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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,603 records · Page 89
All sourcesNASA NTRSDOE OSTI
DOE OSTI2014

Requirements Document for the Redesign of the DIM-based Diagnostics Transport and Handling System at the National Ignition Facility (NIF)

The National Ignition Facility (NIF, Figure 1) is the world’s leading user research facility for inertial confinement fusion. Diagnostic instruments that collect data from the experiment shots are transported around the facility using a series of disjointed, suboptimal transport and handling (T&H) subsystems that compromise user efficiency and ergonomics. Significant time savings and improvements to the diagnostic exchange process could be realized by designing a new transport and handling system that minimizes the hand-offs between T&H subsystems, reduces operator hassle and ergonomic strain, and improves the long-term maintainability of the system. In contrast to the current system – which employs several manually-operated carts and containers to transport the diagnostic, dock it to its destination, and install it – the new diagnostic transporter integrates the contamination container with the transport cart and provides a dynamic range of adjustability to interface with its destination. This single transporter has the requisite maneuverability, height adjustability, and fine adjustment capabilities without any rigging transactions to support contaminated diagnostic transport and handling at the alignment station and Equatorial and Polar DIMs. A remote-controlled user interface device allows operators a more hands-off experience that reduces ergonomic strain and improves safety. Assuming the cost is not prohibitive, diagnostic storage will be accomplished by simply stowing the transporter in its lowest position in the designated area of NIF. This concept for a new diagnostic transport and handling system would be better aligned with the core values of NIF: safety, quality, and reliability.

42 ENGINEERING↗
DOE OSTI2024

Excited-State and Nonadiabatic Molecular Dynamics Methods with Broad Applicability

Electronically excited states play a pivotal role in the capture, transformation, storage, and emission of radiative energy. Despite much recent progress for small model systems, excited state properties and dynamics in many larger molecular devices and materials have remained elusive for experiment and theory. Nonadiabatic transitions between electronic states turn radiative energy into heat and are particularly difficult to control. This project aims to develop new electronic structure and nonadiabatic molecular dynamics (NAMD) methods to simulate, predict, and ultimately control the flow and transformation of excitation energy in a wide-range of light-driven molecular devices such as dyes, photocatalysts, and fluorescence emitters.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

The Roadrunner Trap: A QSCOUT Device

The Roadrunner ion trap is a micro-fabricated surface-electrode ion trap based on silicon technology. This trap has one long linear section and a junction to allow for chain storage and reconfiguration. It uses a symmetric rf-rail design with segmented inner and outer control electrodes and independent control in the junction arms. The trap is fabricated on Sandia’s High Optical Access (HOA) platform to provide good optical access for tightly focused laser beams skimming the trap surface. It is packaged on our custom Bowtie-102 ceramic pin or land grid array packages using a 2.54 mm pitch for backside pins or pads. This trap also includes an rf sensing capacitive divider and tungsten wires for heating or temperature monitoring. The Roadrunner builds on the knowledge gained from previous surface traps fabricated at Sandia while improving ion control capabilities.

42 ENGINEERING↗
DOE OSTI2017

Conformal construction of polyaniline shell on cobalt oxide nanoflake core for enhanced Li ion storage

Highlights: • Construct non-axial polyaniline shell on Co{sub 3}O{sub 4} nanoflake core. • Non-axial core/shell arrays show enhanced Li storage properties. • Ultrathin PANI shell is favorable for fast ion and electron transfer. - Abstract: It is of great importance to controllably synthesize non-axial metal oxide/conducting polymers arrays for construction of high-performance electrochemical devices. In this work, we develop a facile electro-polymerization method to conformally coat interwoven polyaniline (PANI) shell on the preformed porous Co{sub 3}O{sub 4} nanoflakes forming non-axial Co{sub 3}O{sub 4}/PANI core/shell arrays. Uniform conductive PANI network and high porosity are realized in the non-axial core/shell arrays. As active materials for Li ion storage, the Co{sub 3}O{sub 4}/PANI core/shell arrays show superior high-rate performance including lower polarization, higher reactivity and better cycling life, as compared to the unmodified Co{sub 3}O{sub 4} nanoflake arrays. The capacity deterioration of the Co{sub 3}O{sub 4}/PANI arrays is restricted to a very lower level with a capacity of 871 mAh g{sup −1} at 0.25 A g{sup −1} after 100 cycles, better than the Co{sub 3}O{sub 4} counterpart (669 mAh g{sup −1} at 0.25 A g{sup −1}). This non-axial combination opens up a new door for developing advanced composite arrays for energy storage.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Electrochemical ion insertion from the atomic to the device scale

Electrochemical ion insertion involves coupled ion–electron transfer reactions, transport of guest species and redox of the host. The hosts are typically anisotropic solids with 2D conduction planes but can also be materials with 1D or isotropic transport pathways. These insertion compounds have traditionally been studied in the context of energy storage but also find extensive applications in electrocatalysis, optoelectronics and computing. Recent developments in operando, ultrafast and high-resolution characterization methods, as well as accurate theoretical simulation methods, have led to a renaissance in the understanding of ion-insertion compounds. In this Review, we present a unified framework for understanding insertion compounds across timescales and length scales ranging from atomic to device levels. Using graphite, transition metal dichalcogenides, layered oxides, oxyhydroxides and olivines as examples, we explore commonalities in these materials in terms of point defects, interfacial reactions and phase transformations. We illustrate similarities in the operating principles of various ion-insertion devices, ranging from batteries and electrocatalysts to electrochromics and thermal transistors, with the goal of unifying research across disciplinary boundaries.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Envisioning the Future Renewable and Resilient Energy Grids—A Power Grid Revolution Enabled by Renewables, Energy Storage, and Energy Electronics

Today’s power grids are facing tremendous challenges because of the ever-increasing power demand, system complexity, infrastructure cost, knowledge base, and policy and regulatory issues to achieve supply–demand power balance and resiliency with respect to more frequent extreme weather events and cyberattacks. It is particularly challenging when the transition toward 100% intermittent renewable energy sources is considered. Many countries are calling for building up more transmission and distribution lines to increase power delivery capacities. This article is an attempt to answer two urgent questions: Is more transmission and distribution infrastructure really needed to meet the increasing power demand? What kind of future grid infrastructure should we envision and build? This article attempts to answer these questions and proposes the concept of community-centric asynchronous renewable and resilient energy grids. By clearly differentiating the concepts of grid resilience and reliability, the importance of building resilient power electronics’ devices and robust system-level control algorithms to achieve 100% renewable energy integrated resilient grids is presented. To identify the shortcomings and propose advancements, power electronics’ technologies are categorized using the proposed concepts of natural source frequencies (NSf), energy storage, direct energy conversion/control and fault protection (DeCaFp), and high-efficiency energy consumption and buffering (heECaB) technology. The ability of networked microgrids to greatly reduce power outages and power system restoration time is demonstrated by leveraging robust decentralized and centralized control algorithms, identified through a comprehensive literature review. Future research areas are proposed to further enhance grid stability, controllability, cybersecurity, and protection against faults in the presence of 100% renewable sources by leveraging the advanced capabilities of NSf, DeCaFp, and heECaB devices and system-level control algorithms.

14 SOLAR ENERGY↗
DOE OSTI2014

Charging Graphene for Energy Storage

Since 2004, graphene, including single atomic layer graphite sheet, and chemically derived graphene sheets, has captured the imagination of researchers for energy storage because of the extremely high surface area (2630 m2/g) compared to traditional activated carbon (typically below 1500 m2/g), excellent electrical conductivity, high mechanical strength, and potential for low cost manufacturing. These properties are very desirable for achieving high activity, high capacity and energy density, and fast charge and discharge. Chemically derived graphene sheets are prepared by oxidation and reduction of graphite1 and are more suitable for energy storage because they can be made in large quantities. They still contain multiply stacked graphene sheets, structural defects such as vacancies, and oxygen containing functional groups. In the literature they are also called reduced graphene oxide, or functionalized graphene sheets, but in this article they are all referred to as graphene for easy of discussion. Two important applications, batteries and electrochemical capacitors, have been widely investigated. In a battery material, the redox reaction occurs at a constant potential (voltage) and the energy is stored in the bulk. Therefore, the energy density is high (more than 100 Wh/kg), but it is difficult to rapidly charge or discharge (low power, less than 1 kW/kg)2. In an electrochemical capacitor (also called supercapacitors or ultracapacitor in the literature), the energy is stored as absorbed ionic species at the interface between the high surface area carbon and the electrolyte, and the potential is a continuous function of the state-of-charge. The charge and discharge can happen rapidly (high power, up to 10 kW/kg) but the energy density is low, less than 10 Wh/kg2. A device that can have both high energy and high power would be ideal.

energy density↗
DOE OSTI2025

200 h of discharge cycling with an all-aqueous copper thermally regenerative ammonia battery

Thermally regenerative ammonia batteries (TRABs) offer an approach to energy storage and electricity generation by harnessing low-grade heat (T < 150 °C). A TRAB discharge resembles that of a flow battery, where electrochemical reactions produce electrical power from energy stored within aqueous electrolytes. While there are many types of TRABs, the all-aqueous copper TRAB (Cu aq -TRAB) has produced the largest power and energy storage densities. Despite many improvements to TRAB performance, most tests have only lasted a few hours, which are not representative of operation times expected of these devices. Herein, we operated a Cu aq -TRAB for 200 h of constant current discharging to assess battery performance and component stability. After 200 h of testing, the average power density increased slightly to 7.2 mW cm -2 , which was within 0.01 % of starting conditions. Likewise, the average energy density for the final cycle was only 0.03 % lower than the initial cycle. The overall insensitivity of the power cell to cycling represents a major milestone in the advancement of TRAB systems. In conclusion, energy dispersive X-ray spectroscopy provides evidence to suggest that these small changes in power and energy density are likely to the membrane acclimating to TRAB electrolytes.

25 ENERGY STORAGE↗
DOE OSTI2013

Innovative Application of Maintenance-Free Phase-Change Thermal Energy Storage for Dish-Engine Solar Power Generation

This final report summarizes the final results of the Phase II Innovative Application of Maintenance-Free Phase-Change Thermal Energy Storage for Dish-Engine Solar Power Generation project being performed by Infinia Corporation for the U.S. Department of Energy under contract DE-FC36-08GO18157 during the project period of September 1, 2009 - August 30, 2012. The primary objective of this project is to demonstrate the practicality of integrating thermal energy storage (TES) modules, using a suitable thermal salt phase-change material (PCM) as its medium, with a dish/Stirling engine; enabling the system to operate during cloud transients and to provide dispatchable power for 4 to 6 hours after sunset. A laboratory prototype designed to provide 3 kW-h of net electrical output was constructed and tested at Infinia's Ogden Headquarters. In the course of the testing, it was determined that the system's heat pipe network - used to transfer incoming heat from the solar receiver to both the Stirling generator heater head and to the phase change salt - did not perform to expectations. The heat pipes had limited capacity to deliver sufficient heat energy to the generator and salt mass while in a charging mode, which was highly dependent on the orientation of the device (vertical versus horizontal). In addition, the TES system was only able to extract about 30 to 40% of the expected amount of energy from the phase change salt once it was fully molten. However, the use of heat pipes to transfer heat energy to and from a thermal energy storage medium is a key technical innovation, and the project team feels that the limitations of the current device could be greatly improved with further development. A detailed study of manufacturing costs using the prototype TES module as a basis indicates that meeting DOE LCOE goals with this hardware requires significant efforts. Improvement can be made by implementing aggressive cost-down initiatives in design and materials, improving system performance by boosting efficiencies, and by refining cost estimates with vendor quotes in lieu of mass-based approaches. Although the prototype did not fully demonstrate performance and realize projected cost targets, the project team believes that these challenges can be overcome. The test data showed that the performance can be significantly improved by refining the heat pipe designs. However, the project objective for phase 3 is to design and test on sun the field ready systems, the project team feels that is necessary to further refine the prototype heat pipe design in the current prototype TES system before move on to field test units, Phase 3 continuation will not be pursued.

14 SOLAR ENERGY↗
DOE OSTI2022

Opportunities and Challenges in Passive Thermal-Fluid and Energy Systems

Abstract This article focuses on passive systems that are used in energy and thermal-fluid applications. These passive systems do not have moving parts and are reliable and cost-effective. Fluid motion in these passive devices could be driven by capillary force, gravity, osmotic pressure, and/or concentration gradient. The fundamental mechanisms and limitations of transport phenomena for passive systems are highlighted, followed by their applications in heat pipes, fuel cells, thermal energy storage, and desalination systems. The capabilities of the passive systems are limited by the balance between the driving force and transport resistance. Based on the fundamental understanding of fluid flow and phase change in passive systems, this study proposes associated transport phenomena and quantitative criteria to determine the maximum heat transfer rate, the transport distance, and minimum pore size of wick structures (when relevant) in these passive devices. This article concludes with the discussion of challenges and future opportunities of passive systems.

Engineering↗
DOE OSTI2024

A Pseudo Planar Heterojunction Structure for Eco‐Friendly Printable Organic Solar Cells Achieving 19.05% Efficiency

Abstract Obtaining a well‐accurate vertical distribution active layer morphology through the air‐printing process is an essential task for achieving efficient scalable large‐area organic solar cells (OSCs). In this target, the desired and controllable pseudo planar heterojunction (PPHJ) active layer structure with suitable phase separation is developed by pre‐deposited D18‐Cl layer under the PM6:BTP‐eC9 film via an eco‐friendly manufacturing method. The addition of the D18‐Cl regulates molecular crystallization and leads to an ideal vertical stratification while simultaneously suppressing voltage loss, optimizing energetic disorder, and carrier management. Impressively, the optimal PPHJ devices perform superior power conversion efficiencies (PCEs) of 19.05% (100 nm), 17.33% (300 nm), and 14.14% (4 cm 2 ) compared to the BHJ devices. Importantly, the PPHJ OSCs also exhibit an impressive extrapolated T 80 (the time required to reach 80% of initial PCE) of long‐time storage and operational stability, as well as thermal stability.

Chemistry↗
DOE OSTI2016

Direct observation of localized radial oxygen migration in functioning tantalum oxide memristors

Oxygen migration in tantalum oxide, a promising next-generation storage material, is studied using in operando x-ray absorption spectromicroscopy and is used to microphysically describe accelerated evolution of conduction channel and device failure. Furthermore, the resulting ring-like patterns of oxygen concentration are modeled using thermophoretic forces and Fick diffusion, establishing the critical role of temperature-activated oxygen migration that has been under question lately.

36 MATERIALS SCIENCE↗
DOE OSTI2016

Thin insulating tunneling contacts for efficient and water-resistant perovskite solar cells

Here, we demonstrated that inserting a tunneling layer between perovskite and electron transport layer could significantly increase device performance by suppressing carrier recombination at the cathode contact. The tunneling layer can also serve as an encapsulation layer to prevent perovskite film from damage caused by water or moisture. This method is simple because it does not need lattice matching between the buffer layer and perovskite. The low temperature solution process makes it compatible with many types of perovskite materials, and may be applied for anode contact as well. The freedom to choose any insulating layer for contact enables more device designs and manufacturing.

25 ENERGY STORAGE↗
DOE OSTI2020

Removal of Na + and Ca2 + with Prussian blue analogue electrodes for brackish water desalination

Desalination of brackish water sources is critical to addressing the growing global freshwater demand. One promising approach is electrically driven desalination using intercalation electrodes. While intercalation electrodes have been widely researched for energy storage applications, only a small subset of those materials is suitable for desalination. In this work, we report the synthesis, characterization, and in-device testing of three Prussian blue analogue intercalation compounds: copper, manganese, and zinc hexacyanoferrate with formulas K x M[Fe(CN) 6 ] z ·nH 2 O (M = Cu, Mn, Zn). The desalination performance for each of these materials against carbon electrodes is reported for Na + intercalation and for Ca 2+ intercalation using 1000 ppm NaCl and 1000 ppm CaCl 2 feed solutions, respectively. While the copper and manganese analogs showed promising performance for Na + and Ca 2+ intercalation, the zinc compound was unstable and underwent rapid dissolution. Manganese hexacyanoferrate showed the best desalination performance in terms of salt removal capacities and salt removal rates with NaCl while copper hexacyanoferrate performed the best with CaCl 2 . The manganese analog proved to be the most stable intercalation material, retaining 83% and 72% of its salt removal capacity after 280 cycles in NaCl and CaCl 2 feed solutions respectively.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Tailoring electric dipole of hole-transporting material p-dopants for perovskite solar cells

We report Li-TFSI/t-BP are the most widely employed p-dopants for hole-transporting materials (HTMs) within the state-of-the-art perovskite solar cells (PSCs). The hygroscopicity and migration of these dopants, however, lead to devices with limited stability. To solve this problem, we report here on a diphenyl iodide cation and pentafluorophenyl boric acid anion-based dopant (DIC-PBA) with an oriented interfacial dipole moment as an alternative to Li-TFSI/t-BP. Theoretical and experimental data reveal that DIC-PBA exhibits deep doping of poly[bis(4-phenyl)(2,4,6-triMethylphenyl)aMine] (PTAA) and also creates p-doping of perovskite surface, which originates from ionic interactions-derived dipole arrangement that yields fast interfacial charge transport. The improved intrinsic stability of PSCs originates from the inhibition of dipole moment degeneration on the perovskite surface. Devices prepared with DIC-PBA yielded high efficiency of 22.86%, and the modules (aperture area: 33.2 cm 2 ) efficiency reached 19.13%. Importantly, the storage stability also significantly improved exceeding to 90% after aging 1,200 h under air ambient.

14 SOLAR ENERGY↗
DOE OSTI2019

Targeting GPUs with OpenMP directives on Summit: A simple and effective Fortran experience

We use OpenMP to target hardware accelerators (GPUs) on Summit, a newly deployed supercomputer at the Oak Ridge Leadership Computing Facility (OLCF), demonstrating simplified access to GPU devices for users of our astrophysics code GenASiS and useful speedup on a sample fluid dynamics problem. We modify our workhorse class for data storage to include members and methods that significantly streamline the persistent allocation of and association to GPU memory. Users offload computational kernels with OpenMP target directives that are rather similar to constructs already familiar from multi-core parallelization. In this initial example we ask, “With a given number of Summit nodes, how fast can we compute with and without GPUs?”, and find total wall time speedups of ~ 12X. We also find reasonable weak scaling up to 8000 GPUs (1334 Summit nodes). We make available the source code from this work at https://github.com/GenASiS/GenASiS_Basics.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2022

Wavefront Preservation in Soft X-Ray Beamlines for the Advanced Light Source Upgrade

In the 4th generation of X-ray light sources, including Free-Electron Lasers (FEL) and Diffraction-Limited Storage Rings (DLSR), the emittance of the electron beam is small or negligible compared to the emittance of the photon beam produced by insertion devices, thus generating coherent beams of light. Over the next few years, several lightsource facilities will be built or upgraded to produce X-ray beams of unprecedented coherent flux. Delivering these exceptional beams to the sample chambers requires beamline optical systems that are designed to preserve the wavefront properties. Our goal in the Advanced Light Source upgrade project (ALS-U) is to create a new class of beamlines that reach diffraction-limited X-ray optical quality through tightly integrated, efficient optical systems, diagnostics, and adaptive mirrors, thus providing users with new scientific capabilities offered by coherent X-ray light interactions with matter. Herein we describe aspects of the beamlines’ design as they enter the project’s final design phase.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2018

Chameleon: An Adaptive Wear Balancer for Flash Clusters

NAND flash-based Solid State Devices (SSDs) offer the desirable features of high performance, energy efficiency, and fast growing capacity. Thus, the use of SSDs is increasing in distributed storage systems. A key obstacle in this context is that the natural unbalance in distributed I/O workloads can result in wear imbalance across the SSDs in a distributed setting. This, in turn can have significant impact on the reliability, performance, and lifetime of the storage deployment. Extant load balancers for storage systems do not consider SSD wear imbalance when placing data, as the main design goal of such balancers is to extract higher performance. Consequently, data migration is the only common technique for tackling wear imbalance, where existing data is moved from highly loaded servers to the least loaded ones. In this paper, we explore an innovative holistic approach, Chameleon, that employs data redundancy techniques such as replication and erasure-coding, coupled with endurance-aware write offloading, to mitigate wear level imbalance in distributed SSD-based storage. Chameleon aims to balance the wear among different flash servers while meeting desirable objectives of: extending life of flash servers; improving I/O performance; and avoiding bottlenecks. Evaluation with a 50 node SSD cluster shows that Chameleon reduces the wear distribution deviation by 81% while improving the write performance by up to 33%.

Zhao, Nannan↗