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All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

Monte Carlo simulation of PET and SPECT imaging of {sup 90}Y

Purpose: Yittrium-90 ({sup 90}Y) is traditionally thought of as a pure beta emitter, and is used in targeted radionuclide therapy, with imaging performed using bremsstrahlung single-photon emission computed tomography (SPECT). However, because {sup 90}Y also emits positrons through internal pair production with a very small branching ratio, positron emission tomography (PET) imaging is also available. Because of the insufficient image quality of {sup 90}Y bremsstrahlung SPECT, PET imaging has been suggested as an alternative. In this paper, the authors present the Monte Carlo-based simulation–reconstruction framework for {sup 90}Y to comprehensively analyze the PET and SPECT imaging techniques and to quantitatively consider the disadvantages associated with them. Methods: Our PET and SPECT simulation modules were developed using Monte Carlo simulation of Electrons and Photons (MCEP), developed by Dr. S. Uehara. PET code (MCEP-PET) generates a sinogram, and reconstructs the tomography image using a time-of-flight ordered subset expectation maximization (TOF-OSEM) algorithm with attenuation compensation. To evaluate MCEP-PET, simulated results of {sup 18}F PET imaging were compared with the experimental results. The results confirmed that MCEP-PET can simulate the experimental results very well. The SPECT code (MCEP-SPECT) models the collimator and NaI detector system, and generates the projection images and projection data. To save the computational time, the authors adopt the prerecorded {sup 90}Y bremsstrahlung photon data calculated by MCEP. The projection data are also reconstructed using the OSEM algorithm. The authors simulated PET and SPECT images of a water phantom containing six hot spheres filled with different concentrations of {sup 90}Y without background activity. The amount of activity was 163 MBq, with an acquisition time of 40 min. Results: The simulated {sup 90}Y-PET image accurately simulated the experimental results. PET image is visually superior to SPECT image because of the low background noise. The simulation reveals that the detected photon number in SPECT is comparable to that of PET, but the large fraction (approximately 75%) of scattered and penetration photons contaminates SPECT image. The lower limit of {sup 90}Y detection in SPECT image was approximately 200 kBq/ml, while that in PET image was approximately 100 kBq/ml. Conclusions: By comparing the background noise level and the image concentration profile of both the techniques, PET image quality was determined to be superior to that of bremsstrahlung SPECT. The developed simulation codes will be very useful in the future investigations of PET and bremsstrahlung SPECT imaging of {sup 90}Y.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2013

SNM neutron detection using a time-gated synthetic aperture hybrid approach

This work focuses on using forward and adjoint transport in a hybrid application of 3-D deterministic (PENTRAN) and Monte Carlo (MCNP5) codes to model a series of neutron detector blocks. These blocks, or 'channels, ' contain a unique set of moderators with 4 atm He-3 detectors tuned to detect and profile a gross energy spectrum of a passing neutron (SNM) source. Ganging the units together as a large area system enables one to apply time gating the source-detector response to maximize signal to noise responses from a passing source with minimal background; multiple units may be positioned as a collective synthetic aperture detector array to be used as a way of performing real time neutron spectroscopy for detecting special nuclear materials in moving vehicles. The initial design, detector response coupling, confirmation of initial design functionality using adjoint transport calculations, and realistic simulation using PENTRAN and MCNP5 are presented. Future work will include optimization and application to realistic scenarios and additional sources. (authors)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

FCC-ee interaction region backgrounds

The FCC-ee machine induced backgrounds on the two proposed detectors (CLD and IDEA) have been studied in detail. Synchrotron Radiation (SR) considerations dictate the Interaction Region (IR) optimization. An asymmetric IR design limits the final bend critical energy to 100 keV. Masks placed before the final focus quadrupole protect the detector from direct hits, and a shield placed around the beam pipe from secondary particles, keeping the effect of SR on the detector to negligible levels. The most important source of background is expected to be the Incoherent Pair Creation (IPC). Its effect has been studied in full simulation and reconstruction, and it was shown that it will not pose a problem for the detector, even if conservative estimations for the time resolution of the detector sensors are assumed. Moreover, the γγ → hadrons, radiative Bhabhas and beam-gas interaction induced backgrounds were studied. All were found to have small to negligible effect on the detector. Finally overall, the FCC–ee interaction region backgrounds are not expected to compromise the detector performance.

47 OTHER INSTRUMENTATION↗
DOE OSTI2014

Analog neutron transport for nuclear instrumentation applications with the Monte-Carlo code TRIPOLI-4 - Paper 3

Monte-Carlo codes simulating particle transport usually make use of well-known variance reduction techniques, leading to more efficient simulations. Even in configurations which do not deal with deep-penetration, some of these techniques, such as the implicit capture, are actually often used by default. The statistical weight of the simulated particles is then modified in order to take into account the modification of the sampling without introducing any bias in the estimation process. For instance, the implicit capture decreases the statistical weight of the particles at each collision, whereas the sampling of a single outgoing particle increases this statistical weight in case of scattering reactions producing multiple neutrons. In addition, Russian roulette and splitting operations, which are usually also played at each collision, lead to other modifications of the statistical weights. As a result, Monte-Carlo codes provide particle histories that are valid on average, but collect statistical weights which differ from 1, when tallying the estimation of the quantities of interest. Yet, some nuclear instrumentation calculations inherently need to work with statistical weights equal to 1, since either individual events have to be collected (such as the arrival of a particle at a detector, the measurement of a time of flight, etc), or the coincidence of events or also correlations between individual events have to be taken into account. To address these specific applications with Monte-Carlo simulation codes, users need a full analog simulation mode. The continuous-energy Monte-Carlo code TRIPOLI4{sup R} is mainly dedicated to shielding, reactor physics and criticality safety calculations. Its capabilities have recently been extended to widen its use to nuclear instrumentation with the possibility of γ-spectrometry calculations and the simulation of photonuclear reactions for instance. Other features needed by nuclear instrumentation applications have been available in TRIPOLI-4 for a long time, such as the sampling of the time variable and the possibility of tallying in a time grid for most of the available tallies (fluxes, reaction rates, dose equivalent rates, energy depositions, etc). In TRIPOLI-4, the transport between two consecutive collisions is analog if no variance reduction technique is requested by the user to handle deep-penetration configurations. However, up to the version 9 of the code, the collision itself is sampled in a non-analog way. This paper presents a first implementation of a full analog neutron transport mode in TRIPOLI-4, preliminary verification results and an application of this functionality to the simulation of the Nucifer detector located in Saclay, France. It should be noted that only neutron transport is dealt with in this work and that all nuclear data come from JEFF-3.1.1 or ENDF/B-VII.0 evaluations, including fission data when needed. (authors)

61 RADIATION PROTECTION AND DOSIMETRY↗
NASA NTRS2004

Neural network tracking and extension of positive tracking periods

Feature detectors have been considered for the role of supplying additional information to a neural network tracker. The feature detector focuses on areas of the image with significant information. Basically, if a picture says a thousand words, the feature detectors are looking for the key phrases (keypoints). These keypoints are rotationally invariant and may be matched across frames. Application of these advanced feature detectors to the neural network tracking system at JPL has promising potential. As part of an ongoing program, an advanced feature detector was tested for augmentation of a neural network based tracker. The advance feature detector extended tracking periods in test sequences including aircraft tracking, rover tracking, and simulated Martian landing. Future directions of research are also discussed.

feature extraction↗
DOE OSTI2019

Investigating the practicality of a minimally defined co-axial HPGe detector model using MCNP

An MCNP model of a co-axial HPGe detector, defined by the specification sheet and without parameter optimization, was used to assess practicality for efficiency characterization and complex spectra simulation. Simulated efficiencies, with and without Gaussian energy broadening, were compared against an experimental calibration for a standard counting geometry. Results show that this minimal detector model predicted efficiencies within 6% of experimental values at energies above 100 keV, while including energy broadening offered little improvement. Furthermore, this work shows that extensive detector characterization and optimization of parameters is not absolutely necessary, thereby reducing the experimental burden associated with detector modeling for many applications.

42 ENGINEERING↗
DOE OSTI2010

DynamiX, numerical tool for design of next-generation x-ray telescopes

We present a new code aimed at the simulation of grazing-incidence x-ray telescopes subject to deformations and demonstrate its ability with two test cases: the Simbol-X and the International X-ray Observatory (IXO) missions. The code, based on Monte Carlo ray tracing, computes the full photon trajectories up to the detector plane, accounting for the x-ray interactions and for the telescope motion and deformation. The simulation produces images and spectra for any telescope configuration using Wolter I mirrors and semiconductor detectors. This numerical tool allows us to study the telescope performance in terms of angular resolution, effective area, and detector efficiency, accounting for the telescope behavior. We have implemented an image reconstruction method based on the measurement of the detector drifts by an optical sensor metrology. Using an accurate metrology, this method allows us to recover the loss of angular resolution induced by the telescope instability. In the framework of the Simbol-X mission, this code was used to study the impacts of the parameters on the telescope performance. In this paper we present detailed performance analysis of Simbol-X, taking into account the satellite motions and the image reconstruction. To illustrate the versatility of the code, we present an additional performance analysis with a particular configuration of IXO.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2026

A Cryogenic Muon Tagging System Integrated with a Superconducting Qubit Device for Radiation-Induced Error Mitigation

Superconducting qubits are highly sensitive to ionizing radiation, which can induce correlated errors and limit scalable fault-tolerant quantum computing. In particular, cosmic-ray muons can deposit energy in the substrate, generating phonon bursts that break Cooper pairs and produce quasiparticles, leading to correlated decoherence events across multiple qubits. We present the development of a cryogenic muon tagging system based on Kinetic Inductance Detectors (KIDs) and its integration with superconducting quantum hardware. Originally developed within the ACE-SuperQ project and validated as a standalone detector, the system demonstrated a muon tagging efficiency of approximately 90% and excellent agreement with Monte Carlo simulations. Building on this validation, the tagging system has been integrated with a multi-qubit superconducting chip operated in a dilution refrigerator. The detector configuration consists of a multi-layer KID stack arranged above and below the quantum device, enabling time-coincident identification of muon-induced events within the same cryogenic environment. The integrated setup has been successfully commissioned, enabling simultaneous operation of the qubit chip and the muon tagging system. A first measurement campaign has been carried out, and preliminary data show time-correlated events between the muon tagging detectors and the qubit readout. A quantitative analysis of radiation-induced effects on qubit performance is currently ongoing. This work represents a step toward the implementation of event-level radiation tagging as a tool for characterizing and potentially mitigating correlated errors in superconducting quantum processors, while establishing a modular platform for future studies at the interface between particle physics and quantum information science.

Roy, Tanay [Fermilab] (ORCID:000000019442862X)↗
DOE OSTI2019

Active interrogation of Special Nuclear Material containers using AmBe quasi-forward biased directional source and PGNAA

Special Nuclear Material (SNM) including 95% 235 U and 239 Pu is capable of being identified by utilizing a quasi-forward directional AmBe source from Patent No: US20190013109A1 using Prompt Gamma Neutron Activation Analysis (PGNAA) simulated with Monte-Carlo N-Particle transport 6.2 (MCNP). HPGe and LaBr 3 detector arrays were used to identify and quantify the peak-to-background and peak-to-total ratios of the associated photon spectra from the SNM encased in a polyethylene shield. The conducted simulations varied the volume of the SNM and neutron source strength in the MCNP data card to conduct an uncertainty analysis. Photopeaks identified include K-shell X-rays from 235 U and 239 Pu, 61 keV from fission, 2.223 MeV prompt gamma from hydrogen, 511 keV annihilation, and a single and double escape peak from the prompt gamma interaction from hydrogen. Relationships between peak-to-total and peak-to-background as a function of SNM and particle history were investigated to aid in the analysis. The capabilities of both detector systems to acquire well resolved photopeak with a 5% relative error or less, with a 1 Ci source activity, and a peak-to-background ratio of 1.15. Finally, this was determined to take 326 s for LaBr 3 and 163 s for HPGe which is comparable to current methods for material detection which take between 100 and 900 s to acquire.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2011

Hadron-therapy beam monitoring: Towards a new generation of ultra-thin p-type silicon strip detectors

Hadron-therapy has gained increasing interest for cancer treatment especially within the last decade. System commissioning and quality assurance procedures impose to monitor the particle beam using 2D dose measurements. Nowadays, several monitoring systems exist for hadron-therapy but all show a relatively high influence on the beam properties: indeed, most devices consist of several layers of materials that degrade the beam through scattering and energy losses. For precise treatment purposes, ultra-thin silicon strip detectors are investigated in order to reduce this beam scattering. We assess the beam size increase provoked by the Multiple Coulomb Scattering when passing through Si, to derive a target thickness. Monte-Carlo based simulations show a characteristic scattering opening angle lower than 1 mrad for thicknesses below 20 {mu}m. We then evaluated the fabrication process feasibility. We successfully thinned down silicon wafers to thicknesses lower than 10 {mu}m over areas of several cm{sup 2}. Strip detectors are presently being processed and they will tentatively be thinned down to 20 {mu}m. Moreover, two-dimensional TCAD simulations were carried out to investigate the beam detector performances on p-type Si substrates. Additionally, thick and thin substrates have been compared thanks to electrical simulations. Reducing the pitch between the strips increases breakdown voltage, whereas leakage current is quite insensitive to strips geometrical configuration. The samples are to be characterized as soon as possible in one of the IBA hadron-therapy facilities. For hadron-therapy, this would represent a considerable step forward in terms of treatment precision. (authors)

43 PARTICLE ACCELERATORS↗
NASA NTRS2005

Lightning NOx Production and Its Consequences for Tropospheric Chemistry

Cloud-resolving case-study simulations of convective transport and lightning NO production have yielded results which are directly applicable to the design of lightning parameterizations for global chemical transport models. In this work we have used cloud-resolving models (the Goddard Cumulus Ensemble Model (GCE) and MMS) to drive an off-line cloud-scale chemical transport model (CSCTM). The CSCTM, in conjunction with aircraft measurements of NO x in thunderstorms and ground-l;>ased lightning observations, has been used to constrain the amount of NO produced per flash. Cloud and chemistry simulations for several case studies of storms in different environments will be presented. Observed lightning flash rates have been incorporated into the CSCTM, and several scenarios of NO production per intracloud (IC) and per cloud-to-ground (CG) flash have been tested for each storm. The resulting NOx mixing ratios are compared with aircraft measurements taken within the storm (typically the anvil region) to determine the most likely NO production scenario. The range of values of NO production per flash (or per meter of lightning channel length) that have been deduced from the model will be shown and compared with values of production in the literature that have been deduced from observed NO spikes and from anvil flux calculations. Results show that on a per flash basis, IC flashes are nearly as productive of NO as CG flashes. This result simplifies the lightning parameterization for global models (ie., an algorithm for estimating the IC/CG ratio is not necessary). Vertical profiles of lightning NOx mass at the end of the 3-D storm simulations have been summarized to yield suggested profiles for use in global models. Estimates of mean NO production per flash vary by a factor of three from one simulated storm to another. When combined with the global flash rate of 44 flashes per second from NASA's Optical Transient Detector (OTD) measurements, these estimates and the results from other techniques yield global NO production rates of2-9 TgN/year. Simulations of the photochemistry over the 24 hours following a storm has been performed to determine the additional ozone production which can be attributed to lightning NO. Convective transport of HOx precursors leads to the generation of a HOx plume which substantially aids the downstream ozone production.

Pickering, Kenneth E.↗
DOE OSTI2020

GADRAS Batch Inject Tool User Guide

Gamma Detector Response and Analysis Software (GADRAS) is used by the radiation detection and emergency response community to perform modeling and spectral analysis for gamma detector systems. Built into GADRAS is the ability to define a detector, geometry, background characteristics and source composition to generate synthetic spectra for drills and exercises (injects). Consequence Management is currently in development of a sample result data simulator tool in which a deposition model is probed for source conditions at moments in time and locations in space. These values are used to generate realistic sample results for use in drills and exercises. In addition to sample results, there is a need to simulate the actual spectra that would be observed in the field by downlooking HPGe instruments given a deposition activity. This way, the FRMAC Gamma Spectroscopist can practice their process of generating quantified results from spectra on realistic data as well. Recognizing the decades of work done in GADRAS to accurately generate synthetic spectra, this team decided to build a link between the new simulator and GADRAS to generate these spectra quickly and easily. The simulator tool will generate a file that specifies the name of the spectra, its location, date/time of measurement, duration of measurement, height off the ground, and the deposition activity and age for every radionuclide in the simulation. Then, a new tool within the Inject Tab of GADRAS was developed to read in this file given a detector selection and generate In-Situ spectra for each row in the file in any file format the user chooses. This way, simulation cell staff can take these files and then upload them to the appropriate data system (RAMS or RadResponder) for use during drills and exercises. An advanced feature of this tool allows for generating any spectra given an appropriate model and mapping of source to model layer in the batch inject tool. This way, spectra from field sample counts, mobile laboratories, or even fixed laboratories can be generated in bulk given an estimate of the radioactivity concentration or total radioactivity in an import file. This expands the capabilities of this tool a great deal and will make it a more useful tool for CM and others to help estimate detector response for nearly any situation. This user guide will explain the steps needed to perform a batch inject file generation.

61 RADIATION PROTECTION AND DOSIMETRY↗
DOE OSTI2022

Super-porous Pt/CuO/Pt hybrid platform for ultra-sensitive and selective H 2 O 2 detection

A super-porous Pt/CuO/Pt hybrid electrode is demonstrated with extremely high sensing performance parameters for the hydrogen peroxide (H 2 O 2 ) detection. A unique physiochemical approach is adapted for the fabrication of 3-D super-porous Pt/CuO/Pt sensing platform. Here, the super-porous Pt/CuO/Pt hybrid platform demonstrates a superior sensitivity of 16,694 µA mM -1 cm -2 with a limit of detection of 2.91 nM (S/N = 3). It also demonstrates an excellent selectivity against the interfering molecules such as NaCl, fructose, ascorbic acid, citric acid, dopamine and glucose with a wide linear range. The demonstrated performance ranks the Pt/CuO/Pt hybrid platform as one of the best H 2 O 2 sensors as summarized in the Table 2. The super-porous CuO layer is fabricated by a dynamic hydrogen bubbling technique of electrochemical deposition and metallic Pt NP decoration is achieved by the physical vapor deposition (PVD) and post-annealing. The super-porous CuO layer offers a drastically improved electrochemical active surface area, and the Pt NP decoration offers a significantly improved conductivity and improved charge accumulation for the H 2 O 2 reduction. The DFT simulations confirm the predominance of CuO over Cu 2 O and Pt over Pd for the H 2 O 2 detection based on the adsorption energy, density of states and charge accumulation calculations.

36 MATERIALS SCIENCE↗
DOE OSTI2011

A Pulse Shape Analysis Technique for the MAJORANA Experiment

In order to achieve background count rates sufficiently low as to allow the observation of rare events such as neutrinoless double beta (0 ) decay, background suppression techniques are routinely employed. In this paper we present details of a novel Pulse Shape Analysis algorithm which allows single-site events such as 0 decay to be distinguished from multi site background events. The algorithm, which is based on the event by event 2 fitting of experimental signals to a basis data set of unique single site pulse shapes, has been developed through simulation studies and tested experimentally using a Broad Energy Germanium detector. It is found experimentally that the technique is able to successfully identify and reject 99% of multi site events in the single escape peak associated with the gamma decay of 208Tl, whilst maintaining a survival probability of 98% for '0 like' double escape peak events.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2016

Evaluation of Am–Li neutron spectra data for active well type neutron multiplicity measurements of uranium

Safeguarding nuclear material is an important and challenging task for the international community. One particular safeguards technique commonly used for uranium assay is active neutron correlation counting. This technique involves irradiating unused uranium with ( α,n) neutrons from an Am-Li source and recording the resultant neutron pulse signal which includes induced fission neutrons. Although this non-destructive technique is widely employed in safeguards applications, the neutron energy spectra from an Am-Li sources is not well known. Several measurements over the past few decades have been made to characterize this spectrum; however, little work has been done comparing the measured spectra of various Am-Li sources to each other. This paper examines fourteen different Am-Li spectra, focusing on how these spectra affect simulated neutron multiplicity results using the code Monte Carlo N-Particle eXtended (MCNPX). Two measurement and simulation campaigns were completed using Active Well Coincidence Counter (AWCC) detectors and uranium standards of varying enrichment. The results of this work indicate that for standard AWCC measurements, the fourteen Am-Li spectra produce similar doubles and triples count rates. Finally, the singles count rates varied by as much as 20% between the different spectra, although they are usually not used in quantitative analysis.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Background discrimination for neutrinoless double beta decay in liquid xenon using Cherenkov light

Neutrinoless double beta decays in liquid xenon produce a significant amount of Cherenkov light, with a photon number and angular distribution that distinguishes these events from common backgrounds. A GEANT4 simulation was used to simulate Cherenkov photon production and measurement in a liquid xenon detector and a multilayer perceptron was used to analyze the resulting distributions to classify events based on their Cherenkov photons. Our results show here that a modest improvement in the sensitivity of neutrinoless double beta decay searches is possible using this technique, but the kinematics of the neutrinoless double beta decay and electron scattering in liquid xenon substantially limit this approach.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Measurements of photo-nuclear jet production in Pb + Pb collisions with ATLAS

Ultra-peripheral heavy ion collisions provide a unique opportunity to study the parton distributions in the colliding nuclei via the measurement of photo-nuclear jet production. An analysis of jet production in ultra-peripheral Pb+Pb collisions at √ s NN = 5.02 TeV performed using data collected with the ATLAS detector in 2015 is described. The data set corresponds to a total Pb+Pb integrated luminosity of 0.38 nb -1 . The ultra-peripheral collisions are selected using a combination of forward neutron and rapidity gap requirements. The cross-sections, not unfolded for detector response, are compared to results from Pythia Monte Carlo simulations re-weighted to match a photon spectrum obtained from the STARlight model. As a result, qualitative agreement between data and these simulations is observed over a broad kinematic range suggesting that using these collisions to measure nuclear parton distributions is experimentally realisable.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗