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At least 163 records · Page 9

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DOE OSTI2024

Abstract for CRADA between Capture6 CORP and NETL

The National Energy Technology Laboratory (NETL) and Capture6 CORP (Participant) will collaborate to refine Capture6’s transformative air contactor design for optimal direct air capture (DAC) under an awarded project from the Department of Energy’s Direct Air Capture Pre-Commercialization Technology Prize. Current cooling tower designs require exponentially more resources as the concentration of CO 2 in the gas phase decreases, resulting in a low conversion rate of carbonates, a large physical footprint, and high evaporation of water, which consequently limits the energy and water benefits that a DAC process can create. Capture6’s innovative tower design AURA (Absorption Unit Reactor for Ambient air) seeks to improve the mass transfer characteristics of legacy cooling towers and reduces total energy demand by: (1) introducing laminar and turbulent flow to increase mass transfer, (2) generating a solvent gradient to improve CO 2 absorption, (3) leveraging venturi and packed towers to increase the surface for the mass-transfer process, (4) adding charged/cool plates to reduce overall water loss in the system, and (5) utilizing surfactant additives to increase mass transfer. The collaboration will facilitate the deployment of technologies that reduce the total energy required and carbon footprint of solvent-based carbon dioxide removal (CDR) technologies. The anticipated results support NETL’s goal of fostering rapid development and commercialization pathways for technologies that remove CO 2 from the atmosphere.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

DOE OSTI2024

Preliminary Screening of Features, Events, and Processes for an Arctic-Focused Climate Intervention Performance Assessment

Geoengineering, the deliberate large-scale intervention in Earth's climate system, holds significant potential in the rapidly warming Arctic, where temperatures currently rise at more than twice the global average, accelerating ice sheet and permafrost melt. This contributes to global sea-level rise and releases methane, a potent greenhouse gas. Strategies like solar radiation management (SRM) and carbon dioxide removal (CDR) could mitigate these effects; for instance, SRM techniques aim to reflect a portion of the sun's energy back into space, potentially slowing ice melt and stabilizing permafrost. However, geoengineering in the Arctic faces challenges, including potential unintended consequences on the fragile ecosystem, disruption of local weather patterns, and impacts on indigenous communities. Effective governance requires robust international cooperation, environmental impact assessments, and regulatory frameworks. Despite these challenges, geoengineering's potential benefits make it a critical research area. This report explores application of the Performance Assessment (PA) methodology to Arctic Climate Intervention, providing an initial screening of relevant features, events, and processes (FEPs). At the core of the PA approach is the identification and evaluation of FEPs that could impact the performance of the intervention scheme. Here we provide an initial screening of FEPs to consider in the application of PA to Arctic Climate Intervention.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

Wind-Driven Direct Air Capture System Using 3D Printed, Passive, Amine-Loaded Contactors (WEDAC)

This project advanced the development of a novel wind-driven direct air capture (WEDAC) system for removing carbon dioxide (CO 2 ) from the atmosphere. Our research focused on combining passive air contact with electrothermal desorption using specially designed carbon fiber modules, aiming to provide a scalable, low-cost, and energy-efficient alternative to conventional carbon capture systems.

36 MATERIALS SCIENCE↗

DOE OSTI2025

Second generation non-aqueous solvents (gen2nas) for co 2 capture from natural gas combined cycle plants

This final technical report submitted to DOE/NETL presents all the research activities performed during the Cooperative Agreement DE-FE0032218 entitled Second Generation Non-Aqueous Solvents (GEN2NAS) for CO 2 Capture from Natural Gas Combined Cycle Plants, which spanned from April 2023 through March 2025. In this project, Research Triangle Institute (RTI) International has developed the second-generation of its non-aqueous solvent (NAS), herein referred to as GEN2NAS, to remove carbon dioxide (CO 2 ) from natural-gas combined cycle (NGCC) flue gas. The technology aims to substantially reduce the cost of CO 2 capture while minimizing the environmental impacts through lower secondary emissions and wastewater generated from the CO 2 capture plant.

01 COAL, LIGNITE, AND PEAT↗

DOE OSTI2025

Technical and Community Foundations for High-Integrity CDR MRV Standards (Final Report)

The goal of this project (hereafter referred to as the “umbrella project”) was to establish cross-cutting technical foundations for carbon dioxide removal (CDR) accounting decisions. These cross-cutting and science driven technical foundations are necessary to increase trust in standards-setting and protocol development. According to key stakeholders in the industry, establishment of trusted standards is necessary to unlock and catalyze investment in the CDR industry as well as commercialization and deployment of verified, accepted high quality CDR technologies. Additionally, our umbrella project served as the lead coordinator of the cohort of three additional CDR pathway-focused projects funded under this award. In this role, we brought together the project teams to share insights, industry feedback, and approaches to CDR accounting standards development.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

Carbon neutrality in Malaysia and Kuala Lumpur: Insights from stakeholder-driven integrated assessment modeling

Several cities in Malaysia have established plans to reduce their CO2 emissions, in addition to Malaysia submitting a Nationally Determined Contribution to reduce its carbon intensity (against GDP) by 45% in 2030 compared to 2005. Meeting these emissions reduction goals will require a joint effort between governments, industries, and corporations at different scales and across sectors. In collaboration with national and sub-national stakeholders, we developed and used a global integrated assessment model to explore emissions mitigation pathways in Malaysia and Kuala Lumpur. Guided by current climate action plans, we created a suite of scenarios to reflect uncertainties in policy ambition, level of adoption, and implementation for reaching carbon neutrality. Through iterative engagement with all parties, we refined the scenarios and focus of the analysis to best meet the stakeholders’ needs. We found that Malaysia can reduce its carbon intensity and reach carbon neutrality by 2050, and that action in Kuala Lumpur can play a significant role. Decarbonization of the power sector paired with extensive electrification, energy efficiency improvements in buildings, transportation, and industry, and the use of advanced technologies such as hydrogen and carbon capture and storage will be major drivers to mitigate emissions, with carbon dioxide removal strategies being key to eliminate residual emissions. This study highlights the participatory process in which stakeholders contributed to the development of the model and guided the analysis, as well as insights into Malaysia’s decarbonization potential and the role of multilevel governance.

cities↗

DOE OSTI2024

Global and regional hydrological impacts of global forest expansion

Abstract. Large-scale reforestation, afforestation, and forest restoration schemes have gained global support as climate change mitigation strategies due to their significant carbon dioxide removal (CDR) potential. However, there has been limited research into the unintended consequences of forestation from a biophysical perspective. In the Community Earth System Model version 2 (CESM2), we apply a global forestation scenario, within a Paris Agreement-compatible warming scenario, to investigate the land surface and hydroclimate response. Compared to a control scenario where land use is fixed to present-day levels, the forestation scenario is up to 2 °C cooler at low latitudes by 2100, driven by a 10 % increase in evaporative cooling in forested areas. However, afforested areas where grassland or shrubland are replaced lead to a doubling of plant water demand in some tropical regions, causing significant decreases in soil moisture (∼ 5 % globally, 5 %–10 % regionally) and water availability (∼ 10 % globally, 10 %–15 % regionally) in regions with increased forest cover. While there are some increases in low cloud and seasonal precipitation over the expanded tropical forests, with enhanced negative cloud radiative forcing, the impacts on large-scale precipitation and atmospheric circulation are limited. This contrasts with the precipitation response to simulated large-scale deforestation found in previous studies. The forestation scenario demonstrates local cooling benefits without major disruption to global hydrodynamics beyond those already projected to result from climate change, in addition to the cooling associated with CDR. However, the water demands of extensive forestation, especially afforestation, have implications for its viability, given the uncertainty in future precipitation changes.

Environmental Sciences & Ecology↗

DOE OSTI2020

Reaching 1.5 and 2.0 °C global surface temperature targets using stratospheric aerosol geoengineering

A new set of stratospheric aerosol geoengineering (SAG) model experiments has been performed with Community Earth System Model version 2 (CESM2) with the Whole Atmosphere Community Climate Model (WACCM6) that are based on the Coupled Model Intercomparison Project phase 6 (CMIP6) overshoot scenario (SSP5-34-OS) as a baseline scenario to limit global warming to 1.5 or 2.0 °C above 1850–1900 conditions. The overshoot scenario allows us to applying a peak-shaving scenario that reduces the needed duration and amount of SAG application compared to a high forcing scenario. In addition, a feedback algorithm identifies the needed amount of sulfur dioxide injections in the stratosphere at four pre-defined latitudes, 30 °N, 15 °N, 15 °S, and 30 °S, to reach three surface temperature targets: global mean temperature, and interhemispheric and pole-to-Equator temperature gradients. These targets further help to reduce side effects, including overcooling in the tropics, warming of high latitudes, and large shifts in precipitation patterns. These experiments are therefore relevant for investigating the impacts on society and ecosystems. Comparisons to SAG simulations based on a high emission pathway baseline scenario (SSP5-85) are also performed to investigate the dependency of impacts using different injection amounts to offset surface warming by SAG. We find that changes from present-day conditions around 2020 in some variables depend strongly on the defined temperature target (1.5 °C vs. 2.0 °C). These include surface air temperature and related impacts, the Atlantic Meridional Overturning Circulation, which impacts ocean net primary productivity, and changes in ice sheet surface mass balance, which impacts sea level rise. Others, including global precipitation changes and the recovery of the Antarctic ozone hole, depend strongly on the amount of SAG application. Furthermore, land net primary productivity as well as ocean acidification depend mostly on the global atmospheric CO 2 concentration and therefore the baseline scenario. Multi-model comparisons of experiments that include strong mitigation and carbon dioxide removal with some SAG application are proposed to assess the robustness of impacts on societies and ecosystems.

42 ENGINEERING↗

DOE OSTI2020

Electrochemical devices and fuel cell systems

Electrochemical devices including electrochemical pumps (ECPs) and fuel cell systems comprising a fuel cell and an ECP are disclosed. In particular, this electrochemical device can be an ECP that comprises an anode, a cathode and an anion exchange polymer separating the anode from the cathode. The ECP can be coupled to a hydroxide exchange membrane fuel cell (HEMFC) that is disclosed herein as a fuel cell system. These devices can be used in methods for removing carbon dioxide from air and for generating electricity.

Yan, Yushan↗

DOE OSTI2022

Process Modeling and Optimization of DAC Systems and Novel Sorbent Materials

This poster presents an overview of the general methodology to be implemented in Task 9.0, Advanced Modeling Support of CDR Pilot Projects, of the Carbon Dioxide Removal program (CDR FWP22). Specifically, the poster presents the multi-scale modelling framework and optimization approaches to develop DAC systems, and how this can support bench/pilot scale tests that improve data collection and minimize uncertainty for scale-up of DAC technologies.

Caballero, Daison↗

DOE OSTI2023

Process Modeling and Analysis of a Novel Sorbent Material for Direct Air Capture Applications

This poster presents results of Task 9.0, Advanced Modeling Support of CDR Pilot Projects, of the Carbon Dioxide Removal program (CDR FWP23). Specifically, the poster presents the multi-scale modelling framework to investigate alternate processes configuration for DAC applications including Vacuum-Assisted Temperature Swing Adsorption (TVSA) process and sweep gas for regeneration.

Caballero, Daison↗

DOE OSTI2023

Electrochemical devices and fuel cell systems

Yan, Yushan↗

DOE OSTI2022

Heirloom Carbon Technologies, Inc. Final Scientific/Technical Report A transformative low-cost approach for Direct Air Mineralization of CO2 via repeated cycles of ambient weathering of metal oxides

Explore the source record for details and available documents.

42 ENGINEERING↗

DOE OSTI2023

Hierarchical Porous Activated Carbon from Wheat Bran Agro-Waste: Applications in Carbon Dioxide Capture, Dye Removal, Oxygen and Hydrogen Evolution Reactions

Here this work reports an efficient method for facile synthesis of hierarchically porous carbon (WB-AC) utilizing wheat bran waste. Obtained carbon showed 2.47 mmol g -1 CO 2 capture capacity with good CO 2 /N 2 selectivity and 27.35 to 29.90 kJ mol -1 isosteric heat of adsorption. Rapid removal of MO dye was observed with a capacity of ~555 mg g -1 . Moreover, WB-AC demonstrated a good OER activity with 0.35 V low overpotential at 5 mA cm -2 and a Tafel slope of 115 mV dec -1 . It also exhibited high electrocatalytic HER activity with 57 mV overpotential at 10 mA cm -2 and a Tafel slope of 82.6 mV dec -1 . The large SSA (757 m 2 g -1 ) and total pore volume (0.3696 cm 3 g -1 ) result from N 2 activation contributing to selective CO 2 uptake, high and rapid dye removal capacity and superior electrochemical activity (OER/HER), suggesting the use of WB-AC as cost effective adsorbent and metal free electrocatalyst.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2020

Guanidine compounds for removal of oxyanions from aqueous solutions and for carbon dioxide capture

Methods for removing oxyanions from water according to the following steps: (i) dissolving an oxyanion precipitating compound into the aqueous source to result in precipitation of an oxyanion salt of the oxyanion precipitating compound; and (ii) removing the oxyanion salt from the water containing the oxyanion to result in water substantially reduced in concentration of the oxyanion; wherein the oxyanion precipitating compound has the following composition: wherein A is a ring-containing moiety and Xm− is an anionic species with a magnitude of charge m. The invention employs bis-iminoguanidinium compounds according to Formula (1a) as well as neutral precursor compounds according to Formula (1), which can be used for removing undesirable species from aqueous solutions or air, such as removal of sulfate from water and carbon dioxide from air.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2024

A Model of Large Scale Electrochemical Direct Ocean Capture Under Variable Power

Since limiting warming to 1.5 degrees C by 2100 will not only require an energy transition but also billions of tons of carbon dioxide (CO2) removal per year, it is essential to expand these efforts. This can be done offshore via electrochemical direct ocean capture (eChem DOC) which extracts CO2 from seawater that can later be stored underground or converted to products. Deployments of eChem DOC will be powered by renewable energy and therefore need to function with variable power inputs. This project aims to support future large-scale deployments by developing a model of eChem DOC operation, informed by industry and literature, and assessing its performance under variable power and varying designs. Initial analysis suggests that discretizing the eChem system has a higher impact on increasing overall capture than storing the chemical solutions to continue capture during periods of lower power availability, but this is likely situation dependent. Future work will use more realistic power profiles.

direct ocean capture↗

DOE OSTI2024

Parts-Per-Million Carbonate Mineral Quantification with Thermogravimetric Analysis–Mass Spectrometry

Mitigating the deleterious effects of climate change requires the development and implementation of carbon capture and storage technologies. To expand the monitoring, verification, and reporting (MRV) capabilities of geologic carbon mineralization projects, we developed a thermogravimetric analysis–mass spectrometry (TGA–MS) methodology to enable quantification of <100 ppm calcite (CaCO 3 ) in complex samples. We extended TGA–MS calcite calibration curves to enable a higher measurement resolution and lower limits of quantification for evolved CO 2 from a calcite–corundum mixture. We demonstrated <100 ppm carbonate mineral quantification with TGA–MS for the first time, an outcome applicable across earth, environmental, and materials science fields. We applied this carbonate quantification method to a suite of Columbia River Basalt Group (CRBG) well cuttings recovered in 2009 from Pacific Northwest National Laboratory’s Wallula #1 Well. Our execution of this new combined calcite and calcite–corundum calibration curve TGA–MS method on our CRBG sample suite indicated average carbonate contents of 0.050 wt % in flow interiors (caprocks) and 0.400 wt % in interflow zones (reservoirs) in the upper 1250 m of the Wallula #1 Well. Finally, by advancing our knowledge of continental flood basalt-hosted carbonates in the mafic subsurface and reaching new TGA–MS quantification limits for carbonate minerals, we expand MRV capabilities and support the commercial-scale deployment of carbon mineralization projects in the Pacific Northwest United States and beyond.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2025

Advancing a Low-Temperature, Low-Cost Direct Air Capture System Based on Organic Chemistry

Holocene Climate Corporation (Holocene) partnered with Oak Ridge National Laboratory (ORNL) to conduct bench-scale testing of a new optimized Direct Air Capture (DAC) process to assist the U.S. Department of Energy (DOE) in achieving the Carbon Negative Shot target of under $\$$100/net tonne CO₂ removed by 2031. Holocene’s DAC process for carbon dioxide (CO₂) removal uses amino acids and guanidine compounds, an ORNL-invented chemical process and licensed by Holocene. Holocene will use this novel chemistry to develop a new process and deploy the technology commercially.

36 MATERIALS SCIENCE↗