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At least 163 records · Page 9
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NASA NTRS1995

The annual cycle of stratospheric water vapor in a general circulation model

The application of general circulation models (GCM's) to stratospheric chemistry and transport both permits and requires a thorough investigation of stratospheric water vapor. The National Center for Atmospheric Research has redesigned its GCM, the Community Climate Model (CCM2), to enable studies of the chemistry and transport of tracers including water vapor; the importance of water vapor to the climate and chemistry of the stratosphere requires that it be better understood in the atmosphere and well represented in the model. In this study, methane is carried as a tracer and converted to water; this simple chemistry provides an adequate representation of the upper stratospheric water vapor source. The cold temperature bias in the winter polar stratosphere, which the CCM2 shares with other GCM's, produces excessive dehydration in the southern hemisphere, but this dry bias can be ameliorated by setting a minimum vapor pressure. The CCM2's water vapor distribution and seasonality compare favorably with observations in many respects, though seasonal variations including the upper stratospheric semiannual oscillation are generally too small. Southern polar dehydration affects midlatitude water vapor mixing ratios by a few tenths of a part per million, mostly after the demise of the vortex. The annual cycle of water vapor in the tropical and northern midlatitude lower stratosphere is dominated by drying at the tropical tropopause. Water vapor has a longer adjustment time than methane and had not reached equilibrium at the end of the 9 years simulated here.

Mote, Philip W.↗
NASA NTRS2000

Satellite Measured Solar Protons from 1963-1993 and Their Influence on Ozone in a Changing Stratosphere

The fluxes of solar protons have been measured by a series of Interplanetary Monitoring Platform (IMP) satellites since 1963. Eight IMP satellites have been launched since 1963 providing excellent coverage of solar protons with energies from a few MeV to several hundred MeV. IMP 8, launched in October 1973, continues to provide proton measurements, twenty-six and a half (26 1/2) years after launch. These high energy solar protons rain down on the earth's polar atmosphere sporadically, primarily during solar proton events (SPEs) which typically last a few days. Solar protons with energies of 30 MeV or greater are capable of reaching the stratosphere and causing increases in odd nitrogen (NO(y)) constituents at polar latitudes ($>$ 60 degrees geomagnetic) which last for several months to years past the events. These enhanced NO(y) species can lead to significant upper stratospheric ozone depletions $ greater than $10\% during the gigantic SPEs that occurred in August 1972 and October 1989. We studied the effects of SPEs on the stratosphere from 1963 to the mid 1990s. During this time period, the stratospheric chlorine levels changed from relatively small in 1963 ($\sim$ 1 ppbv) to fairly substantial amounts in the mid-1990s ($\sim$ 3.3 ppbv). Our recently improved two-dimensional chemistry and transport atmospheric model was used to compute the effects of SPEs in this changing stratosphere. The long-lived SPE-produced NO(y) constituents were transported to lower stratospheric levels during winter after the events and caused impacts in the middle and lower stratosphere. Generally, the SPEs resulted in a decrease in ozone. However, during periods of high halogen loading these impacts resulted in interference with the chlorine and bromine loss cycles for ozone destruction. This interference actually led to a predicted total ozone increase that was especially notable in the time period 1992-4, a few years after the October 1989 SPE.

Jackman, Charles H.↗
NASA NTRS2000

What Controls the Temperature of the Arctic Stratosphere during the Spring?

Understanding the mechanisms that control the temperature of the polar lower stratosphere during spring is key to understanding ozone loss in the Arctic polar vortex. Spring ozone loss rates are directly tied to polar stratospheric temperatures by the formation of polar stratospheric clouds, and the conversion of chlorine species to reactive forms on these cloud particle surfaces. In this paper, we study those factors that control temperatures in the polar lower stratosphere. We use the National Centers for Environmental Prediction (NCEP)/NCAR reanalysis data covering the last two decades to investigate how planetary wave driving of the stratosphere is connected to polar temperatures. In particular, we show that planetary waves forced in the troposphere in mid- to late winter (January-February) are principally responsible for the mean polar temperature during the March period. These planetary waves are forced by both thermal and orographic processes in the troposphere, and propagate into the stratosphere in the mid and high latitudes. Strong mid-winter planetary wave forcing leads to a warmer Arctic lower stratosphere in early spring, while weak mid-winter forcing leads to cooler Arctic temperatures.

Newman, Paul A.↗
NASA NTRS2001

Climate and Ozone Response to Increased Stratospheric Water Vapor

Stratospheric water vapor abundance affects ozone, surface climate, and stratospheric temperatures. From 30-50 km altitude, temperatures show global decreases of 3-6 K over recent decades. These may be a proxy for water vapor increases, as the Goddard Institute for Space Studies (GISS) climate model reproduces these trends only when stratospheric water vapor is allowed to increase. Observations suggest that stratospheric water vapor is indeed increasing, however, measurements are extremely limited in either spatial coverage or duration. The model results suggest that the observed changes may be part of a global, long-term trend. Furthermore, the required water vapor change is too large to be accounted for by increased production within the stratosphere, suggesting that ongoing climate change may be altering tropospheric input. The calculated stratospheric water vapor increase contributes an additional approximately equals 24% (approximately equals 0.2 W/m(exp 2)) to the global warming from well-mixed greenhouse gases over the past two decades. Observed ozone depletion is also better reproduced when destruction due to increased water vapor is included. If the trend continues, it could increase future global warming and impede stratospheric ozone recovery.

Shindell, Drew T.↗
NASA NTRS2000

Occurrence of Ice Supersaturations, Ice Clouds, and Ternary Aerosols in the Arctic Lowermost Stratosphere

Relative humidity, aerosol concentration, and ice crystals all have important impacts on chemistry and radiative transfer in the lowermost stratosphere. In this study, we have combined SOLVE measurements with meteorological analyses to investigate the statistics of humidity, aerosols, and clouds in the arctic lower stratosphere. First, we will present a statistical analysis of relative humidity with respect to ice in the lowermost stratosphere, used on the DC-8 in situ measurements. We will show examples of ice supersaturation well within the stratosphere. Generally, these cases were associated with extremely low temperatures near the tropopause. Next, we will discuss the climatological occurrence frequency of tropopause temperatures low enough for ice saturation even with typically low stratospheric water vapor mixing ratios. Really, we will examine case studies of ice clouds observed in the lowermost stratosphere during SOLVE. We will discuss the possible origin of these clouds (i.e., precipitation from higher type II PSCs, injection of tropospheric air into the lower stratosphere, etc.).

Jensen, Eric↗
NASA NTRS2001

The Variability of the Horizontal Circulation in the Troposphere and Stratosphere: A Comparison

The variability of the horizontal circulation in the stratosphere and troposphere of the Northern Hemisphere (NH) is compared by using various approaches. Spatial degrees of freedom (dof) on different time scales were derived. Modes of variability were computed in geopotential height fields at the tropospheric and stratospheric pressure levels by applying multivariate statistical approaches. Features of the spatial and temporal variability of the winterly zonal wind were studied with the help of recurrence and persistence analyses. The geopotential height and zonally-averaged zonal wind at the 50-, 500- and 1000-hPa level are used to investigate the behavior of the horizontal circulation in the lower stratosphere, mid-troposphere and at the near surface level, respectively. It is illustrated that the features of the variability of the horizontal circulation are very similar in the mid-troposphere and at the near surface level. Due to the filtering of tropospheric disturbances by the stratospheric and upper tropospheric zonal mean flow, the variability of the stratospheric circulation exhibits less spatial complexity than the circulation at tropospheric pressure levels. There exist enormous differences in the number of degrees of freedom (or free variability modes) between both atmospheric layers. Results of the analyses clearly show that the concept of a zonally symmetric AO with a simple structure in the troposphere similar to the one in the stratosphere is not valid. It is concluded that the spatially filtered climate change signal can be detected earlier in the stratosphere than in the mid-troposphere or at the near surface level.

Perlwitz, Judith↗
NASA NTRS1998

Stratospheric Aerosol Measurements

Stratospheric aerosols affect the atmospheric energy balance by scattering and absorbing solar and terrestrial radiation. They also can alter stratospheric chemical cycles by catalyzing heterogeneous reactions which markedly perturb odd nitrogen, chlorine and ozone levels. Aerosol measurements by satellites began in NASA in 1975 with the Stratospheric Aerosol Measurement (SAM) program, to be followed by the Stratospheric Aerosol and Gas Experiment (SAGE) starting in 1979. Both programs employ the solar occultation, or Earth limb extinction, techniques. Major results of these activities include the discovery of polar stratospheric clouds (PSCs) in both hemispheres in winter, illustrations of the impacts of major (El Chichon 1982 and Pinatubo 1991) eruptions, and detection of a negative global trend in lower stratospheric/upper tropospheric aerosol extinction. This latter result can be considered a triumph of successful worldwide sulfur emission controls. The SAGE record will be continued and improved by SAGE III, currently scheduled for multiple launches beginning in 2000 as part of the Earth Observing System (EOS). The satellite program has been supplemented by in situ measurements aboard the ER-2 (20 km ceiling) since 1974, and from the DC-8 (13 km ceiling) aircraft beginning in 1989. Collection by wire impactors and subsequent electron microscopic and X-ray energy-dispersive analyses, and optical particle spectrometry have been the principle techniques. Major findings are: (1) The stratospheric background aerosol consists of dilute sulfuric acid droplets of around 0.1 micrometer modal diameter at concentration of tens to hundreds of monograms per cubic meter; (2) Soot from aircraft amounts to a fraction of one percent of the background total aerosol; (3) Volcanic eruptions perturb the sulfuric acid, but not the soot, aerosol abundance by several orders of magnitude; (4) PSCs contain nitric acid at temperatures below 195K, supporting chemical hypotheses implicating manmade fluorocarbons as cause of the --'ozone hole'; (5) The current soot loading is too small to be of environmental (radiative and chemical) consequence. However, the fractal nature of soot distinguishes it aerodynamically and radiatively from sulfuric acid droplets such that its stratospheric residence time is longer, mainly because of vertical transport against gravity due to gravito-photophoretic forces. Thus it may accumulate and become of environmental concern in the future.

Pueschel, Rudolf, F.↗
NASA NTRS2007

CALIPSO Observations of Stratospheric Aerosols: A Preliminary Assessment

We have examined the 532-nm aerosol backscatter coefficient measurements by the Cloud- Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) for their use in the observation of stratospheric aerosol. CALIPSO makes observations that span from 82 S to 82 N each day and, for each profile, backscatter coefficient values reported up to approx. 40 km. The possibility of using CALIPSO for stratospheric aerosol observations is demonstrated by the clear observation of the 20 May 2006 eruption of Montserrat in the earliest CALIPSO data in early June as well as by observations showing the 7 October 2006 eruption of Tavurvur (Rabaul). However, the very low aerosol loading within the stratosphere makes routine observations of the stratospheric aerosol far more difficult than relatively dense volcanic plumes. Nonetheless, we found that averaging a complete days worth of nighttime only data into 5-deg latitude by 1-km vertical bins reveals a stratospheric aerosol data centered near an altitude of 20 km, the clean wintertime polar vortices, and a small maximum in the lower tropical stratosphere. However, the derived values are clearly too small and often negative in much of the stratosphere. The data can be significantly improved by increasing the measured backscatter (molecular and aerosol) by approximately 5% suggesting that the current method of calibrating to a pure molecular atmosphere at 30 km is most likely the source of the low values.

Thomason, Larry W.↗
NASA NTRS2011

Titan's Aerosol and Stratospheric Ice Opacities Between 18 and 500 Micrometers: Vertical and Spectral Characteristics from Cassini CIRS

Vertical distributions and spectral characteristics of Titan's photochemical aerosol and stratospheric ices are determined between 20 and 560 per centimeter (500-18 micrometers) from the Cassini Composite Infrared Spectrometer (CIRS). Results are obtained for latitudes of 15 N, 15 S, and 58 S, where accurate temperature profiles can be independently determined. In addition, estimates of aerosol and ice abundances at 62 N relative to those at 15 S are derived. Aerosol abundances are comparable at the two latitudes, but stratospheric ices are approximately 3 times more abundant at 62 N than at 15 S. Generally, nitrile ice clouds (probably HCN and HC3N), as inferred from a composite emission feature at approximately 160 per centimeter, appear to be located over a narrow altitude range in the stratosphere centered at approximately 90 km. Although most abundant at high northern latitudes, these nitrile ice clouds extend down through low latitudes and into mid southern latitudes, at least as far as 58 S. There is some evidence of a second ice cloud layer at approximately 60 km altitude at 58 S associated with an emission feature at approximately 80 per centimeter. We speculate that the identify of this cloud may be due to C2H6 ice, which in the vapor phase is the most abundant hydrocarbon (next to CH4) in the stratosphere of Titan. Unlike the highly restricted range of altitudes (50-100 km) associated with organic condensate clouds, Titan's photochemical aerosol appears to be well-mixed from the surface to the top of the stratosphere near an altitude of 300 km, and the spectral shape does not appear to change between 15 N and 58 S latitude. The ratio of aerosol-to-gas scale heights range from 1.3-2.4 at about 160 km to 1.1-1.4 at 300 km, although there is considerable variability with latitude, The aerosol exhibits a very broad emission feature peaking at approximately 140 per centimeter. Due to its extreme breadth and low wavenumber, we speculate that this feature may be caused by low-energy vibrations of two-dimensional lattice structures of large molecules. Examples of such molecules include polycyclic aromatic hydrocarbons (PAHs) and nitrogenated aromatics. Finally, volume extinction coefficients N chi EPSILON derived from 15 S CIRS data at a wavelength of lambda = 62.5 micrometers are compared with those derived from the 10 S Huygens Descent Imager/Spectral Radiometer (DISR) data at 1.583 micrometers. This comparison yields volume extinction coefficient ratios N chi EPSILON (1.583 micrometers)/N chi EPSILON (62.5 micrometers) of roughly 70 and 20, respectively, for Titan's aerosol and stratospheric ices, The inferred particle cross-section ratios chi EPSILON(1.583 micrometers)/chi EPSILON (62.5 micrometers) appear to be consistent with sub-micron size aerosol particles, and effective radii of only a few microns for stratospheric ice cloud particles.

Anderson, Carrie M.↗
NASA NTRS2010

Finding the Missing Stratospheric Br(sub y): A Global Modeling Study of CHBr3 and CH2Br2

Recent in situ and satellite measurements suggest a contribution of ~5 pptv to stratospheric inorganic bromine from short-lived bromocarbons. We conduct a modeling study of the two most important short-lived bromocarbons, bromoform (CHBr3) and dibromomethane (CH2Br2), with the Goddard Earth Observing System Chemistry Climate Model (GEOS CCM) to account for this missing stratospheric bromine. We derive a "top-down" emission estimate of CHBr3 and CH2Br2 using airborne measurements in the Pacific and North American troposphere and lower stratosphere obtained during previous NASA aircraft campaigns. Our emission estimate suggests that to reproduce the observed concentrations in the free troposphere, a global oceanic emission of 425 Gg Br yr(exp -1) for CHBr3 and 57 Gg Br yr(exp -l) for CH2Br2 is needed, with 60% of emissions from open ocean and 40% from coastal regions. Although our simple emission scheme assumes no seasonal variations, the model reproduces the observed seasonal variations of the short-lived bromocarbons with high concentrations in winter and low concentrations in summer. This indicates that the seasonality of short-lived bromocarbons is largely due to seasonality in their chemical loss and transport. The inclusion of CHBr3 and CH2Br2 contributes ~5 pptv bromine throughout the stratosphere. Both the source gases and inorganic bromine produced from source gas degradation (Br~SLS) in the troposphere are transported into the stratosphere, and are equally important. Inorganic bromine accounts for half (2.5 pptv) of the bromine from the inclusion of CHBr3 and CHzBr2 near the tropical tropopause and its contribution rapidly increases to ~ 100% as altitude increases. More than 85% of the wet scavenging of Br(sub y)(sup VSLS) occurs in large-scale precipitation below 500 hPa. Our sensitivity study with wet scavenging in convective updrafts switched off suggests that Br(sub y)(sup SLS) in the stratosphere is not sensitive to convection. Convective scavenging only accounts for ~0.2 pptv (4%) difference in inorganic bromine delivered to the stratosphere.

Liang, Q.↗
NASA NTRS2012

Titan's Stratospheric Condensibles at High Northern Latitudes During Northern Winter

The Infrared Interferometer Spectrometer (IRIS) instrument on board Voyager 1 caught the first glimpse of an unidentified particulate feature in Titan's stratosphere that spectrally peaks at 221 per centimeter. Until recently, this feature that we have termed 'the haystack,' has been seen persistently at high northern latitudes with the Composite Infrared Spectrometer (CIRS) instrument onboard Cassini, The strength of the haystack emission feature diminishes rapidly with season, becoming drastically reduced at high northern latitudes, as Titan transitions from northern winter into spring, In contrast to IRIS whose shortest wavenumber was 200 per centimeter, CIRS extends down to 10 per centimeter, thus revealing an entirely unexplored spectral region in which nitrile ices have numerous broad lattice vibration features, Unlike the haystack, which is only found at high northern latitudes during northern winter/early northern spring, this geometrically thin nitrile cloud pervades Titan's lower stratosphere, spectrally peaking at 160 per centimeter, and is almost global in extent spanning latitudes 85 N to 600 S, The inference of nitrile ices are consistent with the highly restricted altitude ranges over which these features are observed, and appear to be dominated by a mixture of HCN and HC3N, The narrow range in altitude over which the nitrile ices extend is unlike the haystack, whose vertical distribution is significantly broader, spanning roughly 70 kilometers in altitude in Titan's lower stratosphere, The nitrile clouds that CIRS observes are located in a dynamically stable region of Titan's atmosphere, whereas CH4 clouds, which ordinarily form in the troposphere, form in a more dynamically unstable region, where convective cloud systems tend to occur. In the unusual situation where Titan's tropopause cools significantly from the HASI 70.5K temperature minimum, CH4 should condense in Titan's lower stratosphere, just like the aforementioned nitrile clouds, although in significantly larger abundances. We will present the spectral and vertical distribution of Titan's stratospheric particulates during northern winter on Titan. The drastically changing abundance of the haystack over a small latitude range will be highlighted, specifically comparing the IRIS and CIRS epochs, Finally, we will discuss the situation in which CH4 condenses in Titan's lower stratosphere, forming an unexpected quasi steady-state stratospheric Ice cloud.

Anderson, Carrie↗
NASA NTRS2013

Stratosphere-to-Troposphere Transport Revealed by Ground-based Lidar and Ozonesonde at a Midlatitude Site

This paper presents ozone structures measured by a ground-based ozone lidar and ozonesonde at Huntsville, Alabama, on 27-29 April 2010 originating from a stratosphere-to-troposphere transport event associated with a cutoff cyclone and tropopause fold. In this case, the tropopause reached 6 km and the stratospheric intrusion resulted in a 2-km thick elevated ozone layer with values between 70 and 85 ppbv descending from the 306-K to 298-K isentropic surface at a rate of 5 km day1. The potential temperature was provided by a collocated microwave profiling radiometer. We examine the corresponding meteorological fields and potential vorticity (PV) structures derived from the analysis data from the North American Mesoscale model. The 2-PVU (PV unit) surface, defined as the dynamic tropopause, is able to capture the variations of the ozone tropopause estimated from the ozonesonde and lidar measurements. The estimated ozone/PV ratio, from the measured ozone and model derived PV, for the mixing layer between the troposphere and stratosphere is approximately 41 ppbv/PVU with an uncertainty of approximately 33%. Within two days, the estimated mass of ozone irreversibly transported from the stratospheric into the troposphere is between 0.07 Tg (0.9 10(exp33) molecules) and 0.11 Tg (1.3 10(exp33) molecules) with an estimated uncertainty of 59%. Tropospheric ozone exhibited enormous variability due to the complicated mixing processes. Low ozone and large variability were observed in the mid-troposphere after the stratospheric intrusion due to the westerly advection including the transition from a cyclonic system to an anticyclonic system. This study using high temporal and vertical-resolution measurements suggests that, in this case, stratospheric air quickly lost its stratospheric characteristics once it is irreversibly mixed down into the troposphere.

Kuang, Shi↗
NASA NTRS2015

Stratospheric Benzene and Hydrocarbon Aerosols Detected in Saturn's Auroral Regions

Context. Saturn's polar upper atmosphere exhibits significant auroral activity; however, its impact on stratospheric chemistry (i.e. the production of benzene and heavier hydrocarbons) and thermal structure remains poorly documented. Aims. We aim to bring new constraints on the benzene distribution in Saturn's stratosphere, to characterize polar aerosols (their vertical distribution, composition, thermal infrared optical properties), and to quantify the aerosols' radiative impact on the thermal structure. Methods. Infrared spectra acquired by the Composite Infrared Spectrometer (CIRS) on board Cassini in limb viewing geometry are analysed to derive benzene column abundances and aerosol opacity profiles over the 3 to 0.1 mbar pressure range. The spectral dependency of the haze opacity is assessed in the ranges 680-900 and 1360-1440 cm(exp −1). Then, a radiative climate model is used to compute equilibrium temperature profiles, with and without haze, given the haze properties derived from CIRS measurements. Results. On Saturn's auroral region (80 deg S), benzene is found to be slightly enhanced compared to its equatorial and mid-latitude values. This contrasts with the Moses & Greathouse (2005, J. Geophys. Res., 110, 9007) photochemical model, which predicts a benzene abundance 50 times lower at 80◦S than at the equator. This advocates for the inclusion of ion-related reactions in Saturn's chemical models. The polar stratosphere is also enriched in aerosols, with spectral signatures consistent with vibration modes assigned to aromatic and aliphatic hydrocarbons, and presenting similarities with the signatures observed in Titan's stratosphere. The aerosol mass loading at 80 deg S is estimated to be 1−4 × 10(exp −5) g cm(exp −2), an order of magnitude less than on Jupiter, which is consistent with the order of magnitude weaker auroral power at Saturn.We estimate that this polar haze warms the middle stratosphere by 6 K in summer and cools the upper stratosphere by 5 K in winter. Hence, aerosols linked with auroral activity can partly account for the warm polar hood observed in Saturn's summer stratosphere.

satellites↗
NASA NTRS2019

Global Assimilation of Loon Stratospheric Balloon Observations

Accurate analyses of stratospheric winds are important for determining realistic constituent transport and providing improved diagnostic studies and forecasts of the stratosphere. This study examines impacts on global meteorological analyses resulting from using winds derived from Loon superpressure balloons in the lower stratosphere (hereafter Loon winds) as additional input observations to the Goddard Earth Observing System (GEOS) data assimilation system. To fully investigate the impacts of assimilating the Loon winds, two steps are taken: (1) comparison of the GEOS analysis winds with Loon winds (Control experiment) and (2) examination of the impacts of assimilating the Loon winds into the GEOS data assimilation system (Loon experiment). The time period selected is June–August 2014 when over 150 Loon balloons were launched, mainly in the Southern Hemisphere. In the middle latitudes, the Loon winds and Control winds agree well (Loon balloon zonal wind observation minus forecast, O − F, root‐mean‐square (RMS) values of ~2.75 m/s) and assimilating the Loon winds has a small impact (O − F RMS values unchanged). In the tropics, the Loon observations and Control analysis winds differ more than in middle latitudes (zonal wind O − F RMS ~3.75 m/s) and assimilating the Loon winds improves the zonal wind O − F RMS by ~1 m/s. In selected cases where the Loon observations and Control analysis differ greatly (O − F RMS values greater than 10 m/s), assimilating Loon winds significantly decreases the zonal wind O − F RMS by 5 m/s. These decreases in O − F RMS values show that the 6‐hr forecasts are improved at the Loon balloon observation locations. While satellites routinely measure Earth's global temperatures from space, in situ wind measurements are relatively scarce, consisting mainly of a network of ground‐based weather balloons. Since only a limited number of the weather balloons even reach stratospheric altitudes, there is a need for additional stratospheric observations. One option for addition wind information is the use of experimental superpressure balloons (SPBs). SPBs can remain in the stratosphere for many months traveling with the winds and hence, by reporting their changing positions, providing in situ wind observations. These SPBs experiments are generally limited in terms of time period and number of balloons. However, over the past few years Loon has been launching hundreds of SPBs (hereafter called Loon balloons) providing a more consistent set of observations of wind in the stratosphere. Here we assimilate some of the Loon balloon winds into the NASA GEOS global data assimilation system. The data assimilation system combines all observations with an atmospheric model to produce global analysis of winds and temperatures. Results show that including the Loon balloon wind information noticeably affects the global analysis as well as forecasts with the largest impact in the tropics. These results provide direction to future model and analysis improvements.

L. Coy↗
NASA NTRSDate not supplied

M2-SCREAM: A Stratospheric Composition Reanalysis of Aura MLS

Stratospheric composition and transport patterns are changing because of increasing greenhouse gas concentrations and declining levels of ozone depleting substances. Superimposed on forced trends are: dynamical variability at a range of time scales and unforeseen perturbations such as those resulting from injections of volcanic material and smoke from PyroCb events. Chemical reanalyses can be powerful tools for studying the composition of the stratosphere and disentangling forced responses from internal variability. This presentation introduces a new chemical reanalysis of stratospheric constituents developed and produced at NASA’s Global Modeling and Assimilation Office (GMAO) using the recently developed GMAO Constituent Data Assimilation System. Called the MERRA-2 Stratospheric Composition Reanalysis with Aura MLS (M2-SCREAM), this reanalysis consists of assimilated global three-dimensional fields of stratospheric ozone, water vapor, hydrogen chloride (HCl), nitric acid (HNO3) and nitrous oxide (N2O) mixing ratios and covers the period since the beginning of MLS observations in September 2004 to the present. M2-SCREAM assimilates version 4.2 MLS profiles of the five constituents alongside total ozone column from the Ozone Monitoring Instrument. The dynamics and tropospheric water vapor are constrained by assimilated meteorological fields from MERRA-2. The assimilated constituent fields and meteorology are provided to users at a 50-km horizontal resolution and a three-hourly frequency. Monthly analysis uncertainties and flags are also provided to the users. M2-SCREAM is an accurate and dynamically consistent high-resolution data record of the five constituents, all of which are of primary importance to stratospheric chemistry and transport studies. We will present a description of M2-SCREAM and selected results of a process-based evaluation of this product using independent data. As an illustration, we will discuss the perturbation to stratospheric composition from the eruption of Hunga Tonga–Hunga Ha'apai in January 2022 as seen in the reanalysis. We will also propose potential scientific applications of M2-SCREAM and outline plans for an upcoming comprehensive composition reanalysis that is being developed at NASA GMAO.

MERRA-2↗
NASA NTRSDate not supplied

Disruption of the 2022-2023 stratospheric circulation by the Hunga Tonga-Hunga Ha'apai volcano

In January 2022 the Hunga Tonga-Hunga Ha'apai (HTHH) volcano erupted, injecting an unprecedented amount of water vapor into the stratosphere that increased the total stratospheric water burden by ~10%. As the initial plume of water vapor spread throughout the stratosphere, radiative heating and cooling anomalies affected the stratospheric circulation altering the climatological mean residual circulation. Here we compare the 1980-2021 MERRA-2 (Modern Era Reanalysis for Research and Applications, Version 2) mean residual circulation climatology to the years 2022-2023 to identify stratospheric circulation changes associated with the anomalous water vapor. The HTHH water vapor is explicitly tracked using the M2-SCREAM (MERRA-2 Stratospheric Composition Reanalysis of Aura Microwave Limb Sounder) water vapor analysis. Anomalies in temperature, jet location, polar vortex strength and ozone advection in response to the HTHH water vapor anomaly are also documented. These results reveal details of the evolution of the HTHH induced stratospheric circulation anomalies with special emphasis on how these circulation anomalies affected the 2023 ozone hole.

Lawrence Coy↗
NASA NTRSDate not supplied

Disruption of the 2022-2023 Stratospheric Circulation By the Hunga Tonga-Hunga Ha'apai Volcano

In January 2022 the Hunga Tonga-Hunga Ha'apai (HTHH) volcano erupted, injecting an unprecedented amount of water vapor into the stratosphere that increased the total stratospheric water burden by ~10%. As the initial plume of water vapor spread throughout the stratosphere, radiative heating and cooling anomalies affected the stratospheric circulation altering the climatological mean residual circulation. Here we compare the 1980-2021 MERRA-2 (Modern Era Reanalysis for Research and Applications, Version 2) mean residual circulation climatology to the years 2022-2023 to identify stratospheric circulation changes associated with the anomalous water vapor. The HTHH water vapor is explicitly tracked using the M2-SCREAM (MERRA-2 Stratospheric Composition Reanalysis of Aura Microwave Limb Sounder) water vapor analysis. Anomalies in temperature, jet location, polar vortex strength and ozone advection in response to the HTHH water vapor anomaly are also documented. These results reveal details of the evolution of the HTHH induced stratospheric circulation anomalies with special emphasis on how these circulation anomalies affected the 2023 ozone hole.

Lawrence Coy↗
NASA NTRSDate not supplied

Relationships Between Variability in the Stratospheric Polar Vortex, Upper Tropospheric Jets, Tropopauses, and UTLS Ozone

The impacts of stratospheric polar vortex variations on upper troposphere / lower stratosphere (UTLS) circulation and composition are not well understood. We use stratospheric polar vortex geometry / strength diagnostics combined with characterisation of tropopauses and UTLS jets to show links between stratospheric polar vortex variability and regional variations in UTLS jet and tropopause characteristics. Polar vortex diagnostics are from Characterization and Analysis of Vortex Evolution using Algorithms for Region Tracking (CAVE-ART), while UTLS diagnostics are from JEt and Tropopause Products for Analysis and Characterization (JETPAC). We will present results showing UTLS jet and tropopause characteristics for strong and weak stratospheric vortex states (defined using vortex-focused metrics that are less dependent on geometry and position than commonly used diagnostics), as well as regional variations in correlations between CAVE-ART and JETPAC diagnostics. Furthermore, we will focus on preliminary results extending the stratospheric vortex, UTLS jet, and tropopause relationships to assess their impacts on regional ozone variations diagnosed from the M2-SCREAM (MERRA-2 Stratospheric Composition Reanalysis of Aura Microwave Limb Sounder) composition reanalysis.

Gloria Manney↗