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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,657 records · Page 92
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Momentum-resolved lattice dynamics of parent and electron-doped Sr2IrO4

The mixing of orbital and spin character in the wavefunctions of the 5d iridates has led to predictions of strong couplings between their lattice, electronic and magnetic degrees of freedom. As well as realising a novel spin-orbit assisted Mott-insulating ground state, the perovskite iridate Sr 2 IrO 4 has strong similarities with the cuprate La 2 CuO 4 , which on doping hosts a charge density wave that appears intimately connected to high-temperature superconductivity. These phenomena can be sensitively probed through momentum-resolved measurements of the lattice dynamics, made possible by meV-resolution inelastic x-ray scattering. Here we report the rst such measurements for both parent and electron-doped Sr2IrO4. We nd that the low-energy phonon dispersions and intensities in both compounds are well described by the same non-magnetic DFT calculation. In the parent compound, no changes of the phonons upon magnetic ordering are discernible within the experimental resolution, and in the doped compound no anomalies are apparent due to charge density waves. These measurements extend our knowledge of the lattice properties of (Sr 1-x La x ) 2 IrO 4 , and constrain the couplings of the phonons to magnetic and charge order.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Scaling within the spectral function approach

Scaling features of the nuclear electromagnetic response functions unveil aspects of nuclear dynamics that are crucial for interpreting neutrino-and electron-scattering data. In the large momentum-transfer regime, the nucleon-density response function defines a universal scaling function, which is independent of the nature of the probe. In this work, we analyze the nucleon-density response function of 12 C, neglecting collective excitations. We employ particle and hole spectral functions obtained within two distinct many-body methods, both widely used to describe electroweak reactions in nuclei. We show that the two approaches provide compatible nucleon-density scaling functions that for large momentum transfers satisfy first-kind scaling. Both methods yield scaling functions characterized by an asymmetric shape, although less pronounced than that of experimental scaling functions. Finally, this asymmetry, only mildly affected by final state interactions, is mostly due to nucleon-nucleon correlations, encoded in the continuum component of the hole spectral function.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Measurements of the separated longitudinal structure function F L from hydrogen and deuterium targets at low Q 2

Structure functions, as measured in lepton-nucleon scattering, have proven to be very useful in studying the partonic dynamics within the nucleon. Furthermore, it is experimentally difficult to separately determine the longitudinal and transverse structure functions, and consequently there are substantially less data available in particular for the longitudinal structure function. Here, we present separated structure functions for hydrogen and deuterium at low four-momentum transfer squared, Q 2 < 1 GeV 2 , and compare them with parton distribution parametrization and k T factorization approaches. While differences are found, the parametrizations generally agree with the data, even at the very low-Q 2 scale of the data. The deuterium data show a smaller longitudinal structure function and a smaller ratio of longitudinal to transverse cross section, R, than the proton. This suggests either an unexpected difference in R for the proton and the neutron or a suppression of the gluonic distribution in nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Microwave Spectroscopy of a Weakly Pinned Charge Density Wave in a Superinductor

A chain of small Josephson junctions (a.k.a. superinductor) emerged recently as a high-inductance, low-loss element of superconducting quantum devices. We notice that the intrinsic parameters of a typical superinductor in fact place it into the Bose glass universality class for which the propagation of waves in a sufficiently long chain is hindered by pinning. Its weakness provides for a broad crossover from the spectrum of well-resolved plasmon standing waves at high frequencies to the low-frequency excitation spectrum of a pinned charge density wave. We relate the scattering amplitude of microwave photons reflected off a superinductor to the dynamics of a Bose glass. The dynamics at long and short scales compared to the Larkin pinning length determines the low- and high-frequency asymptotes of the reflection amplitude.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1993

Compact Raman Spectrometers Would Detect Hydrogen

Compact Raman spectrometers developed to measure concentrations of hydrogen as low as hundreds of parts per million in air, nitrogen, or other carrier gases. Advantages include speed, dynamic range, and ease of calibration. Design concept incorporates Raman-scattering apparatus into compact instrument of hydrogen leaking into stream of gas or into gas enclosed in small space. Should hydrogen-fueled cars and trucks come into widespread use, instruments used to detect leaks from vehicles and supply equipment, to help prevent explosions. Similar spectrometers developed to detect other gases emitting characteristic Raman spectra.

Helms, William R.↗
NASA NTRS1996

A Diagnostic System for Studying Energy Partitioning and Assessing the Response of the Ionosphere during HAARP Modification Experiments

This research program focused on the construction of several key radio wave diagnostics in support of the HF Active Auroral Ionospheric Research Program (HAARP). Project activities led to the design, development, and fabrication of a variety of hardware units and to the development of several menu-driven software packages for data acquisition and analysis. The principal instrumentation includes an HF (28 MHz) radar system, a VHF (50 MHz) radar system, and a high-speed radar processor consisting of three separable processing units. The processor system supports the HF and VHF radars and is capable of acquiring very detailed data with large incoherent scatter radars. In addition, a tunable HF receiver system having high dynamic range was developed primarily for measurements of stimulated electromagnetic emissions (SEE). A separate processor unit was constructed for the SEE receiver. Finally, a large amount of support instrumentation was developed to accommodate complex field experiments. Overall, the HAARP diagnostics are powerful tools for studying diverse ionospheric modification phenomena. They are also flexible enough to support a host of other missions beyond the scope of HAARP. Many new research programs have been initiated by applying the HAARP diagnostics to studies of natural atmospheric processes.

Djuth, Frank T.↗
NASA NTRS2017

Chorus Whistler Wave Source Scales As Determined From Multipoint Van Allen Probe Measurements

Whistler mode chorus waves are particularly important in outer radiation belt dynamics due to their key role in controlling the acceleration and scattering of electrons over a very wide energy range. The key parameters for both nonlinear and quasi-linear treatment of wave-particle interactions are the temporal and spatial scales of the wave source region and coherence of the wave field perturbations. Neither the source scale nor the coherence scale is well established experimentally, mostly because of a lack of multipoint VLF waveform measurements. We present an unprecedentedly long interval of coordinated VLF waveform measurements (sampled at 16384 s(exp -1)) aboard the two Van Allen Probes spacecraft-9 h (0800-1200 UT and 1700-2200 UT) during two consecutive apogees on 15 July 2014. The spacecraft separations varied from about 100 to 5000 km (mostly radially); measurements covered an L shell range from 3 to 6; magnetic local time 0430-0900, and magnetic latitudes were approximately 15 and approximately 5 deg during the two orbits. Using time-domain correlation techniques, the single chorus source spatial extent transverse to the background magnetic field has been determined to be about 550-650 km for upper band chorus waves with amplitudes less than 100 pT and up to 800 km for larger amplitude, lower band chorus waves. The ratio between wave amplitudes measured on the two spacecraft is also examined to reveal that the wave amplitude distribution within a single chorus element generation area can be well approximated by a Gaussian exp(-0.5 x r (exp 2)/r(sub 0)(exp 2)), with the characteristic scale r(sub 0) around 300 km. Waves detected by the two spacecraft were found to be coherent in phase at distances up to 400 km.

Agapitov, O.↗
DOE OSTI2022

Dual Energy Electron Storage Ring Cooler Design for Relativistic Ion Beams

Collider experiments demand small beam emittances in order to achieve high luminosity. For light particles such as electrons, there exists a natural synchrotron radiation damping resulting in low emittance beams at equilibrium. In the case of heavy particle beams such as proton or ion beams, there is no significant synchrotron radiation damping effect and some cooling mechanism is needed to get to low emittance beams. A dual energy storage ring cooler is a novel concept proposed to cool hadron beams at higher energies. The design consists of two rings: a low energy ring and a high energy ring connected by the energy recovering linac (ERL) that provides the necessary energy difference. The low energy ring has an electron cooler where the cooling interaction takes place between the electron and hadron beams whereas electron beam going through the high energy ring undergoes synchrotron radiation damping. In this document, we present a possible design of a dual energy storage ring-based electron cooler for high energy proton beam cooling suitable for the Electron Ion Collider (EIC) to be built at Brookhaven National laboratory (BNL). A special feature of a dual energy storage ring cooler design is that the electron beam energy in the low energy section must be tuned to match the hadron beam velocity in the cooling section, and the electron beam energy in the high energy section is chosen to provide an adequate synchrotron radiation damping. In addition, the ring optics design is carried out considering chromaticity correction, dynamic aperture, momentum aperture, beam lifetime, radiation damping and the intrabeam scattering effect. Finally, the cooling performance is simulated for 275 GeV proton beams at the top energy of the EIC. In such a collider it is desirable to cool the hadron beams to balance the emittance growth rates due to intra-beam scattering (IBS) to maintain a high luminosity during the collision runs. In such a situation, a dual energy storage ring based cooler could be a practical approach to be used for hadron beam cooling.

Dhital, Bhawin↗
DOE OSTI2026

Neural-network quantum states for the nuclear many-body problem

A long-standing goal of nuclear theory is to explain how the structure and dynamics of atomic nuclei and neutron-star matter emerge from the underlying interactions among protons and neutrons. Achieving this goal requires solving the nuclear quantum many-body problem with high accuracy across a wide range of length scales and density regimes. In this review, we discuss how artificial neural network representations of the nuclear many-body wave function have significantly extended the capabilities of continuum quantum Monte Carlo methods. In particular, neural network quantum states enable calculations of larger systems than were previously accessible and provide a flexible framework for capturing phenomena that challenge conventional approaches, including the emergence of nuclear clusters and superfluid phases in dense matter. We highlight recent applications to finite nuclei, infinite nuclear and neutron matter, and dynamical processes relevant to lepton-nucleus and nucleus-nucleus scattering. We also discuss conceptual and methodological connections with condensed matter physics, emphasizing developments in neural network quantum states that bridge strongly correlated systems across disciplines. Together, these developments demonstrate how neural-network methods open new avenues toward unified and accurate descriptions of nuclear structure, matter, and reactions.

Lovato, Alessandro [Argonne; TIFPA-INFN, Trento; V↗
DOE OSTI2019

Efficient ab initio calculations of electron-defect scattering and defect-limited carrier mobility

Electron-defect ($e - \mathrm{d}$) interactions govern charge carrier dynamics at low temperature, where they limit the carrier mobility and give rise to phenomena of broad relevance in condensed matter physics. Ab initio calculations of $e - \mathrm{d}$ interactions are still in their infancy, mainly because they require large supercells and computationally expensive workflows. Here we develop an efficient ab initio approach for computing elastic $e - \mathrm{d}$ interactions, their associated $e - \mathrm{d}$ relaxation times (RTs), and the low-temperature defect-limited carrier mobility. The method is applied to silicon with simple neutral defects, such as vacancies and interstitials. Contrary to conventional wisdom, the computed $e - \mathrm{d}$ RTs depend strongly on carrier energy and defect type, and the defect-limited mobility is temperature dependent. These results highlight the shortcomings of widely employed heuristic models of $e - \mathrm{d}$ interactions in materials. Finally, our method opens avenues for studying $e - \mathrm{d}$ scattering and low-temperature charge transport from first principles.

36 MATERIALS SCIENCE↗
NASA NTRS1997

Microgravity Foam Structure and Rheology

To exploit rheological and multiple-light scattering techniques, and ultimately microgravity conditions, in order to quantify and elucidate the unusual elastic character of foams in terms of their underlying microscopic structure and dynamics. Special interest is in determining how this elastic character vanishes, i.e. how the foam melts into a simple viscous liquid, as a function of both increasing liquid content and shear strain rate. The unusual elastic character of foams will be quantified macroscopically by measurement of the shear stress as a function of static shear strain, shear strain rate, and time following a step strain; such data will be analyzed in terms of a yield stress, a static shear modulus, and dynamical time scales. Microscopic information about bubble packing and rearrangement dynamics, from which these macroscopic non-Newtonian properties presumably arise, will be obtained non-invasively by novel multiple-light scattering diagnostics such as Diffusing-Wave Spectroscopy (DWS). Quantitative trends with materials parameters, such as average bubble size, and liquid content, will be sought in order to elucidate the fundamental connection between the microscopic structure and dynamics and the macroscopic rheology.

Durian, Douglas J.↗
DOE OSTI2020

Surface Enhanced Raman Scattering Selectivity in Proteins Arises from Electron Capture and Resonant Enhancement of Radical Species

Plasmon-enhanced Raman scattering is a powerful approach to detecting and characterizing proteins in live and dynamic biological systems. However, the selective detection/enhancement of specific residues as well as spectral diffusion and fluctuations have complicated the interpretation of enhanced Raman spectra and images of biological matter. In this paper, we therefore demonstrate that the amino acid tryptophan (Trp) can capture an electron from an excited plasmon, which generates a radical anion that is resonantly enhanced: a visible excited electronic state slides into resonance upon charging. This surface enhanced resonance Raman scattering (SERRS) mechanism explains the persistence of Trp signatures in the SERS and TERS spectra of proteins. Evidence for this picture includes the observation of visible resonances in the UV-Vis extinction spectrum, changes in the ground state vibrational spectrum, and plasmon-resonance dependent behavior. DFT calculations support the experimental observations. The behavior observed from the free Trp molecule is shown to explain the SERS spectrum of the Trp-cage protein. In effect, resonant Raman scattering from radicals formed through plasmonic excitation represents an under-investigated mechanism that may be exploited for chemical sensing applications. This work was supported by the National Institutes of Health Award R01-GM109988. The authors thank Hannah Shafaat for helpful discussions and providing an azurin sample for comparison. The authors also thank Joel Harris for providing constructive comments on our manuscript.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2019

Dynamic bound states in the continuum

All-dielectric metasurfaces are a versatile platform to investigate a host of unconventional physical scattering responses. Effects, including high absorption and Huygens’ surfaces, have been demonstrated; however, a more exotic materialization—termed bound states in the continuum (BSCs)—exists and consists of nonradiating localized waves that lie within the energy spectrum of the continuum. Here we experimentally demonstrate a dynamic BSC at terahertz frequencies that realizes a material-limited high-quality factor ( Q ) resonance Q = 8.7 × 10 3 , which may be modified by over 2 orders of magnitude through photodoping with band gap light. We elucidate the nature of the BSC resonance, and our experimental results are well supported by eigenvalue and S -parameter simulations. The demonstrated system and underlying theory establish a path to realize extremely high- Q dynamic resonances, which may be useful for detection of hazardous materials and frequency-diverse imaging.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

On the Ion Precipitation due to Field Line Curvature (FLC) and EMIC Wave Scattering and Their Subsequent Impact on Ionospheric Electrodynamics

Both field line curvature (FLC) and electromagnetic ion cyclotron (EMIC) wave scattering are believed to be associated with energetic ion precipitation, but their relative contributions to ionospheric ion precipitation and subsequent effects are still unclear. Here, in this study, by using a kinetic ring current model, we investigate their impact on the ionosphere from two aspects: the global distribution of ion precipitation and resulting ionospheric conductance. Our results show that the intensity and coverage of ion precipitation due to EMIC waves are larger than that due to FLC scattering, while the latter mostly contributes to ion precipitation in outer regions (L > 4–5). We then estimate the conductance with empirical models using the simulated ion precipitation energy flux. When the EMIC wave associated proton precipitation is included, the conductance is significantly enhanced in the dusk-to-midnight sector and has a wide magnetic latitude (MLAT) range from around 52° to 62°, considerably altering the electric potential in the dusk sector, which further influences particle dynamics in the magnetosphere. On the contrary, the proton precipitation caused by FLC scattering only occurs at higher latitudes above MLAT = 60° and the corresponding conductance is slightly enhanced at midnight, with negligible influence on the convective electric potential. Although electron precipitation-associated conductance is predominant globally, the results show that proton precipitation can also play an important role in ionospheric electrodynamics, especially when EMIC wave-associated precipitating proton energy flux exceeds that of electrons in the dusk sector, a region where many subauroral coupling processes occur.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Additive Molar Volumes in Amorphous Ca/Sr Carbonate Solid Solutions

The development of predictive models of minor element incorporation in crystalline carbonate end products requires an understanding of the fundamental controls on metastable intermediate phase composition. In this study, we used small-angle X-ray scattering (SAXS), X-ray pair distribution function (PDF), thermogravimetric analysis (TGA), inductively coupled plasma mass spectrometry (ICP-MS), and transmission electron microscopy (TEM) to determine the composition-dependent density of an amorphous calcium–strontium carbonate (ACSC) solid solution. The amorphous calcium carbonate (ACC) and strontium carbonate (ASC) measured densities were ρ ACC = 2.19 ± 0.04 g/cm 3 and ρ ASC = 2.97 ± 0.05 g/cm 3 . Throughout our work, the experiments showed a dependence of the water content of the amorphous solid solution on the Sr mole fraction. An equation that relates the molar volume to the average cation radius, the carbonate ion radius, and the water volume was parameterized for hydrated crystalline carbonates and predicted well the molar volume of the ACSC solid solution. This finding indicates that, as for hydrated crystalline carbonates, the molar volumes of amorphous carbonates are additive and that water is a structural component of ACSC. Ab initio molecular dynamics (AIMD) simulations of the ACSC solid solutions showed strong linear correlations between calculated molar volumes and Sr and H 2 O contents, thus supporting the experimental results. In conclusion, our findings highlight the need to consider the full CaCO 3 –MeCO 3 –H 2 O ternary when quantifying metal cation incorporation in ACC.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2017

Dynamic Stabilization of Metal Oxide–Water Interfaces

The interaction of water with metal oxide surfaces plays a crucial role in the catalytic and geochemical behavior of metal oxides. In a vast majority of studies, the interfacial structure is assumed to arise from a relatively static lowest energy configuration of atoms, even at room temperature. Using hematite (α-Fe 2 O 3 ) as a model oxide, we show through a direct comparison of in situ synchrotron X-ray scattering with density functional theory-based molecular dynamics simulations that the structure of the ($1\bar{10}2 $) termination is dynamically stabilized by picosecond water exchange. Simulations show frequent exchanges between terminal aquo groups and adsorbed water in locations and with partial residence times consistent with experimentally determined atomic sites and fractional occupancies. Frequent water exchange occurs even for an ultrathin adsorbed water film persisting on the surface under a dry atmosphere. The resulting time-averaged interfacial structure consists of a ridged lateral arrangement of adsorbed water molecules hydrogen bonded to terminal aquo groups. Surface pK a prediction based on bond valence analysis suggests that water exchange will influence the proton-transfer reactions underlying the acid/base reactivity at the interface. Our findings provide important new insights for understanding complex interfacial chemical processes at metal oxide–water interfaces.

58 GEOSCIENCES↗
NASA NTRS2005

A Dynamic Fountain Model for Lunar Dust

During the Apollo era of exploration it was discovered that sunlight was scattered at the terminators giving rise to horizon glow and streamers above the lunar surface. This was observed from the dark side of the Moon during sunset and sunrise by both surface landers and astronauts in orbit. These observations were quite unexpected, as the Moon was thought to be a pristine environment with a negligible atmosphere or exosphere. Subsequent investigations have shown that the sunlight was most likely scattered by electrostatically charged dust grains originating from the surface. It has since been demonstrated that this dust population could have serious implications for astronomical observations from the lunar surface. The lunar surface is electrostatically charged by the Moon s large-scale interaction with the local plasma environment and the photoemission of electrons due to solar ultra-violet (UV) light and X-rays. The like-charged surface and dust grains then act to repel each other, such that under certain conditions the dust grains are lifted above the surface. We present a dynamic fountain model which can explain how sub-micron dust is able to reach altitudes of up to approximately 100 km above the lunar surface. Previous static dust levitation models are most applicable to the heavier micron-sized grains in close proximity proximity to the surface, but they cannot explain the presence of extremely light grains at high altitudes. If we relax the static constraint applied to previous models, and instead assume that the grains are in constant motion (under the action of dynamic forces), a new picture emerges for the behavior of sub-micron lunar dust.

Stubbs, T. J.↗
DOE OSTI2026

In Situ High-Temperature Ultrafast Electron Diffraction through Integrated Furnace and MEMS Platforms

Temperature fundamentally governs phase stability, defect evolution, and transport behavior in materials. Despite its central role, direct measurements of structural evolution at elevated temperatures on ultrafast timescales have remained limited. Here, we report the design, integration, and validation of 2 complementary in situ heating platforms that substantially extend the thermal operating range of ultrafast electron diffraction (UED). A compact furnace-type heating stage enables stable diffraction measurements from room temperature to 800 K with ±0.1 K stability under ultrahigh vacuum, achieved through multi-sensor feedback control, dual air-cooling channels, and a thermally isolated motion stage. In parallel, a microelectromechanical system (MEMS)-based heating platform provides rapid thermal response and access to extreme temperatures ≥1,373 K with ±0.1 K stability over hundreds-micrometer regions while supporting simultaneous electrical biasing for electrothermal coupling studies. Absolute temperature calibration is established using diffraction-based thermometry via aluminum lattice expansion and independently validated through in situ melting of bismuth thin films. UED measurements further reveal pronounced temperature-dependent nonequilibrium lattice dynamics in bismuth, including modifications to electron–phonon coupling and Debye–Waller behavior, as well as enhanced ultrafast diffuse scattering in aluminum at elevated temperatures. Together, these developments establish a practical framework for quantitative, time-resolved studies of temperature-driven kinetics and nonequilibrium structural dynamics under extreme thermal environments.

Bai, Qianqian [Chinese Academy of Sciences (CAS), ↗