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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,603 records · Page 89
All sourcesNASA NTRSDOE OSTI
DOE OSTI2014

Optically tunable spin-exchange energy at donor:acceptor interfaces in organic solar cells

Spin-exchange energy is a critical parameter in controlling spin-dependent optic, electronic, and magnetic properties in organic materials. This article reports optically tunable spin-exchange energy by studying the line-shape characteristics in magnetic field effect of photocurrent developed from intermolecular charge-transfer states based on donor:acceptor (P3HT:PCBM) system. Specifically, we divide magnetic field effect of photocurrent into hyperfine (at low field < 10 mT) and spin-exchange (at high field > 10 mT) regimes. We observe that increasing photoexcitation intensity can lead to a significant line-shape narrowing in magnetic field effect of photocurrent occurring at the spin-exchange regime. We analyze that the line-shape characteristics is essentially determined by the changing rate of magnetic field-dependent singlet/triplet ratio when a magnetic field perturbs the singlet-triplet transition through spin mixing. Based on our analysis, the line-shape narrowing results indicate that the spin-exchange energy at D:A interfaces can be optically changed by changing photoexcitation intensity through the interactions between intermolecular charge-transfer states. Therefore, our experimental results demonstrate an optical approach to change the spin-exchange energy through the interactions between intermolecular charge-transfer states at donor:acceptor interface in organic materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Plasma acceleration using a radio frequency self-bias effect

In this work plasma acceleration using a RF self-bias effect is experimentally studied. The experiments are conducted using a novel plasma accelerator system, called Neptune, consisting of an inductively coupled plasma source and a RF-biased set of grids. The plasma accelerator can operate in a steady state mode, producing a plasma flow with separately controlled plasma flux and velocity without any magnetic configuration. The operating pressure at the source output is as low as 0.2 mTorr and can further be decreased. The ion and electron flows are investigated by measuring the ion and electron energy distribution functions both space resolved and with different orientations with respect to the flow direction. It is found that the flow of electrons from the source is highly anisotropic and directed along the ion flow and this global flow of accelerated plasma is well localized in the plasma transport chamber. The maximum flux is about 7.5·10{sup 15} ions s{sup −1} m{sup −2} (at standard conditions) on the axis and decreasing to almost zero at a radial distances of more than 15 cm from the flow axis. Varying the RF acceleration voltage in the range 20–350 V, the plasma flow velocity can be changed between 10 and 35 km/s. The system is prospective for different technology such as space propulsion and surface modification and also interesting for fundamental studies for space-related plasma simulations and investigation of the dynamo effect using accelerated rotating plasmas.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

A graphene edge-mediated quantum gate

We propose a quantum gate architecture that allows for the systematic control of the effective exchange interactions between magnetic impurities embedded in nanoscale graphene flakes connected by a gated bridge. The entanglement between the magnetic moment and the edge states of the fragments is used to electrostatically tune the exchange interaction from ferro to antiferromagnetic by merely changing the bridge's carrier density. By characterizing the effects of size and coupling parameters, we explore different operation regimes of this device by means of exact calculations with the density matrix renormalization group. We analyze the results utilizing a simplified model that accounts for the main many-body mechanisms. Finally, we discuss how to use arrays of these devices to build quantum simulators for quantum many-body Hamiltonians.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Ligand field exciton annihilation in bulk CrCl 3

The layered van der Waals material CrCl 3 exhibits very strongly bound ligand field excitons that control optoelectronic applications and are connected with magnetic ordering by virtue of their d-orbital origin. Time-resolved photoluminescence of these exciton populations at room temperature shows that their relaxation is dominated by exciton–exciton annihilation and that the spontaneous decay lifetime is very long. Furthermore, these observations allow the rough quantification of the exciton annihilation rate constant and contextualization in light of a recent theory of universal scaling behavior of the annihilation process.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Microwave-photonic control of optically accessible spin defects in diamond

A growing variety of optically accessible spin qubits have emerged in recent years as key components for quantum sensors, computers, and memories. However, the scalability of conventional spin-based quantum architectures remains limited by direct microwave delivery, which introduces thermal noise, electromagnetic crosstalk, and design constraints for cryogenic, high-field, and distributed systems. In this work, we present a unified framework for RF-over-fiber (RFoF) control of spins accessible through optically detected magnetic resonance (ODMR) spectroscopy of nitrogen-vacancy (NV) centers in diamond. The RFoF platform relies on an intensity-modulated 1310 nm laser carrying microwave signals over fiber and a high-speed photodiode for optical-to-electrical conversion to drive NV spin transitions. We report an RFoF power-conversion efficiency of 3.42% for an RF output PRF,out=-5.5 dBm at 2.87 GHz, enabling clear resolution of Zeeman splitting in

Rahman, M Reefaz [ORNL] (ORCID:0000000323541611)↗
DOE OSTI2016

Access to edge scenarios for testing a scraper element in early operation phases of Wendelstein 7-X

The edge topology of magnetic fusion devices is decisive for the control of the plasma exhaust. In Wendelstein 7-X, the island divertor concept will be used, for which the edge topology can change significantly as the internal currents in a plasma discharge evolve towards steady-state. Consequently, the device has been optimized to minimize such internal currents, in particular the bootstrap current [1]. Nonetheless, there are predicted pulse scenarios where effects of the remaining internal currents could potentially lead to overload of plasma-facing components. These internal currents are predicted to evolve on long time scales (tens of seconds) so their effects on the edge topology and the divertor heat loads may not be experimentally accessible in the first years of W7-X operation, where only relatively short pulses are possible. However, we show here that for at least one important long-pulse divertor operation issue, relevant physics experiments can be performed already in short-pulse operation, through judicious adjustment of the edge topology by the use of the existing coil sets. The specific issue studied here is a potential overload of the divertor element edges. This overload might be mitigated by the installation of an extra set of plasma-facing components, so-called scraper elements, as suggested in earlier publications. It is shown here that by a targeted control of edge topology, the effectiveness of such scraper elements can be tested already with uncooled test-scraper elements in short-pulse operation. Furthermore, this will allow an early and well-informed decision on whether long-pulse-capable (actively cooled) scraper elements should be built and installed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Characterizing the plasma-induced thermal loads on a 200 kW light-ion helicon plasma source via infra-red thermography

The light-ion helicon plasma source of the Proto-MPEX linear plasma device has been recently upgraded to enable pulsed (0.5–1 s) operation up to 200 kW. The main objective of this work is to report on the plasma-induced surface heat fluxes incident on the helicon window during high power operation (60–150 kW net power) for the purpose of the design of the upcoming material plasma exposure eXperiment (MPEX). The IR imaging system and associated physics models for the extraction of surface heat fluxes are presented. Furthermore, experimental results demonstrate that the control of the plasma strike point via magnetic flux mapping and the use of dedicated limiters is effective at reducing the heat loads on the dielectric window. Moreover, it is found that the flux mapping must create a gap between the plasma and the dielectric window of at least the plasma radial decay length. Extrapolated to 200 kW net RF power, this mode of operation can reduce the power lost to the dielectric window by 33%. The results presented have direct application to the design of high-powered helicon plasma sources that operate in a steady state. Examples include linear divertor simulators such as MPEX, electric thrusters, negative ion sources for NBI and linear plasma–material interaction test stands.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2017

Impurity screening behavior of the high-field side scrape-off layer in near-double-null configurations: prospect for mitigating plasma–material interactions on RF actuators and first-wall components

The impurity screening response of the high-field side (HFS) scrape-off layer (SOL) to localized nitrogen injection is investigated on Alcator C-Mod for magnetic equilibria spanning lower-single-null, double-null and upper-single-null configurations under otherwise identical plasma conditions. L-mode, EDA H-mode and I-mode discharges are investigated. HFS impurity screening is found to depend on magnetic flux balance and the direction of B × $\nabla$B relative to the most active divertor. Impurity 'plume' emission patterns indicate that both parallel and perpendicular (E × B) flows in the SOL contribute to the 'flushing' of impurities towards the active divertor, thereby affecting the overall impurity screening behavior. Despite the fact that the HFS SOL is extremely narrow in near-double-null configurations, this SOL is able to screen locally injected nitrogen at least as effectively as the low-field side (LFS) SOL—up to a factor of 10 more effective, depending on specific plasma conditions and whether the magnetic geometry produces parallel flows that work with or against E × B flows. For situations in which the E × B drift of the impurity ions opposes parallel flow toward the primary divertor, HFS impurity screening is found to be least effective. When E × B drifts assist parallel flow toward the primary divertor, HFS impurity screening is found to be very effective. These data support the idea of placing RF actuators and close-fitting wall components on the HFS of the tokamak. Finally, with this configuration, near-double-null magnetic topologies may be used for active control of plasma parameters at the antenna/plasma interface for optimal RF coupling, mitigate the generation of local impurities from plasma–material interactions and, taking advantage of favorable plasma flows and good screening properties of the HFS SOL, further minimize the impact of wall-born impurity sources on the plasma core.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Ultra-fast transverse beam orbit control in LCLS copper linac. Part I

We report current and future experiments at LCLS require x-ray pulse trains of variable time separation on the nanosecond scale. For instance, the cavity-based XFEL (CBXFEL) will use up to 4 pulses separated by 218.5 ns, the X-ray Laser Oscillator (XLO) will use 15 to 25 ns spaced pulses, and the Matter under Extreme Conditions (MEC) experiments use pulse trains separated by 5 nanoseconds or less. In this paper, we demonstrate an ultra-fast e-beam trajectory control method based on transverse electro-magnetic (TEM) striplines and state-of-the-art power sources, to enhance LCLS operations in these regimes.

47 OTHER INSTRUMENTATION↗
DOE OSTI2019

Bias current dependence of superconducting transition temperature in superconducting spin-valve nanowires

Competition between superconducting and ferromagnetic ordering at interfaces between ferromagnets (F) and superconductors (S) gives rise to several proximity effects such as odd-triplet superconductivity and spin-polarized supercurrents. A prominent example of an S/F proximity effect is the spin switch effect (SSE) observed in S/F/N/F superconducting spin-valve multilayers, in which the superconducting transition temperature T c is controlled by the angle $\phi$ between the magnetic moments of the F layers separated by a nonmagnetic metallic spacer N. Here we present an experimental study of SSE in Nb/Co/Cu/Co/CoO x nanowires measured as a function of bias current flowing in the plane of the layers. In this work, these measurements reveal an unexpected dependence of T c ($\phi$) on the bias current: T c (π)–T c (0) changes sign with increasing current bias. We attribute the origin of this bias dependence of the SSE to a spin Hall current flowing perpendicular to the plane of the multilayer, which suppresses T c of the multilayer. The bias dependence of SSE can be important for hybrid F/S devices such as those used in cryogenic memory for superconducting computers as device dimensions are scaled down to the nanometer length scale.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Streamer self-focusing in an external longitudinal magnetic field

The numerical simulation of the development of a streamer discharge in a gap with an external longitudinal magnetic field was used to demonstrate the self-focusing of such discharges. Self-focusing is caused by a sharp deceleration of the radial ionization wave due to a change in the electron energy distribution function, a decrease in the average electron energy, the rate of gas ionization, and the electron mobility in crossed electric and magnetic fields as compared to the case of the discharge development without a magnetic field. The self-focusing effect of a streamer discharge in an external longitudinal magnetic field is observed for both positive and negative pulse polarities. The work proposes an estimate of the critical value of the magnetic field, which makes it possible to control the development of pulsed high-voltage discharges at various gas pressures.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Instability and evolution of the magnetic ground state in metallic perovskites GdRh 3 C 1-x B x

In this paper, we report investigations of the structural, magnetic, electrical transport and thermal properties of five compositions of the metallic perovskite GdRh 3 C 1–x B x (0.00 ≤ x ≤ 1.00). Our results show that all the five compositions undergo magnetic ordering at low temperatures, but the nature of the ordered state is significantly different in the carbon- and the boron-rich compositions, where the former shows signatures of an amplitude-modulated magnetic structure and the latter exhibits evidences of an equal-moment incommensurate antiferromagnetic ordering. We also observe a remarkable field-dependent evolution of conduction carrier polarization in the compositionally disordered compounds. The outcomes indicate that this system is energetically situated in proximity to a magnetic instability where small variations in the control parameter(s), such as lattice constant and/or electron density, lead to considerably different ground states.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Single-Shot Readout and Weak Measurement of a Tin-Vacancy Qubit in Diamond

The negatively charged tin-vacancy center in diamond (SnV − ) is an emerging platform for building the next generation of long-distance quantum networks. This is due to the SnV − ’s favorable optical and spin properties including bright emission, insensitivity to electronic noise, and long spin coherence times at temperatures above 1 K. Here, we demonstrate measurement of a single SnV − electronic spin with a single-shot readout fidelity of 87.4%, which can be further improved to 98.5% by conditioning on multiple readouts. In the process, we develop understanding of the relationship between strain, magnetic field, spin readout, and microwave spin control. We show that high-fidelity readout is compatible with rapid microwave spin control, demonstrating a favorable parameter regime for use of the SnV − center as a high-quality spin-photon interface. Finally, we use weak quantum measurement to study measurement-induced dephasing; this illuminates the fundamental interplay between measurement and decoherence in quantum mechanics, and provides a universal method to characterize the efficiency of color-center spin readout. Taken together, these results overcome an important hurdle in the development of the SnV − -based quantum technologies and, in the process, develop techniques and understanding broadly applicable to the study of solid-state quantum emitters.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Landau-phonon polaritons in Dirac heterostructures

Polaritons are light-matter quasiparticles that govern the optical response of quantum materials at the nanoscale, enabling on-chip communication and local sensing. Here, we report Landau-phonon polaritons (LPPs) in magnetized charge-neutral graphene encapsulated in hexagonal boron nitride (hBN). These quasiparticles emerge from the interaction of Dirac magnetoexciton modes in graphene with the hyperbolic phonon polariton modes in hBN. Using infrared magneto-nanoscopy, we reveal the ability to completely halt the LPP propagation in real space at quantized magnetic fields, defying the conventional optical selection rules. The LPP-based nanoscopy also tells apart two fundamental many-body phenomena: the Fermi velocity renormalization and field-dependent magnetoexciton binding energies. Our results highlight the potential of magnetically tuned Dirac heterostructures for precise nanoscale control and sensing of light-matter interaction.

36 MATERIALS SCIENCE↗
DOE OSTI2017

On the longitudinal distribution of electric field in the acceleration zones of plasma accelerators and thrusters with closed electron drift

The long-term experience in controlling the electric field distribution in the discharge gaps of plasma accelerators and thrusters with closed electron drift and the key ideas determining the concepts of these devices and tendencies of their development are analyzed. It is shown that an electrostatic mechanism of ion acceleration in plasma by an uncompensated space charge of the cloud of magnetized electrons “kept” to the magnetic field takes place in the acceleration zones and that the electric field distribution can be controlled by varying the magnetic field in the discharge gap. The role played by the space charge makes the mechanism of ion acceleration in this type of thrusters is fundamentally different from the acceleration mechanism operating in purely electrostatic thrusters.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2018

National Spherical Torus Experiment Upgrade Collaborative Research on Configuration Optimization of Advanced Operating Scenarios and Control Including Macroscopy Stability EOG for Period 3/1/14 through 2/28/18

General Atomics has collaborated with PPPL since 1999 in support of NSTX and NSXT-U by leveraging DIII-D program expertise. John Ferron was the principal investigator (PI) for the first nine years (to 2008) and Rob La Haye since then. The research effort evolved over a number of three-year grants and originally included both the core (control, stability, resonant error fields) and the boundary (ELMs, divertor, error fields). In 2014 the current and last grant extension was stretched to four years and split into a core grant (advanced scenarios and control, macroscopic plasma stability and extending 3D magnetics diagnostics) and a boundary grant. Todd Evans is the PI for the new boundary grant which while also for four years expires later than the core grant; a separate end of grant (EOG) report for that is due in July 2018.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2018

Final Report : Experiments and Theory on Nonlinear Wave Couplings and the Saltpeter Screening Effect

This Final Technical Report gives a brief overview of the apparatus upgrades, experimental results, and theory development which was funded by DOE grant DE-SC0008693 from 1-Aug-2012 to 31-Jul-2018. Experiments were performed on the "IV" apparatus, which contains un-neutralized Mg+ ion plasmas in a 3.Tesla magnetic field, with sophisticated laser diagnostics and control. The apparatus upgrade utilized a 4-channel absolute WaveMeter, with feedback control to stabilize the laser frequencies, enabling ultra-cold, highly-correlated plasma states. The Saltpeter enhancement of collisionality due to plasma correlations was verified experimentally, ruling out competing "dynamical screening" theories. This represents the only quantitative experimental tests of the Saltpeter enhancement, which is incorporated into all models of stellar nucleosynthesis. In closely related work, quantitative measurements of cyclotron modes for majority and minority ion species were obtained, verifying the theoretically-predicted dependence on the plasma electric field. Substantial experimental and theoretical work was devoted to understanding the (parametric) decay of large-amplitude plasma waves into longer-wavelength plasma waves. Here, there are simple "fluid theory" predictions, but the experimentally observed (dominant) process depends on subtle "kinetic" effects due to particles trapped in the wave-fields. The theory of this novel instability was augmented by several types of simulations, which are in broad agreement with the experiments. This research formed the basis for two Ph.D. theses, and also included undergraduate trainees. A list of journal publications is provided, in which the detailed scientific results are described.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Characterization and Damping Control of Mechanical Connections to Improve Performance of Horn Stripline

Magnetic focusing horns are critical components for creating a stable beam of neutrinos for neutrino facilities, such as the Long Baseline Neutrino Facility (LBNF) and the Neutrinos and Main Injector (NuMI) beam lines at Fermilab. The pulsed magnetic horns are powered by high current electricity through long striplines, which must survive in a harsh radiation environment for the operational life of the component. Each stripline assembly consists of four layers of Al 6101-T6. As an electro-mechanical system, the stripline layers are bolted together with ceramic isolators for electrical insulation and to facilitate passive cooling and mechanical stability. The striplines experience vibrational force in addition to clamping force, repetitive thermal and electro-magnetic loading. The holes of stripline plates for ceramic joints represent one of the weak links for potential failure. Damping can be achieved by adding damp material to the joint. By characterizing behavior of the joint and optimizing their damping properties through FEA and EMA, the stripline performance and longevity can be improved. Appropriate damp materials are the key.

Liu, Zunping [Fermilab]↗