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At least 163 records · Page 9

Radiation Transmission Properties of In-Situ Materials

The development of a permanent human presence in space is a key element of NASA's strategic plan for the Human Exploration and Development of Space (HEDS). The habitation of the International Space Station (ISS) is one near-term HEDS objective; the exploration and settlement of the moon and Mars are long-term goals of that plan. Achieving these goals requires maintaining the health and safety of personnel involved in such space operations at a high level, while at the same time reducing the cost of those operations to a reasonable level. Among the limiting factors to prolonged human space operations are the health risks from exposure to the space ionizing radiation environment. In order to keep the risk of radiation induced cancer at acceptable levels, it is necessary to provide adequate shielding from the ionizing radiation environment. The research presented here is theoretical and ground-based experimental study of the neutron production from interactions of GCR-like particles in various shielding components. An emphasis is placed here on research that will aid in the development of in-situ resource utilization. The primary goal of the program is to develop an accurate neutron-production model that is relevant to the NASA HEDS program of designing technologies that will be used in the development of effective shielding countermeasures. A secondary goal of the program is the development of an experimental data base of neutron production cross sections and thick-target yields which will aid model development.

Heilbronn, L.↗

Lunar and Planetary Science XXXVI, Part 13

Contents include the following: A Fast, Non-Destructive Method for Classifying Ordinary Chondrite Falls Using Density and Magnetic Susceptibility. An Update on Results from the Magnetic Properties Experiments on the Mars Exploration Rovers, Spirit and Opportunity. Measurement Protocols for In Situ Analysis of Organic Compounds at Mars and Comets. Piping Structures on Earth and Possibly Mars: Astrobiological Implications. Uranium and Lead in the Early Planetary Core Formation: New Insights Given by High Pressure and Temperature Experiments. The Mast Cameras and Mars Descent Imager (MARDI) for the 2009 Mars Science Laboratory. MGS MOC: First Views of Mars at Sub-Meter Resolution from Orbit. Analysis of Candor Chasma Interior Layered Deposits from OMEGA/MEX Spectra. Analysis of Valley Networks on Valles Marineris Plateau Using HRSC/MEX Data. Solar Abundance of Elements from Neutron-Capture Cross Sections. Preliminary Evaluation of the Secondary Ion/Accelerator Mass Spectrometer, MegaSIMS. Equilibrium Landforms in the Dry Valleys of Antarctica: Implications for Landscape Evolution and Climate Change on Mars. Continued Study of Ba Isotopic Compositions of Presolar Silicon Carbide Grains from Supernovae. Paleoenviromental Evolution of the Holden-Uzboi Area. Stability of Magnesium Sulfate Minerals in Martian Environments. Tungsten Isotopic Constraints on the Formation and Evolution of Iron Meteorite Parent Bodies. Migration of Dust Particles and Volatiles Delivery to the Inner Planets. On the Sitting of Trapped Noble Gases in Insoluble Organic Matter of Primitive Meteorites. Trapping of Xenon Upon Evaporation-Condensation of Organic Matter Under UV Irradiation: Isotopic Fractionation and Electron Paramagnetic Resonance Analysis. Stability of Water on Mars. A Didactic Activity. Analysis of Coronae in the Parga Chasma Region, Venus. Photometric and Compositional Surface Properties of the Gusev Crater Region, Mars, as Derived from Multi-Angle, Multi-Spectral Investigation of Mars Express HRSC Data. Mapping Compositional Diversity on Mars: Spatial Distribution and Geological Implications. A New Simulation Chamber for Studying Planetary Environments. Folded Structure in Terra Sirenum. Mars. Nitrogen-Noble Gas Static Mass Spectrometry of Genesis Collector Materials. Neon Isotope Heterogeneity in the Terrestrial Mantle: Implication for the Acquisition of Volatile Elements in Terrestrial Planets. The Cosmic Clock, the Cycle of Terrestrial Mass Extinctions.

Source record↗

Additive Manufacture of Porous ZrC for NTP In-Core Insulators

Nuclear Thermal Propulsion (NTP) requires the use of in-core insulators to manage to thermal environment between high temperature fuel elements and lower temperature structural components. The unforgiving in-core operating conditions severely limit potential material candidates. Zirconium Carbide (ZrC) is a promising candidate due to a high melting temperature, high compressive strength, hardness, wear resistance, hydrogen compatibility, and low neutron absorption cross sections. However, fully dense ZrC is not an insulator but it has been found that the thermal conductivity of ZrC decreases by increasing porosity to approximately 60 % theoretical density (%TD). Previous methods for generating porous ZrC were difficult, expensive, and time consuming. Binder jet additive manufacture (AM) can print ceramic materials to near net shape. Binder jet AM is not utilized in many applications due to an inherently low post-sintering density on the order of 60 %TD. For this specific application the inherent lower density is leveraged as an advantage in production porous ZrC in order to control the thermal conductivity. A feasibility study was conducted to investigate binder jet AM parameter development for ZrC, heat treatment optimization (burn-out and sinter), microstructural characterization, mechanical testing, and thermal testing to generate near-net shape ZrC components with ~60 %TD with the desired thermal conductivity and mechanical strength.

Omar Mireles↗

Additive Manufacture of Porous Zirconium Carbide for Nuclear Thermal Propulsion In-Core Insulators

Nuclear Thermal Propulsion (NTP) requires the use of in-core insulators to manage to thermal environment between high temperature fuel elements and lower temperature structural components. The unforgiving in-core operating conditions severely limit potential material candidates. Zirconium Carbide (ZrC) is a promising candidate due to a high melting temperature, high compressive strength, hardness, wear resistance, hydrogen compatibility, and low neutron absorption cross sections. However, fully dense ZrC is not an insulator but it has been found that the thermal conductivity of ZrC decreases by increasing porosity to approximately 60 % theoretical density (%TD). Previous methods for generating porous ZrC were difficult, expensive, and time consuming. Binder jet additive manufacture (AM) can print ceramic materials to near net shape. Binder jet AM is not utilized in many applications due to an inherently low post-sintering density on the order of 60 %TD. For this specific application the inherent lower density is leveraged as an advantage in production porous ZrC in order to control the thermal conductivity. A feasibility study was conducted to investigate binder jet AM parameter development for ZrC, heat treatment optimization (burn-out and sinter), microstructural characterization, mechanical testing, and thermal testing to generate near-net shape ZrC components with ~60 %TD with the desired thermal conductivity and mechanical strength.

Zirconium Carbide Additive Manufacture↗

Additive Manufacture of Porous Zirconium Carbide for Nuclear Thermal Propulsion In-Core Insulators

Nuclear Thermal Propulsion (NTP) requires the use of in-core insulators to manage to thermal environment between high temperature fuel elements and lower temperature structural components. The unforgiving in-core operating conditions severely limit potential material candidates. Zirconium Carbide (ZrC) is a promising candidate due to a high melting temperature, high compressive strength, hardness, wear resistance, hydrogen compatibility, and low neutron absorption cross sections. However, fully dense ZrC is not an insulator but it has been found that the thermal conductivity of ZrC decreases by increasing porosity to approximately 60 % theoretical density (%TD). Previous methods for generating porous ZrC were difficult, expensive, and time consuming. Binder jet additive manufacture (AM) can print ceramic materials to near net shape. Binder jet AM is not utilized in many applications due to an inherently low post-sintering density on the order of 60 %TD. For this specific application the inherent lower density is leveraged as an advantage in production porous ZrC in order to control the thermal conductivity. A feasibility study was conducted to investigate binder jet AM parameter development for ZrC, heat treatment optimization (burn-out and sinter), microstructural characterization, mechanical testing, and thermal testing to generate near-net shape ZrC components with ~60 %TD with the desired thermal conductivity and mechanical strength.

Zirconium Carbide Additive Manufacture↗

New constraint on the Np 237 ( n , γ ) Np 238 integral cross section using the Godiva-IV critical assembly

Accurate knowledge of the 237 Np(n, γ) 238 Np cross section at fast neutron energies is important for applied nuclear science. The presently available experimental data has large disagreements in the fast neutron region. Perform a model-independent measurement of the 237 Np(n, γ) 238 Np integral cross section using a well characterized fast neutron source and compare the result with previous measurements and current nuclear data evaluations. Provide an integral measurement that can be used as a benchmark for current evaluations. Multiple samples of 237 Np were irradiated in the Godiva-IV critical assembly. Following the irradiation, the samples placed in a γ-ray counting setup and the γ-rays emitted from the decay of 238 Np were measured over a time period of approximately 7 days. Multiple γ-ray decay branches of 238 Np were observed. The observed activity of 238 Np was used to calculate the amount of 238 Np produced during the irradiation via the 237 Np(n, γ) 238 Np reaction and an integral cross section of 342(11) mb was measured for the Godiva-IV neutron spectrum. Further, the 238 Np half-life has been measured with a result of 50.31(5) hours. The 237 Np(n, γ) 238 Np integral cross section measured in this work is in agreement with overlapping 1σ error bands to ENDF/B-VIII.0. However, the measured value is 3σ away from the calculated integral cross section using JENDL-5. This measurement offers a reliable benchmark for future 237 Np(n, γ) 238 Np cross section evaluations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Experimental uncertainty quantification using templates of expected measurement uncertainties for fast neutron-induced total, capture, and scattering cross sections

Careful experimental uncertainty quantification (UQ) is key for developing trustworthy evaluated nuclear data. Templates to account for missing or under-reported experimental uncertainties were recently developed by the covariance committee of Cross Section Evaluation Working Group (CSEWG). In this work, we illustrate the practical application and limitations of these templates for selected neutron-induced reactions, including (n, tot), (n, γ), and (n, xn) in the fast energy range, to illustrate their use in data analyses for nuclear data evaluations. We show that while the templates provide consistent framework, proper implementation still requires detailed knowledge of experimental conditions and careful treatment of nonlinear effects in cross section derivation. Case studies highlight how template-assisted UQ improves consistency with previous evaluations such as ENDF/B and reveals open challenges in propagating uncertainties across different energy regimes. The main contribution of this paper is to connect formal template recommendations with their use in practical evaluation workflows, clarifying both their benefits and current limitations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Fission foil detector calibrations with high energy protons

Fission foil detectors (FFD's) are passive devices composed of heavy metal foils in contact with muscovite mica films. The heavy metal nuclei have significant cross sections for fission when irradiated with neutrons and protons. Each isotope is characterized by threshold energies for the fission reactions and particular energy-dependent cross sections. In the FFD's, fission fragments produced by the reactions are emitted from the foils and create latent particle tracks in the adjacent mica films. When the films are processed surface tracks are formed which can be optically counted. The track densities are indications of the fluences and spectra of neutrons and/or protons. In the past, detection efficiencies have been calculated using the low energy neutron calibrated dosimeters and published fission cross sections for neutrons and protons. The problem is that the addition of a large kinetic energy to the (n,nucleus) or (p,nucleus) reaction could increase the energies and ranges of emitted fission fragments and increase the detector sensitivity as compared with lower energy neutron calibrations. High energy calibrations are the only method of resolving the uncertainties in detector efficiencies. At high energies, either proton or neutron calibrations are sufficient since the cross section data show that the proton and neutron fission cross sections are approximately equal. High energy proton beams have been utilized (1.8 and 4.9 GeV, 80 and 140 MeV) for measuring the tracks of fission fragments emitted backward and forward.

Benton, E. V.↗

A compact, low-power epithermal neutron counter for lunar water detection

The detection and characterization of lunar water are critical for enabling sustainable human and robotic exploration of the Moon. Orbital neutron spectrometers, such as instruments on Lunar Prospector and the Lunar Reconnaissance Orbiter, have revealed hydrogen-rich regions near the poles but are limited by coarse spatial resolution and low counting efficiency. We present a compact, lightweight, and low-power epithermal neutron detector based on boron-coated silicon imagers, designed to probe subsurface hydrogen at decimeter scales from mobile platforms such as lunar rovers. This instrument leverages the high neutron capture cross-section of 10 B to convert epithermal neutrons into detectable α and 7 Li ions in a fully-depleted silicon imager, providing a unique event topology to identify neutrons while suppressing backgrounds. Monte Carlo simulations demonstrate that a 3 μm boron layer achieves optimal neutron detection efficiency, further enhanced with polyethylene moderation to improve sensitivity to the 0.4 eV–500 keV epithermal energy range. For a 10 cm 2 active area, the detector achieves sensitivity to H 2 O weight fractions as low as 0.01 wt% in a 15 minute measurement. This scalable, portable, low-mass design is well-suited for integration into upcoming Artemis and commercial lunar rovers, providing a transformative capability for in-situ resource prospecting and ground-truth validation of orbital measurements.

Detector modelling and simulations I (interaction ↗

Light Ion Double-Differential Cross Sections for Space Radiation

Neutrons and light ions have been shown to make large contributions to space radiation dose equivalent for realistic shielding scenarios. However, there are considerable uncertainties in the calculation of light ion production. Efficient and accurate calculation of light ion double-differential cross sections are required for input into space radiation transport codes. A thermal proton cross section model is developed which includes proton production from the 3 sources of projectile, central fireball, and target. It is shown that this 3-source model is able to explain the low-momentum, small-angle shoulder seen in proton spectra. Using the coalescence model, the thermal proton model is used to calculate light ion double-differential cross sections for use in space radiation transport codes. The 3-source model is also seen to be essential to explain the light ion shoulders, which are even more pronounced than the proton shoulders. Extensive comparisons between models and experimental measurements are shown and necessary future work is discussed.

Norbury, John W.↗

Fine Temperature Grid Continuous Energy Cross Section Generation for Monte Carlo Analysis of Xe-100 Design

The standard “A Compact ENDF (ACE)” data libraries used by Monte Carlo based reactor physics codes calculations are provided by Los Alamos National Laboratory (LANL) with a temperature interval mostly of 300 K (e.g. 300 K, 600 K, 900 K) for the cross sections and between 100 K and 200 K for the thermal scattering libraries (TSL). However, some codes such as MCNP lack capability to perform on-the-fly temperature interpolation during simulation both for neutron and TSL cross-sections. To evaluate the impact related to Doppler broadening and spectrum shift associated with TSL changes, this paper explores the potential of adopting a temperature grid finer than the ones contained in the standard data libraries. A 50 K temperature grid was employed to quantify the error in neutronics calculations due to temperature grid resolution. This was achieved by comparing the results of this study (50 K temperature interval) against the results obtained with standard data libraries (>100 K temperature interval). While the adopted grid primarily relies on the ENDF/B-VII.1 library, for neutron cross-sections, it utilizes ENDF/B-VIII.0 library for TSL. The analyses confirmed that the accuracy of neutronics calculations is satisfactory when using a 50 K temperature grid. Notably, adopting a 50 K temperature grid, as opposed to standard libraries or coarser temperature grids, could lead to a difference of no more than a few hundred pcm in dk for both fresh fuel and burnt fuel. The most sensitive reaction type to the temperature grid was as expected identified as the capture cross-section of U-238.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Neutron-induced capture-to-fission cross section ratio measured at LANSCE

Capture-to-fission cross section ratios are used as an alternative to absolute cross section measurements. This is due to the simplification on the calculations and the reduction of the uncertainties with respect to an absolute measurement of the cross section by eliminating experimental complications like self-absorption, beam/target overlap and non-uniformities. Different capture-to-fission reactions have been measured through the years at the Los Alamos Neutron Science Center (LANSCE) at Los Alamos National Laboratory (LANL) using the Detector for Advanced Neutron Capture Experiments (DANCE) combined with different fission detectors. Some of these are a Parallel Plate Avalanche Counter (PPAC) to detect fission fragments (FF), and the NEUtron detector array at DANCE (NEUANCE) to detect fission neutrons. As DANCE detects the γ-rays produced in capture and fission reactions, the fission instrument placed inside the DANCE cavity is used to tag the fission γ-rays for background identification and subtraction. Some examples of capture-to-fission ratio measurements performed with DANCE in the last years are the 233 U, 235 U and 239 Pu. The measurement technique, the different setups, and other potential applications of the instruments will be explained.

Nuclear Criticality Safety Program (NCSP)↗

An integral test of the inelastic cross sections of Pb and Mo using measured neutron spectra

Comparison of measurements and calculations of fast neutron spectra from a radioactive neutron source inside spheres of Mo or Pb and from a cylindrical reactor containing a thick Pb or Mo reflector are used as a test of ENDF cross sections. The sphere leakage spectra were measured at a sphere-to-spectrometer distance of 2 meters using a 54 Ci spherical Am-Be neutron source. Reactor leakage spectrum measurements were made at the surface of the ZP-1 reactor when bare, with a Pb radial reflector 21 cm thick, and with a metallic Mo radial reflector 10 cm thick. In the case of the thin Mo sphere there is agreement between the calculation and measurement. The Pb calculation is much lower than the measurement except at the highest neutron energy. Two-dimensional calculations of reactor spectra result indicate that the reactor source is reasonably well known. Significant differences in leakage spectrum shape for both Mo and Pb reflectors suggest that there are large uncertainties in the inelastic cross sections for Pb and some for Mo.

Shook, D. F.↗

Benchmarking fast-neutron response of 7 Li-enriched C 7 LYC scintillators: Simulations and experiment

New insights into the fast neutron response of 7 Li-enriched C 7 LYC scintillators have been obtained through detailed Geant4 simulations of 35 Cl(n,p) and 35 Cl(n, α) reactions that are primarily responsible for the fast neutron response of C 7 LYC. The light output of a 1” x1” C 7 LYC detector was simulated using the Birks equation for light quenching in scintillators. The simulations were benchmarked against neutron scattering data from a 12 C target obtained with a white neutron beam at the Los Alamos LANSCE facility and fourteen 1”x1” C 7 LYC detectors. Incident neutron energies extracted from time-of-flight measurements, and appropriate recoil corrections for the different detector angles were used to map the response of C 7 LYC to mono-energetic neutrons. Resonances in the 35 Cl(n,p) reaction cross-section below 3 MeV incident neutron energy were directly observed in C 7 LYC. The experimental data and simulations are compared with ENDF databases, as well as recent direct cross-section measurements of neutrons scattered from a 35 Cl target. In conclusion, the results suggest a scrutiny of the 35 Cl(n,p) and 35 Cl(n, α) cross sections at low energy in the ENDF library.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Discovery of new isotopes in the fragmentation of 82 Se and insights into their production

The production cross sections of neutron-rich nuclei for elements just above 60 Ca were measured at the Facility for Rare Isotope Beams (FRIB). Four previously unobserved isotopes ( 63 Sc, 65,66 Ti, and 68 V) were produced, separated, and identified for the first time using the Advanced Rare Isotope Separator (ARIS). One event was found to be consistent with 61 Ca . The new isotopes were created through the interaction of an 82 Se beam with a carbon target at an energy of 228 MeV/𝑢 and a primary beam current of 1.07 p⁢µ⁢A. The event-by-event particle identification of the mass number (𝐴), atomic number (𝑍), and ionic charge state (𝑞) for the reaction products was achieved by combining measurements of energy loss, time of flight, magnetic rigidity, and total kinetic energy. This successful search for new isotopes, conducted at the beginning of FRIB's third year of operation, highlights the facility's discovery potential, which will continue to grow as the beam current increases. The production cross sections were analyzed in the context of the newly developed Δ⁢𝐵⁢𝐸 systematics that provides trends in neutron-rich regions and increased sensitivity to nuclear binding, an important nuclear structure observable. Furthermore, the new systematics addresses gaps in 𝑄 𝑔 -based methods commonly used to interpret the production cross sections of light neutron-rich elements, and provides an efficient empirical approach to describe cross-section trends across isotopic chains. Good agreement with the measured data was obtained when the Δ⁢𝐵⁢𝐸 systematics and abrasion-ablation calculations were performed using the Hartree-Fock-Bogoliubov (HFB-22) mass table.

59 ≤ A ≤ 89↗

Neutron capture production rates of cosmogenic 60Co, 59Ni and 36Cl in stony meteorites

Results for neutron flux calculations in stony meteoroids (of various radii and compositions) and production rates for Cl-36, Ni-59, and Co-60 are reported. The Ni-59/Co-60 ratio is nearly constant with depth in most meteorites: this effect is consistent with the neutron flux and capture cross section properties. The shape of the neutron flux energy spectrum, varies little with depth in a meteorite. The size of the parent meteorite can be determined from one of its fragments, using the Ni-59/Co-60 ratios, if the parent meteorite was less than 75 g/cm(2) in radius. If the parent meteorite was larger, a lower limit on the size of the parent meteorite can be determined from a fragment. In C3 chondrites this is not possible. In stony meteorites with R less than 50 g/cm(2) the calculated Co-60 production rates (mass less than 4 kg), are below 1 atom/min g-Co. The highest Co-60 production rates occur in stony meteorites with radius about 250 g/cm(2) (1.4 m across). In meteorites with radii greater than 400 g/cm(2), the maximum Co-60 production rate occurs at a depth of about 175 g/cm(2) in L-chondrite, 125 g/cm(2) in C3 chrondrite, and 190 g/cm(2) in aubrites.

Spergel, M. S.↗