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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,567 records · Page 87
All sourcesNASA NTRSDOE OSTI
DOE OSTI2017

Recent advances in understanding secondary organic aerosol: Implications for global climate forcing: Advances in Secondary Organic Aerosol

Anthropogenic emissions and land use changes have modified atmospheric aerosol concentrations and size distributions over time. Understanding preindustrial conditions and changes in organic aerosol due to anthropogenic activities is important because these features (1) influence estimates of aerosol radiative forcing and (2) can confound estimates of the historical response of climate to increases in greenhouse gases. Secondary organic aerosol (SOA), formed in the atmosphere by oxidation of organic gases, represents a major fraction of global submicron-sized atmospheric organic aerosol. Over the past decade, significant advances in understanding SOA properties and formation mechanisms have occurred through measurements, yet current climate models typically do not comprehensively include all important processes. Our review summarizes some of the important developments during the past decade in understanding SOA formation. We also highlight the importance of some processes that influence the growth of SOA particles to sizes relevant for clouds and radiative forcing, including formation of extremely low volatility organics in the gas phase, acid-catalyzed multiphase chemistry of isoprene epoxydiols, particle-phase oligomerization, and physical properties such as volatility and viscosity. Several SOA processes highlighted in this review are complex and interdependent and have nonlinear effects on the properties, formation, and evolution of SOA. Current global models neglect this complexity and nonlinearity and thus are less likely to accurately predict the climate forcing of SOA and project future climate sensitivity to greenhouse gases. Efforts are also needed to rank the most influential processes and nonlinear process-related interactions, so that these processes can be accurately represented in atmospheric chemistry-climate models.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1981

4-day waves in the Venus atmosphere

Ultraviolet albedo contrasts in the Venus atmosphere are probably large-scale atmospheric waves propagating slowly with respect to the rapid cloud-top zonal winds. Using a simple theoretical model and profiles of mean wind and thermal structure based on Pioneer Venus data, planetary-scale gravity waves with phase velocities matching the speeds of the UV markings are found. An upward-propagating wave, and waves trapped at cloud levels are proposed as candidates to explain the observed UV features.

Covey, C.↗
NASA NTRS2019

Comparisons of Cloud In-Situ Microphysical Properties of Deep Convective Clouds to Appendix D/P, Using Data from the HAIC-HIWC and HIWC RADAR I Flight Campaigns

In-situ cloud data from three international flight campaigns is compared to the new Federal Aviation Administration (FAA) Title 14 Code of Federal Regulations Part 33 Appendix D mixed-phase/glaciated environmental envelope (1), and the corresponding identical European Aviation Safety Agency (EASA) CS-25 Appendix P envelope (2) (hereafter "Appendix D/P"). Appendix D/P consists of a temperature-altitude envelope, a 99th percentile total water content (TWC99) envelope at the 17.4 Nm distance scale, a distance factor to estimate TWC99 values at other distance scales, ice crystal median mass diameter (MMD), and recommended liquid water content (LWC) levels in mixed-phase icing conditions. The dataset is from 45 flight missions in 3 tropical locations, with 472 runs in approximately 115 clouds, providing about 29,600 Nm of in-cloud data in deep convection over four targeted temperature intervals: 10, 30, 40, and 50 +5 C. The measurements span altitueds from about 17,000' to 39,000'. The comparisons will serve as a basis for regulatory and industry assessment of the efficacy of Appendix D/P.

Strapp, J. Walter↗
DOE OSTI2015

CLOUD FORMATION AND ACCELERATION IN A RADIATIVE ENVIRONMENT

In a radiatively heated and cooled medium, thermal instability (TI) is a plausible mechanism for forming clouds, while the radiation force provides a natural acceleration, especially when ions recombine and opacity increases. Here we extend Field’s theory to self-consistently account for a radiation force resulting from bound–free and bound–bound transitions in the optically thin limit. We present physical arguments for clouds to be significantly accelerated by a radiation force due to lines during a nonlinear phase of the instability. To qualitatively illustrate our main points, we perform both one- and two-dimensional (1D/2D) hydrodynamical simulations that allow us to study the nonlinear outcome of the evolution of thermally unstable gas subjected to this radiation force. Our 1D simulations demonstrate that the TI can produce long-lived clouds that reach a thermal equilibrium between radiative processes and thermal conduction, while the radiation force can indeed accelerate the clouds to supersonic velocities. However, our 2D simulations reveal that a single cloud with a simple morphology cannot be maintained due to destructive processes, triggered by the Rayleigh–Taylor instability and followed by the Kelvin–Helmholtz instability. Nevertheless, the resulting cold gas structures are still significantly accelerated before they are ultimately dispersed.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2011

Matsu: An Elastic Cloud Connected to a SensorWeb for Disaster Response

This slide presentation reviews the use of cloud computing combined with the SensorWeb in aiding disaster response planning. Included is an overview of the architecture of the SensorWeb, and overviews of the phase 1 of the EO-1 system and the steps to improve it to transform it to an On-demand product cloud as part of the Open Cloud Consortium (OCC). The effectiveness of this system is demonstrated in the SensorWeb for the Namibia flood in 2010, using information blended from MODIS, TRMM, River Gauge data, and the Google Earth version of Namibia the system enabled river surge predictions and could enable planning for future disaster responses.

Mandl, Daniel↗
DOE OSTI2020

Convectively Forced Diurnal Gravity Waves in the Maritime Continent

Long-lived, zonally propagating diurnal rainfall disturbances are a highly pronounced and common feature in the Maritime Continent (MC). A recent study argues that these disturbances can be explained as diurnally phase-locked gravity waves. Here we explore the origins of these waves through regional cloud-permitting numerical model experiments. The gravity waves are reproduced and isolated in the model framework through the combined use of realistic geography and diurnally cyclic lateral boundary conditions representative of both characteristic easterly and westerly background zonal flow regimes. These flow regimes are characteristic of the Madden–Julian oscillation (MJO) suppressed and active phase in the MC, respectively. Tests are conducted wherein Borneo, Sumatra, or both islands and/or their orography are removed. These tests imply that the diurnal gravity waves are excited and maintained directly by latent heating from the vigorous mesoscale convective systems (MCSs) that form nocturnally in both Borneo and Sumatra. Removing orography has only a secondary impact on both the MCSs and the gravity waves, implying that it is not critical to these waves. We therefore hypothesize that diurnal gravity waves are fundamentally driven by mesoscale organized deep convection, and are only sensitive to orography to the measure that the convection is affected by the orography and its mesoscale flows. Factor separation further reveals that the nonlinear interaction of synchronized diurnal cycles in Sumatra and Borneo slightly amplifies this gravity wave mode compared to if either island existed in isolation. This nonlinear feedback appears most prominently at longitudes directly between the two islands.

Ruppert, Jr., James H.↗
NASA NTRS1997

The great annihilator 1E 1740.7-2942: Molecular cloud connection and coronal structure

Using (12)CO and (13)CO observations, column density maps of the molecular cloud in the direction of 1E 1740.7-2942 are presented. Hydrogen column densities of the cloud vary between N(sub H) = 3.5 x 10(exp 22)/cu cm and 11 x 10(exp 22)/cu cm, depending on the method employed. From this, it is concluded that, despite the weakness of the iron fluorescent 6.4 keV line, the source may lie inside the cloud, or at least close to its edge. The combined spectra from the Advanced Satellite for Cosmology and Astrophysics (ASCA) and the burst and transient source experiment (BATSE) can be modeled with a two phase accretion disk corona model, where the hot region is detached from the cold disk. Geometrically, the hot phase can be interpreted as a number of active regions above the disk, or as a spherical hot cloud about the central object.

Vilhu, Osmi↗
NASA NTRS1979

Metastable isomers - A new class of interstellar molecules

The abundances of a variety of metastable isomers of small organic molecules, analogous to HNC/HCN, in dense interstellar clouds are considered. These metastable species, some of which are thought to exist as intermediates in laboratory organic chemical reactions, are of considerable interest to chemists. Current ideas of gas-phase, ion-molecule chemistry are utilized to demonstrate that such metastable species should often be present in dense clouds in sufficient abundance to be observed. Unfortunately, the spectral constants of metastable isomers have rarely been determined in the laboratory, and quantum chemical calculations of a varying degree of accuracy must be utilized; results are included of some new quantum chemical calculations. The interstellar chemistry and expected microwave spectra of a representative sample of possibly important interstellar metastable isomers are discussed.

Green, S.↗
NASA NTRS1985

Adiabatic deceleration of secondary antiprotons in the envelopes of supernova exploding in dense clouds

On the basis of well established cosmic ray propagation models, the expected flux of antiprotons in cosmic rays within the few-hundred MeV region is small by comparison with the observed flux. Observational data are presently approached through the examination of the possibility of antiproton production by supernova (SN) envelopes during the expansion phase and while undergoing the consequent adiabatic deceleration. In the case of the SN explosions in dense clouds treated, the SN remnant is decelerated within a few thousand years, generating may antiprotons whose spectrum can be calculated by taking all energy loss processes into account and examining the remnant's spectral evolution. Attention is also given to the possibility of obtaining the antiproton spectrum with enhanced flux at low energies.

Stephens, S. A.↗
DOE OSTI2010

Assessment of Differences in Phase 1 and Phase 2 Test Observations for Waste Treatment Plant Pulse Jet Mixer Tests with Non-Cohesive Solids

The purpose of this work was to assess the apparent discrepancy in critical suspension velocity (UCS) between M3 Phase 1 (Meyer et al. 2009) and Phase 2 testing conducted by Energy Solutions (ES) at Mid-Columbia Engineering (MCE) and to address the applicability of Phase 1 scale-up laws to Phase 2 test results. Three Phase 2 test sequences were analyzed in detail. Several sources of discrepancy were identified including differences in nominal versus actual velocity, definition of model input parameters, and definition of UCS. A remaining discrepancy was shown to not be solely an artifact of Phase 1 data correlations, but was fundamental to the tests. The non-prototypic aspects of Phase 1 testing were reviewed and assessed. The effects of non-prototypic refill associated with the closed loop operation of the jets, previously known to affect cloud height, can be described in terms of a modified settling velocity. When the modified settling velocity is incorporated into the Phase 1 “new” physical model the adjusted new physical model does a better job of predicting the Phase 2 test results. The adjusted new physical model was bench marked with data taken during three prototypic drive tests. Scale-up behavior of the Phase 1 tests was reviewed. The applicability of the Phase 1 scale-up behavior to Phase 2 prototypic testing was analyzed. The effects of non-prototypic refill caused measured values of UCS to be somewhat reduced at larger scales. Hence the scale-up exponents are believed to be smaller than they would have been had there been prototypic refill. Estimated scale-up exponents for the Phase 2 testing are 0.40 for 8-tube tests and 0.36 for 12-tube tests.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗
NASA NTRSDate not supplied

Evaluating and Constraining Models’ Stratocumulus and Cumulus Cloud Feedbacks in the Tropics using Satellite Observations to Reduce Uncertainties in Future Climate Projections

Low-cloud feedbacks are thought to be the greatest source of uncertainty in climate projections on the centennial scale. Past research has mainly focused on the global low-cloud feedback as a whole whereas only a few studies have examined separated contributions from the two main low cloud categories: stratocumulus (Sc) and shallow cumulus (Cu). Here we aim to evaluate and constrain Sc and Cu cloud feedbacks in models using satellite observations to ultimately reduce their contribution to the spread in equilibrium climate sensitivity. We utilize the Cumulus and Stratocumulus CloudSat-CALIPSO Dataset (CASCCAD) recently developed by Cesana et al. (2019), which discriminates Sc from Cu clouds. This algorithm – based on cloud morphological characteristics at the orbital level – outperforms previous cloud-type classifications stemming from passive-sensor measurements. We investigate the observed relationship between the Sc and Cu cloud cover in tropical subsidence oceanic regions and their link to the primary low-cloud controlling factors (sea surface temperature, estimated inversion strength). To gain further insight into the Sc-Cu cloud partitioning, we explore the Sc-Cu relationship during the four meteorological seasons (DJF, MAM, JJA, SON) as well as on monthly timescale. We find a substantial negative correlation between the Sc and Cu cloud cover on annual, seasonal and monthly timescales. We finally evaluate how well climate models of the Coupled Model Intercomparison Project phase 5 (CMIP5) and phase 6 (CMIP6) agree with the observations. These results establish a framework to advance model parameterizations of the underlying physical processes driving the stratocumulus and shallow cumulus clouds (turbulence and convection).

Cloud feedbacks↗
NASA NTRS1989

Stochastic evolution of refractory interstellar dust during the chemical evolution of a two-phase interstellar medium

The evolution course of refractoary interstellar dust during the chemical evolution of a two-phase interstellar medium (ISM) is studied using a simple model of the chemical evolution of ISM. It is assumed that, in this medium, the stars are born in molecular clouds, but new nucleosynthesis products and stellar return are entered into a complementary diffuse medium; the well-mixed matter of each interstellar phase is repeatedly cycled stochastically through the complementary phase and back. The dust is studied on a particle-by-particle bases as it is sputtered by shock waves in the diffuse medium, accretes an amorphous mantle of gaseous refractory atoms while its local medium joins the molecular cloud medium, and encounters the possibility of astration within molecular clouds. Results are presented relevant to the size spectrum of accreted mantles, its age spectrum and the distinction among its several lifetimes, depletion factors of refractory atoms in the diffuse gas, and isotopic anomalies.

Liffman, Kurt↗
DOE OSTI2016

Report on the Second ARM Mobile Facility (AMF2) Roll, Pitch, and Heave (RPH) Stabilization Platform: Design and Evaluation

One of the primary objectives of the U.S. Department of Energy’s Atmospheric Radiation Measurement (ARM) Climate Research Facility’s second Mobile Facility (AMF2) is to obtain reliable measurements of solar, surface, and atmospheric radiation, as well as cloud and atmospheric properties, from ocean-going vessels. To ensure that these climatic measurements are representative and accurate, many AMF2 instrument systems are designed to collect data in a zenith orientation. A pillar of the AMF2 strategy in this effort is the use of a stable platform. The purpose of the platform is to 1) mitigate vessel motion for instruments that require a truly vertical orientation and keep them pointed in the zenith direction, and 2) allow for accurate positioning for viewing or shading of the sensors from direct sunlight. Numerous ARM instruments fall into these categories, but perhaps the most important are the vertically pointing cloud radars, for which vertical motions are a critical parameter. During the design and construction phase of AMF2, an inexpensive stable platform was purchased to perform the stabilization tasks for some of these instruments. The first table compensated for roll, pitch, and yaw (RPY) and was reported upon in a previous technical report (Kafle and Coulter, 2012). Subsequently, a second table was purchased specifically for operation with the Marine W-band cloud radar (MWACR). Computer programs originally developed for RPY were modified to communicate with the new platform controller and with an inertial measurements platform that measures true ship motion components (roll, pitch, yaw, surge, sway, and heave). This platform could not be tested dynamically for RPY because of time constraints requiring its deployment aboard the container ship Horizon Spirit in September 2013. Hence the initial motion tests were conducted on the initial cruise. Subsequent cruises provided additional test results. The platform, as tested, meets all the design and performance criteria established for its use. This is a report of the results of those efforts and the critical points in moving forward

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2011

DEUTERIUM FRACTIONATION AS AN EVOLUTIONARY PROBE IN MASSIVE PROTOSTELLAR/CLUSTER CORES

Clouds of high infrared extinction are promising sites of massive star/cluster formation. A large number of cloud cores discovered in recent years allow for the investigation of a possible evolutionary sequence among cores in early phases. We have conducted a survey of deuterium fractionation toward 15 dense cores in various evolutionary stages, from high-mass starless cores to ultracompact H II regions, in the massive star-forming clouds of high extinction, G34.43+0.24, IRAS 18151-1208, and IRAS 18223-1243, with the Submillimeter Telescope. Spectra of N{sub 2}H{sup +} (3-2), N{sub 2}D{sup +} (3-2), and C{sup 18}O (2-1) were observed to derive the deuterium fractionation of N{sub 2}H{sup +}, D{sub frac} {identical_to} N(N{sub 2}D{sup +})/N(N{sub 2}H{sup +}), as well as the CO depletion factor for every selected core. Our results show a decreasing trend in D{sub frac} with both gas temperature and line width. Since colder and quiescent gas is likely to be associated with less evolved cores, larger D{sub frac} appears to correlate with early phases of core evolution. Such decreasing trend resembles the behavior of D{sub frac} in the low-mass protostellar cores and is consistent with several earlier studies in high-mass protostellar cores. We also find a moderate increasing trend of D{sub frac} with the CO depletion factor, suggesting that sublimation of ice mantles alters the competition in the chemical reactions and reduces D{sub frac}. Our findings suggest a general chemical behavior of deuterated species in both low- and high-mass protostellar candidates at early stages. In addition, upper limits to the ionization degree are estimated to be within 2 Multiplication-Sign 10{sup -7} and 5 Multiplication-Sign 10{sup -6}. The four quiescent cores have marginal field-neutral coupling and perhaps favor turbulent cooling flows.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1998

Validation of POLDER/ADEOS data using a ground-based lidar network: Preliminary results for semi-transparent and cirrus clouds

At mid and tropical latitudes, cirrus clouds are present more than 50% of the time in satellites observations. Due to their large spatial and temporal coverage, and associated low temperatures, cirrus clouds have a major influence on the Earth-Ocean-Atmosphere energy balance through their effects on the incoming solar radiation and outgoing infrared radiation. At present the impact of cirrus clouds on climate is well recognized but remains to be asserted more precisely, for their optical and radiative properties are not very well known. In order to understand the effects of cirrus clouds on climate, their optical and radiative characteristics of these clouds need to be determined accurately at different scales in different locations i.e. latitude. Lidars are well suited to observe cirrus clouds, they can detect very thin and semi-transparent layers, and retrieve the clouds geometrical properties i.e. altitude and multilayers, as well as radiative properties i.e. optical depth, backscattering phase functions of ice crystals. Moreover the linear depolarization ratio can give information on the ice crystal shape. In addition, the data collected with an airborne version of POLDER (POLarization and Directionality of Earth Reflectances) instrument have shown that bidirectional polarized measurements can provide information on cirrus cloud microphysical properties (crystal shapes, preferred orientation in space). The spaceborne version of POLDER-1 has been flown on ADEOS-1 platform during 8 months (October 96 - June 97), and the next POLDER-2 instrument will be launched in 2000 on ADEOS-2. The POLDER-1 cloud inversion algorithms are currently under validation. For cirrus clouds, a validation based on comparisons between cloud properties retrieved from POLDER-1 data and cloud properties inferred from a ground-based lidar network is currently under consideration. We present the first results of the validation.

Chepfer, H.↗
NASA NTRS2003

The Lifetimes of Nitriles (-C*N) and Acids (-COOH) during Ultraviolet Photolysis and Their Survival in Space

Nitriles are one of the most common classes of molecules observed in the gas phase in space, with over a dozen having been positively identified in interstellar and circumstellar environments through the detection of their rotational transitions. Acids, in contrast, are much less common. In this paper we present laboratory data comparing the stability of two structurally related acid-nitrile pairs to ultraviolet (UV) photolytic destruction: acetic acid vs. acetonitrile (CH3-COOH vs. CH3-CN) and glycine vs. aminoacetonitrile (H2N-CH2-COOH vs. H2N-CH2-CN). We find that the nitriles are destroyed ten and five times more slowly (respectively) by UV photolysis than are the corresponding acids. This suggests that whatever their relative formation rates, acids may be less abundant than nitriles in interstellar environments in part because they are more rapidly destroyed by photolysis. The results of this infrared (IR) spectral matrix isolation study indicate that during the lifetime of a typical interstellar cloud, even in its darkest regions, a population of acids in the gas phase will likely be diminished by at least half. Since aminoacetonitrile is a precursor to the amino acid glycine, and far more stable, presolar aminoacetonitrile may be a contributor to the deuterium enriched glycine detected in meteorites. It would clearly be informative to search for aminoacetonitrile (the nitrile corresponding to glycine) in the regions where the amino acid glycine has been reported.

Bernstein, Max P.↗
DOE OSTI2013

Dynamic Modeling and Control Studies of a Two-Stage Bubbling Fluidized Bed Adsorber-Reactor for Solid-Sorbent CO{sub 2} Capture

A one-dimensional, non-isothermal, pressure-driven dynamic model has been developed for a two-stage bubbling fluidized bed (BFB) adsorber-reactor for solid-sorbent carbon dioxide (CO{sub 2}) capture using Aspen Custom Modeler® (ACM). The BFB model for the flow of gas through a continuous phase of downward moving solids considers three regions: emulsion, bubble, and cloud-wake. Both the upper and lower reactor stages are of overflow-type configuration, i.e., the solids leave from the top of each stage. In addition, dynamic models have been developed for the downcomer that transfers solids between the stages and the exit hopper that removes solids from the bottom of the bed. The models of all auxiliary equipment such as valves and gas distributor have been integrated with the main model of the two-stage adsorber reactor. Using the developed dynamic model, the transient responses of various process variables such as CO{sub 2} capture rate and flue gas outlet temperatures have been studied by simulating typical disturbances such as change in the temperature, flowrate, and composition of the incoming flue gas from pulverized coal-fired power plants. In control studies, the performance of a proportional-integral-derivative (PID) controller, feedback-augmented feedforward controller, and linear model predictive controller (LMPC) are evaluated for maintaining the overall CO{sub 2} capture rate at a desired level in the face of typical disturbances.

42 ENGINEERING↗