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At least 163 records · Page 9

Convolutional neural network based non-iterative reconstruction for accelerating neutron tomography *

Abstract Neutron computed tomography (NCT), a 3D non-destructive characterization technique, is carried out at nuclear reactor or spallation neutron source-based user facilities. Because neutrons are not severely attenuated by heavy elements and are sensitive to light elements like hydrogen, neutron radiography and computed tomography offer a complementary contrast to x-ray CT conducted at a synchrotron user facility. However, compared to synchrotron x-ray CT, the acquisition time for an NCT scan can be orders of magnitude higher due to lower source flux, low detector efficiency and the need to collect a large number of projection images for a high-quality reconstruction when using conventional algorithms. As a result of the long scan times for NCT, the number and type of experiments that can be conducted at a user facility is severely restricted. Recently, several deep convolutional neural network (DCNN) based algorithms have been introduced in the context of accelerating CT scans that can enable high quality reconstructions from sparse-view data. In this paper, we introduce DCNN algorithms to obtain high-quality reconstructions from sparse-view and low signal-to-noise ratio NCT data-sets thereby enabling accelerated scans. Our method is based on the supervised learning strategy of training a DCNN to map a low-quality reconstruction from sparse-view data to a higher quality reconstruction. Specifically, we evaluate the performance of two popular DCNN architectures—one based on using patches for training and the other on using the full images for training. We observe that both the DCNN architectures offer improvements in performance over classical multi-layer perceptron as well as conventional CT reconstruction algorithms. Our results illustrate that the DCNN can be a powerful tool to obtain high-quality NCT reconstructions from sparse-view data thereby enabling accelerated NCT scans for increasing user-facility throughput or enabling high-resolution time-resolved NCT scans.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Final Report for Grant

This is the final report for this project. The major objectives were to develop full models and standard cells of CMOS silicon photomultipliers (SiPM) for neutron detection applications. Specifically, the research seeks to replace photomultiplier tubes, used in neutron detection applications, with SiPMs containing integrated readout electronics fabricated in standard CMOS processes. The detectors improve on the detection efficiency, readout speed, resolution (sensitivity), and spatial resolution of current systems. In particular, this work involved collaboration with the instrument and detector group at ORNL who build detectors based on discrete commercially available PMTs and SiPMs. The SiPM detectors developed in this work are based on Perimeter Gated Single Photon Avalanche Diodes (PGSPAD). These devices have tunable breakdown voltage which affects other performance characteristics of the detectors. The ability of the detectors to have integrated readout and tune the noise floor and dynamic range in addition to offering a method for non-uniformity compensation in a compact form significantly impacts the imaging research field and includes the nuclear sciences field, circuits and systems field in addition to varied fields such as geography and biology/medicine.

42 ENGINEERING↗

Prediction and observation of intermodulation sidebands from anharmonic phonons in NaBr

A quantum Langevin model, like models from optomechanics, was developed for phonons. It predicts intermodulation phonon sidebands (IPSs) in anharmonic crystals. Ab initio calculations of anharmonic phonons in rock-salt NaBr showed these spectral features as many-body effects. Modern inelastic neutron scattering measurements on a crystal of NaBr at 300 K revealed diffuse intensity at high phonon energy from a predicted upper IPS. The transverse optical (TO) part of the new features originates from phonon intermodulation between the transverse acoustic (TA) and TO phonons. The longitudinal optical spectral features originate from three-phonon coupling between the TA modes and the TO lattice modes. The partner lower IPS proves to be an intrinsic localized mode. Interactions with the thermal bath broaden and redistribute the spectral weight of the IPS pair. These sidebands are a probe of the anharmonicity and quantum noise of phonons in NaBr and suggest novel interactions between photons and phonons.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

The APOGEE Data Release 16 Spectral Line List

The updated H-band spectral-line list (from λ15000–17000) adopted by the Apache Point Observatory Galactic Evolution Experiment (APOGEE) for the SDSS-IV Data Release 16 (DR16) is presented in this work. The APOGEE line list is a combination of atomic and molecular lines, with data drawn from laboratory, theoretical, and astrophysical sources. Oscillator strengths and damping constants are adjusted using high signal-to-noise, high-resolution spectra of the Sun, and α Boo (Arcturus), as “standard stars.” Updates to the DR16 line list, as compared to the previous DR14 version, include the addition of molecular H{sub 2}O and FeH lines, as well as a much larger (by a factor of ∼4) atomic line list, including a significantly greater number of transitions with hyperfine splitting. More recent references and line lists for the crucial molecules, CO and OH, as well as for C{sub 2} and SiH, are also included. In contrast to DR14, DR16 contains measurable lines from the heavy neutron-capture elements cerium (as Ce ii), neodymium (as Nd ii), and ytterbium (as Yb ii), as well as one line from rubidium (as Rb i), which may be detectable in a small fraction of APOGEE red giants.

74 ATOMIC AND MOLECULAR PHYSICS↗

Optimal Control for the Quantum Simulation of Nuclear Dynamics

We propose a method for enacting the unitary time propagation of two interacting neutrons at leading order of chiral effective-field theory by efficiently encoding the nuclear dynamics into a single multilevel quantum device. The emulated output of the quantum simulation shows that, by applying a single gate that draws on the underlying characteristics of the device, it is possible to observe multiple cycles of the nuclear dynamics before the onset of decoherence. Owing to the signal's longevity, we can then extract spectroscopic properties of the simulated nuclear system. This allows us to validate the encoding of the nuclear Hamiltonian and the robustness of the simulation in the presence of quantum-hardware noise by comparing the extracted spectroscopic information to exact calculations. This work paves the way for transformative calculations of the dynamical properties of nuclei on near-term quantum devices.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Using quantum noise correlation analysis to measure ion temperature

Quantum noise correlation analysis was tested at the proof-of-concept level as a technique to measure ion temperature in a plasma. If eventually successful, this technique could enable a compact, inexpensive, and robust ion temperature diagnostic suitable for a burning plasma environment. Ion temperature is a key parameter determining the fusion performance of a burning plasma, as the fusion cross-section has a strong dependence on ion temperature. This ion temperature diagnostic would require only a small optical view of the plasma through a port to passively record impurity line emission. The instrumentation would be remote from the reactor behind the neutron and bio-shielding. The technique relies solely on quantum correlations of the photons emitted by a plasma impurity to measure ion temperature; there is no grating dispersion of an emission line-width or pulse-height analysis of photon energy. This measurement innovation was tested with instrumentation consisting of two single-photon detectors with high timing resolution, a time-tagging unit, and simple light collection optics. This instrumentation measures the second-order correlation between the light intensity falling on the two detectors. The next steps beyond the proof-of-concept level will be development of diagnostic designs for application of this technique to high-temperature and burning plasmas. Arrays of single-photon avalanche detectors to multiplex measurements of photon correlation will be required to reduce signal integration time to an acceptable duration.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Comparing Control Performance Between Simulation and Experiment using the Microreactor Automated Control System Testbed

In the advanced reactor domain, a flexible and scalable software/hardware infrastructure is crucial for integrating and validating various control technologies. This study used the Microreactor Automated Control System (MACS) hardware platform as a testbed. MACS was originally designed to mirror Idaho National Laboratory (INL)'s Microreactor Applications Research Validation and Evaluation (MARVEL), a 85-kW thermal fission microreactor. It features control drums for simulated reactivity control; lights that function as a surrogate reactor core, with the brightness being proportional to the reactor power; and light sensors that emulate neutron detectors. To transform MACS into a physical twin of MARVEL for evaluating control methods, the Control and Optimization Modular Modeling Application for Nuclear Deployment (COMMAND) software was employed. This software integrated the hardware with two models of the MARVEL core, based on Reactor Excursion and Leak Analysis Program (RELAP5-3D) and Monte Carlo N-Particle (MCNP) models. The study aimed to demonstrate the gap between control theory and actual practice—a gap that often necessitates empirical adjustments such as control gain retuning, filters, time discretization, and integrator anti-windup measures. Controllers were developed based on increasingly complex simulations without hardware, starting from the base MARVEL model and then introducing actuator saturation constraints and sensor noise. The final control strategy was then tested using MACS, and a comparative performance analysis was conducted.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗

Control optimization for parametric Hamiltonians by pulse reconstruction

Optimal control techniques provide a means to tailor the control pulses required to generate customized quantum gates, which helps to improve the resilience of quantum simulations to gate errors and device noise. However, the significant amount of (classical) computation required to generate customized gates can quickly undermine the effectiveness of this approach, especially when pulse optimization needs to be iterated. We propose a method to reduce the computational time required to generate the control pulse for a Hamiltonian that is parametrically dependent on a time-varying quantity. We use simple interpolation schemes to accurately reconstruct the control pulses from a set of pulses obtained in advance for a discrete set of predetermined parameter values. We obtain a reconstruction with very high fidelity and a significant reduction in computational effort. We report the results of the application of the proposed method to device-level quantum simulations of the unitary (real) time evolution of two interacting neutrons based on superconducting qubits.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Two methods to study inelastic neutron-scattering measurements based on ω n (q) versus S(q, ω) applied to the magnetic open honeycomb lattice Tb 2 Ir 3 Ga 9

This work describes two methods to fit the inelastic neutron-scattering spectrum S(q, ω) with wavevector q and frequency ω. The common and well-established method extracts the experimental spin-wave branches ω n (q) from the measured spectra S(q, ω) and then minimizes the difference between the observed and predicted frequencies. When n branches of frequencies are predicted but the measured frequencies overlap to produce only m < n branches, the weighted average of the predicted frequencies must be compared to the observed frequencies. A penalty is then exacted when the width of the predicted frequencies exceeds the width of the observed frequencies. The second method directly compares the measured and predicted intensities S(q, ω) over a grid {q i , ω j } in wavevector and frequency space. After subtracting background noise from the observed intensities, the theoretical intensities are scaled by a simple wavevector-dependent function that reflects the instrumental resolution. Furthermore, the advantages and disadvantages of each approach are demonstrated by studying the open honeycomb material Tb 2 Ir 3 Ga 9 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

High-bandwidth frequency domain multiplexed readout of transition-edge sensors for neutrinoless double beta decay searches

The next-generation of cryogenic neutrinoless double-beta decay experiments require increasingly fast readout in order to improve background discrimination. These experiments, operated as cryogenic calorimeters at ∼ 10 mK, are usually read out by high-impedance neutron transmutation doped (NTD) thermistors, which provide good energy resolution, but are limited by ∼ 1 ms response times. Superconducting detectors, such as transition-edge sensors (TESs) with a time resolution of ∼ 100 μs, offer superior timing performance over NTD semiconductor bolometers. To make this technology viable for an application to a thousand or more channels, multiplexed readout is necessary in order to minimize the thermal load and radioactive contamination induced by the readout. Frequency-domain multiplexing readout (fMUX) for TESs, previously developed at Berkeley Lab and McGill University, is currently in use for mm-wave telescopes with detector sampling rates in the order of 100 Hz. We demonstrate a new readout system, based on the McGill/Berkeley digital fMux readout, to satisfy the higher bandwidth and noise requirements of the next generation of TES-instrumented cryogenic calorimeters. Each multiplexing readout module comprises 10 superconducting resonators in the 1–5 MHz range and a DC superconducting quantum interference device (DC-SQUID), interfaced to high-speed field programmable gate array (FPGA)-based electronics for digital signal processing and low-latency SQUID feedback. The new readout samples detectors at 156 kHz, three orders of magnitude faster than its cosmology-oriented predecessor, and demonstrates a stable feedback bandwidth of 3 kHz in a real TES-based system.

47 OTHER INSTRUMENTATION↗

Novel Signatures Beyond the Standard Model: From Extreme Environments to Precision Measurements

Most of our universe is dark. It is dark literally—visible matter makes up only 5% of the energy density—and conceptually, as many outstanding questions remain unsolved. The discovery of particle dark matter would shed light on our dark universe and throw open a window on the highest energy scales. This research made progress toward dark matter and new particle searches in three ways. Extreme compact objects, such as black holes, neutron stars, and stellar cores, can parametrically increase the production rates of feebly interacting particles and yield observable signatures. Specifically, a process known as superradiance leads to exponential growth of the number of ultralight particles gravitationally bound to rotating black holes, and turns astrophysical black holes into particle detectors. This research broadened the scope of applicability of superradiance studies to particles with a wide range of interactions and masses, predicting multi messenger signals. When ultralight particles are produced as dark matter in the early universe, they can be detected directly in laboratory experiments. However, these feebly interacting particles lead to small signals that are inevitably difficult to tease out from backgrounds; their detection requires the theoretical development of unique signatures that can be searched for in low-noise experiments. Some dark matter particles could be detectable with thin film metamaterials combined with low noise single-photon detectors. This research develop the theoretical framework and supported experimental efforts for ambitious searches for a wider class of ultralight particles. Overall, the outcome of this theoretical particle physics program developed novel signatures of new dark matter particles, and thereby expanded the particle parameter space which can be explored with astrophysical observations and precision experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Searches for New Physics With Muon Conversion at Fermilab and Triboson Production at the LHC

We report on several efforts to search for physics beyond the standard model of particle physics at broad energy scales. The Mu2e experiment at Fermilab will search for charged lepton flavor violation via the muon to electron conversion process, which is suppressed in the Standard Model. Mu2e will be operated at a low energy, yet can probe New Physics at very high mass scales (O(1e3 - 1e4 ) TeV). At high energies, the CMS experiment at the CERN LHC continues to deliver an impressive suite of Standard Model measurements and limits on a variety of New Physics signatures. Mu2e is under construction and slated to collect its first physics data in the coming years. This thesis describes work done during the construction phase of Mu2e and focuses on two critical areas: magnetic field modeling and statistical analysis. We describe a novel method for field modeling which we validate using a simulated dataset representing the expected magnetic field in the Detector Solenoid. This method blends a standard least-squares fitting technique that utilizes physically motivated analytical model functions with a novel physics informed network that is constructed to obey Maxwell’s equations. We show the technique can model the field with an accuracy of 10−7 despite the presence of injected noise in the pseudo-measurements at the 10−5 level. We then present preliminary results of the calibration of 3D Hall probes at the sub-10−4 level. These probes will be used to directly measure the Mu2e Detector Solenoid magnetic field on a sparse grid; these measurements serve as the input to the field model fitting. Finally, we describe the first implementation of both an unbinned shape analysis and a Bayesian interpretation applied to Mu2e pseudo-data. Up to 20% tighter limits can be set by the shape analysis compared to a standard cut & count analysis. The AlCap experiment collected data at PSI in 2015 to measure several important quantities related to nuclear muon capture on an aluminum target, which is a significant background process for Mu2e. The neutron emission from muon capture can introduce background hits in the Mu2e detectors and can increase radiation damage in various elements of the apparatus. We present measurements of the neutron group fluence and mean neutron multiplicity for muon capture on aluminum nuclei. Finally, we discuss an analysis of triboson production at CMS using an Effective Field Theory framework. Standard Model triboson production, which was first observed at CMS in 2020, has a relatively small cross section and provides direct access to both anomalous triple gauge couplings and quartic gauge couplings. These couplings, interpreted in the Standard Model Effective Field Theory, are studied in the present work. We target the boosted regime where the background rate is low and yields are enhanced when dimension-6 and dimension-8 Wilson coefficients are non-zero. We do not observe an excess in the data and therefore set bounds on the Wilson coefficients. For dimension-6 coefficients the tightest observed (expected) bounds are set on cW /Λ2 where Λ is the mass scale of new physics; the bounds are [−0.13, 0.12] TeV−2 ([−0.12, 0.12] TeV−2 ) at 95% CL. The tightest bounds in dimension-8 are set on fT,0 / Λ4 ; the observed (expected) bounds at 95% CL are [−0.63, 0.69] TeV−4 ([−0.54, 0.62] TeV−4 ). Additional results are presented which include scenarios where multiple Wilson coefficients are non-zero, the application of signal model clipping to address unitarity violation in Effective Field Theories, and a novel template fit developed for easier reinterpretation of our results.

Kampa, Cole Erik [Northwestern U. (main)] (ORCID:0↗

The Local Seismoacoustic Wavefield of a Research Nuclear Reactor and Its Response to Reactor Power Level

In this article, we describe the seismoacoustic wavefield recorded outdoors but inside the facility fence of the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory (Tennessee). HFIR is a research nuclear reactor that generates neutrons for scattering, irradiation research, and isotope production. This reactor operates at a nominal power of 85 MW, with a full-power period between 24 and 26 days. This study uses data from a single seismoacoustic station that operated for 60 days and sampled a full operating reactor cycle, that is, full-power operation and end-of-cycle outage. The analysis presented here is based on identifying signals that characterize the steady, that is, full-power operation and end-of-cycle outage, and transitional, that is, start-up and shutdown, states of the reactor. We found that the overall seismoacoustic energy closely follows the main power cycle of the reactor and identified spectral regions excited by specific reactor operational conditions. In particular, we identified a tonal noise sequence with a fundamental frequency around 21.4 Hz and multiple harmonics that emerge as the reactor reaches 90% of nominal power in both seismic and acoustic channels. We also utilized temperature measurements from the monitoring system of the reactor to suggest links between the operation of reactor’s subsystems and seismoacoustic signals. We demonstrate that seismoacoustic monitoring of an industrial facility can identify and track some industrial processes and detect events related to operations that involve energy transport.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Gamma-Ray and Cosmic Ray Muon Modalities for Cargo Inspection

Screening and inspection of cargo containers are two essential methods to nondestructively examine the contents of shipment. These methods enable the detection of illicit transportation of unauthorized materials such as nuclear and radioactive materials, explosives, drugs, and so on, typically at borders or secure facilities. Although high-energy X-ray transmission is a standard system and is widely used for cargo inspection, the inherent challenges of high false-positive rates and high attenuation factors necessitate the development of complementary techniques that can increase the detection efficiency and accuracy in large and dense materials. Gamma-rays, which possess higher penetration characteristics because of their high energy, offer an alternative nonintrusive modality for cargo scanning. They represent a promising inspection method when compared to X-rays for three reasons: (1) improved ability to detect nuclear and radioactive materials, (2) higher inspection throughput rates, and (3) lower false-positive rates. Currently, there are two main gamma-ray inspection techniques, active and passive interrogation. Active interrogation can be further grouped into (1) gamma-ray transmission imaging and (2) neutron-induced gamma-ray emission detection. Gamma-ray transmission imaging utilizes differences in material densities for mapping the shipment contents and detecting anomalies. It is analogous to the X-ray transmission method; however, the high-energy photons make it more difficult to shield against, which enables more efficient performance in large and dense material inspection. Neutron-induced gamma-ray emission inspection is designed for the detection of nuclear and radioactive material because those materials emit characteristic gamma-rays when they are activated by neutron absorption. On the other hand, passive interrogation techniques rely on high-efficiency detectors to detect radiation emitted from hidden special nuclear or other radioactive materials. Similar to passive interrogation, cosmic ray muon monitoring and imaging are relatively new techniques that do not require external radioactive sources. These techniques have received attention as a potential next-generation radiographic probe to identify illicit transportation of nuclear and radioactive materials in cargo containers. Cosmic ray muons have unique features, (1) much higher energies than X-rays or gamma-rays (on the order of 10−1—104 GeV), (2) enhanced penetration capability, and (3) natural occurrence, thereby eliminating the need for induced radiation sources. These features enable cosmic ray muons to be utilized for detection of special nuclear materials in high-background-noise environments. By analyzing incoming and outgoing muon trajectories, scattering angles, and energies, it has been shown that it would be possible to locate hidden and well-shielded materials in cargo containers via three-dimensional muon tomography images or signal analysis. Gamma-rays, cosmic ray muons, and other nonintrusive cargo inspection modalities are complementary to each other, allowing them to address various cargo inspection conditions (i.e., scanning time, cost, radiation exposure level, and types of target materials). This chapter presents a detailed review of the theoretical fundamentals and technical principles behind the current gamma-ray and cosmic ray muon modalities for cargo inspection. Additionally, critical assessments and suggestions for the future directions to advance the use of gamma and muon modalities are discussed.

Bae, Junghyun↗

Multi-Probe 24A: Post shot Data and Analysis

The Multi-Probe 24A experiments took place on the Omega EP laser in November 2023. The experiments consisted of shots alternating between Omega EP’s two short-pulse laser beams to generate proton and deuteron ion beams from a range of film thicknesses, and x-ray sources from the established CPC+Ta wire targets. The backlighter was used for ion acceleration in the pitcher series, in which deuteron and proton beams characterized as a function of CD film thickness to develop a pitcher for a pitcher-catcher neutron radiographic source, while also characterizing electrons and x-rays emitted perpendicular to the target (i.e. Crosstalk for sidelighter-driven x-ray beams). The sidelighter was used for electron acceleration in the x-ray series, in which the electron acceleration and subsequent x-rays was characterized from the CPC+Ta wire targets and radiography was conducted with and without electro-magnetic electron defection. For the pitcher series, we found that at 500 J and 0.7 ps the 700-800 nm CD films yielded the greatest number and highest energy for both protons and deuterons. For the x-ray series, results demonstrated: a significant number of <100 keV x-rays are produced within the glue that fills the CPC cone, on-axis electron signal from the x-ray targets produce electrons resolvable up to ~10 MeV, and electron deflection (using MIFEDS) has a notable effect radiograph on noise reduction.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Examination of decay heat measurements and their relevance for understanding the origin of the reactor antineutrino anomaly

Measurements of the decay energy released as a function of time following the thermal neutron induced fission of 235 U and 239,241 Pu were performed in the 1970s at Oak Ridge National Laboratory with the purpose of quantifying possible loss of coolant accident scenarios. The derivative of this decay energy with respect to time, known in technical parlance as decay heat, is mainly composed of two terms, that of the electrons produced together with antineutrinos in the $β$-minus decay of the neutron-rich fission products, and that of the $γ$ rays produced in the subsequent decay of excited nuclear levels. In this work we study if this extensive set of decay energy measurements can be used to assess the reactor antineutrino anomaly, that is, the approximately 5% deficit of electron antineutrinos produced by nuclear reactors, first deduced by Mention and collaborators in 2011, and observed by the major reactor antineutrino experiments since. Furthermore, with the assistance of nuclear databases, we are able to obtain the ratio of electron spectra under equilibrium conditions for 235 U to 239 Pu, in better agreement with the lower trend recently reported by Kopeikin and collaborators, as well as those for 235 U to 241 Pu and 241 Pu to 239 Pu, which do not agree well with those measured at the Institut Laue-Langevin in the 1980s. We conclude that a new experimental campaign is needed to measure the electron spectra utilizing a high resolution and signal-to-noise-ratio electron spectrometer and a highly precise fission normalization procedure.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Updated universal relations for tidal deformabilities of neutron stars from phenomenological equations of state

Equation of state (EOS) insensitive relations, so-called universal relations, between the neutron star (NS) compactness, its multipolar tidal deformability coefficients, and between the tidal parameters for binary systems are essential to break degeneracies in gravitational wave data analysis. Here, we validate and recalibrate these universal relations using a large set of almost 2 million phenomenological EOSs that are consistent with current observations. In doing so, we extend universal relations to a larger region of the EOS parameter space, most notably to softer EOSs and larger compactnesses. We show that waveform models that neglect higher-than-leading-order tidal deformations of the NSs accumulate as much as 3.5 radians of dephasing from 20Hz to merger. Further, we also perform a full Bayesian parameter estimation of the GW170817 data, and we compare the NS radius constraints produced using universal relations from the literature and the updated fits we propose here. We find that the new fits yield a NS radius that is smaller by about 500 meters. This difference is less than the statistical uncertainty on the radius at the signal-to-noise-ratio of GW170817, but it is significantly larger than the precision anticipated for next-generation detectors.

79 ASTRONOMY AND ASTROPHYSICS↗

Characterization and Quantification of Radiation-Induced Clusters/Precipitates in RPV Steels Using STEM-EDS and Machine Learning

Over the operational lifespan of a nuclear reactor, reactor pressure vessel (RPV) steels are subjected to significant neutron irradiation, resulting in complex microstructural changes and the consequent degradation of mechanical properties. Various physically motivated correlation models have been developed to predict neutron irradiation-induced embrittlement of RPVs under different irradiation conditions. However, the efficient and accurate characterizations and quantification of radiation-induced clusters in RPVs are still challenging, which will affect the precision of the predictive models for embrittlement of RPV components. In the DOE Visiting Faculty Program (VFP) research work at Oak Ridge National Lab (ORNL), I integrate machine learning to aid Scanning Transmission Electron Microscopy – Energy Dispersive X-ray Spectroscopy (STEM-EDS) analyses, which improve the characterization and quantification of radiation-induced clusters in RPV steels, thereby enabling more accurate predictions of material behavior under irradiation. The surveillance base- and welded- RPV steels were annealed at various temperatures of 340 °C, 450 °C and 500 °C for up to 168 hours, respectively. Afterwards, I have characterized radiation-induced clusters using advanced STEM-EDS techniques and subsequently applying machine learning algorithms to analyze and refine STEM-EDS datasets, enhancing the quantification of clusters compositions and distributions. In the end, an efficient workflow for integrating STEM-EDS data analysis with machine learning to address challenges including noise reduction has been developed. The completion of this VFP work will support bridge critical gaps in the accurate quantification of radiation-induced clusters in RPV steels using STEM-EDS and support the development of more precise models for predicting RPV embrittlement in the Light Water Reactor Sustainability program supported by Department of Energy and enhancing the collaboration between ORNL and Alred University. The outcome of the VFP project will leverage a few research papers submission to peer-reviewed journals in the relevant scientific field and a few oral presentations at national and international conferences.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗