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DOE OSTI2025

Probing Surface Plasmon Dynamics in Periodic Nanostructures through Ultrafast Electron Microscopy

Surface plasmon polaritons (SPPs) can be manipulated to localize and guide light in subwavelength distances, enabling them to find applications in a wide range of areas, from sensing to quantum computing. Among several methods of SPP excitation, periodic arrays of nano- and microstructures are of particular interest, as they enable engineering SPP properties through structural parameters. Here, in this study, using the photon-induced near-field electron microscopy (PINEM) technique, we investigated the mode formation, coupling, interference, and decay of SPPs in square and hexagonal arrays of circular nanoholes under both visible and near-infrared excitation. Polarization-resolved analysis revealed the key factors governing SPP localization and interference patterns, showing that the periodicity and symmetry of the array primarily determine the SPP interference patterns and their orientation, while pump polarization mainly modulates their intensity. Time-resolved PINEM measurements demonstrated the spatial dependence of the SPP temporal characteristics. In addition, cathodoluminescence (CL) spectroscopy was employed to examine the intrinsic plasmonic characteristics of the structure. Finite difference time domain (FDTD) simulations showed strong agreement with both PINEM and CL measurements on the spatial and spectral behavior of SPPs. Understanding the spatiotemporal dynamics of SPPs on nanostructures beyond the diffraction limit is crucial for optimizing plasmonic structures for advanced photonic and quantum technologies.

Plasmonics↗

DOE OSTI2025

High-fidelity remote entanglement of trapped atoms mediated by time-bin photons

Abstract Photonic interconnects between quantum processing nodes are likely the only way to achieve large-scale quantum computers and networks. The bottleneck in such an architecture is the interface between well-isolated quantum memories and flying photons. We establish high-fidelity entanglement between remotely separated trapped atomic qubit memories, mediated by photonic qubits stored in the timing of their pulses. Such time-bin encoding removes sensitivity to polarization errors, enables long-distance quantum communication, and is extensible to quantum memories with more than two states. Using a measurement-based error detection process and suppressing a fundamental source of error due to atomic recoil, we achieve an entanglement fidelity of 97% and show that fundamental limits due to atomic recoil still allow fidelities in excess of 99.9%.

Science & Technology - Other Topics↗

DOE OSTI2022

FilDReaMS: II. Application to the analysis of the relative orientations between filaments and the magnetic field in four Herschel fields

Context. Both simulations and observations of the interstellar medium show that the study of the relative orientations between filamentary structures and the magnetic field can bring new insight into the role played by magnetic fields in the formation and evolution of filaments and in the process of star formation. Aims. We provide a first application of FilDReaMS, the new method presented in the companion paper to detect and analyze filaments in a given image. The method relies on a template that has the shape of a rectangular bar with variable width. Our goal is to investigate the relative orientations between the detected filaments and the magnetic field. Methods. We apply FilDReaMS to a small sample of four Herschel fields (G210, G300, G82, G202) characterized by different Galactic environments and different evolutionary stages. First, we look for the most prevalent bar widths, and we examine the networks formed by filaments of different bar widths as well as their hierarchical organization. Second, we compare the filament orientations to the magnetic field orientation inferred from Planck polarization data and, for the first time, we study the statistics of the relative orientation angle as functions of both spatial scale and H2 column density. Results. We find preferential relative orientations in the four Herschel fields: small filaments with low column densities tend to be slightly more parallel than perpendicular to the magnetic field; in contrast, large filaments, which all have higher column densities, are oriented nearly perpendicular (or, in the case of G202, more nearly parallel) to the magnetic field. In the two nearby fields (G210 and G300), we observe a transition from mostly parallel to mostly perpendicular relative orientations at an H 2 column density ≃ 1.1 × 10 21 cm -2 and 1.4 × 10 21 cm -2 , respectively, consistent with the results of previous studies. Conclusions. Our results confirm the existence of a coupling between magnetic fields at cloud scales and filaments at smaller scale. They also illustrate the potential of combining Herschel and Planck observations, and they call for further statistical analyses with our dedicated method.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2022

Polarization angle requirements for CMB B-mode experiments. Application to the LiteBIRD satellite

A methodology to provide the polarization angle requirements for different sets of detectors, at a given frequency of a CMB polarization experiment, is presented. The uncertainties in the polarization angle of each detector set are related to a given bias on the tensor-to-scalar ratio r parameter. The approach is grounded in using a linear combination of the detector sets to obtain the CMB polarization signal. In addition, assuming that the uncertainties on the polarization angle are in the small angle limit (lower than a few degrees), it is possible to derive analytic expressions to establish the requirements. The methodology also accounts for possible correlations among detectors, that may originate from the optics, wafers, etc. The approach is applied to the LiteBIRD space mission. We show that, for the most restrictive case (i.e., full correlation of the polarization angle systematics among detector sets), the requirements on the polarization angle uncertainties are of around 1 arcmin at the most sensitive frequency bands (i.e., ≈ 150 GHz) and of few tens of arcmin at the lowest (i.e., ≈ 40 GHz) and highest (i.e., ≈ 400 GHz) observational bands. Conversely, for the least restrictive case (i.e., no correlation of the polarization angle systematics among detector sets), the requirements are ≈ 5 times less restrictive than for the previous scenario. At the global and the telescope levels, polarization angle knowledge of a few arcmins is sufficient for correlated global systematic errors and can be relaxed by a factor of two for fully uncorrelated errors in detector polarization angle. The reported uncertainty levels are needed in order to have the bias on r due to systematics below the limit established by the LiteBIRD collaboration.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2026

Cryogenic light detectors with thermal signal amplification for 0 νββ search experiments

As a step towards the realization of cryogenic-detector experiments to search for neutrinoless double-beta decay (such as CROSS, BINGO, and CUPID), we investigated a batch of 10 Ge light detectors (LDs) assisted by Neganov-Trofimov-Luke (NTL) signal amplification. Each LD was assembled with a large cubic light-emitting crystal (45 mm side) using the recently developed CROSS mechanical structure. The detector array was operated at milli-Kelvin temperatures in a pulse-tube cryostat at the Canfranc underground laboratory in Spain. We achieved good performance with scintillating bolometers from CROSS, made of Li 2 100 MoO 4 crystals and used as reference detectors of the setup, and with all LDs tested (except for a single device that encountered an electronics issue). No leakage current was observed for 8 LDs with an electrode bias up to 100 V. Operating the LDs at an 80 V electrode bias applied in parallel, we obtained a gain of around 9 in the signal-to-noise ratio of these devices, allowing us to achieve a baseline noise RMS of O(10 eV). Thanks to the strong current polarization of the temperature sensors, the time response of the devices was reduced to around half a millisecond in rise time. The achieved performance of the LDs was extrapolated via simulations of pile-up rejection capability for several configurations of the CUPID detector structure. Despite the sub-optimal noise conditions of the LDs (particularly at high frequencies), we demonstrated that the NTL technology provides a viable solution for background reduction in CUPID.

47 OTHER INSTRUMENTATION↗

DOE OSTI2021

Temporal coherent control of resonant two-photon double ionization of the hydrogen molecule via doubly excited states

Here, we use time-delayed, counter-rotating, circularly polarized few-cycle attosecond nonoverlapping pulses to study the temporal coherent control of the resonant process of two-photon double ionization (TPDI) of hydrogen molecule via doubly excited states for pulse propagation direction along $\hat k$ either parallel or perpendicular to the molecular axis $\hat R$. For $\hat k$∥ $\hat R$ and a pulse carrier frequency of 36 eV resonantly populating the Q 2 1 Π$^+_u$ (1) doubly excited state as well as other 1 Π$^+_u$ doubly excited states, we find that the indirect ionization pathway through these doubly excited states changes the character of the kinematical vortex-shaped momentum distribution produced by the two direct ionization pathways from fourfold to twofold rotational symmetry. This result is similar to what found in TPDI of the He atom involving 1 P$^ o_ {±1}$ doubly excited states; however, angular distributions exhibiting a quantum beat effect between the ground state and a doubly excited state seen for the He atom are observed here for its molecular counterpart with an anomaly in shape and magnitude, not in frequency. The sixfold differential probability integrated over the azimuthal angle of the photoelectron pair shows that this anomaly is due to autoionization decays and quantum beats between doubly excited states. For $\hat k$⟂$\hat R$ and a broadband pulse carrier frequency of 30 eV populating the Q 1 1 Π$^+_u$(1), Q 1 1 Σ$^+_u$(1), Q 2 1 Π$^+_u$(1) , and Q 1 1 Σ$^+_u$ (2) doubly excited states, the momentum distribution is shown to exhibit dynamical electron vortices with four spiral arms, which originates from the interplay between the 1 Δ$^+_ g$ , 1 Π$^+_ g$, and 1 Σ$^+_ g$ dynamical ionization amplitudes. Our treatment within either the adiabatic-nuclei approximation or fixed-nuclei approximation shows that the latter provides a very good account for this correlated process.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2020

Ultrafast nonequilibrium evolution of excitonic modes in semiconductors

We study the time evolution of excitonic states after photoexcitation in the one-dimensional spinless extended Falicov-Kimball model. Several numerical methods are employed and benchmarked against each other: time-dependent mean-field simulations, the second-Born approximation (2BA) within the Kadanoff-Baym formalism, the generalized Kadanoff-Baym ansatz (GKBA) implemented with the 2BA, and the infinite time-evolving block decimation (iTEBD) method. It is found that the GKBA gives the best agreement with iTEBD and captures the relevant physics. Excitations to the particle-hole continuum and resonant excitations of the equilibrium exciton result in a qualitatively different dynamics. In the former case, the exciton binding energy remains positive and the frequency of the corresponding coherent oscillations is smaller than the band gap. On the other hand, resonant excitations trigger a collective mode whose frequency is larger than the band gap. We discuss the origin of these different behaviors by evaluating the nonequilibrium susceptibility using the nonthermal distribution and a random phase approximation. We note the peculiar mode with frequency larger than the band gap is associated with a partial population inversion with a sharp energy cutoff. We also discuss the effects of the cooling by a phonon bath. We demonstrate the real-time development of coherence in the polarization, which indicates excitonic condensation out of equilibrium.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2025

Ultrafast renormalization of the magnetic continuum in the proximal Kitaev quantum spin liquid H 3 LiIr 2 O 6 by tr-RIXS [Invited]

We present the first circularly polarized non-resonant pump time-resolved resonant inelastic X-ray scattering (tr-RIXS) experiment in H 3 LiIr 2 O 6 , an iridium-based Kitaev system. Our calculations and experimental results are consistent with the modification of the low-energy magnetic excitations in H 3 LiIr 2 O 6 only during illumination by the laser pulse. We discuss these results in a cooperative framework between the Floquet engineering of the exchange interactions and the dynamic renormalization of electron-electron correlations. However, the penetration length mismatch between the X-ray probe and laser pump and the intrinsic complexity of Kitaev magnets prevents us from unequivocally extracting towards which ground state H 3 LiIr 2 O 6 is driven. We outline possible solutions to these challenges for light-driven stabilization and observation of the Kitaev quantum spin liquid limit by RIXS.

Kim, Jungho [Argonne National Laboratory (ANL), Ar↗

DOE OSTI2024

Daytime variation in the aerosol indirect effect for warm marine boundary layer clouds in the eastern North Atlantic

Abstract. Warm boundary layer clouds in the eastern North Atlantic region exhibit significant diurnal variations in cloud properties. However, the diurnal cycle of the aerosol indirect effect (AIE) for these clouds remains poorly understood. This study takes advantage of recent advancements in the spatial resolution of geostationary satellites to explore the daytime variation in the AIE by estimating the cloud susceptibilities to changes in cloud droplet number concentration (Nd). Cloud retrievals for the month of July over 4 years (2018–2021) from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) on Meteosat-11 over this region are analyzed. Our results reveal a significant “U-shaped” daytime cycle in susceptibilities of the cloud liquid water path (LWP), cloud albedo, and cloud fraction. Clouds are found to be more susceptible to Nd perturbations at noon and less susceptible in the morning and evening. The magnitude and sign of cloud susceptibilities depend heavily on the cloud state defined by cloud LWP and precipitation conditions. Non-precipitating thin clouds account for 44 % of all warm boundary layer clouds in July, and they contribute the most to the observed daytime variation. Non-precipitating thick clouds are the least frequent cloud state (10 %), and they exhibit more negative LWP and albedo susceptibilities compared to thin clouds. Precipitating clouds are the dominant cloud state (46 %), but their cloud susceptibilities show minimal variation throughout the day. We find evidence that the daytime variation in LWP and albedo susceptibilities for non-precipitating clouds is influenced by a combination of the diurnal transition between non-precipitating thick and thin clouds and the “lagged” cloud responses to Nd perturbations. The daytime variation in cloud fraction susceptibility for non-precipitating thick clouds can be attributed to the daytime variation in cloud morphology (e.g., overcast or broken). The dissipation and development of clouds do not adequately explain the observed variation in cloud susceptibilities. Additionally, daytime variation in cloud susceptibility is primarily driven by variation in the intensity of cloud response rather than the frequency of occurrence of cloud states. Our results imply that polar-orbiting satellites with an overpass time at 13:30 LT underestimate daytime mean values of cloud susceptibility, as they observe susceptibility daily minima in the study region.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

First study of polarized proton-proton scattering with small-𝑥 helicity evolution

We perform a phenomenological study of helicity-dependent parton distribution functions (PDFs) using small-𝑥 helicity evolution equations, incorporating for the first time single-inclusive jet production data in polarized proton-proton (𝑝⁢𝑝) scattering at parton momentum fractions 𝑥 <0.1. We also simultaneously include double-longitudinal spin asymmetries in inclusive and semi-inclusive deep-inelastic scattering probing 𝑥 <0.1. Employing the polarized small-𝑥 pure-glue calculation of 𝑝⁢𝑝 → 𝑔⁡𝑋 for the jet production cross section, we modify the large-𝑁 𝑐 &𝑁 𝑓 KPS-CTT evolution equations by setting 𝑁 𝑓 = 0 to replicate the large-𝑁𝑐 (pure-glue) limit, while retaining external quark flavors for the spinor field operators. We find that the 𝑝⁢𝑝 data have a considerable impact on the helicity PDFs at small 𝑥, reducing their uncertainties and leading to a total quark and gluon helicity in the proton for 𝑥 < 0.1 of −0.04 ±0.23. Combining our analysis with a recent JAM helicity PDF analysis of the world polarized data, which includes 𝑥 > 0.1, we find a total quark and gluon helicity contribution for 𝑥 >10 −7 of between 0.02 and 0.51.

Adamiak, Daniel [Michigan State University] (ORCID↗

DOE OSTI2020

A Sensorless Coil Detection Scheme based on Dead-Time Effect in Dynamic Wireless Power Transfer Systems

The detection of electric vehicles in dynamic wireless power transfer (DWPT) systems is important to reduce the standby losses and comply with the electromagnetic-field emission guidelines recommended by the International Commission for Non-Ionizing Radiation Protection. This paper discusses a novel sensorless coil detection scheme, which exploits the phenomenon of voltage-polarity reversal/notches caused by the dead-time effect in the full-bridge inverter. The variations in the system impedance and dead-time effects are collectively exploited to detect the receiver coil in the DWPT system. The proposed coil detection scheme is accomplished at low excitation voltage, which reduces the inverter standby losses. The theoretical analysis of the notch occurrence and open-loop simulation results are presented using a DWPT model developed in the piecewise linear electrical circuit simulation software.

Kavimandan, Utkarsh↗

DOE OSTI2024

Enhancements of electric field and afterglow of non-equilibrium plasma by Pb(ZrxTi1−x)O3 ferroelectric electrode

Abstract Manipulating surface charge, electric field, and plasma afterglow in a non-equilibrium plasma is critical to control plasma-surface interaction for plasma catalysis and manufacturing. Here, we show enhancements of surface charge, electric field during breakdown, and afterglow by ferroelectric barrier discharge. The results show that the ferroelectrics manifest spontaneous electric polarization to increase the surface charge by two orders of magnitude compared to discharge with an alumina barrier. Time-resolved in-situ electric field measurements reveal that the fast polarization of ferroelectrics enhances the electric field during the breakdown in streamer discharge and doubles the electric field compared to the dielectric barrier discharge. Moreover, due to the existence of surface charge, the ferroelectric electrode extends the afterglow time and makes discharge sustained longer when alternating the external electric field polarity. The present results show that ferroelectric barrier discharge offers a promising technique to tune plasma properties for efficient plasma catalysis and electrified manufacturing.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2024

Transverse Λ polarization in unpolarized $pp$ → jet Λ ↑ X

In this Letter, we investigate the spontaneous transverse polarization of Λ hyperons produced in unpolarized pp collisions inside a jet, by adopting a TMD approach where transverse momentum effects are included only in the fragmentation process. We will present predictions based on the parametrizations of the Λ polarizing fragmentation function as extracted from fits to Belle e + e – data. These estimates will be compared against preliminary STAR data. We will then be able to explore the universality properties of the quark polarizing fragmentation function and, for the first time, the role of its gluon counterpart.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2021

First-principles Prediction of X-Ray Polarization from Magnetic Reconnection in High-frequency BL Lacertae Objects

Relativistic magnetic reconnection is a potential particle acceleration mechanism for high-frequency BL Lac objects (HBLs). The Imaging X-ray Polarimetry Explorer (IXPE) scheduled to launch in 2021 has the capability to probe the evolution of magnetic field in HBLs, examining the magnetic reconnection scenario for the HBL flares. In this paper, we make the first attempt to self-consistently predict HBL X-ray polarization signatures arising from relativistic magnetic reconnection via combined particle-in-cell and polarized radiation transfer simulations. Here, we find that although the intrinsic optical and X-ray polarization degrees are similar on average, the X-ray polarization is much more variable in both the polarization degree and angle (PD and PA). Given the sensitivity of the IXPE, it may obtain one to a few polarization data points for one flaring event of nearby bright HBLs Mrk 421 and 501. However, it may not fully resolve the highly variable X-ray polarization. Due to temporal depolarization, where the integration of photons with variable polarization states over a finite period of time can lower the detected PD, the measured X-ray PD can be considerably lower than the optical counterpart or even undetectable. The lower X-ray PD than the optical thus can be a characteristic signature of relativistic magnetic reconnection. For very bright flares where the X-ray polarization is well resolved, relativistic magnetic reconnection predicts smooth X-ray PA swings, which originate from large plasmoid mergers in the reconnection region.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2023

Quantum efficiency enhancement in simulated nanostructured negative electron affinity GaAs photocathodes

We report nanostructured negative electron affinity GaAs photocathodes for a polarized electron source are studied using finite difference time domain optical simulation. The structures studied are nanosquare columns, truncated nanocones, and truncated nanopyramids. Mie-type resonances in the 700–800 nm waveband, suitable for generation of polarized electrons, are identified. At resonance wavelengths, the nanostructures can absorb up to 99% of the incident light. For nanosquare columns and truncated nanocones, the maximum quantum efficiency (QE) at 780 nm obtained from simulation is 27%, whereas for simulated nanopyramids, the QE is ~21%. The high photocathode quantum efficiency is due to the shift of Mie resonance toward the longer wavelength, leading to increased light absorption. The field profile distribution shows the excitation of dipole and quadrupole modes within the nanostructures at resonant frequencies. This leads to enhanced photoabsorption and photoelectron generation closer to emission surfaces than for a flat photocathode. The enhanced photoabsorption and reduced electron transport distance for the nanostructured photocathode enhance its QE compared to that for the flat surface wafer.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2022

A time‐varying formulation of the curled wake model within the FAST.Farm framework

Abstract In this article, we present a time‐varying formulation of the curled wake model that we implemented in FAST.Farm. The curled wake model, originally developed for steady‐state conditions, is used to produce realistic wake profiles behind a wind turbine in yawed (or skewed) conditions. We begin by introducing the key elements of the FAST.Farm framework. Then, after briefly summarizing the original wake dynamics formulation of FAST.Farm based on a polar wake profile, we present the new time‐varying formulation of the curled wake model, compare the two, and highlight the differences with the original curled wake model. After discussing some implementation details, we present different applications with increasing levels of complexity: single turbine with uniform and turbulent inflow, fixed and transient yaw, and multiple turbines. We verify our results using the original FAST.Farm implementation and large‐eddy simulations. The results with the new curled wake model are improved compared to the original implementation, as they include cross‐flow velocities and wake asymmetry. Yet, large‐eddy simulation results show a more pronounced lateral convection of the wake and a stronger concentration of vorticity at the top vortex. The new curled wake implementation in FAST.Farm should enable the calculation of not only generator power but also wind turbine structural loads for applications involving intentional or unintentional skewed flow and wind‐farm control involving wake steering.

17 WIND ENERGY↗

DOE OSTI2020

Comparison of Dead-Time Effects in a WPT System Inverter for Different Fixed-Frequency Modulation Techniques

In this paper, a comparative study of the dead-time effects in a wireless power transfer (WPT) system inverter is performed for different fixed-frequency control techniques. The dead-time is provided between the complementary switching instances of the inverter phase-legs to ensure safe operation of the input power source. Under certain operating conditions, the dead-time results in waveform distortions or voltage-polarity reversal (VPR) at the inverter output. The VPR affects the switching characteristics, harmonic spectrum, switching losses, and output voltage/power of the system. A detailed analysis of the dead-time effect on the WPT system parameters such as output voltage and output power is conducted for the different fixed-frequency control strategies (i.e., traditional phase-shift control, asymmetrical clamped-mode, and asymmetrical duty-cycle control). Furthermore, the impact of dead-time on the inverter switching losses is compared for the different control strategies.

Kavimandan, Utkarsh↗

DOE OSTI2023

Connectivity between Static Field and Continuous Wave Field Effects on Excitation-Induced H 2 Activation

Due to the tremendous applications of the plasmon resonance excitation process, such as improvements in catalytic efficiency due to plasmonic enhancement and/or hot-electron processes, understanding the mechanism behind these processes has become a popular topic in recent years. In this work, we focus on unraveling the mechanism of excitation-induced H 2 activation using a simplified triangular Au 6 /Ag 6 cluster to investigate the effects of the electric field on electron redistribution and bond activation. We applied both static and continuous wave fields to investigate how these fields affect the systems. Geometrical changes (such as bond lengthening), molecular orbital reordering (affecting the relative energies of orbitals corresponding to hot-electron and charge-transfer excited states), and electronic charge redistribution between the cluster and the adsorbate occur upon application of a static electric field. To study H 2 activation, we apply Ehrenfest dynamics with real-time time-dependent density functional theory and examine how different excitation frequencies and polarizations affect bond activation. Moreover, electron-only dynamics are examined with real-time time-dependent density functional theory, and the time-dependent variations in the orbital populations and electronic transitions provide information about the excitation and relaxation processes of hot electrons with applied electric fields. Here, the static field results represent structures that can be accessed during the evolution of the systems when applying continuous wave fields. Through these studies, the effects of static and continuous wave field effects on plasmon-induced H 2 activation can be understood.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗