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At least 163 records · Page 9

Integrated Data Analysis to Improve Te and Zeff Measurement on NSTX-U

The multi-energy soft x-ray (ME-SXR) camera is a new concept for a fusion plasma diagnostic based on a pixelated detector with adjustable photon cutoff thresholds. It is a single, compact, solid-state detector which combines spatial and spectral sensitivity and can be configured remotely at run time, making it ideal for a fusion environment. The detector can be configured for application to a wide range of physics problems including impurity transport, electron temperature profiles, and non-thermal effects. The detector has been installed on the Madison Symmetric Torus (MST) as part of a collaboration between Princeton Plasma Physics Laboratory and the University of Wisconsin–Madison to develop the technology and analysis techniques. A full diagnostic forward model of the ME-SXR diagnostic has been developed to enable analysis of the raw photon count data. This model incorporates the atomic physics underlying the plasma emission, diagnostic geometry, and detector response characteristics. Employing this model, a Bayesian analysis approach is used to extract electron temperature from the raw data. This analysis approach uses all available information, clearly quantifies prior information, and handles uncertainties transparently. The ME-SXR camera is being used to study the 3D (helical, stellarator-like) state that forms in the MST device. This helical core structure has improved energy confinement. The transition to the helical state is accompanied by a rise in electron temperature in the central part of the helical structure, but then this enhancement fluctuates. The characteristics of this fluctuation are being compared to a magneto-hydrodynamics model.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

An Evaluation of the Impact of Glycolate and Glycolate Mitigation on the Defense Waste Processing Facility Recycle Diversion Project Flowsheet

The Savannah River Site (SRS) Defense Waste Processing Facility (DWPF) processes radioactive High Level Waste (HLW) sludge solids from the Concentration, Storage, and Transfer Facilities (CSTF); which includes the SRS Tank Farm and Evaporator facilities, and a concentrated Cs-137 laden stream and a Monosodium Titanate (MST) and sludge solids stream from the SRS Salt Waste Processing Facility (SWPF). The waste is chemically adjusted with acids and reductant (currently with 50 wt.% nitric acid and ~90 wt.% formic acid, but eventually formic acid will be substituted with ~70 wt.% glycolic acid), and frit is added so that a durable, borosilicate glass waste form can be produced when the material is vitrified in the melter. As a result of the evaporation of water during both the melter feed preparation and the melter feed vitrification steps in DWPF, a recycle waste stream is generated, neutralized, and sent back to the CSTF. The recycle waste is a dilute aqueous stream originating from the collection of condensate liquids containing some minor sludge, MST, and frit solids and other waste components resulting from melter feed entrainment during foamover events and transfer of volatile species into the condensate. The recycle stream volume is significant and is expected to approach 3 million gallons per year once SWPF reaches full operation, requiring the use of multiple large CSTF tanks for storage. The recycle waste is currently collected in the SRS Tank Farm and periodically evaporated in the 242-16H (2H) Evaporator to conserve storage space.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Granta:MI Record Review Procedure for Materials Testing Projects

This document is intended to serve as a guide for the review of records in LANL’s Weapons Materials Database. Specifically, this guide provides step-by-step instructions for the review of records associated with a materials testing project. This is the type of dataset that testing organizations such as MST-7 & MST-8 at LANL commonly produce for the weapons complex and want to archive in Granta:MI.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Measurement Acceptance Region (MAR) Assessment Results Based On Sludge Batch 10 Projections from December 2021, February 2022 and August 2022

The Defense Waste Processing Facility (DWPF) is currently preparing to initiate processing of Sludge Batch 10 (SB10), which is comprised of material from Tanks 11H, 13H, 15H, and 26F, Alternate Feed Stock-2 and Sodium Reactor Experiment material from H-Canyon. Frit 473 (8B 2 O 3 -8Li 2 O-5Na 2 O-79SiO 2 , in weight percent) was recommended for sludge-only (SO) and coupled processing with the Salt Waste Processing Facility (SWPF) based on previous assessments of SB10 projections with the DWPF Product Composition Control System (PCCS) glass property models and their associated Measurement Acceptance Region (MAR) constraints. Due to the lower processing rate of Sludge Batch 9 (SB9), the heel in Tank 40 is anticipated to be greater than 40 inches at the projected start of SB10 processing to meet the upcoming Accelerated Basin Deinventory addition dates in Tank 51 for Sludge Batch 11. In December 2021 and February 2022, Savannah River Remediation System Planning provided updated SB10 Tank 40 blend projections based on heels of 74 inches, 84 inches, 94 inches and 103.4 inches. Savannah River Mission Completion (SRMC) subsequently pursued Wash Cycle Y to further reduce the total sulfur in the sludge batch and increase processing flexibility at DWPF. In August 2022, SRMC System Planning provided an updated SB10 Tank 40 blend projection with a 76 inch-heel representing Decant Y2 and 60 kilogallons of bearing water inleakage that is anticipated during the Tank 51 to Tank 40 transfer. The objectives of this task were to: • Determine the impact on the operating windows for SO and coupled processing • Determine whether any composition gaps exist between the already completed SB10 variability study and the reprojected SB10 glass composition region • Compare the SB10 reprojected glass composition region to the DWPF PCCS model development and validation ranges to ensure that compositional gaps do not exist between the data sets. This report documents the results of these evaluations. Calculation-based frit assessments were performed using the DWPF PCCS glass property models and their associated MAR constraints. Evaluated parameters for coupled processing included the following transfer volumes per Sludge Receipt and Adjustment Tank batch: 5700 gallons of Tank 40 sludge, 2400-4500 gallons of the SWPF monosodium titanate (MST) and sludge solids stream, and 15,000 gallons of strip effluent. Based on these MAR assessment results, Frit 473 remains viable for SB10 processing. A target waste loading (WL) of 36% is possible for SO operation and single strike (0.4 g/L MST) coupled processing up to 600 mg/L of SB9 insoluble sludge solids at a nominal transfer volume of ~2800 gallons. Increasing the single strike transfer volume to 4500 gallons may reduce the maximum WL below 40%. Operating windows are 12 percentage points for SO processing and 14-16 percentage points for coupled processing. Frit 625 allows for a target WL of 36% and is acceptable for use during the SB9 to SB10 transition to deplete remaining inventory as needed. Operating windows are 8 percentage points for SO processing and 12-14 percentage points for coupled processing. Predictive PCCS evaluations performed at DWPF will provide insight into batch-specific acceptability at desired WLs for compositions having expected oxide ratios during processing versus the extreme vertices (corner points) evaluated in this study. The reprojected SB10 glass composition region generally overlaps the previously evaluated SB10 variability study composition region. Thus, the minor composition shift of these updated SB10 projections indicates that no additional glasses are necessary to demonstrate acceptability relative to the chemical durability of the Environmental Assessment benchmark glass and predictability using the current PCCS models for durability. Based on a comparison of the PCCS model development and validation data to the reprojected SB10 glass composition region, the viscosity and liquidus temperature models will reliably predict SB10 compositions. No additional glasses are necessary to demonstrate predictability of these models.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Review and Assessment of Available Data Regarding the Behavior of Sodium Aerosols

Recently, there has been a resurgence of interest in advanced (non-light water) reactor designs, including sodium fast reactors (SFRs). In parallel, multiple efforts are underway to develop risk informed, performance-based licensing pathways for advanced reactors. However, such licensing approaches depend on the accuracy of the associated safety assessments, including mechanistic source term (MST) analyses. Unlike historical source term assessments, which utilizes bounding estimates of radionuclide release, MSTs attempt to realistically estimate the transport and retention of radionuclides for specific transient scenarios. For SFR MST analyses, the behavior of radionuclide aerosols is a key factor, as noted in recent studies. Due to the use of sodium as the primary coolant, many potential transient scenarios involve the release of radionuclide aerosols in conjunction with sodium aerosols. For such scenarios, sodium may be the dominant aerosol species, compared to that of released radionuclides. Therefore, understanding the behavior of sodium aerosols is particularly important to an accurate assessment of aerosol transport. Although many approaches to aerosol modeling exist, it is vital to establish their capabilities in evaluating sodium aerosol behavior for SFR analyses.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

A Novel Standard Gibbs Energy of Formation Model for High-Enthalpy Water Systems

This work provides an advanced standard molar Gibbs energy of formation model, informed by molecular statistical thermodynamics (MST), and validated by mineral solubility and ion association reactions. This new model aligns with experimental data within uncertainties and highlights the role of specific MST interactions around the critical point. This work will provide a reliable tool for the optimization of industrial processes operating at the edges of the supercritical domain.

Hall, Derek↗

Benchmark Exercise Report for Experimental Study of Bubble Scrubbing in Sodium Pool

Mechanistic source term (MST) analyses are likely to be an important part of advanced reactor licensing applications. For the purpose, an MST analysis code applicable to newly introduced advanced reactors, called SRT (Simplified Radionuclide Transport) code, has been developed by Argonne National Laboratory. SRT can track overall behaviors of radionuclides especially in metal fuel-based sodium fast reactors (SFRs) and microreactors. Throughout the simulation, migration inside fuel pins before failure, interaction with coolant (for SFR), removal/leakage in cover gas and containment (or confinement), and environmental dose impacts are considered alongside radioactive decay for short-lived nuclides. Among the postulated process, pool scrubbing phenomenon, especially under sodium pool condition, has been identified as high importance with limited supportive data. The phenomenon plays a crucial role in assessing the degree of radiological impacts as radioactive aerosols or vapors are efficiently and effectively removed during the process. To provide validation basis for SRT in assessing pool scrubbing performance inside sodium pools, the University of Wisconsin-Madison performed tests including extensive parametric effects. Separate effect tests were conducted to directly evaluate the SRT models and to estimate degree of contribution by each contributing factor. Specifically, bubble size, aerosol size, aerosol density, aerosol concentration, pool depth, system temperature, and bubble swarm effects were considered. According to the parametric effects, decontamination performance enhances with decreasing bubble size, large density, and deeper pool height. Aerosol concentration provides no effect for the whole range of interest, and pool temperature variation shows minor effects under the considered temperature condition. When multiple bubbles are injected generating a bubble swarm condition, DF performance further enhances by bubble interactions and turbulence characteristics. The measurement shows the exceptional importance of aerosol size range considered, with the lowest decontamination, where most radionuclides are expected to escape.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Characterization of Precipitate Reactor Feed Tank (PRFT) Batches 44 and 49 from the Defense Waste Processing Facility (DWPF)

The Savannah River Site (SRS) Defense Waste Processing Facility (DWPF) processes a Monosodium Titanate/Sludge Solids (MST/SS) waste stream received from the Salt Waste Processing Facility (SWPF) via the Precipitate Reactor Feed Tank (PRFT). During processing, DWPF is required to provide evidence of compliance with the Waste Acceptance Product Specifications (WAPS). Savannah River Mission Completion (SRMC) has requested Savannah River National Laboratory (SRNL) to analyze PRFT samples representing each SWPF salt batch for thirty-two radionuclides. Additionally, elemental analysis of PRFT slurry and MST/SS solids was performed to aid SRMC in further refinement of the inputs and assumptions used in future frit development and Material Tracking Program calculations. The analyses of PRFT Batches 44 and 49, which correspond to material from the processing of Salt Batches (StB) 12 and 11, respectively, are reported herein. The unwashed dried solids of the PRFT Batches 44 and 49 are predominately MST, ~63-59% MST. The two batches have a much higher amount of Fe, Mn, and Ni compared to all previous batches. For Batch 44 this appears to be due to the use of a sludge simulant filter aid during processing of StB 12 and for Batch 49, it is possibly due to the larger amount of insoluble solids for StB 11 in comparison to all previous salt batches. Like previous PRFT batches, a significant amount of the unwashed dried solids are alkaline earth metals. The total sulfate, in mg/kg of slurry, for PRFT Batches 44 and 49 is 119 and 139, respectively, which is well below the current sulfate concentration used in Material Tracking Program calculations and is in agreement with DWPF laboratory sulfate measurements.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Graphical Optimization of Spectral Shift Reconstructions for Optical Backscatter Reflectometry

Optical backscatter reflectometry (OBR) is an interferometric technique that can be used to measure local changes in temperature and mechanical strain based on spectral analyses of backscattered light from a singlemode optical fiber. The technique uses Fourier analyses to resolve spectra resulting from reflections occurring over a discrete region along the fiber. These spectra are cross-correlated with reference spectra to calculate the relative spectral shifts between measurements. The maximum of the cross-correlated spectra—termed quality—is a metric that quantifies the degree of correlation between the two measurements. Recently, this quality metric was incorporated into an adaptive algorithm to (1) selectively vary the reference measurement until the quality exceeds a predefined threshold and (2) calculate incremental spectral shifts that can be summed to determine the spectral shift relative to the initial reference. Using a graphical (network) framework, this effort demonstrated the optimal reconstruction of distributed OBR measurements for all sensing locations using a maximum spanning tree (MST). By allowing the reference to vary as a function of both time and sensing location, the MST and other adaptive algorithms could resolve spectral shifts at some locations, even if others can no longer be resolved.

47 OTHER INSTRUMENTATION↗

Determination of vertical and horizontal wavelengths of gravity waves

The determination of horizontal and vertical wavelengths of gravity waves obviously relies on measurement of wave parameters in horizontal and vertical directions. A very suitable parameter, measured fairly easily with MST radars, is the fluid velocity. Average velocities and superimposed turbulent fluctuations are much larger in the horizontal than in the vertical direction. Vertical and horizontal fluid velocities due to wave-like events are mostly about equal in magnitude. Vertical fluid velocities due to waves therefore can be more reliably detected than horizontal velocities. Estimates of gravity wave events using MST radar data are calculated and results are indicated.

Rottger, J.↗

School of Electrical Engineering.

The possibility of making the antenna of an MST radar too large is pointed out. It is not that the signal ceases to become stronger beyond some critical antenna size; the received scattered signal actually becomes weaker as the antenna size is increased whenever the target is in the near field, Fresnel region of the antenna. The Arecibo antenna is a case in point. It is supposed that MST work would benefit to use a feed which illuminated only a portion of the dish.

Farley, D. T.↗

Decoding: Codes and hardware implementation

The MST radars vary considerably from one installation to the next in the type of hardware, operating schedule and associated personnel. Most such systems do not have the computing power to decode in software when the decoding must be performed for each received pulse, as is required for certain sets of phase codes. These sets provide the best signal to sidelobe ratio when operating at the minimum band length allowed by the bandwidth of the transmitter. The development of the hardware phase decoder, and the applicability of each to decoding MST radar signals are discussed. A new design for a decoder which is very inexpensive to build, easy to add to an existing system and is capable of decoding on each received pulse using codes with a band length as short as one microsecond is presented.

Sulzer, M. P.↗

Coherent integration

Coherent integration which is a digital filtering process and was applied to MST radar observations is discussed. It is simple to implement with either hardware or software and is appropriate for the very narrow band signals usually received by MST radars. By filtering the signal before performing spectral processing, the computations required for FFT or similar analysis are greatly reduced. Coherent integration does not increase the signal-to-noise ratio per unit bandwidth in the signal band. It filters out much of the wideband noise, which could also be done by full FFT processing of the raw signal.

Farley, D. T.↗

General circulation of the middle atmosphere, part 1.4B

In both the tropical and extratropical regions there are a large number of dynamical problems which can be addressed by mesosphere-stratosphere-troposphere (MST) radars. The distinct advantage the MST radar has over rocket observations is continuous data acquisition. Without a doubt, the time-space spectrum of the mesospheric flow field is rich in high frequency motions associated with gravity waves rather than turbulent (random) fluctuations, and these events are particularly amenable to analysis with continuous data sets. In addition to the high frequency motions these are longer period fluctuations in the upper stratosphere and mesosphere wind fields which, combined with temperature fields derived from satellite data or lidars, can greatly enhance our knowledge of the upper atmosphere.

Schoeberl, M. R.↗

Morphology of the scattering targets: Fresnel and turbulent mechanisms, part 2.1A

Refractive index fluctuations cause coherent scattering and reflection of VHF radio waves from the clear air in the altitude region between 0 and approximately 90 km. Similar echoes from the stratosphere/troposphere and the mesosphere are observed at UHF and MF/HF frequencies, respectively. The nature of the refractive index fluctuations has been studied for many years without producing a clear consensus on what mechanism causes them. It is believed that the irregularities can originate from two different mechanisms: turbulent mixing of the gradient of refractive index, and stable horizontally stratified laminae of sharp gradients in the refractive index. In order to explain observations of volume dependence and aspect sensitivity of the echo power in the MST region, a diversity of submechanisms has been proposed. They include isotropic and anisotropic turbulent scattering, Fresnel scattering and reflection, and diffuse reflection. Isotropic turbulent scattering is believed to cause a majority of the clear air echoes observed by MST radars. The mechanism requires active turbulence mixing of a preexisting gradient in the refractive index profile.

Royrvik, O.↗

Techniques for the study of gravity waves and turbulence (keynote paper), part 4

Probably one of the most important achievements mesosphere stratosphere troposphere (MST) radars can make toward increasing the understanding of the dynamics of the atmosphere is to determine the exact relationship between the generation of turbulence and the sources of high shear or convectively unstable flows. An important theoretical tool, the gravity-wave breaking through which one can begin to understand spontaneous generation of turbulence model is discussed. In this model, large amplitude gravity waves produce local regions where the Richardson number (N sup 2/U sub Z sup 2) is less than 1/4 thus giving rise to turbulent flows. Thus the appearance of turbulent layers can often be interpreted as a breaking-gravity-wave signature. Even though the techniques for studying gravity waves and turbulence may be quite different (and historically have resulted in somewhat separate bodies of literature), it is clear from the wave-breaking model that the phenomena are intimately linked. The techniques for measurements of gravity wave flow fields and turbulent regions by MST radar should show cognizance of some of the theoretical questions raised by the wave-breaking model.

Schoeberl, M. R.↗

MENTOR: Adding an outlying receiver to an ST radar for meteor-wind measurement

Radar scattering from ionized meteor trails has been used for many years as a way to determine mesopause-level winds. Scattering occurs perpendicular to the trails, and since the ionizing efficiency of the incoming meteoroids depends on the cosine of the zenith angle of the radiant, echoes directly overhead are rare. Stratosphere-troposphere (ST) radars normally sample within 15 deg of the vertical, and thus receive few meteor echoes. Even the higher powdered mesosphere-stratosphere-troposphere (MST) radars are not good meteor radars, although they were used to successfully retrieved meteor winds from the Poker Flat, Alaska MST radar by averaging long data intervals. It has been suggested that a receiving station some distance from an ST radar could receive pulses being scattered from meteor trails, determine the particular ST beam in which the scattering occurred, measure the radial Doppler velocity, and thus determine the wind field. This concept has been named MENTOR (Meteor Echoes; No Transmitter, Only Receivers).

Roper, R. G.↗

Summary of progress at the Poker Flat Observatory in Alaska

A description of the status of the Poker Flat MST Radar as of early 1983 is included in the 1983 mesosphere-stratosphere-troposphere MST Workshop Proceedings. The Observatory continues to operate in a continuous data-taking mode, except for a three-week planned campaign experiment concurrent with the STATE rocket program during June 1983. Construction of the digital preprocessing system mentioned in the last status report is all but complete. This additional improvement should be operational by late summer. The possibility of steering the array also mentioned in the last status report is being investigated. A project is underway to electronically steer the one-quarter vertical section of the array. Steering will be in finite steps within about + or - 5 deg of vertical. Successful testing of this modification may lead to eventually steering the entire array in this manner. Data analysis of the data base (now more than four years in length) continues with well over one dozen extramural scientific groups participating.

Balsley, B. B.↗