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All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Neutrino-Nucleus Interactions in the Precision Era

Current and future accelerator-based neutrino facilities, leveraging intense neutrino beams and advanced detectors, aim to precisely determine neutrino properties and probe signals of weakly interacting beyond the Standard Model physics. Achieving discovery-level precision and fully exploring the physics potential of these experiments critically depends on the accuracy of our understanding of fundamental underlying neutrino-nucleus interaction processes. This talk will focus on neutrino interactions spanning energies from tens of MeV to a few GeV a complex, multi-scale and multi-process domain spanning from low-energy nuclear physics to perturbative QCD, with no unified underlying framework currently known. In this talk, I will provide an overview of the field, discuss recent advancements, and share examples of ongoing cross-community efforts addressing these challenges.

Pandey, Vishvas [Fermilab] (ORCID:0000000230827987↗
DOE OSTI2026

SEARCHING FOR MESONIC DARK MATTER WITH THE HEAVY PHOTON SEARCH EXPERIMENT

Several highly-sensitive astrophysical experiments over the past couple of decades have demonstrated that the current abundance of visible Standard Model matter cannot explain galactic rotation curves, the expansion history of the Universe, or the apparent warping of light in empty space. Instead, one finds strong agreement with this body of experimental results upon positing the existence of an invisible particulate field, dark matter. Namely, a cold, weakly interacting dark matter component can explain all these phenomena. A number of accelerator-based experiments have been developed to search for the weak couplings/interactions of these particles, many of them concentrating on particle models with masses of tens to thousands of GeV. A relatively new, well-motivated model is a dark sector coupled to the Standard Model via a dark photon. The current abundance of dark matter can be obtained if one assumes that dark matter is coupled to light by a MeV to GeV particle with a U(1) symmetry. The parameter space of these models remains largely unexplored because they are difficult to probe experimentally. In this thesis, I analyze data from the Heavy Photon Search (HPS) detector, whose two detector halves closely surround the electron beam, providing acceptance to far-forward boosted interactions. This forward acceptance to highly boosted particles yields unprecedented sensitivity to MeV-scale invariant masses. I exhaustively optimize the offline reconstruction of the HPS detector. Each reconstruction object, from Silicon Vertex Tracker hits to tracks, is studied to maximize acceptance of dark matter events. I then use the 2021 run data to search for one model of dark-photon-mediated matter, the Strongly Interacting Massive Particle (SIMP). SIMP models provide self-interacting dark matter candidates that can form bound states resembling dark mesons. HPS can detect SIMPs through the decay of a dark vector boson (either a dark ¿ or ¿) into e+e- pairs. I obtain exclusion contours for SIMPs using both an optimized cuts-based selection and a machine-learning-based selection, advancing our knowledge of the nature of dark matter.

O'Dwyer, Rory [Stanford Univ., CA (United States).↗
DOE OSTI2021

Fischer-Tropsch Synthesis: The Characterization and Testing of Pt-Co/SiO 2 Catalysts Prepared with Alternative Cobalt Precursors

Different low-cost cobalt precursors (acetate, chloride) and thermal treatments (air calcination/H 2 reduction versus direct H 2 -activation) were investigated to alter the interaction between cobalt and silica. H 2 -activated catalysts prepared from cobalt chloride had large Co 0 particles (XRD, chemisorption) formed by weak interactions between cobalt chloride and silica (temperature programmed reduction (TPR), TPR with mass spectrometry (TPR-MS), TPR with extended X-ray absorption fine structure (EXAFS) and X-ray absorption near edge spectroscopy (XANES) techniques) and retained Cl-blocked active sites, resulting in poor activity. In contrast, unpromoted Co/SiO 2 catalysts derived from cobalt acetate had strong interactions between Co species and silica (TPR/TPR-MS, TPR-EXAFS/XANES); adding Pt increased the extent of the Co reduction. For these Pt-promoted catalysts, the reduction of uncalcined catalysts was faster, resulting in larger Co 0 clusters (19.5 nm) in comparison with the air-calcined/H 2 -activated catalyst (7.8 nm). Both catalysts had CO conversions 25% higher than that of the Pt-promoted catalyst prepared in the traditional manner (air calcination/H 2 reduction using cobalt nitrate) and three times higher than that of the traditional unpromoted Co/silica catalyst. The retention of residual cobalt carbide (observed in XANES) from cobalt acetate decomposition impacted performance, resulting in a higher C 1 –C 4 selectivity (32.2% for air-calcined and 38.7% for uncalcined) than that of traditional catalysts (17.5–18.6%). The residual carbide also lowered the α-value and olefin/paraffin ratio. Future work will focus on improving selectivity through oxidation–reduction cycles.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

A study of events with photoelectric emission in the DarkSide-50 liquid argon Time Projection Chamber

Finding unequivocal evidence of dark matter interactions in a particle detector is a major goal of research in physics. Liquid argon time projection chambers offer a path to probe Weakly Interacting Massive Particles scattering cross sections on nuclei down to the so-called neutrino floor, in a mass range from a few GeV to hundreds of TeV. Based on the successful operation of the DarkSide-50 detector at LNGS, a new and more sensitive experiment, DarkSide-20k, has been designed and is now under construction. A thorough understanding of the DarkSide-50 detector response and, therefore, of all types of events observed in the detector, is essential for the optimal design of the new experiment. In this article, we report on a specific set of events, namely, standard two-pulse scintillation–ionization signals with a third small amplitude pulse, occurring within the 440 μ s data acquisition window of standard events. Some of these events are due to the photoionization of the TPC cathode. We compare our results with those published by collaborations using liquid xenon time projection chambers, which observed a similar phenomenon, and, in particular, with a recent paper by the LUX Collaboration (D.S. Akerib et al. Phys.Rev.D 102, 092004 (2020)) From the measured rate of these events, we estimate for the first time the quantum efficiency of the tetraphenyl butadiene deposited on the DarkSide-50 cathode at wavelengths of around 128 nm, in liquid argon. Also, both experiments observe events likely related to the photoionization of impurities in the liquid. The probability of photoelectron emission per unit length turns out to be an order of magnitude lower in DarkSide-50 than in LUX.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Rapid Acceleration of Outcomes in Physics: Final Report for the Nuclear Physics, Particle Physics, Astrophysics, and Cosmology (NPAC) Umbrella Project

The Nuclear Physics, Particle Physics, Astrophysics, and Cosmology (NPAC) Initiative addresses the first question by supporting experiments that would directly detect dark matter when it interacts with very sensitive detectors. There are two leading candidates for dark matter that are plausibly detectable in terrestrial searches: axions and weakly-interacting massive particles, or WIMPs. Early NPAC investments supported PNNL involvement in the Axion Dark Matter eXperiment (ADMX), which has produced the world’s most sensitive axion search to date. Work associated with the current generation of the experiment is funded by the DOE Office of High Energy Physics (HEP), while R&D toward future searches for higher mass axions proceeds under NPAC. Likewise, early NPAC support for WIMP searches has graduated to the HEP-supported Super Cold Dark Matter Search (SuperCDMS) experiment. SuperCDMS has produced world-leading limits on potential WIMP candidates as well as a number of other exotic candidates and processes.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Weak scale as a trigger

Does the value of the Higgs mass parameter affect the expectation value of local operators in the Standard Model? For essentially all local operators the answer to this question is "no", and this is one of the avatars of the hierarchy problem: nothing is "triggered" when the Higgs mass parameter crosses zero. In this letter, we explore settings in which Higgs mass parameters $can$ act as a "trigger" for some local operators ${\cal O}_T$. In the Standard Model, this happens for ${\cal O}_T = {\rm Tr} (G \tilde G)$. We also introduce a "type-0" two Higgs doublet model, with a $Z_4$ symmetry, for which ${\cal O}_T = H_1 H_2$ is triggered by the Higgs masses, demanding the existence of new Higgs states necessarily comparable to or lighter than the weak scale, with no wiggle room to decouple them whatsoever. Surprisingly, this model is not yet entirely excluded by collider searches, and will be incisively probed by the high-luminosity run of the LHC, as well as future Higgs factories. We also discuss a possibility for using this trigger to explain the origin of the weak scale, invoking a landscape of extremely light, weakly interacting scalars $\phi_i$, with a coupling to ${\cal O}_T$ needed to make it possible to find vacua with small enough cosmological constant. The weak scale trigger links the tuning of the Higgs mass to that of the cosmological constant, while coherent oscillations of the $\phi_i$ can constitute dark matter.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

On the stability of the open-string QED neutron and dark matter

We study the stability of a hypothetical QED neutron, which consists of a color-singlet system of two d quarks and a u quark interacting with the QED interaction. As a quark cannot be isolated, the intrinsic motion of the three quarks in the lowest-energy state may lie predominantly in 1 + 1 dimensions, as in a d-u-d open string. The attractive d-u and u-d QED interactions may overcome the weaker repulsive d-d QED interaction to bind the three quarks together. We examine the QED neutron in a phenomenological three-body problem in 1 + 1 dimensions with an effective interaction extracted from Schwinger’s exact QED solution in 1 + 1 dimensions. The phenomenological model in a variational calculation yields a stable QED neutron at 44.5 MeV. The analogous QED proton with two u quarks and a d quark has been found to be too repulsive to be stable and does not have a bound or continuum state, onto which the QED neutron can decay via the weak interaction. Consequently, the QED neutron is stable against the weak decay, has a long lifetime, and is in fact a QED dark neutron. It may be produced following the deconfinement-to-confinement phase transition of the quark gluon plasma in high-energy heavy-ion collisions. Because of the long lifetime of the QED dark neutron, self-gravitating assemblies of QED dark neutrons or dark antineutrons may be good candidates for a part of the primordial dark matter produced during the phase transition of the quark gluon plasma in the evolution of the early Universe.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Study of few-electron backgrounds in the LUX-ZEPLIN detector

The LUX-ZEPLIN (LZ) experiment aims to detect rare interactions between dark matter particles and xenon. Although the detector is designed to be the most sensitive to GeV/𝑐 2 –TeV/𝑐 2 weakly interacting massive particles (WIMPs), it is also capable of measuring low-energy ionization signals down to a single electron that may be produced by scatters of sub-GeV/𝑐 2 dark matter. The major challenge in exploiting this sensitivity is to understand and suppress the ionization background in the few-electron regime. We report a characterization of the delayed electron backgrounds following energy depositions in the LZ detector under different detector conditions. In addition, we quantify the probability for photons to be emitted in coincidence with electron emission from the high voltage grids. We then demonstrate that spontaneous grid electron emission can be identified and rejected with a high efficiency using a coincident photon tag, which provides a tool to improve the sensitivity of future dark matter searches.

Akerib, D. S. [SLAC National Accelerator Laborator↗
DOE OSTI2024

Peter Higgs (1929–2024)

Peter Ware Higgs, a particle physics icon, died on 8 April at the age of 94. Higgs illuminated the path to understanding how exact symmetries obeyed by the laws of nature might be masked by an asymmetric ground state that is an outcome of symmetrical laws. In 1964, he posited that a field filling all of space could be the agent that hides the underlying symmetries of the fundamental interactions. Additionally, when excited, the field reveals itself as a massive unstable particle. In the context of a joint theory of electromagnetism and the weak interaction, that particle—popularly called the Higgs boson—emerged as the keystone of the standard model of particle physics. The decades-long search for the boson engaged the passion of thousands of scientists and engineers and stirred the curiosity of the public the world over.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS2002

A Proposed Model for Protein Crystal Nucleation and Growth

How does one take a molecule, strongly asymmetric in both shape and charge distribution, and assemble it into a crystal? We propose a model for the nucleation and crystal growth process for tetragonal lysozyme, based upon fluorescence, light, neutron, and X-ray scattering data, size exclusion chromatography experiments, dialysis kinetics, AFM, and modeling of growth rate data, from this and other laboratories. The first species formed is postulated to be a 'head to side' dimer. Through repeating associations involving the same intermolecular interactions this grows to a 4(sub 3) helix structure, that in turn serves as the basic unit for nucleation and subsequent crystal growth. High salt attenuates surface charges while promoting hydrophobic interactions. Symmetry facilitates subsequent helix-helix self-association. Assembly stability is enhanced when a four helix structure is obtained, with each bound to two neighbors. Only two unique interactions are required. The first are those for helix formation, where the dominant interaction is the intermolecular bridging anion. The second is the anti-parallel side-by-side helix-helix interaction, guided by alternating pairs of symmetry related salt bridges along each side. At this stage all eight unique positions of the P4(sub3)2(sub 1),2(sub 1) unit cell are filled. The process is one of a) attenuating the most strongly interacting groups, such that b) the molecules begin to self-associate in defined patterns, so that c) symmetry is obtained, which d) propagates as a growing crystal. Simple and conceptually obvious in hindsight, this tells much about what we are empirically doing when we crystallize macromolecules. By adjusting the growth parameters we are empirically balancing the intermolecular interactions, preferentially attenuating the dominant strong (for lysozyme the charged groups) while strengthening the lesser strong (hydrophobic) interactions. In the general case for proteins the lack of a singularly defined association pathway may lead to formation of multiple species, i.e., amorphous precipitation. Weak interactions, such as hydrogen bonds, are promiscuous, serving to strengthen rather than define specific interactions. Participation in an interaction sequesters that surface from subsequent interactions, and we expect the strongest bonds to form first. This model, its basis, how it fits into the currently understood osmotic second virial coefficient approach to crystallization, and what it suggests will be discussed.

Pusey, Marc↗
DOE OSTI2024

Single-Molecule Detection of the Encounter and Productive Electron Transfer Complexes of a Photosynthetic Reaction Center

Small, diffusible redox proteins play an essential role in electron transfer (ET) in respiration and photosynthesis, sustaining life on Earth by shuttling electrons between membrane-bound complexes via finely tuned and reversible interactions. Ensemble kinetic studies show transient ET complexes form in two distinct stages: an “encounter” complex largely mediated by electrostatic interactions, which subsequently, through subtle reorganization of the binding interface, forms a “productive” ET complex stabilized by additional hydrophobic interactions around the redox-active cofactors. Here, using single-molecule force spectroscopy (SMFS) we dissected the transient ET complexes formed between the photosynthetic reaction center-light harvesting complex 1 (RC-LH1) of Rhodobacter sphaeroides and its native electron donor cytochrome c 2 (cyt c 2 ). Importantly, SMFS resolves the distribution of interaction forces into low (~150 pN) and high (~330 pN) components, with the former more susceptible to salt concentration and to alteration of key charged residues on the RC. Thus, the low force component is suggested to reflect the contribution of electrostatic interactions in forming the initial encounter complex, whereas the high force component reflects the additional stabilization provided by hydrophobic interactions to the productive ET complex. Employing molecular dynamics simulations, we resolve five intermediate states that comprise the encounter, productive ET and leaving complexes, predicting a weak interaction between cyt c 2 and the LH1 ring near the RC-L subunit that could lie along the exit path for oxidized cyt c 2 . The multimodal nature of the interactions of ET complexes captured here may have wider implications for ET in all domains of life.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Quasiparticle Energy Relaxation in a Gas of One-Dimensional Fermions with Coulomb Interaction

We consider a system of charged one-dimensional spin-1/2 fermions at low temperature. We study how the energy of a highly excited quasiparticle (or hole) relaxes toward the chemical potential in the regime of weak interactions. The dominant relaxation processes involve collisions with two other fermions. We find a dramatic enhancement of the relaxation rate at low energies, with the rate scaling as the inverse sixth power of the excitation energy. Furthermore, this behavior is caused by the long-range nature of the Coulomb interaction.

1-dimensional systems↗
DOE OSTI2020

C HIMERA : A Massively Parallel Code for Core-collapse Supernova Simulations

Herein we provide a detailed description of the C HIMERA code, a code developed to model core collapse supernovae (CCSNe) in multiple spatial dimensions. The CCSN explosion mechanism remains the subject of intense research. Progress to date demonstrates that it involves a complex interplay of neutrino production, transport, and interaction in the stellar core, three-dimensional stellar core fluid dynamics and its associated instabilities, nuclear burning, and the fundamental physics of the neutrino–stellar core weak interactions and the equations of state of all stellar core constituents—particularly, the nuclear equation of state associated with core nucleons, both free and bound in nuclei. C HIMERA , by incorporating detailed neutrino transport, realistic neutrino–matter interactions, three-dimensional hydrodynamics, realistic nuclear, leptonic, and photonic equations of state, and a nuclear reaction network, along with other refinements, can be used to study the role of neutrino radiation, hydrodynamic instabilities, and a variety of input physics in the explosion mechanism itself. It can also be used to compute observables such as neutrino signatures, gravitational radiation, and the products of nucleosynthesis associated with CCSNe. The code contains modules for neutrino transport, multidimensional compressible hydrodynamics, nuclear reactions, a variety of neutrino interactions, equations of state, and modules to provide data for post-processing observables such as the products of nucleosynthesis, and gravitational radiation. C HIMERA is an evolving code, being updated periodically with improved input physics and numerical refinements. We detail here the current version of the code, from which future improvements will stem, which can in turn be described as needed in future publications.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Polycaprolactone: A Promising Addition to the Sequential Infiltration Synthesis Polymer Family Identified through In Situ Infrared Spectroscopy

Infiltration of inorganic oxides inside polymers using sequential infiltration synthesis (SIS) is an effective method for creating materials for a broad range of applications. The reactions between various polymer functional groups and organometallic/inorganic precursors are unique, which makes it essential to understand the specific interactions for a range of precursors and polymers to enable predictive process design and to extend the utility of SIS to applications. In this paper, in situ Fourier transform infrared spectroscopy (FTIR) measurements have been performed during Al 2 O 3 and TiO 2 SIS in three different homopolymers: poly(methyl methacrylate) (PMMA), poly(epsilon-caprolactone) (PCL), and poly(2-vinylpyridine) (P2VP). From the FTIR intensity changes after precursor exposure and during the subsequent purge times, it is demonstrated quantitatively that the interaction dynamics and the stability of the intermediate complexes of these polymers with the metal precursors are substantially different. A key finding from this comparative study is that PCL interacts far more strongly with metal precursors, even though its carbonyl (C=O) and ester (C-O-R) functional groups are similar to those of the more weakly interacting PMMA. This behavior suggests that additional factors beyond the identity of the functional groups dictate how polymers interact with metal compounds in SIS. PCL, which has not previously been reported in SIS processes, may be an attractive polymeric template for implementing SIS with improved uniformity and cost-effectiveness.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Global anomalies of Green's function zeros.

We study global anomalies of nonlocal effective theories proposed to describe symmetry-preserving Luttinger surfaces, i.e., the momentum-space manifolds of Green’s function zeros (GFZs) at zero energy, in strongly interacting fermionic systems. In particular, we focus on the simplest possible cases associated with a gapless Dirac zero, which is the counterpart of the gapless Dirac quasiparticle in weakly interacting systems. These theories may be derived by integrating out low-energy degrees of freedom that do not couple to the relevant gauge field. We discuss the global anomaly, the bulk-boundary correspondence, and the constraint on phases consistent with the anomaly, such as non-Fermi liquids and emergent gapless quasiparticles on Luttinger surfaces. Failing to avoid spontaneous symmetry breaking in the thermodynamical limit inevitably leads to unstable GFZs. We also provide some perspective on why the related nonlocal fermionic effective theory studied recently is not a suitable starting point for a symmetrically gapped phase

Su, Lei↗
DOE OSTI2022

Enhancing Li + Transport in NMC811||Graphite Lithium–Ion Batteries at Low Temperatures by Using Low–Polarity–Solvent Electrolytes

LiNi x Co y MnzO 2 (x+y+z=1)||graphite lithium-ion battery (LIB) chemistry promises practical applications. However, its low-temperature (≤ –20°C) performance is poor because the increased resistance encountered by Li + transport in and across the bulk electrolytes and the electrolyte/electrode interphases induces capacity loss and battery failures. Though tremendous efforts have been made, there is still no effective way to reduce the charge transfer resistance (R ct ) which dominates low-temperature LIBs performance. In this work, we propose a strategy of using low-polarity-solvent electrolytes which have weak interactions between the solvents and the Li + to reduce R ct , achieving facile Li + transport at sub-zero temperatures. The exemplary electrolyte enables LiNi 0.8 Mn 0.1 Co 0.1 O 2 ||graphite cells to deliver a capacity of ≈113 mAh g –1 (98% full-cell capacity) at 25°C and to remain 82% of their room-temperature capacity at –20°C without lithium plating at 1/3C. They also retain 84% of their capacity at –30°C and 78% of their capacity at –40°C and show stable cycling at 50°C.

25 ENERGY STORAGE↗
DOE OSTI2023

Topological order in interacting semimetals

It has recently been demonstrated that it is possible to open a gap in a magnetic Weyl semimetal, while preserving the chiral anomaly along with the charge conservation and translational symmetries, which all protect the gapless nodes in a weakly interacting semimetal. The resulting state was shown to be a nontrivial generalization of a non-Abelian fractional quantum Hall liquid to three dimensions. Here we point out that a second fractional quantum Hall state exists in this case. This state has exactly the same electrical and thermal Hall responses as the first, but a distinct (fracton) topological order. Moreover, the existence of this second fractional quantum Hall state necessarily implies a gapless phase, which has identical topological response to a noninteracting Weyl semimetal, but is distinct from it. Here, this may be viewed as a generalization (in a weaker form) of the known duality between a noninteracting two-dimensional Dirac fermion and QED 3 to 3+1 dimensions. In addition we discuss a (3+1)-dimensional topologically ordered state, obtained by gapping a nodal line semimetal without breaking symmetries.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1980

Viscous-inviscid calculations of jet entrainment effects on the subsonic flow over nozzle afterbodies

A viscous-inviscid interaction model was developed to account for jet entrainment effects in the prediction of the subsonic flow over nozzle afterbodies. The model is based on the concept of a weakly interacting shear layer in which the local streamline deflections due to entrainment are accounted for by a displacement-thickness type of correction to the inviscid plume boundary. The entire flow field is solved in an iterative manner to account for the effects on the inviscid external flow of the turbulent boundary layer, turbulent mixing and chemical reactions in the shear layer, and the inviscid jet exhaust flow. The components of the computational model are described, and numerical results are presented to illustrate the interactive effects of entrainment on the overall flow structure. The validity of the model is assessed by comparisons with data obtained form flow-field measurements on cold-air jet exhausts. Numerical results and experimental data are also given to show the entrainment effects on nozzle boattail drag under various jet exhaust and free-stream flow conditions.

Wilmoth, R. G.↗