile observations.

Li, Zhijin↗
NASA NTRS2006

Use of In Situ Cloud Condensation Nuclei, Extinction, and Aerosol Size Distribution Measurements to Test a Method for Retrieving Cloud Condensation Nuclei Profiles From Surface Measurements

If the aerosol composition and size distribution below cloud are uniform, the vertical profile of cloud condensation nuclei (CCN) concentration can be retrieved entirely from surface measurements of CCN concentration and particle humidification function and surface-based retrievals of relative humidity and aerosol extinction or backscatter. This provides the potential for long-term measurements of CCN concentrations near cloud base. We have used a combination of aircraft, surface in situ, and surface remote sensing measurements to test various aspects of the retrieval scheme. Our analysis leads us to the following conclusions. The retrieval works better for supersaturations of 0.1% than for 1% because CCN concentrations at 0.1% are controlled by the same particles that control extinction and backscatter. If in situ measurements of extinction are used, the retrieval explains a majority of the CCN variance at high supersaturation for at least two and perhaps five of the eight flights examined. The retrieval of the vertical profile of the humidification factor is not the major limitation of the CCN retrieval scheme. Vertical structure in the aerosol size distribution and composition is the dominant source of error in the CCN retrieval, but this vertical structure is difficult to measure from remote sensing at visible wavelengths.

Ghan, Stephen J.↗
NASA NTRS1973

Spectral structure of tropospheric vertical temperature profiles over Cape Kennedy, Florida.

Recent Jimsphere/Jimsonde measurements of tropospheric temperature profile spectra in the wavelength band from 50 to 2000 meters above the atmospheric boundary layer, taken over Cape Kennedy, Florida, are summarized. The results suggest that the spectra can be represented in the nondimensional form (omega sub g/sigma sub w)phi(k)/sigma sub T squared = S(K), where phi(k) is the temperature profile spectrum at wave number k, omega sub g is the Brunt-Vasala frequency, sigma sub w and sigma sub T denote the standard deviations of the vertical velocity and temperature profiles, and S is a universal function of nondimensional wave number K = k sigma sub w/omega sub g.

Fichtl, G. H.↗
NASA NTRS2023

New Insights on the 7[superscript]Be Cycle in the Ocean

The cosmogenic radionuclide 7[superscript]Be has been applied as a tracer of dynamical processes in the upper ocean and of atmospheric deposition of trace elements at the sea surface. These applications usually assume that 7[superscript]Be is entirely in the dissolved form, and that scavenging and downward export of 7[superscript]Be by settling particles can be neglected. In this work, we explore these assumptions and more generally assess the significance of the 7[superscript]Be activity in the particulate fraction, through the generation of vertical profiles of particulate 7[superscript]Be in the open ocean. From detailed measurements obtained from low-background gamma spectrometers placed in underground facilities, we report vertical profiles of 7[superscript]Be activity in suspended particles (7[superscript]Bep[subscript]) collected in various oceanic regions: the Mediterranean Sea (DYFAMED station), the Indian Sector of the Southern Ocean (station A3-2 from the KEOPS2 cruise), the Sargasso Sea (OFP station), and the subpolar North Atlantic Ocean (GEOVIDE cruise). We find that, in each oceanic region, 7[superscript]Bep[subscript] activities are generally higher in the mixed layer than in the thermocline. They vary in the mixed layer from 3.0 dpm/m3 at DYFAMED to 33.1dpm/m3 at GEOVIDE cross-over station 51/60, i.e., within a range consistent with previous 7[superscript]Bep[subscript] measurements for the open ocean. For the GEOVIDE cruise, the 7[superscript]Bep[subscript] activities measured on different filter types at different depths are corrected for filter offsets derived from multiple 7[superscript]Bep[subscript] measurements at a near-coastal station in the western Mediterranean Sea. We then combine measurements of total 7[superscript]Be activity (Shelley et al., 2017) with our measurements of 7[superscript]Bep[subscript] activity to estimate the solid/solution partitioning of 7[superscript]Be. On average, the particulate fraction would represent 6% of total 7[superscript]Be activity at 5-m water depth (n = 6), 22% at 20 m (n = 2) and 9% at 70 m (n = 3). At GEOVIDE stations, 7[superscript]Bep[subscript] inventories range from 5% to 19% of the total 7[superscript]Be inventories. In the Labrador Sea, the measured 7[superscript]Bep[subscript] inventories are lower than the dry 7[superscript]Be deposition fluxes estimated from aerosol samples collected during GEOVIDE, suggesting that a significant portion of 7[superscript]Bep[subscript] may be removed by sinking particles. The distribution coefficient Kd for 7Be increases with depth, with log10Kd averaging 5.2 ± 0.1 at 5 m to 6.1 ± 0.1 between 70 and 150 m, suggesting that scavenging of dissolved 7[superscript]Be by particles is more pronounced in the thermocline than in the mixed layer when differences in particle concentrations are taken into account. Overall, our study suggests that, at least in some oceanic regions, the removal of 7[superscript]Be by marine particles may be significant and that it may need to be considered in applications of 7[superscript]Be as a tracer of oceanic processes and atmospheric deposition.

Beryllium-7↗
NASA NTRS1979

Inversion of stratospheric aerosol and gaseous constituents from spacecraft solar extinction data in the 0.38-1.0-micron wavelength region

The paper discusses a possible data retrieval technique for the spaceborne Stratospheric Aerosol and Gas Experiment (SAGE). The SAGE instrument has four radiometric channels located at selected intervals in the 0.38-1.0-micron wavelength range. A data reduction procedure is described for minimization of experimental errors on the basis of a detailed simulation of the measurement sequence. An efficient and accurate inversion method is then used for the retrieval of all the constituent vertical profiles. Also, the effects of horizontally inhomogeneous distributions of the constituent vertical profiles are studied based on available data of their global distributions. A simple horizontally inhomogeneous model of stratospheric aerosol and ozone is employed to estimate the perturbation on the retrieval accuracies.

Chu, W. P.↗
NASA NTRS1981

Effects of multiple scattering and surface albedo on the photochemistry of the troposphere

The effect of treatment of incoming solar radiation on the photochemistry of the troposphere is discussed. A one dimensional photochemical model of the troposphere containing the species of the nitrogen, oxygen, carbon, hydrogen, and sulfur families was developed. The vertical flux is simulated by use of the parameterized eddy diffusion coefficients. The photochemical model is coupled to a radiative transfer model that calculates the radiation field due to the incoming solar radiation which initiates much of the photochemistry of the troposphere. Vertical profiles of tropospheric species were compared with the Leighton approximation, radiative transfer, matrix inversion model. The radiative transfer code includes the effects of multiple scattering due to molecules and aerosols, pure absorption, and surface albedo on the transfer of incoming solar radiation. It is indicated that significant differences exist for several key photolysis frequencies and species number density profiles between the Leighton approximation and the profiles generated with, radiative transfer, matrix inversion technique. Most species show enhanced vertical profiles when the more realistic treatment of the incoming solar radiation field is included

Augustsson, T. R.↗
NASA NTRS2009

Production of Lightning NO(x) and its Vertical Distribution Calculated from 3-D Cloud-scale Chemical Transport Model Simulations

A 3-D cloud scale chemical transport model that includes a parameterized source of lightning NO(x), based on observed flash rates has been used to simulate six midlatitude and subtropical thunderstorms observed during four field projects. Production per intracloud (P(sub IC) and cloud-to-ground (P(sub CG)) flash is estimated by assuming various values of P(sub IC) and P(sub CG) for each storm and determining which production scenario yields NO(x) mixing ratios that compare most favorably with in-cloud aircraft observations. We obtain a mean P(sub CG) value of 500 moles NO (7 kg N) per flash. The results of this analysis also suggest that on average, P(sub IC) may be nearly equal to P(sub CG), which is contrary to the common assumption that intracloud flashes are significantly less productive of NO than are cloud-to-ground flashes. This study also presents vertical profiles of the mass of lightning NO(x), after convection based on 3-D cloud-scale model simulations. The results suggest that following convection, a large percentage of lightning NO(x), remains in the middle and upper troposphere where it originated, while only a small percentage is found near the surface. The results of this work differ from profiles calculated from 2-D cloud-scale model simulations with a simpler lightning parameterization that were peaked near the surface and in the upper troposphere (referred to as a "C-shaped" profile). The new model results (a backward C-shaped profile) suggest that chemical transport models that assume a C-shaped vertical profile of lightning NO(x) mass may place too much mass neat the surface and too little in the middle troposphere.

Ott, Lesley↗
NASA NTRS2007

Multi-Sensor Data from A-Train Instruments Brought Together for Atmospheric Research

The A-Train is comprised of a series of instruments, developed independently, that measure highly related atmospheric components along the same flight path. In order to intercompare data from this multitude of sensors, researchers must access, subset, visualize, analyze and correlate distributed atmosphere measurements from the various A-Train instruments. The A-Train Data Depot (ATDD) has been operational for over a year, successfully performing the aforementioned functions on behalf of researchers, thus providing co-registered data from the Cloudsat, CALIOP, AIRS, and MODIS instruments for further intercomparisons. Of late, significant data from OM1 and POLDER are now included in the 'depot'. By specifying the desired spatial and temporal range, the researcher can subset, visualize, co-register, and access multi-sensor A-Train data related to: Cloud, aerosol, atmospheric temperature, and water vapor parameters (vertical profile visualizations); Cloud Pressure, cloud top temperature, water vapor, cloud optical thickness, and aerosol products (horizontal strips subsetted +/- 100km from the profile visualizations), and; Cloud pressure parameters (2-D line plots overlayed on the vertical profiles). All data is plotted using the GIOVANNI data exploration tool. A new feature of GIOVANNI is its ability to have collocated and subsetted data sets as well as PNG image files downloaded to the researcher's computing facility. By providing a convenient way to visualize and acquire multi-sensor data, ATDD affords users more time and effort to further their research.

Smith, Peter M.↗