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Ozone and temperature trends

An update of the extensive reviews of the state of knowledge of measured ozone trends published in the Report of the International Ozone Trends Panel is presented. The update contains a review of progress since these reports, including reviewing of the ozone records, in most cases through March 1991. Also included are some new, unpublished reanalyses of these records including a complete reevaluation of 29 stations located in the former Soviet Union. The major new advance in knowledge of the measured ozone trend is the existence of independently calibrated satellite data records from the Total Ozone Mapping Spectrometer (TOMS) and Stratospheric Aerosol and Gas Experiment (SAG) instruments. These confirm many of the findings, originally derived from the Dobson record, concerning northern mid-latitude changes in ozone. We now have results from several instruments, whereas the previously reported changes were dependent on the calibration of a single instrument. This update will compare the ozone records from many different instruments to determine whether or not they provide a consistent picture of the ozone change that has occurred in the atmosphere. The update also briefly considers the problem of stratospheric temperature change. As in previous reports, this problem received significantly less attention, and the report is not nearly as complete. This area needs more attention in the future.

Stolarski, Richard S.↗

Spectroscopic Evidence Against Nitric Acid Trihydrate in Polar Stratospheric Clouds

Heterogeneous reactions on polar stratospheric clouds (PSC's) play a key role in the photochemical mechanism thought to be responsible for ozone depletion in the Antarctic and Arctic. Reactions of PSC particles activate chlorine to forms that are capable of photochemical ozone destruction, and sequester nitrogen oxides (NOx) that would otherwise deactivate the chlorine. Although the heterogeneous chemistry is now well established, the composition of the clouds themselves is uncertain. It is commonly thought that they are composed of nitric acid trihydrate, although observations have left this question unresolved. Here we reanalyse infrared spectra of type 1 PSCs obtained in Antarctica in September 1987, using recently measured optical constants of the various compounds that might be present in PSCs. We find these PSCs were not composed of nitric acid trihydrate but instead had a more complex compositon, perhaps that of a ternary solution. Because cloud formation is sensitive to their composition, this finding will alter our understanding of the locations and conditions in which PSCs form. In addition, the extent of ozone loss depends on the ability of the PSCs to remove NOx permanently through sedimentation, The sedimentation rates depend on PSC particle size which in turn is controlled by the composition and formation mechanism.

Toon, Owen B.↗

Spectroscopic Evidence Against Nitric Acid Trihydrate in Polar Stratospheric Clouds

Heterogeneous reactions on polar stratospheric clouds (PSC's) play a key role in the photochemical mechanisms thought to be responsible for ozone depletion in the Antarctic and the Arctic. Reactions on PSC particles activate chlorine to forms that are capable of photochemical ozone destruction, and sequester nitrogen oxides (NOx) that would otherwise deactivate the chlorine. Although the heterogeneous chemistry is now well established, the composition of the clouds themselves is uncertain. It is commonly thought that they are composed of nitric acid trihydrate, although observations have left this question unresolved. Here we reanalyse infrared spectra of type I PCS's obtained in Antarctica in September 1987, using recently measured optical constraints of the various compounds that might be present in PSC's. We find that these PSC's were not composed of nitric acid trihydrate but instead had a more complex composition perhaps that of a ternary solution. Because cloud formation is sensitive to their composition, this finding will alter our understanding of the locations and conditions in which PSCs form. In addition, the extent of ozone loss depends on the ability of the PSC's to remove NOx permanently through sedimentation. The sedimentation rates depend on PSC particle size which in turn is controlled by the composition and formation mechanism.

Toon, Owen B.↗

Technical Report Series on Global Modeling and Data Assimilation: Interannual Variability and Potential Predictability in Reanalysis Products - Volume 13

The Data Assimilation Office (DAO) at Goddard Space Flight Center and the National Center for Environmental Prediction and National Center for Atmospheric Research (NCEP/NCAR) have produced multi-year global assimilations of historical data employing fixed analysis systems. These "reanalysis" products are ideally suited for studying short-term climatic variations. The availability of multiple reanalysis products also provides the opportunity to examine the uncertainty in the reanalysis data. The purpose of this document is to provide an updated estimate of seasonal and interannual variability based on the DAO and NCEP/NCAR reanalyses for the 15-year period 1980-1995. Intercomparisons of the seasonal means and their interannual variations are presented for a variety of prognostic and diagnostic fields. In addition, atmospheric potential predictability is re-examined employing selected DAO reanalysis variables.

Min, Wei↗

Decadal Air-Sea Interaction in the North Atlantic Based on Observations and Modeling Results

The decadal, 12-14 year, cycle observed in the North Atlantic SST and tide gauge data was examined using the NCEP/NCAR reanalyses, COADS data and an ocean model simulation. Besides this decadal mode, a shorter, subdecadal period of about 8 years exists in tide gauge data north of 40N, in the subpolar SST and in the winter North Atlantic Oscillation (NAO) index and in subpolar winter heat flux values. The decadal cycle is a well separated mode in a singular spectrum analysis (SSA) for a time series of SST EOF mode 1 with a center over the Gulf Stream extension. Tide gauge and SST data are consistent in that both show a significant subdecadal periodicity exclusively in the subpolar gyre, but in subtropics the 12-14 year period is the prominent, but nonstationary, decadal signal. The main finding of this study is that this 12-14 year cycle can be constructed based on the leading mode of the surface heat flux. This connection to the surface heat flux implicates the participation of the thermohaline circulation in the decadal cycle. During the cycle starting from the positive index phase of NAO, SST and oceanic heat content anomalies are created in subtropics due to local heat flux and intensification of the thermohaline circulation. The anomalies advect to the subpolar gyre where they are amplified by local heat flux and are part of the negative feedback of thermohaline circulation on itself. Consequently the oceanic thermohaline circulation slows down and the opposite cycle starts. The oscillatory nature would not be possible without the active atmospheric participation in the cycle, because it provides the unstable interaction through heat flux, without it, the oceanic mode would be damped. This analysis suggests that the two principal modes of heat flux variability, corresponding to patterns similar to North Atlantic Oscillation (NAO) and Western Atlantic (WA), are part of the same decadal cycle and an indirect measure of the north-south movement of the storm tracks.

Hakkinen, Sirpa↗

Trends in the Vertical Distribution of Ozone

Recent reanalyses of satellite, ground-based and balloon measurements allow updated estimates of trends in the vertical profile of ozone during 1980-96. The results show overall consistency between several independent measurement systems, particularly for northern hemisphere mid-latitudes where most ground-based measurements are made. Combined trend estimates over these latitudes show statistically significant negative trends at all altitudes between 10 and 45 km, with two local maxima: -7.4 +/- 2.0%/decade at 40 km and -7.6 +/- 4.6%/decade at 15 km altitude. There is a strong seasonal variation in trends over northern mid-latitudes in the altitude range of 10- 18 km. The profile trends are in quantitative agreement with independently measured trends in column ozone.

Randel, William J.↗

The Tropical Upper Troposphere and Lower Stratosphere in the GEOS-2 GCM

The structure of the tropical upper troposphere and lower stratosphere in the GEOS-2 General Circulation Model (GCM) is discussed. The emphasis of this study is on the reality of monthly-mean temperature and water vapor distributions in the model, compared to reasonable observational estimates. It is shown that although the zonal-mean temperature is in good agreement with observations, the GCM supports an excessive zonal asymmetry near the tropopause compared to the ECMWF Reanalyses. In reality there is a QBO-related variability in the zonally averaged lower stratospheric temperature which is not captured by the model. The observed upper tropospheric temperature and humidity fields show variations related to those in the sea surface temperature, which are not incorporated in the GCM; nevertheless, there is some interannual variability in the GCM, indicating a component arising from internal processes. The model is too moist in the middle troposphere (500 hPa) but too dry in the upper troposphere, suggesting that there is too little vertical transport or too much drying in the GCM. Transport into the stratosphere shows a pronounced annual cycle, with drier air entering the tropical stratosphere when the tropopause is coldest in northern winter; while the alternating dry and moist air masses can be traced ascending through the tropical lower stratosphere, the progression of the anomalies is too rapid.

Pawson, S.↗

The East Asian Jet Stream and Asian-Pacific Climate

In this study, the NASA GEOS and NCEP/NCAR reanalyses and GPCP rainfall data have been used to study the variability of the East Asian westerly jet stream and its impact on the Asian-Pacific climate, with a focus on interannual time scales. Results indicate that external forcings such as sea surface temperature (SST) and land surface processes also play an important role in the variability of the jet although this variability is strongly governed by internal dynamics. There is a close link between the jet and Asian-Pacific climate including the Asian winter monsoon and tropical convection. The atmospheric teleconnection pattern associated with the jet is different from the ENSO-related pattern. The influence of the jet on eastern Pacific and North American climate is also discussed.

Yang, Song↗

Asian Monsoons: Variability, Predictability, and Sensitivity to External Forcing

In this study, we have addressed the interannual variations of Asian monsoons including both broad-scale and regional monsoon components. Particular attention is devoted to the identities of the South China Sea monsoon and Indian monsoon. We use CPC Merged Analysis of Precipitation and NCEP reanalyses to define regional monsoon indices and to depict the various monsoons. Parallel modeling studies have also been carried out to assess the role of boundary forcing and the potential predictability of the monsoons. Each monsoon is characterized by its unique features. While the South Asian monsoon represents a classical monsoon in which anomalous circulation is governed by Rossby-wave dynamics, the Southeast Asian monsoon symbolizes a "hybrid" monsoon that features multi-cellular meridional circulation over eastern Asia. The broad-scale Asian monsoon links to the basin-wide atmospheric circulation over the Indian-Pacific oceans. Both SST and land surface processes are important for determining the variations of all monsoons. For the broad-scale monsoon, SST anomalies are more important than land surface processes. For regional monsoons, however, land surface processes may become equally important. Both observation and model shows that the broad-scale monsoon is potentially more predictable than regional monsoons, and that the Southeast Asian monsoon may possess higher predictability than the South Asian monsoon.

Yang, Song↗

Asian Monsoons: Variability, Predictability, and Sensitivity to External Forcing

In this study, we have addressed the interannual variations of Asian monsoons including both broad-scale and regional monsoon components. Particular attention is devoted to the identities of the South China Sea monsoon and Indian monsoon. We use CPC Merged Analysis of Precipitation and NCEP reanalyses to define regional monsoon indices and to depict the various monsoons. Parallel modeling studies have also been carried out to assess the potential predictability of the broad-scale and regional monsoons. Each monsoon is characterized by its unique features. While the South Asian monsoon represents a classical monsoon in which anomalous circulation is governed by Rossby-wave dynamics, the Southeast Asian monsoon symbolizes a "hybrid" monsoon that features multi-cellular meridional circulation over eastern Asia. The broad-scale Asian monsoon links to the basin-wide atmospheric circulation over the Indian-Pacific oceans. Both Sea Surface Temperatures (SST) and land surface processes are important for determining the variations of all monsoons. For the broad-scale monsoon, SST anomalies are more important than land surface processes. However, for regional monsoons, land surface processes may become equally important. Both observation and model shows that the broad-scale monsoon is potentially more predictable than regional monsoons, and that the Southeast Asian monsoon may possess higher predictability than the South Asian monsoon.

Yang, Song↗

Intercomparisons of Total Precipitable Water from Satellite and Other Long Term Data Sets

Global water vapor data sets from satellite (NVAP) and reanalysis (NCEP and DAO) are intercompared for a 5 year period (1988-1992). Global average indicates that the NCEP and DAO reanalyses are dryer than NVAP over much of the period. Spatial patterns of the NCEP/NVAP and DAO/NVAP differences show regional variations in the 60 month climatogical fields. For example, in the Eastern Pacific just south of the equator NVAP is much dryer than the NCEP and more moist than DAO. Rather large discrepancies exist in other regions as well. North Africa, Saudi Arabia, India, and Australia show that NVAP TPW values are more moist than the NCEP and DAO model analyses by 4-8 mm. In general, the NCEP and DAO exhibits a tendency to be dryer than NVAP over the tropical ocean region. Over the Americas little differences exist except over the west coast. The shapes of the differences fields over the Eastern Pacific region are significantly different between NCEP/NVAP and DAO/NVAP differences. Over South America and Central Africa, DAO TPW values are significantly higher than those of NVAP. These difference fields show monthly and seasonal variability as well. These results will be highlighted in the paper and on the poster.

Chang, Fong-Chiau↗

Role of Ocean Currents and Bottom Pressure Variability on Seasonal Polar Motion

Changes in the ocean angular momentum (OAM) components about the equatorial axes, either due to fluctuations in currents or bottom pressure (mass redistribution), can induce movements of the Earth's pole of rotation, commonly referred to as polar motion or wobble. Output from a 1 deg resolution ocean model is used to calculate the effective equatorial OAM functions chi(sub 1, sup O) and chi(sub 2, sup O), corresponding to polar motion excitation about the equatorial axis pointing to the Greenwich and 90 deg E meridians, respectively. Time series of chi(sup O) are combined with similar atmospheric series chi(sup A), computed from the National Centers for Environmental Prediction/National Center for Atmospheric Research reanalyses, to interpret the observed low-frequency polar motion excitation for the period 1985-1996. Results indicate that the oceans are a very important excitation source for the Chandler (approximately 433 days), annual, and semiannual wobbles, providing for much better amplitude and phase agreement with the observed excitation at these periods, in comparison with what is obtained when only the atmosphere is considered. Both oceanic mass and motion terms are found to be important but with mass signals having somewhat larger amplitudes. The role of regional variability in ocean currents and bottom pressure in contributing to chi(sup O) signals is quantified. Midlatitude regions (approximately 30 deg - 70 deg) figure prominently as places of strong local oceanic excitation signals. The North Pacific basin is found to be generally important for chi(sup O) excitation, while the Southern Ocean is important for both chi(sub 1, sup O) and chi(sub 2, sup O). The largest positive covariances of local with global chi(sup O) signals occur in the Kuroshio region near the western boundary of the North Pacific for chi(sub 1, sup O) and southwest of Australia for chi(sub 2, sup O).

Ponte, Rui M.↗

Diagnosing Warm Season Precipitation Over the GCIP Region from a GCM and Reanalysis

A 45 year simulation using a global general circulation model (GCM), the National Center for Atmospheric Research (NCAR) Community Climate Model v.3 (CCM3), forced with observed sea surface temperatures (SST), and 39 years of global National Centers for Environmental Prediction (NCEP) reanalyses were analyzed to determine Mississippi River basin warm season (May, June, July or MJJ) wet and dry year composites in the water and energy budgets. Years that have increased MJJ soil moisture over the GEWEX (Global Water and Energy Experiment) Continental Interior Project (GCIP) region also have high precipitation, lower surface temperature, decreased Bowen ratio, and reduced 500 hPa geopotential height (essentially reduced MJJ ridging). The reverse is true for years that have reduced MJJ soil moisture. Wet years are also accompanied by a general increase in moisture transport from the Gulf of Mexico into the central U.S. There is some indication (though weaker) that soil moisture may then affect precipitation and other quantities and be affected in turn by 500 hPa geopotential heights. The correlations are somewhat low, however, demonstrating the difficulty in providing definitive physical links between the remote and local effects. Analysis of two individual years with an extreme wet event (1993) and an extreme dry event (1988) yields the same general relationships as with the wet and dry composites. The composites from this study are currently serving as the basis for a series of experiments aimed at determining the predictability of the land surface and remote SST on the Mississippi River basin and other large-scale river basins.

Oglesby, Robert↗

Atlas of Seasonal Means Simulated by the NSIPP 1 Atmospheric GCM

This atlas documents the climate characteristics of version 1 of the NASA Seasonal-to-Interannual Prediction Project (NSIPP) Atmospheric General Circulation Model (AGCM). The AGCM includes an interactive land model (the Mosaic scheme), and is part of the NSIPP coupled atmosphere-land-ocean model. The results presented here are based on a 20-year (December 1979-November 1999) "ANIIP-style" integration of the AGCM in which the monthly-mean sea-surface temperature and sea ice are specified from observations. The climate characteristics of the AGCM are compared with the National Centers for Environmental Prediction (NCEP) and the European Center for Medium-Range Weather Forecasting (ECMWF) reanalyses. Other verification data include Special Sensor Microwave/Imager (SSNM) total precipitable water, the Xie-Arkin estimates of precipitation, and Earth Radiation Budget Experiment (ERBE) measurements of short and long wave radiation. The atlas is organized by season. The basic quantities include seasonal mean global maps and zonal and vertical averages of circulation, variance/covariance statistics, and selected physics quantities.

Suarez, Max J.↗

Predictability of Seasonal Means in the NSIPP-1 AGCM

The predictability of seasonal means during 1980-99 is examined from 720 seasonal integrations with version 1 of NASA's Seasonal to Interanual Prediction Project (NSIPP-1) atmospheric general circulation model (AGCM). The AGCM is the atmospheric (and land) component of the NSIPP fully-coupled atmosphere-land-ocean model. For these runs, the initial atmospheric conditions are taken from the National Centers for Environmental Prediction/National Center for Atmospheric Research (NCEP/NCAR) reanalyses, and sea surface temperatures and sea ice are specified from observations. Results from the northern winter integrations show that the model has a very realistic El Nino/Southern Oscillation (ENSO) response in both the tropics and extratropics. Early results from the northern summer runs show a robust extratropical ENSO response in the Southern Hemisphere Pacific, as well as, a pronounced zonally-symmetric component to the ENSO response in both hemispheres. Results will be presented at the meeting highlighting the seasonal evolution in predictability and skill of the NSIPP model on both global and regional scales. A further analysis of the zonally-symmetric response will be discussed in terms of its potential impact on the predictability of middle-latitude climate variability on seasonal to interannual time scales.

Schubert, Siegfried↗

Predictability of the 1997 and 1998 South Asian Summer Monsoons on the Intraseasonal Time Scale Based on 10 AMIP2 Model Runs

Predictability of the 1997 and 1998 South Asian summer monsoons is examined using National Centers for Environmental Prediction/National Center for Atmospheric Research (NCEP/NCAR) reanalyses, and 100 two-year simulations with ten different Atmospheric General Circulation Models (AGCMs) with prescribed sea surface temperature (SST). We focus on the intraseasonal variations of the south Asian summer monsoon associated with the Madden-Julian Oscillation (MJO). The NCEP/NCAR reanalysis shows a clear coupling between SST anomalies and upper level velocity potential anomalies associated with the MJO. We analyze several MJO events that developed during the 1997 and 1998 focusing of the coupling with the SST. The same analysis is carried out for the model simulations. Remarkably, the ensemble mean of the two-year AGCM simulations show a signature of the observed MJO events. The ensemble mean simulated MJO events are approximately in phase with the observed events, although they are weaker, the period of oscillation is somewhat longer, and their onset is delayed by about ten days compared with the observations. Details of the analysis and comparisons among the ten AMIP2 (Atmospheric Model Intercomparison Project) models will be presented in the conference.

Wu, Man Li C.↗

Diagnosing Tropical Divergent Circulations From Satellite-Derived Diabatic Forcing and Variational Integral Constraints

Large-scale divergent circulations are part of the atmospheric dynamic response to diabatic heating from condensation, radiative processes, and surface energy fluxes. Vertical motion and the associated divergent wind is thus intimately tied to the hydrologic cycle and the global beat balance. Despite its importance, the divergent circulation is too small in comparison to the rotational flow to measure directly with any accuracy. Vertical motions are recovered diagnostically from reanalyses and, as such, are subject to shortcomings in model physics, numerics, and data availability. While reanalysis estimates of tropical divergent circulations are much improved over those from the Global Weather Experiment, there are still substantial differences between products from operational centers. This is because these circulations are still forced largely by model physics and only secondarily by observations. In order to produce a refined estimate of tropical divergence and its interannual variability we have used a number of remotely-sensed data sets along with variational constraints to improve upon reanalysis estimates. Among these are: precipitation from SSM/I and GPCP, TOVS Path-A vertical cloud distributions; ISCCP radiative cooling rates; TOA radiative fluxes from ERBS, surface radiative fluxes from the SRB project, and surface latent and sensible flux estimates from SSM/I. The TOVS Path-A data constrain the divergent outflow in precipitating regions to have the same vertical structure as observed cloudiness. Using integral constraints for moisture, heat, and mass balance, we retrieve consistent divergent wind flows. We examine the ability of this type analysis to capture regional details of ENSO related perturbations to the divergent wind and associated tropical energy balance. Precipitation from satellite is found to be the major constraint in supplying this horizontal structure. We also consider the ability of this analysis to quantify integrated (land vs. ocean) fluctuations in the global monsoonal flow and energy balance. This depends, of course, on the error characteristics of the data constraints. Some estimate of these properties and their relative importance is provided.

Robertson, Franklin R.↗

Modeling Modern Methane Emissions from Natural Wetlands: Interannual Variations 1982-1993 - 2

A global run of a process-based methane model [Walter et al., this issue] is performed using high-frequency atmospheric forcing fields from ECMWF reanalyses of the period from 1982 to 1993. We calculate global annual methane emissions to be 260 Tg/ yr. 25% of methane emissions originate from wetlands north of 30 deg. N. Only 60% of the produced methane is emitted, while the rest is re-oxidized. A comparison of zonal integrals of simulated global wetland emissions and results obtained by an inverse modeling approach shows good agreement. In a test with data from two wetlands, the seasonality of simulated and observed methane emissions agrees well. The effects of sub-grid scale variations in model parameters and input data are examined. Modeled methane emissions show high regional, seasonal and interannual variability. Seasonal cycles of methane emissions are dominated by temperature in high latitude wetlands, and by changes in the water table in tropical wetlands. Sensitivity tests show that +/- 1 C changes in temperature lead to +/- 20 % changes in methane emissions from wetlands. Uniform changes of +/- 20% in precipitation alter methane emissions by about +/- 18%. Limitations in the model are analyzed. Simulated interannual variations in methane emissions from wetlands are compared to observed atmospheric growth rate anomalies. Our model simulation results suggest that contributions from other sources than wetlands and/or the sinks are more important in the tropics than north-of 30 deg. N. In higher northern latitudes, it seems that a large part, of the observed interannual variations can be explained by variations in wetland emissions. Our results also suggest that reduced wetland emissions played an important role in the observed negative methane growth rate anomaly in 1992.

Walter, Bernadette P.↗