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NASA NTRS1984

The photochemistry of a remote marine stratiform cloud

The coupled gas- and aqueous-phase photochemistry of a stratiform cloud in a remote region of the marine atmosphere is investigated with a time-dependent box model. Both scavenging of ambient acidic aerosols and gases as well as aqueous-phase chemical reactions within droplets are found to be important sources of acidity to cloud water and can lead to pH levels in cloud water in the remote marine atmosphere well below 5.6. The major sources of acidity via aqueous-phase chemical reactions are the generation of sulfuric acid from dissolved SO2 and the generation of formic acid from dissolved formaldehyde. In both cases, aqueous-phase free radicals can play a significant role either directly by oxidizing dissolved SO2 and HCHO or indirectly by producing the aqueous-phase oxidant H2O2. The rate of SO2 conversion to sulfuric acid is sensitive to a variety of parameters including the accommodation or sticking coefficient for SO2, H2O2, HO2, and OH, the liquid water content, and the ambient levels of SO2, HNO3, and other acidic or basic gases. Because high levels of SO2 tend to deplete cloud water of H2O3, the possibility exists that the pH of precipitation in polluted regions will respond nonlinearly to reduced SO2 emissions.

Chameides, W. L.↗

NASA NTRS2006

Relationships of Upper Tropospheric Water Vapor, Clouds and SST: MLS Observations, ECMWF Analyses and GCM Simulations

The relationships of upper tropospheric water vapor (UTWV), cloud ice and sea surface temperature (SST) are examined in the annual cycles of ECMWF analyses and simulations from 15 atmosphere-ocean coupled models which were contributed to the IPCC AR4. The results are compared with the observed relationships based on UTWV and cloud ice measurements from MLS on Aura. It is shown that the ECMWF analyses produce positive correlations between UTWV, cloud ice and SST, similar to the MLS data. The rate of the increase of cloud ice and UTWV with SST is about 30% larger than that for MLS. For the IPCC simulations, the relationships between UTWV, cloud ice and SST are qualitatively captured. However, the magnitudes of the simulated cloud ice show a considerable disagreement between models, by nearly a factor of 10. The amplitudes of the approximate linear relations between UTWV, cloud ice and SST vary by a factor up to 4.

sea surface temperature (SST)↗

NASA NTRS2012

Applications for Near-Real Time Satellite Cloud and Radiation Products

At NASA Langley Research Center, a variety of cloud, clear-sky, and radiation products are being derived at different scales from regional to global using geostationary satellite (GEOSat) and lower Earth-orbiting (LEOSat) imager data. With growing availability, these products are becoming increasingly valuable for weather forecasting and nowcasting. These products include, but are not limited to, cloud-top and base heights, cloud water path and particle size, cloud temperature and phase, surface skin temperature and albedo, and top-of-atmosphere radiation budget. Some of these data products are currently assimilated operationally in a numerical weather prediction model. Others are used unofficially for nowcasting, while testing is underway for other applications. These applications include the use of cloud water path in an NWP model, cloud optical depth for detecting convective initiation in cirrus-filled skies, and aircraft icing condition diagnoses among others. This paper briefly describes a currently operating system that analyzes data from GEOSats around the globe (GOES, Meteosat, MTSAT, FY-2) and LEOSats (AVHRR and MODIS) and makes the products available in near-real time through a variety of media. Current potential future use of these products is discussed.

Minnis, Patrick↗

NASA NTRS1997

Cloud Radiation Forcings and Feedbacks: General Circulation Model Tests and Observational Validation

Using an atmospheric general circulation model (the National Center for Atmospheric Research Community Climate Model: CCM2), the effects on climate sensitivity of several different cloud radiation parameterizations have been investigated. In addition to the original cloud radiation scheme of CCM2, four parameterizations incorporating prognostic cloud water were tested: one version with prescribed cloud radiative properties and three other versions with interactive cloud radiative properties. The authors' numerical experiments employ perpetual July integrations driven by globally constant sea surface temperature forcings of two degrees, both positive and negative. A diagnostic radiation calculation has been applied to investigate the partial contributions of high, middle, and low cloud to the total cloud radiative forcing, as well as the contributions of water vapor, temperature, and cloud to the net climate feedback. The high cloud net radiative forcing is positive, and the middle and low cloud net radiative forcings are negative. The total net cloud forcing is negative in all of the model versions. The effect of interactive cloud radiative properties on global climate sensitivity is significant. The net cloud radiative feedbacks consist of quite different shortwave and longwave components between the schemes with interactive cloud radiative properties and the schemes with specified properties. The increase in cloud water content in the warmer climate leads to optically thicker middle- and low-level clouds and in turn to negative shortwave feedbacks for the interactive radiative schemes, while the decrease in cloud amount simply produces a positive shortwave feedback for the schemes with a specified cloud water path. For the longwave feedbacks, the decrease in high effective cloudiness for the schemes without interactive radiative properties leads to a negative feedback, while for the other cases, the longwave feedback is positive. These cloud radiation parameterizations are empirically validated by using a single-column diagnostic model. together with measurements from the Atmospheric Radiation Measurement program and from the Tropical Ocean Global Atmosphere Combined Ocean-Atmosphere Response Experiment. The inclusion of prognostic cloud water produces a notable improvement in the realism of the parameterizations, as judged by these observations. Furthermore, the observational evidence suggests that deriving cloud radiative properties from cloud water content and microphysical characteristics is a promising route to further improvement.

Lee,Wan-Ho↗

NASA NTRS2019

Seasonal Variation in Martian Water Ice Cloud Particle Size

We employ the complete record of Mars limb-viewing observations by the Compact Reconnaissance Imaging Spectrometer, totaling 922 successful retrievals, to chart the seasonal variation in water ice cloud particle size. Low-latitude clouds exhibit particle size sorting with altitude at all seasons, with particles ranging from >3.0 m in effective radius to 1.01.5 m. However, at a given altitude, the ice particle size often varies through the year. Ice particle sizes in the tropics follow a different seasonal cycle than ice mixing ratio. North polar clouds have a complex seasonal cycle, with a sloped size profile with altitude as the polar hood cloud forms in early fall trending to a roughly uniform 1.5 m profile by the end of winter. These data are an important metric to validate and improve general circulation model microphysical routines and to better understand how martian water ice clouds influence the atmospheric radiative budget.

Scott D. Guzewich↗

NASA NTRS1990

Determination of cloud liquid water content using the SSM/I

As part of a calibration/validation effort for the special sensor microwave/imager (SSM/I), coincident observations of SSM/I brightness temperatures and surface-based observations of cloud liquid water were obtained. These observations were used to validate initial algorithms and to derive an improved algorithm. The initial algorithms were divided into latitudinal-, seasonal-, and surface-type zones. It was found that these initial algorithms, which were of the D-matrix type, did not yield sufficiently accurate results. The surface-based measurements of channels were investigated; however, the 85V channel was excluded because of excessive noise. It was found that there is no significant correlation between the SSM/I brightness temperatures and the surface-based cloud liquid water determination when the background surface is land or snow. A high correlation was found between brightness temperatures and ground-based measurements over the ocean.

Alishouse, John C.↗

NASA NTRS1989

Determinations of cloud liquid water in the tropics from the SSM/I

Upward-looking microwave radiometric observations were used to validate the SSM/I determinations, and also as a basis for the determination of new coefficients. Due to insufficiency of the initial four channel algorithm for cloud liquid water, the improved algorithm was derived from the CORRAD (the University of Massachusetts autocorrelation radiometer) measurements of cloud liquid water and the matching SSM/I brightness temperatures using the standard linear regression. The correlation coefficients for the possible four channel combinations, and subsequently the best and the worst combinations were determined.

Alishouse, John C.↗

NASA NTRS1991

Microwave simulations of a tropical rainfall system with a three-dimensional cloud model

A three-dinensional cloud model-microwave radiative transfer model combination is used to study the relations among the precipitation and other microphysical characteristics of a tropical oceanic squall line and the upwelling radiance at pertinent microwave frequencies. Complex brightness temperature-rain rate relations are evident at the full horizontal resolution (1.5 km) of the models, with spatial averaging producing smoother, shifter relations in most cases. Nonprecipitating cloud water is shown to be important in understanding the resulting distribution of brightness temperature. At the mature stage, convective portions of the cloud system are shown to produce different brightness temperature relations than the stratiform portion, primarily related to the distribution of cloud water. The evolution of the convective system from a small convective complex through its mature stage and the beginning of its dissipation also is shown to result in a variation of brightness temperature-rain relations, related to the distribution of cloud water and the evolution of ice in the precipitating system. The results of the study point to the need to take into account the evolution of nonprecipitating cloud water and precipitation-sized ice in the retrieval of rain from passive microwave space observations. This effect is evident for both the life cycle of individual convective elements and the life cycle of the convective system as a whole.

Adler, Robert A.↗

NASA NTRS2011

Collisional Evolution of the Enceladus Neutral Cloud

Water vapor ejected from Saturn's small moon Enceladus easily escapes its meager gravity to form a Saturn-encircling cloud with a low collision rate. Observations show that the cloud is quite broad in the radial direction, and we show here that collisions, though quite rare, may be largely responsible for this radial spreading. We modeled this cloud using the Direct Simulation Monte Carlo method, as fluid methods would be inappropriate for such a tenuous gas.

magnetic fields↗

NASA NTRS2002

New Concepts for Refinement of Cumulus Parameterization in GCM's the Arakawa-Schubert Framework

Several state-of-the-art models including the one employed in this study use the Arakawa-Schubert framework for moist convection, and Sundqvist formulation of stratiform. clouds, for moist physics, in-cloud condensation, and precipitation. Despite a variety of cloud parameterization methodologies developed by several modelers including the authors, most of the parameterized cloud-models have similar deficiencies. These consist of: (a) not enough shallow clouds, (b) too many deep clouds; (c) several layers of clouds in a vertically demoralized model as opposed to only a few levels of observed clouds, and (d) higher than normal incidence of double ITCZ (Inter-tropical Convergence Zone). Even after several upgrades consisting of a sophisticated cloud-microphysics and sub-grid scale orographic precipitation into the Data Assimilation Office (DAO)'s atmospheric model (called GEOS-2 GCM) at two different resolutions, we found that the above deficiencies remained persistent. The two empirical solutions often used to counter the aforestated deficiencies consist of a) diffusion of moisture and heat within the lower troposphere to artificially force the shallow clouds; and b) arbitrarily invoke evaporation of in-cloud water for low-level clouds. Even though helpful, these implementations lack a strong physical rationale. Our research shows that two missing physical conditions can ameliorate the aforestated cloud-parameterization deficiencies. First, requiring an ascending cloud airmass to be saturated at its starting point will not only make the cloud instantly buoyant all through its ascent, but also provide the essential work function (buoyancy energy) that would promote more shallow clouds. Second, we argue that training clouds that are unstable to a finite vertical displacement, even if neutrally buoyant in their ambient environment, must continue to rise and entrain causing evaporation of in-cloud water. These concepts have not been invoked in any of the cloud parameterization schemes so far. We introduced them into the DAO-GEOS-2 GCM with McRAS (Microphysics of Clouds with Relaxed Arakawa-Schubert Scheme).

Sud, Y. C.↗

NASA NTRS1980

Water-ice and water-updraft relationships near -10 C within populations of Florida cumuli

Evidence is presented for a sequential development of cloud water, rainwater, graupel, and crystalline ice with the aging of the cloud. This evidence is based on in-cloud microphysical data set collected in Florida convective towers that were penetrated close to their tops near -10 C; the very rapid onset of graupel that appears on repeat penetrations of some towers is of particular interest. A separate data set shows a large scatter in the relationship between the maximum value of cloud water and vertical velocity which indicates that measurements of cloud water can be misleading as an indication of growth activity. The sequential pass data showing the evolution of ice and water are consistent with a rime-splintering, secondary ice production hypothesis.

Sax, R. I.↗

NASA NTRS2004

Entrainment, Drizzle, and Cloud Albedo

Increased aerosol and hence droplet concentrations in polluted clouds are expected to inhibit precipitation and thereby increase cloud water, leading to more reflective clouds that partially offset global warming. Yet polluted clouds are not generally observed to hold more water. Much of the uncertainty regarding the indirect aerosol effect stems from inadequate understanding of such changes in cloud water. Detailed simulations show that the relative humidity of air overlying stratocumulus is a leading factor determining whether cloud water increases or decreases when precipitation is suppressed. When the overlying air is dry, cloud water can decrease as droplet concentrations increase.

Ackerman, A. S.↗

NASA NTRS2022

Hexagonal Prisms Form in Water-ice Clouds on Mars, Producing Halo Displays Seen by Perseverance Rover

Observations by several cameras on the Perseverance rover showed a 22° scattering halo around the Sun over several hours during northern midsummer (solar longitude 142°). Such a halo has not previously been seen beyond Earth. The halo occurred during the aphelion cloud belt season and the cloudiest time yet observed from the Perseverance site. The halo required crystalline water-ice cloud particles in the form of hexagonal columns large enough for refraction to be significant, at least 11 μm in diameter and length. From a possible 40-50 km altitude, and over the 3.3-hour duration of the halo, particles could have fallen 3-12 km, causing downward transport of water and dust. Halo-forming clouds are likely rare due to the high supersaturation of water that is required but may be more common in northern subtropical regions during northern midsummer.

M.T. Lemmon↗

NASA NTRS1978

Numerical experiments on the climatic sensitivity of an atmospheric hydrologic cycle

It is shown for an intermediate numerical model that fractional cloudiness and relative humidity decrease with increasing temperature. The fractional cloudiness decreases at a rate about 1 per deg K. This occurs in spite of an increase in the evaporation, water transport, condensation, precipitation and cloud water content with increasing temperature. These results are quite similar to those found from models with more highly parameterized clouds, notably the NCAR model. The fractional cloudiness in this model is measured by the fractional coverage of total cloud water and the fractional coverage of positive condensation, in addition to the relative humidity. It is also shown that some of the characteristics of a temperate climate can be simulated in an intermediate numerical model with periodic, antisymmetric and symmetric boundary conditions on an f plane. Intermediate models of this sort may therefore be useful to investigate general questions about the earth's hydrologic cycle on climatic space and time scales

Roads, J. O.↗

NASA NTRSDate not supplied

Validation of Modis Cloud Liquid Water Path to Prepare for Pace Evaluation Efforts

The Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) mission will launch in January 2024, extending and improving NASA’s global satellite observations in its eponymous domains. PACE’s hyperspectral Ocean Color Instrument (OCI) will offer daily near-global spatial coverage with a 1.2 km horizontal pixel size at the subsatellite point. PACE will also have two multi-angle polarimeters (HARP2 and SPEXone) capable of advanced atmospheric characterization. Validation of cloud retrievals is challenging. Here we evaluate liquid water path (LWP) from MODIS from the standard (MOD06) product. The same cloud optical properties retrieval algorithm will be applied to OCI data. This will allow us to understand the expected performance of this algorithm and to develop the processing and analysis code needed to evaluate PACE data. Please tell us what you think and if we should be doing something differently!

MODIS↗

NASA NTRS2019

Estimating the Altitudes of Martian Water-Ice Clouds Above the Mars Science Laboratory Rover Landing Site

This study retrieved estimated altitudes of Martian water-ice clouds through a comparison of observations taken by the Mars Science Laboratory (MSL, Curiosity) rover and the Mars Regional Atmospheric Modelling System (MRAMS). The vertical pointing of a Zenith Movie (ZM) allows many wind velocities and directions to be measured when clouds are observed, however without a lidar onboard the altitude of these clouds cannot be directly determined. By simulating conditions at Gale Crater with MRAMS, wind properties found in ZMs can be correlated with model outputs to estimate cloud altitudes at Gale Crater from the surface for the first time. These results are evaluated to assess any diurnal and seasonal cloud altitude patterns above Gale crater.

Campbell, Charissa L.↗

NASA NTRS2002

Clouds and Water Vapor in the Climate System and Radiative Transfer in Clear Air and Cirrus Clouds in the Tropics

Research supported under this grant was aimed at attacking unanswered scientific questions that lie at the intersection of radiation, dynamics, chemistry, and climate. Considerable emphasis was placed on scientific collaboration and the innovative development of instruments required to address these issues. Specific questions include water vapor distribution in the tropical troposphere, atmospheric radiation, thin cirrus clouds, stratosphere-troposphere exchange, and correlative science with satellite observations.

Anderson, James G.↗

NASA NTRS2002

Enhancement of Cloud Cover and Suppression of Nocturnal Drizzle in Stratocumulus Polluted by Haze

Recent satellite observations indicate a significant decrease of cloud water in ship tracks, in contrast to an ensemble of in situ ship-track measurements that show no average change in cloud water relative to the surrounding clouds. We find through large-eddy simulations of stratocumulus that the trend in the satellite data is likely an artifact of sampling only overcast clouds. The simulations instead show cloud cover increasing with droplet concentrations. Our simulations also show that increases in cloud water from drizzle suppression (by increasing droplet concentrations) are favored at night or at extremely low droplet concentrations.

Ackerman, Andrew S.↗