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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 163 records · Page 9
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Probing Microstructure-induced Swelling & Thermal Property Changes in Ion-Irradiated Oxide Fuels using Laser-generated Surface Acoustic Waves

Radiation of fuel rods with neutrons during a fission reaction in a nuclear reactor is known to affect the material microstructure of the fuel as a result of fission fragment damage, and lead to the formation of atomic-level defects such as voids, dislocation loops, and lattice swelling from fission-gas release. A consequence of the radiation-induced damage in nuclear fuels is the drastic alteration of material properties, in particular, the reduction of the thermal conductivity – a key parameter that governs the transport of thermal energy released from fissile fuel atoms to the surrounding coolant. Swelling can induce high stresses and ultimate failure of the cladding. A fundamental understanding of the role of radiation-induced damage on the thermal transport and mechanical properties of nuclear fuels is therefore critical for efficient, reliable and safe operation of a nuclear power plant. As opposed to conventional post-irradiation examination techniques that are often time-consuming and require significant sample preparation, laser-based characterization methods have emerged as promising non-contact, non-destructive tools to measure the evolution of microstructure-induced material property changes. Moreover, laser methods offer the promise of in-situ characterization while the material is being irradiated. This project aims to develop an improved understanding of the impact of radiation-induced changes to material microstructure on the thermal and elastic properties of nuclear materials. A laser ultrasonic technique, known as the transient grating (TG) spectroscopy method, is used to simultaneously measure thermal diffusivity and elastic properties in unirradiated and ion-irradiated oxide nuclear fuel samples. The results will complement on-going investigations on electron- and phonon-mediated thermal transport in nuclear materials and will provide foundational work for incorporating the influence of defects in fuel performance codes.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
NASA NTRS1973

Surface electrical properties experiment study phase, volume 2

The choice of an antenna for a subsurface radio sounding experiment is discussed. The radiation properties of the antennas as placed on the surface of the medium is examined. The objective of the lunar surface electrical properties experiment is described. A numerical analysis of the dielectric permittivity and magnetic permeability of a subsurface domain is developed. The application of electromagnetic field measurements between one or more transmitting antennas and a roving receiving station is explained.

Source record↗
DOE OSTI2020

Macquarie Island Cloud and Radiation Experiment (MICRE) Field Campaign Report

The U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility, the Australian Antarctic Division (AAD), and the Australian Bureau of Meteorology (BOM) collaborated in deploying a variety of ground instrumentation to Macquarie Island between March 2016 and March 2018. Macquarie Island is located at 54.5° S, 158.9° E and is well situated for studying clouds over the Southern Ocean. The primary objective of the March 2016 to March 2018 deployment, hereafter the Macquarie Island Cloud and Radiation Experiment (MICRE), was to collect observations of surface radiation, cloud, precipitation, and aerosol properties. This report describes the instruments deployed and data sets collected, along with a summary of key data quality issues and information on some value-added products that are being developed to assist scientists in using the data.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1978

Climate modeling

The requirements for radiation measurements suitable for the understanding, improvement, and verification of models used in performing climate research are considered. Both zonal energy balance models and three dimensional general circulation models are considered, and certain problems are identified as common to all models. Areas of emphasis include regional energy balance observations, spectral band observations, cloud-radiation interaction, and the radiative properties of the earth's surface.

Source record↗
NASA NTRS1996

Importance of the Natural Terrestrial Environment with Regard to Advanced Launch Vehicle Design and Development

The terrestrial environment is an important forcing function in the design and development of the launch vehicle. The scope of the terrestrial environment includes the following phenomena: Winds; Atmospheric Thermodynamic Models and Properties; Thermal Radiation; U.S. and World Surface Environment Extremes; Humidity; Precipitation, Fog, and Icing; Cloud Characteristics and Cloud Cover Models; Atmospheric Electricity; Atmospheric Constituents; Vehicle Engine Exhaust and Toxic Chemical Release; Occurrences of Tornadoes and Hurricanes; Geological Hazards, and Sea States. One must remember that the flight profile of any launch vehicle is in the terrestrial environment. Terrestrial environment definitions are usually limited to information below 90 km. Thus, a launch vehicle's operations will always be influenced to some degree by the terrestrial environment with which it interacts. As a result, the definition of the terrestrial environment and its interpretation is one of the key launch vehicle design and development inputs. This definition is a significant role, for example, in the areas of structures, control systems, trajectory shaping (performance), aerodynamic heating and take off/landing capabilities. The launch vehicle's capabilities which result from the design, in turn, determines the constraints and flight opportunities for tests and operations.

Pearson, S. D.↗
NASA NTRSDate not supplied

Novel Hourly-Resolved Global Cloud Property Composite from Operational Satellites Imagers

Numerous applications in satellite remote sensing of surface properties, atmospheric state, composition, and radiation require accurate knowledge of the location and characteristics of clouds. Operational satellite imager radiances are valuable for cloud detection and for deriving many different physical parameters that can be used for a variety of weather, aviation, and energy applications. The NASA Satellite ClOud and Radiation Property retrieval System (SatCORPS) applies a suite of algorithms to meteorological satellite data to provide cloud properties, radiative fluxes and other parameters on a global scale. This paper describes a new global high-resolution dataset of cloud properties made available for community use that is constructed from analyses of a constellation of meteorological satellite imagers. Data taken from Meteosat-8/9 and -11, Himawari-8/9, GOES-16, and -17/-18, Aqua, Terra, Suomi-NPP and NOAA-20 are processed and composited on a 3-km grid to provide hourly global coverage. A historical multi-year dataset is available to serve various needs including modeling challenges related to cloud evaluations and parameterizations. Near real-time data products are also currently available between 60N and 60S. Efforts are underway to operationalize polar orbiting satellite cloud detection methods for low-latency applications over polar regions. The cloud detection and retrieval algorithms have been developed over many years to support NASA weather and climate programs such as the Clouds and Earth’s Radiant Energy System (CERES). To improve the utility of the data products, machine learning and other innovative methods are applied in various ways to help minimize data product uncertainties under the most challenging conditions and to improve their consistency at all times of day. A brief description of the methods highlighting the unique aspects of the SatCORPS data products will be presented along with information on their status and availability.

SatCORPS↗
NASA NTRS1960

Space-Environment Simulation at the Lewis Research Center

A knowledge of the environmental conditions in space and an understanding of the possible effect on objects in that environment is necessary in order to make a full-scale, systematic exploration of outer space. Once these conditions have been determined, the understanding of the behavior of objects in space may be gained by simulating the environment in the laboratory and conducting experiments in the simulated environment. Among the conditions in space which have been determined and may be simulated are the pressure, the temperature, and the radiant energy. Quantitatively, simulating these conditions would require a pressure as low as 10 (exp -16) mm Hg, a sink temperature of approximately 30 to 40 K, and radiation similar to that from a 6,000 K black body. The features of the space environment directly affect the thermal balance of the spacecraft. The temperature of the object is that temperature which provides equilibrium between the energy absorbed by the object and the energy emitted by the object. Hence, a knowledge of the absorption and emission characteristics for materials under space environmental conditions must be obtained. High-speed particles may impact and erode the material surfaces and in that way alter the radiation properties of the materials and finally change the equilibrium temperature. Also, since most of the radiant energy (that from the sun) is from one direction, the-heat-transfer within the body will provide surface-temperature variations which depend upon the shape and orientation of the object and the properties of the material. These variations may be effectively studied in the simulated environment. Finally, because of the vacuum the heat transferred to and from the object must be accomplished solely by radiation. Thus, if heat-cycle power-generation equipment is to be used, the necessary rejection of heat must be accomplished by radiation from waste heat radiators whose design must be investigated in order to determine optimum configurations.

Nichols, Lester D.↗
DOE OSTI2022

Temperature-dependent diffuse reflectance measurements of ceramic powders in the near- and mid-infrared spectra

Radiative properties are critical to quantify radiative energy fluxes between surfaces and in participating media. However, there is limited experimental data on temperature-dependent radiative properties of materials. Herein, this work focuses on experimentally measuring temperature-dependent diffuse reflectance in the near- and mid-infrared spectra (1–20 μm) for ceramic particles with applications as heat-transfer and thermal-storage media in concentrated solar power (CSP) plants. Specifically, a commercially available sintered bauxite proppant, ACCUCAST ID80, and its primary chemical constituents—alumina (Al 2 O 3 ) and silica (SiO 2 )—are measured in powder form using a Fourier transform infrared spectrometer (FTIR) coupled with a specialized diffuse reflectance accessory and a heated stage. Room-temperature diffuse reflectance measurements show increased absorption in tests with greater mass fractions of the ceramic samples. There is a strong correlation in the measured reflectance spectra of ACCUCAST with alumina and silica in the spectral range 2000–500 cm –1 (5–20 μm). Whereas, for shorter wavelengths (< 5 μm), the absorptance for ACCUCAST is greater than the absorptance for alumina and silica, indicating contributions from other chemical species present in the composite material. For the first time, temperature-dependent diffuse reflectance measurements are reported for ACCUCAST up to 1000 °C. These results are compared against those of alumina and silica through the calculation of a thermal emittance. All three materials exhibit a calculated emittance of ~0.9 at room temperature. However, this value decreases to ~0.6 for ACCUCAST and drops to less than 0.4 for alumina and silica at 1000 °C. Thermal cycling in air at 1000 °C resulted in a visible color change from dark grey to light orange for ACCUCAST and a subsequent larger increase in reflectance for wavelengths less than 5 μm as compared to ACCUCAST thermally cycled at 1000 °C in vacuum. Alumina and silica spectra proved to be largely unaffected by thermal cycling under atmospheric conditions. Overall, this study establishes a powerful technique for the characterization of radiative properties of particulate materials as a function of temperature and presents a detailed case study of ACCUCAST, a candidate for next-generation particle-based CSP.

14 SOLAR ENERGY↗
NASA NTRS2013

ARM Research in the Equatorial Western Pacific: A Decade and Counting

The tropical western Pacific (TWP) is an important climatic region. Strong solar heating, warm sea surface temperatures, and the annual progression of the intertropical convergence zone (ITCZ) across this region generate abundant convective systems, which through their effects on the heat and water budgets have a profound impact on global climate and precipitation. In order to accurately evaluate tropical cloud systems in models, measurements of tropical clouds, the environment in which they reside, and their impact on the radiation and water budgets are needed. Because of the remote location, ground-based datasets of cloud, atmosphere, and radiation properties from the TWP region have come primarily from short-term field experiments. While providing extremely useful information on physical processes, these short-term datasets are limited in statistical and climatological information. To provide longterm measurements of the surface radiation budget in the tropics and the atmospheric properties that affect it, the Atmospheric Radiation Measurement program established a measurement site on Manus Island, Papua New Guinea, in 1996 and on the island republic of Nauru in late 1998. These sites provide unique datasets now available for more than 10 years on Manus and Nauru. This article presents examples of the scientific use of these datasets including characterization of cloud properties, analysis of cloud radiative forcing, model studies of tropical clouds and processes, and validation of satellite algorithms. New instrumentation recently installed at the Manus site will provide expanded opportunities for tropical atmospheric science.

tropical regions↗
DOE OSTI2023

Science Plan for the Deployment of the Third ARM Mobile Facility to the Southeastern United States at the Bankhead National Forest, Alabama (AMF3 BNF)

In 2018, the U.S. Department of Energy (DOE) held a workshop for the Atmospheric Radiation Measurement (ARM) (Mather and Voyles 2013) user facility to discuss critical climate challenges and locations where key ARM Mobile Facility (AMF) observational assets could impact Earth system modeling (ESM). As an outcome, the southeast United States (SE U.S.) was identified as a high-priority region to target climate-process studies that promote a deeper understanding of the climate system and bolster ARM interactions with the community to drive ESM advancement. The DOE ARM user facility is a globally recognized leader in deploying and operating strategically located observation sites around the world for studying the properties of aerosols and clouds and their interaction with radiation, precipitation, and the Earth’s surface. In partnering with the DOE Atmospheric System Research (ASR) program, ARM solicited a multi-agency Site Science Team approach to provide input and close interaction with ARM management towards a successful SE U.S. deployment of the ARM third Mobile Facility (AMF3) (Miller et al. 2016). These efforts included identifying key locations, science drivers and instruments, and measurement strategies to address the wider climate-process needs and ESM improvement. Community input served a vital role in establishing, refining, and informing the relevant drivers and decisions regarding this AMF3 deployment. The team has identified Northern Alabama (N. AL) as regionally representative to unlock the key opportunities that will improve our understanding and model representation of aerosol, cloud, and land surface processes and their couplings in the SE U.S. A defining aspect of the AMF3 deployment is its commitment to long-term (anticipated five-year) observations to mitigate potential seasonal-to-annual variability that often limits appropriate attribution of phenomena to local or larger-scale processes. The proposed location may leverage nearby surface networks and multi-agency and partner assets to enrich this multi-year deployment. One motivation is to understand the role of spatiotemporal variability (thermodynamic, land-surface) across aspects of the climate system, with our AMF3 team anticipating future demands on characterizing the relationships between local-to-regional cloud development and surface processes across a diverse patchwork of natural, managed, and urban landscapes as found throughout the N. AL regions. The main site targets an intact, representative, forested region – the Bankhead National Forest (BNF) – underscoring further team commitment to regionally important land atmosphere two-way interactive studies “from the canopy to the clouds”, with enhanced tower instrumentation augmenting traditional ARM capabilities adjacent to this site. Multiple supplemental sites will also be distributed across this region, prioritizing added needs for biodiversity. Anticipated high-priority cloud science themes will target N. AL as a regional SE U.S. hotbed for high-impact weather, convective cloud onset, and shallow to-deep cloud transitioning. Anticipated aerosol drivers will focus on chemical processes that control the evolution of organic aerosol, the seasonality and spatial distribution of water vapor and particle-phase water, and its role on aerosol optical properties. Anticipated land atmosphere drivers consider the two-way feedbacks between surface influence on aerosols, clouds, and precipitation properties and the associated radiative impacts on plant physiology and canopy-scale fluxes. Emphasis will include the study of the impact of surface processes on aerosols via precursor emission, and on clouds via moisture flux and thermal development.

Doppler lidar, aerosols, convection↗
DOE OSTI2023

Science Plan for the Deployment of the Third ARM Mobile Facility to the Southeastern United States at the Bankhead National Forest, Alabama (AMF3 BNF)

In 2018, the U.S. Department of Energy (DOE) held a workshop for the Atmospheric Radiation Measurement (ARM) (Mather and Voyles 2013) user facility to discuss critical climate challenges and locations where key ARM Mobile Facility (AMF) observational assets could impact Earth system modeling (ESM). As an outcome, the southeast United States (SE U.S.) was identified as a high-priority region to target climate-process studies that promote a deeper understanding of the climate system and bolster ARM interactions with the community to drive ESM advancement. The DOE ARM user facility is a globally recognized leader in deploying and operating strategically located observation sites around the world for studying the properties of aerosols and clouds and their interaction with radiation, precipitation, and the Earth’s surface. In partnering with the DOE Atmospheric System Research (ASR) program, ARM solicited a multi-agency Site Science Team approach to provide input and close interaction with ARM management towards a successful SE U.S. deployment of the ARM third Mobile Facility (AMF3) (Miller et al. 2016). These efforts included identifying key locations, science drivers and instruments, and measurement strategies to address the wider climate-process needs and ESM improvement. Community input served a vital role in establishing, refining, and informing the relevant drivers and decisions regarding this AMF3 deployment. The team has identified Northern Alabama (N. AL) as regionally representative to unlock the key opportunities that will improve our understanding and model representation of aerosol, cloud, and land-surface processes and their couplings in the SE U.S. A defining aspect of the AMF3 deployment is its commitment to long-term (anticipated five-year) observations to mitigate potential seasonal-to-annual variability that often limits appropriate attribution of phenomena to local or larger-scale processes. The proposed location may leverage nearby surface networks and multi-agency and partner assets to enrich this multi-year deployment. One motivation is to understand the role of spatiotemporal variability (thermodynamic, land-surface) across aspects of the climate system, with our AMF3 team anticipating future demands on characterizing the relationships between local-to-regional cloud development and surface processes across a diverse patchwork of natural, managed, and urban landscapes as found throughout the N. AL regions. The main site targets an intact, representative, forested region – the Bankhead National Forest (BNF) – underscoring further team commitment to regionally important land-atmosphere two-way interactive studies “from the canopy to the clouds”, with enhanced tower instrumentation augmenting traditional ARM capabilities adjacent to this site. Multiple supplemental sites will also be distributed across this region, prioritizing added needs for biodiversity. Anticipated high-priority cloud science themes will target N. AL as a regional SE U.S. hotbed for high-impact weather, convective cloud onset, and shallow-to-deep cloud transitioning. Anticipated aerosol drivers will focus on chemical processes that control the evolution of organic aerosol, the seasonality and spatial distribution of water vapor and particle-phase water, and its role on aerosol optical properties. Anticipated land-atmosphere drivers consider the two-way feedbacks between surface influence on aerosols, clouds, and precipitation properties and the associated radiative impacts on plant physiology and canopy-scale fluxes. Emphasis will include the study of the impact of surface processes on aerosols via precursor emission, and on clouds via moisture flux and thermal development.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

U-Surf: a global 1 km spatially continuous urban surface property dataset for kilometer-scale urban-resolving Earth system modeling

High-resolution urban climate modeling has faced substantial challenges due to the absence of a globally consistent, spatially continuous, and accurate dataset to represent the spatial heterogeneity of urban surfaces and their biophysical properties. This deficiency has long obstructed the development of urban-resolving Earth system models (ESMs) and ultra-high-resolution urban climate modeling, over large domains. Here, we present U-Surf, a first-of-its-kind 1 km resolution present-day (circa 2020) global continuous urban surface parameter dataset. Using the urban canopy model (UCM) in the Community Earth System Model as a base model for satisfying dataset requirements, U-Surf leverages the latest advances in remote sensing, machine learning, and cloud computing to provide the most relevant urban surface biophysical parameters, including radiative, morphological, and thermal properties, for UCMs at the facet and canopy level. Generated using a systematically unified workflow, U-Surf ensures internal consistency among key parameters, making it the first globally coherent urban canopy surface dataset. U-Surf significantly improves the representation of the urban land heterogeneity both within and across cities globally; provides essential, high-fidelity surface biophysical constraints to urban-resolving ESMs; enables detailed city-to-city comparisons across the globe; and supports next-generation kilometer-resolution Earth system modeling across scales. U-Surf parameters can be easily converted or adapted to various types of UCMs, such as those embedded in weather and regional climate models, as well as air quality models. The fundamental urban surface constraints provided by U-Surf can also be used as features for machine learning models and can have other broad-scale applications for socioeconomic, public health, and urban planning contexts. We expect U-Surf to advance the research frontier of urban system science, climate-sensitive urban design, and coupled human–Earth systems in the future. The dataset is publicly available at https://doi.org/10.5281/zenodo.11247598 (Cheng et al., 2024).

Cheng, Yifan [Univ. of Illinois at Urbana-Champaig↗
NASA NTRS2018

Surface Irradiances of Edition 4.0 Clouds and the Earth's Radiant Energy System (CERES) Energy Balanced and Filled (EBAF) Data Product

The algorithm to produce the Clouds and the Earth’s Radiant Energy System (CERES) Edition 4.0 (Ed4) Energy Balanced and Filled (EBAF)-surface data product is explained. The algorithm forces computed topof- atmosphere (TOA) irradiances to match with Ed4 EBAF-TOA irradiances by adjusting surface, cloud, and atmospheric properties. Surface irradiances are subsequently adjusted using radiative kernels. The adjustment process is composed of two parts: bias correction and Lagrange multiplier. The bias in temperature and specific humidity between 200 and 500 hPa used for the irradiance computation is corrected based on observations by Atmospheric Infrared Sounder (AIRS). Similarly, the bias in the cloud fraction is corrected based on observations by Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) and CloudSat. Remaining errors in surface, cloud, and atmospheric properties are corrected in the Lagrange multiplier process. Ed4 global annual mean (January 2005 through December 2014) surface net shortwave (SW) and longwave (LW) irradiances increase by 1.3Wm22 and decrease by 0.2Wm22, respectively, compared to EBAF Edition 2.8 (Ed2.8) counterparts (the previous version), resulting in an increase in net SW 1LWsurface irradiance of 1.1Wm22. The uncertainty in surface irradiances over ocean, land, and polar regions at various spatial scales are estimated. The uncertainties in all-sky global annual mean upward and downward shortwave irradiance are 3 and 4Wm22, respectively, and the uncertainties in upward and downward longwave irradiance are 3 and 6Wm22, respectively. With an assumption of all errors being independent, the uncertainty in the global annual mean surface LW 1 SW net irradiance is 8Wm22.

Kato, Seiji↗
NASA NTRS1985

The First International Satellite Land-Surface Climatology Project (ISLSCP) Field Experiment (FIFE)

The International Satellite Land Surface Climatology Project (ISLSCP) will verify the use of satellite data for the estimation of land-surface properties through field experiments using point measurements on the ground and areal measurements from aircraft overflights. In addition to validating satellite estimates of surface properties, it studies approaches for obtaining areal averages of the radiation, moisture and heat fluxes made using remotely sensed data. The procedure suggested combines the surface point measurements of the fluxes with the aircraft areal observations using a surface energy balance model to interpolate between the point estimates of these fluxes and calculate area-averaged quantities. The surface parameters to be estimated from aircraft observations include: surface radiation temperature, albedo, land cover or vegetation index, and surface soil moisture (the latter to be obtained using passive and active microwave approaches). The area-averages of the surface properties are compared with satellite data where possible. The First ISLSCP Field Experiment is planned for l987 at a site having relatively uniform vegetation cover in the central great plains of the USA. for 1987 at a site having relatively uniform vegetation cover in the central great plains of the USA.

Schmugge, T. J.↗
NASA NTRS1998

Smoke, Clouds, and Radiation-Brazil (SCAR-B) Experiment

The Smoke, Clouds, and Radiation-Brazil (SCAR-B) field project took place in the Brazilian Amazon and cerrado regions in August-September 1995 as a collaboration between Brazilian and American scientists. SCAR-B, a comprehensive experiment to study biomass burning, emphasized measurements of surface biomass, fires, smoke aerosol and trace gases, clouds, and radiation. their climatic effects, and remote sensing from aircraft and satellites. It included aircraft and ground-based in situ measurements of smoke emission factors and the compositions, sizes, and optical properties of the smoke particles; studies of the formation of ozone; the transport and evolution of smoke; and smoke interactions with water vapor and clouds. This overview paper introduces SCAR-B and summarizes some of the main results obtained so far. (1) Fires: measurements of the size distribution of fires, using the 50 m resolution MODIS Airborne Simulator, show that most of the fires are small (e.g. 0.005 square km), but the satellite sensors (e.g., AVHRR and MODIS with I km resolution) can detect fires in Brazil which are responsible for 60-85% of the burned biomass: (2) Aerosol: smoke particles emitted from fires increase their radius by as much as 60%, during their first three days in the atmosphere due to condensation and coagulation, reaching a mass median radius of 0.13-0.17 microns: (3) Radiative forcing: estimates of the globally averaged direct radiative forcing due to smoke worldwide, based on the properties of smoke measured in SCAR-B (-O.l to -0.3 W m(exp -2)), are smaller than previously modeled due to a lower single-scattering albedo (0.8 to 0.9), smaller scattering efficiency (3 square meters g(exp -2) at 550 nm), and low humidification factor; and (4) Effect on clouds: a good relationship was found between cloud condensation nuclei and smoke volume concentrations, thus an increase in the smoke emission is expected to affect cloud properties. In SCAR-B, new techniques were developed for deriving the absorption and refractive index of smoke from ground-based remote sensing. Future spaceborne radiometers (e.g., MODIS on the Earth Observing System), simulated on aircraft, proved to be very useful for monitoring smoke properties, surface properties, and the impacts of smoke on radiation and climate.

Kaufman, Y. J.↗
NASA NTRSDate not supplied

TPSAS-NF1676L-10735-DND

The Clouds and the Earth's Radiant Energy System (CERES) project has now surpassed the 10-year mark, has combined rigorous calibration, improved scene identification, and multi-satellite data fusion to produce a climate-accuracy data set of global 1° gridded radiative surface and TOA fluxes, and cloud properties. CERES provides the climate community with four observed TOA flux products. The ERBE-like product uses the same algorithms as ERBE in order to be compared with the ERBE time period. The SSF product uses the improved scene identification and radiance to flux conversion. The SYN product uses GEO derived clouds and fluxes to provide diurnally complete TOA fluxes. The EBAF product provides net balanced fluxes tied to the ocean heat storage term. This product is suited for climate modelers estimating the global mean energy budget. Each successive CERES flux product applies the improvements over the previous product. This presentation will focus on the diurnal averaging improvements by the inclusion of imager radiances from 5 geostationary (GEO) satellites at 3-hourly intervals to estimate the flux in between CERES observations. The regional monthly mean flux differences based on SYN (CERES/GEO) and SSF (CERES-only) can exceed 20 Wm^-2. CERES shortwave and longwave fluxes have been rigorously validated and are key elements in evaluating the ability of climate models to predict both past and future climate states. The CERES normalization of GEO derived fluxes in order to maintain the CERES instrument calibration and are consistent globally within 0.1 Wm^-2, even if the GEO calibration is artificially altered by ±5%, twice the anticipated calibration error. The predicted GEO TOA fluxes normalized to Terra have been compared at Aqua times to Aqua flux observations, as well as with GERB hourly fluxes over the METEOSAT domain. Similarly ground based radiometers have been used to validate the CERES radiative transfer computed surface fluxes and have confirmed that the CERES/GEO fluxes have improved the computed surface flux product. Although the GEO based fluxes are of inferior quality then the CERES observed fluxes, they capture the diurnal signal more effectively than using constant meteorology between CERES measurements. The validation of the GEO derived fluxes and clouds will be shown.

D. R. Doelling↗
DOE OSTI2021

Aerosols from anthropogenic and biogenic sources and their interactions – modeling aerosol formation, optical properties, and impacts over the central Amazon basin

The Green Ocean Amazon experiment – GoAmazon 2014–2015 – explored the interactions between natural biogenic forest emissions from central Amazonia and urban air pollution from Manaus. Previous GoAmazon 2014–2015 studies showed that nitrogen oxide (NO x = NO + NO 2 ) and sulfur oxide (SO x ) emissions from Manaus strongly interact with biogenic volatile organic compounds (BVOCs), affecting secondary organic aerosol (SOA) formation. In previous studies, ground-based and aircraft measurements provided evidence of SOA formation and strong changes in aerosol composition and properties. Aerosol optical properties also evolve, and their impacts on the Amazonian ecosystem can be significant. As particles age, some processes, such as SOA production, black carbon (BC) deposition, particle growth and the BC lensing effect change the aerosol optical properties, affecting the solar radiation flux at the surface. This study analyzes data and models SOA formation using the Weather Research and Forecasting with Chemistry (WRF-Chem) model to assess the spatial variability in aerosol optical properties as the Manaus plumes interact with the natural atmosphere. The following aerosol optical properties are investigated: single scattering albedo (SSA), asymmetry parameter (g aer ), absorption Ångström exponent (AAE) and scattering Ångström exponent (SAE). These simulations were validated using ground-based measurements at three experimental sites, namely the Amazon Tall Tower Observatory – ATTO (T0a), downtown Manaus (T1), Tiwa Hotel (T2) and Manacapuru (T3), as well as the U.S. Department of Energy (DOE) Gulfstream 1 (G-1) aircraft flights. WRF-Chem simulations were performed over 7 d during March 2014. Results show a mean biogenic SOA (BSOA) mass enrichment of 512 % at the T1 site, 450 % in regions downwind of Manaus, such as the T3 site, and 850 % in areas north of the T3 site in simulations with anthropogenic emissions. The SOA formation is rather fast, with about 80 % of the SOA mass produced in 3–4 h. Comparing the plume from simulations with and without anthropogenic emissions, SSA shows a downwind reduction of approximately 10 %, 11 % and 6 % at the T1, T2 and T3 sites, respectively. Other regions, such as those further downwind of the T3 site, are also affected. The g aer values increased from 0.62 to 0.74 at the T1 site and from 0.67 to 0.72 at the T3 site when anthropogenic emissions are active. During the Manaus plume-aging process, a plume tracking analysis shows an increase in SSA from 0.91 close to Manaus to 0.98 160 km downwind of Manaus as a result of SOA production and BC deposition.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRSDate not supplied

Shock-Layer Radiation Insights Available Through Flowfield Property Binning

This paper introduces a method for assessing similarity between available shock-layer radiation measurements and the radiative heating to a vehicle of interest. This method will be referred to as the flowfield property binning (FPB) approach. The challenge in developing this approach is that radiometer measurements from a surface normal line of sight, observed radiation measurements of the entire shock-layer from a distance, or measured shock-tube nonequilibrium profiles are notably different geometrically than the radiative flux to a vehicle surface. Therefore, the relative contributions of various regions of the shock-layer to the measurement, and how these relative contributions compare with the radiative heating to a vehicle of interest, are unclear. By tracking the radiation contribution from each flowfield location, and then grouping this contribution based on two local flowfield properties, these geometric differences are removed. This provide a two dimensional group, or bin, distribution that represents the radiation environment in the same format for various types of radiation simulations, such as observed radiation or radiative flux to a vehicle surface. In the limits of optically-thin radiation transport and thermochemical equilibrium flow, the choice of pressure and temperature as the binning flowfield properties is shown to provide a bin distribution that uniquely defines the radiation simulation. This concept is found to be sufficient for establishing similarity between two cases even when the optically-thin radiation transport and thermochemical equilibrium assumptions are not satisfied. A simple metric of comparison between bin distributions from different cases is provided by the histogram intersection algorithm. This algorithm results in a histogram intersection factor (H) between 0 and 1, which represents the fraction of the radiation that is similar between the two cases. Therefore, if H evaluated between bin distributions for two completely different radiation problems is near 1, then they represent essentially the same radiation problem. This means that they depend on the same weighting of various radiation modeling parameters evaluated at the same pressure and temperature. If one of these cases agrees well with a radiation measurement, then the matching bin distributions provide justification for applying this experimental validation to the other case. Even for H values as low as 0.2, the measurement case could be considered relevant if there are no other useful measurements. This approach allows observed radiation measurements to directly inform radiative heating simulations, which allows NASA’s past and future investments in observed radiation measurements to directly inform the radiative heating uncertainty or margins for future vehicle design. This FPB approach is also used to determine shock-tube conditions for informing backshell radiative heating simulations, where the normal shock velocity and Lagrangian time from the shock is used for the binning variables instead of pressure and temperature.

Shock Layer Radiation↗