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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,531 records · Page 85
All sourcesNASA NTRSDOE OSTI
NASA NTRS1977

A saturation model of the atmosphere of Uranus

A model of the atmospheric structure of Uranus is presented which differs from previous types of models in two important respects: (1) the CH4/H2 ratio is sufficiently large that CH4 is saturated to large depths in the Uranian atmosphere and (2) the internal energy flux is small compared with that due to solar heating. Because of the small internal flux, the thermal flux decreases rapidly with depth and the atmosphere is radiative to large optical depths. A CH4 droplet cloud forms where the atmosphere finally becomes convective due to the internal flux. The model is shown to be in reasonable agreement with published observations of the H2 quadrupole 3-0 and 4-0 bands, the visible (4000-6000 A) CH4 bands, and the infrared emission spectrum.

Danielson, R. E.↗
DOE OSTI2017

MACv2-SP: a parameterization of anthropogenic aerosol optical properties and an associated Twomey effect for use in CMIP6

A simple plume implementation of the second version (v2) of the Max Planck Institute Aerosol Climatology, MACv2-SP, is described. MACv2-SP provides a prescription of anthropogenic aerosol optical properties and an associated Twomey effect. It was created to provide a harmonized description of post-1850 anthropogenic aerosol radiative forcing for climate modeling studies. MACv2-SP has been designed to be easy to implement, change and use, and thereby enable studies exploring the climatic effects of different patterns of aerosol radiative forcing, including a Twomey effect. MACv2-SP is formulated in terms of nine spatial plumes associated with different major anthropogenic source regions. The shape of the plumes is fit to the Max Planck Institute Aerosol Climatology, version 2, whose present-day (2005) distribution is anchored by surface-based observations. Two types of plumes are considered: one predominantly associated with biomass burning, the other with industrial emissions. These differ in the prescription of their annual cycle and in their optical properties, thereby implicitly accounting for different contributions of absorbing aerosol to the different plumes. A Twomey effect for each plume is prescribed as a change in the host model's background cloud-droplet population density using relationships derived from satellite data. Year-to-year variations in the amplitude of the plumes over the historical period (1850–2016) are derived by scaling the plumes with associated national emission sources of SO 2 and NH 3 . Experiments using MACv2-SP are performed with the Max Planck Institute Earth System Model. The globally and annually averaged instantaneous and effective aerosol radiative forcings are estimated to be -0.6 and -0.5 W m -2 , respectively. Forcing from aerosol–cloud interactions (the Twomey effect) offsets the reduction of clear-sky forcing by clouds, so that the net effect of clouds on the aerosol forcing is small; hence, the clear-sky forcing, which is more readily measurable, provides a good estimate of the total aerosol forcing.

Stevens, Bjorn↗
DOE OSTI2022

A review of coarse mineral dust in the Earth system

Mineral dust particles suspended in the atmosphere span more than three orders of magnitude in diameter, from <0.1 µm to more than 100 µm. This wide size range makes dust a unique aerosol species with the ability to interact with many aspects of the Earth system, including radiation, clouds, hydrology, atmospheric chemistry, and biogeochemistry. This review focuses on coarse and super-coarse dust aerosols, which we respectively define as dust particles with a diameter of 2.5–10 µm and 10–62.5 µm. We review several lines of observational evidence indicating that coarse and super-coarse dust particles are transported farther than previously expected and that the abundance of these particles is substantially underestimated in current global models. We synthesize previous studies that used observations, theories, and model simulations to highlight the impacts of coarse and super-coarse dust aerosols on the Earth system, including their effects on dust-radiation interactions, dust-cloud interactions, atmospheric chemistry, and biogeochemistry. Specifically, coarse and super-coarse dust aerosols produce a net positive direct radiative effect (warming) at the top of the atmosphere and can modify temperature and water vapor profiles, influencing the distribution of clouds and precipitation. In addition, coarse and super-coarse dust aerosols contribute a substantial fraction of ice-nucleating particles, especially at temperatures above –23 °C. They also contribute a substantial fraction to the available reactive surfaces for atmospheric processing and the dust deposition flux that impacts land and ocean biogeochemistry by supplying important nutrients such as iron and phosphorus. Furthermore, we examine several limitations in the representation of coarse and super-coarse dust aerosols in current model simulations and remote-sensing retrievals. Because these limitations substantially contribute to the uncertainties in simulating the abundance and impacts of coarse and super-coarse dust aerosols, we offer some recommendations to facilitate future studies. Overall, we conclude that an accurate representation of coarse and super-coarse properties is critical in understanding the impacts of dust aerosols on the Earth system.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1985

Mesoscale generation of available potential energy in the warm sector of an extratropical cyclone

The generation of available potential energy (APE) was evaluated in the warm sector of an extratropical cyclone containing intense convective activity. Mesoscale rawinsonde data from AVE-SESAME '79 was employed. Parametrization techniques were used for latent and sensible heating components, and variations for the Kuo scheme provided convective latent heat release. Radiative transfer models were used to obtain estimates of infrared and solar processes. The results indicated that solar heating was greater than IR cooling near midday. An extensive low-level cloud deck was the most radiatively active area. Negative generation of APE occurred during most of the period for the SESAME domain as a whole. The leading contributor was convective latent heating located primarily in regions of negative efficiency. Infrared cooling was the only component to consistently produce positive generation. Sensible heating provided an important sink of APE in the low levels during the afternoon.

Fuelberg, H. E.↗
DOE OSTI2021

Vertical variation of turbulent entrainment mixing processes in marine stratocumulus clouds using high-resolution digital holography

Marine stratocumulus clouds contribute signi?cantly to the Earth’s radiation budget due to their extensive coverage and high albedo. Yet, subgrid variability in cloud properties such as aerosol concentration, droplet number and precipitation rates lead to considerable errors in global climate models. While these clouds usually have small vertical ex-tent, turbulent entrainment-mixing and precipitation can generate signi?cant variations in droplet number, size and relative dispersion with altitude. In this paper, we analyze turbulent entrainment-mixing processes and the variability in cloud microphysical properties as a function of height within a warm marine stratocumulus cloud layer over the Eastern North Atlantic. We use high resolution airborne holographic measurements and compare them with local turbulence measurements. We ?nd that entrainment-mixing is primarily inhomogeneous near cloud top leading to larger droplet sizes and homogeneous near cloud base leading to smaller droplet sizes. Further analysis of Damk¨ohler number measurements are able to explain the mixing mechanisms at di?erent cloud heights, reinforcing the importance of turbulent mixing and microphysical time scales in deter-mining cloud microphysics.

Desai, Neel↗
DOE OSTI2020

CMIP5 Climate Models Overestimate Cooling by Volcanic Aerosols

We compare projections of the observed hemispherical mean surface temperature (HadCRUT4.6.0.0) and the ensemble mean of CMIP5 climate models' simulations on a set of standard regression model forcing variables. We find that the volcanic aerosol regression coefficients of the CMIP5 simulations are consistently significantly larger (by 40–49%) than the volcanic aerosol coefficients of the observed temperature. The probability that the observed differences are caused just by chance is much less than 0.01. The overestimate is due to the climate models' response to volcanic aerosol radiative forcing. The largest overestimate occurs in the winter season of each hemisphere. We hypothesize that the models' parameterization of aerosol-cloud interactions within ice and mixed phase clouds is a likely source of this discrepancy. Furthermore, the models significantly underestimate the effect of solar variability on temperature for both hemispheres.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1980

Greenhouse models of Venus' high surface temperature, as constrained by Pioneer Venus measurements

Recent measurements conducted from the Pioneer Venus probes and orbiter have provided a significantly improved definition of the solar net flux profile, the gaseous composition, temperature structure, and cloud properties of Venus' lower atmosphere. Using these data, we have carried out a series of one-dimensional radiative-convective equilibrium calculations to determine the viability of the greenhouse model of Venus' high surface temperature and to assess the chief contributors to the greenhouse effect. New sources of infrared opacity include the permitted transitions of SO2, CO, and HCl as well as opacity due to several pressure-induced transitions of CO2. We find that the observed surface temperature and lapse rate structure of the lower atmosphere can be reproduced quite closely with a greenhouse model that contains the water vapor abundance reported by the Venera spectrophotometer experiment. Thus the greenhouse effect can account for essentially all of Venus' high surface temperature. The prime sources of infrared opacity are, in order of importance, CO2, H2O, cloud particles, and SO2, with CO and HCl playing very minor roles.

Pollack, J. B.↗
NASA NTRS2012

Applications for Near-Real Time Satellite Cloud and Radiation Products

At NASA Langley Research Center, a variety of cloud, clear-sky, and radiation products are being derived at different scales from regional to global using geostationary satellite (GEOSat) and lower Earth-orbiting (LEOSat) imager data. With growing availability, these products are becoming increasingly valuable for weather forecasting and nowcasting. These products include, but are not limited to, cloud-top and base heights, cloud water path and particle size, cloud temperature and phase, surface skin temperature and albedo, and top-of-atmosphere radiation budget. Some of these data products are currently assimilated operationally in a numerical weather prediction model. Others are used unofficially for nowcasting, while testing is underway for other applications. These applications include the use of cloud water path in an NWP model, cloud optical depth for detecting convective initiation in cirrus-filled skies, and aircraft icing condition diagnoses among others. This paper briefly describes a currently operating system that analyzes data from GEOSats around the globe (GOES, Meteosat, MTSAT, FY-2) and LEOSats (AVHRR and MODIS) and makes the products available in near-real time through a variety of media. Current potential future use of these products is discussed.

Minnis, Patrick↗
DOE OSTI2024

Microphysical properties of atmospheric soot and organic particles: measurements, modeling, and impacts

Atmospheric soot and organic particles from fossil fuel combustion and biomass burning modify Earth’s climate through their interactions with solar radiation and through modifications of cloud properties by acting as cloud condensation nuclei and ice nucleating particles. Recent advancements in understanding their individual properties and microscopic composition have led to heightened interest in their microphysical properties. This review article provides an overview of current advanced microscopic measurements and offers insights into future avenues for studying microphysical properties of these particles. To quantify soot morphology and ageing, fractal dimension ( D f ) is a commonly employed quantitative metric which allows to characterize morphologies of soot aggregates and their modifications in relation to ageing factors like internal mixing state, core-shell structures, phase, and composition heterogeneity. Models have been developed to incorporate D f and mixing diversity metrics of aged soot particles, enabling quantitative assessment of their optical absorption and radiative forcing effects. The microphysical properties of soot and organic particles are complex and they are influenced by particle sources, ageing process, and meteorological conditions. Furthermore, soluble organic particles exhibit diverse forms and can engage in liquid–liquid phase separation with sulfate and nitrate components. Primary carbonaceous particles such as tar balls and soot warrant further attention due to their strong light absorbing properties, presence of toxic organic constituents, and small size, which can impact human health. Future research needs include both atmospheric measurements and modeling approaches, focusing on changes in the mixing structures of soot and organic particle ensembles, their effects on climate dynamics and human health.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2023

Assessing the Performance of the South American Land Data Assimilation System Version 2 (SALDAS-2) Energy Balance across Diverse Biomes

Understanding the exchange of energy between the surface and the atmosphere is important in view of the climate scenario. However, it becomes a challenging task due to a sparse network of observations. This study aims to improve the energy balance estimates for the Amazon, Cerrado, and Pampa biomes located in South America using the radiation and precipitation forcing obtained from the Clouds and the Earth’s Radiant Energy System (CERES) and the precipitation CPTEC/MERGE datasets. We employed three surface models—Noah-MP, Community Land Model (CLSM), and Integrated Biosphere Simulator (IBIS)—and conducted modeling experiments, termed South America Land Data Assimilation System (SALDAS-2). The results showed that SALDAS-2 radiation estimates had the smallest errors. Moreover, SALDAS-2 precipitation estimates were better than the Global Land Data Assimilation System (GLDAS) in the Cerrado (MBE = −0.16) and Pampa (MBE = −0.19). Noah-MP presented improvements compared with CLSM and IBIS in 100% of towers located in the Amazon. CLSM tends to overestimate the latent heat flux and underestimate the sensible heat flux in the Amazon. Noah-MP and Ensemble outperformed GLDAS in terms latent and sensible heat fluxes. The potential of SALDAS-2 should be emphasized to provide more accurate estimates of surface energy balance.

modeling↗
DOE OSTI2018

Characteristic Atmospheric Radiative Heating Rate Profiles in Arctic Clouds as Observed at Barrow, Alaska

Abstract A 2-yr cloud microphysical property dataset derived from ground-based remote sensors at the Atmospheric Radiation Measurement site near Barrow, Alaska, was used as input into a radiative transfer model to compute radiative heating rate (RHR) profiles in the atmosphere. Both the longwave (LW; 5–100 μm) and shortwave (SW; 0.2–5 μm) RHR profiles show significant month-to-month variability because of seasonal dependence in the vertical profiles of cloud liquid and ice water contents, with additional contributions from the seasonal dependencies of solar zenith angle, water vapor amount, and temperature. The LW and SW RHR profiles were binned to provide characteristic profiles as a function of cloud type and liquid water path (LWP). Single-layer liquid-only clouds are shown to have larger (10–30 K day−1) LW radiative cooling rates at the top of the cloud layer than single-layer mixed-phase clouds; this is due primarily to differences in the vertical distribution of liquid water between the two classes. However, differences in SW RHR profiles at the top of these two classes of clouds are less than 3 K day−1. The absolute value of the RHR in single-layer ice-only clouds is an order of magnitude smaller than in liquid-bearing clouds. Furthermore, for double-layer cloud systems, the phase and condensed water path of the upper cloud strongly modulate the radiative cooling both at the top and within the lower-level cloud. While sensitivity to cloud overlap and phase has been shown previously, the characteristic RHR profiles are markedly different between the different cloud classifications.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2002

Towards a Multisensor Approach to Improve on Current TRMM Retrievals of Clouds and Precipitation

The Tropical Rainfall Measuring Mission (TRMM) was designed to measure tropical rainfall and its variation from a low inclination orbiting satellite. The TRMM payload was carefully chosen to overcome a number of limitations of past satellite observing systems. This payload is predicated on the combination of active and passive observations from the TRMM Precipitation Radar (PR) and TRMM Microwave Imager (TMI) and Visible and Infrared Scanner (VIRS). Our research over the past three years has been devoted to the challenge of developing the most effective way of combining complementary information from these sensors to provide the most consistent estimate of precipitation. We have approached this problem from three directions. The first was to carry out preliminary analysis of passive microwave and infrared data from the TMI and VIRS instruments to understand the character of clear and cloudy skies in the basis defined by polarization and brightness temperature differences. Using this information as a foundation, the properties of two retrieval algorithms were analyzed, one for retrieving ice clouds from VIRS that was developed in parallel with this project and the other for rainfall from the TMI. Finally, the knowledge gleaned from each of these studies, coupled with ancillary data from NWP models and a broadband radiative transfer model, was used to create and algorithm for synthesizing the principal components of the Earth's energy budget from the basic building blocks of the atmosphere, gases, clouds, and precipitation. Principal results from each of these areas of research and their role in the TRMM and climate communities are summarized.

Stephens, Graeme L.↗
NASA NTRS1984

Theoretical development of Monte Carlo codes for modeling cumulus cloud fields

Reflected fluxes are calculated for stratocumulus cloud fields as a function of skycover, cloud aspect ratio, and cloud shape. Cloud liquid water volume is held invariant as cloud shape is varied so that the results can be utilized more effectively by general circulation models and climate models. On the basis of required accuracy in the Earth Radiation Budget Experiment program, an order of magnitude value of 10 W/sq m is used to estimate significant differences between plane parallel and broken cloudiness. This limit is exceeded for cloud covers between 10% and 90%, indicating that plane paralel calculations are not satisfactory at most values of cloud cover. The choice of cloud shape also leads to large differences in reflected fluxes. These differences are traced to the anisotropic intensity pattern out the cloud sides, to the size and shape of the holes between clouds, and to variations in cloud area as viewed from the solar direction. An empirical relationship for effective cloud cover is given at solar zenith angle of theta = 60 deg. This relationship allows for the relatively accurate (delta F = 10 - 15 W/sq m.) computation of broken cloud field reflected fluxes from plane parallel calculations.

Welch, R. M.↗
DOE OSTI2025

Collaborative Proposal: Improving understanding of the internal structure and dynamics of deep convection using ARM observations and large eddy simulations

Recent observational and large eddy simulation (LES) modeling studies have nearly unanimously supported the view of deep cumulus convection being composed of a series of quasi-spherical bubbles of buoyant air, known as moist thermals. Despite the prevalence of moist thermals in deep convection, a comprehensive theory for the dynamics of these structures is lacking. Most current conceptual models for cumulus convection are based on canonical scaling theories for dry thermals or plumes; however, there is considerable evidence that the behavior of moist thermals differs markedly from these theories. Furthermore, the theoretical basis for most cumulus parameterizations originates from the plume conceptual model, and therefore these parameterizations are inconsistent with the real structure of moist convection. Motivated by the aforementioned knowledge gaps, this “end-to-end” research effort use theory, observations, numerical simulations, and direct improvements to the Zhang-McFarlane (ZM) convection scheme in the global climate Community Atmosphere Model (CAM) to address the following research questions: What key environmental parameters determine whether or not shallow convection will transition into deep convection, in the context of thermal-like updrafts? What factors regulate the size of thermals within cumulus updrafts? How does vertical wind shear influence thermal behavior, and as a consequence, vertical velocity and mass flux profiles and the shallow-to-deep convective transition? What are the critical processes that determine updraft vertical velocities and their connection to the vertical mass flux profile for thermal-like updrafts? Idealized LES modeling will be used in conjunction with theoretical models for the core properties of thermal-like updrafts to better understand key processes that regulate thermal ascent rates and entrainment properties. Thermal-tracking procedures will be used to characterize the behavior of thermals within the LES, and recently developed direct measures of entrainment and detrainment will be used to quantify entrainment/detrainment rates. Building from these results, we will analyze the structure of moist thermals from hemispheric range-height indicator scans taken during the Atmospheric Radiation Measurement Cloud, Aerosol, and Complex Terrain Interactions (CACTI) field campaign, and from “real case” LES of CACTI events. This combined modeling and observational analysis will provide essential validation for the existing body of research on moist thermal dynamics, which is based primarily on modeling studies. With the insight gained from the aforementioned activities, we will modify the Zhang-McFarlane convection scheme to improve its representation of updraft vertical velocity and entrainment rate profiles. These process-level changes will be tested in the Community Atmosphere Model to assess the impact on global climate simulations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

The Interaction Between Climate Forcing and Feedbacks

A Perturbed Parameter Ensemble (PPE) with the Community Atmosphere Model version 6 (CAM6) is used to better understand the sensitivity of aerosol forcing and cloud feedbacks to changes in model processes. Aerosol forcing through aerosol-cloud interactions is mostly negative (a cooling) due to shortwave radiation, while feedbacks are positive or negative in different regions due to contrasting longwave and shortwave effects. Both forcing and feedbacks are related to the mean climate state. Higher magnitude cloud radiative effects generally mean larger magnitude net negative forcing and larger magnitude net positive feedback. Aerosol forcing is broadly related to the susceptibility of clouds to drop number. Feedbacks also related to susceptibility, but to a lesser extent and in different regions to aerosol forcing. Aerosol forcing and cloud feedbacks are anti-correlated in the CAM6 PPE such that stronger negative forcing is associated with stronger positive feedbacks. Even the processes governing forcing and feedback sensitivity in the PPE are similar. These include the warm rain formation process, ice loss processes and deep convective intensity.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Cloud Water Chemistry and Aerosol Processing: Assessing the Hydroxyl Radical Burst in Newly Formed Cloud Droplets (Field Campaign Report)

Aerosol particles are tiny liquid or solid particles in the atmosphere, ranging in size from a few nanometers to several micrometers in diameter. Aerosol-cloud interactions are the most uncertain aspect of the climate system, and models routinely underpredict aerosol particle formation. Clouds are well known to alter aerosol size, chemical composition, and radiative properties, but the processes are poorly characterized. Organics and sulfates are the most abundant materials in particles, and for each of these there are significant gaps in the understanding of the role of clouds in their formation and/or aging. Many of the cloud processes are driven by aqueous chemistry that depends on hydroxyl (OH) radicals, the subject of this project.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2016

Stratospheric sulfate geoengineering could enhance the terrestrial photosynthesis rate

Stratospheric sulfate geoengineering could impact the terrestrial carbon cycle by enhancing the carbon sink. With an 8 Tg yr -1 injection of SO 2 to produce a stratospheric aerosol cloud to balance anthropogenic radiative forcing from the Representative Concentration Pathway 6.0 (RCP6.0) scenario, we conducted climate model simulations with the Community Earth System Model – the Community Atmospheric Model 4 fully coupled to tropospheric and stratospheric chemistry (CAM4–chem). During the geoengineering period, as compared to RCP6.0, land-averaged downward visible (300–700 nm) diffuse radiation increased 3.2 W m -2 (11%). The enhanced diffuse radiation combined with the cooling increased plant photosynthesis by 0.07±0.02 µmol C m -2 s -1 , which could contribute to an additional 3.8±1.1 Gt C yr -1 global gross primary productivity without explicit nutrient limitation. This increase could potentially increase the land carbon sink. Suppressed plant and soil respiration due to the cooling would reduce natural land carbon emission and therefore further enhance the terrestrial carbon sink during the geoengineering period. In conclusion, this potentially beneficial impact of stratospheric sulfate geoengineering would need to be balanced by a large number of potential risks in any future decisions about the implementation of geoengineering.

54 ENVIRONMENTAL SCIENCES↗