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NASA NTRS1997

Consistency Between Divergent Circulations from Reanalysis Data Sets and Satellite-Derived Precipitation, Radiation, and Surface Fluxes

Large-scale divergent circulations are part of the atmospheric dynamic response to diabatic heating from condensation, radiative processes, and surface heat fluxes. Vertical motion and the associated divergent wind is thus intimately tied to the hydrologic cycle and the global heat balance. Despite its importance, the divergent circulation is too small in comparison to the rotational flow to measure directly with any accuracy. Vertical motions are recovered diagnostically from reanalyses and, as such, are subject to shortcomings in model physics, numerics, and data availability. We use several GEWEX pre-EOS data sets derived from satellite data to assess interannual divergent flow anomalies in the NCEP, GSFC, and GSFC DAO analyse. Among the data sets are monthly, 2.5 degree gridded precipitation (MSU and SSM/I-based), TOA radiative fluxes from ERBS, surface radiative fluxes from the SRB project, and surface latent and sensible flux estimates from SSM/I. Most of these data sets can be considered as independent of the reanalysis fields. We focus largely on the period 1987-1989 encompassing a strong El Nino / la Nina couplet. Consequently we emphasize interannual changes rather than climatological aspects of the reanalyses. In the processes of this study we use simple integral constraints enforced through the satellite-derived data sets to derive corrections to the divergent circulation produced from the reanalyses. We examine the implications of these corrections in describing how perturbations to the tropical heat balance evolve during a warm / cool couplet. In particular the perturbations to the planetary scale water vapor transport, and the resulting changes in TOA and surface radiative fluxes are considered.

Robertson, Franklin R.↗

NASA NTRS1983

Dielectronic recombination rates, ionization equilibrium, and radiative emission rates for Mn ions in low-density high-temperature plasmas

The analysis of optically-thin far-ultraviolet and X-ray emission lines of multiply-charged ions is one of the basic methods for determining the temperatures and densities of laboratory and astrophysical plasmas. In addition, the energy balance in these plasmas can be significantly influenced by the emission of radiation from relatively low concentrations of multiple-charged atomic ions. Because the populations of the excited levels are expected to depart substantially from their local thermodynamic equilibrium values a detailed treatment of the elementary collisional and radiative processes must be employed in order to predict the emission line intensities. In this investigation the authors present the results of calculations based on a corona equilibrium model in which a detailed evaluation is made of the dielectronic recombination rate coefficients. The ionization and autoionization following inner-shell electron excitation from each ground state are balanced by direct radiative and dielectronic recombination. The spectral line intensities emitted by the low-lying excited states, which are assumed to undergo spontaneous radiative decay in times that are short compared with the collision time, are evaluated in terms of the corona ionization equilibrium distributions of the ground states and their electron-impact excitation states.

Jacobs, V. L.↗

NASA NTRS1999

Consistency Between Tropical Divergent Circulations from Reanalysis Data Sets and Satellite-Derived Precipitation, Radiation, and Surface Fluxes

Large-scale divergent circulations are part of the atmospheric dynamic response to diabatic heating from condensation, radiative processes, and surface heat fluxes. Vertical motion and the associated divergent wind is thus intimately tied to the hydrologic cycle and the global heat balance. Vertical motions are recovered diagnostically from reanalyses and, as such, are subject to shortcommings in model physics, numerics, and data availability. We use several Global Energy and Water Cycle Experiment (GEWEX) Earth Observation System (EOS) data sets derived from satellite data to assess interannual divergent flow anomalies in the National Centers for Environmental Prediction (NCEP), Goddard Space Flight Center (GSFC), and GSFC Data Assimilation Office (DAO) analyses. Among the data sets are monthly, 2.5 degree gridded precipitation (Microwave Sounding Unit (MSU) and Special Sensor Microwave Imager (SSM/I-based)), Top or the atmosphere (TOA) radiative fluxes from ERBS, surface radiative fluxes from the SRB project, and surface latent and sensible flux estimates from SSM/I. These data sets can be considered as independent of the reanalysis fields. We focus largely on the period 1987-1989 encompassing a strong El Nino / la Nina couplet. Consequently we emphasize interannual changes as well as climatological aspects of the reanalyses. In the processes of this study we use simple integral constraints enforced through the satellite-derived data sets to derive corrections to the divergent circulation produced from the reanalyses. We examine the implications of these corrections in describing how perturbations to the tropical heat balance evolve during a warm / cool couplet. In particular the perturbations to the planetary scale water vapor transport, and the resulting changes in TOA and surface radiative fluxes are considered.

Robertson, Franklin R.↗

NASA NTRS2009

The Unique Capabilities of the Global Hawk Aircraft for the Study of Climate Changes

Due to unprecedented extent and flexibility of the coverage that is now attainable both in space and time, stratospheric unmanned aircraft, such as the Global Hawk (GH), offers new opportunities for the study of climate changes. The capability of performing long flights at altitudes close to the boundary conditions of radiative processes, and of following the diurnal variation of chemical species and clouds, make the GH competitive with LEO and geosynchronous satellites, and even capable of new observations that are not possible from satellites. This paper discusses how the GH can be used to make relevant advancements in most of the issues that are related to climate change studies, such as: Earth Radiation Budget, Water Cycle, Ecosystems and Upper Troposphere-Lower Stratosphere, as well as to the monitoring and control of Greenhouse Gases and Air Quality . Collaboration between NASA and Italian scientific institutions, within the framework of the US.-Italy Cooperation on Climate Change, is providing the opportunity to rapidly deploy new instruments on the GH and to possibly operate the aircraft from an Italian site in the Mediterranean area. From this area, which is considered highly vulnerable to climate change, meridional transects would allow the crossing of Polar and Sub Tropical Jets, as well as a complete crossing of the Inter Tropical Convergence Zone, while latitudinal ones would follow the influx from Asia and North America. Regions otherwise difficult to access, such as Central Africa and the Tibetan Plateau, could be reached and better investigated. An overview of these new opportunities will be given and discussed.

Cairo, F.↗

NASA NTRS2000

GCSS Idealized Cirrus Model Comparison Project

The GCSS Working Group on Cirrus Cloud Systems (WG2) is conducting a systematic comparison and evaluation of cirrus cloud models. This fundamental activity seeks to support the improvement of models used for climate simulation and numerical weather prediction through assessment and improvement of the "process" models underlying parametric treatments of cirrus cloud processes in large-scale models. The WG2 Idealized Cirrus Model Comparison Project is an initial comparison of cirrus cloud simulations by a variety of cloud models for a series of idealized situations with relatively simple initial conditions and forcing. The models (16) represent the state-of-the-art and include 3-dimensional large eddy simulation (LES) models, two-dimensional cloud resolving models (CRMs), and single column model (SCM) versions of GCMs. The model microphysical components are similarly varied, ranging from single-moment bulk (relative humidity) schemes to fully size-resolved (bin) treatments where ice crystal growth is explicitly calculated. Radiative processes are included in the physics package of each model. The baseline simulations include "warm" and "cold" cirrus cases where cloud top initially occurs at about -47C and -66C, respectively. All simulations are for nighttime conditions (no solar radiation) where the cloud is generated in an ice supersaturated layer, about 1 km in depth, with an ice pseudoadiabatic thermal stratification (neutral). Continuing cloud formation is forced via an imposed diabatic cooling representing a 3 cm/s uplift over a 4-hour time span followed by a 2-hour dissipation stage with no cooling. Variations of these baseline cases include no-radiation and stable-thermal-stratification cases. Preliminary results indicated the great importance of ice crystal fallout in determining even the gross cloud characteristics, such as average vertically-integrated ice water path (IWP). Significant inter-model differences were found. Ice water fall speed is directly related to the shape of the particle size distribution and the habits of the ice crystal population, whether assumed or explicitly calculated. In order to isolate the fall speed effect from that of the associated ice crystal population, simulations were also performed where ice water fall speed was set to the same constant value everywhere in each model. Values of 20 and 60 cm/s were assumed. Current results of the project will be described and implications will be drawn. In particular, this exercise is found to strongly focus the definition of issues resulting in observed inter-model differences and to suggest possible strategies for observational validation of the models. The next step in this project is to perform similar comparisons for well observed case studies with sufficient high quality data to adequately define model initiation and forcing specifications and to support quantitative validation of the results.

Starr, David OC.↗

NASA NTRS1987

On the global mean structure of the thermosphere

A self-consistent model of the global mean structure of the thermosphere is used to examine the ionospheric and thermospheric processes that control the structure of the thermosphere for solar minimum and maximum conditions during geomagnetic quiet periods. The model includes the physical and chemical processes believed to be dominant in the thermosphere and ionosphere. The total solar energy input available in the extreme ultraviolet and in the Schumann-Runge continuum portion of the solar spectrum is 14.1 x 10 to the 11th W and 21.5 x 10 to the 11th W for solar minumum and maximum, respectively. The calculated exospheric temperature is too small if maintained only by radiative processes, and an auroral heat source is necessary to bring the calculated global mean structure into agreement with the MSIS-83 empirical model for both solar minimum and maximum conditions. These results support the consensus that there is high-latitude heat source present at all times.

Roble, R. G.↗

NASA NTRS2003

A Search for Signs of Life and Habitability on Europa

Europa is a key target in the search for life beyond the Earth because of consistent evidence that below the icy surface there is liquid water. Future missions to Europa could confirm the presence and nature of the ocean and determine the thickness of the ice layer. Confirming the presence of an ocean and determining the habitability of Europa are key astrobiology science objectives. Nevertheless, the highest priority objective for astrobiology will be a search for life. How could a search for life be accomplished on a near-term mission given the thick ice cover? One answer may lie in the surface materials. If Europa has an ocean, and if that ocean contains life, and if water from the ocean is carried up to the surface, then signs of life may be contained in organic material on the surface. Organics that derive from biological processes (dead organisms) are distinct from organics derived from non-biological processes in several aspects. First, biology is selective and specific in its use of molecules. For example, Earth life uses 20 left-handed amino acids. Second, biology can leave characteristic isotopic patterns. Third, biology often produces large complex molecules in high concentrations, for example lipids. Organic material that has been on the surface of Europa for long periods of time would be reprocessed by the strong radiation field probably erasing any signature of biological origin. Evidence of life in the ocean may be found on the surface of Europa if regions of the surface contained relatively recent material carried up from the ocean through cracks in the icy lithosphere. But organic material that has been on the surface of Europa for long periods of time would be reprocessed by the strong radiation field probably erasing any signature of biological origin. Thus, the detailed analysis required may not be possible via remote sensing but direct sampling of the material below the radiation processed upper meter is probably required.

Fonda, Mark↗

NASA NTRS2004

Effects of Cloud-Microphysics on Tropical Atmospheric Hydrologic Processes in the GEOS GCM

The sensitivity of tropical atmospheric hydrologic processes to cloud-microphysics is investigated using the NASA GEOS GCM. Results show that a faster autoconversion - rate produces more warm rain and less clouds at all levels. Fewer clouds enhances longwave cooling and reduces shortwave heating in the upper troposphere, while more warm rain produces increased condensation heating in the lower troposphere. This vertical heating differential destablizes the tropical atmosphere, producing a positive feedback resulting in more rain over the tropics. The feedback is maintained via a two-cell secondary circulation. The lower cell is capped by horizontal divergence and maximum cloud detrainment near the melting/freezing, with rising motion in the warm rain region connected to descending motion in the cold rain region. The upper cell is found above the freezing/melting level, with longwave-induced subsidence in the warm rain and dry regions, coupled to forced ascent in the deep convection region. The tropical large scale circulation is found to be very sensitive to the radiative-dynamic effects induced by changes in autoconversion rate. Reduced cloud-radiation processes feedback due to a faster autoconversion rate results in intermittent but more energetic eastward propagating Madden and Julian Oscillations (MJO). Conversely,-a slower autconversion rate, with increased cloud radiation produces MJO's with more realistic westward propagating transients, resembling a supercloud cluster structure. Results suggests that warm rain and associated low and mid level clouds, i.e., cumulus congestus, may play a critical role in regulating the time-intervals of deep convections and hence the fundamental time scales of the MJO.

Lau, K. M.↗

NASA NTRSDate not supplied

Lapse-Rate Feeback: The Key to Reconciling TOA and Surface Attributions of Surface Warming

The impact of climate feedbacks on surface warming is conventionally evaluated using a decomposition of the top-of-atmosphere (TOA) energy budget. Alternatively, the climate feedback analysis can also be carried out using the surface energy budget. However, the two perspectives do not provide the same interpretation of process contributions to surface warming, particularly when executing a spatial analysis. The TOA energy budget is equal to the sum of the surface and atmospheric energy budgets. Using the CMIP5 RCP 8.5 model projections, we show that the major discrepancies between the surface and TOA climate feedback attributions of surface warming are due to non-negligible changes in the atmospheric energy budget that differ from their counterparts at the surface. Individual radiative and non-radiative processes cause vertically non-uniform energy flux perturbations, in response to an external forcing, that naturally lead to a vertically non-uniform temperature change. The TOA lapse-rate feedback is the manifestation of these multiple processes that produce a vertically non-uniform warming response such that it accounts for the asymmetry between the changes in the atmospheric and surface energy budgets. Using the climate feedback-response analysis method, we can decompose the lapse-rate feedback into contributions by individual processes. The negative lapse-rate feedback in the tropics is due to greater moist convection and condensational heating along with ocean heat storage. On the other hand, the positive lapse-rate feedback in polar regions is primarily due to the surface albedo and water vapor feedbacks. Combining the process contributions that are hidden within the lapse-rate feedback with their respective direct impacts on the TOA energy budget allows for a very consistent picture of process contributions to surface warming and its inter-model spread as that given by the surface energy budget approach. With the modified approach, both perspectives indicate water vapor feedback is the largest contributor in the tropics, while surface albedo feedback is the greatest contributor in polar regions. Dynamics and ocean heat storage are the main suppressors of surface warming, except over Antarctica. Both perspectives show there is large inter-model uncertainty in the contributions of water vapor, clouds, albedo, and dynamics plus ocean heat storage.

Sergio A Sejas↗

NASA NTRS2016

A Ten-Year Global Record of Absorbing Aerosols Above Clouds from OMI's Near-UV Observations

Aerosol-cloud interaction continues to be one of the leading uncertain components of climate models, primarily due to the lack of an adequate knowledge of the complex microphysical and radiative processes associated with the aerosol-cloud system. The situations when aerosols and clouds are found in the same atmospheric column, for instance, when light-absorbing aerosols such as biomass burning generated carbonaceous particles or wind-blown dust overlay low-level cloud decks, are commonly found over several regional of the world. Contrary to the cloud-free scenario over dark surface, for which aerosols are known to produce a net cooling effect (negative radiative forcing) on climate, the overlapping situation of absorbing aerosols over cloud can potentially exert a significant level of atmospheric absorption and produces a positive radiative forcing at top-of-atmosphere. The magnitude of direct radiative effects of aerosols above cloud depends directly on the aerosol loading, microphysical-optical properties of the aerosol layer and the underlying cloud deck, and geometric cloud fraction. We help in addressing this problem by introducing a novel product of optical depth of absorbing aerosols above clouds retrieved from near-UV observations made by the Ozone Monitoring Instrument (OMI) on board NASA's Aura platform. The presence of absorbing aerosols above cloud reduces the upwelling radiation reflected by cloud and produces a strong 'color ratio' effect in the near-UV region, which can be unambiguously detected in the OMI measurements. Physically based on this effect, the OMACA algorithm retrieves the optical depths of aerosols and clouds simultaneously under a prescribed state of atmosphere. The algorithm architecture and results from a ten-year global record including global climatology of frequency of occurrence and above-cloud aerosol optical depth, and a discussion on related future field campaigns are presented.

Ozone Monitoring Instrument↗

NASA NTRS2002

Evidence of an Intrinsic Intraseasonal Oscillation over Tropical South America During Austral Summer

The intraseasonal variation (ISV) in the 30-60 day band, also known as Madden-Julian oscillation (MJO), has been studied for decades. Madden and Julian showed that the oscillation originated from the western Indian Ocean, propagated eastward, got enhanced over the maritime continent and weakened after passing over the dateline. Composite studies showed evidences of a signal in upper and lower level zonal wind propagating around the globe during an oscillation. Theoretical studies pointed out that the interaction with the warm ocean surface and the coupling with the convective and radiative processes in the atmosphere could manifest the oscillation, which propagates eastward via mutual feedbacks between the wave motions and the cumulus heating. Over tropical South America, no independent 30-60 day oscillation has been reported so far, despite that Amazon is the most distinct tropical convection center over the western hemisphere and the fluxes from its surface of tropical rainforests are close to that from the warm tropical ocean. Liebmann et al. showed a distinct spectral peak of 40-50 day oscillation in outgoing longwave radiation (OLR) over tropical South America and considered that was manifested by the MJO propagation. Nogues-Paegle et al. (2000) focused on a dipole pattern of the OLR anomaly with centers of action over the South Atlantic Convergence Zone (SACZ) and the subtropical plain. They used the regional 10-90 day filtered data and demonstrated this pattern could be represented by the fifth mode of the rotated empirical orthogonal function. Its principal component was further analyzed using the singular spectrum analysis. Their result showed two oscillatory modes with periods of 36-40 days and 22-28 days, of which the former was related to the MJO influence and the latter linked to the remote forcing over southwest of Australia, which produced a wave train propagating southeastward, rounding the southern tip of South America and returning back toward the northeast. The 22-28 day mode has distinct impact on SACZ, responsible for the regional seesaw pattern of alternating dry and wet conditions. In this study we will focus on the 30-60-day spectral band and investigate whether the independent oscillation source over tropical South America is existed. First, we will show the seasonal dependence of the tropical South American ISV in Section 3. Then, the leading principal modes of 30-60 day bandpass filtered 850-hPa velocity potential (VP850) will be computed to distinguish the stationary ISV over tropical South America (SISA) from the propagating MJO in the austral summertime in Section 4. The importance of SISA in representing the regional ISV over South America will be discussed. In Section 5, we will demonstrate the mass oscillation regime of SISA, which is well separated from that of MJO by the Andes, and the convective coupling with rainfall. The dynamical response of SISA and the impact on the South American summer monsoon (SASM) will be presented. Finally, we will give the concluding remarks.

Zhou, Jiayu↗

NASA NTRS2010

A SNAPshot of the FUV (1320 - 1460 A) Spectrum of Lambda Vel (K4Ib-II)

The FUV spectrum (l330-1460A) of the K4Ib-II supergiant Lambda Vel was observed with the Cosmic Origins Spectrograph (COS) on HST, as part of the Ayres and Redfield Cycle 17 SNAP program "SNAPing Coronal Iron". This spectrum covers a region not previously seen in Lambda Vel at high resolution and reveals a rich emission-line spectrum superposed on a bright continuum, with contributions from a variety of atomic and molecular sources. Evidence of the stellar wind is seen in the P Cygni profiles of selected lines and the results of fluorescence processes are visible throughout the region. The spectrum has remarkable similarities to that of Alpha Boo (K1.5 III), but significant differences as well, including substantial FUV continuum emission, reminiscent of the M2 lab supergiant Alpha Ori, but minus the CO fundamental absorption bands seen in the latter star. However, fluoresced CO emission is present and strong, as in the K-giant stars Alpha Boo and Alpha Tau (K5 III). We present the details of this spectrum, in comparison to stars of similar temperature or luminosity and discuss the implications for the structure of and the radiative processes active in, the outer atmospheres of these stars.

Carpenter, Kenneth G.↗

NASA NTRS1978

Measurements of kinetic processes in a self-sustained discharge XeF laser

Measurements are presented for processes occurring in XeF self-sustained discharges including fluorescence, gain, and absorption at different wavelengths as a function of F2, Xe, and He partial pressures. Time-correlated oscillograms are given for the laser discharge current, metastable XeF small-signal gain at 351.1 nm, transient absorptions at 333.6 and 363.8 nm, metastable-XeF B-state sidelight emission at about 350 nm, metastable-F emission at 634.8 nm, and metastable-F emission at 731.1 nm. It is found that He atoms are necessary for the production of metastable-XeF in its lower vibrational levels and that radiative processes and He quenching are the primary mechanisms for metastable-XeF decay. For small-signal gains of as low as about 8%/cm, the transient absorption at the laser wavelength may be as large as about 1-2%/cm.

Gower, M. C.↗

NASA NTRS2013

Irradiated Benzene Ice Provides Clues to Meteoritic Organic Chemistry

Aromatic hydrocarbons account for a significant portion of the organic matter in carbonaceous chondrite meteorites, as a component of both the low molecular weight, solvent-extractable compounds and the insoluble organic macromolecular material. Previous work has suggested that the aromatic compounds in carbonaceous chondrites may have originated in the radiation-processed icy mantles of interstellar dust grains. Here we report new studies of the organic residue made from benzene irradiated at 19 K by 0.8 MeV protons. Polyphenyls with up to four rings were unambiguously identified in the residue by gas chromatography-mass spectrometry. Atmospheric pressure photoionization Fourier transform mass spectrometry was used to determine molecular composition, and accurate mass measurements suggested the presence of polyphenyls, partially hydrogenated polyphenyls, and other complex aromatic compounds. The profile of low molecular weight compounds in the residue compared well with extracts from the Murchison and Orgueil meteorites. These results are consistent with the possibility that solid phase radiation chemistry of benzene produced some of the complex aromatics found in meteorites.

benzene↗

NASA NTRS2011

Satellite Observations and Chemistry Climate Models - A Meandering Path Towards Better Predictions

Knowledge of the chemical and dynamical processes that control the stratospheric ozone layer has grown rapidly since the 1970s, when ideas that depletion of the ozone layer due to human activity were put forth. The concept of ozone depletion due to anthropogenic chlorine increase is simple; quantification of the effect is much more difficult. The future of stratospheric ozone is complicated because ozone is expected to increase for two reasons: the slow decrease in anthropogenic chlorine due to the Montreal Protocol and its amendments and stratospheric cooling caused by increases in carbon dioxide and other greenhouse gases. Prediction of future ozone levels requires three-dimensional models that represent physical, photochemical and radiative processes, i.e., chemistry climate models (CCMs). While laboratory kinetic and photochemical data are necessary inputs for a CCM, atmospheric measurements are needed both to reveal physical and chemical processes and for comparison with simulations to test the conceptual model that CCMs represent. Global measurements are available from various satellites including but not limited to the LIMS and TOMS instruments on Nimbus 7 (1979 - 1993), and various instruments on the Upper Atmosphere Research Satellite (1991 - 2005), Envisat (2002 - ongoing), Sci-Sat (2003 - ongoing) and Aura (2004 - ongoing). Every successful satellite instrument requires a physical concept for the measurement, knowledge of physical chemical properties of the molecules to be measured, and stellar engineering to design an instrument that will survive launch and operate for years with no opportunity for repair but providing enough information that trend information can be separated from any instrument change. The on-going challenge is to use observations to decrease uncertainty in prediction. This talk will focus on two applications. The first considers transport diagnostics and implications for prediction of the eventual demise of the Antarctic ozone hole. The second focuses on the upper stratosphere, where ozone is predicted to increase both due to chlorine decrease and due to temperature decrease expected as a result of increased concentrations Of CO2 and other greenhouse gases. Both applications show how diagnostics developed from global observations are being used to explain why the ozone response varies among CCM predictions for stratospheric ozone in the 21st century.

Douglass, Anne R.↗

NASA NTRS1999

Interaction Between Tropical Convection and its Embedding Environment: An Energetics Analysis of a 2-D Cloud Resolving Simulation

The phase relation between the perturbation kinetic energy (K') associated with the tropical convection and the horizontal-mean moist available potential energy (bar-P) associated with environmental conditions is investigated by an energetics analysis of a numerical experiment. This experiment is performed using a 2-D cloud resolving model forced by the TOGA-COARE derived vertical velocity. The imposed upward motion leads to a decrease of bar-P directly through the associated vertical advective cooling, and to an increase of K' directly through cloud related processes, feeding the convection. The maximum K' and its maximum growth rate lags and leads, respectively, the maximum imposed large-scale upward motion by about 1-2 hours, indicating that convection is phase locked with large-scale forcing. The dominant life cycle of the simulated convection is about 9 hours, whereas the time scales of the imposed large-scale forcing are longer than the diurnal cycle. In the convective events, maximum growth of K' leads maximum decay of the perturbation moist available potential energy (P') by about 3 hours through vertical heat transport by perturbation circulation, and perturbation cloud heating. Maximum decay of P' leads maximum decay of bar-P by about one hour through the perturbation radiative, processes, the horizontal-mean cloud heating, and the large-scale vertical advective cooling. Therefore, maximum gain of K' occurs about 4-5 hours before maximum decay of bar-P.

Li, Xiaofan↗

NASA NTRS1997

Metamorphism of Cosmic Dust: Processing from Circumstellar Outflows to the Cometary Regolith

Nucleation is a non-equilibrium process: the products of this process are seldom the most thermodynamically stable condensates but are instead those which form fastest. It should therefore not be surprising that grains formed in a circumstellar outflow will undergo some degree of metamorphism if they are annealed or are exposed to a chemically active reagent. Metamorphism of refractory particles continues in the interstellar medium (ISM) where the driving forces are sputtering by cosmic ray particles, annealing by high energy photons and grain destruction in supernova generated shocks. Studies of the depletion of the elements from the gas phase of the interstellar medium tell us that if grain destruction occurs with high efficiency in the ISM, then there must be some mechanism by which grains can be formed in the ISM. Various workers have shown that refractory mantles could form on refractory cores by radiation processing of organic ices. A similar process may operate to produce refractory inorganic mantles on grain cores which survived the supernova shocks. Most grains in a cloud which collapses to form a star will be destroyed; many of the surviving grains will be severely processed. Grains in the outermost regions of the nebula may survive relatively unchanged by thermal processing or hydration. It is these grains which we hope to find in comets. However, only those grains encased in ice at low temperature can be considered pristine since a considerable degree of hydrous alteration might occur in a cometary regolith if the comet enters the inner solar system. Some discussion of the physical, chemical and isotopic properties of a refractory grain at each stage of its life cycle will be attempted based on the limited laboratory data available to date. Suggestions will be made concerning the types of experimental data which are needed in order to better understand the processing history of cosmic dust.

Nuth, Joseph A., III↗

NASA NTRS2004

Cloud-Vegetation Radiative Interaction: What Can We Learn from it about Cloud Optical Properties?

Because of their radiative interactions, the vegetation canopy and the atmosphere are coupled together; each serves as a boundary condition to the radative transfer equations in the adjacent medium. To better understand radiative processes in these media we need an accurate description of their interactions. This presentation outlines a technique needed to describe interactions between vegetation and clouds and exploits it to retrieve cloud optical depth from ground-based radiance measurements. measurements of zenith radiance in the RED and NIR spectral regions. In addition to an algebraic combinations of spectral radiances such as Normalized Difference Cloud Index (NDCI) that can result in poor retrievals due to its insensitivity to cloud fraction, both RED and NIR radiances as points on the "RED vs. NIR" plane are proposed to be used for retrieval. The proposed method is applied to a multi-channel sunphotometer (as a part of AERONET) measurements at the ARM site in Oklahoma. In addition to cloud optical depth, the new method also infers a "radiatively effective" cloud fraction.

Marshak, Alexander↗