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All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Monitoring Potential Transport of Radioactive Contaminants in Shallow Ephemeral Channels: FY2018

Desert Research Institute (DRI) is conducting a field assessment of the potential for contaminated soil to be transported from the Smoky Site Contamination Area (CA) as a result of storm runoff. This activity supports U.S. Department of Energy (DOE) Environmental Management Nevada Program (EM NV) efforts to establish post-closure monitoring plans for the Smoky Site Soils Corrective Action Unit (CAU) 550. The work is intended to confirm the likely mechanism of transport and determine the meteorological conditions that might cause the movement of contaminated soils, as well as determine the particle size fraction that is most closely associated with transported radionuclide-contaminated soils. These data will facilitate the design of the appropriate post-closure monitoring program. In 2011, DRI installed a meteorological monitoring station on the west side of the Smoky Site CA and a hydrologic (runoff) monitoring station within the CA, near the east side. The meteorological station collects air temperature, wind speed, wind direction, relative humidity, precipitation, solar radiation, barometric pressure, soil temperature, and soil water content data. The maximum, minimum, and average or total values (as appropriate) for each of these parameters are recorded for each 10-minute interval. The maximum, minimum, and average water depth in the flume installed at the hydrologic station are also recorded for each 10-minute interval. This report presents the data collected from these stations during fiscal year (FY) 2018. During the FY2018 reporting period, the warmest months were June, July, and August and the coldest were December through March. Solar radiation showed the same seasonal trend. Monthly mean wind speeds were highest in the spring (March through May) and early summer (June). Winds were generally from the west during the summer and from the north throughout the fall and winter. The monthly average relative humidity ranged from the mid-teens to approximately 50 percent. Humidity was lowest in the fall and highest in the winter. Monthly total precipitation ranged from 0 in October, December, and June to approximately 1.38 inches (in) (35.05 millimeters [mm]) in July. Total precipitation for FY2018 was 3.86 in (98.04 mm). During the reporting period, two runoff events were recorded at the flume. One occurred on July 14, 2018, in response to precipitation earlier the same day. This event produced a peak water depth of 11.26 in (28.60 centimeters [cm]) in the flume, which is equivalent to a discharge of 1.86 cubic feet per second (cfs) (0.05 cubic meters per second [cm/s]) and a velocity of 3.97 feet per second (fps) (1.21 meters per second [m/s]) through the flume. Applying the flume hydraulic measurements to the channel geometry at the nearest surveyed cross-section it was determined that the velocity through the channel was 1.29 fps (0.39 m/s), which is sufficient to transport silts and fine sands. The second flow event occurred in response to earlier precipitation on September 4, 2018. This event produced a peak water depth of 0.78 in (1.98 cm) in the flume, which is equivalent to a discharge of 0.03 cfs (0.001 cm/s) and a velocity of 1.17 fps (0.36 m/s) through the flume. Applying the flume hydraulic measurements to the channel geometry at the nearest surveyed cross-section it was determined that the velocity through the channel was 0.03 fps (0.01 m/s). Although neither runoff event produced sufficient flow velocities through the natural channel to cause local erosion and transport of coarser bedload materials, the velocity of the first runoff event was sufficient to transport silts and fine sands, which have been shown to be preferentially associated with radionuclide contaminants. Therefore, a sampling event was planned after the first flow event in conjunction with a periodic maintenance inspection. As no suspended load sampling is available at this location, bedload samples were collected from the vicinity of the flume on August 7, 2018. The collected sediment was separated into three particle size fractions and each fraction was analyzed for americium-241 (Am-241), plutonium-238 (Pu-238), and plutonium-239/240 (Pu-239/240) by alpha spectrometry. The two smaller particle size fractions had higher concentrations of all three radionuclides than the largest particle size fraction. Additionally, Pu-239/240 had the highest concentration and Pu-238 had the lowest concentration in all samples. The same relationship between the concentrations of Pu-238 and Pu-239/240 was seen in samples reported in FY2013 and FY2014. Observation of meteorological and environmental conditions that lead to storm runoff will help identify parameters and threshold conditions that should be incorporated into postclosure monitoring plans for this and similar sites as well as aid in determining appropriate closure strategies for other Soils CAUs.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2017

Radioactive Decay Chain Truncation Rules for Emergency Response Radiological Assessments

A set of radionuclide - decay chain truncation rules have been developed for use in the Turbo FRMAC and Specialized Hazard Assessment Response Capability (SHARC) software programs used to support radiological emergency response activities . Following the proposed rules, the software will truncate a decay chain after it encounters a progeny radionuclide with a half - life greater than 5,000 years. An analysis of the projected dose from many parent and progeny radionuclides over a 50 - year time period yielded that a radionuclide half - life cutoff of 5,000 years will exclude a negligible dose. Implementing the truncation rules will reduce the time required for assessments and minimize computer hardware requ irements without having a significant detrimental effect on dose projections and emergency response decisions. It is noted that the truncation rules may not be suited for long - term ( greater than 50 year) environmental assessments.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2020

Monitoring Potential Transport of Radioactive Contaminants in Shallow Ephemeral Channels: FY2019

Desert Research Institute (DRI) conducted a field assessment of the potential for contaminated soil to be transported from the Smoky Site Contamination Area (CA) because of storm runoff. This activity supported U.S. Department of Energy (DOE) Environmental Management Nevada Program (EM NV) efforts to establish post-closure monitoring plans for the Smoky Site Soils Corrective Action Unit (CAU) 550. The work was intended to confirm the likely mechanism of transport and determine the meteorological conditions that might cause the movement of contaminated soils, as well as determine the particle size fraction most closely associated with transported radionuclide-contaminated soils. These data will facilitate the design of the appropriate post-closure monitoring program. In 2011, DRI installed a meteorological monitoring station on the west side of the Smoky Site CA and a hydrologic (runoff) monitoring station within the CA, near the east side. The meteorological station collected air temperature, wind speed, wind direction, relative humidity, precipitation, solar radiation, barometric pressure, soil temperature, and soil water content data. The maximum, minimum, and average or total values (as appropriate) for each of these parameters were recorded for each 10-minute interval. The maximum, minimum, and average water depth in the flume installed at the hydrologic station were also recorded for each 10-minute interval. This report presents the data collected from these stations during fiscal year (FY) 2019. During the FY2019 reporting period, the warmest months were June, July, and August and the coldest were December and February. The highest monthly solar radiation (i.e., sunshine) values were recorded in June, July, and August, whereas December through February had the lowest solar radiation values. Monthly mean wind speeds were highest in the spring (April) and early summer (June). Winds were predominantly from the north, except in February, July, August, and September when winds were mostly from the west. The monthly average relative humidity ranged from 17 percent to approximately 60 percent. Humidity was lowest in the summer and highest in the winter. Monthly total precipitation ranged from 0.0 during August and September to 2.22 inches (in) (56.39 millimeters [mm]) in February. Total precipitation for FY2019 was 7.83 in (198.88 mm). During the reporting period, a single, nonzero, flow event was recorded at the flume. This occurred over two days between March 6 and 7, 2019, in response to 1.16 in (29.46 mm) of precipitation falling within 9.3 hours on March 6, 2019. This event produced a peak water depth of 0.39 in (0.99 centimeters [cm]) in the flume, and runoff was measured for approximately 23.5 hours. However, the maximum recorded flow depth was less than the limit for flow discharge and velocity that can be calculated for the six-inch (15 cm) throat of a Parshall flume. The runoff event produced insufficient flow velocities through the natural channel to cause local erosion and transport of bedload materials. No bedload samples were collected for radiological analysis. Observing meteorological and environmental conditions that lead to storm runoff will help identify the parameters and threshold conditions that should be incorporated into post-closure monitoring plans for this and similar Soils CAU sites. Routine monitoring of meteorological and hydrologic parameters at the Smoky Site CA has been discontinued at the request of EM NV, effective at the conclusion of FY2019. Environmental data acquisition was completed and the meteorological and runoff monitoring stations were removed from the Smoky Site on October 15, 2019.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Radioactive Material Dynamics @ NSLS-II [Slides]

RMD @ NSLS-II helps pave the path to a DMMSC: Developing expertise in techniques and experimental methods for DMMSC science; Improving capabilities for models to become microstructurally aware; Workforce training and development; Help refine DMMSC scientific requirements; Complementary to DMMSC XFEL science (EDXD/EXAFS)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2018

Development of an international security standard for devices containing high-activity radioactive sources

Radioisotopes such as Cs-137 and Co-60 are utilized in various medical, industrial, and research applications. This radiological material can be a theft or sabotage target, which necessitates a certain level of security to adequately protect it. The presented work will explore the necessity of an international security standard for devices used in clinical settings that contain high activity radiological material and the facilities that contain these devices. This standard intends to complement existing safety standards; however, it serves a very different purpose: to reduce the threat of radiological theft and sabotage while taking into full consideration the effect on the patient, user safety, and patient workflow with the aim to minimize the unwanted effects of the security measures. The proposed standard will complement existing International Atomic Energy Agency (IAEA) guidance, published in the IAEA Nuclear Security Series. While those documents primarily focus on the state, competent authorities, and regulatory agencies, the proposed industry standard will involve device manufacturers, source producers, and medical staff.

62 RADIOLOGY AND NUCLEAR MEDICINE↗
DOE OSTI2021

Focused Ion Beam analysis of non radioactive samples [PowerPoint]

The presentation includes various images to illustrate the analysis. Helios G4 Plasma FIB: Xe ion columns mills material 30 times faster than Ga; Options include: Energy Dispersive Spectroscopy (EDS), Wavelength Dispersive spectroscopy (WDS) Electron backscattered Diffraction (EBSD), Time of Flight Sims (ToF SIMS), Inert gas/vacuum sample transfer system; Excels at micromachining and collecting 3D datasets using various detection systems.

42 ENGINEERING↗
DOE OSTI2022

International Workshop on Security of Radioactive Sources during Extraordinary Events

On May 2, 2019, a subcontractor to Los Alamos National Laboratory (LANL) inadvertently breached a sealed Cs-137 source while attempting to remove the source for disposition as part of a United States (US) government-sponsored program. The source breach resulted in contamination of personnel, the building, and a release of material to the local environment.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗
DOE OSTI2022

Detection of Marine Borne Radioactive Sources Report

This report describes a preliminary analysis on the utility of modern capabilities to localize radiological sources in marine environment. This study analyzed expected background sources and identified possible approaches based on modeling and simulation analyses. The effort culminated in the design and fabrication of validation experiments which provided favorable supporting data. The conclusions of this effort are not conclusive as to the viability of the approach nor is the underlining hypothesis discounted. Continuation of the experimental approach is recommended with a focus on open-water experimentation.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Trinity 78th Anniversary: re-discovered and newly edited unclassified footage shows use of tanks to collect radioactive samples immediately after Trinity test (Rev. 1)

On July 16, 1945, at 5:29 a.m., a team of Los Alamos scientists successfully detonated the world’s first atomic bomb at a remote section of south-central New Mexico desert, then known as the Alamogordo Bombing Range. This full-scale test, dubbed “Trinity” by the Lab’s first Director J. Robert Oppenheimer, proved the viability of the implosion-type bomb known as The Gadget and ushered in the Atomic Age. Three weeks after Trinity, two Los-Alamos created atomic weapons – Little Boy and Fat Man – were released above Japan, helping to end World War II and changing the course of history forever.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗