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DOE OSTI2020

Deep Learning for Intelligent Bubble Size Detection in the Spallation Neutron Source Visual Target

The Spallation Neutron Source (SNS) at Oak Ridge National Laboratory (ORNL) will undergo proton power upgrade (PPU), increasing the proton beam power from 1.4 MW to 2.8 MW. From 2.8 MW, 2.0 MW will go to the current First Target Station and the rest will go to the future Second Target Station (STS). The First Target Station uses a liquid mercury target that is contained in a 316L stainless steel vessel. The proton beam is pulsed at 60 Hz, with a pulse of about 0.7μs. When the proton beam hits the target, the intense energy deposition leads to a rapid rise in temperature in the mercury. This temperature rise creates pressure waves that propagate through the mercury and cause cavitation erosion. The power upgrade will cause stronger pressure waves that will further increase damage because of cavitation. Injecting small helium bubbles in the mercury has been an efficient method of mitigating the pressure wave at 1.4 MW. However, at higher power, additional mitigation is necessary. Therefore, the 2 MW target vessel will be equipped with swirl bubblers and an additional gas injection port near the nose to inject more gas in the target. To develop a gas injection strategy and design, flow visualization in water with a transparent prototypical target (“visual target”) was performed. Bubble sizes and their spatial distribution in the flow loop are crucial to understanding the effectiveness of the bubbles in mitigating pressure waves. Bubbles were generated in the visual target under varied conditions of input pressures with helium and air. Images were captured using a high-speed camera at varied frame rates at different positions away from the swirl bubbler and different depths in the flow loop under varying lighting conditions. Initially, methods such as circular Hough transforms were applied after a series of images processing to obtain a general distribution of bubble sizes. Bubbles smaller than 500 μm are preferred to effectively mitigate the effect of pressure waves, which demands an accurate bubble detection and sizing system. Intelligent detection and identification of bubble sizes alleviate misdetection and improves accuracies. Employing neural networks, intelligent detection of bubble sizes and their distribution was developed and provides a robust alternative to traditional techniques. Human intervention was employed to label in-focus and out-of-focus bubbles in the set of training images. An object detection network using a pretrained convolutional neural network was created that extracted the features from the training images. Data augmentation was used to improve network accuracy through a random transformation of the original data.

Rasheed, Fayaz↗

DOE OSTI2021

Fed-batch production of deuterated protein in Escherichia coli for neutron scattering experimentation

Neutron scattering is a powerful technique for determining the structure and dynamics of biological materials in a variety of environmental conditions. A distinguishing property of the neutron is its sensitivity to detecting hydrogen and distinguishing it from its isotope deuterium. This enables unique types of experiments that take advantage of this differential sensitivity called isotopic contrast variation. Using this approach, the chemistry of the system is not changed, but the visibility of individual sample components can be tuned by varying the deuterium content of the system under investigation. Deuterated proteins are commonly produced in bacterial systems that are adapted to growth in D2O minimal media. To maximize the yield of deuterium-labeled protein and efficiently utilize D2O and occasionally the deuterated substrate, fed-batch processes are routinely used to maximize biomass production without compromising cell viability. A step-by-step procedure will be described along with a case study of the production of deuterated green fluorescent protein. Limitations of the process will also be discussed.

Weiss, Kevin L.↗

DOE OSTI2021

Determining elastic anisotropy of textured polycrystals using resonant ultrasound spectroscopy

Abstract Polycrystalline materials can have complex anisotropic properties depending on their crystallographic texture and crystal structure. In this study, we use resonant ultrasound spectroscopy (RUS) to nondestructively quantify the elastic anisotropy in extruded aluminum alloy 1100-O, an inherently low-anisotropy material. Further, we show that RUS can be used to indirectly provide a description of the material’s texture, which in the present case is found to be transversely isotropic. By determining the entire elastic tensor, we can identify the level and orientation of the anisotropy originated during extrusion. The relative anisotropy of the compressive (c 11 /c 33 ) and shear (c 44 /c 66 ) elastic constants is 1.5% ± 0.5% and 5.7% ± 0.5%, respectively, where the elastic constants (five independent elastic constants for transversely isotropic) are those associated with the extrusion axis that defines the symmetry of the texture. These results indicate that the texture is expected to have transversely isotropic symmetry. This finding is confirmed by two additional approaches. First, we confirm elastic constants and the degree of elastic anisotropy by direct sound velocity measurements using ultrasonic pulse echo. Second, neutron diffraction (ND) data confirm the symmetry of the bulk texture consistent with extrusion-induced anisotropy, and polycrystal elasticity simulations using the elastic self-consistent model with input from ND textures and aluminum single-crystal elastic constants render similar levels of polycrystal elastic anisotropy to those measured by RUS. We demonstrate the ability of RUS to detect texture-induced anisotropy in inherently low-anisotropy materials. Therefore, as many other common materials have intrinsically higher elastic anisotropy, this technique should be applicable for similar levels of texture, providing an efficient general diagnostic and characterization tool.

36 MATERIALS SCIENCE↗

DOE OSTI2020

AWCC Simulations

Neutron well counters provide a means to measure fissile mass by detecting coincident neutrons, which is a unique signature to fission. For coincidence counting, mass is determined using a calibration curve established with items that have the same material characteristics. Multiplicity analysis solves the point model equations for mass using known detector parameters. In both cases, mass measurements may exhibit a bias due to item characteristics and should be corrected for. Experiments can be done to estimate bias and material effects, but they require having both the well counter and the material well defined. In pursuit of estimating measurement bias and uncertainty in a High Efficiency Neutron Counter (HENC), an MCNP simulation was matched to measurements performed with an Active Well Coincidence Counter (AWCC) to de ne a neutron source term. The neutron source term will be used to predict measurement performance of similar material types in a HENC.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2020

The CLAS12 forward electromagnetic calorimeter

The CLAS12 Forward Detector includes six independent lead-scintillator electromagnetic sampling calorimeters to provide the primary electron trigger and extend the CLAS12 detection capability to photons and neutrons. Each calorimeter package consists of two modules, the legacy Electromagnetic Calorimeter (EC) previously used in the CLAS detector, and a new pre-shower calorimeter (PCAL) located in front of the EC to extend the total detector radiation length, in order to fully absorb the electromagnetic showers induced by electrons with energies up to 12 GeV. Both calorimeters use a novel triangular hodoscope geometry with stereo readout. The PCAL uses an upgraded design to provide the high spatial resolution necessary for reconstructing π 0 and η decays, and neutrons with high efficiency. Here, this paper treats the design, construction, and calibration of the PCAL and the preliminary combined performance of both detectors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2022

On the novel 3-D neutron transport kinetic tRAPID algorithm and its validation

The Real-time Analysis for Particle-transport and In-situ Detection (RAPID) Code System, based on the Multi-stage Response-function Transport (MRT) methodology, allows for real-time simulation of nuclear systems based on 3-D continuous-energy particle transport. RAPID's steady-state (criticality) neutron transport algorithm is based on the Fission Matrix (FM) method, and has been extensively verified and validated against computational benchmarks and experiments. This paper introduces the novel 3-D time-dependent transport algorithm that has been implemented into the code, tRAPID, and its validation using the JSI TRIGA Mark-II reactor. tRAPID accurately and efficiently calculates neutron kinetics parameters (such as β{sub eff}, l{sub eff} , Λ, α{sub Rossi}) and 3-D time-dependent neutron fission source distribution and neutron importances for both prompt and delayed neutrons. tRAPID is used to simulate a rod insertion experiment performed at the JSI TRIGA Mark-II reactor, during which signals from four fission chambers at four different locations in the core were collected. The results demonstrate how tRAPID is capable of calculating detailed and accurate results with only a minimal use computational resources and time.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2021

A new generation of uranium coincidence fast neutron collars for assay of LWR fresh fuel assemblies

The active uranium neutron coincidence collar provides a means of non-destructively assaying the fissile linear density of Light Water Reactor fresh fuel assemblies containing low enriched uranium. These neutron collars can operate in two modes: a thermal and a fast mode. In fast mode, a neutron collar has an added cadmium (Cd) liner in the sample cavity of the detector to reduce the impact of the burnable poison (thermal neutron absorber) on the detector signal (doubles). The main advantage for operating in fast mode is a detected signal that is less dependent of the burnable neutron poison content and thus less dependent on facility operator declarations. The drawback is that operating in fast mode requires a longer measurement time (~hour vs tens of minutes for thermal mode) to achieve the statistically needed precision in the measurements. The trend in the modern reactor fuel assemblies is moving to higher burnup by using higher initial enrichment and, consequently, a higher number of burnable poison rods to compensate the initial neutron reactivity. The increase of the burnable poison loading has motivated the development of a new generation of high efficiency fast neutron collars to allow practical measurements in-field by nuclear inspectors. This paper describes the development and performance evaluation of a new generation of neutron collars, for both boiling water reactor (BWR) and pressurized water reactor (PWR) fuels, jointly developed between the US Department of Energy, through Los Alamos National Laboratory, and the Euratom Safeguards Directorate of the European Commission. In this work, we present here calibrations with reference fuel assemblies at Los Alamos National Laboratory as well as the results of in-field measurement campaigns in fuel fabrication plants with modern commercial fuel assemblies. The experimental results show that a typical PWR verification can be made in a total time of 30 min with an uncertainty in the measured mass of 2% at one standard deviation (1σ). A BWR verification can be made in 47 min with an uncertainty in the measured mass of 1.9% at 1σ, or a total time of 20 min with 1σ uncertainty in the measured mass of 2.5%.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2023

A Fission-like Neutron Spectrum Shaping Assembly based on D-T Generator

For nearly five decades, 252 Cf sources have been used for testing and calibration over a wide range of neutron detection devices used for nuclear safety and radiation protection. However, the vastly increased cost of 252 Cf sources, its short half-life, and concerns about future shortage have prompted nuclear facilities and radiological calibration laboratories that rely on high-intensity neutron sources to seek alternatives. While there appear to be no other radionuclide neutron sources that would match the 252 Cf performance characteristics, all of them, including 252 Cf, present similar concerns in terms of hazards, safety, and security. As a possible solution to this issue, the Pacific Northwest National Laboratory (PNNL) developed a low-risk, cost-efficient alternative to produce fission-like spectra based on commercially available deuterium-tritium (D-T) neutron generators. The alternative of producing a fission-like neutron spectrum without any fissionable materials or beryllium would enable the nuclear facilities across the entire complex to eliminate their reliance on high intensity 252 Cf sources for nuclear safety and radiation protection applications, substantially reducing risks and associated costs. This report describes efforts of designing the spectrum shaping assembly, its construction and characterization of the neutron field produced. Performance of this newly developed D-T generator based neutron field is demonstrated via calibration of a criticality detector, neutron survey instruments, and personal dosimeters verified against current standardized fields produced by 252 Cf spontaneous fission sources.

42 ENGINEERING↗

DOE OSTI2026

Astrometric microlensing probes of the isolated neutron star population with Roman

Notoriously hard to detect and study, isolated neutron stars (NSs) might provide valuable answers to fundamental questions about stellar evolution and explosion physics. With the upcoming Roman Space Telescope, scheduled for launch in 2026, a new and powerful channel for their detection will become available: astrometric microlensing. We set out to create a realistic sample of simulated gravitational microlensing events as observed by Roman with the Galactic Bulge Time Domain Survey. We focus in particular on the population of NS lenses, which has until now been largely understudied. We used dedicated Galactic models tailored for application to microlensing by compact objects. In addition to populations of stars, white dwarfs, and black holes, we simulated four different NS populations with Maxwellian natal kick distributions: v = (150, 250, 350, 450) km/s. For each simulation, we applied projected Roman precision, cadence, and detectability criteria. We found that the parameter space log10 t E –log 10 θ E , which will be accessible to Roman observations, is efficient for the classification of stellar remnants. We found a feature in this space that is characteristic of NSs; using this feature, optimal samples of NS candidates can be constructed from Roman -like datasets. We describe the dependence of the observable parameter distributions on the assumed mean kick velocities. As the effects of natal kicks are very complex and mutually counteracting, we suggest that more detailed studies focused on the dynamics of NSs are needed in anticipation of Roman and future surveys. We estimate that Roman will observe approximately 11 000 microlensing events, including ~100 with NS lenses, whose photometric and astrometric signals are detectable; the event yield decreases by 38% when gap-filling low-cadence observations are not included. We make all simulated microlensing event datasets publicly available in preparation for Roman data.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2023

Systematic Source Determination and X-Ray Radiography Detection of Nonuniformities on High-Density Carbon Ablators

Recent deuterium-tritium (D-T)–layered implosion experiments at the National Ignition Facility have achieved a burning plasma and >1-MJ neutron yield. A series of repeat experiments have shown that the degree of performance is very likely dependent on capsule quality, including the quantity of what are collectively termed “high- Z particles.” These particles are detected on a custom-built radiography system, known as the Sagometer, during the final target qualification process. The term particles is misleading, as the source of these nonuniformities in the capsule images is uncertain; the term detection will be used instead. An increased number of D-T targets have been rejected at the final stages of production due to Sagometer detections. Late detections are deleterious in terms of loss of production parts, effort, and overall operating efficiency. In response, we undertook an effort to determine the origin of these detections and to ultimately mitigate target losses caused by them. Through careful testing and analysis, we have determined neither insufficient production cleanliness nor hohlraum shedding is responsible for the detections on the capsule. Here, we determined that the detections are inherent to the capsule and have made efforts to use the Zeiss Xradia to identify them earlier in the production process. While testing revealed the Xradia is not currently sufficient for identifying such particles using radiography images, we continue to look to other forms of metrology to down select the capsules early in the process.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2020

A DESGW Search for the Electromagnetic Counterpart to the LIGO/Virgo Gravitational-wave Binary Neutron Star Merger Candidate S190510g

In this work, we present the results from a search for the electromagnetic counterpart of the LIGO/Virgo event S190510g using the Dark Energy Camera (DECam). S190510g is a binary neutron star (BNS) merger candidate of moderate significance detected at a distance of 227 ± 92 Mpc and localized within an area of 31 (1166) square degrees at 50% (90%) confidence. While this event was later classified as likely nonastrophysical in nature within 30 hours of the event, our short latency search and discovery pipeline identified 11 counterpart candidates, all of which appear consistent with supernovae following offline analysis and spectroscopy by other instruments. Later reprocessing of the images enabled the recovery of six more candidates. Additionally, we implement our candidate selection procedure on simulated kilonovae and supernovae under DECam observing conditions (e.g., seeing and exposure time) with the intent of quantifying our search efficiency and making informed decisions on observing strategy for future similar events. This is the first BNS counterpart search to employ a comprehensive simulation-based efficiency study. We find that using the current follow-up strategy, there would need to be 19 events similar to S190510g for us to have a 99% chance of detecting an optical counterpart, assuming a GW170817-like kilonova. We further conclude that optimization of observing plans, which should include preference for deeper images over multiple color information, could result in up to a factor of 1.5 reduction in the total number of follow-ups needed for discovery.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2021

Constraints on the Electromagnetic Counterpart of the Neutron-star–Black-hole Merger GW200115

We report the results of our follow-up campaign for the neutron-star—black-hole (NSBH) merger GW200115 detected during the O3 run of the Advanced LIGO and Advanced Virgo detectors. We obtained wide-field observations with the Deca-Degree Optical Transient Imager covering ~20% of the total probability area down to a limiting magnitude of w = 20.5 AB at ~23 hr after the merger. Our search for counterparts returns a single candidate (AT2020aeo), likely not associated with the merger. In total, only 25 sources of interest were identified by the community and later discarded as unrelated to the GW event. We compare our upper limits with the emission predicted by state-of-the-art kilonova simulations and disfavor high-mass ejecta (>0.1 M⊙), indicating that the spin of the system is not particularly high. By combining our optical limits with gamma-ray constraints from Swift and Fermi, we disfavor the presence of a standard short-duration burst for viewing angles ≲15° from the jet axis. Our conclusions are, however, limited by the large localization region of this GW event, and accurate prompt positions remain crucial to improving the efficiency of follow-up efforts.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2020

Warming nuclear pasta with dark matter: kinetic and annihilation heating of neutron star crusts

Neutron stars serve as excellent next-generation thermal detectors of dark matter, heated by the scattering and annihilation of dark matter accelerated to relativistic speeds in their deep gravitational wells. However, the dynamics of neutron star cores are uncertain, making it difficult at present to unequivocally compute dark matter scattering in this region. On the other hand, the physics of an outer layer of the neutron star, the crust, is more robustly understood. We show that dark matter scattering solely with the low-density crust still kinetically heats neutron stars to infrared temperatures detectable by forthcoming telescopes. We find that for both spin-independent and spin-dependent scattering on nucleons, the crust-only cross section sensitivity is 10 -43 - 10 -41 cm 2 for dark matter masses of 100 MeV - 1 PeV, with the best sensitivity arising from dark matter scattering with a crust constituent called nuclear pasta (including gnocchi, spaghetti, and lasagna phases). For dark matter masses from 10 eV to 1 MeV, the sensitivity is 10 -39 - 10 -34 cm 2 , arising from exciting collective phonon modes in a neutron superfluid in the inner crust. Furthermore, for any s-wave or p-wave annihilating dark matter, we show that dark matter will efficiently annihilate by thermalizing just with the neutron star crust, regardless of whether the dark matter ever scatters with the neutron star core. This implies efficient annihilation in neutron stars for any electroweakly interacting dark matter with inelastic mass splittings of up to 200 MeV, including Higgsinos. We conclude that neutron star crusts play a key role in dark matter scattering and annihilation in neutron stars.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2023

J/ψ Near-Threshold Photoproduction off the Proton and Neutron with CLAS12

In recent years, J/? photoproduction in the near-threshold region has seen a renewed theoretical interest due to the wealth of information it has to offer. Near-threshold J/? photopro-duction proceeds through the exchange of gluons in the t-channel and is expected to provide unique insight about the nucleon gluonic gravitational form factors (GFFs). Previous studies at the Thomas Jefferson National Accelerator Facility (JLab) in Virginia, USA, have already measured the total and differential cross section of J/? near-threshold photoproduction on the free proton. This thesis presents the first measurements of J/? near-threshold photoproduction on the bound proton and bound neutron in a deuteron target. The CEBAF Large Acceptance Spectrometer at 12 GeV (CLAS12) based at JLab?s Hall B uses a 11 GeV electron beam impinging on a fixed liquid deuteron target. J/? is then produced via the exchange of a quasi-real photon and decays to a lepton pair which is detected along-side the recoil nucleon by CLAS12. Analysis procedures and in particular machine learning based techniques were developed in order to correctly identify final state particles and select J/? photoproduction events. The total and differential cross section of J/? near-threshold photoproduction on the bound proton and bound neutron were then measured from the detected J/? photoproduction events. The measurements of the cross sections on the bound proton and bound neutron agree well within their statistical uncertainty. This is consistent with the assumed two-gluon exchange production mechanism which is isospin invariant. Overall a first measurement of the J/? near-threshold photoproduction cross sections on the bound proton and bound neutron was achieved. A better understanding of the mechanical properties of the nucleon, such as pressure and mass distributions, can be obtained by relating J/? production to the nucleon GFFs. This opens the way for exciting new insights into the internal structure of the nucleon, and in particular of the nucleon?s gluonic content. An upcoming overhaul of the CLAS12 reconstruction will increase the reconstruction efficiency and the statis- tical precision of the preliminary measurements described in this thesis, with an expected gain in statistics of at least 50%. Future upgrades at JLab will allow to test some of the theoretical assumptions made in relating J/? near-threshold photoproduction to the nucleon GFFs

Tyson, Richard↗

DOE OSTI2022

Free spectator nucleons in ultracentral relativistic heavy-ion collisions as a probe of neutron skin

Besides the yield ratio of free spectator neutrons produced in ultracentral 96 Zr + 96 Zr to 96 Ru + 96 Ru collisions, we propose that the yield ratio N n /N p of free spectator neutrons to protons in a single collision system at the BNL Relativistic Heavy Ion Collider or the CERN Large Hadron Collider can be a more sensitive probe of the neutron-skin thickness Δrnp and the slope parameter L of the symmetry energy. Here, the idea is demonstrated based on the proton and neutron density distributions of colliding nuclei obtained from Skyrme-Hartree-Fock-Bogolyubov calculations, and on a Glauber model that provides information of spectator matter. The final spectator particles are produced from direct emission, clusterization by a minimum spanning tree algorithm or a Wigner function approach, and deexcitation of heavy clusters by gemini. A larger Δr np associated with a larger L value increases the isospin asymmetry of spectator matter and thus leads to a larger N n /N p , especially in ultracentral collisions where the multiplicity of free nucleons are free from the uncertainties of cluster formation and deexcitation. We have further shown that the double ratio of N n /N p in isobaric collision systems or in collisions by isotopes helps to cancel the detecting efficiency for protons. Effects from nuclear deformation and electromagnetic excitation are studied, and they are found to be subdominant compared to the expected sensitivity to Δr np .

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2026

Python-EPICS RF Conditioning Automatic Control System at the Spallation Neutron Source

The RF Test Facility (RFTF) at the Spallation Neutron Source (SNS) is used for the conditioning of RF compo-nents such as ceramic vacuum windows and power cou-plers prior to their installation in the H- ion linear accel-erator. This process exposes components to high-power RF fields and thermal cycling to improve performance and remove surface impurities. To automate and optimize this process, a Python-based EPICS control system was developed alongside targeted hardware upgrades. The system enables real-time monitoring and control of RF power levels, temperature, and vacuum pressure. A user-friendly graphical interface was implemented using CS-Studio (Phoebus), allowing operators to adjust parameters and collect data efficiently. The system integrates a High-Power Protection Module (HPM) for interlocks based on vacuum and arc detection, ensuring safe operation. These upgrades have significantly improved the efficiency, accuracy, and safety of RF conditioning at the SNS RFTF. This paper describes the updated RF conditioning sys-tem, highlighting the software and hardware develop-ments and their application in support of the Proton Pow-er Upgrade (PPU) project.

Lee, Sung-Woo [ORNL] (ORCID:000000030915835X)↗

DOE OSTI2024

A new hybrid gadolinium nanoparticles-loaded polymeric material for neutron detection in rare event searches

Experiments aimed at direct searches for WIMP dark matter require highly effective reduction of backgrounds and control of any residual radioactive contamination. In particular, neutrons interacting with atomic nuclei represent an important class of backgrounds due to the expected similarity of a WIMP-nucleon interaction, so that such experiments often feature a dedicated neutron detector surrounding the active target volume. In the context of the development of DarkSide-20k detector at INFN Gran Sasso National Laboratory (LNGS), several R&D projects were conceived and developed for the creation of a new hybrid material rich in both hydrogen and gadolinium nuclei to be employed as an essential element of the neutron detector. Thanks to its very high cross-section for neutron capture, gadolinium is one of the most widely used elements in neutron detectors, while the hydrogen-rich material is instrumental in efficiently moderating the neutrons. In this paper results from one of the R&Ds are presented. In this effort the new hybrid material was obtained as a poly(methyl methacrylate) (PMMA) matrix, loaded with gadolinium oxide in the form of nanoparticles. We describe its realization, including all phases of design, purification, construction, characterization, and determination of mechanical properties of the new material.

Dark Matter detectors (WIMPs, axions, etc.)↗

DOE OSTI2023

6 Li-loaded liquid scintillators produced by direct dissolution of compounds in diisopropylnaphthalene (DIPN)

Here, this paper describes preparation of 6 Li-loaded liquid scintillators by methods involving direct dissolution of 6Li salts in the commercial diisopropylnaphthalene (DIPN) solvent, without the formation of water-in-oil emulsions. Methods include incorporation of 6 Li that, unlike previously reported formulations, does not require additions of water or a strong acid such as hydrochloric acid (HCl). Results of the conducted experiments show that dissolution of aromatic and aliphatic 6 Li salts in DIPN can be easily achieved at 0.1%–0.3% by weight of atomic 6 Li, using small additions of waterless surfactants, or mild carboxylic acids. An alternative way suggests incorporation of 6 Li as a part of a surfactant molecule that can be dissolved in DIPN without any solubilizing additions. Proposed methods enable preparation of efficient 6 Li-loaded liquid scintillators that, at a large scale of 50 cm, exhibit good pulse shape discrimination (PSD) properties combined with up to 107% of light output and up to 115% of the attenuation length measured relative to standard undoped EJ-309 liquid scintillator.

36 MATERIALS SCIENCE↗