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NASA NTRS2006

Constraints from Comets

Crystalline silicates identified in the laboratory examinations of cometary interplanetary dust particles, in Stardust particles, and in the IR spectra of comets and protoplanetary disks typically have high Mg and low Fe contents. In contrast, the amorphous silicates in IDPs and comets are predominantly Fe-rich. Mg-rich crystalline silicates are hypothesized to form by heating of amorphous silicates at temperatures above 1000 K. Annealing does not change the stoichiometry, i.e., the chemistry of the grains. Therefore, annealing is not expected to change an Fe-bearing amorphous silicate into a Mg-rich crystal. We discuss this challenge to the annealing scenario, review the condensation scenarios, and discuss the possibility that Fe reduction, a process thought to contribute in chondrule-formation, is the missing link between Fe-rich amorphous silicates and Mg rich crystalline silicates. We discuss the time scales for these processes in terms of time dependent 2D models of disks (by Gail & collaborators) and in terms of shocks. We mention the Stardust sample return results on Mg-rich crystalline silicates.

Wooden, Diane H.↗
NASA NTRS2007

The Mineralogy of Comet Wild-2 Nucleus Samples - What We Think We Know And What We Do Not Know

The sample return capsule of the Stardust spacecraft was successfully recovered in northern Utah on January 15, 2006, and its cargo of coma grains from Comet Wild-2 has now been the subject of intense investigation by approximately 200 scientists scattered across five continents. We can now perform mineralogical and petrographic analyses of particles derived directly from the Jupiter-family Comet Wild-2

Zolensky, Michael E.↗
NASA NTRS2005

Chandra Observations of Comet 2P/Encke 2003: First Detection of a Collisionally Thin, Fast Solar Wind Charge Exchange System

We report the results of 15 hr of Chandra observations of comet 2P/Encke 2003 on November 24. X-ray emission from comet Encke was resolved on scales of 500-40,000 km, with unusual morphology due to the presence of a low-density, collisionally thin (to charge exchange) coma. A light curve with peak-to-peak amplitude of 20% consistent with a nucleus rotational period of 11.1 hr was found, further evidence for a collisionally thin coma. We confirm emission lines due to oxygen and neon in the 800-1000 eV range but find very unusual oxygen and carbon line ratios in the 200-700 eV range, evidence for low-density, high effective temperature solar wind composition. We compare the X-ray spectral observation results to contemporaneous measurements of the coma and solar wind made by other means and find good evidence for the dominance of a postshock bubble of expanding solar wind plasma, moving at 600 km/s with charge state composition between that of the "fast" and "slow" solar winds.

Lisse, C. M.↗
NASA NTRS2007

The Mineralogy of Comet Wild 2

The nature of cometary solids is of fundamental importance to our understanding of the early solar nebula and protoplanetary history. Samples of Comet Wild 2, provided by the Stardust Mission, have now been examined in terrestrial labs for two years, and are very surprising! Here we describe mainly the critical phases olivine, pyroxene and Fe-Ni sulfides in Wild 2 grains, as a guide to the general mineralogy of the returned comet samples.

Zolensky, Michael↗
NASA NTRS2008

Mineralogy, Three Dimensional Structure, and Oxygen Isotope Ratios of Four Crystalline Particles from Comet 81P/Wild 2

Preliminary examinations of small dust particles from comet 82P/Wild 2 revealed many expected and unexpected features. Among them the most striking feature is the presence of abundant crystalline material in the comet. Synchrotron radiation X-ray diffraction and microtomography are the most efficient methods to detect and describe bulk mineralogical features of crystalline cometary particles. In the present study, in addition to these two non-destructive techniques, electron microscopy and ion-probe mass spectrometry were carried out on the four crystalline particles.

Nakamura, T.↗
NASA NTRS2010

Isotopic Fractionation in Comets: Quantifying the Contribution of Interstellar Chemistry

Anomalously fractionated isotopic material is found in many primitive Solar System objects, such as meteorites and comets. It is thought, in some cases, to trace interstellar matter that was incorporated into the Solar Nebula without undergoing significant processing. We will present the results of models of the nitrogen, oxygen, and carbon fractionation chemistry in dense molecular clouds, particularly in cares where substantial freeze-taut of molecules on to dust has occurred. The range of fractionation ratios expected in different interstellar molecules will be discussed and compared to the ratios measured in molecular clouds, comets and meteoritic material. These models make several predictions that can be tested in the near future by molecular line observations, particularly with the GBT.

Charnley, Steven↗
NASA NTRS2010

Comparison of the Mineralogy of Comet Wild 2 Coma Grains to Other Astromaterials

We propose that Kuiper Belt samples (in this case comet coma grains from the Jupiter family comet Wild 2) are recognizably different from the bulk of materials in outer belt asteroids, because of their different formation positions and times in the early solar system. We believe this despite similarities found between some Wild 2 grains and components of carbonaceous chondrites (i.e. some CAI and chondrules). Kuiper Belt samples must preserve measurable mineralogical and compositional evidence of formation at unique positions and times in the early solar nebula, and these formational differences must have imparted recognizable special characteristics. We hypothesize that these characteristics include: (1) Unique major element compositional ranges of common astromaterial minerals, especially olivine and pyroxene; (2) Unique minor element compositions of major silicate phases, especially olivine and low-Ca pyroxene; (3) Degree and effects of radiation processing -- including amorphous rims, metal coatings, and Glass with Embedded Metal and Sulfides (GEMS); (4) Presence of abundant presolar silicate grains as recognized by anomalous oxygen in silicates; (5) Oxidation state of the mineral assemblage. We are working our way through all available Wild 2 samples, selecting 1-2 non-consecutive viable TEM grids from each possible extracted Wild 2 grain. We especially prefer TEM grids from grains for which complete mineralogical details have not been published (which is to say the majority of the extracted grains). We are performing a basic mineralogic survey by E-beam techniques, to establish the essential features of the extracted Wild 2 grains. We are making a particular effort to carefully and accurately measure minor elements of olivine and pyroxene, as these minerals are widespread in astromaterials, and comparisons of their compositions will serve to place the Wild 2 silicates in contact with asteroids, meteorites and chondritic interplanetary dust particles processing. We are also making a special effort to search for mineralogical products of aqueous alteration, since their presence would reveal that Wild 2 was once internally heated, a result with dramatic implications for models of early solar system primitive bodies. Thus far carbonates are the only potential evidence for aqueous alteration for Wild 2.

Frank, David↗
NASA NTRS2010

Millimeter and Submillimeter Observations of Comet 103P/Hartley 2

The close approach (0.12 AU) of Comet 103P/Hartley 2 to the Earth only S days prior to perihelion provides a unique opportunity to probe the chemical composition of this object. We will employ the Arizona Radio Observatory's Kitt Peak 12m (KPH12M) and the Submillimeter Telescope (SMT) for observations of multiple molecular species and their isotopologs towards the comet. There will also be an attempt to monitor this object during the EPOXI (Extrasolar Planet Observation. and Deep Impact Extended Investigation) flyby mission, which will obtain high resolution infrared spectra, for a comparison of the molecular inventory and a more accurate assessment of the abundances, sources (e.g. jets or cometismals), and chemistry.

Milan, S. N.↗
NASA NTRS2010

Highly Depleted Ethane and Slightly Depleted Methanol in Comet 21P/Giacobini-Zinner: Application of Empirical g-Factors for CH3OH Near 50K

We report high resolution (lambda/delta lambda approximately 24,000) observations of Comet 21 P/Giacobini-Zinner (21P) between approximately 2.85 -- 3.54 micrometers, obtained with NIRSPEC at Keck 2 on UT 2005 June 03 (R(sub h) = 1.12 AU, delta = 1.45 AU). These simultaneously sampled multiple emissions from the v7 band of C2H6 and the v2 and v3 bands of CH3OH, together with several hot bands of H2O, permitting a direct measure of parent volatile abundances in 21P. Our spectra reveal highly depleted C2H6 (0.13-0.14 percent relative to H2O) and CH3OH/C2H6 approximately 10, consistent with previously published abundances from observations in the IR [1,2] and millimeter sub-mm (reporting CH3OH/H2O [3]) during its previous apparition in 1998. We observed similarly high CH3OH/C2H6, and also similar rotational temperature to that measured for 21 P, in Comet 8P/Tuttle [4,5]. We used our (higher signal-to-noise) NIRSPEC observations of 8P to produce effective (empirical) CH3OH g-factors for several lines in the v2 band. These will be presented together with interpretation of our results, including constraints on the spin temperature of water. We acknowledge support from the NASA Planetary Atmospheres, Planetary Astronomy, and Astrobiology Programs and from the NSF Astronomy and Astrophysics Research Grants Program.

DiSanti, Michael A.↗
NASA NTRS2011

Primary Volatiles During the 2010 Apparition of Comet 103P/Hartley-2 as Revealed at Infrared Wavelengths: Production Rates and Spatial Profiles

We acquired high resolution near-infrared spectra of comet 103P/Hartley-2 with NIRSPEC at the W. M. Keck Observatory and CRIRES at the ESO VLT, emphasizing primary volatiles before, during, and after the comet's close approach to Earth (July-December 2010; R(sub h) =1.62 right arrow 1.26 AU). We will present the mixing ratios for trace volatiles (C2H6, HCN, CH3OH, etc.), their rotational temperatures, and their spatial distributions in the coma both along the polar jet (UT 19.5 October) and nearly orthogonal to the jet (UT 22.5 October).

Mumma, M. J.↗
NASA NTRS2011

Centimeter, Millimeter, and Submillimeter Observations of Comet l03P/Hartley 2

The close approach (0.12 AU) of Comet 103P/Hartley 2 to the Earth only 8 days prior to perihelion provided a unique opportunity to probe the chemical composition of this object. Additionally, supporting data was acquired during the EPOXI (Extrasolar Planet Observation and Deep Impact Extended Investigation) flyby mission [1], which provided high resolution infrared spectra and images. Observations were conducted from four facilities, contributing to the large ground-based consortium organized in support of the EPOXI mission [2]. The Arizona Radio Observatory's 12m telescope, Kitt Peak, AZ, and Submillimeter telescope, Mt. Graham, AZ, as well as the James Clerk Maxwell Telescope, Mauna Kea, HI and the Greenbank 100m telescope, Greenbank, WV, were employed for this study covering 20 cm, 3 cm, and 0.8-3 mm. Data were obtained, collectively, from 12 October 2010 to 5 November 2010 [3]. HCN, CH3OH, H2CO, HNC, OH, and CS were detected, and upper limits on the abundance of H2S, SO2, c-C3H2, and deuterated isotopologues of HCN, H2CO, and H2O were measured. Upper limits on the D/H ratio derived from DCN gave D/H less than 0.01[3]. Detailed analysis of these data will help constrain the temperature, abundances, variance or periodicity of a given species, and can be compared to results from other comets, as well as support the data obtained from the EPOXI mission. The full analysis and comparison will be presented.

Milam, Stefanie N.↗
NASA NTRS2011

Surface Contact Model for Comets and Asteroids

A contact force model was developed for use in touch and go (TAG) surface sampling simulations on small celestial bodies such as comets and asteroids. In TAG scenarios, a spacecraft descending toward the surface of a small body comes into contact with the surface for a short duration of time, collects material samples with a sampler device, and then ascends to leave the surface. The surface contact required 6-DOF (degrees of freedom) dynamics models due to coupling of the attitude and translation dynamics during the contact. The model described here is for contact scenarios that utilize a rotating brush wheel sampler (BWS) to collect surface material. The model includes stiffness and damping of the surface material during BWS vertical motion, lateral friction from the BWS dragging across the surface, and lateral shear from the rotating BWS scooping the surface material. This model is useful for any mission to asteroids or comets that incorporates surface sampling operations.

Blackmore, Lars James C.↗
NASA NTRS2011

Laboratory Studies of Fischer-Tropsch-Type Reactions and Their Implications for Organics in Asteroids and Comets

We have been studying Fischer-Tropsch type (FTT) reactions as a source for organic materials both in the gas phase of the solar nebula and incorporated into primitive comets and asteroids for almost 10 years, and over this time our concept has evolved greatly from the standard "catalytic" model to a much more robust chemical scenario. Our simulations have been conducted at temperatures that are much higher than we like, primarily for practical reasons such as the timescale of individual reactions, and we are just starting a series of measurements to allow us to measure reaction rates at temperatures from 873K down to as low as 373K. We have preliminary data on the carbon (d13C = -50) & nitrogen (d15N = +9.5) isotopic fractionation at 873K, but not on materials produced at lower temperature. Isotope values are on the VPDB scale for carbon and vs. Air for nitrogen. We have also investigated the noble gas trapping efficiency of the FTT process by adding a small amount of a noble gas mix to our standard synthesis mix. The noble gas ratio is 49:49:1:1::Ne:Ar:Kr:Xe. Xe and Kr are trapped at 873K and are more efficiently trapped at 673K with no isotopic fractionation at either temperature. Ar trapping is detected at 673K, but not at 873K. Ne has not yet been observed in our samples. The solar nebula was an extremely complex system, mixing materials from the innermost regions out to well into the zones where comets formed and thus mixing highly processed nebular materials with grains and coatings formed before the nebula began to collapse. Laboratory studies may provide the means to separate such diverse components based on carbon or nitrogen isotopic fractionation or the quantities of noble gases trapped in grain coatings and their thermal release patterns, among other observables. The ultimate goal of laboratory synthesis of nebular analogs is to provide the means to identifY the conditions under which natural samples were formed and the signatures of subsequent metamorphic events.

Nuth, Joseph↗
NASA NTRS2012

Dynamics of Dust Particles Released from Oort Cloud Comets and Their Contribution to Radar Meteors

The Oort Cloud Comets (OCCs), exemplified by the Great Comet of 1997 (Hale-Bopp), are occasional visitors from the heatless periphery of the solar system. Previous works hypothesized that a great majority of OCCs must physically disrupt after one or two passages through the inner solar system, where strong thermal gradients can cause phase transitions or volatile pressure buildup. Here we study the fate of small debris particles produced by OCC disruptions to determine whether the imprints of a hypothetical population of OCC meteoroids can be found in the existing meteor radar data. We find that OCC particles with diameters D < or approx. 10 microns are blown out from the solar system by radiation pressure, while those with D > or approx. 1 mm have a very low Earth-impact probability. The intermediate particle sizes, D approx. 100 microns represent a sweet spot. About 1% of these particles orbitally evolve by Poynting-Robertson drag to reach orbits with semimajor axis a approx. 1 AU. They are expected to produce meteors with radiants near the apex of the Earth s orbital motion. We find that the model distributions of their impact speeds and orbits provide a good match to radar observations of apex meteors, except for the eccentricity distribution, which is more skewed toward e approx. 1 in our model. Finally, we propose an explanation for the long-standing problem in meteor science related to the relative strength of apex and helion/antihelion sources. As we show in detail, the observed trend, with the apex meteors being more prominent in observations of highly sensitive radars, can be related to orbital dynamics of particles released on the long-period orbits.

Nesvorny, David↗
NASA NTRS2011

Crystalline Silicates in Comets: Modeling Irregularly-Shaped Forsterite Crystals and Its Implications on Condensation Conditions

Crystalline silicates in comets are a product of the condensation in the hot inner regions (T > or approx. equals 1400 K [1]) of our proto-planetary disk or annealing at somewhat lower temperatures (T > or approx. equals 1000-1200 K) [2, 3, 4] in shocks coupled with disk evolutionary processes that include radial transport of crystals from their formation locations out to the cold outer regions where comet nuclei formed. The grain shape of forsterite (crystals) could be indicative of their formation pathways at high temperatures through vapor-solid condensation or at lower temperatures through vapor-liquid-solid formation and growth [5, 6, 7]. Experiments demonstrate that crystals that formed from a rapidly cooled highly supersaturated silicate vapor are characterized by bulky, platy, columnar/needle and droplet shapes for values of temperature and supersaturation, T and sigma, of 1000-1450 C and < 97, 700-1000 C and 97-161, 580-820 C and 131-230, and <500 C and > 230, respectively [7]. The experimental columnar/needle shapes, which form by vapor-liquid-solid at lower temperatures (<820 C), are extended stacks of plates, where the extension is not correlated with an axial direction: columnar/needles may be extended in the c-axis or a-axis direction, can change directions, and/or are off-kilter or a bit askew extending in a combination of the a- and c-axis direction.

Wooden, Diane H.↗
NASA NTRS2012

Collisional Histories of Comets and Trojan Asteroids: Insights from Forsterite and Enstatite Impact Studies

Impacts into forsterite and orthoenstatite at speeds typically encountered by comets demonstrate that shock imparted by collisions is detectable in the infrared signatures of their dust. The spectral signatures can be traced to physical alterations in their crystalline structures, as observed in TEM imaging and modeled using a dipole approximation. These results yield tantalizing insights into the collisional history of our solar system, as well as the history of individual comets and Trojan asteroids.

Lederer. S. M.↗
NASA NTRS2012

Amino Acids in Asteroids and Comets: Implications for the Origin of Life on Earth and Possibly Elsewhere

Meteorites provide a record of the chemical processes that occurred in the early solar system before life began on Earth. The delivery of organic matter by asteroids, comets, and their fragments to the Earth and other planetary bodies in our solar system could have been an important source of the prebiotic organic inventory needed for the emergence of life. Amino acids are essential components of proteins and enzymes in life on Earth and these prebiotic organic compounds have been detected in a wide variety of carbon-rich meteorites, the majority of which have been determined to be extraterrestrial in origin. In addition, many amino acids are structurally chiral (they possess handedness) and with a few very rare exceptions, only left handed (L) amino acids are found in biology, while all known abiotic syntheses of amino acids result in equal mixtures of left and right handed (L~D) amino acids. The discovery of a significant left handed amino acid imbalance of up to 20% in several different carbonaceous meteorites, could point toward a possible prebiotic contribution to the origin of biological homochirality by the exogenous delivery of extraterrestrial organic material to the early Earth. In this talk, I will focus on recent state-of-the-art measurements of the distribution, chirality, and isotopic composition of amino acids in meteorites and cometary samples carried out at the Goddard Astrobiology Analytical Laboratory. Results from the analyses of a variety of Antarctic meteorites, samples from comet Wild 2 returned by the STARDUST mission, and meteorite fragments of asteroid 2008 TC3 called Almahata Sitta recovered from northern Sudan will be discussed

Glavin, Daniel↗
NASA NTRS2012

A Quantum Band Model of the nu3 Fundamental of Methanol (CH3OH) and Its Application to Fluorcescence Spectra of Comets

Methanol (CH3OH) radiates efficiently at infrared wavelengths, dominating the C-H stretching region in comets, yet inadequate quantum-mechanical models have imposed limits on the practical use of its emission spectra. Accordingly, we constructed a new line-by-line model for the 3 fundamental band of methanol at 2844 / cm (3.52 micron) and applied it to interpret cometary fluorescence spectra. The new model permits accurate synthesis of line-by-line spectra for a wide range of rotational temperatures, ranging from 10 K to more than 400 K.We validated the model by comparing simulations of CH3OH fluorescent emission with measured spectra of three comets (C/2001 A2 LINEAR, C/2004 Q2 Machholz and 8P/Tuttle) acquired with high-resolution infrared spectrometers at high-altitude sites. The new model accurately describes the complex emission spectrum of the nu3 band, providing distinct rotational temperatures and production rates at greatly improved confidence levels compared with results derived from earlier fluorescence models. The new model reconciles production rates measured at infrared and radio wavelengths in C/2001 A2 (LINEAR). Methanol can now be quantified with unprecedented precision and accuracy in astrophysical sources through high-dispersion spectroscopy at infrared wavelengths

Villanueva, Geronimo L.↗