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DOE OSTI2022

β — -delayed fission in the coupled quasiparticle random-phase approximation plus Hauser-Feshbach approach

Beta-delayed neutron emission and β-delayed fission (βdf) probabilities were calculated for heavy, neutronrich nuclei using the Los Alamos coupled quasiparticle random-phase approximation plus Hauser-Feshbach (QRPA + HF) approach. In this model, the compound nucleus is initially populated by β decay and is followed through subsequent statistical decays taking into account competition among neutrons, γ rays, and fission. The primary output of these calculations includes branching ratios along with neutron and γ -ray spectra. Here, we find a relatively large region of heavy nuclides where the probability of βdf is near 100%. For a subset of nuclei near the neutron drip line, delayed neutron emission and the probability of fission are both large, which leads to the possibility of multichance βdf (mc-βdf). We comment on prospective neutron-rich nuclei that could be probed by future experimental campaigns and provide a full table of branching ratios in ASCII format in the Supplemental Material for use in various applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Measurement of the 238 U( n,f ) prompt fission neutron spectrum from 10 keV to 10 MeV induced by neutrons with 1.5–20 MeV energy

With the recent emergence of fast nuclear reactors, there has been a corresponding increasing interest in 238 U-related nuclear data. However, while existing literature data span much of the energy ranges of interest for the prompt fission neutron spectrum (PFNS) for neutron-induced fission of 238U, most literature data sets are highly correlated, and thus new, independent measurements of this quantity are needed. In this work, we report the results of a new measurement of the 238 U PFNS at the Los Alamos Neutron Science Center for incident neutron energies from 1.5–20.0 MeV, and outgoing neutron energies of 0.01–10.0 MeV. With some notable exceptions, the present results generally agree with existing literature data, especially with regard to features relating to multichance fission and pre-equilibrium features in the PFNS, thus adding confidence to existing nuclear data evaluations and filling in gaps of knowledge at previously unmeasured incident neutron energies. This result is the third in a series of PFNS measurements by the Chi-Nu collaboration now spanning all three major actinides, 239 Pu, 235 U, and 238 U. Thus, for the first time, we report reliable experimental PFNS ratios and average PFNS energy comparisons for measurements of all three of these isotopes including accurate correlations between the different, but correlated experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Energy dependence of fission product yields in the second-chance fission region

An extensive dataset of cumulative fission product yields has been generated under a joint collaboration between Los Alamos National Laboratory (LANL), Lawrence Livermore National Laboratory (LLNL), and the Triangle Universities Nuclear Laboratory (TUNL). The energy dependence of the cumulative yield for a select number of high-yield fission products has been measured using quasimonoenergetic neutrons with energies between 5.5 and 11.0 MeV. This is in addition to previously published data covering 0.5–4.5 and 14.8 MeV. The absolute number of fissions was determined during the irradiation period using dual-fission ionization chambers, and the fission products were measured postactivation by whole target γ-ray spectroscopy. Here this paper presents the absolute cumulative fission product yields as a function of incident neutron energy from the neutron-induced fission of 235 U, 238 U, and 239 Pu isotopes at four incident energies in the second-chance fission region and compares them with existing literature values. Corrections relevant to this collaboration's previously published data are also discussed.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2024

Measurement of the prompt fission neutron spectrum from 800 keV to 10 MeV for 240 Pu(sf) and for the 240 Pu($n,f$) reaction induced by neutrons of energy from 1–20 MeV

Here, the presence of 240 Pu in nuclear fuels for reactors has resulted in high uncertainties in the results of reactor and nuclear transmutation calculations because of deficiencies in 240 Pu-related nuclear data. Specifically for the prompt fission neutron spectrum (PFNS) of 240 Pu, there is only one neutron-induced, (n,f), measurement at 0.85 MeV incident neutron energy and only one complete spontaneous fission, (sf), measurement. This limited availability of data does not sufficiently guide nuclear data evaluations of these quantities. Here we report on a measurement of both the 240 Pu(sf) and the 240 Pu(n,f) PFNS, both over the emitted neutron energy range of 0.79–10.0 MeV, and from incident neutron energies of 1.0–20.0 MeV for the (n,f) reaction. Measurements were made with a hemispherical array of liquid scintillators at the high-energy Los Alamos Neutron Science Center white neutron source at the Weapons Neutron Research facility as part of the joint LANL-LLNL Chi-Nu experimental campaign to measure actinide fission neutron spectra. These measurements are the first of their kind, and provide clear experimental evidence for second-chance fission, third chance fission, and pre-equilibrium neutron emission processes in neutron-induced fission of 240 Pu, and are the first ever measurements above 1 MeV incident neutron energy.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2016

Absolute measurement of the 242 Pu neutron-capture cross section

Here, the absolute neutron-capture cross section of 242 Pu was measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. The first direct measurement of the 242 Pu(n,γ) cross section was made over the incident neutron energy range from thermal to ≈ 6 keV, and the absolute scale of the (n,γ) cross section was set according to the known 239 Pu(n,f) resonance at E n,R = 7.83 eV. This was accomplished by adding a small quantity of 239 Pu to the 242 Pu sample. The relative scale of the cross section, with a range of four orders of magnitude, was determined for incident neutron energies from thermal to ≈ 40 keV. Our data, in general, are in agreement with previous measurements and those reported in ENDF/B-VII.1; the 242 Pu(n,γ) cross section at the E n,R = 2.68 eV resonance is within 2.4% of the evaluated value. However, discrepancies exist at higher energies; our data are ≈30% lower than the evaluated data at E n ≈ 1 keV and are approximately 2σ away from the previous measurement at E n ≈ 20 keV.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2016

Measurement of neutron capture on Xe 136

136 Xe is a 0νββ decay candidate isotope, and is used in multiple experiments searching for this hypothetical decay mode. These experiments require precise information about neutron capture for their background characterization and minimization. Thermal and resonant neutron capture on 136 Xe have been measured at the Detector for Advanced Neutron Capture Experiments (DANCE) at the Los Alamos Neutron Science Center. A neutron beam ranging from thermal energy to greater than 100 keV was incident on a gas cell filled with isotopically pure 136 Xe. The relative neutron capture cross sections for neutrons at thermal energies and the first resonance at 2.154 keV have been measured. Furthermore, the γ cascades for these captures have been measured, and cascade models have been developed which may be used by 0νββ experiments using 136 Xe.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2016

Feeding of Rh and Ag isomers in fast-neutron-induced reactions

In (n,n') reactions on stable Ir and Au isotopes in the mass A=190 region, the experimentally established feeding of the isomers relative to the feeding of the corresponding ground states increases with increasing neutron energy, up to the neutron energy where the (n,2n) reaction channel opens up, and then decreases. In order to check for similar behavior in the mass A=100 region, the feeding of isomers and ground states in fast-neutron-induced reactions on stable isotopes in this mass region was studied. This is of especial interest for Rh which can be used as a radiochemical detector. Here, excited states were studied using the (n,n'γ), (n,2nγ), and (n,3nγ) reactions on 103 Rh and 109 Ag. A germanium detector array for γ-ray detection and the broad-spectrum pulsed neutron source of the Los Alamos Neutron Science Center's Weapons Neutron Research facility were used for the measurement. The energy of the incident neutrons was determined using the time-of-flight technique. Absolute partial γ-ray cross sections were measured for 57 transitions feeding isomers and ground states in 101,102,103 Rh and 107,108,109 Ag. The feeding of the isomers was found to be very similar in the corresponding reaction channels and it is compared to the feeding determined for the ground states. In conclusion, the opening of reaction channels at higher neutron energies removes angular momentum from the residual nucleus and reduces the population of the higher-spin isomers relative to the feeding of the lower-spin ground states. Similar behavior was observed in the mass A=190 region in the feeding of higher-spin isomers, but the reverse behavior was observed in 176 Lu with a lower-spin isomer and a higher-spin ground state.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Measurement of the Am 242 m neutron-induced reaction cross sections

The neutron-induced reaction cross sections of 242m Am were measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. A new neutron-capture cross section was determined, and the absolute scale was set according to a concurrent measurement of the well-known 242m Am(n,f) cross section. The (n,γ) cross section was measured from thermal energy to an incident energy of 1 eV at which point the data quality was limited by the reaction yield in the laboratory. Our new 242m Am fission cross section was normalized to ENDF/B-VII.1 to set the absolute scale, and it agreed well with the (n,f) cross section from thermal energy to 1 keV. Lastly, the average absolute capture-to-fission ratio was determined from thermal energy to E n = 0.1 eV, and it was found to be 26(4)% as opposed to the ratio of 19% from the ENDF/B-VII.1 evaluation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2017

Production of energetic light fragments in extensions of the CEM and LAQGSM event generators of the Monte Carlo transport code MCNP6 [Production of energetic light fragments in CEM, LAQGSM, and MCNP6]

We extend the cascade-exciton model (CEM), and the Los Alamos version of the quark-gluon string model (LAQGSM), event generators of the Monte Carlo N-particle transport code version 6 (MCNP6), to describe production of energetic light fragments (LF) heavier than 4 He from various nuclear reactions induced by particles and nuclei at energies up to about 1 TeV/nucleon. In these models, energetic LF can be produced via Fermi breakup, preequilibrium emission, and coalescence of cascade particles. Initially, we study several variations of the Fermi breakup model and choose the best option for these models. Then, we extend the modified exciton model (MEM) used by these codes to account for a possibility of multiple emission of up to 66 types of particles and LF (up to 28 Mg) at the preequilibrium stage of reactions. Then, we expand the coalescence model to allow coalescence of LF from nucleons emitted at the intranuclear cascade stage of reactions and from lighter clusters, up to fragments with mass numbers A ≤ 7, in the case of CEM, and A ≤ 12, in the case of LAQGSM. Next, we modify MCNP6 to allow calculating and outputting spectra of LF and heavier products with arbitrary mass and charge numbers. The improved version of CEM is implemented into MCNP6. Lastly, we test the improved versions of CEM, LAQGSM, and MCNP6 on a variety of measured nuclear reactions. The modified codes give an improved description of energetic LF from particle- and nucleus-induced reactions; showing a good agreement with a variety of available experimental data. They have an improved predictive power compared to the previous versions and can be used as reliable tools in simulating applications involving such types of reactions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Radiative neutron capture cross section from U 236

In this study, the 236 U(n,γ) reaction cross section has been measured for the incident neutron energy range from 10 eV to 800 keV by using the Detector for Advanced Neutron Capture Experiments (DANCE) γ-ray calorimeter at the Los Alamos Neutron Science Center. The cross section was determined with the ratio method, which is a technique that uses the 235 U(n,f) reaction as a reference. The results of the experiment are reported in the resolved and unresolved resonance energy regions. Individual neutron resonance parameters were obtained below 1 keV incident energy by using the R-matrix code sammy. The cross section in the unresolved resonance region is determined with improved experimental uncertainty. Lastly, it agrees with both ENDF/B-VII.1 and JEFF-3.2 nuclear data libraries. In conclusion, the results above 10 keV agree better with the JEFF-3.2 library.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Constraining the calculation of U 234 , 236 , 238 ( n , γ ) cross sections with measurements of the γ -ray spectra at the DANCE facility

The cross section for neutron capture in the continuum region has been difficult to calculate accurately. Previous results for 238 U show that including an M 1 scissors-mode contribution to the photon strength function resulted in very good agreement between calculation and measurement. Our paper extends that analysis to 234 , 236 U by using γ -ray spectra measured with the Detector for Advanced Neutron Capture Experiments (DANCE) at the Los Alamos Neutron Science Center to constrain the photon strength function used to calculate the capture cross section. Calculations using a strong scissors-mode contribution reproduced the measured γ -ray spectra and were in excellent agreement with the reported cross sections for all three isotopes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Measurement of the normalized U 238 ( n , f ) / U 235 ( n , f ) cross section ratio from threshold to 30 MeV with the NIFFTE fission Time Projection Chamber

We present that the normalized 238 U(n,f)/ 235 U(n,f) cross section ratio has been measured using the NIFFTE fission Time Projection Chamber (fissionTPC) from the reaction threshold to 30 MeV . The fissionTPC is a two-volume MICROMEGAS time projection chamber that allows for full three-dimensional reconstruction of fission-fragment ionization profiles from neutron-induced fission. The measurement was performed at the Los Alamos Neutron Science Center, where the neutron energy is determined from neutron time of-flight. The 238 U(n,f)/ 235 U(n,f) ratio reported here is the first cross section measurement made with the fissionTPC, and will provide new experimental data for evaluation of the 238 U(n,f) cross section, an important standard used in neutron-flux measurements. Use of a development target in this work prevented the determination of an absolute normalization, to be addressed in future measurements. Instead, the measured cross section ratio has been normalized to ENDF/B-VIII.β5 at 14.5 MeV.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

New result for the neutron β -asymmetry parameter A 0 from UCNA

Background: The neutron β-decay asymmetry parameter A 0 defines the angular correlation between the spin of the neutron and the momentum of the emitted electron. Values for A 0 permit an extraction of the ratio of the weak axial-vector to vector coupling constants, λ≡g A /g V , which under assumption of the conserved vector current hypothesis (g V =1) determines g A . Precise values for g A are important as a benchmark for lattice QCD calculations and as a test of the standard model. Purpose: The UCNA experiment, carried out at the Ultracold Neutron (UCN) source at the Los Alamos Neutron Science Center, was the first measurement of any neutron β-decay angular correlation performed with UCN. This article reports the most precise result for A 0 obtained to date from the UCNA experiment, as a result of higher statistics and reduced key systematic uncertainties, including from the neutron polarization and the characterization of the electron detector response. Methods: UCN produced via the downscattering of moderated spallation neutrons in a solid deuterium crystal were polarized via transport through a 7 T polarizing magnet and a spin flipper, which permitted selection of either spin state. The UCN were then contained within a 3-m long cylindrical decay volume, situated along the central axis of a superconducting 1 T solenoidal spectrometer. With the neutron spins then oriented parallel or anti-parallel to the solenoidal field, an asymmetry in the numbers of emitted decay electrons detected in two electron detector packages located on both ends of the spectrometer permitted an extraction of A 0 . Results: The UCNA experiment reports a new 0.67% precision result for A 0 of A 0 = -0.12054(44) stat (68) syst , which yields λ=g A /g V = -1.2783(22). Combination with the previous UCNA result and accounting for correlated systematic uncertainties produces A 0 = -0.12015(34) stat (63) syst and λ=g A /g V = -1.2772(20).Conclusions: This new result for A 0 and g A /g V from the UCNA experiment has provided confirmation of the shift in values for g A /g V that has emerged in the published results from more recent experiments, which are in striking disagreement with the results from older experiments. Individual systematic corrections to the asymmetries in older experiments (published prior to 2002) were >10%, whereas those in the more recent ones (published after 2002) have been of the scale of <2%. Finally, the impact of these older results on the global average will be minimized should future measurements of A 0 reach the 0.1% level of precision with central values near the most recent results.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2018

Unifying measurement of Pu 239 ( n , γ ) in the keV to MeV energy regime

A single, unifying measurement of the 239 Pu capture cross section from 1 keV to 1.3 MeV has been performed for the first time using the Detector for Advanced Neutron Capture Experiments (DANCE) at the Los Alamos Neutron Science Center (LANSCE). The experimental method combines a prior experiment's characterization of prompt fission γ rays in conjunction with a fission tagging detector with a separate experiment using a thick 239 Pu sample to extract the neutron capture cross section in ratio to 239 Pu (n, f). We have made new predictions of the capture cross section taking into account recent results for the M1 scissors mode present in other actinides. The results show deviations from current evaluations which are 30% higher at the highest energies, and will be used to improve calculations relevant for several applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Neutron inelastic scattering measurements on Xe 136 at E n = 0.7 to 100 MeV

Experiments searching for neutrinoless double ${\beta}$ decay ($0{\nu}{\beta}{\beta}$) require precise energy calibration and extremely low backgrounds. One of the most popular isotopes for $0{\nu}{\beta}{\beta}$ experiments is $^{136}\mathrm{Xe}$. In support of these experiments, the neutron inelastic scattering properties of this isotope have been measured at the GErmanium Array for Neutron Induced Excitations (GEANIE) at the Los Alamos Neutron Science Center. Time-of-flight techniques are utilized with high-purity germanium detectors to search for inelastic scattering ${\gamma}$ rays for neutron energies between 0.7 and 100 MeV. Limits are set on production of yet-unobserved ${\gamma}$ rays in the energy range critical for $0{\nu}{\beta}{\beta}$ studies, and measurements are made of multiple ${\gamma}$-ray production cross sections. In particular, we have measured the production of the 1313 keV ${\gamma}$ ray, which comes from the transition of the first-excited to ground state of $^{136}\mathrm{Xe}$. This neutron-induced ${\gamma}$ line may be useful for a novel energy calibration technique.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2019

Statistical neutron capture in the limit of low nuclear level density

A major barrier in the study of neutron-induced nuclear reactions is the impossibility of direct measurements with short-lived radioactive isotopes. For these exotic nuclei, theoretical inputs such as the Photon Strength Function (PSF) are poorly constrained. At Los Alamos National Laboratory, the Detector for Advanced Neutron Capture Experiments (DANCE) provides direct measurements of γ-ray cascades following neutron capture reactions on stable or long-lived radioactive nuclei. While Hauser-Feshbach calculations can provide reasonable predictions for neutron capture on heavy nuclei, their application to neutron-rich light nuclei with low nuclear level densities and low neutron separation energies is questionable. In this paper, we report on the γ-ray spectra from individual neutron resonances from the 96 Zr(n, γ) reaction, with an emphasis on the sensitivity of of the γ-ray spectra to different PSF models. The comparison of the measured γ-ray spectra with predicted spectra does not support the addition of a low-energy enhancement of the size reported in many charged-particle reaction measurements, but the sensitivity of the γ-ray spectra to different PSF models is weak.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Ergodic and nonergodic many-body dynamics in strongly nonlinear lattices

The study of nonlinear oscillator chains in classical many-body dynamics has a storied history going back to the seminal work of Fermi et al. [Los Alamos Scientific Laboratory Report No. LA-1940, 1955 (unpublished)]. Here, we introduce a family of such systems which consist of chains of N harmonically coupled particles with the nonlinearity introduced by confining the motion of each individual particle to a box or stadium with hard walls. The stadia are arranged on a one-dimensional lattice but they individually do not have to be one dimensional, thus permitting the introduction of chaos already at the lattice scale. For the most part we study the case where the motion is entirely one dimensional. We find that the system exhibits a mixed phase space for any finite value of N . Computations of Lyapunov spectra at randomly picked phase space locations and a direct comparison between Hamiltonian evolution and phase space averages indicate that the regular regions of phase space are not significant at large system sizes. While the continuum limit of our model is itself a singular limit of the integrable sinh Gordon theory, we do not see any evidence for the kind of nonergodicity famously seen in the work of Fermi et al. Finally, we examine the chain with particles confined to two-dimensional stadia where the individual stadium is already chaotic and find a much more chaotic phase space at small system sizes.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗