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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 163 records · Page 9
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Impact of imposed mode 2 laser drive asymmetry on inertial confinement fusion implosions

Low-mode asymmetries have emerged as one of the primary challenges to achieving high-performing inertial confinement fusion implosions. These asymmetries seed flows in the implosions, which will manifest as modifications to the measured ion temperature (T ion ) as inferred from the broadening of primary neutron spectra. The effects are important to understand (i) to learn to control and mitigate low-mode asymmetries and (ii) to experimentally more closely capture thermal T ion used as input in implosion performance metric calculations. Here, in this paper, results from and simulations of a set of experiments with a seeded mode 2 in the laser drive are described. The goal of this intentionally asymmetrically driven experiment was to test our capability to predict and measure the signatures of flows seeded by the low-mode asymmetry. The results from these experiments [first discussed in M. Gatu Johnson et al., Phys. Rev. E 98, 051201(R) (2018)] demonstrate the importance of interplay of flows seeded by various asymmetry seeds. In particular, measured T ion and self-emission x-ray asymmetries are expected to be well captured by interplay between flows seeded by the imposed mode 2 and the capsule stalk mount. Measurements of areal density asymmetry also indicate the importance of the stalk mount as an asymmetry seed in these implosions. The simulations brought to bear on the problem (1D LILAC, 2D xRAGE, 3D ASTER, and 3D Chimera) show how thermal T ion is expected to be significantly lower than T ion as inferred from the broadening of measured neutron spectra. They also show that the electron temperature is not expected to be the same as T ion for these implosions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2019

Simulation of Inelastic Neutron Scattering Spectra Using OCLIMAX

Studying the vibration of atoms is of fundamental importance and can provide critical insight for the understanding of materials behavior, such as structure and phase transition, thermodynamics, and chemical reactions. The atomic vibration can be probed using vibrational spectroscopy with various incident particles such as photons, neutrons, or electrons. A major challenge when applying these techniques is often how to interpret the vibrational spectra and how to make connections to the theory. To this end, methods that can simulate the spectra from atomistic models are highly desired. In this paper, we present a program developed for the simulation of inelastic neutron scattering spectra. We report it has many new and useful features that were not previously available and will greatly facilitate the analysis and understanding of inelastic neutron scattering data.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

Three-dimensional simulations of National Ignition Facility implosions: Insight into experimental observables

We simulate in 3D both the hydrodynamics and, simultaneously, the X-ray and neutron diagnostic signatures of National Ignition Facility (NIF) implosions. We apply asymmetric radiation drive to study the impact of low mode asymmetry on diagnostic observables. We examine X-ray and neutron images as well as neutron spectra for these perturbed implosions. The X-ray images show hot spot evolution on small length scales and short time scales, reflecting the incomplete stagnation seen in the simulation. The neutron images show surprising differences from the X-ray images. The neutron spectra provide additional measures of implosion asymmetry. Flow in the hot spot alters the neutron spectral peak, namely, the peak location and width. The changes in the width lead to a variation in the apparent temperature with viewing angle that signals underlying hot spot asymmetry. We compare our new expectations based on the simulated data with NIF data. We find that some recent cryogenic layered experiments show appreciable temperature anisotropy indicating residual flow in the hot spot. We also find some trends in the data that do not reflect our simulation and theoretical understanding.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2026

A new layered kagome strip structure Na 2 Co 3 (AsO 4 ) 2 (OH) 2 : static and dynamic magnetic properties

One-dimensional kagome strip chains share much of the same frustrated structural motif as two-dimensional kagome antiferromagnets, making them valuable for deepening our understanding of kagome lattice magnetism. In this paper, we report the hydrothermal synthesis and detailed structural and property characterization of Na 2 Co 3 (AsO 4 ) 2 (OH) 2 , a striped kagome system. The crystal structure was characterized using single crystal X-ray diffraction which reveals that Na 2 Co 3 (AsO 4 ) 2 (OH) 2 crystallizes in monoclinic crystal system C2/m. The structure features a one-dimensional kagome strip lattice built from Co 2+ ions and undergoes an antiferromagnetic transition at T N = 14 K. The magnetic ground state at zero field was characterized using neutron powder diffraction. Below the magnetic transition, Na 2 Co 3 (AsO 4 ) 2 (OH) 2 orders into an antiferromagnetic structure with a k-vector (0.5, 0.5, 0.5). In the proposed model, the Co1 moment is predominantly confined to the ac-plane while the Co2 moment is primarily aligned along the b-axis. Two flat bands were observed in the inelastic neutron spectra below the magnetic transition, 5 and 10 meV. Inelastic neutron spectra were modeled with a Heisenberg Hamiltonian including three nearest-neighbor exchange interactions (J 1 , J 2 , J 3 ) and strong single-ion anisotropy to stabilize the observed magnetic structure. Our study highlights the complexity of Co 2+ -based kagome strip magnetic lattice compound Na 2 Co 3 (AsO 4 ) 2 (OH) 2 which provides an excellent platform to broaden our understanding of the frustrated kagome magnetic lattice space.

Liurukara, Duminda S. [Oak Ridge National Laborato↗
NASA NTRS2003

Preliminary Analysis of the Multisphere Neutron Spectrometer

Crews working on present-day jet aircraft are a large occupationally exposed group with a relatively high average effective dose from galactic cosmic radiation. Crews of future high-speed commercial aircraft flying at higher altitudes would be even more exposed. To help reduce the significant uncertainties in calculations of such exposures, the Atmospheric Ionizing Radiation (AIR) Project, an international collaboration of 15 laboratories, made simultaneous radiation measurements with 14 instruments on five flights of a NASA ER-2 high-altitude aircraft. The primary AIR instrument was a highly sensitive extended-energy multisphere neutron spectrometer with lead and steel shells placed within the moderators of two of its 14 detectors to enhance response at high energies. Detector responses were calculated for neutrons and charged hadrons at energies up to 100 GeV using MCNPX. Neutron spectra were unfolded from the measured count rates using the new MAXED code. We have measured the cosmic-ray neutron spectrum (thermal to greater than 10 GeV), total neutron fluence rate, and neutron effective dose and dose equivalent rates and their dependence on altitude and geomagnetic cutoff. The measured cosmic-ray neutron spectra have almost no thermal neutrons, a large "evaporation" peak near 1 MeV and a second broad peak near 100 MeV which contributes about 69% of the neutron effective dose. At high altitude, geomagnetic latitude has very little effect on the shape of the spectrum, but it is the dominant variable affecting neutron fluence rate, which was 8 times higher at the northernmost measurement location than it was at the southernmost. The shape of the spectrum varied only slightly with altitude from 21 km down to 12 km (56 - 201 grams per square centimeter atmospheric depth), but was significantly different on the ground. In all cases, ambient dose equivalent was greater than effective dose for cosmic-ray neutrons.

Goldhagen, P.↗
DOE OSTI2021

Reconstruction of β-Delayed Neutron Energy Spectra from Recoil-Ion Spectroscopy of Trapped Ions

Here Beta-delayed one-neutron (βn) emission has been investigated by confining radioactive ions in an ion trap and detecting the β particles and recoiling nuclei that emerge following decay. In this approach, the βn energy spectrum and branching ratio can be deduced without needing to detect the neutrons, as the neutron emission is inferred from the observed time of flight of the recoiling ions. This paper details the dominant effects that influence the extraction of the neutron energy from the time-of-flight measurement and explores the impact they have on the energy calibration and resolution.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Dual-energy fast neutron imaging using tunable short-pulse laser-driven sources

Here a novel dual-energy fast neutron imaging technique is presented using short-pulse laser-driven neutron sources to leverage their inherent adaptive spectral control to enable 3D volume segmentation and reconstruction. Laser-accelerated ion beams incident onto secondary targets create directional, broadband, MeV-class neutrons. Synthetic radiographs are produced of multi-material objects using ion and neutron spectra derived from analytic and numerical models. It is demonstrated that neutron images generated from small changes to the neutron spectra, controlled by altering the initial laser conditions, are sufficient to isolate materials with differing attenuation coefficients. This is first demonstrated using a simplistic combinatorial isolation method and then by employing more advanced reconstruction algorithms to reduce artifacts and generate a segmentation volume of the constituent materials.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2013

Predicting Reactor Antineutrino Emissions Using New Precision Beta Spectroscopy

Neutrino experiments at nuclear reactors are currently vital to the study of neutrino oscillations. The observed antineutrino rates at reactors are typically lower than model expectations. This observed deficit is called the “reactor neutrino anomaly”. A new understanding of neutrino physics may be required to explain this deficit, though model estimation uncertainties may also play a role in the apparent discrepancy. PNNL is currently investigating an experimental technique that promises reduced uncertainties for measured data to support these hypotheses and interpret reactor antineutrino measurements. The experimental approach is to 1) direct a proton accelerator beam on a metal target to produce a source of neutrons, 2) use spectral tailoring to modify the neutron spectrum to closely simulate the energy distribution of a power reactor neutron spectrum, 3) irradiate isotopic fission foils (235U, 238U, 239Pu, 241Pu) in this neutron spectrum so that fissions occur at energies representative of a reactor, 4) transport the beta particles released by the fission products in the foils to a beta spectrometer, 5) measure the beta energy spectrum, and 6) invert the measured beta energy spectrum to an antineutrino energy spectrum. A similar technique using a beta spectrometer and isotopic fission foils was pioneered in the 1980’s at the ILL thermal reactor. Those measurements have been the basis for interpreting all subsequent antineutrino measurements at reactors. A basic constraint in efforts to reduce uncertainties in predicting the antineutrino emission from reactor cores is any underlying limitation of the original measurements. This may include beta spectrum energy resolution, the absolute normalization of beta emission to number of fission, statistical counting uncertainties, lack of 238U data, the purely thermal nature of the IIL reactor neutrons used, etc. An accelerator-based neutron source that can be tailored to match various reactor neutron spectra provides an advantage for control in studying how changes in the neutron spectra (i.e. "in the reactor core") affects the resulting fission product beta spectrum. Furthermore, the 238U antineutrino spectrum, which has not been measured, can be studied directly because of the enhanced 1 MeV fast neutron flux available at the accelerator source. A facility such as the Project X Injector Experiment (PXIE) 30 MeV proton linear accelerator at Fermilab is being considered for this experiment. The hypothesis is that a new approach utilizing the flexibility of an accelerator neutron source with spectral tailoring coupled with a careful design of an isotopic fission target and beta spectrometer and the inversion of the beta spectrum to the neutrino spectrum will allow further reduction in the uncertainties associated with prediction of the reactor antineutrino spectrum.

Asner, David M.↗
DOE OSTI2019

Development of a neutron spectrometer utilizing rubberized Eu:LiCAF wafers

A portable ten-layer neutron spectrometer has been developed using a novel material, LiCAF. The spectrometer consists of rubber matrix wafers with embedded europium doped lithium calcium aluminum uoride (Eu:LiCAF) crystals and crosshatched wave shifting fibers (WSF). Layers of high density polyethylene (HDPE) separating each Eu:LiCAF wafer serve as neutron moderating material. Neutrons entering the spec- trometer react in the Eu:LiCAF crystal, creating scintillation photons. The photons travel down the WSFs to silicon photomultipliers (SiPMs) that convert the photons to an electrical signal. Custom electronics are used to gather, amplify, process, and readout the signal. A library of several neutron response curves was created in Geant4 and MCNP. The experimental output of the spectrometer was unfolded using a maximum entropy algorithm, MAXED. The spectrometer was tested using two separate DD generators. These two tests resulted in unfolded neutron spectra with average neutron energies of 2.71 and 2.78 MeV and chi-squared values of 0.88 and 1.51 χ 2 /D.O.F. respectively, when fit to a 2.45 MeV monoenergetic energy spectrum.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2013

STAYSL PNNL Suite

The STAYSL PNNL Suite of software provides a set of tools for working with neutron activation rates measured in a nuclear fission reactor, an accelerator-based neutron source, or any neutron field to determine the neutron flux spectrum through a generalized least-squares approach. This process is referred to as neutron spectral adjustment since the preferred approach is to use measured data to adjust neutron spectra provided by neutron physics calculations. The input data consist of the reaction rates based on measured activities, an initial estimate of the neutron flux spectrum, neutron activation cross sections and their associated uncertainties (covariances), and relevant correction factors. The output consists of the adjusted neutron flux spectrum and associated covariance matrix, which is useful for neutron dosimetry and radiation damage calculations. The software suite consists of the STAYSL PNNL, SHIELD, BCF, and NJpp Fortran codes and the SigPhi Calculator spreadsheet tool. In addition, the development of this software suite and associated data libraries used the third-party NJOY99 Fortran code (http://t2.lanl.gov/nis/codes/njoy99/). The NJOY99 and NJpp codes are used to assemble cross section and covariance input data libraries (for both SHIELD and STAYSL PNNL) from the International Reactor Dosimetry File of 2002 (IRDF-2002; http://www-nds.iaea.org/irdf2002/) developed by the Nuclear Data Section of the International Atomic Energy Agency (Vienna, Austria). The BCF, SigPhi Calculator, and SHIELD software tools are used to calculate corrected activation rates and neutron self-shielding correction factors, which are inputs to the STAYSL PNNL code.

Greenwood, L.R.↗
DOE OSTI2017

Latest Results from DIII-D and Their Implications for Future Devices

The DIII-D Tokamak has become one of the major sources of physics and technology data for the design of future large machines such as ITER and CIT. In large part this is because of its extremely flexible design and the ability to run tests or add new diagnostic devices with a minimum of down-time and expense. Fundamental plasma physics studies are still the major focus of our experimental program, but increasingly, we are looking at new ways to answer the complex fusion technology questions emerging from the design studies for the next-generation devices. Recent results have demonstrated world record beta plasmas, long quiescent H-mode operation, partial noninductive current drive using both neutral beam and rf power injection, single- and double-null divertor operation, and divertor particle- and heat-load management. The recently installed Advanced Divertor hardware will allow critical transport experiments to be run with independent control of the density. It will also permit the concept of dc helicity injection current drive to be tested. This paper summarizes our most important recent findings and also outlines a few of the many interesting problems that are now under study to address fusion technology questions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2013

User Guide for the STAYSL PNNL Suite of Software Tools

The STAYSL PNNL software suite provides a set of tools for working with neutron activation rates measured in a nuclear fission reactor, an accelerator-based neutron source, or any neutron field to determine the neutron flux spectrum through a generalized least-squares approach. This process is referred to as neutron spectral adjustment since the preferred approach is to use measured data to adjust neutron spectra provided by neutron physics calculations. The input data consist of the reaction rates based on measured activities, an initial estimate of the neutron flux spectrum, neutron activation cross sections and their associated uncertainties (covariances), and relevant correction factors. The output consists of the adjusted neutron flux spectrum and associated covariance matrix, which is useful for neutron dosimetry and radiation damage calculations.

Reactor dosimetry, neutron spectral adjustment↗
DOE OSTI2015

Chi-Nu Level 2 Review

This series of slides presents information on Chi-Nu measurements and analysis of prompt fission neutron spectra (PFNS) for neutron energy below 1 MeV for 235 U. A key focus of the Chi-Nu measurement is to address the energy dependence of the low-energy emissions. The 235 U PFNS evaluation is in progress. Chi-Nu delivered preliminary experimental data and input for part of the old experimental data base. The 239 Pu PFNS evaluation is finalized and submitted for testing. Data from 252 Cf spontaneous fission will also be obtained.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2013

Analysis of Neutron Fluence Monitors for The USU ATR NSUF Project

The USU (Utah State University) Advanced Test Reactor Nation Science User Facility (ATR NSUF) experiments to test the performance of hafnium-aluminum composites were conducted in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL) during cycles 149A through 151A from April 14, 2011, to February 13, 2012. Four sets of two neutron fluence monitor capsules wee irradiated in four different combinations of reactor cycles. The assemblies were irradiated in B2 position of the ATR. Neutron fluence monitors were located at 8 positions in the assemblies. These monitors were previously fabricated at Pacific Northwest National Laboratory (PNNL). After irradiation, the monitors were sent to PNNL for analysis. The measured activation rates were used to adjust the neutron spectra at each location in the assemblies to determine the best fit to the neutron fluence spectra. Radiation damage (dpa) calculations were performed at all locations using the adjusted neutron spectra. The report was revised after receipt of corrected irradiation history for Cycle 149A. A plot of the fast neutron flux as a function of height in the B2 position was also added to the report.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2018

Improved yield and control of spectra from high-intensity laser-generated neutron beams

Abstract Kinetic modeling of laser-ion beam generation from the “break-out afterburner” (BOA) has been modeled for several deuteron-rich solid-density target foils. Modeling the transport of these beams in a beryllium converter shows as much as a fourfold increase in neutron yield over the present state of the art through the use of alternative target materials. Additionally, species-separation dynamics during the BOA can be exploited to control the hardness of the neutron spectra, of interest for, for example, enhancing penetrability in shielded material in active neutron interrogation settings.

laser based neutron sources, active interrogation↗
DOE OSTI2015

Recent Work Leading Towards a New Evaluation of the Neutron Standards

A new version of the ENDF/B library has been planned. The first step in producing this new library is evaluating the neutron standards. An evaluation is now underway with support from a Data Development Project of the IAEA. In addition to the neutron cross section standards, new evaluations are being done for prompt fission neutron spectra and a number of reference data. Efforts have been made to handle uncertainties in a proper way in these evaluations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2014

Phonon self-energy and origin of anomalous neutron scattering spectra in SnTe and PbTe thermoelectrics

The anharmonic lattice dynamics of rock-salt thermoelectric compounds SnTe and PbTe are investigated with inelastic neutron scattering (INS) and first-principles calculations. The experiments show that, surprisingly, although SnTe is closer to the ferroelectric instability, phonon spectra in PbTe exhibit a more anharmonic character. This behavior is reproduced in first-principles calculations of the temperature-dependent phonon self-energy. Our simulations reveal how the nesting of phonon dispersions induces prominent features in the self-energy, which account for the measured INS spectra and their temperature dependence. We establish that the phase-space for three-phonon scattering processes, rather than just the proximity to the lattice instability, is the mechanism determining the complex spectrum of the transverse-optical ferroelectric mode.

first-principles simulations↗