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DOE OSTI2026

The impact of aerosol mixing state on immersion freezing: insights from classical nucleation theory and particle-resolved simulations

Immersion freezing, initiated by ice-nucleating particles (INPs) in supercooled aqueous droplets, plays an important role in the formation of ice crystals within clouds. The efficiency of immersion freezing depends strongly on INP composition and, crucially, on the mixing state – how chemical species are distributed across the particle population. Here, we quantify the impact of aerosol mixing state on immersion freezing using a combined theoretical and particle-resolved modeling approach. We derive analytical expressions for the frozen fraction of internally and externally mixed INP populations based on classical nucleation theory, showing that the frozen fraction is sensitive to whether ice-active species are present in all particles or only in a subset of the population. We introduce a multi-species immersion freezing scheme into the particle-resolved model PartMC, using the water activity-based immersion freezing model (ABIFM) to compute freezing probabilities for mixed-composition particles. To improve computational efficiency, we implement a Binned Tau-Leaping algorithm and demonstrate an order-of-magnitude speedup with minimal accuracy loss. Simulations reproduce the analytical trends in limiting cases and extend the analysis to more general aerosol populations, where mixing state continues to exert a substantial control on frozen fraction. Sensitivity analyses across particle size, species type, and cooling condition reveal that the mixing state effect is most pronounced when small amounts of highly efficient INPs are mixed with less efficient materials. These findings underscore the need to represent aerosol mixing state explicitly in models of heterogeneous ice nucleation to reduce uncertainty in cloud-phase partitioning.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2015

The Formation of N- and O-Heterocycles from the Irradiation of Benzene and Naphthalene in H2O- and NH3-Containing Ices

Polycyclic aromatic hydrocarbons (PAHs) are ubiquitous in many astrophysical environments, and are likely present in interstellar clouds and protostellar disks [1]. In dense molecular clouds,PAHs and other gas-phase species are expected tocondense onto grains to form mixed molecular ice mantles dominated by small molecules like H2O, CH3OH, NH3, CO, and CO2 [2]. These icy mantleslikely undergo energetic processing from ionizing radiation in the form of cosmic rays and high-energy photons.

Materese, C. K.↗

NASA NTRS2024

Lightning and Radar Measures of Mixed Phase Updraft Variability in Tracked Storms During the TRACER Field Campaign in Houston, Texas

Properties of 7488 thunderstorms are summarized for June-September 2022 during the TRACER field campaign Houston, Texas using polarimetric weather radar and VHF 3D lightning mapping array data. Automated tracking of storms linked each instrument’s measurements to a data-defined, time-evolving storm footprint. Within each storm, the depth and magnitude of episodic columns of radar differential reflectivity and specific differential phase quantified the prevalence of updrafts that activated mixed-phase precipitation pathways. Lightning measurements further distinguished the degree of rimed precipitation formation: the fraction of tracks with lightning varied from day to day, and cells with lightning had stronger polarimetric columns. Track-level correlation of lightning flash rate with radar polarimetric measures had substantial spread, showing that lightning provides an additional signal of mixed-phase precipitation processes that can complement future studies of thermodynamic and aerosol controls on cloud microphysics in the Houston region.

TRACER field campaign↗

NASA NTRS2001

The Green Ocean Over the Amazon: Implications for Cloud Electrification

A convective regime with distinct maritime characteristics (weak updraft, low CCN, prevalent coalescence and rainout, weak mixed phase reflectivity, low glaciation temperature, and little if any lightning) is documented over the Amazon basin of the South American continent, and dubbed the "green ocean". Radar, lightning, thermodynamic and AVHRR satellite observations are examined to shed light on the roles of updraft and aerosol in providing departures from the green ocean regime toward continental behavior. Extreme case studies are identified in which the updraft control is dominant and in which the aerosol control is dominant. The tentative conclusion gives importance to both updrafts and aerosol in shaping the electrification of tropical convection.

Williams, E.↗

NASA NTRS1984

The mesoscale stability of entrainment into cloud-topped mixed layers

The Lilly-type models for stratocumulus-capped mixed layers are shown to allow for a mesoscale instability in which mesoscale fluctuations of buoyancy and humidity are reinforced in phase by entrainment. In a model of an AMTEX mixed layer, this mesoscale instability has a maximum growth rate of about 0.00002 per sec at wavelengths 30 times the depth of the mixed layer. The instability is able to account for the existence and broad scale of the stratiform cloud patterns known as mesoscale cellular convection.

Fiedler, B. H.↗

NASA NTRS2011

Cloud Condensation in Titan's Lower Stratosphere

A 1-D condensation model is developed for the purpose of reproducing ice clouds in Titan's lower stratosphere observed by the Composite Infrared Spectrometer (CIRS) onboard Cassini. Hydrogen cyanide (HCN), cyanoacetylene (HC3N), and ethane (C2H6) vapors are treated as chemically inert gas species that flow from an upper boundary at 500 km to a condensation sink near Titan's tropopause (-45 km). Gas vertical profiles are determined from eddy mixing and a downward flux at the upper boundary. The condensation sink is based upon diffusive growth of the cloud particles and is proportional to the degree of supersaturation in the cloud formation regIOn. Observations of the vapor phase abundances above the condensation levels and the locations and properties of the ice clouds provide constraints on the free parameters in the model. Vapor phase abundances are determined from CIRS mid-IR observations, whereas cloud particle sizes, altitudes, and latitudinal distributions are derived from analyses of CIRS far-IR observations of Titan. Specific cloud constraints include: I) mean particle radii of2-3 J.lm inferred from the V6 506 cm- band of HC3N, 2) latitudinal abundance distributions of condensed nitriles, inferred from a composite emission feature that peaks at 160/cm , and 3) a possible hydrocarbon cloud layer at high latitudes, located near an altitude of 60 km, which peaks between 60 and 80 cm l . Nitrile abundances appear to diminish substantially at high northern latitudes over the time period 2005 to 2010 (northern mid winter to early spring). Use of multiple gas species provides a consistency check on the eddy mixing coefficient profile. The flux at the upper boundary is the net column chemical production from the upper atmosphere and provides a constraint on chemical pathways leading to the production of these compounds. Comparison of the differing lifetimes, vapor phase transport, vapor phase loss rate, and particle sedimentation, sheds light on temporal stability of the clouds.

Romani, Paul N.↗

NASA NTRS2008

Forecasting Lightning Threat using Cloud-Resolving Model Simulations

Two new approaches are proposed and developed for making time and space dependent, quantitative short-term forecasts of lightning threat, and a blend of these approaches is devised that capitalizes on the strengths of each. The new methods are distinctive in that they are based entirely on the ice-phase hydrometeor fields generated by regional cloud-resolving numerical simulations, such as those produced by the WRF model. These methods are justified by established observational evidence linking aspects of the precipitating ice hydrometeor fields to total flash rates. The methods are straightforward and easy to implement, and offer an effective near-term alternative to the incorporation of complex and costly cloud electrification schemes into numerical models. One method is based on upward fluxes of precipitating ice hydrometeors in the mixed phase region at the-15 C level, while the second method is based on the vertically integrated amounts of ice hydrometeors in each model grid column. Each method can be calibrated by comparing domain-wide statistics of the peak values of simulated flash rate proxy fields against domain-wide peak total lightning flash rate density data from observations. Tests show that the first method is able to capture much of the temporal variability of the lightning threat, while the second method does a better job of depicting the areal coverage of the threat. Our blended solution is designed to retain most of the temporal sensitivity of the first method, while adding the improved spatial coverage of the second. Exploratory tests for selected North Alabama cases show that, because WRF can distinguish the general character of most convective events, our methods show promise as a means of generating quantitatively realistic fields of lightning threat. However, because the models tend to have more difficulty in predicting the instantaneous placement of storms, forecasts of the detailed location of the lightning threat based on single simulations can be in error. Although these model shortcomings presently limit the precision of lightning threat forecasts from individual runs of current generation models,the techniques proposed herein should continue to be applicable as newer and more accurate physically-based model versions, physical parameterizations, initialization techniques and ensembles of forecasts become available.

McCaul, Eugene W., Jr.↗

NASA NTRS2018

Total Temperature Measurements Using a Rearward Facing Probe in Supercooled Liquid Droplet and Ice Crystal Clouds

Engine Icing Performance loss: rollback, surge, flameout, and even internal engine damagePartial melting and refreeze of ice inside engine core (Mason et al., 2006). Ingestion of ice crystals and aggregates, mixed-phase droplets, or supercooled liquid dropletsNeed to better understand the conditions and properties that lead to engine icing.Simulation and analysis (physical and computational, and modeling)Test facilities (PSL, NRC, ...). Thermal and computational models and analysisProbesMultiple probes (aerothermal probes and ice cloud characterization probes and techniques). Total temperatureTraditional total temperature probes (vented forward facing)Heated total temperature probes (Goodyear). Rearward facing (developmental). Total temperature relevance. Thermal interaction between the icing cloud and air flow impinging particles contribute to kinetic heating effect (Gent et al., 2000). Measurement considerations Temperature sensor accuracy. Incomplete recovery of total temperature. Thermal surfaces (sources and sinks). Flow effects (viscous losses). Debris contamination, including icing and ice ingestion.

Agui, Juan H.↗

NASA NTRS1984

Lidar observations of mixed layer dynamics - Tests of parameterized entrainment models of mixed layer growth rate

Ground based lidar measurements of the atmospheric mixed layer depth, the entrainment zone depth and the wind speed and wind direction were used to test various parameterized entrainment models of mixed layer growth rate. Six case studies under clear air convective conditions over flat terrain in central Illinois are presented. It is shown that surface heating alone accounts for a major portion of the rise of the mixed layer on all days. A new set of entrainment model constants was determined which optimized height predictions for the dataset. Under convective conditions, the shape of the mixed layer height prediction curves closely resembled the observed shapes. Under conditions when significant wind shear was present, the shape of the height prediction curve departed from the data suggesting deficiencies in the parameterization of shear production. Development of small cumulus clouds on top of the layer is shown to affect mixed layer depths in the afternoon growth phase.

Boers, R.↗

NASA NTRS2018

An Investigation of Glaciated Cloud Capabilities in the NASA Glenn Icing Research Tunnel

In 2015 the FAA added Appendix D to Part 33 engine certification requirements that included Mixed Phase and Ice Crystal Icing to aircraft engine certification. Replicating the ice crystal environment that is seen in nature has proven to be a challenge, which multiple engine ground testing facilities and icing wind tunnels have achieved to varying degrees. The Icing Research Tunnel (IRT) at NASA Glenn has always been focused on super-cooled liquid water to produce FAA Part 23 and Part 25 regulations, targeting Appendix C and lately also Appendix O. However, due to a growing interest in the field of ice crystals and the high cost of operating engine icing facilities, the IRT staff have recently completed testing using the Multi-Element Sensor (also known as the multi-wire) to measure glaciated cloud conditions. Results indicate that turning off the heat to the nozzle air and water supply can create a stable, fully glaciated cloud in the test section for a small range of conditions: drop-size distribution values below 20 microns (median volumetric diameter), air temperatures as warm as -7 deg C, and airspeeds between 100 and 250 knots. These tests also revealed how varying the total temperature, airspeed, nozzle air pressure, and nozzle water pressure affect the glaciation of the IRT cloud.

ice water content↗

NASA NTRS1995

Condensed Water in Tropical Cyclone "Oliver", 8 February 1993

On February 8, 1993, the NASA DC-8 aircraft profiled from 10,000 to 37,000 feet (3.1-11.3 km) pressure altitude in a stratified section of tropical cyclone "Oliver" over the Coral Sea northeast of Australia. Size, shape and phase of cloud and precipitation particles were measured with a 2-D Greyscale probe. Cloud/precipitation particles changed from liquid to ice as soon as the freezing level was reached near 17,000 feet (5.2 km) pressure altitude. The cloud was completely glaciated at -5 C. There was no correlation between ice particle habit and ambient temperature. In the liquid phase, the precipitation-cloud drop concentration was 4.0 x 10(exp 3)/cu m, the geometric mean diameter D(sub g) = 0.5-0.7 mm, and the liquid water content 0.7-1.9 g m(exp-3). The largest particles anywhere in the cloud, dominated by fused dendrites at concentrations similar to that of raindrops (2.5 x 10(exp 3) m(exp -3)) but a higher condensed water content(5.4 g/cu m estimated) were found in the mixed phase; condensed water is removed very effectively from the mixed layer due to high settling velocities of the large mixed particles. The highest number concentration (4.9 x 10(exp 4)/cu m, smallest size (D(sub g) = 0.3-0.4 mm), largest surface area (up to 2.6 x 10 (exp 2) sq cm/cu m at 0.4- 1.0 g/cu m of condensate) existed in the ice phase at the coldest temperature (- 40 C) at 35,000 feet ( 10.7 km). Each cloud contained aerosol (haze particles) in addition to cloud particles. The aerosol total surface area exceeded that of the cirrus particles at the coldest temperature. Thus, aerosols must play a significant role in the upscattering of solar radiation. Light extinction (6.2/km) and backscatter (0.8/sr/km) was highest in the coldest portion of the cirrus cloud at the highest altitude.

Pueschel, R. F.↗

NASA NTRS1991

Cloud albedo control by cloud-top entrainment

Marine stratus and stratocumulus clouds exert a considerable influence on the earth's heat budget, mainly due to their high albedos relative to the ocean surface. It is therefore important to understand the processes that control the radiative properties of these extensive cloud systems, particularly during daylight hours. Aircraft measurements of a stratocumulus cloud deck taken around local noon during the 1987 field phase of the First International Satellite Cloud Climatology Project Regional Experiment are the topic of this paper. A mixing line analysis of data from a series of flight tracks across a strong gradient in cloud albedo provides evidence that variations in the water vapor content of the air above the marine inversion can be responsible for the albedo change. The implications of this unexpected result for climate modeling are discussed.

Hanson, Howard P.↗

NASA NTRS2006

Instrument for Aircraft-Icing and Cloud-Physics Measurements

The figure shows a compact, rugged, simple sensor head that is part of an instrumentation system for making measurements to characterize the severity of aircraft-icing conditions and/or to perform research on cloud physics. The quantities that are calculated from measurement data acquired by this system and that are used to quantify the severity of icing conditions include sizes of cloud water drops, cloud liquid water content (LWC), cloud ice water content (IWC), and cloud total water content (TWC). The sensor head is mounted on the outside of an aircraft, positioned and oriented to intercept the ambient airflow. The sensor head consists of an open housing that is heated in a controlled manner to keep it free of ice and that contains four hot-wire elements. The hot-wire sensing elements have different shapes and sizes and, therefore, exhibit different measurement efficiencies with respect to droplet size and water phase (liquid, frozen, or mixed). Three of the hot-wire sensing elements are oriented across the airflow so as to intercept incoming cloud water. For each of these elements, the LWC or TWC affects the power required to maintain a constant temperature in the presence of cloud water.

Lilie, Lyle↗

NASA NTRS2003

Sensitivity of Precipitation Processes to Microphysics and Resolution in a Cloud-Resolving Model

The Goddard Cumulus Ensemble (GCE) model is used to examine the impact of various microphysical schemes, and vertical and horizontal resolution on the development, intensity and rainfall associated with mesoscale convective systems, idealized hurricanes and an ensemble of clouds. The model variables include horizontal and vertical velocities, potential temperature, perturbation pressure, turbulent kinetic energy, and mixing ratios of all water phases (vapor, liquid, and ice). The major characteristics of the GCE model are the explicit representation of warm rain and ice microphysical processes, and their complex interactions with solar and infrared radiative transfer processes, and with surface processes. For idealized hurricane, an axisymmetric version of the GCE model was developed and used successfully to simulate the tropical cyclogenesis process using both a Rankin vortex and saturated air within a specified radius as initial conditions. For mesoscale convective systems, the 3-D version of the GCE model was used to simulate squall lines that developed in the western Pacific, eastern Atlantic and central US. For the cloud ensemble, the GCE model was integrated for several days in order to have good sampling of cloud statistics. In this paper, the sensitivities of hurricane intensity to various microphysical processes and model grid resolution will be examined.

Tao, Wei-Kuo↗

NASA NTRS2003

Sensitivity of Precipitation Processes of Microphysics and Resolution in a Cloud-Resolving Model

The Goddard Cumulus Ensemble (GCE) model is used to examine the impact of various microphysical schemes, and vertical and horizontal resolution ion the development, intensity and rainfall associated with mesoscale convective systems, idealized hurricanes and an ensemble f clouds. The model variables include horizontal and vertical velocities, potential temperatures, perturbation pressure, turbulent kinetic energy, and mixing ratios of all water phases (vapor, liquid, and ice). The major characteristics of the GCE model are the explicit representation of warm rain and ice microphysical processes, and their complex interactions with solar and infrared radiative transfer processes, and with surface processes. For idealized hurricane, an axisymmetric version of the GCE model was developed and used successfully to simulate the tropical cyclogenesis process using both a Rankin vortex and saturated air within a specified radius as initial conditions. For mesoscale convective systems, the 3-D version of the GCE model was used to simulated squall lines that developed in the western Pacific, eastern Atlantic and central US. For the cloud ensemble, the GCE model was integrated for several days in order to have good sampling of cloud statistics. In this paper, the sensitivities of hurricane intensity to various microphysical processes and model grid resolution will be examined. This will be mainly achieved by performing sensitivity tests using various horizontal (from 1- to 5-km) and vertical resolutions (from 20- to 200-m in the lower troposphere to 200- to 500-m in the middle and upper troposphere). Sensitivity tests using various microphysical schemes (warm rain only, and three ice with either graupel or hail) will also be performed. The thermodynamic and water budget associated with various types of precipitation systems will also be evaluated. The budgets will be calculated for different regions (i.e., convective and stratiform regions).

Tao, Wei-Kuo↗

NASA NTRS2003

Sensitivity of Precipitation Processes to Microphysics and Resolution in a Cloud-resolving Model

Tao, Wei-Kuo↗

NASA NTRS2003

Sensitivity of Precipitation Processes to Microphysics and Resolution in a Cloud Resolving Model

The Goddard Cumulus Ensemble (GCE) model examines the impact of various microphysical schemes, and vertical and horizontal resolution in the development, intensity and rainfall associated with mesoscale convective systems, idealized hurricanes and an ensemble of clouds. The model variables include horizontal and vertical velocities, potential temperature, perturbation pressure, turbulent kinetic energy, and mixing rations of all water phases (vapor, liquid and ice). The major characteristics of the GCE model are the explicit representation of warm rain and ice microphysical processes, and their complex interactions with solar and infrared radiative transfer processes and with surface processes. For idealized hurricanes, an axisymmetric version of the GCE model was developed and used to simulate the tropical cyclogenesis process using both a Rankin vortex and saturated air within a specified radius as initial conditions. For mesoscale convective systems, the 3-D version of the GCE model was use to simulate squall lines that developed in the western Pacific, South China Sea, eastern Atlantic, South America and central U.S. FOr the cloud ensemble, the GCE model was integrated for several days in order to have a good sampling of cloud statistics. In this paper, the sensitivities of hurricane intensity to various microphysical processes and model grid resolutio will be examined. This will be mainly achieved by performing sensitivity tests using various horizontal (from 1-to 5-km) and vertical resolutions (from 20- to 200-m in the lower troposphere to 200- to 500m in the middle and upper troposphere). Sensitivity test using various microphysical schemes (warm rain only, and three ice with either graupel or hail) will also be performed. The thermodynamic and water budget associated with various types of precipitation systems will also be evaluated. The budgets will be calculated for different regions (i.e., convective and stratiform regions).

Tao, Wei-Kuo↗

NASA NTRS2003

Sensitivity of Precipitation Processes to Microphysics and Resolution in a Cloud-Resolving Model

The Goddard Cumulus Ensemble (GCE) model is used to examine the impact of various microphysical schemes, and vertical and horizontal resolution on the development, intensity and rainfall associated with mesoscale convective systems, idealized hurricanes and an ensemble of clouds. The model variables include horizontal and vertical velocities, potential temperature, perturbation pressure, turbulent kinetic energy, and mixing ratios of all water phases (vapor, liquid, and ice). The major characteristics of the GCE model are the explicit representation of warm rain and ice microphysical processes, and their complex interactions with solar and infrared radiative transfer processes, and with surface processes. For idealized hurricane, an axisymmetric version of the GCE model was developed and used successfully to simulate the tropical cyclogenesis process using both a Rankin vortex and saturated air within a specified radius as initial conditions. For mesoscale convective systems, the 3-D version of the GCE model was used to simulate squall lines that developed in the western Pacific, South China Sea, eastern Atlantic, South America and central U.S. For the cloud ensemble, the GCE model was integrated for several days in order to have good sampling of cloud statistics. In this paper, the sensitivities of hurricane intensity to various microphysical processes and model grid resolution will be examined. This will be mainly achieved by performing sensitivity tests using various horizontal (from 1- to 5-kilometers) and vertical resolutions (from 20- to 200-meters in the lower troposphere to 200- to 500-m in the middle and upper troposphere). Sensitivity tests using various microphysical schemes (warm rain only, and three ice with either graupel or hail) will also be performed. The PBL and diurnal variation of precipitation processes will also be evaluated. The budgets will be calculated for different regions (i.e., convective and stratiform regions).

Tao, Wei-Kao↗