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NASA NTRS1989

Infrared spectra of crystalline and glassy silicates and application to interstellar dust

The infrared spectra of crystalline minerals predicted in theoretical condensation sequences do not match the astronomical observations. Since the astronomical spectra are a closer match to glassy silicates, the authors undertook a study to measure the infrared spectra of glassy silicates that have compositions similar to silicate minerals predicted in theoretical condensation sequences. The data should support observations aimed at elucidating condensation chemistry in dust forming regions. The authors measured the mass absorption coefficients, from 2.5 to 25 microns, of ground samples of olivine, diopside, and serpentine and also smoke samples that were prepared from these minerals. The smoke samples prepared in this way are predominantly glassy with nearly the same composition as the parent minerals. The crystalline samples consisted of pure olivine ((Fe(0.1)Mg(0.9))(2)SiO(4)), serpentine, diopside. Sample purity was confirmed by x ray diffraction. Each mineral was ground for 10 hours and a measured mass of the powder was mixed with KBr powder for absorption measurements using the method of Borghesi et a. (1985). The smoke samples were prepared from the same samples used for grinding by vaporizing the minerals using pulsed laser radiation in air. The smoke samples formed by condensation of the resulting vapor. The smoke settled onto infrared transparent KRS-5 substrates and onto a quartz crystal microbalance used to obtain mass measurements. A description of the preparation method is given in Stephens (1980). The glassy diopside showed only diffuse electron diffraction peaks and hence was nearly amorphous, while the serpentine smoke showed a weak diffraction pattern corresponding to MgO. The smoke from olivine showed a weak diffraction pattern corresponding to Fe2O3 and/or Fe3O4. The mass absorption coefficients, from 2.5 to 25 microns, of crystalline diopside, olivine, and serpentine and their corresponding smoke samples are shown in figures.

Stephens, John R.↗

NASA NTRS2018

Delayed Shock-Induced Dust Formation in the Dense Circumstellar Shell Surrounding the Type IIn Supernova SN 2010jl

The light curves of Type IIn supernovae are dominated by the radiative energy released through the interaction of the supernova shock waves with their dense circumstellar medium (CSM). The ultraluminous Type IIn supernova SN2010jl exhibits an infrared emission component that is in excess of the extrapolated UV-optical spectrum as early as few weeks postexplosion. This emission has been considered by some as evidence for the rapid formation of dust in the cooling postshock CSM. We investigate the physical processes that may inhibit or facilitate the formation of dust in the CSM. When only radiative cooling is considered, the temperature of the dense shocked gas rapidly drops below the dust condensation temperature. However, by accounting for the heating of the postshock gas by the downstream radiation from the shock, we show that dust formation is inhibited until the radiation from the shock weakens as it propagates into the less dense outer regions of the CSM. In SN2010jl, dust formation can therefore only commence after day ∼380. Only the IR emission since that epoch can be attributed to the newly formed CSM dust. Observations on day 460 and later show that the IR luminosity exceeds the UV-optical luminosity. The postshock dust cannot extinct the radiation emitted by the expanding SN shock. Therefore, its IR emission must be powered by an interior source, which we identify as the reverse shock propagating through the SN ejecta. IR emission before day 380 must therefore be an IR echo from preexisting CSM dust.

Sarangi, Arkaprabha↗

NASA NTRS2015

Investigation of the CCN Activity, BC and UVBC Mass Concentrations of Biomass Burning Aerosols during the 2013 BASELInE Campaign

Biomass-burning (BB) aerosols, acting as cloud condensation nuclei (CCN), can influence cloud microphysical and radiative properties. In this study, we present CCN measured near the BB source regions over northern Southeast Asia (Doi Ang Khang, Thailand) and at downwind receptor areas (Lulin Atmospheric Background Station, Taiwan), focusing exclusively on 13-20 March 2013 as part of 2013 spring campaign of the Seven SouthEast Asian Studies (7-SEAS) intensive observation. One of the campaigns objectives is to characterize BB aerosols serving as CCN in SouthEast Asia (SEA). CCN concentrations were measured by a CCN counter at 5 supersaturation (SS) levels: 0.15%, 0.30%, 0.45%, 0.60%, and 0.75%. In addition, PM2.5 and black carbon mass concentrations were analyzed by using a tapered element oscillating microbalance and an aethalometer. It was found the number-size distributions and the characteristics of hygroscopicity (e.g., activation ratio and k) of BB aerosols in SEA have a strong diurnal pattern, and different behaviors of patterns were characterized under two distinct weather systems. The overall average value was low (0.05-0.1) but comparable with previous CCN studies in other BB source regions. Furthermore, a large fraction of UV-absorbing organic material (UVBC) and high Delta-C among BB aerosols were also observed, which suggest the existence of substantial particulate organic matter in fresh BB aerosols. These data provide the most extensive characterization of BB aerosols in SEA until now.

biomass burning aerosol↗

NASA NTRS1996

Fundamental Phenomena on Fuel Decomposition and Boundary-Layer Combustion Precesses with Applications to Hybrid Rocket Motors: Experimental Investigation - Part 1

This final report summarizes the major findings on the subject of 'Fundamental Phenomena on Fuel Decomposition and Boundary-Layer Combustion Processes with Applications to Hybrid Rocket Motors', performed from 1 April 1994 to 30 June 1996. Both experimental results from Task 1 and theoretical/numerical results from Task 2 are reported here in two parts. Part 1 covers the experimental work performed and describes the test facility setup, data reduction techniques employed, and results of the test firings, including effects of operating conditions and fuel additives on solid fuel regression rate and thermal profiles of the condensed phase. Part 2 concerns the theoretical/numerical work. It covers physical modeling of the combustion processes including gas/surface coupling, and radiation effect on regression rate. The numerical solution of the flowfield structure and condensed phase regression behavior are presented. Experimental data from the test firings were used for numerical model validation.

Kuo, Kenneth K.↗

NASA NTRS1984

The Orion Molecular Cloud at Far-infrared Wavelengths

A new, 34 in resolution far-infrared continuum map of Orion Molecular Cloud 1 and its environs, including M43 is presented. The source is dominated by a single, bright peak at the position of the embedded infrared cluster, with the 60 micro m flux density falling off steeply in all directions away from it. A total luminosity for IRc2 of 20,000 L(solar) is estimated, although this may be a lower limit, depending upon the transfer of radiation in the vicinity of the object. Several condensations appear in this map, which, along with radio molecular observations, support the view that significant fragmentation has taken place within the cloud.

Thronson, H. A., Jr.↗

NASA NTRS1992

Effects of aerosol from biomass burning on the global radiation budget

An analysis is made of the likely contribution of smoke particles from biomass burning to the global radiation balance. These particles act to reflect solar radiation directly; they also can act as cloud condensation nuclei, increasing the reflectivity of clouds. Together these effects, although uncertain, may add up globally to a cooling effect as large as 2 watts per square meter, comparable to the estimated contribution to sulfate aerosols. Anthropogenic increases of smoke emission thus may have helped weaken the net greenhouse warming from anthropogenic trace gases.

Penner, Joyce E.↗

NASA NTRS1992

Modeling interannual variability in the Martian seasonal CO2 cycle

One aspect of the seasonal pressure variations measured at the Viking Lander sites is their nearly perfect interannual repeatability. This presents a problem because it implies that the behavior of the seasonal polar caps should be highly repeatable from year to year as well. There are a number of observations and theories suggesting that the presence of dust and water ice clouds in the Martian atmosphere should have significant direct and indirect effects on the rates of CO2 condensation and sublimation in the north and south polar regions. These effects include (1) reduced rates of CO2 frost condensation during polar night seasons due to the radiative effects of dust and water ice clouds and associated CO2 clouds or elevated atmospheric temperatures and (2) reduced or elevated rates of frost sublimation due to the radiative effects of atmospheric dust or to changes in frost emissivities and albedos due to contamination by water ice and dust. The Viking Landing pressure observations are examined to determine the range and character of the interannual variations present. Then a diurnal and seasonal thermal model is used to examine the effects of interannual variations in the polar heat balance on seasonal pressure variations.

Wood, S. E.↗

NASA NTRS1992

Galaxies and gas in a cold dark matter universe

We use a combined gravity/hydrodynamics code to simulate the formation of structure in a random 22 Mpc cube of a cold dark matter universe. Adiabatic compression and shocks heat much of the gas to temperatures of 10 exp 6 - 10 exp 7 K, but a fraction of the gas cools radiatively to about 10 exp 4 K and condenses into discrete, highly overdense lumps. We identify these lumps with galaxies. The high-mass end of their baryonic mass function fits the form of the observed galaxy luminosity function. They retain independent identities after their dark halos merge, so gravitational clustering produces groups of galaxies embedded in relatively smooth envelopes of hot gas and dark matter. The galaxy correlation function is approximately an r exp -2.1 power law from separations of 35 kpc to 7 Mpc. Galaxy fluctuations are biased relative to dark matter fluctuations by a factor b about 1.5. We find no significant 'velocity bias' between galaxies and dark matter particles. However, virial analysis of the simulation's richest group leads to an estimated Omega of about 0.3, even though the simulation adopts Omega = 1.

Katz, Neal↗

NASA NTRS1981

The cooling and condensation of flare coronal plasma

A model is investigated for the decay of flare heated coronal loops in which rapid radiative cooling at the loop base creates strong pressure gradients which, in turn, generate large (supersonic) downward flows. The coronal material cools and 'condenses' onto the flare chromosphere. The features which distinguish this model from previous models of flare cooling are: (1) most of the thermal energy of the coronal plasma may be lost by mass motion rather than by conduction or coronal radiation; (2) flare loops are not isobaric during their decay phase, and large downward velocities are present near the footpoints; (3) the differential emission measure q has a strong temperature dependence.

Antiochos, S. K.↗

NASA NTRS1978

Effects of proton irradiation on a gas phase in which condensation takes place. I Negative Mg-26 anomalies and Al-26

In the present paper, isotopic effects in magnesium generated in a proton-irradiated gas phase are examined, taking only (p,n), (p,d), and (p, alpha) reactions in magnesium, aluminum, and silicon into consideration. In the presence of proton radiation, the three elements are 'removed' from the gas phase by condensation. It is required that a value of Al-26/Al-27 greater than 6 times 10 to the -5th must be reached, consistent with the value deduced by Lee Papanastassiou, and Wasserburg (1976) from their studies of the Allende meteorite. The calculations show that fast aluminum condensation reduces the required proton fluence substantially, that a significant fraction of aluminum remains uncondensed when the above value of the Al-26/Al-27 ratio is reached, that a detectable MG-24 excess is very likely to occur, that detectable negative MG-28 anomalies can be generated, and that proton fluxes and irradiation times can be varied simultaneously, and over a wide range of values, without significant changes in the required proton fluence.

Heymann, D.↗

NASA NTRS1972

Investigation of gaseous nuclear rocket technology

The experimental and theoretical investigations conducted during the period from September 1969 through September 1972 are reported which were directed toward obtaining information necessary to determine the feasibility of the full-scale nuclear light bulb engine, and of small-scale nuclear tests involving fissioning uranium plasmas in a unit cell installed in a driver reactor, such as the Nuclear Furnace. Emphasis was placed on development of RF simulations of conditions expected in nuclear tests in the Nuclear Furnace. The work included investigations of the following: (1) the fluid mechanics and containment characteristics of one-component and two-component vortex flows, both unheated and RF-induction heated; (2) heating of particle-seeded streams by thermal radiation from a dc arc to simulate propellant heating; (3) condensation and separation phenomena for metal-vapor/heated-gas mixtures to provide information for conceptual designs of components of fuel exhaust and recycle systems; (4) the characteristics of the radiant energy spectrum emitted from the fuel region, with emphasis on definition of fuel and buffer-gas region seed systems to reduce the ultraviolet radiation emitted from the nuclear fuel; and (5) the effects of nuclear radiation on the optical transmission characteristics of transparent materials.

Kendall, J. S.↗

NASA NTRS2021

Rapid Cloud Removal of Dimethyl Sulfide Oxidation Products Limits SO 2 and Cloud Condensation Nuclei Production in the Marine Atmosphere

Oceans emit large quantities of dimethyl sulfide (DMS) to the marine atmosphere. The oxidation of 60 DMS leads to the formation and growth of cloud condensation nuclei (CCN) with consequent effects on Earth’s radiation balance and climate. Quantitative assessment of the impact of DMS emissions on CCN concentrations necessitates a detailed description of the oxidation of DMS in the presence of existing aerosol particles and clouds. In the unpolluted marine atmosphere, DMS is efficiently oxidized to hydroperoxymethyl thioformate (HPMTF), a stable intermediate in the chemical trajectory towards sulfur dioxide (SO 2 ) and ultimately sulfate aerosol (Veres et al. 2020). Using direct airborne flux measurements, we demonstrate that irreversible loss of HPMTF to clouds in the marine boundary layer determines the HPMTF lifetime (τ HPMTF < 2 hours) and terminates DMS oxidation to SO 2 in the cloudy marine boundary layer. When accounting for HPMTF cloud loss in a global chemical transport model, we show that SO 2 production from DMS is reduced by 35% globally and near surface (0-3km) SO 2 concentrations over the ocean are lowered by 24%. This large, previously unconsidered loss process for volatile sulfur accelerates the timescale for conversion of DMS to sulfate, while limiting new particle formation in the marine atmosphere and changing the dynamics of aerosol growth. This loss process potentially reduces the spatial scale over which DMS emissions contribute to aerosol production and growth and weakens the link between DMS emission and marine CCN production with subsequent implications for cloud formation, radiative forcing, and climate.

dimethyl sulfide↗

NASA NTRS1984

Radiative tearing - Magnetic reconnection on a fast thermal-instability time scale

Two energy modification mechanisms which are known to occur in sheared magnetic fields are the tearing and thermal instabilities. These processes can be studied separately with formalisms incorporating just the effective driving mechanism of interest (finite resistivity for the tearing mode and unstable radiation for the thermal mode). A model which includes both effects, and a temperature-dependent resistivity, indicates that modified forms of these two instabilities may coexist for identical physical conditions. When they are isolated computationally, one can show that their limiting growth rates are approximately those of the uncoupled instabilities. The spatial structure and energy content of these two new hybrid processes are then individually examined and are found to differ considerably from those obtained from separate treatments of the driving mechanisms. The faster radiative instability, which has a hydromagnetically scaled growth rate like the condensation mode of the thermal instability, is shown to involve a substantial amount of magnetic field reconnection. This can be partially explained by a large temperature drop (or resistivity rise) at the X-point. The island width of the Coulomb-coupled radiative mode is 30 percent of that produced by a comparable level of the slower tearing instability. In addition, the perturbed magnetic energy in the radiative instability is 5 times that of the perturbed thermal energy, indicating an appreciable modification of the initial magnetic structure.

Steinolfson, R. S.↗

NASA NTRS1997

Anthropogenic Sulfate, Clouds, and Climate Forcing

This research work is a joint effort between research groups at the Battelle Pacific Northwest Laboratory, Virginia Tech University, Georgia Institute of Technology, Brookhaven National Laboratory, and Texas A&M University. It has been jointly sponsored by the National Aeronautics and Space Administration, the U.S. Department of Energy, and the U.S. Environmental Protection Agency. In this research, a detailed tropospheric aerosol-chemistry model that predicts oxidant concentrations as well as concentrations of sulfur dioxide and sulfate aerosols has been coupled to a general circulation model that distinguishes between cloud water mass and cloud droplet number. The coupled model system has been first validated and then used to estimate the radiative impact of anthropogenic sulfur emissions. Both the direct radiative impact of the aerosols and their indirect impact through their influence on cloud droplet number are represented by distinguishing between sulfuric acid vapor and fresh and aged sulfate aerosols, and by parameterizing cloud droplet nucleation in terms of vertical velocity and the number concentration of aged sulfur aerosols. Natural sulfate aerosols, dust, and carbonaceous and nitrate aerosols and their influence on the radiative impact of anthropogenic sulfate aerosols, through competition as cloud condensation nuclei, will also be simulated. Parallel simulations with and without anthropogenic sulfur emissions are performed for a global domain. The objectives of the research are: To couple a state-of-the-art tropospheric aerosol-chemistry model with a global climate model. To use field and satellite measurements to evaluate the treatment of tropospheric chemistry and aerosol physics in the coupled model. To use the coupled model to simulate the radiative (and ultimately climatic) impacts of anthropogenic sulfur emissions.

Ghan, Steven J.↗

NASA NTRS1977

Space radiation resistant transparent polymeric materials

A literature search in the field of ultraviolet and charged particle irradiation of polymers was utilized in an experimental program aimed at the development of radiation stable materials for space applications. The rationale utilized for material selection and the synthesis, characterization and testing performed on several selected materials is described. Among the materials tested for ultraviolet stability in vacuum were: polyethyleneoxide, polyvinylnaphthalene, and the amino resin synthesized by the condensation of o-hydroxybenzoguanamine with formaldehyde. Particularly interesting was the radiation behavior of poly(ethyleneoxide), irradiation did not cause degradation of optical properties but rather an improvement in transparency as indicated by a decrease in solar absorptance with increasing exposure time.

Giori, C.↗

NASA NTRS1983

Influence of radiative heating and cumulus convection on development of mean monsoon circulation in July

Numerical simulations of July mean monsoon circulation in the tropics are described. The model used in the simulations was based on a series of primitive equations for the combined effects of variations of solar radiation, radiative diurnal warming, and large-scale and deep cumulus condensation, and the kinematic effects of topography. The initial states of the model were derived from the observed mean distributions of pressure and humidity. Analysis of the numerical results showed that the large-scale features of the mean July monsoon circulation in the tropics are created mainly by differential diabatic heating under the influence of the specific topography. The time necessary to establish the large scale features was only about 5 days when the diurnal variation of solar radiation was taken into account. Graphic illustrations of the simulated mean July flow conditions are provided.

Kuo, H. L.↗

NASA NTRS1993

Impact of the CO2 and H2O clouds of the Martian polar hood on the polar energy balance

Clouds covering extensive areas above the martian polar caps have regularly been observed during the fall and winter seasons of each hemisphere. These 'polar hoods' are thought to be made of H2O and CO2. In particular, the very cold temperatures observed during the polar night by Viking and Mariner 9 around both poles have been identified as CO2 clouds and several models, including GCM, have indicated that the CO2 can condense in the atmosphere at all polar latitudes. Estimating the impact of the polar hood clouds on the energy balance of the polar regions is necessary to model the CO2 cycle and address puzzling problems like the polar caps assymetry. For example, by altering the thermal radiation emitted to space, CO2 clouds alter the amount of CO2 that condenses during the fall and winter season. The complete set of Viking IRTM data was analyzed to define the spatial and temporal properties of the polar hoods, and how their presence affects the energy radiated by the atmosphere/caps system to space was estimated. The IRTM observations provide good spatial and temporal converage of both polar regions during fall, winter, and spring, when a combination of the first and the second Viking year is used. Only the IRTM brightness temperatures at 11, 15, and 20 microns are reliable at martian polar temperatures. To recover the integrated thermal fluxes from the IRTM data, a simple model of the polar hood, thought to consist of 'warm' H2O clouds lying above colder and opaque CO2 clouds was developed. Such a model is based on the analysis of the IRIS spectra, and is consistent with the IRTM data used.

Forget, Francois↗

NASA NTRS1977

Change in the thermionic work function of semiconductor powders exposed to electromagnetic radiation

The variations of the thermoelectronic work function of titanium dioxide, submitted to an ultraviolet or visible and infrared radiation, in the presence of oxygen, are studied by the vibrating condenser method. It is shown that during the ultraviolet irradiation, a desorption of a first species of oxygen simultaneously occurs with the adsorption of a second species of oxygen and that this phenomenon is found for any structure of TiO2 (anatase or rutile) any texture, oxygen pressure, radiation intensity, and nature of introduced dopes.

Bourasseau, S.↗