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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 163 records · Page 9
All sourcesNASA NTRSDOE OSTI
NASA NTRS2005

The Effect of Asian Dust Aerosols on Cloud Properties and Radiative Forcing from MODIS and CERES

The effects of dust storms on cloud properties and radiative forcing are analyzed over northwestern China from April 2001 to June 2004 using data collected by the Moderate Resolution Imaging Spectroradiometer (MODIS) and Clouds and the Earth's Radiant Energy System (CERES) instruments on the Aqua and Terra satellites. On average, ice cloud effective particle diameter, optical depth and ice water path of the cirrus clouds under dust polluted conditions are 11%, 32.8%, and 42% less, respectively, than those derived from ice clouds in dust-free atmospheric environments. The humidity differences are larger in the dusty region than in the dust-free region, and may be caused by removal of moisture by wet dust precipitation. Due to changes in cloud microphysics, the instantaneous net radiative forcing is reduced from -71.2 W/m2 for dust contaminated clouds to -182.7 W/m2 for dust-free clouds. The reduced cooling effects of dusts may lead to a net warming of 1 W/m2, which, if confirmed, would be the strongest aerosol forcing during later winter and early spring dust storm seasons over the studied region.

Huang, Jianping↗
NASA NTRS1974

An aerodynamic study of scramjet fuel injectors

The aerodynamic drag and fuel distribution patterns of injectors designed for a supersonic combustion ramjet were measured at Mach numbers of 2, 2.5, and 3. The most significant parameter effecting the drag was found to be the injector thickness ratio. A twofold reduction in the thickness ratio caused a 65% decrease in drag. Changing the injector sweep angle by a factor of 2 resulted in only a small change in drag. A reversal of injector sweep, from sweepback to sweepforward, did not change the measured drag. Helium gas was injected through the struts to simulate the penetration and spreading patterns of hydrogen. Sampling measurements were made at approximately two duct heights downstream of the combustor. The spacing required between fuel injectors was found to be about 10 jet diameters. The effect of gas injection on the measured drag was found to be minor.

Povinelli, L. A.↗
NASA NTRS1974

An aerodynamic study of scramjet fuel injectors

The aerodynamic drag and fuel distribution patterns of injectors designed for a supersonic combustion ramjet were measured at Mach numbers of 2, 2.5, and 3. The most significant parameter effecting the drag was found to be the injector thickness ratio. A two-fold reduction in the thickness ratio caused a 65 percent decrease in drag. Changing the injector sweep angle a factor of 2 resulted in only a small change in drag. A reversal of injector sweep, from sweepback to sweepforward, did not change the measured drag. Helium gas was injected through the struts to simulate the penetration and spreading patterns of hydrogen. Sampling measurements were made at approximately 2 duct heights downstream of the combustor. The spacing required between fuel injectors was found to be about 10 jet diameters. The effect of gas injection on the measured drag was found to be minor.

Povinelli, L. A.↗
DOE OSTI2022

Size-Dependent Adsorption and Adhesion Energetics of Ag Nanoparticles on Graphene Films on Ni(111) by Calorimetry

Interest in the use of carbon supports for late transition metal nanoparticle catalysts has expanded rapidly due to the increasing importance of electrocatalysts for clean energy and environmental technologies and the use and storage of renewable electricity. Compared to oxide supports, almost nothing is known about the effect of metal nanoparticle size on the energies of the metal atoms within carbon-supported nanoparticles, yet these energies are crucial for understanding their surface reactivity and sintering kinetics. Here, the growth morphology and adsorption energetics of vapor-deposited Ag onto clean graphene/Ni(111) surfaces have been studied using a combination of single-crystal adsorption calorimetry (SCAC) and He + low-energy ion scattering (LEIS). The differential heat of Ag adsorption is 207 kJ/mol for making ~30 atom Ag particles on graphene terraces at 100 K and 16 kJ/mol higher for making ~9 atom Ag clusters at defect sites at the same temperature. The heat of adsorption increases rapidly with Ag coverage as 3D Ag nanoparticles nucleate and grow in size, asymptotically reaching within 5 kJ/mol of the bulk Ag sublimation enthalpy (285 kJ/mol) by 2 ML. The heats of adsorption and Ag nanoparticle densities from LEIS (~10 16 /m 2 ) were combined to provide the Ag/graphene adhesion energy (E adh = 1.8 J/m 2 in the large-particle limit) and the Ag chemical potential (μ) versus effective particle diameter (D). The Ag chemical potential was well-fitted by μ(D) = (3γ v /M – E adh )(1 + (1.5 nm)/D)(2V m /D), where γ v /M is the surface energy of bulk Ag and V m is its molar volume. The same equation is known to fit similar data for late transition metals on clean surfaces of metal oxide single crystals. The adhesion energy of Ag measured here on graphene falls within the wide range measured for Ag on those oxide surfaces and is almost as large as on the oxide that binds Ag particles most strongly, namely CeO 2 (111), which is well-known to be very effective at resisting catalyst deactivation by metal sintering. Furthermore, these results imply that carbon supports will be effective at resisting sintering and that Ag particles smaller than 6 nm on graphene will bind small adsorbed reaction intermediates more weakly than supports with weaker adhesion to Ag, like MgO(100).

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Molecular speciation controls arsenic and lead bioaccessibility in fugitive dusts from sulfidic mine tailings

Communities nearby mine wastes in arid and semi-arid regions are potentially exposed to high concentrations of toxic metal(loid)s from fugitive dusts deriving from impoundments. To assess the relation between potentially lofted particles and human health risk, we studied the relationship between pharmacokinetic bioaccessibility and metal(loid) molecular speciation for mine tailings dust particulate matter (PM), with elevated levels of arsenic and lead (up to 59 and 34 mmol kg -1 , respectively), by coupling in vitro bioassay (IVBA) with X-ray absorption spectroscopy (XAS). Mine tailing efflorescent salts (PM ES ) and PM from the surface crust (0–1 cm, PM SC ) and near surface (0–25 cm) were isolated to <10 μm and <150 μm effective spherical diameter (PM 10 and PM 150 ) and reacted with synthetic gastric and lung fluid for 30 s to 100 h to investigate toxic metal(loid) release kinetics. Bioaccessible (BAc) fractions of arsenic and lead were about 10 and 100 times greater in gastric than in lung fluid simulant, respectively, and 10–100% of the maximum gastric BAc from PM 10 and PM 150 occurred within 30 s, with parabolic dissolution of fine, highly-reactive particles followed by slower release from less soluble sources. Evaporite salts were almost completely solubilized in gastric-fluid simulants. Arsenate within jarosite and sorbed to ferrihydrite, and lead from anglesite, were identified by XAS as the principal contaminant sources in the near surface tailings. In the synthetic lung fluid, arsenic was released continuously to 100 h, suggesting that residence time in vivo must be considered for risk determination. Analysis of pre- and post-IVBA PM indicated the release of arsenic in lung fluid was principally from arsenic-substituted jarosite, whereas in synthetic gastric fluid arsenic complexed on ferrihydrite surfaces was preferentially released and subsequently repartitioned to jarosite-like coordination at extended exposures. Lead dissolved at 30 s was subsequently repartitioned back to the solid phase as pyromorphite in phosphate rich lung fluid. The bioaccessibility of lead in surface tailings PM was limited due to robust sequestration in plumbojarosite. Kinetic release of toxic elements in both synthetic biofluids indicated that a single IVBA interval may not adequately describe release dynamics.

63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTAN↗
DOE OSTI2020

Light scattering study of highly absorptive, non-fractal, hematite aggregates

In this paper, we present measurements of the scattered light intensity by aerosolized hematite aggregate particles. The measurements were made at a wavelength of 532 nm in the scattering angle range from 0.32° to 157°. Hematite has high values of the real and imaginary parts of the refractive index m = n + iκ = 3 + i0.5 at the studied wavelength. Scanning electron micrographs (SEM) indicated that the particles were aggregates whereas the optical microscope pictures showed that the aerosol had a bimodal distribution with effective mean diameters of roughly 1 and 10 µm. This is consistent with the light scattering results which displayed two Guinier regimes. The aggregates were composed of smaller grains with an approximate size of 200 nm. Ultra Small-Angle X-ray Scattering (USAXS) indicate that the aggregates were uniform and non-fractal. Mie calculations for a sphere equivalent to the aggregate size were compared to the experimentally observed results. The observed results showed an enhanced backscattering, whereas the Mie calculations did not due to the large imaginary part of the refractive index. Hematite aggregates were simulated by assuming they were composed of spherical monomers inside a spherical volume. Then the light scattering was calculated using the T-matrix method for these simulated aggregates. The calculated results show an enhanced backscattering. We present a dimensional analysis to estimate the extent of multiple scattering within the aggregate and find a correlation between the average number of scattering events within the aggregate and the enhancement in the backscattering.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

Retrieving microphysical properties of concurrent pristine ice and snow using polarimetric radar observations

Abstract. Ice and mixed-phase clouds play a key role in our climate system because of their strong controls on global precipitation and radiation budget. Their microphysical properties have been characterized commonly by polarimetric radar measurements. However, there remains a lack of robust estimates of microphysical properties of concurrent pristine ice and aggregates because larger snow aggregates often dominate the radar signal and mask contributions of smaller pristine ice crystals. This paper presents a new method that separates the scattering signals of pristine ice embedded in snow aggregates in scanning polarimetric radar observations and retrieves their respective abundances and sizes for the first time. This method, dubbed ENCORE-ice, is built on an iterative stochastic ensemble retrieval framework. It provides the number concentration, ice water content, and effective mean diameter of pristine ice and snow aggregates with uncertainty estimates. Evaluations against synthetic observations show that the overall retrieval biases in the combined total microphysical properties are within 5 % and that the errors with respect to the truth are well within the retrieval uncertainty. The partitioning between pristine ice and snow aggregates also agrees well with the truth. Additional evaluations against in situ cloud probe measurements from a recent campaign for a stratiform cloud system are promising. Our median retrievals have a bias of 98 % in the total ice number concentration and 44 % in the total ice water content. This performance is generally better than the retrieval from empirical relationships. The ability to separate signals of different ice species and to provide their quantitative microphysical properties will open up many research opportunities, such as secondary ice production studies and model evaluations for ice microphysical processes.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1974

Values of the photometric parameters of Mars and their interpretation

Photometric data for the Martian disk obtained by Thorpe from television-camera pictures taken by Mariner 9 were used to derive values for the parameters in the photometric function. The photometric function can be applied to Mars and to the design of cameras for photography of Mars. Values of the parameters are for one wavelength only, 0.56 micros and are average or effective values for the Martian disk. The values derived were interpreted to provide semi-quantitative information on the soil. The results do not disagree with other indications that the effective mean diameter of the surface particles is about 400 micros. Another result is that the mean intercenter spacing of adjacent particles may be about 4/3 of the mean diameter.

Weaver, W. R.↗
NASA NTRS1950

Penetration of Air Jets Issuing from Circular, Square, and Elliptical Orifices Directed Perpendicularly to an Air Stream

An experimental investigation was conducted to determine the penetration of air jets d.irected perpendicularlY to an air stream. Jets Issuing from circular, square, and. elliptical orifices were investigated. and. the jet penetration at a position downstream of the orifice was determined- as a function of jet density, jet velocity, air-stream d.enaity, air-stream velocity, effective jet diameter, and. orifice flow coeffIcient. The jet penetrations were determined for nearly constant values of air-stream density at three tunnel-air velocities arid for a large range of Jet velocities and. densities. The results were correlated in terms of dimensionless parameters and the penetrations of the various shapes were compared. Greater penetration was obtained. with the square orifices and the elliptical orifices having an axis ratio of 4:1 at low tunnel-air velocities and low jet pressures than for the other orifices investigated. The square orifices gave the best penetrations at the higher values of tunnel-air velocity and jet total pressure.

Ruggeri, Robert S.↗
NASA NTRS1982

Magnetospheres and winds of the helium strong stars: Dependence on rotation

Large aperture, low resolution spectra of 24 stars of types 05, 04, and 03 were obtained, and from these the energy distribution between 1200 and 3200 angstrom was derived in absolute units. The energies were combined with energies deduced from uvby and UBV photometry and corrected for interstellar extinction. Angular diameters and effective temperatures are also derived. The effective temperatures range from 24800K to 63000K. There is no correlation between effective temperature and spectral type or luminosity class for the early 0 stars. The size of the expected errors are also studied.

Barker, P. K.↗
NASA NTRS1981

Spectral inversion of radio signals scattered from Saturn's rings

Favorable alignment of contours of constant Doppler frequency with the ringlets that comprise Saturn's ring system formed the basis of an inversion technique that recovered the radar cross-section with radial resolution reaching 1000 km from an experiment carried out by the Voyager 1 spacecraft. The radar cross-section, together with measurements of the direct signal extinction, lead to estimates of effective particle diameters of 2, 8, and 10 meters for ringlets within ring C, Cassini division, and ring A, respectively.

Marouf, E. A.↗
NASA NTRS1987

AC impedance analysis of polypyrrole thin films

The AC impedance spectra of thin polypyrrole films were obtained at open circuit potentials from -0.4 to 0.4 V vs SCE. Two limiting cases are discussed for which simplified equivalent circuits are applicable. At very positive potentials, the predominantly nonfaradaic AC impedance of polypyrrole is very similar to that observed previously for finite porous metallic films. Modeling of the data with the appropriate equivalent circuit permits effective pore diameter and pore number densities of the oxidized film to be estimated. At potentials from -0.4 to -0.3 V, the polypyrrole film is essentially nonelectronically conductive and diffusion of polymer oxidized sites with their associated counterions can be assumed to be linear from the film/substrate electrode interface. The equivalent circuit for the polypyrrole film at these potentials is that previously described for metal oxide, lithium intercalation thin films. Using this model, counterion diffusion coefficients are determined for both semi-infinite and finite diffusion domains. In addition, the limiting low frequency resistance and capacitance of the polypyrrole thin fims was determined and compared to that obtained previously for thicker films of the polymer. The origin of the observed potential dependence of these low frequency circuit components is discussed.

Penner, Reginald M.↗
NASA NTRS1989

Flow boiling with enhancement devices for cold plate coolant channel design

A research program to study the effect of enhancement devices on flow boiling heat transfer in coolant channels, which are heated either from the top side or uniformly, is discussed. Freon 11 is the working fluid involved. The specific objectives are: (1) examine the variations in both the mean and local (axial and circumferential) heat transfer coefficients for a circular coolant channel with either smooth walls or with both a twisted tape and spiral finned walls, (2) examine the effect channel diameter (and the length-to-diameter aspect ratio) variations for the smooth wall channel, and (3) develop an improved data reduction analysis.

Boyd, Ronald D., Sr.↗
NASA NTRS1989

Effects of cardiac phase on diameter measurements from coronary cineangiograms

The measurement variability of end-diastolic frames is compared with frames taken from the other portions of the cardiac cycle. Two computer measurements, average diameter and minimum, are obtained for every frame of two complete cardiac cycles in angiograms of 20 subjects. Six schemes for sampling frames in various portions of the cardiac cycle are defined and the standard deviation is calculated for pairs of measurements from each scheme. The results suggest that the best strategy for frame selection is to use sequential frames in end-diastole. However, it is noted that if random samples are taken anywhere in the cardiac cycle instead of sequentially in end-diastole, the variability of two vessel edge measures changes from 4.9 percent to 6.3 percent, which is considered to be a small penalty.

Selzer, Robert H.↗
NASA NTRS1990

Structures observed on the spot radiance fields during the FIRE experiment

Three Spot images taken during the FIRE experiment on stratocumulus are analyzed. From this high resolution data detailed observations of the true cloud radiance field may be made. The structure and inhomogeneity of these radiance fields hold important implications for the radiation budget, while the fine scale structure in radiance field provides information on cloud dynamics. Wieliki and Welsh, and Parker et al., have quantified the inhomogeneities of the cumulus clouds through a careful examination of the distribution of cloud (and hole) size as functions of an effective cloud diameter and radiance threshold. Cahalan (1988) has compared for different cloud types of (stratocumulus, fair weather cumulus, convective clouds in the ITCZ) the distributions of clouds (and holes) sizes, the relation between the size and the perimeter of these clouds (and holes), and examining the possibility of scale invariance. These results are extended from LANDSAT resolution (57 m and 30 m) to the Spot resolution (10 m) resolution in the case of boundary layer clouds. Particular emphasis is placed on the statistics of zones of high and low reflectivity as a function of a threshold reflectivity.

Seze, Genevieve↗