SEARCH · Search NASA

Results for “net radiation”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

SourceResearch connectionFrom yearThrough year

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 163 records · Page 9

All sources NASA NTRS DOE OSTI

DOE OSTI2025

East Antarctic Ice Sheet variability in the central Transantarctic Mountains since the mid Miocene

The response of the East Antarctic Ice Sheet to warmer-than-present climate conditions has direct implications for projections of future sea level, ocean circulation, and global radiative forcing. Nonetheless, it remains uncertain whether the ice sheet is likely to undergo net loss due to amplified melting coupled with dynamic instabilities or whether such losses will be balanced, or even offset, by enhanced accumulation under a higher-precipitation regime. The glacial depositional record from the central Transantarctic Mountains (TAM) provides a robust geologic means to reconstruct the past behaviour of the East Antarctic Ice Sheet, including during periods thought to have been warmer than today, such as the mid-Pliocene Warm Period (~3.3–3.0 Ma). This study describes a new surface-exposure-dated moraine record from Otway Massif in the central TAM spanning the last ~9 Myr and synthesises these data in the context of previously published moraine chronologies constrained with cosmogenic nuclides. The resulting record, although fragmentary, represents the majority of direct and unambiguous terrestrial evidence for the existence and size of the East Antarctic Ice Sheet during the last 14 Myr, and it thus provides new insight into the long-term relationship between the ice sheet and global climate. At face value, the existing TAM moraine record does not exhibit a clear signature of the mid-Pliocene Warm Period, thus precluding a definitive verdict on the East Antarctic Ice Sheet's response to this event. In contrast, an apparent hiatus in moraine deposition both at Otway Massif and the neighbouring Roberts Massif suggests that the ice sheet surface in the central TAM was potentially lower than present during the late Miocene and earliest Pliocene.

58 GEOSCIENCES↗

DOE OSTI2023

Particle Size Distribution and Its Impacts on Ash Deposition and Radiative Transfer during Oxy-Combustion of Rice Husk–Natural Gas

Rice husk (RH) co-combustion with natural gas in highly oxygen-enriched concentrations presents a net carbon-negative energy production opportunity while minimizing flue gas recycling. However, recent experiments have shown enhanced ash deposition rates in oxygen-enriched conditions, with deposition/shedding also being dependent on the particle size distribution (PSD) of the parent RH fuel. To uncover the causative mechanisms behind these observations, add-on models for ash deposition/shedding and radiative properties were employed in computational fluid dynamics simulations. The combustion scenarios investigated encompassed two types of RH (US RH, Chinese RH) with widely varying ash contents (by % mass) and inlet fuel PSD with air and O2/CO2 (70/30 vol %, OXY70) as oxidizers. Utilizing the measured fly-ash PSDs near the deposit surface and modeling the particle viscosity accurately, particle kinetic-energy (PKE)-based capture and shedding criteria were identified as the keys to accurate deposition/shedding rate predictions. The OXY70 scenarios showed higher ash-capturing propensities due to their lower PKE. Conversely, higher erosion rates were predicted in the AIR firing scenarios. In addition, the radiative characteristics across all the scenarios were dominated by the gases and were not sensitive to the fly-ash PSD. Therefore, the higher particle concentrations in the OXY70 conditions did not negatively impact the heat extraction.

Krishnamoorthy, Gautham (ORCID:0000000255205092)↗

DOE OSTI2022

Relative importance of high-latitude local and long-range-transported dust for Arctic ice-nucleating particles and impacts on Arctic mixed-phase clouds

Dust particles, serving as ice-nucleating particles (INPs), may impact the Arctic surface energy budget and regional climate by modulating the mixed-phase cloud properties and lifetime. In addition to long-range transport from low-latitude deserts, dust particles in the Arctic can originate from local sources. However, the importance of high-latitude dust (HLD) as a source of Arctic INPs (compared to low-latitude dust, LLD) and its effects on Arctic mixed-phase clouds are overlooked. In this study, we evaluate the contribution to Arctic dust loading and INP population from HLD and six LLD source regions by implementing a source-tagging technique for dust aerosols in version 1 of the US Department of Energy's Energy Exascale Earth System Model (E3SMv1). Our results show that HLD is responsible for 30.7 % of the total dust burden in the Arctic, whereas LLD from Asia and North Africa contributes 44.2 % and 24.2 %, respectively. Due to its limited vertical transport as a result of stable boundary layers, HLD contributes more in the lower troposphere, especially in boreal summer and autumn when the HLD emissions are stronger. LLD from North Africa and East Asia dominates the dust loading in the upper troposphere with peak contributions in boreal spring and winter. The modeled INP concentrations show better agreement with both ground and aircraft INP measurements in the Arctic when including HLD INPs. The HLD INPs are found to induce a net cooling effect (-0.24 W m -2 above 60 °N) on the Arctic surface downwelling radiative flux by changing the cloud phase of the Arctic mixed-phase clouds. The magnitude of this cooling is larger than that induced by North African and East Asian dust (0.08 and -0.06 W m -2 , respectively), mainly due to different seasonalities of HLD and LLD. Uncertainties of this study are discussed, which highlights the importance of further constraining the HLD emissions.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

Predicting Radiation-Induced Plutonium Redox Chemistry using Multi-scale Modeling Methods

Over the the last 70 years plutonium (Pu) has been integral in the development of several technologies that have changed the world, yet our fundamental understanding of its chemistry is still far from complete. This is a testament to this element’s unique and complex properties, such as its ability to coexist as multiple oxidation states in aqueous solution. Careful manipulation of plutonium oxidation states is essential in the study and utilization of its rich chemistry. To achieve this level of control, a comprehensive mechanistic understanding of radiation-induced plutonium redox chemistry is critical due to the unavoidable exposure of plutonium to ionizing radiation fields, both inherent and from in-process applications. For this reason, we have developed an experimentally evaluated multi-scale computer model for the prediction of gamma radiation-induced Pu(IV) redox chemistry in concentrated nitric acid solutions (1.0, 3.0, and 6.0 M). Under these acidic, aqueous solution conditions, cobalt-60 gamma irradiation afforded negligible net change in the steady-state oxidation state distribution of Pu(IV). Multi-scale calculations, which are in excellent agreement with experimental data, indicate that this observation is due to radiation-induced redox cycling between Pu(IV) and Pu(III), as achieved by the reduction of Pu(IV) by radiolytic nitrous acid and hydrogen peroxide, and the oxidation of Pu(III) by nitrate and hydroxyl radicals. These radiation-induced redox processes are augmented by plutonium’s inherent disproportionation reactions.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

DOE OSTI2022

Accomplishments of Thermal Neutron Scattering Research at North Carolina State University [Slides]

Thermal neutron scattering law (TSL) data evaluations have been completed and contributed to ENDF. New evaluations are underway. FLASSH is developing as a modern platform for thermal neutron data analysis featuring an enhanced user experience and low learning overhead. Advanced TSL techniques in combination with Doppler analysis have been developed, which were incorporated into FLASSH. ML/DL NeTS method development has been initiated. Experimental capabilities for validation have been developed at the PULSTAR reactor.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2024

BTRIC Technical Support for Appalachia: FY 2024 Summary Report on Net Negative Carbon Building Demonstration with AgPod

This report investigates the effects of various concentrations of CO 2 on the photosynthesis and biomass accumulation of crops growing in an AgPod, using kale as the test crop. In the first year of the study, increasing the CO 2 concentration in the AgPod was found to promote higher photosynthetic rates in kale plants up to 1,300 ppm (the highest CO 2 concentration measured). An interesting finding was that net photosynthetic rates of kale leaves remain unsaturated until reaching unusually high levels of photosynthetically active radiation (PAR, > 1,200 µmol m -1 s -1 ) and CO 2 concentration (> 1,100 ppm). Such high levels of saturating PAR and CO 2 concentration values rarely occur under natural conditions, suggesting a promising potential for carbon capture via enriched controlled environment agriculture (ECEA). During the second year of the study, a second crop was planted to confirm the actual effects on growth with increased CO 2 concentrations. Our results suggest that growing kale plants in the AgPod system at higher CO 2 levels resulted in a successful and highly productive crop, up to three times the amount grown at 415 CO 2 . Further, the kale plants grown under higher CO 2 conditions (1000 ppm) are not CO 2 saturated and can potentially further improve yield at even higher CO 2 environments.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

DOE OSTI2023

Progress on Pu-238 Production at Idaho National Laboratory From February 2022 to December 2022

Idaho National Laboratory (INL) has continued to qualify irradiation positions in the Advanced Test Reactor (ATR) for Pu-238 production to support NASA deep space missions. Over the past year, INL qualified Np-237 targets for ATR’s North East Flux Trap (NEFT), inner A, and H positions. Work has begun to requalify the South Flux Trap (SFT) and qualify the East Flux Trap (EFT) for the ATR GEN I target and is midway through the qualification process. This paper gives an overview of operational and technical activities from February 2022 to December 2022.

07 ISOTOPE AND RADIATION SOURCES↗

DOE OSTI2020

Effect of Confinement of SIA Cluster Diffusion by Impurities on Radiation Defect Accumulation due to 14MeV neutrons in Tungsten

Impurities acting as traps, reduce the self-interstitial atom (SIA) cluster mobility, thereby increasing recombination and in turn enhancing radiation-resistance of polycrystalline materials. However, at elevated temperatures, depending on SIA-trap (impurity) binding energy, SIA clusters may trap and detrap (detach) numerous times. In tungsten, SIA clusters of all sizes glide one-dimensionally (1D) along their Burgers vector direction. Hence, detrapped SIAs would retrace their path, confining their 1D-glide between traps. However, small SIA clusters can change the direction of their 1D-glide by overcoming a rotation barrier. In addition, impurities or solutes are known to reduce this barrier. A lower rotation barrier can result in detrapped SIA clusters that diffuse in a random 1D direction, effectively leading to 3D (net-3D) diffusion. Here we investigate the effect of two cases of SIA diffusion, namely confined-1D diffusion and net-3D diffusion, on the damage accumulation in polycrystalline tungsten under 14 MeV neutron irradiation using the object kinetic Monte Carlo method. Simulations were performed using cascade debris obtained from molecular dynamics simulations with primary knock-on atom (PKA) energies corresponding to 14 MeV neutrons. In the simulations with net-3D diffusion, SIA clusters of all sizes diffuse in a random 1D direction after the clusters detrap. While for the confined 1D diffusion case, SIA clusters larger than size 5 retain their original direction of 1D-glide. In both types of simulations, trapped vacancies are assumed to be permanently immobilized. Unexpectedly, the damage accumulation was lower with confined 1D diffusion than that with net-3D. We present a systematic comparison of the influence of the two cases of SIA diffusion on the radiation damage accumulation as a function of dose rate, detrapping barrier, and impurity concentration at 1025 K.

Accumulation and recovery of lattice damage, tungs↗

DOE OSTI2022

Neural Thermal Scattering (NeTS) Modules for Graphite & Beryllium [Slides]

This presentation discusses the motivations behind the project, which include facilitating compact formulation for TSL data, extending AI knowledge, and providing advanced reactor simulation framework. It also discusses how the project accounts for beryllium and graphite complexity, including atomistic, dynamical, and neural. Additionally, new material-informed neural thermal scattering (NeTS) Modules are examined. The implications, conclusions, and plan future work for the project are also discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2020

Assessing Global and Local Radiative Feedbacks Based on AGCM Simulations for 1980–2014/2017

In order to avoid contamination of unobservable and uncertain effective radiative forcing (ERF) on the diagnosis of radiative feedbacks based on short-term climate variability, we verify the Kernel-Gregory feedback calculation method using atmospheric model experiments with prescribed ERF. We show that both clear-sky radiative fluxes and all-sky radiative feedbacks have a closure between model simulations and kernel derivations. A near-zero global mean net cloud feedback is found in the simulation with prescribed ERF, which results in a more negative global net climate feedback, -2 W m -2 K -1 . Consistent with AMIP6 ensemble mean results, the lapse rate feedback is the largest contributor among all feedbacks to temperature amplification over the three poles (Arctic, Antarctic and Tibetan Plateau), followed by surface albedo feedback and Planck feedback deviation from its global mean. Except for the higher surface albedo feedback in the Antarctic, other feedbacks are almost same between the Arctic and Antarctic.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2022

The Unexpected Oceanic Peak in Energy Input to the Atmosphere and Its Consequences for Monsoon Rainfall

Abstract Monsoons have historically been understood to be caused by the low thermal inertia of land, allowing more energy from summer insolation to be transferred to the overlying atmosphere than over adjacent ocean. Here, we show that during boreal summer, the global maximum net energy input (NEI) to the atmosphere unexpectedly lies over the Indian Ocean, not over land. Observed radiative fluxes suggest that cloud‐radiative effects (CRE) almost double the NEI over ocean, shifting the NEI peak from land to ocean. Global climate model experiments with both land and interactive sea surface temperatures confirm that CRE create the oceanic NEI maximum. Interactions between CRE, NEI, circulation, and land‐sea contrast in surface heat capacity shift precipitation from Southeast to South Asia. CRE thus alter the global partitioning of precipitation between land and ocean and the spatial structure of Earth's strongest monsoon, in ways that can be understood through the NEI.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Application of Refractory High-Entropy Alloys for Higher-Reliability and Higher-Efficiency Brayton Cycles and Advanced Nuclear Reactors

An exceptional set of newly-discovered advanced superalloys known as refractory high-entropy alloys (RHEAs) can provide near-term solutions for wear, erosion, corrosion, high-temperature strength, creep, and radiation issues associated with supercritical carbon dioxide (sCO2) Brayton Cycles and advanced nuclear reactors. In particular, these superalloys can significantly extend their durability, reliability, and thermal efficiency, thereby making them more cost-competitive, safer, and reliable. For this project, it was endeavored to manufacture and test certain RHEAs, to solve technical issues impacting the Brayton Cycle and advanced nuclear reactors. This was achieved by leveraging Sandia’s patents, technical advances, and previous experience working with RHEAs. Herein, three RHEA manufacturing methods were applied: laser engineered net shaping, spark plasma sintering, and spray coating. Two promising RHEAs were selected, HfNbTaZr and MoNbTaVW. To demonstrate their performance, erosion, structural, radiation, and hightemperature experiments were conducted on the RHEAs, stainless steel (SS) 316 L, SS 1020, and Inconel 718 test coupons, as well as bench-top components. The experimental data is presented, analyzed, and confirms the superior performance of the HfNbTaZr and MoNbTaVW RHEAs vs. SS 316 L, SS 1020, and Inconel 718. In addition, to gain more insights for larger-scale RHEA applications, the erosion and structural capabilities for the two RHEAs were simulated and compared with the experimental data. The experimental data confirm the superior performance of the HfNbTaZr and MoNbTaVW RHEAs vs. SS and Inconel. Most importantly, the erosion and the coating material experimental data show that erosion in sCO2 Brayton Cycles can be eliminated completely if RHEAs are used. The experimental suite and validations confirm that HfNbTaZr is suitable for harsh environments that do not include nuclear radiation, while MoNbTaVW is suitable for harsh environments that include radiation.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2021

An Alternative Conceptual Model for the Spent Nuclear Fuel–Water Interaction in Deep Geologic Disposal Conditions

For the long-term safety assessment of direct disposal of spent nuclear fuel in deep geologic repositories, knowledge on the radionuclide release rate from the UO 2 matrix is essential. This work provides a conceptual model to explain the results of leaching experiments involving used nuclear fuel or simulant materials in confirmed reducing conditions. Key elements of this model are: direct effect of radiation from radiolytic species (including defects and excited states) in the solid and in the first water layers in contact with its surface; and excess H 2 may be produced due to processes occurring at the surface of the spent fuel and in confined water volumes, which may also play a role in keeping the spent fuel surface in a reduced state. The implication is that the fractional radionuclide release rate used in most long-term safety assessments (10 -7 year -1 ) is over estimated because it assumes that there is net UO 2 oxidation caused by radiolysis, in contrast with the alternative conceptual model presented here. Furthermore, conventional water radiolysis models and radiation chemical yields published in the literature are not directly applicable to a heterogeneous system such as the spent fuel–water interface. Suggestions are provided for future work to develop more reliable models for the long-term safety assessment of spent nuclear fuel disposal.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2025

Radiation GRMHD Models of Accretion onto Stellar-mass Black Holes. I. Survey of Eddington Ratios

We summarize results from a survey of radiation-dominated black hole accretion flows across a wide range of mass accretion rates, as well as two values of black hole spin and initial magnetic field geometry. These models apply an algorithm targeting direct solutions to the radiation transport equation in full general relativity and have been enabled by access to modern exascale computing systems. Super-Eddington accretion flows form geometrically thick radiation-pressure-supported disks that drive powerful equatorial outflows. A narrow funnel-shaped photosphere in the inner region results in very low radiative efficiencies in this regime. The structure of near- and sub-Eddington accretion depends on whether there is net vertical magnetic flux at the midplane of the disk. With net flux, the disk forms a thin, dense layer at the midplane surrounded by a magnetically dominated corona, whereas without net flux, the disk remains magnetically dominated everywhere. Although none of our models achieve the magnetically arrested disk regime, those with net vertical flux and a rapidly spinning black hole still produce powerful relativistic jets. Our calculations adopt simple opacity models (with scalings appropriate to stellar-mass black hole accretion). We discuss the application of our results to observations of X-ray binaries and ultraluminous X-ray sources such as Cyg X-3 and SS433. We also speculate on the application of our super-Eddington models to the interpretation of little red dots recently discovered by JWST.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2020

Reticular exploration of uranium-based metal—organic frameworks with hexacarboxylate building units

We report that the rational reticular design of metal–organic frameworks (MOFs) from building units of known geometries is essential for enriching the diversity of MOF structures. Unexpected and intriguing structures, however, can also arise from subtle changes in the rigidity/length of organic linkers and/or synthetic conditions. Herein, we report three uranium-based MOF structures—i.e., NU-135X (X = 0, 1, 2)—synthesized from trigonal planar uranyl nodes and triptycene-based hexacarboxylate ligands with variable arm lengths. A new chiral 3,6-connected nuc net was observed in NU-1350, while the extended versions of the ligand led to 3-fold catenated MOFs (NU-1351 and NU-1352) with rare 3,6-connected cml-c3 nets. Lastly, the differences in the topology of NU-1350 and NU-1351/NU-1352 could be attributed to the slight distortions of the shorter linker in the former from the ideal trigonal prism geometry to an octahedral geometry when coordinated to the trigonal planar uranyl nodes.

3,6-connected net↗

DOE OSTI2020

Leaf isoprene and monoterpene emission data-set across hyperdominant tree genera in the Amazon basin

This data package contains the analyzed data used to support the publication "Leaf isoprene and monoterpene emission distribution across hyperdominant tree genera in the Amazon basin," Phytochemistry, in-press. Data was collected from 162 trees across four sites in the Amazon. For all leaf samples studied for volatile isoprenoid emissions, branch cuttings were conducted in the upper canopy with sun exposed leaves with the assistance of a tree climber utilizing a pole pruner or directly accessed from flux towers. Large branches were removed from the upper canopy (up to 0.5-1.0 meter in length) and rapidly recut on the ground under water to maintain the transpiration stream. Net photosynthesis and isoprene and monoterpene emission rates were quantified from leaves during controlled changes in photosynthetically active radiation (PAR) using a commercial leaf photosynthesis system (LI-6400XT, LI-COR Inc., USA) interfaced with a gas chromatograph-mass spectrometer (GC-MS, 5975C series, Agilent Technologies, USA). For detailed methods and raw data, refer to the publication and related material cited in Dataset References.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

Machine learning opportunities for nucleosynthesis studies

Nuclear astrophysics is an interdisciplinary field focused on exploring the impact of nuclear physics on the evolution and explosions of stars and the cosmic creation of the elements. While researchers in astrophysics and in nuclear physics are separately using machine learning approaches to advance studies in their fields, there is currently little use of machine learning in nuclear astrophysics. We briefly describe the most common types of machine learning algorithms, and then detail their numerous possible uses to advance nuclear astrophysics, with a focus on simulation-based nucleosynthesis studies. We show that machine learning offers novel, complementary, creative approaches to address many important nucleosynthesis puzzles, with the potential to initiate a new frontier in nuclear astrophysics research.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2024

Multiscale Modeling of Plutonium Radiation Chemistry in Nitric Acid Solutions. 1. Cobalt-60 Gamma Irradiation of Pu(IV)

We report careful manipulation of the plutonium oxidation states is essential in the study and utilization of its rich redox chemistry. To achieve this level of control, a comprehensive mechanistic understanding of radiation-induced plutonium redox chemistry is critical due to the unavoidable exposure of plutonium to ionizing radiation fields, both inherent and from in-process applications. To this end, we have developed an experimentally evaluated multiscale computer model for the prediction of gamma radiation-induced Pu(IV) redox chemistry in concentrated nitric acid solutions (1.0, 3.0, and 6.0 M). Under these acidic, aqueous solution conditions, cobalt-60 gamma irradiation afforded marginal net conversion of Pu(IV) to Pu(VI), the extent of which was dependent on the concentration of HNO 3 and absorbed gamma dose. Multiscale calculations, which are in excellent agreement with experimental data, indicate that this observation is due to a combination of inherent plutonium disproportionation reactions and several radiation-induced processes, including redox cycling between Pu(IV) and Pu(III), as achieved by the reduction of Pu(IV) by nitrous acid and hydrogen peroxide, the oxidation of Pu(III) by nitrate and hydroxyl radicals, and the sequential oxidation of Pu(IV) to Pu(V) and Pu(VI) by the remaining available yield of nitrate radicals.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗