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Radioactive beams and inverse kinematics: Probing the quantal texture of the nuclear vacuum

The properties of the quantum electrodynamic (QED) vacuum in general, and of the nuclear vacuum (ground) state in particular, are determined by virtual processes implying the excitation of a photon and of an electron-positron pair in the first case and of, for instance, the excitation of a collective quadrupole surface vibration and a particle-hole pair in the nuclear case. Signals of these processes can be detected in the laboratory in terms of what can be considered a nuclear analogue of Hawking radiation. An analogy which extends to other physical processes involving QED vacuum fluctuations like the Lamb shift, pair creation by \(\gamma\) -rays, van der Waals forces and the Casimir effect, to the extent that one concentrates on the eventual outcome resulting by forcing a virtual process to become real, and not on the role of the black hole in defining the event horizon. In the nuclear case, the role of this event is taken over at a microscopic and fully quantum mechanical level, by nuclear probes (reactions) acting on virtual particles of the zero point fluctuations (ZPF) of the nuclear vacuum in a similar irreversible, no-return, fashion as the event horizon does, letting the other particle, entangled with the first one, escape to infinity, and eventually be detected. With this proviso in mind one can posit that the reactions 1 H( 11 Be, 10 Be(2 + ;3.37MeV)) 2 H and 1 H( 11 Li, 9 Li(1/2 - ;2.69MeV)) 3 H together with the associated \( \gamma\) -decay processes suggest a possible nuclear analogy of Hawking radiation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Precise mass measurements of radioactive nuclides for astrophysics

Much of astrophysics is fueled by nuclear physics with observables, such as energy output and elements produced, that are heavily dependent on the masses of the nuclides. A mass precision of at least 50 keV/c 2 for many rare nuclides is needed to adequately discriminate models that explain the observables. In recent decades, the development of new facilities and mass-measurement techniques has made available a wealth of precise and accurate mass data. Further, the new data, in combination with novel codes and models, has greatly enhanced the understanding of astrophysical processes in the universe, but much is still to be learned.

79 ASTRONOMY AND ASTROPHYSICS↗

Rapid insertion of bismuth radioactive isotopes into texaphyrin in aqueous media

Radioisotopes 213 Bi and 207 Bi were successfully inserted into a water-soluble and tumor-targeting texaphyrin ligand. The reaction with 207 Bi(OAc) 3 proceeds in about 15 min in aqueous media without the use of any organic base. The Bi(III) texaphyrin complex formed (3) is stable in aqueous media even in the presence of an excess of competitive chelators (EDTA or citric acid), as well as in human blood plasma. Finally, these results validate texaphyrins as potential candidates for coordinating bismuth radionuclides and set the stage for their use in targeted alpha therapy (TAT).

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Initial dynamic photoactive materials testing of an atmospheric chamber intended for radioactive and hazardous gases

Radioisotopes and hazardous gases can have undetermined environmental pathways. Researchers at Pacific Northwest National Laboratory constructed a chamber that complies with the requirements needed for an atmospheric reaction platform and the safety principles of interacting with hazardous dispersible sources to enable the environmental testing of these gases. Initial dynamic testing showed inter-chamber mixing completed from minutes to 1.5 hours. The photooxidation of butyl iodine showed the presence of signals from reaction products, and intermediaries for up to 50 hours. Current detection limits of the chamber and analytical collection and testing approach were shown to be in the single-digit parts per billion levels. In conclusion, the comparisons between the measured oxidation trends and literature show the utility of performing laboratory experiments to validate the results of modeling for larger-scale scenarios.

54 ENVIRONMENTAL SCIENCES↗

Analysis of Radioactive Releases During Proposed Demolition Activities for the 224-U and 224-UA Buildings - Addendum

A post-demolition modeling analysis is conducted that compares during-demolition atmospheric concentration monitoring results with modeling results based on the actual meteorological conditions during the demolition activities. The 224-U and 224-UA Buildings that were located in the U-Plant UO3 complex in the 200 West Area of the Hanford Site were demolished during the summer of 2010. These facilities converted uranyl nitrate hexahydrate (UNH), a product of Hanford’s Plutonium-Uranium Extraction (PUREX) Plant, into uranium trioxide (UO3). This report is an addendum to a pre-demolition emission analysis and air dispersion modeling effort that was conducted for proposed demolition activities for these structures.

54 ENVIRONMENTAL SCIENCES↗

Air Monitoring Modeling of Radioactive Releases During Proposed PFP Complex Demolition Activities

This report is part of the planning process for the demolition of the 234-5Z, 236-Z, 242-Z, and 291-Z-1 structures at the Plutonium Finishing Plant (PFP) facilities on the Hanford Site. Pacific Northwest National Laboratory (PNNL) supports the U.S. Department of Energy (DOE) and the CH2M HILL Plateau Remediation Company (CHPRC) demolition planning effort by making engineering estimates of potential releases for various potential demolition alternatives. This report documents an analysis considering open-air demolition using standard techniques. It does not document any decisions about the decommissioning approaches; it is expected that this report will be revisited as demolition plans are finalized.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Some Logistical Considerations in Designing a System of Deep Boreholes for Disposal of High-Level Radioactive Waste

Deep boreholes could be a relatively inexpensive, safe, and rapidly deployable strategy for disposing Americaś nuclear waste. To study this approach, Sandia invested in a three year LDRD project entitled “Radionuclide Transport from Deep Boreholes.” In the first two years, the borehole reference design and backfill analysis were completed and the supporting modeling of borehole temperature and fluid transport profiles were done. In the third year, some of the logistics of implementing a deep borehole waste disposal system were considered. This report describes what was learned in the third year of the study and draws some conclusions about the potential bottlenecks of system implementation.

Gray, Genetha Anne↗

DUSEL R&D: BetaCage: A Screener of Ultra-Low-Level Radioactive Surface Contamination (Final Report)

The eventual full-size, radiopure BetaCage will be a low-background, atmospheric-pressure neon drift chamber with unprecedented sensitivity to emitters of low-energy electrons and alpha particles. We expect that the prototype BetaCage already developed will be an excellent screener of alpha particles. Both the prototype and final BetaCage will provide new infrastructure for rare-event science.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗