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At least 163 records · Page 9
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NASA NTRS1976

Prediction of the diffuse far-infrared flux from the galactic plane

A basic model and simple numerical relations useful for future far-infrared studies of the Galaxy are presented. Making use of recent CO and other galactic surveys, the diffuse far-infrared flux distribution from the galactic planes is predicted as a function of galactic longitude for the region between 4 and 90 deg longitude; the far-infrared emissivity is predicted as a function of galactocentric distance. Future measurements of the galactic far-infrared flux would yield valuable information on the physical properties and distribution of dust and molecular clouds in the Galaxy, particularly the inner region.

Fazio, G. G.↗
NASA NTRS1978

A cloud physics radiometer

The paper describes the design features and capabilities of a seven-channel cloud physics radiometer (CPR) for remote sensing of cloud properties. The CPR channel characteristics and functions are tabulated and diagrammed. Each of the first three channels utilizes a photo-multipler detector, with the high-voltage power supply integrated with the tube into a single unit. In operation a heater is used to keep the optics temperature at or above 273 K and this temperature is constantly monitored. The last four channel detectors and filters are all cooled to the temperature of liquid nitrogen. The inclined scanning mirror rotates at a rate of 3.48 rps. Registration pulses are triggered and recorded as the mirror enters and leaves the + or -45 deg earth observation region. The ice-cloud, water cloud, snow discriminator detector has worked quite well in general. Interesting radiometer data have been obtained and their analysis is under way. The combination of the CPR and the Cloud Lidar System will make possible sophisticated remote sensing cloud studies.

Kyle, H. L.↗
NASA NTRS2014

A Comparison of Potential IM-CW Lidar Modulation Techniques for ASCENDS CO2 Column Measurements From Space

Global atmospheric carbon dioxide (CO2) measurements through the Active Sensing of CO2 Emissions over Nights, Days, and Seasons (ASCENDS) Decadal Survey recommended space mission are critical for improving our understanding of CO2 sources and sinks. IM-CW (Intensity Modulated Continuous Wave) lidar techniques are investigated as a means of facilitating CO2 measurements from space to meet the ASCENDS science requirements. In previous laboratory and flight experiments we have successfully used linear swept frequency modulation to discriminate surface lidar returns from intermediate aerosol and cloud contamination. Furthermore, high accuracy and precision ranging to the surface as well as to the top of intermediate clouds, which is a requirement for the inversion of the CO2 column-mixing ratio from the instrument optical depth measurements, has been demonstrated with the linear swept frequency modulation technique. We are concurrently investigating advanced techniques to help improve the auto-correlation properties of the transmitted waveform implemented through physical hardware to make cloud rejection more robust in special restricted scenarios. Several different carrier based modulation techniques are compared including orthogonal linear swept, orthogonal non-linear swept, and Binary Phase Shift Keying (BPSK). Techniques are investigated that reduce or eliminate sidelobes. These techniques have excellent auto-correlation properties while possessing a finite bandwidth (by way of a new cyclic digital filter), which will reduce bias error in the presence of multiple scatterers. Our analyses show that the studied modulation techniques can increase the accuracy of CO2 column measurements from space. A comparison of various properties such as signal to noise ratio (SNR) and time-bandwidth product are discussed.

Campbell, Joel F.↗
NASA NTRS1979

Imaging and polarimetry with the Pioneer Venus Orbiter Cloud Photopolarimeter

The objective of the Orbiter Cloud Photopolarimeter (OCPP) on board the Pioneer Venus Orbiter spacecraft is twofold: (1) to determine the physical properties, vertical and horizontal distribution and the temporal variability of the haze and cloud aerosols on Venus; and (2) to record in images made in the near ultraviolet the varying cloud morphology and the short- and long-term character of the apparent cloud motions. Early images exhibit numerous cloud features and apparent circulation patterns similar to those observed by Mariner 10 in 1974. Features of the polar regions are identified. Polarimetry measurements indicate that the main visible cloud layer of 1-micron-radius sulfuric acid droplets is covered at least in the morning terminator region with a thin haze layer consisting of submicron-size particles. The OCPP performance appears to be excellent.

Travis, L. D.↗
NASA NTRS1976

A spinar model of Cygnus A

It is proposed that a gravitationally bound supermassive object is located in the 'core' of each of the Cyg A radio clouds and that these objects are responsible for the prolonged ejection of magnetic plasma which produces the synchrotron radio emission. The objects are considered to be analogous to the massive rotators, or spinars, which have been used to model the central radio and optical activity of quasars. The formation of Cyg A is described in terms of the breakup of such an object in the central optical galaxy, and the physical properties of both the compact and the giant clouds are discussed, including the effects of intergalactic drag. It is shown that the spinars are capable of effectively replenishing the extended radio clouds with relativistic electrons, even if they are embedded within the compact clouds. The spinars are modeled quantitatively, and their possible detection is considered. The requirements of the proposed model are compared with those of several other models for bright double radio galaxies.

Flasar, F. M.↗
NASA NTRS1990

Radiative properties of visible and subvisible Cirrus: Scattering on hexagonal ice crystals

One of the main objectives of the First International Satellite Cloud Climatology Project (ISCCP) Regional Experiment (FIRE) is to provide a better understanding of the physics of upper level clouds. The focus is on just one specific aspect of cirrus physics, namely on characterizing the radiative properties of single, nonspherical ice particles. The basis for further more extensive studies of the radiative transfer through upper level clouds is provided. Radiation provides a potential mechanism for strong feedback between the divergence of in-cloud radiative flux and the cloud microphysics and ultimately on the dynamics of the cloud. Some aspects of ice cloud microphysics that are relevant to the radiation calculations are described. Next, the Discrete Dipole Approximation (DDA) is introduced and some new results of scattering by irregular crystals are presented. The Anomalous Diffraction Theory (ADT) was adopted to investigate the scattering properties of even larger crystals. In this way the scattering properties of nonspherical particles were determined over a range of particle sizes.

Flatau, Piotr J.↗
NASA NTRS2021

Inference of Precipitation in Warm Stratiform Clouds using Remotely Sensed Observations of the Cloud Top Droplet Size Distribution

Drizzle is a common feature of warm stratiform clouds and it influences their radiative effects by modulating their physical properties and lifecycle. An important component of drizzle formation are processes that lead to a broadening of the droplet size distribution (DSD). Here, we examine observations of cloud and drizzle properties retrieved using colocated airborne measurements from the Research Scanning Polarimeter and the Third Generation Airborne Precipitation Radar. We observe a bimodal DSD as the aircraft transects drizzling open-cells whereby the larger mode reaches a maximum size near cloud center and the smaller mode remains relatively constant in size. We review similarities between our observations with droplet growth processes and their connections with precipitation onset. We estimate droplet sedimentation using the cloud top DSD and find a correlation with rain water path of 0.82. We also examine how changes in liquid water paths and droplet concentrations may act to enhance or suppress precipitation.

Droplet size distribution↗
NASA NTRS2005

A Climatology of Midlatitude Continental Clouds from the ARM SGP Site: Low-Level Cloud Macrophysical, Microphysical, and Radiative Properties - Part I

A record of single-layer and overcast low cloud (stratus) properties has been generated using approximately 4000 hours of data collected from January 1997 to December 2002 at the Atmospheric Radiation Measurement (ARM) Southern Great Plains Central Facility (SCF). The cloud properties include liquid-phase and liquid-dominant, mixed-phase, low cloud macrophysical, microphysical, and radiative properties including cloud-base and -top heights and temperatures, and cloud physical thickness derived from a ground-based radar and lidar pair, and rawinsonde sounding; cloud liquid water path (LWP) and content (LWC), and cloud-droplet effective radius (r(sub e)) and number concentration (N) derived from the macrophysical properties and radiometer data; and cloud optical depth (tau), effective solar transmission (gamma), and cloud/top-of-atmosphere albedos (R(sub cldy)/R(sub TOA)) derived from Eppley precision spectral pyranometer measurements. The cloud properties were analyzed in terms of their seasonal, monthly, and hourly variations. In general, more stratus clouds occur during winter and spring than in summer. Cloud-layer altitudes and physical thicknesses were higher and greater in summer than in winter with averaged physical thicknesses of 0.85 km and 0.73 km for day and night, respectively. The seasonal variations of LWP, LWC, N. tau, R(sub cldy), and R(sub TOA) basically follow the same pattern with maxima and minima during winter and summer, respectively. There is no significant variation in mean r(sub e), however, despite a summertime peak in aerosol loading, Although a considerable degree of variability exists, the 6-yr average values of LWP, LWC, r(sub e), N, tau, gamma, R(sub cldy) and R(sub TOA) are 150 gm(exp -2) (138), 0.245 gm(exp -3) (0.268), 8.7 micrometers (8.5), 213 cm(exp -3) (238), 26.8 (24.8), 0.331, 0.672, 0.563 for daytime (nighttime). A new conceptual model of midlatitude continental low clouds at the ARM SGP site has been developed from this study. The low stratus cloud amount monotonically increases from midnight to early morning (0930 LT), and remains large until around local noon, then declines until 1930 LT when it levels off for the remainder of the night. In the morning, the stratus cloud layer is low, warm, and thick with less LWC, while in the afternoon it is high, cold, and thin with more LWC. Future parts of this series will consider other cloud types and cloud radiative forcing at the ARM SCF.

Dong, Xiquan↗
NASA NTRSDate not supplied

Variability in Modelled Airborne Dust Mineralogy Derived from Global Soil Composition Uncertainties

Dust aerosols consist on a variety of minerals with different physic and chemical properties. As such, they interact with short and long wave radiation, potentially form clouds, act as nutrients modulating biogeochemical cycles, or influence atmospheric chemistry, differently. Most current state-of-the-art Earth System Models (ESMs) neglect the complexity in dust composition, mainly due to computational constraints, but also to the existing uncertainties in the size resolved composition of parent soils, the resulting distribution of minerals in airborne dust, and the scarcity of observations to constrain them. Within this work, we assess the variability of global dust composition due to uncertainties in the characterization of the parent soil mineralogy. To that end, we consider two available global soil mineralogy atlases, developed by Claquin et al. (1999) –C1999- and Journet et al. (2014) –J2014-, which represent respectively 8 and 12 relevant minerals for climate (namely: illite, smectite/montmorillonite, kaolinite, calcite, gypsum, hematite, quartz, and feldspars in C1999, and those plus chlorite, vermiculite, goethite, and mica in J2014). Thanks to a recently developed feature of the MONARCH atmospheric-chemistry model, we are able to explicitly resolve the minerals’ atmospheric cycle. Therefore, we define two global experiments to assess changes on airborne dust composition attributed to the soil mineralogy assumptions and provide a measure of their variability. We also perform a preliminary evaluation of the global mineralogy results against available observations of mineral fractions in surface dust concentration. Our results will inform the climate modelling community about the potential variability in dust composition, an aspect that will gain relevance as ESMs continue growing in complexity and new processes to better characterize aerosols’ forcing or biogeochemical cycles are added. Further observational constraints, such as those that will derive from the EMIT NASA mission on soil composition or the FRAGMENT experimental campaigns on airborne dust characterization, will be key in the near future to improve our understanding of the impact of dust mineralogy on fundamental climate features.

Dust aerosols↗
NASA NTRS1989

Heterogeneous physicochemistry of the polar ozone hole

Processes occurring in the polar winter stratosphere, which involve polar stratospheric clouds (PSCs), are investigated using observations from the Airborne Antarctic Ozone Experiment. In particular, data on the properties of PSCs and their physical chemistry, the microphysical processes and time constants for cloud processes, the heterogeneous chemical processes and their time constants, and nonlinearities in the long-term ozone trend associated with physical and chemical processes are examined. The chemical reactions leading to the depletion of the inert chlorine reservoir in a presence of type I PSCs are established, and it is shown that type II PSCs contribute to chemical processing that sustains the chemical imbalance of the polar stratosphere. It is shown that, using a simple model, the decadal evolution of the Antarctic ozone hole may be understood through nonlinearities in the heterogeneous chemistry, with possible contributing effects of variations in stratospheric temperatures and water vapor concentrations.

Turco, Richard P.↗
NASA NTRS2011

Molecular Anions in Protostars, Prestellar Cores and Dark Clouds

From our recent survey work using the Green Bank Telescope, microwave emission lines from the hydrocarbon anion C6H(-) and its parent neutral C6H have been detected in six new sources. Using HC3N = 10(exp -9) emission maps, we targeted the most carbon-chain-rich sources for our anion survey, which included the low-mass Class 0 protostar L1251A-IRS3, the prestellar cores L1389-SMM1 and L1512, and the interstellar clouds Ll172A, TMC-1C and L1495B. Derived [C6H(-)]/[C6H] anion-to-neutral ratios are approximately 1-10. The greatest C6H(-) column densities are found in the quiescent clouds TMC-1C and L1495B, but the anion-to-neutral ratios are greatest in the prestellar cores and protostars. These results are interpreted in terms of the physical and chemical properties of the sources, and the implications for molecular cloud chemistry are discussed.

Cordiner, Martin↗
NASA NTRS1995

Remote sensing of smoke, clouds, and radiation using AVIRIS during SCAR experiments

During the past two years, researchers from several institutes joined together to take part in two SCAR experiments. The SCAR-A (Sulfates, Clouds And Radiation - Atlantic) took place in the mid-Atlantic region of the United States in July, 1993. remote sensing data were acquired with the Airborne Visible Infrared Imaging Spectrometer (AVIRIS), the MODIS Airborne Simulator (MAS), and a RC-10 mapping camera from an ER-2 aircraft at 20 km. In situ measurements of aerosol and cloud microphysical properties were made with a variety of instruments equipped on the University of Washington's C-131A research aircraft. Ground based measurements of aerosol optical depths and particle size distributions were made using a network of sunphotometers. The main purpose of SCAR-A experiment was to study the optical, physical and chemical properties of sulfate aerosols and their interaction with clouds and radiation. Sulfate particles are believed to affect the energy balance of the earth by directly reflecting solar radiation back to space and by increasing the cloud albedo. The SCAR-C (Smoke, Clouds And Radiation - California) took place on the west coast areas during September - October of 1994. Sets of aircraft and ground-based instruments, similar to those used during SCAR-A, were used during SCAR-C. Remote sensing of fires and smoke from AVIRIS and MAS imagers on the ER-2 aircraft was combined with a complete in situ characterization of the aerosol and trace gases from the C-131A aircraft of the University of Washington and the Cesna aircraft from the U.S. Forest Service. The comprehensive data base acquired during SCAR-A and SCAR-C will contribute to a better understanding of the role of clouds and aerosols in global change studies. The data will also be used to develop satellite remote sensing algorithms from MODIS on the Earth Observing System.

Gao, Bo-Cai↗
NASA NTRS2012

On the Ice Nucleation Spectrum

This work presents a novel formulation of the ice nucleation spectrum, i.e. the function relating the ice crystal concentration to cloud formation conditions and aerosol properties. The new formulation is physically-based and explicitly accounts for the dependency of the ice crystal concentration on temperature, supersaturation, cooling rate, and particle size, surface area and composition. This is achieved by introducing the concepts of ice nucleation coefficient (the number of ice germs present in a particle) and nucleation probability dispersion function (the distribution of ice nucleation coefficients within the aerosol population). The new formulation is used to generate ice nucleation parameterizations for the homogeneous freezing of cloud droplets and the heterogeneous deposition ice nucleation on dust and soot ice nuclei. For homogeneous freezing, it was found that by increasing the dispersion in the droplet volume distribution the fraction of supercooled droplets in the population increases. For heterogeneous ice nucleation the new formulation consistently describes singular and stochastic behavior within a single framework. Using a fundamentally stochastic approach, both cooling rate independence and constancy of the ice nucleation fraction over time, features typically associated with singular behavior, were reproduced. Analysis of the temporal dependency of the ice nucleation spectrum suggested that experimental methods that measure the ice nucleation fraction over few seconds would tend to underestimate the ice nuclei concentration. It is shown that inferring the aerosol heterogeneous ice nucleation properties from measurements of the onset supersaturation and temperature may carry significant error as the variability in ice nucleation properties within the aerosol population is not accounted for. This work provides a simple and rigorous ice nucleation framework where theoretical predictions, laboratory measurements and field campaign data can be reconciled, and that is suitable for application in atmospheric modeling studies.

Barahona, D.↗
NASA NTRS2012

Presolar Organic Globules in Astromaterials

Presolar grains were identified in meteorite residues 20 years ago based on their exotic isotopic compositions [1]. Their study has provide new insights into stellar evolution and the first view of the original building blocks of the solar system. Organic matter in meteorites and IDPs is highly enriched in D/H and N-15/N-14 at micron scales, possibly due to presolar organic grains [2-4]. These anomalies are ascribed to the partial preservation of presolar cold molecular cloud material. Identifying the carriers of these anomalies and elucidating their physical and chemical properties may give new views of interstellar chemistry and better understanding of the original components of the protosolar disk. However, identifying the carriers has been hampered by their small size and the inability to chemically isolate them. Thanks to major advances in nano-scale analytical techniques and advanced sample preparation, we were able to show that in the Tagish Lake meteorite, the principle carriers of these isotopic anomalies are sub-microns, hollow organic globules [5]. The organic globules likely formed by photochemical processing of organic ices in a cold molecular cloud or the outermost regions of the protosolar disk [5]. Organic globules with similar physical, chemical, and isotopic properties are also recently found from Bells CM2 carbonaceous chondrite, in IDPs [6] and in the comet Wild-2 samples returned by Stardust [7]. These results support the view that microscopic organic grains were widespread constituents of the protoplanetary disk. Their exotic isotopic compositions trace their origins to the outermost portions of the protosolar disk or a presolar cold molecular cloud.

Nakamura-Messenger, K.↗
NASA NTRS1993

The embedded young stars in the Taurus-Auriga molecular cloud. I - Models for spectral energy distributions

We describe radiative transfer calculations of infalling, dusty envelopes surrounding pre-main-sequence stars and use these models to derive physical properties for a sample of 21 heavily reddened young stars in the Taurus-Auriga molecular cloud. The density distributions needed to match the FIR peaks in the spectral energy distributions of these embedded sources suggest mass infall rates similar to those predicted for simple thermally supported clouds with temperatures about 10 K. Unless the dust opacities are badly in error, our models require substantial departures from spherical symmetry in the envelopes of all sources. These flattened envelopes may be produced by a combination of rotation and cavities excavated by bipolar flows. The rotating infall models of Terebey et al. (1984) models indicate a centrifugal radius of about 70 AU for many objects if rotation is the only important physical effect, and this radius is reasonably consistent with typical estimates for the sizes of circumstellar disks around T Tauri stars.

Kenyon, Scott J.↗
NASA NTRS2004

Characterization of Individual Aerosol Particles Associated with Clouds (CRYSTAL-FACE)

The aim of our research was to obtain data on the chemical and physical properties of individual aerosol particles from near the bottoms and tops of the deep convective systems that lead to the generation of tropical cirrus clouds and to provide insights into the particles that serve as CCN or IN. We used analytical transmission electron microscopy (ATEM), including energy-dispersive X-ray spectrometry (EDS) and electron energy-loss spectroscopy (EELS), and field-emission electron microscopy (FESEM) to compare the compositions, concentrations, size distributions, shapes, surface coatings, and degrees of aggregation of individual particles from cloud bases and the anvils near the tropopause. Aggregates of sea salt and mineral dust, ammonium sulfate, and soot particles are abundant in in-cloud samples. Cirrus samples contain many H2SO4 droplets, but acidic sulfate particles are rare at the cloud bases. H2SO4 probably formed at higher altitudes through oxidation of SO2 in cloud droplets. The relatively high extent of ammoniation in the upper troposphere in-cloud samples appears to have resulted from vertical transport by strong convection. The morphology of H2SO4 droplets indicates that they had been at least yartiy ammoniated at the time of collection. They are internally mixed with organic materials, metal sulfates, and solid particles of various compositions. Ammoniation and internal mixing of result in freezing at higher temperature than in pure H2SO4 aerosols. K- and S-bearing organic particles and Si-Al-rich particles are common throughout. Sea salt and mineral dust were incorporated into the convective systems from the cloud bases and worked as ice nuclei while being vertically transported. The nonsulfate particles originated from the lower troposphere and were transported to the upper troposphere and lower stratosphere.

Buseck, Peter R.↗
NASA NTRS2009

Presolar Organic Globules in Tagish Lake Meteorite, and other Astromaterials

Presolar grains were identified in meteorite residues 20 years ago based on their exotic isotopic compositions. Their study has provide new insights into stellar evolution and the first view of the original building blocks of the solar system. Organic matter in meteorites and IDPs is highly enriched in D/H and N-15/N-14 at micrometer scales, possibly due to presolar organic grains. These anomalies are ascribed to the partial preservation of presolar cold molecular cloud material. Identifying the carriers of these anomalies and elucidating their physical and chemical properties may give new views of interstellar chemistry and better understanding of the original components of the protosolar disk. However, identifying the carriers has been hampered by their small size and the inability to chemically isolate them. Thanks to immediate careful collection of Tagish Lake meteorite specimen, as well as major advances in nano-scale analytical techniques and advanced sample preparation, we were able to show that in the Tagish Lake meteorite, the principle carriers of these isotopic anomalies are sub-micrometer, hollow organic globules. The organic globules likely formed by photochemical processing of organic ices in a cold molecular cloud or the outermost regions of the protosolar disk. Organic globules with similar physical, chemical, and isotopic properties are also recently found from Bells CM2 carbonaceous chondrite, in IDPs and in the comet Wild-2 samples returned by Stardust. These results support the view that microscopic organic grains were widespread constituents of the protoplanetary disk. Their exotic isotopic compositions trace their origins to the outermost portions of the protosolar disk or a presolar cold molecular cloud.

Nakamura-Messenger, K.↗
NASA NTRS1986

Boundary conditions for the paleoenvironment: Chemical and Physical Processes in dense interstellar clouds

The present research includes searches for important new interstellar constituents; observations relevant to differentiating between different models for the chemical processes that are important in the interstellar environment; and coordinated studies of the chemistry, physics, and dynamics of molecular clouds which are the sites or possible future sites of star formation. Recent research has included the detection and study of four new interstellar molecules; searches which have placed upper limits on the abundance of several other potential constituents of interstellar clouds; quantitative studies of comparative molecular abundances in different types of interstellar clouds; investigation of reaction pathways for astrochemistry from a comparison of theory and the observed abundance of related species such as isomers and isotopic variants; studies of possible tracers of energenic events related to star formation, including silicon and sulfur containing molecules; and mapping of physical, chemical, and dynamical properties over extended regions of nearby cold molecular clouds.

Irvine, W. M.↗