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NASA NTRS2012

Thermally Resilient, Broadband Optical Absorber from UV to IR Derived from Carbon Nanostructures

Optical absorber coatings have been developed from carbon-based paints, metal blacks, or glassy carbon. However, such materials are not truly black and have poor absorption characteristics at longer wavelengths. The blackness of such coatings is important to increase the accuracy of calibration targets used in radiometric imaging spectrometers since blackbody cavities are prohibitively large in size. Such coatings are also useful potentially for thermal detectors, where a broadband absorber is desired. Au-black has been a commonly used broadband optical absorber, but it is very fragile and can easily be damaged by heat and mechanical vibration. An optically efficient, thermally rugged absorber could also be beneficial for thermal solar cell applications for energy harnessing, particularly in the 350-2,500 nm spectral window. It has been demonstrated that arrays of vertically oriented carbon nanotubes (CNTs), specifically multi-walled-carbon- nanotubes (MWCNTs), are an exceptional optical absorber over a broad range of wavelengths well into the infrared (IR). The reflectance of such arrays is 100x lower compared to conventional black materials, such as Au black in the spectral window of 350-2,500 nm. Total hemispherical measurements revealed a reflectance of approximately equal to 1.7% at lambda approximately equal to 1 micrometer, and at longer wavelengths into the infrared (IR), the specular reflectance was approximately equal to 2.4% at lambda approximately equal to 7 micrometers. The previously synthesized CNTs for optical absorber applications were formed using water-assisted thermal chemical vapor deposition (CVD), which yields CNT lengths in excess of 100's of microns. Vertical alignment, deemed to be a critical feature in enabling the high optical absorption from CNT arrays, occurs primarily via the crowding effect with thermal CVD synthesized CNTs, which is generally not effective in aligning CNTs with lengths less than 10 m. Here it has been shown that the electric field inherent in a plasma yields vertically aligned CNTs at small length scales (less than 10 m), which still exhibit broadband, and high-efficiency optical absorption characteristics from the ultraviolet (UV) to IR. A thin and yet highly absorbing coating is extremely valuable for detector applications for radiometry in order to enhance sensitivity. A plasma-based process also increases the potential of forming the optical absorbers at lower synthesis temperatures in the future, increasing the prospects of integrating the absorbers with flexible substrates for low-cost solar cell applications, for example.

Kaul, Anupama B.↗

DOE OSTI2021

Transmission Spectroscopy for the Warm Sub-Neptune HD 3167c: Evidence for Molecular Absorption and a Possible High-metallicity Atmosphere

We present a transmission spectrum for the warm (500−600 K) sub-Neptune HD 3167c obtained using the Hubble Space Telescope Wide Field Camera 3 infrared spectrograph. We combine these data, which span the 1.125–1.643 μm wavelength range, with broadband transit measurements made using Kepler/K2 (0.6–0.9 μm) and Spitzer/IRAC (4–5 μm). We find evidence for absorption by at least one of H{sub 2}O, HCN, CO{sub 2}, and CH{sub 4} (Bayes factor 7.4; 2.5σ significance), although the data precision does not allow us to unambiguously discriminate between these molecules. The transmission spectrum rules out cloud-free hydrogen-dominated atmospheres with metallicities ≤100× solar at >5.8σ confidence. In contrast, good agreement with the data is obtained for cloud-free models assuming metallicities >700× solar. However, for retrieval analyses that include the effect of clouds, a much broader range of metallicities (including subsolar) is consistent with the data, due to the degeneracy with cloud-top pressure. Self-consistent chemistry models that account for photochemistry and vertical mixing are presented for the atmosphere of HD 3167c. The predictions of these models are broadly consistent with our abundance constraints, although this is primarily due to the large uncertainties on the latter. Interior structure models suggest that the core mass fraction is >40%, independent of a rock or water core composition, and independent of atmospheric envelope metallicity up to 1000× solar. We also report abundance measurements for 15 elements in the host star, showing that it has a very nearly solar composition.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2020

Parallel Broadband Femtosecond Reflection Spectroscopy at a Soft X-Ray Free-Electron Laser

X-ray absorption spectroscopy (XAS) and the directly linked X-ray reflectivity near absorption edges yield a wealth of specific information on the electronic structure around the resonantly addressed element. Observing the dynamic response of complex materials to optical excitations in pump–probe experiments requires high sensitivity to small changes in the spectra which in turn necessitates the brilliance of free electron laser (FEL) pulses. However, due to the fluctuating spectral content of pulses generated by self-amplified spontaneous emission (SASE), FEL experiments often struggle to reach the full sensitivity and time-resolution that FELs can in principle enable. Here, we implement a setup which solves two common challenges in this type of spectroscopy using FELs: First, we achieve a high spectral resolution by using a spectrometer downstream of the sample instead of a monochromator upstream of the sample. Thus, the full FEL bandwidth contributes to the measurement at the same time, and the FEL pulse duration is not elongated by a monochromator. Second, the FEL beam is divided into identical copies by a transmission grating beam splitter so that two spectra from separate spots on the sample (or from the sample and known reference) can be recorded in-parallel with the same spectrometer, enabling a spectrally resolved intensity normalization of pulse fluctuations in pump–probe scenarios. We analyze the capabilities of this setup around the oxygen K- and nickel L-edges recorded with third harmonic radiation of the free electron laser in Hamburg (FLASH), demonstrating the capability for pump–probe measurements with sensitivity to reflectivity changes on the per mill level.

36 MATERIALS SCIENCE↗

DOE OSTI2022

Time-resolved CO 2 , CO, and N 2 vibrational population measurements in Ns pulse discharge plasmas

Abstract Time-resolved CO 2 and N 2 vibrational populations and translational-rotational temperature are measured in a CO 2 –N 2 plasma sustained by a ns pulse discharge burst in plane-to-plane geometry. Time-resolved, absolute number density of CO generated in the plasma is also inferred from the experimental data. CO 2 and CO vibrational populations are measured by mid-IR, tunable quantum cascade laser absorption spectroscopy, and N 2 vibrational populations are measured by the ns broadband vibrational CARS. Transient excitation of N 2 and CO 2 asymmetric stretch vibrational energy modes is detected during the discharge burst. The time-resolved rate of CO generation does not correlate with N 2 or CO 2 ( ν 3 ) vibrational temperatures, indicating that CO 2 dissociation via the vibrational excitation is insignificant at the present conditions. The rate of CO generation decreases gradually during the discharge burst. The estimated specific energy cost of the CO product is close to that of N atoms in pure nitrogen, measured previously at similar operating conditions. Comparison of the experimental data with the kinetic modeling analysis indicates that CO 2 dissociation in collisions with electronically excited N 2 molecules is the dominant channel of CO generation at the present conditions, although the inferred CO yield in these processes is significantly lower than 1. The effect of vibrational energy transfer between N 2 and CO 2 on the plasma chemical processes is insignificant. The kinetic model underpredicts a rapid reduction of the N 2 and CO 2 ( ν 3 ) vibrational temperatures during the later half of the discharge burst and in the afterglow. V–T relaxation of N 2 by N and O atoms generated in the ns pulse discharge plasma does not affect the vibrational relaxation rate in a significant way. However, rapid V–T relaxation of CO 2 by O atoms has a significant effect on the relaxation rate. The difference between the experimental data and the modeling predictions may be due to the unknown scaling of the CO 2 –O V–T rates with the vibrational quantum number.

Physics↗

NASA NTRS2012

Satellite Remote Sensing of Snow/Ice Albedo over the Himalayas

The Himalayan glaciers and snowpacks play an important role in the hydrological cycle over Asia. The seasonal snow melt from the Himalayan glaciers and snowpacks is one of the key elements to the livelihood of the downstream densely populated regions of South Asia. During the pre-monsoon season (April-May-June), South Asia not only experiences the reversal of the regional meridional tropospheric temperature gradient (i.e., the onset of the summer monsoon), but also is being bombarded by dry westerly airmass that transports mineral dust from various Southwest Asian desert and arid regions into the Indo-Gangetic Plains in northern India. Mixed with heavy anthropogenic pollution, mineral dust constitutes the bulk of regional aerosol loading and forms an extensive and vertically extended brown haze lapping against the southern slopes of the Himalayas. Episodic dust plumes are advected over the Himalayas, and are discernible in satellite imagery, resulting in dust-capped snow surface. Motivated by the potential implications of accelerated snowmelt, we examine the changes in radiative energetics induced by aerosol transport over the Himalayan snow cover by utilizing space borne observations. Our objective lies in the investigation of potential impacts of aerosol solar absorption on the Top-of-Atmosphere (TOA) spectral reflectivity and the broadband albedo, and hence the accelerated snowmelt, particularly in the western Himalayas. Lambertian Equivalent Reflectivity (LER) in the visible and near-infrared wavelengths, derived from Moderate Resolution Imaging Spectroradiometer radiances, is used to generate statistics for determining perturbation caused due to dust layer over snow surface in over ten years of continuous observations. Case studies indicate significant reduction of LER ranging from 5 to 8% in the 412-860nm spectra. Broadband flux observations, from the Clouds and the Earth's Radiant Energy System, are also used to investigate changes in shortwave TOA flux over dust-laden and dust-free snow covered regions. Additionally, spatio-temporal and intra-seasonal variations of LER, along with snow cover information, are used to characterize the seasonal melt pattern and thus to distinguish the outstanding aerosol-induced snowmelt signal. Results from this observational work are expected to provide better understanding of the radiative impact of aerosols over snow surface, especially its role in the Himalayan hydro-glacialogical variability.

Hsu, N. Christina↗

DOE OSTI2023

Systems and methods for piezoelectric, electronic, and photonic devices with dual inversion layers

An apparatus comprising a substrate, one or more nanowire pillars, each having a base portion and a tip portion, a first electrode connected to the tip portions of the one or more nanowire pillars, an internal hollow cavity positioned between the substrate and the first electrode, such that at least a portion of each of the one or more nanowire pillars extend through the internal hollow cavity, and a second electrode proximate the first side of the substrate. High-performance broadband photodetectors and other optoelectronics for converting light to electricity with enhanced absorption and carrier collection.

30 DIRECT ENERGY CONVERSION↗

DOE OSTI2023

The outburst of the changing-look AGN IRAS 23226-3843 in 2019

IRAS 23226-3843 has previously been classified as a changing-look active galactic nucleus (AGN) based on observations taken in the 1990s in comparison to X-ray data (Swift, XMM-Newton, and NuSTAR) and optical spectra taken after a very strong X-ray decline in 2017. In 2019, Swift observations revealed a strong rebrightening in X-ray and UV fluxes. We aimed to study this outburst in greater detail. We took follow-up Swift, XMM-Newton, and NuSTAR observations of IRAS 23226-3843 together with optical spectra (SALT and SAAO 1.9 m telescope) from 2019 until 2021. IRAS 23226-3843 showed a strong X-ray and optical outburst in 2019. It varied in the X-ray continuum by a factor of 5 and in the optical continuum by a factor of 1.6 within two months. This corresponds to a factor of 3 after correction for the host galaxy contribution. The Balmer and Fe II emission-line intensities showed comparable variability amplitudes during the outburst in 2019. The Hα emission-line profiles of IRAS 23226-3843 changed from a blue-peaked profile in the years 1997 and 1999 to a broad double-peaked profile in 2017 and 2019. However, there were no major profile variations in the extremely broad double-peaked profiles despite the strong intensity variations in 2019. One year after the outburst, IRAS 23226-3843 changed its optical spectral type and became a Seyfert type 2 object in 2020. Blue outflow components are present in the optical Balmer lines and in the Fe band in the X-rays. A deep broadband XMM-Newton/NuSTAR spectrum was taken during IRAS 23226-3843’s maximum state in 2019. This spectrum is qualitatively very similar to a spectrum taken in 2017, but by a factor of 10 higher. The soft X-ray band appears featureless. The soft excess is well modeled with a Comptonization model. A broadband fit with a power-law continuum, Comptonized soft excess, and Galactic absorption gives a good fit to the combined EPIC-pn and NuSTAR spectrum. In addition, we see a complex and broadened Fe K emission-line profile in the X-rays. The changing-look character in IRAS 23226-3843 is most probably caused by changes in the accretion rate – based on the short-term variations on timescales of weeks to months.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS2017

Characterizing Non-Resolved Debris Through Spectral and Photometric Ground-Based Telescopic Data: What Can Laboratory Ground-truth Data Do for You?

NASA's ODPO has recently collected data of unresolved objects at GEO with the 3.8m UKIRT infrared telescope on Mauna Kea and the 1.3m MCAT visible telescope on Ascension Island. Analyses of SWIR data of rocket bodies and HS-376 solar-panel covered buses demonstrate the uniqueness of spectral signatures. Data of 3 classes of rocket bodies show similarities amongst a given class, but distinct differences from one class to another, suggesting that infrared reflectance spectra could effectively be used toward characterizing and constraining potential parent bodies of uncorrelated targets (UCTs). The Optical Measurements Center (OMC) at NASA JSC is designed to collect photometric signatures in the laboratory that can be used for comparison with telescopic data. NASA also has a spectral database of spacecraft materials for use with spectral unmixing models. Spectral unmixing of the HS-376 bus data demonstrates how absorption features and slopes can be used to constrain material characteristics of debris. Broadband photometry likewise can be compared with MCAT data of non-resolved debris images. Similar studies have been applied to IDCSP satellites to demonstrate how color-color photometry can be compared with lab data to constrain bulk materials signatures of spacecraft and debris.

Lederer, Susan↗

DOE OSTI2022

Metallo-graphene nanocomposites and methods for using metallo-graphene nanocomposites for electromagnetic energy conversion

Nanocomposites in accordance with many embodiments of the invention can be capable of converting electromagnetic radiation to an electric signal, such as signals in the form of current or voltage. In some embodiments, metallic nanostructures are integrated with graphene material to form a metallo-graphene nanocomposite. Graphene is a material that has been explored for broadband and ultrafast photodetection applications because of its distinct optical and electronic characteristics. However, the low optical absorption and the short carrier lifetime of graphene can limit its use in many applications. Nanocomposites in accordance with various embodiments of the invention integrates metallic nanostructures, such as (but not limited to) plasmonic nanoantennas and metallic nanoparticles, with a graphene-based material to form metallo-graphene nanostructures that can offer high responsivity, ultrafast temporal responses, and broadband operation in a variety of optoelectronic applications.

Jarrahi, Mona↗

DOE OSTI2023

Carrier and Phonon Dynamics in Multilayer WSe 2 Captured by Extreme Ultraviolet Transient Absorption Spectroscopy

Carrier and phonon dynamics in a multilayer WSe2 film are captured by extreme ultraviolet (XUV) transient absorption (TA) spectroscopy at the W N 6,7 , W O 2,3 , and Se M 4,5 edges (30–60 eV). After the broadband optical pump pulse, the XUV probe directly reports on occupations of optically excited holes and phonon-induced band renormalizations. Here, when compared with density functional theory calculations, XUV transient absorption due to holes is identified below the W O 3 edge whereas signals at the Se M 4,5 edges are dominated by phonon dynamics. Therein, 0.4 ps hole relaxation time, 1.5 ps carrier recombination time, and 1.7 ps phonon heating time are extracted. The acquisition of hole and phonon-induced signals in a single experiment can facilitate the investigation of the correlations between electron and phonon dynamics. Furthermore, the simultaneous observation of signals from different elements can be further extended to explore photochemical processes in multilayers and alloys, thereby providing key information for their applications in electronics, photocatalysts, and spintronics.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2023

Dual Emission Bands of a 2D Perovskite Single Crystal with Charge Transfer State Characteristics

Several hybrid halide 2D-perovskite species emit light with an emergent and controversial broadband emission Stokes-shifted down from the narrow band emission. This work uncovers the sub- and above-bandgap emission and absorption characteristics of PEA 2 PbI 4 prepared with gap states introduced during single crystal growth. Here, gap states led to coexistent intrinsic and heterostructured electronic frameworks that are selectively accessible with ultraviolet (UV) and infrared (IR) light, respectively, resulting in the phenomenon of photoluminescence (PL) switching from narrowband green to broadband red. Electron-energy dependent cathodoluminescence shows a relative increase in the broadband red PL intensity as the electron penetration depth increases from 30 nm to 2 μm, confirming the heterostructured framework is formed in the bulk of the crystal. Excitation–emission power slope of 2.5 and up-conversion pump transient absorption (TA) spectra suggest that the IR up-conversion excitation with red photoluminescence, peaked at 655 nm, is a multiphoton process occurring in the heterostructured framework through a nonlinear optical response. The energetic pathways toward the dual emission bands are revealed by pump–probe transient absorption spectroscopy, showing energetically broad gap states with high sensitivity to an IR pump are upconverted and subsequently quickly relax from high to low energy levels within 4 ps. Furthermore, the up-conversion red PL demonstrates a linear polarization with magnetic field effects, thus affirming that the band-like heterostructured framework is crystallographically aligned with characteristics of spatially extended charge-transfer states.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2025

Improved Representations of Longwave Surface Emissivity to Reduce Surface and Atmospheric Heating Biases in Earth System Models

Abstract Many Earth system models (ESMs) approximate surface emissivity as a broadband constant. This approximation reduces the computational burden, yet omits the spectral structure of emissivity and atmospheric absorption. Neglecting spectral variation in surface emission introduces biases in longwave (LW) atmospheric fluxes and heating. Biases are strongest over surfaces with strongly varying emissivity and minimal atmospheric opacity. We examine these biases over water, ice, and snow surfaces. We partition spectral emissivity into the 16 spectral bands utilized by a single‐column atmospheric radiative transfer model (RRTMG_LW) commonly used in ESMs. We quantify flux and heating biases introduced by broadband assumptions relative to the spectrally resolved case for standard atmospheric profiles over each surface type. Current assumptions tend to overestimate upwelling surface fluxes; for example, the greybody assumption overestimates flux by 1.6 W/m 2 (0.52%) at the bottom of a mid‐latitude winter atmosphere over ice, and by 2.33 (1.0%) at the top of atmosphere. The blackbody assumption tends to artificially cool Earth's surface, stabilizing the lower troposphere. Interestingly, the optimal broadband emissivity can deviate from the Planck‐weighted mean by up to 3% depending on surface type and atmospheric profile. We investigate bias sensitivity to surface temperature, cloud water path, and atmospheric water vapor. Bias is most sensitive to water vapor content, and least sensitive to cloud water path. Lastly, we show that a modified greybody method with updated broadband values can reduce total surface flux bias up to 1.69 , comparable to a five‐band approach and at a fraction of the computational cost.

Manzo, L. [Department of Earth System Science Univ↗

DOE OSTI2025

Discovery of Powerful Multivelocity Ultrafast Outflows in the Starburst Merger Galaxy IRAS 05189–2524 with XRISM

We observed the X-ray-bright ultraluminous infrared galaxy IRAS 05189−2524 with XRISM during its performance verification phase. The unprecedented energy resolution of the onboard X-ray microcalorimeter revealed complex spectral features at ∼7–9 keV, which can be interpreted as blueshifted Fe XXV/XXVI absorption lines with various velocity dispersions, originating from ultrafast outflow (UFO) components with multiple bulk velocities of ∼0.076c, ∼0.101c, and ∼0.143c. In addition, a broad Fe–K emission line was detected around ∼7 keV, forming a P Cygni profile together with the absorption lines. The onboard X-ray CCD camera revealed a 0.4–12 keV broadband spectrum characterized by a neutrally absorbed power-law continuum with a photon index of ∼2.3 and intrinsic flare-like variability on timescales of ∼10 ks, both of which are likely associated with near-Eddington accretion. We also found potential variability of the UFO parameters on a timescale of ∼140 ks. Using these properties, we propose new constraints on the outflow structure and suggest the presence of multiple outflowing regions on scales of about tens to 100 Schwarzschild radii, located within roughly 2000 Schwarzschild radii. Since both the estimated momentum and energy outflow rates of the UFOs exceed those of galactic molecular outflows, our results indicate that powerful, multivelocity UFOs are already well developed during a short-lived evolutionary phase following a major galaxy merger, characterized by intense starburst activity and likely preceding the quasar phase. This system is expected to evolve into a quasar, sustaining strong UFO activity and suppressing star formation in the host galaxy.

Astronomy and AstroPhysics↗

NASA NTRS1993

Measurements of soot formation and hydroxyl concentration in near critical equivalence ratio premixed ethylene flame

The testing and development of existing global and detailed chemical kinetic models for soot formation requires measurements of soot and radical concentrations in flames. A clearer understanding of soot particle inception relies upon the evaluation and refinement of these models in comparison with such measurements. We present measurements of soot formation and hydroxyl (OH) concentration in sequences of flat premixed atmospheric-pressure C2H4/O2/N2 flames and 80-torr C2H4/O2 flames for a unique range of equivalence ratios bracketting the critical equivalence ratio (phi(sub c)) and extending to more heavily sooting conditions. Soot volume fraction and number density profiles are measured using a laser scattering-extinction apparatus capable of resolving a 0.1 percent absorption. Hydroxyl number density profiles are measured using laser-induced fluorescence (LIF) with broadband detection. Temperature profiles are obtained from Rayleigh scattering measurements. The relative volume fraction and number density profiles of the richer sooting flames exhibit the expected trends in soot formation. In near-phi(sub c) visibility sooting flames, particle scattering and extinction are not detected, but an LIF signal due to polycyclic aromatic hydrocarbons (PAH's) can be detected upon excitation with an argon-ion laser. A linear correlation between the argon-ion LIF and the soot volume fraction implies a common mechanistic source for the growth of PAH's and soot particles. The peak OH number density in both the atmospheric and 80-torr flames declines with increasing equivalence ratio, but the profile shape remains unchanged in the transition to sooting, implying that the primary reaction pathways for OH remain unchanged over this transition. Chemical kinetic modeling is demonstrated by comparing predictions using two current reaction mechanisms with the atmospheric flame data. The measured and predicted OH number density profiles show good agreement. The predicted benzene number density profiles correlate with the measured trends in soot formation, although anomalies in the benzene profiles for the richer and cooler sooting flames suggest a need for the inclusion of benzene oxidation reactions.

Inbody, Michael Andrew↗

NASA NTRS1993

Some effects of dust on photometry of high-z galaxies: Confounding the effects of evolution

Photometric observations of very distant galaxies--e.g., color vs. z or magnitude vs. z, have been used over the past decade or so in investigations into the evolution of the stellar component. Numerous studies have predicted significant color variations as a result of evolution, in addition to the shifting of different rest wavelengths into the band of observation. Although there is significant scatter, the data can be fit with relatively straightforward, plausible models for galaxian evolution. In very few cases are the effects of dust extinction included in the models. This is due in a large part to the uncertainty about the distribution and optical properties of the grains, and even whether or not they are present in significant numbers in some types of galaxies such as ellipticals. It is likely that the effects of dust on broadband observations are the greatest uncertainty in studies of very distant galaxies. We use a detailed Monte Carlo radiative transfer model within a spherical geometry for different star/dust distributions to examine the effects of dust on the broadband colors of galaxies as a function of redshift. The model fully accounts for absorption and angular redistribution in scattering. In this summary, we consider only the effects on color vs. redshift for three simple geometries each with the same total dust optical depth. Elsewhere at this conference, Capuano, Thronson, & Witt consider other effects of altering the relative dust/star distribution.

Thronson, H. A., Jr.↗

NASA NTRS1994

Comprehensive stellar population models and the disentanglement of age and metallicity effects

The construction of detailed models for intermediate and old stellar populations is described. Input parameters include metallicity (-2 less than (Fe/H) less than 0.5), single-burst age (between 1.5 and 17 Gyr), and initial mass function (IMF) exponent. Quantities output include broadband magnitudes, spectral energy distributions, surface brightness fluctuation magnitudes, and a suite of 21 absorption feature indices. The models are checked against a wide variety of available observations. Examinations of model output yield the following conclusions. (1) If the percentage change delta age/delta Z approximately equals 3/2 for two populations, they will appear almost identical in most indices. A few indices break this degeneracy by being either more abundance sensitive (Fe4668, Fe5015, Fe5709, and Fe5782) or more age sensitive (G4300, H beta, and presumably higher order Balmer lines) than usual. (2) Present uncertainties in stellar evolution are of the same magnitude as the effects of IMF and Y in the indices studied. (3) Changes in abundance ratios (like (Mg/Fe)) are predicted to be readily apparent in the spectra of old stellar populations. (4) The I-band flux of a stellar population is predicted to be nearly independent of metallicity and only modestly sensitive to age. The I band is therefore recommended for standard candle work or studies of M/L in galaxies. Other conclusions stem from this work. (1) Intercomparison of models and observations of two TiO indices seem to indicate variation of the (V/Ti) ratio among galaxies, but it is not clear how this observation ties into the standard picture of chemical enrichment. (2) Current estimates of (Fe/H) for the most metal-rich globulars that are based on integrated indices are probably slightly too high. (3) Colors of population models from different authors exhibit a substantial range. At solar metallicity and 13 Gyr, this range corresponds to an age error of roughly +/- 7 Gyr. Model colors from different authors applied in a differential sense have smaller uncertainties. (4) In the present models the dominant error for colors is probably the transformation from stellar atmospheric parameters to stellar colors. (5) Stellar B - V is difficult to model, and current spreads among different authors can reach 0.2 mag. (6) If known defects in the stellar flux library are corrected, the population model colors of this work in passbands redder than U would be accurate to roughly 0.03 mag in an absolute sense. These corrections are not made in the tables of model output.

Worthey, Guy↗

NASA NTRS1993

Water-vapor absorption line measurements in the 940-nm band by using a Raman-shifted dye laser

We report water-vapor absorption line measurements that are made by using the first Stokes radiation (930-982 nm) with HWHM 0.015/cm generated by a narrow-linewidth, tunable dye laser. Forty-five absorption line strengths are measured with an uncertainty of 6 percent and among them are fourteen strong lines that are compared with previous measurements for the assessment of spectral purity of the light source. Thirty air-broadened linewidths are measured with 8 percent uncertainty at ambient atmospheric pressure with an average of 0.101/cm. The lines are selected for the purpose of temperature-sensitive or temperature-insensitive lidar measurements. Results for these line strengths and linewidths are corrected for broadband radiation and finite laser linewidth broadening effects and compared with the high-resolution transmission molecular absorption.

Chu, Zhiping↗

NASA NTRS2001

Comparison of Shortwave Cloud Radiative Forcing Derived from ARM SGP Surface and GOES-8 Satellite Measurements During ARESE I and ARESE II

One of the objectives of the ARM Enhanced Shortwave Experiment (ARESE) is to investigate the absorption of solar radiation by clouds over the ARM Southern Great Plains central facility. A variety of techniques employing various combinations Of Surface, aircraft, and satellite data have been used to estimate the absorption empirically. During ARESE-I conducted during fall 1995, conflicting results were produced from different analyses of the combined datasets leading to the need for a more controlled experiment. ARESE-II was conducted during spring 2000. Improved calibrations, different sampling strategies, and broadband satellite data were all available to minimize some of the sources of uncertainty in the data. In this paper, cloud absorption or its parametric surrogates (e.g., Cess et al. 1995) are derived from collocated and coincident surface and satellite radiometer data from both ARESE-I and ARESE-II using the latest satellite and surface instrument calibrations.

Rapp, A. D.↗