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At least 163 records · Page 9

Strong Constraints on Aerosol-Cloud Interactions from Volcanic Eruptions

Aerosols have a potentially large effect on climate, particularly through their interactions with clouds, but the magnitude of this effect is highly uncertain. Large volcanic eruptions produce sulfur dioxide, which in turn produces aerosols; these eruptions thus represent a natural experiment through which to quantify aerosol-cloud interactions. Here we show that the massive 2014-2015 fissure eruption in Holuhraun, Iceland, reduced the size of liquid cloud droplets - consistent with expectations - but had no discernible effect on other cloud properties. The reduction in droplet size led to cloud brightening and global-mean radiative forcing of around minus 0.2 watts per square metre for September to October 2014. Changes in cloud amount or cloud liquid water path, however, were undetectable, indicating that these indirect effects, and cloud systems in general, are well buffered against aerosol changes. This result will reduce uncertainties in future climate projections, because we are now able to reject results from climate models with an excessive liquid-water-path response.

atmospheric science↗

Polarized View of Supercooled Liquid Water Clouds

Supercooled liquid water (SLW) clouds, where liquid droplets exist at temperatures below 0 C present a well known aviation hazard through aircraft icing, in which SLW accretes on the airframe. SLW clouds are common over the Southern Ocean, and climate-induced changes in their occurrence is thought to constitute a strong cloud feedback on global climate. The two recent NASA field campaigns POlarimeter Definition EXperiment (PODEX, based in Palmdale, California, January-February 2013) and Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS, based in Houston, Texas in August- September 2013) provided a unique opportunity to observe SLW clouds from the high-altitude airborne platform of NASA's ER-2 aircraft. We present an analysis of measurements made by the Research Scanning Polarimeter (RSP) during these experiments accompanied by correlative retrievals from other sensors. The RSP measures both polarized and total reflectance in 9 spectral channels with wavelengths ranging from 410 to 2250 nm. It is a scanning sensor taking samples at 0.8deg intervals within 60deg from nadir in both forward and backward directions. This unique angular resolution allows for characterization of liquid water droplet size using the rainbow structure observed in the polarized reflectances in the scattering angle range between 135deg and 165deg. Simple parametric fitting algorithms applied to the polarized reflectance provide retrievals of the droplet effective radius and variance assuming a prescribed size distribution shape (gamma distribution). In addition to this, we use a non-parametric method, Rainbow Fourier Transform (RFT),which allows retrieval of the droplet size distribution without assuming a size distribution shape. We present an overview of the RSP campaign datasets available from the NASA GISS website, as well as two detailed examples of the retrievals. In these case studies we focus on cloud fields with spatial features varying between glaciated and liquid phases at altitudes as high as 10 km, which correspond to temperatures close to the homogeneous freezing temperature of pure water drops (about -35 C or colder). The multimodal droplet size distributions retrieved from RSP data in these cases are consistent with the multi-layer cloud structure observed by correlative Cloud Physics Lidar (CPL) measurements.

Clouds↗

Pyrolysis of Large Black Liquor Droplets

This paper presents the results of experiments involving the pyrolysis of large black liquor droplets in the NASA KC-135 reduced gravity aircraft. The reduced gravity environment facilitated the study of droplets up to 9 mm in diameter extending the results of previous studies to droplet sizes that are similar to those encountered in recovery boilers. Single black liquor droplets were rapidly inserted into a 923 K oven. The primary independent variables were the initial droplet diameter (0.5 mm to 9 mm), the black liquor solids content (66.12% - 72.9% by mass), and the ambient oxygen mole fraction (0.0 - 0.21). Video records of the experiments provided size and shape of the droplets as a function of time. The results show that the particle diameter at the end of the drying stage (D(sub DRY) ) increases linearly with the initial particle diameter (D(sub O)). The results further show that the ratio of the maximum swollen diameter (D(sub MAX)) to D(sub O) decreases with increasing D(sub O) for droplets with D(sub O) less than 4 mm. This ratio was independent of D(sub O) for droplets with D(sub O) greater than 4 mm. The particle is most spherical at the end of drying, and least spherical at maximum swollen size, regardless of initial sphericity and droplet size.

Bartkus, Tadas P.↗

Pyrolysis of Large Black Liquor Droplets

This paper presents the results of experiments involving the pyrolysis of large black liquor droplets in the NASA KC-135 reduced gravity aircraft. The reduced gravity environment facilitated the study of droplets up to 9 mm in diameter extending the results of previous studies to droplet sizes that are similar to those encountered in recovery boilers. Single black liquor droplets were rapidly inserted into a 923 K oven. The primary independent variables were the initial droplet diameter (0.5 mm to 9 mm), the black liquor solids content (66.12% - 72.9% by mass), and the ambient oxygen mole fraction (0.0 - 0.21). Video records of the experiments provided size and shape of the droplets as a function of time. The results show that the particle diameter at the end of the drying stage (D(sub DRY)) increases linearly with the initial particle diameter (D(sub O)). The results further show that the ratio of the maximum swollen diameter (D(sub MAX)) to D(sub O) decreases with increasing D(sub O) for droplets with D(sub O) less than 4 mm. This ratio was independent of D(sub O) for droplets with D(sub O) greater than 4 mm. The particle is most spherical at the end of drying, and least spherical at maximum swollen size, regardless of initial sphericity and droplet size.

Bartkus, Tadas P.↗

Collective effects of temperature gradients and gravity on droplet coalescence

The interaction and coalescence of small spherical drops in dilute, homogeneous dispersions are considered theoretically under conditions, where drop motion results from gravity settling and thermocapillary migration acting simultaneously. A trajectory analysis is used to predict pairwise collision rates, and population dynamics equations are solved to predict the time evolution of the droplet size distribution. The rate of droplet collisions and growth may be reduced dramatically by antiparallel alignment of the gravitational and thermocapillary velocities. For such antiparallel alignment with the gravitational relative velocity exceeding the thermocapillary relative velocity for two widely separated drops, there is a 'collision-forbidden region' in parameter space. This occurs because the gravitational relative velocity decays more rapidly with decreasing separation distance between the drops than does the thermocapillary relative velocity, and so the resultant relative velocity along the line-of-centers from these two sources combined becomes zero at a finite separation and the drops are unable to collide. As a result, small drops which initially collide and coalesce due to thermocapillary motion will only grow until they reach a critical size for which the oppositely directed gravitational motion balances the thermocapillary motion.

Zhang, Xiaoguang↗

An Investigation Into Some Important Aspects of Droplet Breakup/Vaporization Behavior Caused By a Gas Flow (Both Nonreacting & Detonative Combustion) in a Shock Tube

As a part of the rotating detonation engine (RDE) technology enablement project at NASA Glenn Research Center (GRC), an effort was undertaken to extend our current computational capabilities of OpenNCC in some important ways with the implementation of a modeling approach to account for the droplet breakup caused by a shock-induced gas motion, & a vaporization model valid over a wide range of pressure conditions encountered in multiphase detonation. With the modified code, a study was undertaken to investigate the individual droplet behavior followed by the passage of a shock front. The study is carried out by tracking a sparse group of droplets to gain some understanding of shock induced droplet behavior under various shock strengths & fuel injector conditions. The study also looks into the effect of randomization involved in determining the droplet breakup outcomes. Over a wide range of sub-critical conditions examined, larger droplets are observed to undergo significant changes in droplet behavior following their breakup. However, smaller droplets (10 µm or less ) remain unaffected by any shock induced breakup. In a follow-on work, we investigated the impact of shock and droplet interaction in a detonation study involving both gaseous as well as gas/liquid (droplet clouds) fuel/air stoichiometric mixtures in a simple 3D shock-tube configuration. The droplet clouds are made up of different initial droplet sizes of either 6, 10, or 30 µm. We also investigated the individual droplet behavior followed by the passage of a detonation front. The results represent conditions that lead to both overdriven and C-J (ChapmanJouguet) detonations. Under both test conditions, most of the droplet vaporization is completed within a short distance (duration) behind the detonation front & well within the region of complete combustion observed in a corresponding equivalent gas-phase fuel/air mixture. The impact of the shock-induced droplet breakup is found to be significant in the calculations involving the 30-µm droplets. Subsequent to the breakup, the drop sizes vary from 1 to 10 µm. Another factor that contributed to the observed rapid vaporization is the result of vaporization taking place under supercritical conditions. The overall detonation properties of various droplet clouds (made up of different initial sizes) are similar to those observed in a corresponding gaseous fuel/air mixture. In the calculation involving a gaseous fuel, the calculated C-J detonation velocity is 1822 m/s involving Jet-A/air and φ = 1. In the overdriven detonation, it is 2044 m/s. In the calculations involving droplet clouds, the corresponding detonation velocities are lower. The impact of increased droplet size is primarily seen in a higher reduction in the detonation velocity.

shock/droplet interaction↗

Containerless Processing of Undercooled Melts

The physical mechanisms controlling liquid undercooling were studied for application to solidification processing methods. The undercooling potential of containerless processing was assessed on droplet samples of high melting temperature metals drop tube and drop tower facilities and in a laboratory-scale apparatus. New insight into nucleation and crystal growth will be obtained in undercooled liquids of high melting temperature iron and nickel-base systems. The processing parameters include melt superheat, droplet size and particle statistics and droplet surface coating. The solidification behavior is determined by thermal analysis and by structural and metallographic characterization.

Perepezko, J. H.↗

Theory of Ostwald ripening in a two-component system

When a two-component system is cooled below the minimum temperature for its stability, it separates into two or more immiscible phases. The initial nucleation produces grains (if solid) or droplets (if liquid) of one of the phases dispersed in the other. The dynamics by which these nuclei proceed toward equilibrium is called Ostwald ripening. The dynamics of growth of the droplets depends upon the following factors: (1) The solubility of the droplet depends upon its radius and the interfacial energy between it and the surrounding (continuous) phase. There is a critical radius determined by the supersaturation in the continuous phase. Droplets with radii smaller than critical dissolve, while droplets with radii larger grow. (2) The droplets concentrate one component and reject the other. The rate at which this occurs is assumed to be determined by the interdiffusion of the two components in the continuous phase. (3) The Ostwald ripening is constrained by conservation of mass; e.g., the amount of materials in the droplet phase plus the remaining supersaturation in the continuous phase must equal the supersaturation available at the start. (4) There is a distribution of droplet sizes associated with a mean droplet radius, which grows continuously with time. This distribution function satisfies a continuity equation, which is solved asymptotically by a similarity transformation method.

Baird, J. K.↗

Particle size and velocity measurement in flames by laser anemometer

Simultaneous droplet size and velocity measurements by a particle counting Laser Doppler Anemometer (LDA) in kerosene fuel sprays under burning and non-burning conditions are presented. Particle sizes are derived from pulse height analysis of the mean LDA signals and velocities are simultaneously determined by measuring Doppler shift frequencies. The measurements show that droplet velocity is a function of droplet diameter for burning and non-burning conditions, and spatially averaged size distributions are derived from velocity data. A comparison of results obtained under burning and non-burning conditions show changes in size distribution due to preferential vaporization of small droplets, acceleration due to thermal expansion of gases, and corresponding changes in droplet momentum.

Chigier, N. A.↗

The effects of van der Waals attractions on cloud droplet growth by coalescence

The inclusion of van der Waals attractions in the interaction between cloud droplets has been recently shown to significantly increase the collision efficiencies of the smaller droplets. In the current work, these larger values for the collision efficiencies are used in a population dynamics model of the droplet size distribution evolution with time, in hopes of at least partially resolving the long-standing paradox in cloud microphysics that predicted rates of the onset of precipitation are generally much lower than those which are observed. Evolutions of several initial cloud droplet spectra have been tracked in time. Size evolutions are compared as predicted from the use of collision efficiencies computed using two different models to allow for droplet-droplet contact: one which considers slip flow effects only, and one which considers the combined effects of van der Waals forces and slip flow. The rate at which the droplet mass density function shifts to larger droplet sizes is increased by typically 20-25 percent, when collision efficiencies which include van der Waals forces are used.

Rogers, Jan R.↗

Wind Tunnel PSD and MVD Characterization Using New 1D2D Optical Array Probes

This work explores characterization of the liquid clouds using a combination of a forward scattering probe and two Optical Array Probes. Current OAP probes provide particle shape, size, and number concentration from two-dimensional shadow images. However, past studies have shown that such images are subject to distortion when outside of the focal plane. This affects the retrieval of particle size distributions, particularly in the Supercooled Large Droplet size range. In this article, the use of a Droplet Measurement Technologies Cloud Droplet Probe and two new OAPs produced by Science Engineering Associates, is examined using wind tunnel data, to assess suitability for use in a wind tunnel calibration in SLD conditions. The new OAP probes exploit a flexible and simple grey scale imaging method to eliminate some present shortcomings of commonly used OAPs, and to reduce correction factors. Spinning disk measurements were used to specify probe depth of field, and average size errors. Composite spectra covering the nominal 2-3200 µm size range were formed by crossing over from the CDP to 1D2D-X at 48 µm, and then to the 1D2D-Y at about 400 µm. A good overlap was found at the crossover points without any artificial scaling. Composite spectra adequately closed the liquid water content distribution, and provided integrated LWCs within about 35% of the hot-wire LWCs used for tunnel calibration. This discrepancy was at least partially attributed to LWC underestimation by the hot-wire at high MVD. A model of probe performance was used to show an example of expected accuracy of ideal probes subject to the same OAP distortions and using the same mitigating procedures and corrections, predicting PSD Median Volume Diameter and integrated LWC errors of less than 10%.

Aircraft Icing↗

Acid rain: Microphysical model

A microphysical model was used to simulate the case of a ground cloud without dilution by entrainment and without precipitation. The numerical integration techniques of the model are presented. The droplet size spectra versus time and the droplet molalities for each value of time are discussed.

Dingle, A. N.↗

Coaxial injector spray characterization using water/air as simulants

Quantitative information about the atomization of injector sprays is required to improve the accuracy of computational models that predict the performance and stability of liquid propellant rocket engines. An experimental program is being conducted at NASA-Lewis to measure the drop size and velocity distributions in shear coaxial injector sprays. A phase/Doppler interferometer is used to obtain drop size data in water air shear coaxial injector sprays. Droplet sizes and axial component of droplet velocities are measured at different radii for various combinations of water flow rate, air flow rate, injector liquid jet diameter, injector annular gap, and liquid post recess. Sauter mean diameters measured in the spray center 51 mm downstream of the liquid post tip range from 28 to 68 microns, and mean axial drop velocities at the same location range from 37 to 120 m/s. The shear coaxial injector sprays show a high degree of symmetry; the mean drop size and velocity profiles vary with liquid flow rate, post recess, and distance from the injector face. The drop size data can be used to estimate liquid oxygen/hydrogen spray drop sizes by correcting property differences between water-air and liquid oxygen/hydrogen.

Zaller, Michelle M.↗

RSP Data Status, Updates and Plans from the Team

•All radiance (L1C), aerosol and cloud (L2) products are in the archive. •Revised calibration performed at GSFC in July 2021 applied to reprocessing. •Clouds have smaller drops and higher optical depths (larger droplet number concentrations) in winter than in summer. Cloud top droplet size distributions tend to be narrow with roughly 80% having an effective variance of less than 0.07. This is relevant to how well bulk auto-conversion parameterizations are likely to work at cloud top (order of magnitude effects) and also to assumptions used in the remote sensing of droplet number (~ 10% effect). Real refractive index and effective radius retrievals are consistent with hygroscopic growth of aerosols Real refractive index and effective variance retrievals imply the presence of an insoluble fraction of aerosols Future work on clouds will look at differences in cloud top drizzle formation and auto-conversion rates between the different campaigns and at how well mixed phase clouds can be detected (if at all) from sensors such as VIIRS and PACE OCI.

Research Scanning Polarimeter↗

Icing Sensor Probe

Aircraft icing is a serious safety problem for the general aviation and some commuter transport airplanes. There has been tremendous growth in the commuter aviation industry in the last few years, Since these type of aircraft generally operate at lower altitudes they consequently spend a far greater proportion of their time operating in icing conditions. For the past thirty years airborne and ground based facilities have relied primarily on two types of cloud physics instrumentation to measure the characteristics of icing clouds: hot wire liquid water content probes and laser based particle sizing probes for the measurement of water droplet size. The instrumentation is severely limited by the technology that was developed during the 1970's and is quite large in size. The goal of this research is to develop one instrument with a wide bandwidth, better response time, higher resolution, user selectability, and small and lightweight. NASA Glenn Research Center, Droplet Measurement Technology, and Meteorology Society of Canada have developed a collaborative effort to develop such an instrument. This paper describes the development and test results of the prototype Icing Sensor Probe.

Emery, Edward↗

Holographic studies of the vapor explosion of vaporizing water-in-fuel emulsion droplets

Holographic studies were performed which examined the fragmentation process during vapor explosion of a water-in-fuel (hexadecane/water) emulsion droplet. Holograms were taken at 700 to 1000 microseconds after the vapor explosion. Photographs of the reconstructed holograms reveal a wide range of fragment droplet sizes created during the explosion process. Fragment droplet diameters range from below 10 microns to over 100 microns. It is estimated that between ten thousand and a million fragment droplets can result from this extremely violent vapor explosion process. This enhanced atomization is thus expected to have a pronounced effect on vaporization processes which are present during combustion of emulsified fuels.

Sheffield, S. A.↗

Pre-existing seed particles and the onset of condensation in cryogenic wind tunnels

The condensation research at NASA Langley Research Center has used a variety of experimental approaches to gather information on seed particles that can act as sites for condensation growth. Total pressure measurements have suggested that condensation growth is caused by impurities in the flow and not by unevaporated liquid nitrogen (LN2) droplets resulting from the LN2 injected to cool the 0.3-Meter Transonic Cryogenic Tunnel. A separate test with an optical droplet sizing probe, which was designed to detect droplets in the 2- to 300-micron range, confirmed the conclusions from the total pressure measurements and also discovered what appears to be solidified oil droplets having diameters of about 3 microns. These oil droplets appear to be the dominant source of seed particles above 2 microns. However, computer simulations of static pressure test data suggest that the measured condensation effects are the result of more numerous, smaller seeds with number densities on the order of 10 to the 12th per kilogram of the gas and diameters on the order of 0.5 microns.

Hall, R. M.↗

Optical measurement systems

Some of the areas of research conducted at Lewis on optical measurement techniques are described. Two laser anemometer systems developed at Lewis are used to illustrate the special instrumentation needs encountered in aeropropulsion research. Velocity measurements to be made through small viewing ports, close to surfaces within the propulsion system components, and in turbulent or highly-accelerating flows are some of the significant challenges. The application to research facilities of two advanced optical systems, the rainbow schlieren and the combustor viewing system, is presented. The calibration and verification of commercial optical measuring systems, such as droplet sizing systems, are also discussed. Calibration techniques capable of simulating moving droplets for flight-type sizing systems are being developed at Lewis. The presentation concludes with a brief look at the forces driving future research on optical instrumentation.

Lesco, Daniel J.↗