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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Impacts of long-range transport of aerosols on marine-boundary-layer clouds in the eastern North Atlantic

Vertical profiles of aerosols are inadequately observed and poorly represented in climate models, contributing to the current large uncertainty associated with aerosol–cloud interactions. The US Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) aircraft field campaign near the Azores islands provided ample observations of vertical distributions of aerosol and cloud properties. Here we utilize the in situ aircraft measurements from the ACE-ENA and ground-based remote-sensing data along with an aerosol-aware Weather Research and Forecast (WRF) model to characterize the aerosols due to long-range transport over a remote region and to assess their possible influence on marine-boundary-layer (MBL) clouds. The vertical profiles of aerosol and cloud properties measured via aircraft during the ACE-ENA campaign provide detailed information revealing the physical contact between transported aerosols and MBL clouds. The European Centre for Medium-Range Weather Forecasts Copernicus Atmosphere Monitoring Service (ECMWF-CAMS) aerosol reanalysis data can reproduce the key features of aerosol vertical profiles in the remote region. The cloud-resolving WRF sensitivity experiments with distinctive aerosol profiles suggest that the transported aerosols and MBL cloud interactions (ACIs) require not only aerosol plumes to get close to the marine-boundary-layer top but also large cloud top height variations. Based on those criteria, the observations show that the occurrence of ACIs involving the transport of aerosol over the eastern North Atlantic (ENA) is about 62 % in summer. For the case with noticeable long-range-transport aerosol effects on MBL clouds, the susceptibilities of droplet effective radius and liquid water content are -0.11 and +0.14, respectively. When varying by a similar magnitude, aerosols originating from the boundary layer exert larger microphysical influence on MBL clouds than those entrained from the free troposphere.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Important role of stratospheric injection height for the distribution and radiative forcing of smoke aerosol from the 2019–2020 Australian wildfires

More than 1 Tg smoke aerosol was emitted into the atmosphere by the exceptional 2019–2020 southeastern Australian wildfires. Triggered by the extreme fire heat, several deep pyroconvective events carried the smoke directly into the stratosphere. Once there, smoke aerosol remained airborne considerably longer than in lower atmospheric layers. The thick plumes traveled eastward, thereby being distributed across the high and mid-latitudes in the Southern Hemisphere, enhancing the atmospheric opacity. Due to the increased atmospheric lifetime of the smoke plume, its radiative effect increased compared to smoke that remains in lower altitudes. Global models describing aerosol-climate impacts lack adequate descriptions of the emission height of aerosols from intense wildfires. Here, we demonstrate, by a combination of aerosol-climate modeling and lidar observations, the importance of the representation of those high-altitude fire smoke layers for estimating the atmospheric energy budget. Through observation-based input into the simulations, the Australian wildfire emissions by pyroconvection are explicitly prescribed to the lower stratosphere in different scenarios. Based on our simulations, the 2019–2020 Australian fires caused a significant top-of-atmosphere (TOA) hemispheric instantaneous direct radiative forcing signal that reached a magnitude comparable to the radiative forcing induced by anthropogenic absorbing aerosol. Up to +0.50 W m -2 instantaneous direct radiative forcing was modeled at TOA, averaged for the Southern Hemisphere (+0.25 W m -2 globally) from January to March 2020 under all-sky conditions. At the surface, on the other hand, an instantaneous solar radiative forcing of up to -0.81 W m -2 was found for clear-sky conditions, with the respective estimates depending on the model configuration and subject to the model uncertainties in the smoke optical properties. Since extreme wildfires are expected to occur more frequently in the rapidly changing climate, our findings suggest that high-altitude wildfire plumes must be adequately considered in climate projections in order to obtain reasonable estimates of atmospheric energy budget changes.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1993

Megaplumes on Venus

The geoid and topography heights of Atla Regio and Beta Regio, both peaks and slopes, appear explicable as steady-state plumes, if non-linear viscosity eta(Tau, epsilon) is taken into account. Strongly constrained by the data are an effective plume depth of about 700 km, with a temperature anomaly thereat of about 30 degrees, leading to more than 400 degrees at the plume head. Also well constrained is the combination Q(eta)/s(sup 4)(sub 0) = (volume flow rate)(viscosity)/(plume radius): about 11 Pa/m/sec. The topographic slopes dh/ds constrain the combination Q/A, where A is the thickness of the spreading layer, since the slope varies inversely with velocity. The geoid slopes dN/ds require enhancement of the deeper flow, as expected from non-linear viscosity. The Beta data are best fit by Q = 500 m(sup 3)/sec and A equals 140 km; the Atla, by Q equals 440 m(exp 3)/sec and A equals 260 km. The dynamic contribution to the topographic slope is minor.

Kaula, W. M.↗
NASA NTRS2014

Sport Transition of JPSS VIIRS Imagery for Night-time Applications

The NASA/Short‐term Prediction, Research, and Transition (SPoRT) Program and NOAA/Cooperative Institute for Research in the Atmosphere (CIRA) work within the NOAA/Joint Polar Satellite System (JPSS) Proving Ground to demonstrate the unique capabilities of the VIIRS instrument. Very similar to MODIS, the VIIRS instrument provides many high‐resolution visible and infrared channels in a broad spectrum. In addition, VIIRS is equipped with a low‐light sensor that is able to detect light emissions from the land and atmosphere as well as reflected sunlight by the lunar surface. This band is referred to as the Day‐Night Band due to the sunlight being used at night to see cloud and topographic features just as one would typically see in day‐time visible imagery. NWS forecast offices that collaborate with SPoRT and CIRA have utilized MODIS imagery in operations, but have longed for more frequent passes of polar‐orbiting data. The VIIRS instrument enhances SPoRT collaborations with WFOs by providing another day and night‐time pass, and at times two additional passes due to its large swath width. This means that multi‐spectral, RGB imagery composites are more readily available to prepare users for their use in GOES‐R era and high‐resolution imagery for use in high‐latitudes is more frequently able to supplement standard GOES imagery within the SPoRT Hybrid GEO‐LEO product. The transition of VIIRS also introduces the new Day‐Night Band capability to forecast operations. An Intensive Evaluation Period (IEP) was conducted in Summer 2013 with a group of "Front Range" NWS offices related to VIIRS night‐time imagery. VIIRS single‐channel imagery is able to better analyze the specific location of fire hotspots and other land features, as well as provide a more true measurement of various cloud and aerosol properties than geostationary measurements, especially at night. Viewed within the SPoRT Hybrid imagery, the VIIRS data allows forecasters to better interpret the more frequent, but coarse GOES Imagery. Night‐time Microphysics and Dust RGB Imagery provides cloud analysis of cloud height, thickness, and composition in order for operational applications such as separating fog from low clouds, dust plume detection, and determining precipitating clouds in radar-void/ blocked regions. The Day‐Night Band has a particular benefit to seeing light from cities, fires, or other emissions as well as the reflection of moonlight off of clouds and smoke plumes, given the right lunar phase and angle. Examples from the VIIRS transition and IEP will be presented.

Fuell, Kevin↗
NASA NTRS2015

Quantification of Plume-Soil Interaction and Excavation Due to the Sky Crane Descent Stage

The quantification of the particulate erosion that occurs as a result of a rocket exhaust plume impinging on soil during extraterrestrial landings is critical for future robotic and human lander mission design. The aerodynamic environment that results from the reflected plumes results in dust lifting, site alteration and saltation, all of which create a potentially erosive and contaminant heavy environment for the lander vehicle and any surrounding structures. The Mars Science Lab (MSL), weighing nearly one metric ton, required higher levels of thrust from its retro propulsive systems and an entirely new descent system to minimize these effects. In this work we seek to quantify plume soil interaction and its resultant soil erosion caused by the MSL's Sky Crane descent stage engines by performing three dimensional digital terrain and elevation mapping of the Curiosity rover's landing site. Analysis of plume soil interaction altitude and time was performed by detailed examination of the Mars Descent Imager (MARDI) still frames and reconstructed inertial measurement unit (IMU) sensor data. Results show initial plume soil interaction from the Sky Crane's eight engines began at ground elevations greater than 60 meters and more than 25 seconds before the rovers' touchdown event. During this time, viscous shear erosion (VSE) was dominant typically resulting in dusting of the surface with flow propagating nearly parallel to the surface. As the vehicle descended and decreased to four powered engines plume-plume and plume soil interaction increased the overall erosion rate at the surface. Visibility was greatly reduced at a height of roughly 20 meters above the surface and fell to zero ground visibility shortly after. The deployment phase of the Sky Crane descent stage hovering at nearly six meters above the surface showed the greatest amount of erosion with several large particles of soil being kicked up, recirculated, and impacting the bottom of the rover chassis. Image data obtained from MSL's navigation camera (NAVCAM) pairs on Sols 002, 003, and 016 were used to virtually recreate local surface topography and features around the rover by means of stereoscopic depth mapping. Images taken simultaneously by the left and right navigation cameras located on the rover's mast assembly spaced 42 centimeters were used to generate a three dimensional depth map from flat, two dimensional images of the same feature at slightly different angles. Image calibration with physical hardware on the rover and known terrain features were used to provide scaling information that accurately sizes features and regions of interest within the images. Digital terrain mapping analysis performed in this work describe the crater geometry (shape, radius, and depth), eroded volume, volumetric erosion rate, and estimated mass erosion rate of the Hepburn, Sleepy Dragon, Burnside, and Goulburn craters. Crater depths ranged from five to ten centimeters deep influencing an area as wide as two meters in some cases. The craters formed were highly asymmetrical and generally oblong primarily due to the underlying bedrock formations underneath the surface. Comparison with ground tests performed at the NASA AMES Planetary Aeolian Laboratory (PAL) by Mehta showed good agreement with volumetric erosion rates and crater sizes of large particle soil simulants, providing validation to Earth based ground tests of Martian regolith.

Vizcaino, Jeffrey↗
DOE OSTI2021

Experimental Results of 2-m Heptane, Bakken Crude Oil, and Dilbit Crude Oil Pool Fire Tests Performed for the National Research Council of Canada

This report provides results from a series of 2-m pool fire experiments performed in the Thermal Test Complex at Sandia National Laboratories testing heptane, Bakken crude oil, and dilbit crude oil. The effect of the presence and placement of a calorimeter, fuel supply temperature, and maintaining a constant fuel level were assessed. Measurements include burn rate, surface emissive power, flame height, heat flux to an engulfed calorimeter, heat flux to external instruments, thermocouple temperatures within the fuel and fire plume, and heat release rate. The results indicate that the presence and placement of the calorimeter has the most effect on the measured quantities for the Bakken crude oil and indicated no effect for the Dilbit crude oil. The fuel feed temperature had a slight effect for the heptane fuel, but not for the crude oils. Allowing the fuel to burn down did not have a significant effect on any of the fuels. The Bakken crude oil resulted in the highest average total heat flux to the calorimeter by a factor of about 1.5 and 1.3 higher compared to heptane and the dilbit crude oil, respectively.

02 PETROLEUM↗
NASA NTRSDate not supplied

Towards Physics Guided Optical Flow for Tracking Atmospheric Motion

Atmospheric 3D winds in the horizontal and vertical directions are critical for improving short-range and long-range forecasting. Such advancement in forecasting directly applies to research in a number of areas including convective processes, wildfire plumes and tornado prediction. Atmospheric Motion Vectors (AMVs) provide a passively sensed approach to quantifying horizontal motion and cloud heights, which are typically sourced from geostationary sensors due to the availability of high frequency observations. Recent work has shown that estimating AMVs by tracking individual pixels with dense optical flow is a promising new direction. In this work, we use a state-of-the-art convolutional neural network for optical flow (FlowNetS) in a physics-guided deep learning framework for predicting AMVs in the horizontal direction. The approach is semi-supervised and uses physically informed wind vectors from high-resolution numerical simulations (DYAMOND) for supervised learning followed by fine-tuning though warping and reconstruction of full-disk geostationary images (GOES-16). In the vertical direction, we use labels from the CALIPSO low-earth orbit satellite to predict cloud height from 16-band geostationary images with a neural network. We present results for both tasks on held-out time periods and secondary datasets.

geostationary↗
NASA NTRSDate not supplied

Towards Physics Guided Optical Flow for Tracking Atmospheric Motion

Observations of atmospheric 3D winds are critical for improving short-range and long-range forecasting. Such advancement in forecasting directly applies to research in a number of areas including convective processes, wildfire plumes and tornado prediction. Atmospheric Motion Vectors (AMVs) provide a passively sensed approach to quantifying horizontal motion and cloud heights, which are typically sourced from geostationary sensors due to the availability of high frequency observations. Recent work has shown that estimating AMVs by tracking individual pixels with dense optical flow is a promising new direction. In this work, we compare state-of-the-art convolutional neural networks for optical flow in a physics-guided deep learning framework for predicting AMVs. The approach is semi-supervised and uses physically informed wind vectors from high-resolution numerical simulations for supervised learning followed by fine-tuning though warping and reconstruction of full-disk geostationary images (GOES-16). In the vertical direction, we use labels from the CALIPSO low-earth orbit satellite to predict cloud height from 16-band geostationary images with a neural network. We present results for both tasks on held-out time periods and secondary datasets.

Geostationary↗
NASA NTRS2022

Surface-to-Space Atmospheric Waves From Hunga Tonga–Hunga Ha’apai Eruption

The January 2022 Hunga Tonga–Hunga Ha’apai eruption was one of the most explosive volcanic events of the modern era, producing a vertical plume that peaked more than 50 km above the Earth. The initial explosion and subsequent plume triggered atmospheric waves that propagated around the world multiple times. A global-scale wave response of this magnitude from a single source has not previously been observed. Here we show the details of this response, using a comprehensive set of satellite and ground-based observations to quantify it from surface to ionosphere. A broad spectrum of waves was triggered by the initial explosion, including Lamb waves propagating at phase speeds of 318.2 ± 6 m s^(−1) at surface level and between 308 ± 5 to 319 ± 4 m s^(−1) in the stratosphere, and gravity waves propagating at 238 ± 3 to 269 ± 3 m s^(−1) in the stratosphere. Gravity waves at sub-ionospheric heights have not previously been observed propagating at this speed or over the whole Earth from a single source. Latent heat release from the plume remained the most significant individual gravity wave source worldwide for more than 12 h, producing circular wavefronts visible across the Pacific basin in satellite observations. A single source dominating such a large region is also unique in the observational record. The Hunga Tonga eruption represents a key natural experiment in how the atmosphere responds to a sudden point-source-driven state change, which will be of use for improving weather and climate models.

Corwin J. Wright↗
DOE OSTI2020

Using a coupled dispersion model to estimate depletion of a tritium oxide plume by a forest

Tritium processing facilities may release tritium oxide (HTO) to the atmosphere which poses potential health risks to exposed co-located workers and to offsite individuals. Most radiological consequence analyses determine HTO dose by applying Gaussian plume models to simulate the transport of HTO. Within these models, deposition velocity is used to assess the sum of all deposition processes acting on the plume. While this may account for vegetative and soil uptake or respiration processes, it may currently lack inclusion of the complex interactions within heterogeneous forested environments. In this complex morphology, dispersion patterns are significantly altered by changing flow regimes above and below the forest canopy and by the transfer of plume material across the canopy boundary. To determine the effects of a heterogeneous forest canopy on an airborne HTO plume, a Gaussian plume model coupled with an advection-diffusion plume model was applied to estimate transport in the free atmosphere above the forest and within the forest canopy and understory. During 2012, wind speed and wind direction measurements taken at 5 heights, ranging from 2-m to 28-m, on an instrumented meteorological tower located in a loblolly pine forest at the Department of Energy (DOE) Savannah River Site (SRS), near Aiken, SC. From these measurements, model predictions were made over a full spectrum of meteorological conditions. Deposition and resuspension velocities were calculated based on the model-predicted flux of plume material across the top of the forest canopy. Additionally, net deposition velocity of the plume material was calculated as the difference between the deposition and resuspension velocities. The 1st and 5th percentile net deposition velocities were estimated to be 0.7 cm s-1 and 1.2 cm s-1, respectively.

63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTAN↗
NASA NTRS2019

Joint 3D-Wind Retrievals with Stereoscopic Views from MODIS and GOES

Atmospheric motion vectors (AMVs), derived by tracking patterns, represent the winds in a layer characteristic of the pattern. AMV height (or pressure), important for applications in atmospheric research and operational meteorology, is usually assigned using observed IR brightness temperatures with a modeled atmosphere and can be inaccurate. Stereoscopic tracking provides a direct geometric height measurement of the pattern that an AMV represents. We extend our previous work with multi-angle imaging spectroradiometer (MISR) and GOES to moderate resolution imaging spectroradiometer (MODIS) and the GOES-R series advanced baseline imager (ABI). MISR is a unique satellite instrument for stereoscopy with nine angular views along track, but its images have a narrow (380 km) swath and no thermal IR channels. MODIS provides a much wider (2330 km) swath and eight thermal IR channels that pair well with all but two ABI channels, o e ring a rich set of potential applications. Given the similarities between MODIS and VIIRS, our methods should also yield similar performance with VIIRS. Our methods, as enabled by advanced sensors like MODIS and ABI, require high-accuracy geographic registration in both systems but no synchronization of observations. AMVs are retrieved jointly with their heights from the disparities between triplets of ABI scenes and the paired MODIS granule. We validate our retrievals against MISR-GOES retrievals, operational GOES wind products, and by tracking clear-sky terrain. We demonstrate that the 3D-wind algorithm can produce high-quality AMV and height measurements for applications from the planetary boundary layer (PBL) to the upper troposphere, including cold-air outbreaks, wildfire smoke plumes, and hurricanes.

Carr, James L.↗
NASA NTRSDate not supplied

Latest Progress and Results in LEO-GEO and GEO-GEO Stereo AMVs

Atmospheric motion vectors (AMVs), derived by tracking patterns, represent the winds in a layer characteristic of the pattern. AMV height (or pressure), important for applications in atmospheric research and operational meteorology, is usually assigned using observed IR brightness temperatures with a modeled atmosphere and can be inaccurate. Stereoscopic tracking provides a direct geometric height measurement of the pattern that an AMV represents. We extend our previous work with multi-angle imaging spectro–radiometer (MISR) and GOES to moderate resolution imaging spectroradiometer (MODIS) and the GOES-R series advanced baseline imager (ABI). MISR is a unique satellite instrument for stereoscopy with nine angular views along track, but its images have a narrow (380 km) swath and no thermal IR channels. MODIS provides a much wider (2330 km) swath and eight thermal IR channels that pair well with all but two ABI channels, offering a rich set of potential applications. Given the similarities between MODIS and VIIRS, our methods should also yield similar performance with VIIRS. Our methods, as enabled by advanced sensors like MODIS and ABI, require high-accuracy geographic registration in both systems but no synchronization of observations. AMVs are retrieved jointly with their heights from the disparities between triplets of ABI scenes and the paired MODIS granule. We validate our retrievals against MISR-GOES retrievals, operational GOES wind products, and by tracking clear-sky terrain. We demonstrate that the 3D-wind algorithm can produce high-quality AMV and height measurements for applications from the planetary boundary layer (PBL) to the upper troposphere, including cold-air outbreaks, wildfire smoke plumes, and hurricanes.

Atmospheric motion vectors↗
DOE OSTI2024

The Physics behind Precipitation Onset Bias in CMIP6 Models: The Pseudo-Entrainment Diagnostic and Trade-Offs between Lapse Rate and Humidity

Conditional instability and the buoyancy of plumes drive moist convection but have a variety of representations in model convective schemes. Vertical thermodynamic structure information from Atmospheric Radiation Measurement (ARM) sites and reanalysis (ERA5), satellite-derived precipitation (TRMM3b42), and diagnostics relevant for plume buoyancy are used to assess climate models. Previous work has shown that CMIP6 models represent moist convective processes more accurately than their CMIP5 counterparts. However, certain biases in convective onset remain pervasive among generations of CMIP modeling efforts. Here we diagnose these biases in a cohort of nine CMIP6 models with sub-daily output, assessing conditional instability in profiles of equivalent potential temperature θ e and saturation equivalent potential temperature θ es in comparison to a plume model with different mixing assumptions. Most models capture qualitative aspects of the θ es vertical structure, including a substantial decrease with height in the lower free troposphere associated with the entrainment of subsaturated air. We define a “pseudo-entrainment” diagnostic that combines subsaturation and a θ es measure of conditional instability similar to what entrainment would produce under the small-buoyancy approximation. This captures the trade-off between larger θ es lapse rates (entrainment of dry air) and small subsaturation (permits positive buoyancy despite high entrainment). This pseudo-entrainment diagnostic is also a reasonable indicator of the critical value of integrated buoyancy for precipitation onset. Models with poor θ e /θ es structure (those using variants of the Tiedtke Scheme) or low entrainment runs of CAM5, and models with low subsaturation, such as NASA-GISS, lie outside the observational range in this diagnostic.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1998

Prediction Based Design of Fire Detection for Buildings with Ceiling Heights between 9m and 18m

The purpose of this paper is to provide the experimental and theoretical background necessary to extend guidelines to ceiling heights between 9 m and 18 m. Based on the results of experiments conducted in 15 m and 22 m high hangars, detector activation thresholds and detector spacing are analyzed for both smoke and heat detectors. Only ceiling mounted detection devices are analyzed in this paper. In addition to the detector threshold study, the predictive capabilities of computer fire model simulations were compared with experimental results. This comparison, which is based on 12 fire tests, resulted in the development of a new ceiling jet algorithm to model phenomena which had not been included in previous algorithms. The improved algorithm provides a better representation of the development of the ceiling jet temperature to a growing hot layer and a better estimation of plume centerline temperature. Guidelines are examined, based on the experimental results, for fire detector spacing, placement, and sensitivity. Recommendations concerning the use of computer fire models at these heights are made as a function of fire size and hot layer development. The role of draft curtains is discussed and their impact on detector activation is demonstrated.

Davis, W. D.↗
DOE OSTI2024

Green buffers near industrial plants, examples in Jefferson County TX

Green buffers between industrial plants and residential areas have multiple purposes in mitigating air pollution and protecting the environment. This study focuses on providing information on examples of green space development by industries near residential areas in Jefferson County, Texas. One represents a full buffer where residences were totally removed, another is a partial buffer where some residences were removed in a neighborhood and the third represents vegetation of a formerly industrial facility. Additional estimates on benefits of buffer spaces with respect to a pollutant plume are also considered. The study used geospatial and property data from 1966 to 2020. The transition from a residential area to a full or partial buffers highlights possible mitigation of air pollution impacts while serving additional functions, such as boosting stormwater infiltration and improving the aesthetic attractiveness of the area. The transformation from oil tanks to forested space may display the potential for environmental remediation, but not all spaces are suitable for fully forested buffers, as safety and other limitations should be considered. With the analysis of the classic Plume Equation insights can be provided regarding the possible impact of green buffers on ground-level pollutant concentrations. The calculations for atmospheric stability classes A-F and for various stack heights provide an understanding of how different conditions may affect the pollutant concentrations. The presence of a green buffer can play a crucial role in controlling ground-level pollution concentrations and reduce a community’s perception of risk.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2001

Overview of ACE-Asia Spring 2001 Investigations on Aerosol Radiative Effects and Related Aerosol Properties

A primary, ACE-Asia objective was to quantify the interactions between aerosols and radiation in the Asia-Pacific region. Toward this end, radiometric and related aerosol measurements were made from ocean, land, air and space platforms. Models that predict aerosol fields guided the measurements and are helping integrate and interpret results. Companion overview's survey these measurement and modeling components. Here we illustrate how these components were combined to determine aerosol radiative. impacts and their relation to aerosol properties. Because clouds can obscure or change aerosol direct radiative effects, aircraft and ship sorties to measure these effects depended on predicting and finding cloud-free areas and times with interesting aerosols present. Pre-experiment satellite cloud climatologies, pre-flight aerosol and cloud forecasts, and in-flight guidance from satellite imagery all helped achieve this. Assessments of aerosol regional radiative impacts benefit from the spatiotemporal coverage of satellites, provided satellite-retrieved aerosol properties are accurate. Therefore, ACE-Asia included satellite retrieval tests, as part of many comparisons to judge the consistency (closure) among, diverse measurements. Early results include: (1) Solar spectrally resolved and broadband irradiances and optical depth measurements from the C-130 aircraft and at Kosan, Korea yielded aerosol radiative forcing efficiencies, permitting comparisons between efficiencies of ACE-Asia and INDOEX aerosols, and between dust and "pollution" aerosols. Detailed results will be presented in separate papers. (2) Based on measurements of wavelength dependent aerosol optical depth (AOD) and single scattering albedo the estimated 24-h a average aerosol radiative forcing efficiency at the surface for photosynthetically active radiation (400 - 700 nm) in Yulin, China is approx. 30 W sq m per AOD(500 nm). (3) The R/V Brown cruise from Honolulu to Sea of Japan sampled an aerosol optical depth gradient, with AOD(500 nm) extremes from 0.1 to 1.1. On the Pacific transit from Honolulu to Hachijo AOD(500 nm) averaged 0.2, including increases to 0.4 after several storms, suggesting the strong impact of wind-generated seasalt. The AOD maximum, found in the Sea of Japan, was influenced by dust and anthropogenic sources. (4) In Beijing, single scattering albedo retrieved from AERONET sun-sky radiometry yielded midvisible SSA=0.88 with strong wavelength dependence, suggesting a significant black carbon component. SSA retrieved during dust episodes was approx. 0.90 and variable but wavelength neutral reflecting the presence of urban haze with the dust. Downwind at Anmyon Island SSA was considerably higher, approx. 0.94, but wavelength neutral for dust episodes and spectrally dependent during non dust periods. (5) Satellite retrievals show major aerosol features moving from Asia over the Pacific; however, determining seasonal-average aerosol effects is hampered by sampling frequency and large-scale cloud systems that obscure key parts of aerosol patterns. Preliminary calculations using, satellite-retrieved AOD fields and initial ACE-Asia aerosol properties (including sulfates, soot, and dust) yield clear-sky aerosol radiative effects in the seasonal-average ACE-Asia plume exceeding those of manmade greenhouse gases. Quantifying all-sky direct aerosol radiative effects is complicated by the need to define the height of absorbing aerosols with respect to cloud decks.

Russell, Philip B.↗
NASA NTRSDate not supplied

Hyper-Spectral Infrared Remote Sensing for Wildfire-Related Research and Air Quality Monitoring

The National Airborne Sounder Testbed-Interferometer (NAST-I) is an airborne FTS remote sensor that nominally flies on NASA high-altitude aircraft to serve as a spaceborne instrument simulator. NAST-I continues to serve as a pathfinder for future satellite FTS systems and the next generation advanced atmospheric sounders in general. NAST-I provides high resolution spectrally resolved infrared radiances. NAST-I retrieval products characterizing the surface (i.e., skin temperature and spectral emissivity), atmosphere (i.e., profiles of temperature, moisture, ozone, carbon monoxide, and other trace species), and clouds (e.g., optical depth, particle size, temperature, and height) can be used to support fire-related monitoring and research. NAST-I provided 3-d characterizations of wildfire-induced plumes of CO during the FIREX-AQ field campaign (conducted during 2019) which showed the intensity and size evolution of wildfire plumes at high spatial and temporal resolutions. Wildfire-induced CO plumes, in conjunction with their evolution, transport, and age have been identified and recently published in scientific journals. Other research applications, such as surface emissivity changes due to fire burning of ground landscape, have been under investigation. These products could be used in support of wildfire management to better inform decision making and operations for pre-, active, and post-fire environments.

remote sensing↗
DOE OSTI2026

Mechanism-Resolved PFM of Ferroionic and Ferroelectric Responses in Thickness-Gradient Hf 0.5 Zr 0.5 O 2 Libraries

Resolving growth mechanisms and thickness evolution of functional properties is one of the key tasks in materials discovery and optimization involving thin-film materials, traditionally requiring significant experimental budgets. Here we introduce the combination of thickness-gradient libraries and automated scanning probe microscopy as a systematic pathway to elucidate growth modes and disentangle ferroelectric and electrochemical contributions in ferroelectric thin films. As a model system, we explore the Hf 0.5 Zr 0.5 O 2 (HZO) gradient thin films grown on La x Sr 1-x MnO 3 (LSMO) bottom electrode thin films. Automated piezoresponse force microscopy, spectroscopy, and lithography reveals that irreversible topographic deformation arises from electrochemical activity at the LSMO surface, whereas reversible phase inversion in HZO reflects ferroelectric switching. Automated topography height-map scans are used to further quantify nucleation density, particle-size evolution, and roughness correlations across the thickness-gradient, demonstrating that improved plume stabilization during growth suppresses interfacial reactions and promotes dense, fine-grained HZO conducive to ferroelectric phase formation. This combined materials-engineering and automated-SPM framework establishes a platform for high-throughput, mechanism-resolved characterization of ferroionic and ferroelectric responses in complex oxide films.

FOS: Physical sciences↗