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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

X-ray emissivity of old stellar populations: A local group census

We study the unresolved X-ray emission in three Local Group dwarf elliptical (dE) galaxies (NGC 147, NGC 185, and NGC 205) using XMM-Newton observations; this emission most likely originates from a collection of weak X-ray sources, mainly cataclysmic variables and coronally active binaries. Precise knowledge of this stellar X-ray emission is crucial not only for understanding the relevant stellar astrophysics but also for disentangling and quantifying the thermal emission from diffuse hot gas in nearby galaxies. We find that the integrated X-ray emissivities of the individual dEs agree well with those of the solar vicinity, supporting an often assumed but untested view that the X-ray emissivity of old stellar populations is quasi-universal in normal galactic environments, in which dynamical effects on the formation and destruction of binary systems are not important. The average X-ray emissivity of the dEs studied in the literature, including M32, is measured to be L{sub 0.5−2 keV}/M{sub ∗}=(6.0±0.5±1.8)×10{sup 27} erg s{sup −1} M{sub ⊙}{sup −1}. We also compare this value to the integrated X-ray emissivities of Galactic globular clusters and old open clusters and discuss the role of dynamical effects in these dense stellar systems.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

DISSECTING THE POWER SOURCES OF LOW-LUMINOSITY EMISSION-LINE GALAXY NUCLEI VIA COMPARISON OF HST-STIS AND GROUND-BASED SPECTRA

Using a sample of ∼100 nearby line-emitting galaxy nuclei, we have built the currently definitive atlas of spectroscopic measurements of Hα and neighboring emission lines at subarcsecond scales. We employ these data in a quantitative comparison of the nebular emission in Hubble Space Telescope (HST) and ground-based apertures, which offer an order-of-magnitude difference in contrast, and provide new statistical constraints on the degree to which transition objects and low-ionization nuclear emission-line regions (LINERs) are powered by an accreting black hole at ≲10 pc. We show that while the small-aperture observations clearly resolve the nebular emission, the aperture dependence in the line ratios is generally weak, and this can be explained by gradients in the density of the line-emitting gas: the higher densities in the more nuclear regions potentially flatten the excitation gradients, suppressing the forbidden emission. The transition objects show a threefold increase in the incidence of broad Hα emission in the high-resolution data, as well as the strongest density gradients, supporting the composite model for these systems as accreting sources surrounded by star-forming activity. The narrow-line LINERs appear to be the weaker counterparts of the Type 1 LINERs, where the low accretion rates cause the disappearance of the broad-line component. The enhanced sensitivity of the HST observations reveals a 30% increase in the incidence of accretion-powered systems at z ≈ 0. A comparison of the strength of the broad-line emission detected at different epochs implies potential broad-line variability on a decade-long timescale, with at least a factor of three in amplitude.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

The role of the eROSITA all-sky survey in searches for sterile neutrino dark matter

We investigate for the first time the potential of angular auto- and cross-correlation power spectra in identifying sterile neutrino dark matter in the cosmic X-ray background. We take as reference the performance of the soon-to-be-launched eROSITA satellite. The main astrophysical background sources against sterile neutrino decays are active galactic nuclei, galaxies powered by X-ray binaries, and clusters of galaxies. While sterile neutrino decays are always subdominant in the auto-correlation power spectra, they can be efficiently enhanced when cross-correlating with tracers of the dark matter distribution such as galaxies in the 2MASS catalogues. We show that the planned four-years eROSITA all-sky survey will provide a large enough photon statistics to potentially yield very stringent constraints on the decay lifetime, enabling to firmly test the recently claimed 3.56-keV X-ray line found towards several clusters and galaxies and its decaying dark matter interpretation. However, we also show that in order to fully exploit the potential of eROSITA for dark matter searches, it is vital to overcome the shot-noise limitations inherent to galaxy catalogues as tracers for the dark matter distribution.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Search for magnetically-induced signatures in the arrival directions of ultra-high-energy cosmic rays measured at the Pierre Auger Observatory

We search for signals of magnetically-induced effects in the arrival directions of ultra-high-energy cosmic rays detected at the Pierre Auger Observatory. We apply two different methods. One is a search for sets of events that show a correlation between their arrival direction and the inverse of their energy, which would be expected if they come from the same point-like source, they have the same electric charge and their deflection is relatively small and coherent. We refer to these sets of events as “multiplets”. The second method, called “thrust”, is a principal axis analysis aimed to detect the elongated patterns in a region of interest. We study the sensitivity of both methods using a benchmark simulation and we apply them to data in two different searches. The first search is done assuming as source candidates a list of nearby active galactic nuclei and starburst galaxies. The second is an all-sky blind search. We report the results and we find no statistically significant features. We discuss the compatibility of these results with the indications on the mass composition inferred from data of the Pierre Auger Observatory.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2011

Fe K LINE COMPLEX IN THE NUCLEAR REGION OF NGC 253

A bright, nearby edge-on starburst galaxy, NGC 253, was studied using the Suzaku, XMM, and Chandra X-ray observatories. With Suzaku and XMM we detected complex line structure of Fe K, which is resolved into three lines (Fe I at 6.4 keV, Fe XXV at 6.7 keV, and Fe XXVI at 7.0 keV) around the center of NGC 253. Especially, the Fe I and Fe XXVI lines are the first clear detections, with a significance of >99.99% and 99.89% estimated by a Monte Carlo procedure. Imaging spectroscopy with Chandra revealed that the emission is distributed in {approx}60 arcsec{sup 2} region around the nucleus, which suggests that the source is not only the buried active galactic nucleus. The flux of highly ionized Fe lines can be explained by the accumulation of 10-1000 supernova remnants that are the result of high star-forming activity, while the Fe I line flux is consistent with the fluorescent line emission expected with the molecular clouds in the region.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

Destruction and multiple ionization of PAHs by X-rays in circumnuclear regions of AGNs

ABSTRACT The infrared signatures of polycyclic aromatic hydrocarbons (PAHs) are observed in a variety of astrophysical objects, including the circumnuclear medium of active galactic nuclei (AGNs). These are sources of highly energetic photons (0.2–10 keV), exposing the PAHs to a harsh environment. In this work, we examined experimentally the photoionization and photostability of naphthalene (C10H8), anthracene (C14H10), 2-methyl-anthracene (C14H9CH3), and pyrene (C16H10) upon interaction with photons of 275, 310, and 2500 eV. The measurements were performed at the Brazilian Synchrotron Light Laboratory using time-of-flight mass-spectrometry. We determined the absolute photoionization and photodissociation cross-sections as a function of the incident photon energy; the production rates of singly, doubly, and triply charged ions; and the molecular half-lives in regions surrounding AGNs. Even considering moderate X-ray optical depth values (τ = 4.45) due to attenuation by the dusty torus, the half-lives are not long enough to account for PAH detection. Our results suggest that a more sophisticated interplay between PAHs and dust grains should be present in order to circumvent molecular destruction. We could not see any significant difference in the half-life values by increasing the size of the PAH carbon backbone, NC, from 10 to 16. However, we show that the multiple photoionization rates are significantly greater than the single ones, irrespective of the AGN source. We suggest that an enrichment of multiply charged ions caused by X-rays can occur in AGNs.

Monfredini, Thiago↗
DOE OSTI2021

Magnetic Weyl Semimetallic Phase in Thin Films of Eu 2 Ir 2 O 7

The interplay between electronic interactions and strong spin-orbit coupling is expected to create a plethora of fascinating correlated topological states of quantum matter. Of particular interest are magnetic Weyl semimetals originally proposed in the pyrochlore iridates, which are only expected to reveal their topological nature in thin film form. To date, however, direct experimental demonstrations of these exotic phases remain elusive, due to the lack of usable single crystals and the insufficient quality of available films. Here, in this study, we report on the discovery of signatures for the long-sought magnetic Weyl semimetallic phase in (111)-oriented Eu 2 Ir 2 O 7 high-quality epitaxial thin films. We observed an intrinsic anomalous Hall effect with colossal coercivity but vanishing net magnetization, which emerges right below the onset of a peculiar magnetic phase with all-in-all-out (AIAO) antiferromagnetic ordering. The anomalous Hall conductivity obtained experimentally is consistent with the theoretical prediction, likely arising from the nonzero Berry curvature emanated by Weyl node pairs near the Fermi level that act as sources and sinks of Berry flux, activated by broken cubic crystal symmetry at the top and bottom terminations of the thin film.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Bulk transport paths through defects in floating zone and Al flux grown SmB 6

We investigate the roles of disorder on low-temperature transport in SmB 6 crystals grown by both the Al flux and floating zone methods. We used the inverted resistance method with Corbino geometry to investigate whether low-temperature variations in the standard resistance plateau arise from a surface or a bulk channel in floating zone samples. The results show significant sample-dependent residual bulk conduction, in contrast to smaller amounts of residual bulk conduction previously observed in Al flux grown samples with Sm vacancies. In this work, we consider hopping in an activated impurity band as a possible source for the observed bulk conduction, but it is unlikely that the large residual bulk conduction seen in floating zone samples is solely due to Sm vacancies. We therefore propose that one-dimensional defects, or dislocations, contribute as well. Using chemical etching, we find evidence for dislocations in both flux and floating zone samples, with higher dislocation density in floating zone samples than in Al flux grown samples. In addition to the possibility of transport through one-dimensional dislocations, we also discuss our results in the context of recent theoretical models of SmB 6 .

36 MATERIALS SCIENCE↗
DOE OSTI2012

New photomultiplier active base for Hall C Jefferson Lab lead tungstate calorimeter

A new photomultiplier tube active base was designed and tested. The base combines active voltage division circuit and fast amplifier, powered by the current flowing through voltage divider. This base is developed to upgrade older photomultiplier bases of Jefferson Lab lead-tungsten calorimeter (about ˜1200 crystals of PbWO{sub 4} from the PrimEx experimental setup). This is needed for the extension of detectors' rate capability to meet requirements of new Hall C proposal PR12-11-102 of measurements of the L/T separated cross sections and their ratio R = πL/πT in neutral-pion p(e,e'π0)p deep exclusive and p(p(e,e'π{sup 0})p)X semi-inclusive scattering regions. New active base is direct replacement of older passive base circuit without adding of additional power or signal lines. However, it extends detectors rate capability with factor over 20. Moreover, transistorized voltage divider improves detector's amplitude resolution due to reduction of photomultiplier gain dependence from tube anode current. The PMT active base is the invention disclosed in V. Popov's U.S. Patent No. 6,791,269, which successfully works over ten years in several Jefferson Lab Cherenkov detectors. The following design is a new revised and improved electronic circuit with better gain stability and linearity in challenge to meet requirements of new Hall C experimental setup. New active base performance was tested using fast LED light source and Pr:LuAG scintillator and gamma sources. Electronics radiation hardness was tested on JLab accelerator. Results of testing R4125 Hamamatsu photomultiplier tube in new active base are presented.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2011

Modeling a Hypothetical {sup 170}Tm Source for Brachytherapy Applications

Purpose: To perform absorbed dose calculations based on Monte Carlo simulations for a hypothetical {sup 170}Tm source and to investigate the influence of encapsulating material on the energy spectrum of the emitted electrons and photons. Methods: GEANT4 Monte Carlo code version 9.2 patch 2 was used to simulate the decay process of {sup 170}Tm and to calculate the absorbed dose distribution using the GEANT4 Penelope physics models. A hypothetical {sup 170}Tm source based on the Flexisource brachytherapy design with the active core set as a pure thulium cylinder (length 3.5 mm and diameter 0.6 mm) and different cylindrical source encapsulations (length 5 mm and thickness 0.125 mm) constructed of titanium, stainless-steel, gold, or platinum were simulated. The radial dose function for the line source approximation was calculated following the TG-43U1 formalism for the stainless-steel encapsulation. Results: For the titanium and stainless-steel encapsulation, 94% of the total bremsstrahlung is produced inside the core, 4.8 and 5.5% in titanium and stainless-steel capsules, respectively, and less than 1% in water. For the gold capsule, 85% is produced inside the core, 14.2% inside the gold capsule, and a negligible amount (<1%) in water. Platinum encapsulation resulted in bremsstrahlung effects similar to those with the gold encapsulation. The range of the beta particles decreases by 1.1 mm with the stainless-steel encapsulation compared to the bare source but the tissue will still receive dose from the beta particles several millimeters from the source capsule. The gold and platinum capsules not only absorb most of the electrons but also attenuate low energy photons. The mean energy of the photons escaping the core and the stainless-steel capsule is 113 keV while for the gold and platinum the mean energy is 160 keV and 165 keV, respectively. Conclusions: A {sup 170}Tm source is primarily a bremsstrahlung source, with the majority of bremsstrahlung photons being generated in the source core and experiencing little attenuation in the source encapsulation. Electrons are efficiently absorbed by the gold and platinum encapsulations. However, for the stainless-steel capsule (or other lower Z encapsulations) electrons will escape. The dose from these electrons is dominant over the photon dose in the first few millimeter but is not taken into account by current standard treatment planning systems. The total energy spectrum of photons emerging from the source depends on the encapsulation composition and results in mean photon energies well above 100 keV. This is higher than the main gamma-ray energy peak at 84 keV. Based on our results, the use of {sup 170}Tm as a brachytherapy source presents notable challenges.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2023

Revealing the Mechanism Behind Sudden Capacity Loss in Lithium Metal Batteries

Rechargeable Li-metal batteries (LMBs) are attractive energy storage candidates for electric vehicles (EVs) because they offer higher energy density than batteries built with intercalation electrodes. However, one of the main barriers to the commercial deployment of LMBs has been their relatively short cycle life. Re-designing the electrolyte system shows promise in achieving acceptable cycle life, but even so, the resulting cells display a challenging end-of-life (EOL) behavior: a sudden capacity loss. Herein, we report a new method for analyzing voltage profiles during cycling to distinguish between the capacity loss originating from the loss of cathode capacity vs growth in cell resistance. Further, this analysis reveals that sudden capacity loss was preceded by acceleration in the rate of growth of cell resistance, and cycling of multiple cells showed that this phenomenon is sensitive to the initial quantity of electrolyte in the cells. In contrast, the cathode capacity degraded at a constant rate independent of the electrolyte quantity. Combining this evidence with post-analysis of harvested electrolyte and electrodes, we conclude that neither the loss of active lithium nor the loss of active cathode material was the primary source of sudden capacity loss; instead, consumption and decomposition of electrolyte causes the drastic capacity loss at EOL.

25 ENERGY STORAGE↗
DOE OSTI2025

Direct Conversion of MnO2 into Atomic Mn Sites for Oxygen Reduction

Development of platinum group metal (PGM)-free catalysts has been investigated to replace the platinum group metal catalyst in future inexpensive polymer electrolyte membrane (PEM) fuel cells. Usually, synthetic methods for these PGM-free catalysts involve introducing transition-metal salts or molecules. Herein, we demonstrate a facile synthetic method to prepare PGM-free Mn-N-C catalysts by directly converting manganese oxides into highly active MnN4 sites. Typically, MnO2 is used as a Mn source. Ammonium chloride and benzimidazole are introduced during high-temperature treatment to enhance catalytic activity and stability further. Ammonia generated from the decomposition of ammonium chloride can improve the intrinsic ORR activity of MnNx moieties through chemical or electronic effects by introducing additional nitrogen groups. The Mn-N-C catalyst exhibits promising ORR activity, achieving a half-wave potential of 0.83 V in 0.5 M H2SO4, outperforming most PGM-free ORR catalysts. The robust carbon structure resulting from organic-molecule treatment is also verified by electrochemical and physical characterization, thereby improving the catalyst's durability.

Yang, Xiaoxuan↗
DOE OSTI2025

LLNL Microbenchmarks

The LLNL Microbenchmarks repository will contain open-source microbenchmarks for HPC system benchmarking activities. The repository will contain the code for various microbenchmarks developed for Request For Proposal (RFP) response evaluation and system acceptance.

Brink, Stephanie [Lawrence Livermore National Labo↗
DOE OSTI2024

Radionuclide-specific Parameters Dataset

The radionuclide-specific parameters dataset is searchable for radiological information for multiple isotopes simultaneously. After selecting radionuclides of interest and the desired parameters, the RAIS will generate a table containing the values, chosen according to an established hierarchy. Results can be downloaded in Excel format. 50 parameters are available, including atomic number, soil to animal transfer coefficients, plant uptake coefficients, half-life, specific activity, and water solubility. Seven primary sources are used to populate the dataset of radiological-specific parameters. These values should be used in cancer risk assessments for the calculation of preliminary remediation goals (PRGs), hazard characterization, and transport modeling. Users can select up to 1000 radionuclides per query. The dataset supports environmental risk assessments, regulatory decision-making, and environmental planning with tools for benchmarking against risk-based standards. This structured approach ensures a robust evaluation of environmental risks tailored to regulatory needs.

Manning, Karessa [Oak Ridge National Laboratory (O↗
DOE OSTI2022

Integrated Disposal Facility FY2011 Glass Testing Summary Report [Erratum]

Pacific Northwest National Laboratory was contracted by Washington River Protection Solutions, LLC to provide the technical basis for estimating radionuclide release from the engineered portion of the disposal facility (e.g., source term). Vitrifying the low-activity waste at Hanford is expected to generate over 1.6 x 10 5 m 3 of glass (Certa and Wells 2010). The volume of immobilized low-activity waste (ILAW) at Hanford is the largest in the DOE complex and is one of the largest inventories (approximately 8.9 x 10 14 Bq total activity) of long-lived radionuclides, principally 99 Tc (t 1/2 = 2.1 x 10 5 ), planned for disposal in a low-level waste (LLW) facility. Before the ILAW can be disposed, DOE must conduct a performance assessment (PA) for the Integrated Disposal Facility (IDF) that describes the long-term impacts of the disposal facility on public health and environmental resources. As part of the ILAW glass testing program PNNL is implementing a strategy, consisting of experimentation and modeling, in order to provide the technical basis for estimating radionuclide release from the glass waste form in support of future IDF PAs. The purpose of this report is to summarize the progress made in fiscal year (FY) 2011 toward implementing the strategy with the goal of developing an understanding of the long-term corrosion behavior of low-activity waste glasses.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2013

Large-Scale Uncertainty and Error Analysis for Time-dependent Fluid/Structure Interactions in Wind Turbine Applications

The following is the final report covering the entire period of this aforementioned grant, June 1, 2011 - May 31, 2013 for the portion of the effort corresponding to Stanford University (SU). SU has partnered with Sandia National Laboratories (PI: Mike S. Eldred) and Purdue University (PI: Dongbin Xiu) to complete this research project and this final report includes those contributions made by the members of the team at Stanford. Dr. Eldred is continuing his contributions to this project under a no-cost extension and his contributions to the overall effort will be detailed at a later time (once his effort has concluded) on a separate project submitted by Sandia National Laboratories. At Stanford, the team is made up of Profs. Alonso, Iaccarino, and Duraisamy, post-doctoral researcher Vinod Lakshminarayan, and graduate student Santiago Padron. At Sandia National Laboratories, the team includes Michael Eldred, Matt Barone, John Jakeman, and Stefan Domino, and at Purdue University, we have Prof. Dongbin Xiu as our main collaborator. The overall objective of this project was to develop a novel, comprehensive methodology for uncertainty quantification by combining stochastic expansions (nonintrusive polynomial chaos and stochastic collocation), the adjoint approach, and fusion with experimental data to account for aleatory and epistemic uncertainties from random variable, random field, and model form sources. The expected outcomes of this activity were detailed in the proposal and are repeated here to set the stage for the results that we have generated during the time period of execution of this project: 1. The rigorous determination of an error budget comprising numerical errors in physical space and statistical errors in stochastic space and its use for optimal allocation of resources; 2. A considerable increase in efficiency when performing uncertainty quantification with a large number of uncertain variables in complex non-linear multi-physics problems; 3. A solution to the long-time integration problem of spectral chaos approaches; 4. A rigorous methodology to account for aleatory and epistemic uncertainties, to emphasize the most important variables via dimension reduction and dimension-adaptive refinement, and to support fusion with experimental data using Bayesian inference; 5. The application of novel methodologies to time-dependent reliability studies in wind turbine applications including a number of efforts relating to the uncertainty quantification in vertical-axis wind turbine applications. In this report, we summarize all accomplishments in the project (during the time period specified) focusing on advances in UQ algorithms and deployment efforts to the wind turbine application area. Detailed publications in each of these areas have also been completed and are available from the respective conference proceedings and journals as detailed in a later section.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2014

Work Plan for a Limited CCC/USDA Investigation of the Current Carbon Tetrachloride Contamination in Groundwater at Navarre, Kansas

During private well testing in 1990-1991, carbon tetrachloride was identified in the groundwater at several locations in the town of Navarre, Kansas, at levels exceeding the Kansas Tier 2 level and U.S. Environmental Protection Agency (EPA) maximum contaminant level (MCL) of 5.0 μg/L. Several subsequent investigations through 2006 evaluated the concentrations and distribution of carbon tetrachloride in groundwater. This work included the identification of the contaminant sources (Argonne 2007). The history of activities to address the contamination in soil and groundwater is summarized in Table 1.1. The most recent studies, conducted by the Kansas Department of Health and Environment (KDHE), include a brownfields investigation initiated in 2013 (Phase I) and continuing in early 2014 (Phase II), as well as private well testing.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2016

Tosoh SMD, Inc./Production of High-Quality Tantalum: Final CRADA Report

The objectives of the proposed program are: (1) to produce Ta ingot with very high purity (> 99.99% overall, with ppm-level allowable for specific impurity elements); and (2) to provide requisite grain structure in the ingot with special metallurgical processing. We believe this research and development has a high potential to keep Tosoh competitive as the future continues to demand better performance from sputtering sources. We encourage further R&D activities and are looking forward to continued interaction.

36 MATERIALS SCIENCE↗