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All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

DOE CESER 6 GHz Interference Study

DOE CESER has sponsored Idaho National Laboratory (INL) to conduct an objective and independent study of potential 6 GHz interference from outdoor operation of unlicensed devices in the 6 GHz band on fixed service (FS) microwave communication links operated by electrical sector incumbents in that band. INL is collaborating with University of Notre Dame (UND), Electric Power Research Institute (EPRI), Lockard & White, Southern Company, and AT&T, to gather data with real-world 6 GHz interference experiments and identify (1) the potential for interference from unlicensed devices and (2) the interference necessary to cause harm to the incumbents. In addition to the functional assessment, a security assessment of the FCC mandated Automatic Frequency Coordination (AFC) System to regulate use of unlicensed 6 GHz standard power devices is also being conducted. A major objective is to create a science-based and defensible methodology used to produce the necessary data and to derive objective conclusions. This proven methodology can then be used to produce objective data and conclusions for other spectrum bands with similar incumbent uses including 4.4 – 4.9 GHz and 7.125 – 7.4 GHz, identified in the reconciliation bill that was adopted on July 4, 2025, as well as the National Spectrum Strategy discussions that are ongoing. This report contains 6 GHz field experiments and findings in the following real-world scenarios with commercial unlicensed standard power (SP) 6 GHz devices regulated by Automated Frequency Coordination (AFC): • University of Notre Dame (UND) Stadium with a capacity of 80,000 spectators, where Wi-Fi operating in 6 GHz has been deployed recently • Southern Company 6 GHz FS microwave link between Columbus and Fortson, Georgia Following are the following key findings from this study. 1. The AFC is under-protective of FS when line-of-sight exists along the path centerline. Data collected at Southern’s 6 GHz fixed link site shows significant erosion of as much as 21.4-24.4 dB of under-protection that can lead to potential service degradation under typical operating conditions. This first key finding is most likely the result of erroneous use of the RF propagation model. INL will collaborate with EPRI and the AFC Functional Requirements Working Group to submit a change request to the WinnForum TS-1014 standard towards correct use of the propagation model by the AFC. 2. There is additive interference effect of about 3 dB from nearly equal power interferers measured from simultaneous operation of two SP AP's operating co-channel with the FS receive from different locations along the path. This second key finding should be used to add the impact of additive interference of operation of multiple APs in the same geographical area, to the next generation of AFCs. INL will collaborate with FCC on the need for the AFC to consider additive interference. We also recommend that additional experiments are conducted on 6 GHz spectrum interference to further improve the AFC operation as the number of outdoor Wi-Fi devices continues to increase. These proposed steps and recommendations will make the co-existence of the incumbents and the 6 GHz outdoor Wi-Fi providers possible without any impact on the incumbents with a win-win outcome for all.

6 GHz↗
DOE OSTI2024

A Visual Analytic Platform for Interactive Validation of Human Mobility Simulations

Human mobility insights guide domain experts in an array of decisions, including critical infrastructure design, disaster response, epidemic modeling, national security, and policy making. Due to the inherent noise and privacy concerns in real-world individual-level mobility data, it is often preferred to leverage simulators that generate synthetic mobility data instead. However, it is critical to inspect and validate the output of such simulators to ensure the synthetic data is aligned with the characteristics of the population and the area of interest known to domain experts. While there exist many quantitative approaches for validating synthetic data, we argue it is also important to also validate such data qualitatively to capture aspects that are known to domain experts but difficult to quantify. In this work, we demonstrate a visual analytic platform that empowers domain experts to interact with their simulation outputs along spatial and temporal dimensions. By augmenting automated techniques and human skills, our visual analytic platform is a step towards interactive capabilities for model steering and quality control of mobility simulators.

Monadjemi, Shayan↗
DOE OSTI2018

Unconfined Compression Results on Core from Boreholes U-15n#12 and U-15n#13, NNSS in support of SPE

The Nevada National Security Site (NNSS) serves as the geologic setting for a Source Physics Experiment (SPE) program. The SPE provides ground truth data to create and improve strong ground motion and seismic S-wave generation and propagation models. The NNSS was chosen as the test bed because it provides a variety of geologic settings ranging from relatively simple to very complex. Each series of SPE testing will comprise the setting and firing of explosive charges (source) placed in a central borehole at varying depths and recording ground motions in instrumented boreholes located in two rings around the source, positioned at different radii. Modeling using advanced simulation codes will be performed both before and after each test to predict ground response and to improve models based on acquired field data, respectively. A key component in the predictive capability and ultimate validation of the models is the full understanding of the intervening geology between the source and the instrumented boreholes including the geomechanical behavior of the site's rock/structural features. This report summarizes unconfined compression testing (UCS) from coreholes U-15n#12 and U-15n#13 and compares those datasets to UCS results from coreholes U-15n and U-15n#10. U-15n#12 corehole was drilled at -60° to the horizontal and U-15n#13 was drilled vertically in granitic rock (quartz monzonite) after the third SPE shot. Figure 1 illustrates at the surface, U 15n#12 and U-15n#13 coreholes were approximately 30 meters and 10 meters from the central SPE borehole (U-15n) respectively. Corehole U-15n#12 intersects the central SPE borehole (U 15n) at a core depth of 174 feet (approximately 150 feet vertical depth). The location of U 15n#12 and U-15n#13 is the site of the first, second and third SPE's, in Area 15 of the NNSS.

58 GEOSCIENCES↗
DOE OSTI2018

Unconfined Compression Results on Core from Borehole U-15n#10, NNSS, in support of SPE

The Nevada National Security Site (NNSS) serves as the geologic setting for a Source Physics Experiment (SPE) program. The SPE provides ground truth data to create and improve strong ground motion and seismic S-wave generation and propagation models. The NNSS was chosen as the test bed because it provides a variety of geologic settings ranging from relatively simple to very complex. Each series of SPE testing will comprise the setting and firing of explosive charges (source) placed in a central borehole at varying depths and recording ground motions in instrumented boreholes located in two rings around the source, positioned at different radii. Modeling using advanced simulation codes will be performed both before and after each test to predict ground response and to improve models based on acquired field data, respectively. A key component in the predictive capability and ultimate validation of the models is the full understanding of the intervening geology between the source and the instrumented boreholes including the geomechanical behavior of the site's rock/structural features. This memorandum reports on an initial phase of unconfined compression testing from corehole U-15n#10. Specimens tested came from the U-15n#10 core hole, which was drilled at -60° to the horizontal in granitic rock (quartz monzonite) after the second SPE shot (SPE-2). Figure 1 illustrates at the surface, the core hole was approximately 90 feet from the central SPE borehole. Corehole U 15n#10 intersects the central SPE borehole (U-15n) at a core depth of 170 feet (approximately 150 feet vertical depth) which is within the highly damaged zone of SPE-2. The U-15n#10 location is the site of the first, second and third SPE's, in Area 15 of the NNSS.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Analyzing Risks of Virtual Private Network Connections

The use of Splunk for analyzing VPN logs is an effective approach for identifying vulnerabilities in network endpoints. Splunk, a powerful platform for searching, monitoring, and analyzing machine-generated data, enables organizations to aggregate VPN logs in real-time, providing insights into network activity, user behavior, and potential security risks. By indexing VPN traffic and authentication logs, security teams can track abnormal patterns such as multiple failed login attempts, unusual IP addresses, or unexpected changes in bandwidth usage, all of which could indicate potential vulnerabilities or breaches. With Splunk’s advanced search and reporting capabilities, users can create custom dashboards and alerts to detect suspicious activities. Automated searches can flag endpoints exhibiting unusual behavior, while correlation analysis can identify links between compromised devices and broader network vulnerabilities. In particular, Splunk's machine learning capabilities can be leveraged to predict and prevent threats by identifying trends that might otherwise be missed in traditional log analysis. This proactive approach to monitoring VPN logs allows for the early detection of security weaknesses, enabling rapid response and minimizing potential damage to network integrity. By enhancing endpoint visibility, Splunk plays a crucial role in securing remote connections and safeguarding sensitive information. Additionally, Splunk’s automation and alerting features allow teams to create custom workflows that notify them of vulnerable or misconfigured endpoints identified through Shodan. This synergy between Splunk’s log analysis and Shodan’s device intelligence enhances an organization’s ability to proactively identify and mitigate security risks, improving the overall resilience of their VPN infrastructure.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2026

Myriad World Baseline: Global Geodemographic Estimates

The LandScan Myriad World Baseline (MWB) method produces global, residential (nighttime/home-location) gridded geodemographic estimates based on 5-year age/gender cohorts—at 30-arcsecond (≈1 km) resolution. MWB is designed to fill gaps where detailed, georeferenced survey data (e.g., Demographic and Health Surveys (DHS)) are missing or outdated, and to provide a baseline that can support human security analysis, including consequence assessment, “patterns of life” modeling, and scenario-based population futures. MWB’s workflow spatializes household-level age/gender characteristics from the GLOPOP-S dataset by conflating household and gridded expected relative wealth adapted from Global Gridded Relative Deprivation Index (GRDI), then adjusts them to a target year of interest. Age/gender estimates are then applied to harmonize lowest-administrative-level statistics with LandScan residential counts, yielding final geodemographic estimates. Two validation case studies are presented: Ghana (2021) and Tokyo/Kanagawa, Japan (2020), illustrating spatial variability in demographic cohorts and comparing MWB outputs to official gridded statistics. Results show close overall alignment relative to validation criteria including population pyramids and age-dependency ratios.

Tuccillo, Joe [ORNL] (ORCID:0000000259300943)↗
DOE OSTI2024

ARPA-E Grid Optimization (GO) Competition Challenge 3

Synthetic Input Data and Team Results for the GO Competition Challenge 3 for Events 1 - 4 and the Sandbox, along with problem and format descriptions and code to validate data and solutions, are available here. Data for industry scenarios will not be made public. The Grid Optimization (GO) Competition Challenge 3 focused on the security-constrained optimal power flow (SCOPF) problem. It is part of a continuing effort begun with Challenges 1 and 2, to successfully discover, develop, and test innovative and disruptive software solutions for critical energy challenges and to overcome existing barriers. The broader goal of the of the GO Competition is to accelerate the development of transformational and disruptive methods for solving problems related to the electric power grid and to provide a transparent, fair, and comprehensive evaluation of new solution methods. Challenge 3 used multiperiod dynamic markets, including advisory models for extreme weather events, day-ahead markets, and the real-time markets with an extended look-ahead. In Event 4, whose submission window was August 31-September 4, 2023, 14 teams solved for the objective values of 669 scenarios (39 scenarios required solutions both with and without line switching being allowed). The 591 synthetic scenarios from 9 network models (3.6 GB) are available here. Ten teams were funded to participate and 7 won prizes totaling $2,400,000. The largest prize ($550,000) went to Mississippi State University. An additional $600,000 was awarded in Event 3 (6/15-16/2023). No prizes were awarded in Events 1 (1/25-27/2023) or 2 (4/13-14/2023). For more information on the competition and challenge see the "GO Competition Challenge 3 Information" resource below.

ACOPF↗
DOE OSTI2024

The Evaluation of Machine Learning Techniques for Isotope Identification Contextualized by Training and Testing Spectral Similarity

Precise gamma-ray spectral analysis is crucial in high-stakes applications, such as nuclear security. Research efforts toward implementing machine learning (ML) approaches for accurate analysis are limited by the resemblance of the training data to the testing scenarios. The underlying spectral shape of synthetic data may not perfectly reflect measured configurations, and measurement campaigns may be limited by resource constraints. Consequently, ML algorithms for isotope identification must maintain accurate classification performance under domain shifts between the training and testing data. To this end, four different classifiers (Ridge, Random Forest, Extreme Gradient Boosting, and Multilayer Perceptron) were trained on the same dataset and evaluated on twelve other datasets with varying standoff distances, shielding, and background configurations. A tailored statistical approach was introduced to quantify the similarity between the training and testing configurations, which was then related to the predictive performance. Wilcoxon signed-rank tests revealed that the OVR-wrapped XGB significantly outperformed the other algorithms, with confidence levels of 99.0% or above for the 133Ba, 60Co, 137Cs, and 152Eu sources. The findings from this work are significant as they outline techniques to promote the development of robust ML-based approaches for isotope identification.

domain adaptation↗
NASA NTRS1980

Advanced communications satellites

The increase in demand for satellite communications services brought about shortages in available transponder capacity, especially at C-band. Interest shifted to the Ku-band frequency and currently carriers are rapidly moving to secure orbital slots for future satellite development. Projections of communications service demands over the next decade indiate growth in voice, data, and video services such that saturation of both C-band and Ku-band will occur by 1990. Emphasis must and will shift to Ka-band (20/30 GHz) frequency for fixed-satellite service. Advanced technologies such as multibeam antennas coupled with on-board satellite switching to allow implementation in this band of very high capacity satellite systems will be applied to meet the demand. Satellite system concepts that are likely in the 1990's and are likely to bring a new dimension to satellite delivered communication service are presented. The NASA 30/20 GHz communications satellite system demonstration program is discussed with emphasis on the related technology development.

Sivo, J. N.↗
NASA NTRS1996

Aeronautics and Space Report of the President: Fiscal Year 1996 Activities

Topics considered include: (1) Space launch activities: space shuttle missions; expendable launch vehicles. (2) Space science: astronomy and space physics; solar system exploration. (3) Space flight and technology: life and microgravity sciences; space shuttle technology; reuseable launch vehicles; international space station; energy; safety and mission assurance; commercial development and regulation of space; surveillance. (4) Space communications: communications satellites; space network; ground networks; mission control and data systems. (5) Aeronautical activities: technology developments; air traffic control and navigation; weather-related aeronautical activities; flight safety and security; aviation medicine and human factors. (6) Studies of the planet earth: terrestrial studies and applications: atmospheric studies: oceanographic studies; international aeronautical and space activities; and appendices.

Source record↗
NASA NTRS2005

Development Approach of the Advanced Life Support On-line Project Information System

The Advanced Life Support (ALS) Program has recently accelerated an effort to develop an On-line Project Information System (OPIS) for research project and technology development data centralization and sharing. There has been significant advancement in the On-line Project Information System (OPIS) over the past year (Hogan et al, 2004). This paper presents the resultant OPIS development approach. OPIS is being built as an application framework consisting of an uderlying Linux/Apache/MySQL/PHP (LAMP) stack, and supporting class libraries that provides database abstraction and automatic code generation, simplifying the ongoing development and maintenance process. Such a development approach allows for quick adaptation to serve multiple Programs, although initial deployment is for an ALS module. OPIS core functionality will involve a Web-based annual solicitation of project and technology data directly from ALS Principal Investigators (PIs) through customized data collection forms. Data provided by PIs will be reviewed by a Technical Task Monitor (TTM) before posting the information to OPIS for ALS Community viewing via the Web. Such Annual Reports will be permanent, citable references within OPIS. OPlS core functionality will also include Project Home Sites, which will allow PIS to provide updated technology information to the Community in between Annual Report updates. All data will be stored in an object-oriented relational database, created in MySQL(Reistered Trademark) and located on a secure server at NASA Ames Research Center (ARC). Upon launch, OPlS can be utilized by Managers to identify research and technology development (R&TD) gaps and to assess task performance. Analysts can employ OPlS to obtain the current, comprehensive, accurate information about advanced technologies that is required to perform trade studies of various life support system options. ALS researchers and technology developers can use OPlS to achieve an improved understanding of the NASA and ALS Program needs and to understand how other researchers and technology developers are addressing those needs. OPlS core functionality will launch for 'Ihe ALS Program in October, 2005. However, the system has been developed with the ability to evolve with Program needs. Because of open-source construction, software costs are minimized. Any functionality that is technologically feasible can be built into OPIS, and OPlS can expand through module cloning and adaptation, to any level deemed useful to the Agency.

Levri, Julie A.↗
NASA NTRS2010

Criteria for Evaluating Alternative Network and Link Layer Protocols for the NASA Constellation Program Communication Architecture

Selecting a communications and network architecture for future manned space flight requires an evaluation of the varying goals and objectives of the program, development of communications and network architecture evaluation criteria, and assessment of critical architecture trades. This paper uses Cx Program proposed exploration activities as a guideline; lunar sortie, outpost, Mars, and flexible path options are described. A set of proposed communications network architecture criteria are proposed and described. They include: interoperability, security, reliability, and ease of automating topology changes. Finally a key set of architecture options are traded including (1) multiplexing data at a common network layer vs. at the data link layer, (2) implementing multiple network layers vs. a single network layer, and (3) the use of a particular network layer protocol, primarily IPv6 vs. Delay Tolerant Networking (DTN). In summary, the protocol options are evaluated against the proposed exploration activities and their relative performance with respect to the criteria are assessed. An architectural approach which includes (a) the capability of multiplexing at both the network layer and the data link layer and (b) a single network layer for operations at each program phase, as these solutions are best suited to respond to the widest array of program needs and meet each of the evaluation criteria.

Benbenek, Daniel↗
NASA NTRS2011

Future Opportunities and Challenges in Remote Sensing of Drought

The value of satellite remote sensing for drought monitoring was first realized more than two decades ago with the application of Normalized Difference Index (NDVI) data from the Advanced Very High Resolution Radiometer (AVHRR) for assessing the effect of drought on vegetation. Other indices such as the Vegetation Health Index (VHI) were also developed during this time period, and applied to AVHRR NDVI and brightness temperature data for routine global monitoring of drought conditions. These early efforts demonstrated the unique perspective that global imagers such as AVHRR could provide for operational drought monitoring through their near-daily, global observations of Earth's land surface. However, the advancement of satellite remote sensing of drought was limited by the relatively few spectral bands of operational global sensors such as AVHRR, along with a relatively short period of observational record. Remote sensing advancements are of paramount importance given the increasing demand for tools that can provide accurate, timely, and integrated information on drought conditions to facilitate proactive decision making (NIDIS, 2007). Satellite-based approaches are key to addressing significant gaps in the spatial and temporal coverage of current surface station instrument networks providing key moisture observations (e.g., rainfall, snow, soil moisture, ground water, and ET) over the United States and globally (NIDIS, 2007). Improved monitoring capabilities will be particularly important given increases in spatial extent, intensity, and duration of drought events observed in some regions of the world, as reported in the International Panel on Climate Change (IPCC) report (IPCC, 2007). The risk of drought is anticipated to further increase in some regions in response to climatic changes in the hydrologic cycle related to evaporation, precipitation, air temperature, and snow cover (Burke et al., 2006; IPCC, 2007; USGCRP, 2009). Numerous national, regional, and global efforts such as the Famine and Early Warning System (FEWS), National Integrated Drought Information System (NIDIS), and Group on Earth Observations (GEO), as well as the establishment of regional drought centers (e.g., European Drought Observatory) and geospatial visualization and monitoring systems (e.g, NASA SERVIR) have been undertaken to improve drought monitoring and early warning systems throughout the world. The suite of innovative remote sensing tools that have recently emerged will be looked upon to fill important data and knowledge gaps (NIDIS, 2007; NRC, 2007) to address a wide range of drought-related issues including food security, water scarcity, and human health.

Wardlow, Brian D.↗
NASA NTRS2021

Spectrophotometric Modeling and Mapping of (101955) Bennu

Using hyperspectral data collected by OVIRS, the visible and infrared spectrometer onboard the OSIRIS-REx (Origins, Spectral Interpretation, Resource Identification, and Security–Regolith Explorer) spacecraft, we modeled the global average spectrophotometric properties of the carbonaceous asteroid (101955) Bennu and mapped their variations. We restricted our analysis to 0.4–2.5 µm to avoid the wavelengths where thermal emission from the asteroid dominates (>2.5 µm). Bennu has global photometric properties typical of dark asteroids; we found a geometric albedo of 0.046 ± 0.007 and a linear phase slope of 0.024 ± 0.007 mag deg–1 at 0.55 µm. The average spectral slope of Bennu’s normal albedo is –0.0030 µm–1, and the phase reddening parameter is 4.3´10–4 µm–1 deg–1, both over the spectral range of 0.5–2.0 µm. We produced normal albedo maps and phase slope maps at all spectral channels, from which we derived spectral slope and phase reddening maps. Correlation analysis suggests that phase slope variations on Bennu are likely due to photometric roughness variation. A correlation between photometric roughness and thermal roughness is evident, implying that the roughness of Bennu is self-similar on scales from tens of microns to meters. Our analysis reveals latitudinal trends in the spectral color slope and phase reddening on Bennu. The equatorial region appears to be redder than the global average, and the spectral slope decreases towards higher latitudes. Phase reddening on Bennu is relatively weak in the equatorial region and shows an asymmetry between the northern and southern hemispheres. We attributed the latitudinal trend to the geophysical conditions on Bennu that result in a global pattern of mass flow towards the equator.

Jian-Yang Li (李荐扬)↗
DOE OSTI2021

Enabling Computation on Sensitive Data in International Safeguards with Privacy-Preserving Encryption Techniques

Privacy-preserving machine learning is a field of study that explores how to protect and preserve the privacy of sensitive data while allowing the data to be used by machine learning algorithms. This field has had substantial industry investment due to heightened concerns about privacy in the technology industry, with a focus in two broad application areas: financial services and healthcare. Numerous privacy-preserving methods have also been proposed for international safeguards, but they have been difficult to enact because the data they require is con- sidered sensitive or proprietary by the nuclear facility operator. This work examines how current privacy-preserving approaches might be used to enable the International Atomic Energy Agency (IAEA) to use that data to contribute to a safeguards conclusion about a state while giving nuclear operators confidence that their sensitive data is adequately protected. This paper begins by exploring several broad categories of privacy-preserving techniques including homomorphic encryption, secure multiparty computation, secure enclaves, and zero-knowledge proofs. Then we discuss some of the security considerations related to using these methods, potential use cases, and a conceptual system design for applying privacy-preserving methods in international safeguards.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗
NASA NTRS2022

Data-driven Expectations for Electromagnetic Counterpart Searches Based on LIGO/Virgo Public Alerts

Searches for electromagnetic counterparts of gravitational-wave signals have redoubled since the first detection in2017 of a binary neutron star merger with a gamma-ray burst, optical/infrared kilonova, and panchromatic after glow. Yet, one LIGO/Virgo observing run later, there has not yet been a second, secure identification of an electromagnetic counterpart. This is not surprising given that the localization uncertainties of events in LIGO and Virgo’s third observing run, O3, were much larger than predicted. We explain this by showing that improvements in data analysis that now allow LIGO/Virgo to detect weaker and hence more poorly localized events have increased the overall number of detections, of which well-localized, gold-plated events make up a smaller proportion overall. We present simulations of the next two LIGO/Virgo/KAGRA observing runs, O4 and O5, that are grounded in the statistics ofO3 public alerts. To illustrate the significant impact that the updated predictions can have, we study the follow-up strategy for the Zwicky Transient Facility. Realistic and timely forecasting of gravitational-wave localization accuracy is paramount given the large commitments of telescope time and the need to prioritize which events are followed up. We include a data release of our simulated localizations as a public proposal planning resource for astronomers

Polina Petrov↗
NASA NTRS2011

Autonomous Satellite Operations Via Secure Virtual Mission Operations Center

The science community is interested in improving their ability to respond to rapidly evolving, transient phenomena via autonomous rapid reconfiguration, which derives from the ability to assemble separate but collaborating sensors and data forecasting systems to meet a broad range of research and application needs. Current satellite systems typically require human intervention to respond to triggers from dissimilar sensor systems. Additionally, satellite ground services often need to be coordinated days or weeks in advance. Finally, the boundaries between the various sensor systems that make up such a Sensor Web are defined by such things as link delay and connectivity, data and error rate asymmetry, data reliability, quality of service provisions, and trust, complicating autonomous operations. Over the past ten years, researchers from the NASA Glenn Research Center (GRC), General Dynamics, Surrey Satellite Technology Limited (SSTL), Cisco, Universal Space Networks (USN), the U.S. Geological Survey (USGS), the Naval Research Laboratory, the DoD Operationally Responsive Space (ORS) Office, and others have worked collaboratively to develop a virtual mission operations capability. Called VMOC (Virtual Mission Operations Center), this new capability allows cross-system queuing of dissimilar mission unique systems through the use of a common security scheme and published application programming interfaces (APIs). Collaborative VMOC demonstrations over the last several years have supported the standardization of spacecraft to ground interfaces needed to reduce costs, maximize space effects to the user, and allow the generation of new tactics, techniques and procedures that lead to responsive space employment.

Miller, Eric↗
DOE OSTI2022

Effects of Chlorine Capture and a Proposed Density Law on the Reactivity of Plutonium Solution Systems

During fissionable material processing, all normal and credible abnormal conditions must remain safely subcritical. Nuclear Criticality Safety (NCS) uses a number of methods to determine subcriticality, one of which is the use of neutron transport codes such as MCNP6. In order to create models for use with MCNP6, both the geometry and materials in fissionable material processes must be known, or assumptions must be made and quantified for the impact to bias. One of the systems with a significant amount of bias due to material modeling assumptions is in the area of aqueous plutonium processing. These solutions are typically plutonium nitrate solutions or plutonium chloride solutions, which are modeled as fictitious plutonium metal-water mixtures because little is known about the actual density of the solution and there is no current predictive capability approved for use at Los Alamos National Laboratory (LANL) for modeling them. This research is currently underway to fill the gap and develop an algorithm for use with MCNP6 to model the density of plutonium chloride solutions. The method is to be validated with experimental data for density, and also validated with critical experiments using MCNP6. Note that the Chlorine Worth Study (CWS) was performed in December 2021 to help bridge the gap in chlorine data for critical experiments, and is currently awaiting International Criticality Safety Benchmark Evaluation Project (ICSBEP) review. This study was performed by LANL at the National Criticality Experiments Research Center (NCERC) at the Nevada National Security Site (NNSS). Additional information regarding this experiment may currently be found in LA-UR- 22-29180. Additionally, the Chemistry-Actinide Analytical Chemistry (C-AAC) at LANL has performed a number of solution density measurements for PuCl 3 -HC 1 -H 2 O, allowing for such data be used to create a semi-empirical density via the Pitzer method. The published dataset for the measurements is documented in LA-UR-22-25454. This method has already been tested successfully for aqueous plutonium nitrate solutions in SCALE. Current solution density measurements exist of plutonium concentrations of 0-~142g/L, all at 2M HC1, at temperatures 20-40°C. Additional data was taken for HC1-corrected density values, which essentially mimics the data for a pure PuCl x -water solution. The calculations in this report aim to support the current research by demonstrating the difference in system reactivity for the current modeling method when compared to the new proposed modeling with a density law implementation, which is being written as a Python tool to be used with MCNP6.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗