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At least 163 records · Page 9

Global-scale distribution of ozone in the remote troposphere from ATom and HIPPO airborne field missions

Ozone is a key constituent of the troposphere, where it drives photochemical processes, impacts air quality, and acts as a climate forcer. Large-scale in situ observations of ozone commensurate with the grid resolution of current Earth system models are necessary to validate model outputs and satellite retrievals. In this paper, we examine measurements from the Atmospheric Tomography (ATom; four deployments in 2016–2018) and the HIAPER Pole-to-Pole Observations (HIPPO; five deployments in 2009–2011) experiments, two global-scale airborne campaigns covering the Pacific and Atlantic basins. ATom and HIPPO represent the first global-scale, vertically resolved measurements of O3 distributions throughout the troposphere, with HIPPO sampling the atmosphere over the Pacific and ATom sampling both the Pacific and Atlantic. Given the relatively limited temporal resolution of these two campaigns, we first compare ATom and HIPPO ozone data to longer-term observational records to establish the representativeness of our dataset. We show that these two airborne campaigns captured on average 53 %, 54 %, and 38 % of the ozone variability in the marine boundary layer, free troposphere, and upper troposphere–lower stratosphere (UTLS), respectively, at nine well-established ozonesonde sites. Additionally, ATom captured the most frequent ozone concentrations measured by regular commercial aircraft flights in the northern Atlantic UTLS. We then use the repeated vertical profiles from these two campaigns to confirm and extend the existing knowledge of tropospheric ozone spatial and vertical distributions throughout the remote troposphere. We highlight a clear hemispheric gradient, with greater ozone in the Northern Hemisphere, consistent with greater precursor emissions and consistent with previous modeling and satellite studies. We also show that the ozone distribution below 8 km was similar in the extra-tropics of the Atlantic and Pacific basins, likely due to zonal circulation patterns. However, twice as much ozone was found in the tropical Atlantic as in the tropical Pacific, due to well-documented dynamical patterns transporting continental air masses over the Atlantic. Finally, we show that the seasonal variability of tropospheric ozone over the Pacific and the Atlantic basins is driven year-round by transported continental plumes and photochemistry, and the vertical distribution is driven by photochemistry and mixing with stratospheric air. This new dataset provides additional constraints for global climate and chemistry models to improve our understanding of both ozone production and loss processes in remote regions, as well as the influence of anthropogenic emissions on baseline ozone.

ATom, aircraft profiles, Atlantic pollution, ozone↗

A model of the spatial and temporal variation of the Uranus thermal structure

Seasonal variability of the temperature structure of Uranus is modeled for all latitudes in the .0004 to 2 bar pressure range in anticipation of the Voyager encounter in January 1986. Atmospheric heating in the model results on the one hand from an internal heat source and, on the other hand, from absorption of solar energy by methane and by non-conservative aerosols located between the 0.5 and 2 bar levels. Various cases for the behavior of the internal heat flux are investigated, such as constant with latitude or constrained to yield a time-averaged thermal emission independent of latitude. Meridional transport of heat in the stably stratified atmosphere is not taken into account. The results indicate that the Voyager encounter time, very small north-south temperature asymmetry should be expected. Moreover, the northern hemisphere, although not illuminated, should emit as much energy (within one percent) as the southern hemisphere at this date. At a given latitude, extreme temperatures are reached at the equinoxes. At the poles, seasonal amplitudes of about 10 K in the upper stratosphere and 6 K at the 0.6 bar level are predicted, and the variation with time of the emission to space is found to be at most 20 percent. The atmosphere of Uranus appears to be characterized by very long radiative response times (mainly due to its cold temperature) which inhibit the large seasonal variations that one could otherwise expect in view of the high obliquity of the planet and its long orbital period.

Bezard, B.↗

Satellite-Derived Dynamics of Southern Ocean Sea Ice

Antarctic ERS-2, RADARSAT Synthetic Aperture Radar and ERS-1/2 Scatterometer images were analyzed with SMMI radiometer image time-series data to investigate seasonal variability in satellite-tracked sea-ice dynamics in the Southern Ocean during 1992. Supporting field data were acquired during 'in-situ' experiments including the winter 1992 Ice Station Weddell and Winter Weddell Gyre studies. A variety of surface measurements were made during these experiments including Argos-buoy deployment and GPS drift measurements. These are used in conjunction with International Program for Antarctic Buoys drift trajectories for ice-motion tracking validation. Comparisons between gridded Special Sensor Microwave Imager (SSMI) ice-motion vectors and European Center for Medium Range Weather Forecasts/National Centers for Environmental Prediction (ECMWF/NCEP) analyses indicate that large-scale drift is forced predominantly by the long-term mean, large-scale synoptic pressure field. Only sub-daily SAR sea-ice tracking can capture high-frequency fluctuations, driven by polar lows or tidal forcing. In these cases, sea-ice drift can respond rapidly to changes in forcing on semi-diurnal time scales depending on the location with respect to the coastline. Seasonality of ice drift, particularly in the Weddell and Ross Seas, is linked to ice extent and compactness, and internal ice stresses transmitted through the pack ice from the coast. Three-monthly seasonal climatologies are presented of austral winter of ice drift in the Southern Ocean. The large Weddell and Ross Sea gyres are clearly resolved along with key seasonal and spatial attributes of their cyclonic circulation. Regional time series of ice dynamics parameters are used to illustrate correlations with meteorological forcing. Persistent divergence such as that occurring in the Ronne-Filchner polynya system results in large fractions of new ice. Similarly, convergence zones produce large fractions of deformed ice and characterize the dynamics of regions where perennial ice is observed. High shear strains also help delineate the axis of the Antarctic divergence in many places in the ice cover. In these regions, the separation between the coastal 'east wind drift'and ACC-dominated drift regimes is characterized by zonally extended regions of intense shear.

Drinkwater, Mark R.↗

Quantification of Aerosol Type, and Sources of Aerosols Over the Indo- Gangetic Plain

Differences and similarities in aerosol characteristics, for the first time, over two environmentally distinct locations in Indo-Gangetic plain (IGP) e Kanpur (KPR) (urban location) and Gandhi College (GC) (rural site) are examined. Aerosol optical depths (AODs) exhibit pronounced seasonal variability with higher values during winter and premonsoon. Aerosol fine mode fraction (FMF) and Ångstrom exponent (a) are higher over GC than KPR indicating relatively higher fine mode aerosol concentration over GC. Higher FMF over GC is attributed to local biomass burning activities. Analysis of AOD spectra revealed that aerosol size distribution is dominated by wide range of fine mode fractions or mixture of modes during winter and postmonsoon, while during premonsoon and monsoon coarse mode aerosols are more abundant. Single scattering albedo (SSA) is lower over GC than KPR. SSA spectra reveals the abundance of fine mode (coarse mode) absorbing (scattering) aerosols during winter and postmonsoon (premonsoon and monsoon). Spectral SSA features reveal that OC contribution to enhanced absorption is negligible. Analysis shows that absorbing aerosols can be classified as Mostly Black Carbon (BC), and Mixed BC and Dust over IGP. Mixed BC and dust is always higher over KPR, while Mostly BC is higher over GC throughout the year. The amount of long range transported dust exhibits a gradient between KPR (higher) and GC (lower). Results on seasonally varying aerosol types, and absorbing aerosol types and their gradients over an aerosol hotspot are important to tune models and to reduce the uncertainty in radiative and climate impact of aerosols.

Organic Carbon↗

Detecting Trend and Seasonal Changes in Bathymetry Derived from HICO Imagery: A Case Study of Shark Bay, Western Australia

The Hyperspectral Imager for the Coastal Ocean (HICO) aboard the International Space Station has offered for the first time a dedicated space-borne hyperspectral sensor specifically designed for remote sensing of the coastal environment. However, several processing steps are required to convert calibrated top-of-atmosphere radiances to the desired geophysical parameter(s). These steps add various amounts of uncertainty that can cumulatively render the geophysical parameter imprecise and potentially unusable if the objective is to analyze trends and/or seasonal variability. This research presented here has focused on: (1) atmospheric correction of HICO imagery; (2) retrieval of bathymetry using an improved implementation of a shallow water inversion algorithm; (3) propagation of uncertainty due to environmental noise through the bathymetry retrieval process; (4) issues relating to consistent geo-location of HICO imagery necessary for time series analysis, and; (5) tide height corrections of the retrieved bathymetric dataset. The underlying question of whether a temporal change in depth is detectable above uncertainty is also addressed. To this end, nine HICO images spanning November 2011 to August 2012, over the Shark Bay World Heritage Area, Western Australia, were examined. The results presented indicate that precision of the bathymetric retrievals is dependent on the shallow water inversion algorithm used. Within this study, an average of 70% of pixels for the entire HICO-derived bathymetry dataset achieved a relative uncertainty of less than +/-20%. A per-pixel t-test analysis between derived bathymetry images at successive timestamps revealed observable changes in depth to as low as 0.4 m. However, the present geolocation accuracy of HICO is relatively poor and needs further improvements before extensive time series analysis can be performed.

coastal marine↗

A TRMM Rainfall Estimation Method Applicable to Land Areas

Methods developed to estimate rain rate on a footprint scale over land with the satellite-borne multispectral dual-polarization Special Sensor Microwave Imager (SSM/1) radiometer have met with limited success. Variability of surface emissivity on land and beam filling are commonly cited as the weaknesses of these methods. On the contrary, we contend a more significant reason for this lack of success is that the information content of spectral and polarization measurements of the SSM/I is limited. because of significant redundancy. As a result, the complex nature and vertical distribution C, of frozen and melting ice particles of different densities, sizes, and shapes cannot resolved satisfactorily. Extinction in the microwave region due to these complex particles can mask the extinction due to rain drops. Because of these reasons, theoretical models that attempt to retrieve rain rate do not succeed on a footprint scale. To illustrate the weakness of these models, as an example we can consider the brightness temperature measurement made by the radiometer in the 85 GHz channel (T85). Models indicate that T85 should be inversely related to the rain rate, because of scattering. However, rain rate derived from 15-minute rain gauges on land indicate that this is not true in a majority of footprints. This is also supported by the ship-borne radar observations of rain in the Tropical Oceans and Global Atmosphere Coupled Ocean-Atmosphere Response Experiment (TOGA-COARE) region over the ocean. Based on these observations. we infer that theoretical models that attempt to retrieve rain rate do not succeed on a footprint scale. We do not follow the above path of rain retrieval on a footprint scale. Instead, we depend on the limited ability of the microwave radiometer to detect the presence of rain. This capability is useful to determine the rain area in a mesoscale region. We find in a given rain event that this rain area is closely related to the mesoscale-average rain rate. Based on this observation, in this study we have developed a method to estimate the mesoscale-average rain rate over land utilizing microwave radiometer data. Because of the high degree of geographic and seasonal variability in the nature and intensity of rain, this method requires some tuning with 15-minute rain gauge data on land. After tuning the method, it can be applied to an independent set of rain events that are close in time and space. We find that the mesoscale rain rates retrieved over the period of a month on land with this method shows a correlation of about 0.85 with respect to the surface rain-gauge observations. This mesoscale-average rain rate estimation method can be useful to extend the spatial and temporal coverage of the rainfall data provided by the Precipitation Radar on board the Tropical Rainfall Measuring Mission (TRMM) satellite.

Prabhakara, C.↗

Observations of Particle Number Size Distributions and New Particle Formation in Six Indian Locations

Atmospheric new particle formation (NPF) is a crucial process driving aerosol number concentrations in the atmosphere; it can significantly impact the evolution of atmospheric aerosol and cloud processes. This study analyses at least 1 year of asynchronous particle number size distributions from six different locations in India. We also analyze the frequency of NPF and its contribution to cloud condensation nuclei (CCN) concentrations. We found that the NPF frequency has a considerable seasonal variability. At the measurement sites analyzed in this study, NPF frequently occurs in March–May (pre-monsoon, about 21 % of the days) and is the least common in October–November (post-monsoon, about 7 % of the days). Considering the NPF events in all locations, the particle formation rate (J_(SDS)) varied by more than 2 orders of magnitude (0.001–0.6 /cu.cm s) and the growth rate between the smallest detectable size and 25 nm (GR_(SDS-25 nm)) by about 3 orders of magnitude (0.2–17.2 nm/h). We found that JSDS was higher by nearly 1 order of magnitude during NPF events in urban areas than mountain sites. GRSDS did not show a systematic difference. Our results showed that NPF events could significantly modulate the shape of particle number size distributions and CCN concentrations in India. The contribution of a given NPF event to CCN concentrations was the highest in urban locations (4.3 × 10^(3) /cu.cm per event and 1.2 × 10^(3)/cu.cm per event for 50 and 100 nm, respectively) as compared to mountain background sites (2.7 × 10^(3)/cu.cm per event and 1.0 × 10^(3)/cu.cm per event, respectively). We emphasize that the physical and chemical pathways responsible for NPF and factors that control its contribution to CCN production require in situ field observations using recent advances in aerosol and its precursor gaseous measurement techniques.

particle number size distributions↗

A Preliminary Assessment of ERTS Imagery for Marine Resources

The application of ERTS-1 imagery to identifying marine resources is discussed. Specific reference is made to the use of ERTS-1 for observing the onset of the spring growing season in the ocean while it occurs. ERTS-1 data is used for the following purposes: (1) location of large areas of seasonally variable biological activity, (2) measurement of water depth in shallow seas, (3) monitoring of sewer discharges, (4) assessment of erosion damage to beaches and shoreline installations, and (5) navigation through ice-filled waterways.

Ewing, G. C.↗

A search for global and seasonal variation of methane from Nimbus 4 IRIS measurements

The Nimbus 4 infrared interferometer spectrometer (IRIS) measurements in the region around wave number 1304 show absorption due to methane in the earth's atmosphere. From the laboratory measurements of the absorption coefficient and a selected vertical distribution corresponding to 1.13 atm cm of methane, a theoretical model for the transmittance at wave number 1304 is developed. The weighting function deduced from this model shows a maximum around 300 mb. Some weak absorption due to nitrous oxide in the atmosphere has been taken into account. The vertical temperature profile, derived from the 15 micron CO2 band in the IRIS spectrum, together with the methane weighting function have been used in a consistent way to compute the upwelling intensity at wave number 1304. The brightness temperature corresponding to the IRIS observed radiance at wave number 1304 has been compared with the brightness temperature deduced from the calculated upwelling intensity from 80 deg North to 80 deg South and for different periods of the year. This comparison shows that the two brightness temperatures agree with one another to within the accuracy of measurements about 2 K. From this result it was found that global or seasonal variability of methane is less than + or - 0.25 atm cm.

Prabhakara, C.↗

Ice particulates in the mesosphere

The observations of noctilucent clouds, the measurements of hydrated and of large immobile ions, and the light-scattering layer detected by the OGO-6 satellite suggest the presence of particulates, probably ice, in the mesosphere. The correlation between temperature and positive ion conductivity where the vapor pressure over ice becomes greater than atmospheric pressure in the stratopause region indicates the presence of ice crystals throughout the mesosphere over a wide range of latitudes during all seasons. Between one and ten billion ice crystals per cubic meter of order 10 nanometers in diameter can dominate ionization loss processes in the mesosphere, and can explain a variety of experimental observations, including observed solar angle dependence and seasonal variability of electron density.

Chesworth, E. T.↗

Interpretations of the EOLE experiment. II - Spatial variation of transient and stationary modes

An upper tropospheric and hemispheric scale data set, resulting from the EOLE constant density balloon experiment (conducted between August 1971 and July 1972) is used to study the spatial variation of various measured and derived fields. The quality and density of the data set is shown to be sufficient for such a study during the Southern Hemisphere spring, summer and autumn of the data period but inadequate during winter. The stationary modes of the Southern Hemisphere are shown to be relatively weak compared to their Northern Hemisphere counterparts and possess distinct seasonal phase shifts. The transient fields, on the other hand, show definite longitudinal anomalies in their seasonal mean properties with magnitudes up to thrice the zonal average. The transient fields show little seasonal variability in position. Furthermore, it appears that most of their magnitude results from the contribution of a relatively few but extremely intense disturbances which appear to possess a fairly regular variability in the 18-23 day range.

Webster, P. J.↗

Remote sensing of the ozone profile in the lower stratosphere using UV and IR measurements from Nimbus 4

With a three-parameter analytical model, the ozone profile below 10 mbar to the surface is derived from the Nimbus 4 satellite backscattered ultraviolet and infrared measurements. Comparison of the derived profiles with those observed by ozonesondes shows that gross features are satisfactorily reproduced. Meridional cross section of the ozone partial pressure derived from the satellite data reveal the significant equator-to-pole features, as well as seasonal variability. An examination of the sensitivity of the method shows that an error in infrared radiance of approximately 1 erg leads to an error of about 10 mbar in the weighted mean pressure of the ozone layer in the tropics.

Prabhakara, C.↗

Seasonal and geographical variation of blocking

An examination of grid point values of daily 500 mb geopotential height over the Northern Hemisphere for the 1963-1977 period has been conducted in order to calculate the seasonal frequency blocking variation and its geographical location, where blocking events require the persistence of a large positive anomaly for seven days or more. The geographical locations of the maximum frequency, characterized by three distinctly different maxima, remain nearly the same for all four seasons. Large persistent negative anomalies during the winter season are mostly associated with local high index flow. An examination of the seasonal variability of persistent characteristics of wave numbers 1-4, for 500 mb geopotential height between 50 and 70 deg N, shows that the large scale planetary waves have preferred phase locations for persistence beyond seven days.

Shukla, J.↗

Nimbus 7 CZCS - Reduction of its radiometric sensitivity with time

Preliminary results are described for an effort to quantify the sensitivity decay of a radiometry sensor (the Coastal Zone Color Scanner or CZCS aboard Nimbus 7). The method used in the study is to (1) compute the water-leaving radiance for imagery acquired in regions where this radiance is known or can be independently estimated, and (2) adjust the sensor calibration to force agreement between the two radiances. Decay factors for orbit numbers from 0 to 20,000 are plotted, and surface and space measurements are compared for the Gulf Stream and the Northern Sargasso Sea at different seasons. The fact that a seasonal variability in the chlorophyll a concentration in the Sargasso Sea was found in the sensor analysis (apparently the first such satellite observation) increases confidence in the method.

Gordon, H. R.↗

Measurements of stratospheric bromine

From 1974 to 1977, molecules containing acidic bromine were sampled in the stratosphere by using tetrabutyl ammonium hydroxide impregnated filters. Sampling was accomplished by WB-57F aircraft and high-altitude balloons, spanning latitudes from the equator to 75 deg N and altitudes up to 36.6 km. Analytical results are reported for 4 years of measurements and for laboratory simulations that determined the filter collection efficiencies for a number of brominated species. Mass mixing ratios for the collected bromine species in air average about 27 pptm in the stratosphere. Seasonal variability seems to be small.

Sedlacek, W. A.↗

Participation in the Mars Data Analysis Program: Analysis of cloud forms in Viking and Mariner 9 images

The first systematic account of the climate of Mars, based upon observations was produced. Cloud data were used to determine spatially and temporally varying near-surface wind direction, relative wind speed, static stability, and humidity conditions on a global scale. Existing models of meteorological processes were critically reexamined in light of the data, and more stringent constraints were set on global processes. Several discoveries were made, including the large extent and seasonal variability of the Mars equatorial Hadley cell, the failure of high latitude winds to reverse direction in early northern spring, the change in meridional wind component in southern midautum, and the almost constant cloud cover in the northern hemisphere, during spring and summer primarily by condensate clouds and in fall and winter by condensates and dust. The implications of these observations are discussed.

Gierasch, P.↗

Vertical distribution of dimethylsulfide, sulfur dioxide, aerosol ions, and radon over the northeast Pacific Ocean

The vertical distributions, in temperate latitudes, of dimethylsulfide (DMS), SO2, radon, methanesulfonate (MSA), nonsea-salt sulfate (nss-sulfate), and aerosol Na(+), NH4(+), and NO(-) ions were determined in samples collected by an aircraft over the northeast Pacific Ocean during May 3-12, 1985. DMS was also determined in surface seawater. It was found that DMS concentrations, both in seawater and in the atmospheric boundary layer, were significantly lower than the values reported previously for subtropical and tropical regions, reflecting the seasonal variability in the temperate North Pacific. The vertical profiles of DMS, MSA, SO2, and nss-sulfate were found to be strongly dependent on the convective stability of the atmosphere and on air mass origin. Biogenic sulfur emissions could account for most of the sulfur budget in the boundary layer, while the long-range transport of continentally derived air masses was mainly responsible for the elevated levels of both SO2 and nss-sulfate in the free troposphere.

Andreae, M. O.↗

Martian surface physical properties to be derived by radar altimeter on the Mars observer spacecraft

The potential is described of a candidate Mars Observer altimeter for determining dielectric properties of Mars regolith. It is pointed out that it is straightforward to use the time between altimeter pulse trains for passive radiometry (hence dielectric properties) and roughness can be derived. Given the mission plan the whole surface can be mapped at least three times, yielding data on seasonal variability.

Garvin, J. B.↗