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Review of the TREAT Conversion Conceptual Design and Fuel Qualification Plan

The U.S. Department of Energy (DOE) is preparing to re establish the capability to conduct transient testing of nuclear fuels at the Idaho National Laboratory (INL) Transient Reactor Test (TREAT) facility. The original TREAT core went critical in February 1959 and operated for more than 6,000 reactor startups before plant operations were suspended in 1994. DOE is now planning to restart the reactor using the plant's original high-enriched uranium (HEU) fuel. At the same time, the National Nuclear Security Administration (NNSA) Office of Material Management and Minimization Reactor Conversion Program is supporting analyses and fuel fabrication studies that will allow for reactor conversion to low-enriched uranium (LEU) fuel (i.e., fuel with less than 20% by weight 235U content) after plant restart. The TREAT Conversion Program's objectives are to perform the design work necessary to generate an LEU replacement core, to restore the capability to fabricate TREAT fuel element assemblies, and to implement the physical and operational changes required to convert the TREAT facility to use LEU fuel.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Predictive Data Analytics Framework Using Advanced Test Reactor Acoustic Data

Although a nuclear reactor is a hostile environment for sensing and electrical communications, the reactor core is amenable to acoustic communication. An acoustic measurement infrastructure (AMI) has been installed at the Advanced Test Reactor (ATR) nozzle trench area to record acoustic signals that has the ability to capture different operating regime of the reactor. This AMI includes ATR in-pile structural components, coolant, acoustic receivers, primary coolant pumps (PCP) as signal sources, a data acquisition system, and signal-processing algorithms, enabling real-time. This report will discusses development of recursive Fast Fourier Transform approach to process in real-time acoustic signals, application of short time Fast Fourier Transform to the ATR brush data to understand the vibration level and to develop spectrograms for different primary coolant pump combinations. The combination of primary coolant pumps for normal and power axial locator mechanism of ATR are different and generates different signatures. These acoustic signatures were used to develop machine learning approaches to automatically classify different operating regimes. This lay the foundation for predictive analytic framework that can be leverage by ATR to optimize their operation and maintenance. The path forward involves continued engagement with ATR and expanded implementation of AMI and predictive framework at ATR and other facilities within INL and at other experimental reactors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Initial Findings in Qualifying the Instrument Thimble 11 Position in the Advanced Test Reactor Critical

The Advanced Test Reactor (ATR) is a versatile nuclear research reactor located at the Idaho National Laboratory (INL) in Eastern Idaho, United States of America. It is one of the most powerful and flexible research reactors in the world and is primarily used for materials testing, isotope production and basic nuclear science research. The ATR is a light-water-cooled, beryllium-moderated reactor with a nominal thermal power capacity of 250 MW utilizing specially designed fuel, arranged in a serpentine pattern to create 9 flux traps. The special design of ATR allows for the neutron flux within each of the flux traps providing flexibility for experiments, programs and allowing experiments with different dose requirements to be irradiated simultaneously. The Advance Test Reactor Critical (ATRC) is a full-scale replica of the ATR core but is housed in a pool instead of a pressure vessel. ATRC is usually operated at less than 600 watts [1]. There are 12 dry instrument thimbles located around the outside of the core tank where a variety of measurement equipment is housed to facilitate reactor operations. Currently Instrument Thimble 11 (IT-11) is not utilized in ATR or ATRC. A range of measurements is ongoing to qualify IT-11 as a test platform for nuclear instrumentation research, development and further experimentation.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗

A radiological assessment of space nuclear power operations near Space Station Freedom

In order to accomplish NASA's more ambitious exploration goals, nuclear reactors may be used in the vicinity of Space Station Freedom (SSF) either as power sources for coorbiting platforms or as part of the propulsion system for departing and returning personnel or cargo vehicles. This study identifies ranges of operational parameters, such as parking distances and reactor cooldown times, which would reasonably guarantee that doses to the SSF crew from all radiation sources would be below guidelines recently recommended by the National Council of Radiation Protection and Measurements. The specific scenarios considered include: (1) the launch and return of a nuclear electric propulsion vehicle, (2) the launch and return of a nuclear thermal rocket vehicle, (3) the operation of an SP-100 class reactor on a coorbiting platform, (4) the activation of materials near operating reactors, (5) the storage and handling of radioisotope thermal generator units, and (6) the storage and handling of fresh and previously operated reactors. Portable reactor shield concepts were examined for relaxing the operational constraints imposed by unshielded (for human proximity operations) reactors and that might also be used to provide additional SSF crew protection from natural background radiation.

Stevenson, Steve↗

Application of Molten Salt Reactor Technology to Nuclear Electric Propulsion Mission

Nuclear electric propulsion (NEP) and planetary surface power missions require reactors that are lightweight, operationally robust, and scalable in power for widely varying scientific mission objectives. Molten salt reactor technology meets all of these requirements and offers an interesting alternative to traditional gas cooled, liquid metal, and heat pipe space reactors.

Patton, Bruce↗

Application of Molten Salt Reactor Technology to MMW In-Space NEP and Surface Power Missions

Anticipated manned nuclear electric propulsion (NEP) and planetary surface power missions will require multimegawatt nuclear reactors that are lightweight, operationally robust, and scalable in power for widely varying scientific mission objectives. Molten salt reactor technology meets all of these requirements and offers an interesting alternative to traditional multimegawatt gas-cooled and liquid metal concepts.

Patton, Bruce↗

Advanced Materials Program Summary

Advanced Reactor Technologies (ART) Advanced Materials Program: Provide material solutions to enable design, construction, and operation of licensable advanced reactors Including Gas-cooled Reactors, Fast Reactors, Molten Salt Reactors (solid or liquid fuel) Could be of modular design, and from 350 to 1 Mwe Conduct developmental R&D on structural materials that are best addressed by the national program Integrate program-directed work at national labs & universities and collaboration with international partners to address advanced reactor developer needs Provide qualification data (to NQA-1 or equivalent) on structural materials and develop & validate improved high temperature design methodology Utilize consensus standards organizations when appropriate (e.g., ASME, ASTM, etc.) Target resolution of issues needed for near to mid-term deployment of advanced reactors

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development of a Representative Molten Chloride Fast Reactor Model to Assess the Impact of Nuclear Data

The SCALE code system was employed to conduct a preliminary investigation of nuclear data impacts for a fast spectrum molten chloride salt reactor. A computationally effective depletion model that is representative of the reactor system was successfully developed and used to conduct fuel depletion simulations. Development of this model draws from the SLICE method that was developed at Oak Ridge National Laboratory to enable generation of fuel compositions for an advanced reactor core at equilibrium operation. Eigenvalue uncertainty calculations using the ENDF/B-VII.1 nuclear data library were performed for the reactor in the fresh fuel state and an irradiated fuel state. It was determined that the primary driver of eigenvalue uncertainty was the uncertainty in the 235U (n, 𝛾) cross section. Uncertainty calculation results from this study were compared to results available for a different fast system, a sodium-cooled fast reactor, to confirm similarities and identify differences with respect to nuclear data impacts between the two fast advanced reactor systems.

Hirji, Rakim [Georgia Institute of Technology]↗

A Burst Mode, Ultrahigh Temperature UF4 Vapor Core Reactor Rankine Cycle Space Power System Concept

Static and dynamic neutronic analyses have been performed on an innovative burst mode (100's of MW output for a few thousand seconds) Ulvahigh Temperature Vapor Core Reactor (UTVR) space nuclear power system. The NVTR employs multiple, neutronically-coupled fissioning cores and operates on a direct, closed Rankine cycle using a disk Magnetohydrodynamic (MHD) generater for energy conversion. The UTVR includes two types of fissioning core regions: (1) the central Ultrahigh Temperature Vapor Core (UTVC) which contains a vapor mixture of highly enriched UF4 fuel and a metal fluoride working fluid and (2) the UF4 boiler column cores located in the BeO moderator/reflector region. The gaseous nature of the fuel the fact that the fuel is circulating, the multiple coupled fissioning cores, and the use of a two phase fissioning fuel lead to unique static and dynamic neutronic characteristics. Static neutronic analysis was conducted using two-dimensional S sub n, transport theory calculations and three-dimensional Monte Carlo transport theory calculations. Circulating-fuel, coupled-core point reactor kinetics equations were used for analyzing the dynamic behavior of the UTVR. In addition to including reactivity feedback phenomena associated with the individual fissioning cores, the effects of core-to-core neutronic and mass flow coupling between the UTVC and the surrounding boiler cores were also included in the dynamic model The dynamic analysis of the UTVR reveals the existence of some very effectlve inherent reactivity feedback effects that are capable of quickly stabilizing this system, within a few seconds, even when large positive reactivity insertions are imposed. If the UTVC vapor fuel density feedback is suppressed, the UTVR is still inherently stable because of the boiler core liquid-fuel volume feedback; in contrast, suppression of the vapor fuel density feedback in 'conventional" gas core cavity reactors causes them to become inherently unstable. Due to the strength of the negative reactivity feedback in the UTVR, it is found that external reactivity insertions alone are inadequate for bringing about significant power level changes during normal reactor operations. Additional methods of reactivity control such as variations in the gaseous fuel mass flow rate, are needed to achieve the desired power level oontrol.

Dugan, E. T.↗

Qualifying the Instrument Thimble 11 Test Position in the Advanced Test Reactor Critical

The Advanced Test Reactor (ATR) is a versatile nuclear research reactor located at the Idaho National Laboratory (INL) in Eastern Idaho, United States of America. It is one of the most powerful and flexible research reactors in the world and is primarily used for materials testing, isotope production and basic nuclear science research. The ATR is a light-water-cooled, beryllium-moderated reactor with a nominal thermal power capacity of 250 MW utilizing specially designed fuel, arranged in a serpentine pattern to create 9 flux traps. The special design of ATR allows for the neutron flux within each of the flux traps providing flexibility for experiments, programs and allowing experiments with different dose requirements to be irradiated simultaneously. The Advance Test Reactor Critical (ATRC) is a full-scale replica of the ATR core but is housed in a pool instead of a pressure vessel. ATRC is usually operated at less than 600 watts [1]. There are 12 dry instrument thimbles located around the outside of the core tank where a variety of measurement equipment is housed to facilitate reactor operations. Currently Instrument Thimble 11 (IT-11) is not utilized in ATR or ATRC. A range of measurements is ongoing to qualify IT-11 as a test platform for nuclear instrumentation research, development and further experimentation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Introduction of Diverse Manual Actuation Design for APR1400

APR1400 is an Advanced Light Water Reactor (ALWR) design with enhanced plant safety and advanced design features. One unit is in commercial operation and 11 are currently under construction, 4 abroad and 7 in Korea. APR1400 adopts full digitalized Man-Machine Interface System (MMIS) to perform the function of control, indication and alarming for safety and non-safety systems APR1400 MMIS is designed to operate the plant from the Main Control Room (MCR) under all anticipated operating conditions including design basis accidents. This advanced MMIS is designed to meet the latest codes, standards and regulatory requirements including the defense-in-depth and diversity requirements, which is intended to mitigate the consequence of a total failure of the digital safety system caused by a software Common Cause Failure (CCF) coupled with anyone of the Design Basis Events. The redundancy of the safety system could be defeated during this CCF condition and the protective function could be rendered inoperable.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Fuels and Materials Challenges for the Very High Temperature Reactor

High Temperature Gas-cooled Reactors (HTGRs) featuring particle fuel are a very mature technology. Commercial deployment occurred in the mid-1980's with the Fort St.Vrain and Thorium Hochtemperatur Reaktor by providing electricity to the grids in the United States and West Germany, respectively. The technology was then adopted by Japan and China with the operation of the High Temperature Test Reactor in Oarai, Japan and the High Temperature Reactor (HTR-10) in China. These commercial reactors typically operate with an outlet coolant temperature of 750 deg. C to 800 deg. C. Increasing the outlet temperature of the HTGR to even higher temperatures above 900 deg. C will improve the thermodynamic efficiency of the system and enable application of a new class of gas reactor, the very high temperature reactor (VHTR), to provide process heat, electricity, and hydrogen to a broad range of industrial customers with the attendant benefits of improved energy security and reduced CO{sub 2} emissions. However, the increase in coolant outlet temperature presents a number of technical challenges associated with fuels and materials. For over a decade, the U.S. Department of Energy has been sponsoring a broad program of research and development with a goal of addressing the technical fuels and materials challenges to support deployment of a VHTR that could safely and economically operate at outlet temperatures of 750 to 950 deg. C. In summary, fuels and materials challenges exist with deploying a VHTR with an outlet temperature of 950 deg. C in the areas of structural materials, graphite and TRISO fuel. However, R and D is underway or has recently been completed suggesting that technical solutions are possible. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Metrics for the technical performance evaluation of light water reactor accident-tolerant fuel

The safe, reliable, and economic operation of the nation’s nuclear power reactor fleet has always been a top priority for the nuclear industry. Continual improvement of technology, including advanced materials and nuclear fuels, remains central to the industry’s success. Enhancing the accident tolerance of light water reactors (LWRs) became a topic of serious discussion following the 2011 Great East Japan Earthquake, resulting tsunami, and subsequent damage to the Fukushima Daiichi nuclear power plant complex. The overall goal for the development of accident-tolerant fuel (ATF) for LWRs is to identify alternative fuel system technologies to further enhance the safety, competitiveness, and economics of commercial nuclear power. Designed for use in the current fleet of commercial LWRs or in reactor concepts with design certifications (GEN-III+), fuels with enhanced accident tolerance would endure loss of active cooling in the reactor core for a considerably longer period of time than the current fuel system while maintaining or improving performance during normal operations. The complex multiphysics behavior of LWR nuclear fuel in the integrated reactor system makes defining specific material or design improvements difficult; as such, establishing desirable performance attributes is critical in guiding the design and development of fuels and cladding with enhanced accident tolerance. Research and development of ATF in the United States is conducted under the U.S. Department of Energy (DOE) Fuel Cycle Research and Development Advanced Fuels Campaign. The DOE is sponsoring multiple teams to develop ATF concepts within multiple national laboratories, universities, and the nuclear industry. Concepts under investigation offer both evolutionary and revolutionary changes to the current nuclear fuel system. This study summarizes the technical evaluation methodology proposed in the United States to aid in the optimization and prioritization of candidate ATF designs.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The TRANSCEND Consortium - In-situ Identification of Surface Corrosion Products on Spent Nuclear Fuels - 20276

The management of spent nuclear fuel is a major ongoing concern for the UK owing to the cessation of reprocessing operations at Sellafield and the large, complex inventory arising from Magnox, AGR, PWR and prototype reactors. Retrieval and relocation operations for legacy fuels are imminent and therefore, any models that enhance our understanding of fuel evolution will help mitigate the risks associated with fuel storage and disposal. The TRANSCEND Consortium on nuclear waste management comprises four work packages, within this current paper we provide a summary overview of progress to date and illustrative results from Theme 3: Spent Nuclear Fuels. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

GTRF Cladding Wear Modeling and Experimental Validation

Coolant flow-induced relative motions between certain structural components in the cores of lightwater nuclear reactor cores, a phenomenon called Grid-To-Rod Fretting (GTRF), can result in progressive wear damage. Wear-through of the cladding on fuel rods can introduce radioactive species into the coolant loop. Such an event is termed a “leaker” and may cause premature and expensive reactor shut-down. GTRF results in wear scars of various sizes, shapes, and depths on the sides of the fuel rod cladding. Fretting damage may also occur on the springs and dimples that hold the fuel rods in place, resulting in the formation of gaps. Due to variability in the operating conditions of the reactor (burn-up rates and operating campaigns) and the associated variable cladding surface oxide film growth and removal rates, the wear coefficient is unlikely to remain constant over time. Therefore, constant wear rate models do not accurately account for transients in the operating conditions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Mechanical property degradation and microstructural evolution of cast austenitic stainless steels under short-term thermal aging

Mechanical testing and microstructural characterization were performed on short-term thermally aged cast austenitic stainless steels (CASS) to understand the severity and mechanisms of thermal-aging degradation experienced during extended operation of light water reactor (LWR) coolant systems. Four CASS materials – CF3, CF3M, CF8, and CF8M – were thermally aged for 1500 hours at 290 °C, 330 °C, 360 °C, and 400 °C. All four alloys experienced insignificant change in strength and ductility properties but a significant reduction in absorbed impact energy. The primary microstructural and compositional changes during thermal aging were spinodal decomposition of the δ-ferrite into α/ α`, precipitation of G-phase in the δ-ferrite, segregation of solute to the austenite/ ferrite interphase boundary, and growth of M23C6 carbides on the austenite/ferrite interphase boundary. These changes were shown to be highly dependent on chemical composition, particularly the concentration of C and Mo, and aging temperature. A comprehensive model is being developed to correlate the microstructural evolution with mechanical behavior and simulation for predictive evaluations of LWR coolant system components.

36 MATERIALS SCIENCE↗

Measuring changes in environmental radiological background from construction of an advanced nuclear reactor testing facility

We present a method to survey and track changes in the environmental radiological background during the construction and operation of advanced nuclear reactor facilities. We discuss the results of two surveys of the environmental gamma-radiation background at NEXT Lab, an advanced nuclear reactor research facility on the campus of Abilene Christian University, prior to the introduction of radioactive material. In both surveys, the observed radiation dosage rates are low, with the highest rates at 15% of the average total radiation dosage rate for the United States. We observe ≈20% changes in the radiological background of the property in locations where the environment was changed by construction and ≈20% variations within the facilities correlated with variations in building materials.

Environment↗