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At least 1,585 records · Page 88
All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

Spin freezing into a disordered state in CaFeT i 2 O 6 synthesized under high pressure

Double perovskites exhibit a variety of interesting phenomena due to numerous combinations of cation orderings and distortions. CaMnTi 2 O 6 and CaFeTi 2 O 6 are the only two discovered double perovskites that have the columnar type A-site ordering associated with the a + a + c – titling system. The former perovskite, synthesized recently, has a polar structure below T c and shows an unusual ferroelectricity. The latter, while synthesized decades ago, received less investigation. Here, we have synthesized CaFeTi 2 O 6 under high pressure and carried out thorough characterizations through measurements of x-ray powder diffraction (XRD), second harmonic generation (SHG), dc and ac magnetization, Mössbauer spectra, resistivity, thermoelectric power, and specific heat. Although the structural refinement of the XRD pattern cannot distinguish two possible tetragonal phases, SHG measurements help to rule out the possibility of a polar structure observed in CaMnTi 2 O 6 . Fitting the paramagnetic susceptibility to a Curie-Weiss law gives a negligible Weiss constant. The weak exchange interaction gives way to a dipole-dipole interaction and single-ion anisotropy. An anomaly at 1.2 K in the specific heat is too broad for a magnetic transition, but suggestive of a spin-ice-like state as in the pyrochlores. Mössbauer spectroscopy shows two distinct iron sites, as expected for the crystal structure. Both sites are occupied by high-spin Fe 2+ as indicated by the isomer shift. The sharply different temperature dependence of the quadrupole splitting at the two iron sites can be well explained based on the local structural distortions from the refinement of XRD patterns. In conclusion, the line broadening associated with long spin-relaxation times is observed at 6 K as the spin freezing transition is approached from high temperatures.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Magnetic and dielectric property control in the multivalent nanoscale perovskite Eu 0.5 Ba 0.5 TiO 3

We report nanoscale Eu 0.5 Ba 0.5 TiO 3 , a multiferroic in the bulk and candidate in the search to quantify the electric dipole moment of the electron. Eu 0.5 Ba 0.5 TiO 3 , in the form of nanoparticles and other nanostructures is interesting for nanocomposite integration, biomedical imaging and fundamental research, based upon the prospect of polarizability, f-orbital magnetism and tunable optical/radio luminescence. We developed a [non-hydrolytic]sol–[H 2 O-activated]gel route, derived from in-house metallic Ba (s) /Eu (s) alkoxide precursors and Ti{(OCH(CH 3 ) 2 } 4 . Two distinct nanoscale compounds of Ba:Ti:Eu with the parent perovskite crystal structure were produced, with variable dielectric, magnetic and optical properties, based on altering the oxidizing/reducing conditions. Eu 0.5 Ba 0.5 TiO 3 prepared under air/O 2 atmospheres produced a spherical core–shell nanostructure (30–35 nm), with perovskite Eu 0.5 Ba 0.5 TiO 3 nanocrystal core-insulating oxide shell layer (~3 nm), presumed a pre-pyrochlore layer abundant with Eu 3+ . Fluorescence spectroscopy shows a high intensity 5 D 0 → 7 F 2 transition at 622 nm and strong red fluorescence. The core/shell structure demonstrated excellent capacitive properties: assembly into dielectric thin films gave low conductivity (2133 GΩ mm -1 ) and an extremely stable, low loss permittivity of ε eff ~25 over a wide frequency range (tan δ < 0.01, 100 kHz–2 MHz). Eu 0.5 Ba 0.5 TiO 3 prepared under H 2 /argon produced more irregular shaped nanocrystals (20–25) nm, with a thin film permittivity around 4 times greater ( ε eff 101, tan δ < 0.05, 10 kHz–2 MHz, σ ~59.54 kΩ mm -1 ). Field-cooled magnetization values of 0.025 emu g -1 for EBTO-Air and 0.84 emu g -1 for EBTO-Argon were observed. X-ray photoelectron spectroscopy analysis reveals a complex interplay of Eu II/III /Ti III/IV configurations which contribute to the observed ferroic and fluorescence behavior.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
NASA NTRS1996

Accurate Predictions of Mean Geomagnetic Dipole Excursion and Reversal Frequencies, Mean Paleomagnetic Field Intensity, and the Radius of Earth's Core Using McLeod's Rule

The geomagnetic spatial power spectrum R(sub n)(r) is the mean square magnetic induction represented by degree n spherical harmonic coefficients of the internal scalar potential averaged over the geocentric sphere of radius r. McLeod's Rule for the magnetic field generated by Earth's core geodynamo says that the expected core surface power spectrum (R(sub nc)(c)) is inversely proportional to (2n + 1) for 1 less than n less than or equal to N(sub E). McLeod's Rule is verified by locating Earth's core with main field models of Magsat data; the estimated core radius of 3485 kn is close to the seismologic value for c of 3480 km. McLeod's Rule and similar forms are then calibrated with the model values of R(sub n) for 3 less than or = n less than or = 12. Extrapolation to the degree 1 dipole predicts the expectation value of Earth's dipole moment to be about 5.89 x 10(exp 22) Am(exp 2)rms (74.5% of the 1980 value) and the expected geomagnetic intensity to be about 35.6 (mu)T rms at Earth's surface. Archeo- and paleomagnetic field intensity data show these and related predictions to be reasonably accurate. The probability distribution chi(exp 2) with 2n+1 degrees of freedom is assigned to (2n + 1)R(sub nc)/(R(sub nc). Extending this to the dipole implies that an exceptionally weak absolute dipole moment (less than or = 20% of the 1980 value) will exist during 2.5% of geologic time. The mean duration for such major geomagnetic dipole power excursions, one quarter of which feature durable axial dipole reversal, is estimated from the modern dipole power time-scale and the statistical model of excursions. The resulting mean excursion duration of 2767 years forces us to predict an average of 9.04 excursions per million years, 2.26 axial dipole reversals per million years, and a mean reversal duration of 5533 years. Paleomagnetic data show these predictions to be quite accurate. McLeod's Rule led to accurate predictions of Earth's core radius, mean paleomagnetic field intensity, and mean geomagnetic dipole power excursion and axial dipole reversal frequencies. We conclude that McLeod's Rule helps unify geo-paleomagnetism, correctly relates theoretically predictable statistical properties of the core geodynamo to magnetic observation, and provides a priori information required for stochastic inversion of paleo-, archeo-, and/or historical geomagnetic measurements.

Voorhies, Coerte V.↗
DOE OSTI2021

Single-hole couplings in GaAs/AlGaAs double dots probed with transport and EDSR spectroscopy

Here, we report a detailed study of the tunnel barriers within a single-hole GaAs/AlGaAs double quantum dot device (DQD). For quantum information applications as well as fundamental studies, careful tuning and reliable measurements of the barriers are important requirements. In order to tune a DQD device adequately into the single-hole electric dipole spin resonance regime, one has to employ a variety of techniques to cover the extended range of tunnel couplings. In this work, we demonstrate four separate techniques, based upon charge sensing, quantum transport, time-resolved pulsing, and electron dipole spin resonance spectroscopy to determine the couplings as a function of relevant gate voltages and magnetic field. Measurements were performed under conditions of both symmetric and asymmetric tunnel couplings to the leads. Good agreement was observed between different techniques when measured under the same conditions. The results indicate that even in this relatively simple circuit, the requirement to tune multiple gates and the consequences of real potential profiles result in non-intuitive dependencies of the couplings as a function of the plunger gate voltage and the magnetic field.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2017

Nonlinear propagation of vector extremely short pulses in a medium of symmetric and asymmetric molecules

The nonlinear propagation of extremely short electromagnetic pulses in a medium of symmetric and asymmetric molecules placed in static magnetic and electric fields is theoretically studied. Asymmetric molecules differ in that they have nonzero permanent dipole moments in stationary quantum states. A system of wave equations is derived for the ordinary and extraordinary components of pulses. It is shown that this system can be reduced in some cases to a system of coupled Ostrovsky equations and to the equation intagrable by the method for an inverse scattering transformation, including the vector version of the Ostrovsky–Vakhnenko equation. Different types of solutions of this system are considered. Only solutions representing the superposition of periodic solutions are single-valued, whereas soliton and breather solutions are multivalued.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2022

Hilbert space fragmentation in a 2D quantum spin system with subsystem symmetries

We consider a 2D quantum spin model with ring-exchange interaction that has subsystem symmetries associated to conserved magnetization along rows and columns of a square lattice, which implies the conservation of the global dipole moment. The model is not integrable, but violates the eigenstate thermalization hypothesis through an extensive Hilbert space fragmentation, including an exponential number of inert subsectors with trivial dynamics, arising from kinetic constraints. While subsystem symmetries are quite restrictive for the dynamics, we show that they alone cannot account for such a number of inert states, even with infinite-range interactions. We present a procedure for constructing shielding structures that can separate and disentangle dynamically active regions from each other. Notably, subsystem symmetries allow the thickness of the shields to be dependent only on the interaction range rather than on the size of the active regions, unlike in the case of generic dipole-conserving systems.

Khudorozhkov, Alexey↗
NASA NTRS1974

Convection in a Martian magnetosphere

Data from the Mars 2 and 3 orbiters suggest the existence of a Martian magnetosphere. We wish to point out that the Martian magnetosphere would probably be one in which the drag on magnetic field lines tied to a highly conducting day side ionosphere greatly inhibits the line-merging rate at the magnetopause. We deduce a maximum merging speed that is 1-2 orders of magnitude less than the local Alfven speed. We also conclude that the magnetospheric magnetic fields caused by ionospheric currents should be comparable to those due to the small intrinsic dipole moment implied by the spacecraft data. The shape and the size of the magnetosphere are likely to be highly variable.

Rassbach, M. E.↗
NASA NTRS1975

Particle and field environment of Uranus

In 1985 the spin axis of Uranus points within 10 degrees of the sun and the planet's position is very near the solar apex direction. A Uranus mission with an encounter near 1985 might expect to measure the unusual particle and field configuration of a 'pole-on' magnetosphere and also properties of the interstellar medium. Estimates are given of the particle and field environment of Uranus based on extrapolation of solar-wind data from 1 AU and on scaling relations for an earth-type magnetosphere. Since the magnetic moment of Uranus is unknown, all magnetospheric parameters are derived as a function of the dipole strength. The onsets of special magnetospheric properties are identified as the dipole moment increases from small to large values. A fairly complete set of magnetospheric parameters is given for a specific dipole moment to illustrate the case of a large moment.

Siscoe, G. L.↗
NASA NTRS1980

Observations of ULF oscillations in the ion fluxes at small pitch angles with ATS 6

The ultra-low-frequency modulation of ion flux densities at small pitch angles observed by ATS 6 is examined, with particular attention given to a detailed analysis of a representative event. ULF modulation events with maximum modulation at small pitch angles were identified 14 times during the first eight months of operation of the NOAA low-energy particle detector on ATS 6. For the event of October 23, 1974, maximum flux modulation, with a maximum/minimum intensity ratio of 3.7, was observed in the 100 to 150 keV detector at an angle of 32 deg to the ambient field. Spectral analysis of magnetic field data reveals a right elliptically polarized magnetic perturbation with a 96-sec period and a 5-gamma rms amplitude, propagating in the dipole meridian at an angle of about 15 deg to the ambient field and the dipole axis. Proton flux modulation is found to lag the field by up to 180 deg for the lowest-energy channel. Observations are compared with the drift wave, MHD slow wave, and bounce resonant interaction associated with transverse wave models, and it is found that none of the wave models can adequately account for all of the correlated particle and field oscillations.

Su, S.-Y.↗
DOE OSTI2016

Single-resonator double-negative metamaterial

Resonances can be tuned in dielectric resonators in order to construct single-resonator, negative-index metamaterials. For example, high-contrast inclusions in the form of metallic dipoles can be used to shift the first electric resonance down (in frequency) to the first magnetic resonance, or alternatively, air splits can be used to shift the first magnetic resonance up (in frequency) near the first electric resonance. Degenerate dielectric designs become especially useful in infrared- or visible-frequency applications where the resonator sizes associated with the lack of high-permittivity materials can become of sufficient size to enable propagation of higher-order lattice modes in the resulting medium.

36 MATERIALS SCIENCE↗
NASA NTRS1982

Analyzing the Broken Ridge area of the Indian Ocean using magnetic and gravity anomaly maps and geoid undulation and bathymetry data

A higher resolution anomaly map of the Broken Ridge area (2 degree dipole spacing) was produced and reduced to the pole using quiet time data for this area. The map was compared with equally scaled maps of gravity anomaly, geoid undulation, and bathymetry. The ESMAP results were compared with a NASA MAGSAT map derived by averaging data in two-degree bins. A survey simulation was developed to model the accuracy of MAGSAT anomaly maps as a function of satellite altitude, instrument noise level, external noise model, and crustal anomaly field model. A preliminary analysis of the geophysical structure of Broken Ridge is presented and unresolved questions are listed.

Lazarewicz, A. R.↗
DOE OSTI2024

Assessment of Training Performance, Degradation and Robustness of Paraffin-Wax Impregnated Nb 3 Sn Demonstrator Under High Magnetic Field

In the context of high-energy physics, the use of Nb 3 Sn superconducting magnets as a cost-effective and reliable technology depends on improvements in the following areas: long development and manufacturing cycles, conductor degradation after thermal cycling, long training, as well as a demonstration in accelerator magnets with a beam aperture of the full potential of modern Nb 3 Sn conductors. In short, performance, robustness, and cost are the three issues to be addressed. The Magnet Development project (MagDev) of the Swiss Accelerator Research and Technology initiative (CHART) at the Paul Scherrer Institute (PSI) aims to contribute to the solutions to each of these issues, re-thinking the manufacturing and design process. Here in our program, every innovation is to be validated by means of a panoply of fast-turnaround tools: from non-powered and powered samples and coils, tested under background field, to low-field subscale magnets and high field short prototypes. This work presents one element in this panoply of R&D vehicles: a stress-managed Nb 3 Sn coil called BigBOX, impregnated with paraffin wax, and tested, through a collaboration with the Magnet Development Program of the United States (US-MDP), in the background field of Brookhaven National Laboratory (BNL)’s common coils dipole DCC17.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Two-Layer 16 T Cos θ Dipole Design for the FCC

Here, the Future Circular Collider or FCC is a study aimed at exploring the possibility to reach 100 TeV total collision energy which would require 16 tesla dipoles. Upon the conclusion of the High Luminosity Upgrade, the US LHC Accelerator Upgrade Pro-ject in collaboration with CERN will have extensive Nb 3 Sn magnet fabrication experience. This experience includes robust Nb 3 Sn conductor and insulation scheming, 2-layer cos2θ coil fabrication, and bladder-and-key structure and assembly. By making im-provements and modification to existing technology the feasibility of a two-layer 16 tesla dipole is investigated. Preliminary designs indicate that fields up to 16.6 tesla are feasible with conductor grading while satisfying the HE-LHC and FCC specifications. Key challenges include accommodating high-aspect ratio conductor, narrow wedge design, Nb 3 Sn conductor grading, and especially quench protection of a 16 tesla device.

43 PARTICLE ACCELERATORS↗
NASA NTRS2022

High-energy Photon Opacity in the Twisted Magnetospheres of Magnetars

Magnetars are neutron stars characterized by strong surface magnetic fields generally exceeding the quantum critical value of 44.1 TG. High-energy photons propagating in their magnetospheres can be attenuated by QED processes like photon splitting and magnetic pair creation. In this paper, we compute the opacities due to photon splitting and pair creation by photons emitted anywhere in the magnetosphere of a magnetar. Axisymmetric, twisted dipole field configurations embedded in the Schwarzschild metric are treated. The paper computes the maximum energies for photon transparency that permit propagation to infinity in curved spacetime. Special emphasis is given to cases where photons are generated along magnetic field loops and/or in polar regions; these cases directly relate to resonant inverse Compton scattering models for the hard X-ray emission from magnetars and Comptonized soft gamma-ray emission from giant flares. We find that increases in magnetospheric twists raise or lower photon opacities, depending on both the emission locale and the competition between field-line straightening and field strength enhancement. Consequently, given the implicit spectral transparency of hard X-ray bursts and persistent "tail" emission of magnetars, photon splitting considerations constrain their emission region locales and the twist angle of the magnetosphere; these constraints can be probed by future soft gamma-ray telescopes such as COSI and AMEGO. The inclusion of twists generally increases the opaque volume of pair creation by photons above its threshold, except when photons are emitted in polar regions and approximately parallel to the field.

radiation mechanisms: non-thermal↗
DOE OSTI2026

Predicted third-order sweet spots for phi-junction Josephson parametric amplifiers

Hybrid superconductor-semiconductor nanowire Josephson junctions exhibit skewed and phi-shifted current phase relations when an in-plane magnetic field is applied along the weak link's spin-orbit effective field direction. These junctions can have an asymmetric Josephson potential with odd-order nonlinearities. A dominant third-order nonlinearity can be achieved by tuning the magnetic field to a sweet spot. Sweet spots persist when higher order Josephson harmonics are included. This makes it possible to have a single Josephson junction dipole element with three-wave mixing capability, which is favorable for pump-efficient amplification. Electrostatic gate tunability of the semiconductor weak link can make it operable within an extended range of working frequencies, and the inclusion of micromagnets can facilitate near-zero magnetic field operation.

Reza, Tasnum [Univ. of Pittsburgh, PA (United Stat↗
DOE OSTI2015

Progress with high-field superconducting magnets for high-energy colliders

One of the possible next steps for high-energy physics research relies on a high-energy hadron or muon collider. The energy of a circular collider is limited by the strength of bending dipoles, and its maximum luminosity is determined by the strength of final focus quadrupoles. For this reason, the high-energy physics and accelerator communities have shown much interest in higher-field and higher-gradient superconducting accelerator magnets. The maximum field of NbTi magnets used in all present high-energy machines, including the LHC, is limited to ~10 T at 1.9 K. Fields above 10 T became possible with the use of Nb$_3$Sn superconductors. Nb$_3$Sn accelerator magnets can provide operating fields up to ~15 T and can significantly increase the coil temperature margin. Accelerator magnets with operating fields above 15 T require high-temperature superconductors. Furthermore, this review discusses the status and main results of Nb$_3$Sn accelerator magnet research and development and work toward 20-T magnets.

43 PARTICLE ACCELERATORS↗
DOE OSTI2022

Quantum Sensing and Imaging of Spin–Orbit-Torque-Driven Spin Dynamics in the Non-Collinear Antiferromagnet Mn 3 Sn

Novel non-collinear antiferromagnets with spontaneous time-reversal symmetry breaking, non-trivial band topology, and unconventional transport properties have received immense research interest over the past decade due to their rich physics and enormous promise in technological applications. One of the central focuses in this emerging field is exploring the relationship between the microscopic magnetic structure and exotic material properties. Nanoscale imaging of both spin–orbit-torque-induced deterministic magnetic switching and chiral spin rotation in non-collinear antiferromagnet Mn 3 Sn films using nitrogen-vacancy (NV) centers are reported. Direct evidence of the off-resonance dipole–dipole coupling between the spin dynamics in Mn 3 Sn and proximate NV centers is also demonstrated by NV relaxometry measurements. These results demonstrate the unique capabilities of NV centers in accessing the local information of the magnetic order and dynamics in these emergent quantum materials and suggest new opportunities for investigating the interplay between topology and magnetism in a broad range of topological magnets.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Coexisting charge and magnetic orders in the dimer-chain iridate Ba 5 AlIr 2 O 11

In this paper, we have synthesized and studied single-crystal Ba 5 AlIr 2 O 11 that features dimer chains of two inequivalent octahedra occupied by tetravalent Ir 4+ (5d 5 ) and pentavalent Ir 5+ (5d 4 ) ions, respectively. Ba 5 AlIr 2 O 11 is a Mott insulator that undergoes a subtle structural phase transition near T S =210K and a magnetic transition at T M =4.5K; the latter transition is surprisingly resistant to applied magnetic fields μ o H≤12T but more sensitive to modest applied pressure (dT M /dp ≈ +0.61K/GPa). All results indicate that the phase transition at T S signals an enhanced charge order that induces electrical dipoles and strong dielectric response near T S . It is clear that the strong covalency and spin-orbit interaction (SOI) suppress double exchange in Ir dimers and stabilize a novel magnetic state that is neither S=3/2 nor J=1/2, but rather lies in an “intermediate” regime between these two states. Finally, the novel behavior of Ba 5 AlIr 2 O 11 therefore provides unique insights into the physics of SOI along with strong covalency in competition with double-exchange interactions of comparable strength.

36 MATERIALS SCIENCE↗