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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 163 records · Page 9
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DOE OSTI2025

Enhanced Nuclear Binding near the Proton Drip Line Opens Possible Bypass of the 64 Ge Rapid Proton Capture Process Waiting Point

Abstract We performed astrophysics model calculations with updated nuclear data to identify a possible bypass of the 64 Ge waiting point, a defining feature of the rapid proton capture (rp) process that powers type I X-ray bursts on accreting neutron stars. We find that the rp-process flow through the 64 Ge bypass could be up to 36% for astrophysically relevant conditions. Our results call for new studies of 65 Se, including the nuclear mass, β -delayed proton emission branching, and nuclear structure as it pertains to the 64 As( p , γ ) reaction rate at X-ray burst temperatures.

Nuclear astrophysics↗
DOE OSTI2025

Development and validation of a software for simulating γ-γ coincidence emission and detection probabilities

Gamma-gamma coincidence spectrometers have the potential to significantly enhance detection sensitivity for ultra-trace radionuclide measurements. The implementation of these spectrometers, however, is limited by the complexity of acquisition hardware, data processing and quantification. This work reports development of a novel radionuclide quantification software for γ-γ coincidence measurements. For any radionuclide, the software parses the Evaluated Nuclear Structure Data File (ENSDF) database, recursively simulating all possible γ-γ coincidence signatures and their respective emission and detection probabilities. Implemented using Python programming language, the software employs several strategies to boost overall computational performance. Since coincidence-based spectrometers are of notable interest in monitoring compliance for the Comprehensive Nuclear-Test-Ban Treaty (CTBT), the software’s execution was tested for 84 CTBT-relevant radionuclides. To date, the software has been experimentally validated for 15 radionuclides using the Advanced Radionuclide Gamma spectrOmeter (ARGO) at Pacific Northwest National Laboratory, USA (PNNL). Notably, the software can be operated in convergence mode, whereby coincidence detection efficiency’s convergence behavior can help avoid unreliable radionuclide activity estimates. With growing number of coincidence spectrometers worldwide, this paper aims to assist the radiation metrology community in developing similar software for their system.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2026

Measurement of the Neutron Elastic Electromagnetic Form Factor Ratio at Large Momentum Transfer

Exploring nucleon structure is vital both for understanding its origin and existence as well as for the advancement of the sciences. It helps us answer key questions such as how quark and gluon dynamics create 99% of the nucleon mass. Electron- nucleon scattering has been widely used for precision studies of the nucleon and nuclear structure since the Nobel Prize winning investigations by Robert Hofstadter and collaborators in the 1950s. These studies provide information about the spatial charge and current densities of the nucleon in terms of the electromagnetic form factors. The form factors are functions of four momentum transfer squared (Q2). Extending the electromagnetic form factor measurements to higher Q2 plays a critical role in furthering the understanding of nucleon structure. This motivated the Super BigBite Spectrometer (SBS) program at Jefferson Lab. The open nature of the spectrometers and the direct line of sight from the target to the tracking detector locations in experimental setups such as SBS creates high levels of background at the detectors. This necessitates the use of tracking detectors with high rate capability and good position resolution. Gas Electron Multiplier (GEM) detectors are an excellent choice for tracking detectors in such experiments. Understanding the performance of the GEM detectors is important not just for SBS experiments but also for future high-luminosity experiments. This thesis reports the exploratory results from the measurement of the neutron elastic electromagnetic form factor ratio (Gn E/Gn M) at high momentum transfer. A longitudinally polarized electron beam was scattered off a polarized 3He target, used as an effective polarized neutron target. In this experiment, the polarized 3He target achieved a world record polarization weighted luminosity at a beam current of 45 µA. Double spin asymmetry of the scattered neutron events is used to extract the neutron form factor ratio. Measurements were taken at Q2 = 3.0, 6.8, 9.8 (GeV/c)2. The lowest Q2 measurement is in good agreement with the existing world data, and the higher-Q2 measurements extend the Q2 reach well beyond the existing world data and are expected to remain unmatched for a long time.

Gamage, Vimukthi Haththotuwa [Univ. of Virginia, C↗
DOE OSTI2024

Partial-wave projection of the one-particle exchange in three-body scattering amplitudes

As the study of three-hadron physics from lattice QCD matures, it is necessary to develop proper analysis tools in order to reliably study a variety of phenomena, including resonance spectroscopy and nuclear structure. Reconstructing the three-particle scattering amplitude requires solving integral equations, which can be written in terms of data-constrained dynamical functions and physical on shell quantities. The driving term in these equations is the so-called one-particle exchange, which leads to a kinematic divergence for particles on mass shell. A vital component in defining three-particle amplitudes with definite parity and total angular momentum, which are used in spectroscopic studies, is to project the one-particle exchange into definite partial waves. We present a general procedure to construct exact analytic partial-wave projections of the one-particle exchange contribution for any system composed of three spinless hadrons. Our result allows one full control over the analytic structure of the projection, which we explore for some low-lying partial waves with applications to three pions. Published by the American Physical Society 2024

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Diffusion model approach to simulating electron-proton scattering events

Generative artificial intelligence is a fast-growing area of research offering various avenues for exploration in high-energy nuclear physics. In this work, we explore the use of generative models for simulating electron-proton collisions relevant to experiments like the Continuous Electron Beam Accelerator Facility and the future Electron-Ion Collider (EIC). These experiments play a critical role in advancing our understanding of nucleons and nuclei in terms of quark and gluon degrees of freedom. The use of generative models for simulating collider events faces several challenges such as the sparsity of the data, the presence of global or eventwide constraints, and steeply falling particle distributions. In this work, we focus on the implementation of diffusion models for the simulation of electron-proton scattering events at EIC energies. Our results demonstrate that diffusion models can reproduce relevant observables such as momentum distributions and correlations of particles, momentum sum rules, and the leading electron kinematics, all of which are of particular interest in electron-proton collisions. Although the sampling process is relatively slow compared to other machine-learning architectures, we find diffusion models can generate high-quality samples. We foresee various applications of our work including inference for nuclear structure, interpretable generative machine learning, and searches of physics beyond the Standard Model. Published by the American Physical Society 2024

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Nuclear Isomer Discovery Database Released

Nuclear isomers correspond to excited states in nuclides with finite lifetimes. Here, after the discovery of isotopes–different nuclides of the same element–in 1913 by Frederick Soddy [Citation1], Otto Hahn postulated in 1921 [Citation2] that there are even different metastable states within one isotope. In analogy to chemical isomers, which are the same compounds with distinct structures, nuclear isomers have the same number of protons and neutrons but in different configurations.

Thoennessen, Michael [Michigan State University, E↗
DOE OSTI2025

Nuclear fragmentation at the future electron-ion collider

We explore the potential of conducting low-energy nuclear physics studies, including nuclear structure and decay, at the future Electron-Ion Collider (EIC) at Brookhaven. By comparing the standard theory of electron-nucleus scattering with the equivalent photon method applied to Ultraperipheral Collisions (UPC) at the Large Hadron Collider (LHC) at CERN. In the limit of extremely high beam energies and small energy transfers, very transparent equations emerge. We apply these equations to analyze nuclear fragmentation in UPCs at the LHC and 𝑒𝐴 scattering at the EIC, demonstrating that the EIC could facilitate unique photonuclear physics studies. Furthermore, we have also shown that the fragmentation cross-sections at the EIC are about 1,000 times smaller than those at the LHC. At the LHC, the fragmentation of uranium nuclei displays characteristic double-hump mass distributions from fission events, while at the EIC, fragmentation is dominated by neutron emission and fewer few fission products, about 10,000 smaller number of events.

Bertulani, Carlos A. [East Texas A&M University, C↗
DOE OSTI2025

Photonuclear tomography in ultraperipheral heavy-ion collisions

We present a theoretical investigation of photonuclear tomography as a novel technique for probing the internal structure of nuclei. In this approach, ultraperipheral heavy-ion collisions (UPCs) serve as a source of intense fluxes of virtual photons, which induce coherent production of vector mesons. By analyzing the probabilities and cross sections of these photon-induced processes, we propose a methodology for reconstructing the spatial distribution of nucleons within the nucleus. Our framework provides a systematic way to access information on the nuclear geometry probed in UPCs, offering new opportunities for studies of nuclear structure using particle production as a probe. Numerical calculations for selected examples illustrate the feasibility and potential of this method.

particle & resonance production↗
DOE OSTI2025

Deformation and Collectivity in Doubly Magic 208 Pb

Lead-208 is the heaviest known doubly magic nucleus and its structure is therefore of special interest. Despite this magicity, which acts to provide a strong restorative force toward sphericity, it is known to exhibit both strong octupole correlations and some of the strongest quadrupole collectivity observed in doubly magic systems. In this Letter, we employ state-of-the-art experimental equipment to conclusively demonstrate, through four Coulomb-excitation measurements, the presence of a large, negative, spectroscopic quadrupole moment for both the vibrational octupole 3$^{−}_{1}$ and quadrupole 2$^{+}_{1}$ state, indicative of a preference for prolate deformation of the states. The observed quadrupole moment is discussed in the context of the expected splitting of the 3 − ⊗3 − two-phonon states, due to the coupling of the quadrupole and octupole motion. These results are compared with theoretical values from three different methods, which are unable to reproduce both the sign and magnitude of this deformation. Thus, in spite of its well-studied nature, 208 Pb remains a puzzle for our understanding of nuclear structure.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Fission Evaluation Tools and Analytics (FETA)

This living document presents the Python package FETA. FETA computes observables resulting from the fission process. This document provides the definition of these observables as well as the physics models that are implemented to compute them. Some of these models are used to determine the initial conditions of fission fragments, e.g., the excitation energy E* and spin distribution p(J, π) at scission for prompt decay, while others are related to the nuclear structure and decay properties of the fragments, e.g. the ground-state properties, level density and low-lying excitation spectrum, γ-strength functions and electromagnetic transitions, and neutron transmission coefficients. The end goal for FETA is to enable users to substitute every one of these models by their own files providing these quantities.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

How threshold effects in spectroscopic factors influence heavy-ion knockout reactions

A two-decade-old puzzle in heavy-ion one-nucleon knockout reactions is the strong correlation between the reduction factor R S = σ exp /σ t h and the Fermi surface asymmetry ΔS. Theoretical cross sections typically rely on spectroscopic factors (SFs) from shell model (SM) calculations, which neglect continuum coupling effects. Here, we employ the Gamow shell model (GSM), which explicitly incorporates continuum coupling, to compute SFs for p-shell nuclei and predict corresponding theoretical cross sections. Systematic calculations demonstrate that using GSM-derived SFs substantially reduces discrepancies between theoretical and experimental results. This improvement is particularly significant for deeply bound nucleon knockout in nuclei near the dripline, where traditional SM-based calculations fall short. As a result, using GSM SFs, the ratio R s exhibits no pronounced dependence on ΔS. Furthermore, both the ratio of GSM SFs to SM SFs and their corresponding reaction cross sections ratios exhibit a strong ΔS dependence. We have also compared GSM SFs and cross sections with those from the no-core shell model calculations, giving a similar pronounced sensitivity to ΔS. Detailed analysis attributes these correlations to threshold effects for SFs in weakly bound systems. Overall, incorporating continuum coupling via GSM enhances the reliability of SF predictions for exotic, weakly bound nuclei and provides key insights toward resolving the enduring puzzle in heavy-ion knockout reactions from a nuclear structure perspective.

Gamow shell model↗
DOE OSTI2024

Reduction of spectroscopic overlap across the Z = 8 shell in neutron-rich nuclei

The recent discovery and spectroscopic measurements of 27 O and 28 O suggests the disappearance of the N = 20 shell structure in these neutron-rich oxygen isotopes. We measured one- and two-proton removal cross sections from 27 F and 29 N, respectively, extracting spectroscopic factors and comparing them to shell model overlap functions coupled with eikonal reaction model calculations. The invariant mass technique was used to reconstruct the two-body ( 24 O + n) and three-body ( 24 O + 2n) decay energies from knockout reactions of 27 F (106.2 MeV/u) and 29 Ne (112.8 MeV/u) beams impinging on a 9 Be target. The one-proton removal from 27 F strongly populated the ground state of 26 O and the extracted cross section of $3.4^{+0.3}_{-1.5}$ mb agrees with eikonal model calculations that are normalized by the shell model spectroscopic factors and account for the systematic reduction factor observed for single nucleon removal reactions within the models used. For the two-proton removal reaction from 29 Ne an upper limit of 0.08 mb was extracted for populating states in 27 O decaying though the ground state of 26 O. The measured upper limit for the population of the ground state of 26 O in the two-proton removal reaction from 29 Ne indicates a significant difference in the underlying nuclear structure of 27 F and 29 Ne.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

The Future Polarized Target Program at Jefferson Lab

Polarized targets have played a crucial role in Jefferson Lab's exploration of nuclear structure over the past four decades. The three original experimental halls have seen 19 separate installations of polarized solid or gas targets for use in the particle physics scattering experiments, and this trend will continue in the next decade. Five polarized target systems are in preparation for use at JLab in the coming years. Hall B will see the use of two solid polarized targets, one longitudinally polarized to the beam, the other transversely, as well as a novel 3He gas polarized target. In Hall C, new experiments will augment the tensor polarization in dynamically polarized solids. Plans are under development to bring a polarized solid target to Jefferson Lab's photon beam hall, Hall D, for the first time. To support these efforts, the JLab polarized target group is building a test laboratory to develop dynamic nuclear polarization techniques, as well as an apparatus to irradiate target material using electrons from JLab's injector test facility. In this talk, we will explore the development progress and plans for each of these efforts.

Maxwell, James [Thomas Jefferson National Accelera↗
DOE OSTI2026

Low-energy 17 O(𝑛,𝛾)⁢ 18 O reaction within the microscopic potential model and its role for the weak 𝑟 process

The neutron radiative capture reaction 17 O ⁡(𝑛,𝛾) ⁢18 O plays a pivotal role in both nuclear structure studies and astrophysical nucleosynthesis, particularly in the formation of elements during hydrostatic and explosive stellar environments. We calculated the 17 O ⁡(𝑛,𝛾) ⁢18 O cross section within the Skyrme Hartree-Fock potential model and analyzed electric dipole 𝐸⁢1 transitions to both positive- and negative-parity states below the α-decay threshold in 18 O. Our cross sections are significantly different from the data available in commonly used libraries. We further investigate the impact of the new calculated cross section on weak 𝑟-process nucleosynthesis using large-scale reaction network calculations across a wide range of electron fractions and entropies. Our results show that the 17 O ⁡(𝑛,𝛾) ⁢18 O reaction rate significantly influences the production of first 𝑟-process peak elements, such as strontium, under specific astrophysical conditions. This study highlights the importance of accurate nuclear data for light isotopes in modeling heavy-element synthesis and provides updated reaction rates for future nucleosynthesis simulations.

6 ≤ A ≤ 19↗
DOE OSTI2025

Investigation of an octupole breathing mode of 208 Pb as a resolution to the elliptical-to-triangular azimuthal anisotropy puzzle in ultracentral relativistic heavy ion collisions

Relativistic heavy ion collisions provide a unique opportunity to probe the nuclear structure by taking an instantaneous snapshot of the colliding nuclei and converting it into momentum anisotropies of final emitted hadrons. A long-standing puzzle of too large a ratio of the elliptical-to-triangular (𝑣 2 -to-𝑣 3 ) anisotropies in ultracentral 208 Pb + 208 Pb collisions at the Large Hadron Collider (LHC) cannot be solved simply by hydrodynamic simulations with initial conditions containing the spherical or certain deformed shape of 208 Pb. Here, in this Letter, using the iEBE-VISHNU relativistic viscous hydrodynamic hybrid model simulations with the TR⁢ENTo initial condition, we show that a dynamic octupole deformation—a shape-breathing mode of 208 Pb —could potentially solve the 𝑣2-to-𝑣3 puzzle and simultaneously describe the 𝑣 3 ⁡{4} data measured in experiment. Our results highlight the unique capability of capturing transient collective properties of nuclei on yoctosecond (10 −24 s) timescales, unfeasible with low-energy nuclear reactions.

Xu, Hao-jie [Huzhou University, Zhejiang (China)] ↗
DOE OSTI2025

Ab initio computations of the fourth-order charge density moments of 48 Ca and 208 Pb

Neutron skins of neutron-rich nuclei connect nuclei with the matter in neutron stars. High-precision measurements of nuclear charge densities to extract higher-order moments are proposed to be sensitive to neutron radii and skin thicknesses. We investigate the charge density of 48 Ca and 208 Pb, leading candidates for such studies, with ab initio nuclear structure calculations. We find strong correlations between the fourth-order charge density moment R$^{4}_{ch}$ and the charge and neutron radii, allowing us to predict R$^{4}_{ch}$ for 48 Ca and 208 Pb. We find a substantially weaker correlation between the fourth-order charge density moment and the neutron skin, limiting the ability of high-precision electron scattering to determine the neutron skin in a model-independent manner.

Ab initio nuclear theory↗
DOE OSTI2026

Stochastic mean-field theory and applications to multinucleon transfer and kinetic energy dissipation processes in heavy-ion collisions

In this Review article, a brief description of the stochastic mean-field (SMF) theory for describing reaction dynamics in low-energy heavy-ion collisions at bombarding energies in the vicinity of the Coulomb barrier is presented. In these collisions, as a result of strong Pauli blocking, binary nucleon collisions do not have a significant effect on the dissipation and fluctuations. At low energies, the mean-field fluctuations, due to initial correlations, have a dominant effect on fluctuations of macroscopic variables. The SMF theory proposes the determination of an ensemble of single-particle density matrices by specifying random initial fluctuations according to a distribution law. Employing an ensemble of single-particle density matrices, not only the mean values but also the distribution functions of the one-body observables can be determined. If the di-nuclear structure is maintained in heavy-ion collisions, such as deep inelastic collisions and fast quasi-fission reactions, a much simpler description of the reaction mechanism can be derived in terms of several macroscopic variables such as mass and charge asymmetry, and relative linear and relative angular momentum. In this case, by geometric projection of the SMF equations, it is possible to derive the quantal Langevin equations for macroscopic variables. As an application of quantal transport description, an analysis of multinucleon transfers and kinetic energy dissipation and fluctuations is presented for selected quasi-fission reactions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Precision Mass Measurements Reveal Low Neutron Pairing in Tin beyond 𝑁=82 and Its Impact on Stellar Nucleosynthesis

We present a study on neutron-rich tin (𝑍 =50) isotopes beyond the doubly closed shell of 𝑁 = 82 through high-precision mass measurements, including the first-ever measurements of the masses of 136 Sn, 137 Sn, and 138 Sn isotopes. These measurements enhance our understanding of the nuclear structure and astrophysical nucleosynthesis in this previously unexplored region. The new mass data are used for evaluation of the final abundances of mass numbers 𝐴 =135 and 137 in 𝑟-process network calculations. Our findings reveal a notable change in the empirical pairing gap for tin isotopes beyond the 𝑁 = 82 closed shell and a shift in the two-neutron-separation energy slope compared to heavier elements above the shell closure. A new set of ab initio calculations effectively describes these observed trends.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗