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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 163 records · Page 9
All sourcesNASA NTRSDOE OSTI
NASA NTRS1997

Comparison of Ice Cloud Particle Sizes Retrieved from Satellite Data Derived from In Situ Measurements

Cloud microphysical parameterizations have attracted a great deal of attention in recent years due to their effect on cloud radiative properties and cloud-related hydrological processes in large-scale models. The parameterization of cirrus particle size has been demonstrated as an indispensable component in the climate feedback analysis. Therefore, global-scale, long-term observations of cirrus particle sizes are required both as a basis of and as a validation of parameterizations for climate models. While there is a global scale, long-term survey of water cloud droplet sizes (Han et al.), there is no comparable study for cirrus ice crystals. This study is an effort to supply such a data set.

Han, Qingyuan↗
NASA NTRS1988

Mass accommodation coefficient measurements for HNO3, HCl and N2O5 on water, ice and aqueous sulfuric acid droplet surfaces

Preliminary results are reported of the direct measurement of accommodation coefficients for HNO3, N2O5 and HCl on water drops, aqueous sulfuric acid drops and ice particles. The heterogeneous chemistry of these species together with ClONO2 has been implicated in the ozone depletion observed in the Antarctic stratosphere during the spring in the last eight years. The most plausible chemical mechanism involves the removal of nitrogen oxide species via condensation on ice particles in polar stratospheric clouds resulting in a increase in the active chlorine species responsible for the ozone depletion. The observation of low NO2 and high ClO densities in the Antarctic stratosphere last summer appear to be consistent with such a mechanism.

Worsnop, Douglas↗
NASA NTRS2020

Polarimetric Radar Characteristics of Simulated and Observed Intense Convective Cores for a Midlatitude Continental and Tropical Maritime Environment

This study contrasts midlatitude continental and tropical maritime deep convective cores using polarimetric radar observables and retrievals from selected deep convection episodes during the MC3E and TWPICE field campaigns. The continental convective cores produce stronger radar reflectivities throughout the profiles, while maritime convective cores produce more positive differential reflectivity Z(dr) and larger specific differential phase K(dp) above the melting level. Hydrometeor identification retrievals revealed the presence of large fractions of rimed ice particles (snow aggregates) in the continental (maritime) convective cores, consistent with the Z(dr) and K(dp) observations. The regional cloud-resolving model simulations with bulk and size-resolved bin microphysics are conducted for the selected cases, and the simulation outputs are converted into polarimetric radar signals and retrievals identical to the observational composites. Both the bulk and the bin microphysics reproduce realistic land and ocean (L-O) contrasts in reflectivity, polarimetric variables of rain drops, and hydrometeor profiles, but there are still large uncertainties in describing Zdr and Kdp of ice crystals associated with the ice particle shapes/orientation assumptions. Sensitivity experiments are conducted by swapping background aerosols between the continental and maritime environments, revealing that background aerosols play a role in shaping the distinct L-O contrasts in radar reflectivity associated with raindrop sizes, in addition to the dominant role of background thermodynamics.

Toshihisa Matsui↗
NASA NTRS1990

Cirrus microphysics and radiative transfer: Cloud field study on October 28, 1986

The radiative properties of cirrus clouds present one of the unresolved problems in weather and climate research. Uncertainties in ice particle amount and size and, also, the general inability to model the single scattering properties of their usually complex particle shapes, prevent accurate model predictions. For an improved understanding of cirrus radiative effects, field experiments, as those of the Cirrus IFO of FIRE, are necessary. Simultaneous measurements of radiative fluxes and cirrus microphysics at multiple cirrus cloud altitudes allows the pitting of calculated versus measured vertical flux profiles; with the potential to judge current cirrus cloud modeling. Most of the problems in this study are linked to the inhomogeneity of the cloud field. Thus, only studies on more homogeneous cirrus cloud cases promises a possibility to improve current cirrus parameterizations. Still, the current inability to detect small ice particles will remain as a considerable handicap.

Kinne, Stefan↗
NASA NTRS1978

Millimeter wave propagation modeling of inhomogeneous rain media for satellite communications systems

A theoretical propagation model that represents the scattering properties of an inhomogeneous rain often found on a satellite communications link is presented. The model includes the scattering effects of an arbitrary distribution of particle type (rain or ice), particle shape, particle size, and particle orientation within a given rain cell. An associated rain propagation prediction program predicts attenuation, isolation and phase shift as a function of ground rain rate. A frequency independent synthetic storm algorithm is presented that models nonuniform rain rates present on a satellite link. Antenna effects are included along with a discussion of rain reciprocity. The model is verified using the latest available multiple frequency data from the CTS and COMSTAR satellites. The data covers a wide range of frequencies, elevation angles, and ground site locations.

Persinger, R. R.↗
NASA NTRS2006

Percentage Contributions from Atmospheric and Surface Features to Computed Brightness Temperatures

Over the past few years, a few solid precipitation detection and retrieval algorithms have been developed and shown to be applicable for snowing clouds and blizzards. Current precipitating snow retrieval algorithms require the use of millimeter-wave radiometer observations. The millimeter-wave frequencies are especially sensitive to the scattering and emission properties of frozen particles due to the ice particle refractive index. These channels can also be used to discern information about the frozen particles above the melting layer. Passive radiometric channels respond to both the integrated particle mass throughout the volume and field of view, and to the amount, location, and size distribution of the frozen (and liquid) particles with the sensitivity varying for different frequencies and hydrometeor types. This work will show the percentage of the brightness temperature resulting from the liquid hydrometeor, frozen hydrometeor, relative humidity, and surface contributions. The focus will be on precipitating snow events and millimeter-wave frequencies however, other events and frequencies will be included in the analysis.

SkofronickJackson, Gail↗
NASA NTRS2009

Chemical Evolution in the Interstellar Medium: From Astrochemistry to Astrobiology

Great strides have been made in our understanding of interstellar material thanks to advances in infrared astronomy and laboratory astrophysics. Ionized polycyclic aromatic hydrocarbons (PAHs), shockingly large molecules by earlier astrochemical standards, are widespread and very abundant throughout much of the Universe. In cold molecular clouds, the birthplace of planets and stars, interstellar molecules freeze onto dust and ice particles forming mixed molecular ices dominated by simple species such as water, methanol, ammonia, and carbon monoxide. Within these clouds, and especially in the vicinity of star and planet forming regions, these ices and PAHs are processed by ultraviolet light and cosmic rays forming hundreds of far more complex species, some of biogenic interest. Eventually, these are delivered to primordial planets by comets and meteorites. Astrochemical evolution, highlights of this field from a chemist's perspective, and the astronomer's infrared toolbox will be reviewed.

Allamandola, Louis J.↗
NASA NTRS2012

Analysis of Water Extraction From Lunar Regolith

Distribution of water concentration on the Moon is currently an area of active research. Recent studies suggest the presence of ice particles, and perhaps even ice blocks and ice-cemented regolith on the Moon. Thermal extraction of the in-situ water is an attractive means of sa tisfying water requirements for a lunar mission. In this paper, a model is presented to analyze the processes occurring during the heat-up of icy regolith and extraction of the evolved water vapor. The wet regolith is assumed to be present in an initially evacuated and sealed cell which is subsequently heated. The first step of the analysis invol ves calculating the gradual increase of vapor pressure in the closed cell as the temperature is raised. Then, in the second step, the cell is evacuated to low pressure (e.g., vacuum), allowing the water vapor to leave the cell and be captured. The parameters affecting water vap or pressure build-up and evacuation for the purpose of extracting water from lunar regolith are discussed in the paper. Some comparisons wi th available experimental measurements are also made.

Hegde, U.↗
NASA NTRS2013

Life and the Universe: From Astrochemistry to Astrobiology

Great strides have been made in our understanding of interstellar material thanks to advances in infrared astronomy and laboratory astrophysics. Ionized polycyclic aromatic hydrocarbons (PAHs), shockingly large molecules by earlier astrochemical standards, are widespread and very abundant throughout much of the cosmos. In cold molecular clouds, the birthplace of planets and stars, interstellar atoms and molecules freeze onto extremely cold dust and ice particles forming mixed molecular ices dominated by simple species such as water, methanol, ammonia, and carbon monoxide. Within these clouds, and especially in the vicinity of star and planet forming regions, these ices and PAHs are processed by ultraviolet light and cosmic rays forming hundreds of far more complex species, some of biogenic interest. Eventually, these are delivered to primordial planets by comets and meteorites. As these materials are the building blocks of comets and related to carbonaceous micrometeorites, they are likely to be important sources of complex organic materials delivered to habitable planets (including the primordial Earth) and their composition may be related to the origin of life. This talk will focus on the chemical evolution of these cosmic materials and their relevance to astrobiology.

Atmoshperic Chemistry↗
NASA NTRS1995

Condensed Water in Tropical Cyclone "Oliver", 8 February 1993

On February 8, 1993, the NASA DC-8 aircraft profiled from 10,000 to 37,000 feet (3.1-11.3 km) pressure altitude in a stratified section of tropical cyclone "Oliver" over the Coral Sea northeast of Australia. Size, shape and phase of cloud and precipitation particles were measured with a 2-D Greyscale probe. Cloud/precipitation particles changed from liquid to ice as soon as the freezing level was reached near 17,000 feet (5.2 km) pressure altitude. The cloud was completely glaciated at -5 C. There was no correlation between ice particle habit and ambient temperature. In the liquid phase, the precipitation-cloud drop concentration was 4.0 x 10(exp 3)/cu m, the geometric mean diameter D(sub g) = 0.5-0.7 mm, and the liquid water content 0.7-1.9 g m(exp-3). The largest particles anywhere in the cloud, dominated by fused dendrites at concentrations similar to that of raindrops (2.5 x 10(exp 3) m(exp -3)) but a higher condensed water content(5.4 g/cu m estimated) were found in the mixed phase; condensed water is removed very effectively from the mixed layer due to high settling velocities of the large mixed particles. The highest number concentration (4.9 x 10(exp 4)/cu m, smallest size (D(sub g) = 0.3-0.4 mm), largest surface area (up to 2.6 x 10 (exp 2) sq cm/cu m at 0.4- 1.0 g/cu m of condensate) existed in the ice phase at the coldest temperature (- 40 C) at 35,000 feet ( 10.7 km). Each cloud contained aerosol (haze particles) in addition to cloud particles. The aerosol total surface area exceeded that of the cirrus particles at the coldest temperature. Thus, aerosols must play a significant role in the upscattering of solar radiation. Light extinction (6.2/km) and backscatter (0.8/sr/km) was highest in the coldest portion of the cirrus cloud at the highest altitude.

Pueschel, R. F.↗
NASA NTRS2023

A 1D Model for Nucleation of Ice From Aerosol Particles: An Application to a Mixed-Phase Arctic Stratus Cloud Layer

Mixed-phase clouds (MPCs) have been identified as significant contributors to uncertainties in climate projections, attributable to model representation of processes controlling the formation and loss of supercooled water droplets and ice particles from the atmosphere. Arctic MPCs are commonly widespread and long-lived, with sustained ice crystal formation processes that challenge current understanding. This study examines the ice-nucleating particle (INP) reservoir dynamics governing immersion-mode heterogeneous freezing in an observed case of Arctic MPCs using a simplified 1D aerosol-cloud model. The model setup includes prescribed dynamical forcings and thermodynamic profiles, and represents INPs as multicomponent and polydisperse particle size distributions. Diagnostic and prognostic approaches to immersion freezing parameterization are compared, including time-independent (singular) number- and surface area-based descriptions and a time-dependent description following classical nucleation theory (CNT). The choice of freezing parameterization defines the size of the INP reservoir. The CNT-based description yields an orders of magnitude larger INP reservoir than the singular parameterizations, which is the dominant factor for sustained ice crystal formation. The efficiency of the freezing process and cloud cooling are of secondary importance. A diagnostic treatment neglecting INP loss is only accurate when the INP reservoir size is large and INP depletion weak. Since a larger INP reservoir sustains ice crystal formation substantially longer, and ice water path scales with ice crystal concentrations for the conditions considered, resolving the source of differences in INP reservoir dynamics due to model implementation is a high priority for advancing climate model physics.

aerosol↗
NASA NTRS2017

Comparisons of Mixed-Phase Icing Cloud Simulations with Experiments Conducted at the NASA Propulsion Systems Laboratory

This paper builds on previous work that compares numerical simulations of mixed-phase icing clouds with experimental data. The model couples the thermal interaction between ice particles and water droplets of the icing cloud with the flowing air of an icing wind tunnel for simulation of NASA Glenn Research Centers (GRC) Propulsion Systems Laboratory (PSL). Measurements were taken during the Fundamentals of Ice Crystal Icing Physics Tests at the PSL tunnel in March 2016. The tests simulated ice-crystal and mixed-phase icing that relate to ice accretions within turbofan engines. Experimentally measured air temperature, humidity, total water content, liquid and ice water content, as well as cloud particle size, are compared with model predictions. The model showed good trend agreement with experimentally measured values, but often over-predicted aero-thermodynamic changes. This discrepancy is likely attributed to radial variations that this one-dimensional model does not address. One of the key findings of this work is that greater aero-thermodynamic changes occur when humidity conditions are low. In addition a range of mixed-phase clouds can be achieved by varying only the tunnel humidity conditions, but the range of humidities to generate a mixed-phase cloud becomes smaller when clouds are composed of smaller particles. In general, the model predicted melt fraction well, in particular with clouds composed of larger particle sizes.

Thermal model↗
NASA NTRS1991

Stratospheric soot - Cloud forming properties and transport processes

Soot enters the stratosphere either from the troposphere in deep thunderstorm convection, predominantly in the tropics, from midlatitude forest fires, and directly from aircraft flying above the tropopause. Particles emitted from jet aircraft are relatively ineffective as cloud droplet condensation nuclei (less than 1 percent) compared with those from forest fires (above 50 percent). Chemical and other modification during aging of the particles may influence these results in some circumstances; cloud nucleating properties can be used as a soot tracer. Such aerosols, as they grow to haze drops and ilute in increasing humidity, may form ice particles in the cold polar stratosphere or in tropical cumuli anvils at 18 to 20 km altitude at temperatures as low as -90 C. Ice may also form as particles are removed by descent through troposphere folds and enter midlatitude cirrus at levels below -40 C. In the stratosphere, ice particles may provide surfaces that catalyze heterogeneous chemical reactions; in the upper troposphere, the optical depths of cirrus clouds may be significantly increased.

Hallett, John↗
NASA NTRS1987

Antarctic stratospheric chemistry of chlorine nitrate, hydrogen chloride, and ice - Release of active chlorine

The reaction rate between atmospheric hydrogen chloride (HCl) and chlorine nitrate (ClONO2) is greatly enhanced in the presence of ice particles; HCl dissolves readily into ice, and the collisional reaction probability for ClONO2 on the surface of ice with HCl in the mole fraction range from about 0.003 to 0.010 is in the range from about 0.05 to 0.1 for temperatures near 200 K. Chlorine is released into the gas phase on a time scale of at most a few milliseconds, whereas nitric acid (HNO3), the other product, remains in the condensed phase. This reaction could play an important role in explaining the observed depletion of ozone over Antarctica; it releases photolytically active chlorine from its most abundant reservoir species, and it promotes the formation of HNO3 and thus removes nitrogen dioxide from the gas phase. Hence it establishes the necessary conditions for the efficient catalytic destruction of ozone by halogenated free radicals.

Molina, Mario J.↗
NASA NTRS1990

Scatterers in Triton's atmosphere - Implications for the seasonal volatile cycle

Nitrogen and methane ices on the surface of Triton, Neptune's largest satellite, are exchanged between the summer and winter hemispheres on a seasonal time scale. Images of the satellite's sky obtained by the Voyager 2 spacecraft show the presence of several types of scattering materials that provide insights into this seasonal cycle of volatiles. Discrete clouds, probably composed of N2 ice particles, arise in regions of active sublimation. They are found chiefly poloward of 30 deg S in the southern, summer hemisphere. Haze particles, probably made of hydrocarbon ices, are present above most, but not all places. Recent snowfall may have occurred at low southern latitudes in places where they are absent. The latent heat released in the formation of the discrete clouds may have a major impact on the thermal balance of the lower atmosphere. Triton may have been less red at the time of the Voyager flyby than 12 years earlier due to recent N2 snowfall at a wide range of latitudes.

Pollack, James B.↗