Impact of f-d Kondo cloud on superconductivity of nickelates
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75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
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Effects of Southeastern Pacific Sea Surface Temperature on the Double-ITCZ Bias in NCAR CESM1
The double intertropical convergence zone (ITCZ) is a long-standing bias in the climatology of coupled general circulation models (CGCMs). The warm biases in southeastern Pacific (SEP) sea surface temperature (SST) are also evident in many CGCMs. In this study, the role of SEP SST in the double ITCZ is investigated by prescribing the observed SEP SST in the Community Earth System Model, version 1 (CESM1). Both the double ITCZ and dry equator problems are significantly improved with SEP SST prescribed. Both atmospheric and oceanic processes are involved in the improvements. The colder SST over the SEP decreases the precipitation, which enhances the southeasterly winds outside the prescribed SST region, cooling the ocean via increased evaporation. The enhanced descending motion over the SEP strengthens the Walker circulation. The easterly winds over the equatorial Pacific enhance upwelling and shoal the thermocline over the eastern Pacific. The changes of surface wind and wind curl lead to a weaker South Equatorial Countercurrent and stronger South Equatorial Current, preventing the warm water from expanding eastward, thereby improving both the double ITCZ and dry equator. The enhanced Walker circulation also increases the low-level wind convergence and reduces the wind speed in the tropical western Pacific, leading to warmer SST and stronger convection there. The stronger convection in turn leads to more cloud and reduces the incoming solar radiation, cooling the SST. These competing effects between radiative heat flux and latent heat flux make the atmospheric heat flux secondary to the ocean dynamics in the western Pacific warming.
54 ENVIRONMENTAL SCIENCES↗
Interfacial Dark Aging Is an Overlooked Source of Aqueous Secondary Organic Aerosol
In this work, the relative yields of aqueous secondary organic aerosols (aqSOAs) at the air–liquid (a–l) interface are investigated between photochemical and dark aging using in situ time-of-flight secondary ion mass spectrometry (ToF-SIMS). Our results show that dark aging is an important source of aqSOAs despite a lack of photochemical drivers. Photochemical reactions of glyoxal and hydroxyl radicals (•OH) produce oligomers and cluster ions at the aqueous surface. Interestingly, different oligomers and cluster ions form intensely in the dark at the a–l interface, contrary to the notion that oligomer formation mainly depends on light irradiation. Furthermore, cluster ions form readily during dark aging and have a higher water molecule adsorption ability. This finding is supported by the observation of more frequent organic water cluster ion formation. The relative yields of water clusters in the form of protonated and hydroxide ions are presented using van Krevelen diagrams to explore the underlying formation mechanisms of aqSOAs. Large protonated and hydroxide water clusters (e.g., (H2O)nH+, 17 < n ≤ 44) have reasonable yields during UV aging. In contrast, small protonated and hydroxide water clusters (e.g., (H2O)nH+, 1 ≤ n ≤ 17) form after several hours of dark aging. Moreover, cluster ions have higher yields in dark aging, indicating the overlooked influence of dark aging interfacial products on aerosol optical properties. Molecular dynamic simulation shows that cluster ions form stably in UV and dark aging. AqSOAs molecules produced from dark and photochemical aging can enhance UV absorption of the aqueous surface, promote cloud condensation nuclei (CCN) activities, and affect radiative forcing.
Van Krevelen diagram↗
Supersaturation, buoyancy, and deep convection dynamics
Motivated by recent discussions concerning differences of convective dynamics in polluted and pristine environments, the so-called convective invigoration in particular, this paper provides an analysis of factors affecting convective updraft buoyancy, such as the in-cloud supersaturation, condensate and precipitation loading, and entrainment. We use the deep convective period from simulations of daytime convection development over land discussed in our previous publications. An entraining parcel framework is used in the theoretical analysis. We show that for the specific case considered here, finite (positive) supersaturation noticeably reduces pseudo-adiabatic parcel buoyancy and cumulative convective available potential energy (cCAPE) in the lower troposphere. This comes from keeping a small fraction of the water vapor in a supersaturated state and thus reducing the latent heating. Such a lower-tropospheric impact is comparable to the effects of condensate loading and entrainment in the idealized parcel framework. For the entire tropospheric depth, loading and entrainment have a much more significant impact on the total CAPE. For the cloud model results, we compare ensemble simulations applying either a bulk microphysics scheme with saturation adjustment or a more comprehensive double-moment scheme with supersaturation prediction. We compare deep convective updraft velocities, buoyancies, and supersaturations from all ensembles. In agreement with the parcel analysis, the saturation-adjustment scheme provides noticeably stronger updrafts in the lower troposphere. For the simulations predicting supersaturation, there are small differences between pristine and polluted conditions below the freezing level that are difficult to explain by standard analysis of the in-cloud buoyancy components. By applying the piggybacking technique, we show that the lower-tropospheric buoyancy differences between pristine and polluted simulations come from a combination of temperature (i.e., latent heating) and condensate loading differences that work together to make polluted buoyancies and updraft velocities slightly larger when compared to their pristine analogues. Overall, the effects are rather small and contradict previous claims of a significant invigoration of deep convection in polluted environments.
54 ENVIRONMENTAL SCIENCES↗
Design of the UCLA general circulation model
An edited version is reported of notes distributed at the Summer Workshop on the UCLA General Circulation Model in June 1971. It presents the computational schemes of the UCLA model, along with the mathematical and physical principles on which these schemes are based. Included are the finite difference schemes for the governing fluid-dynamical equations, designed to maintain the important integral constraints and dispersion characteristics of the motion. Also given are the principles of parameterization of cumulus convection by an ensemble of identical clouds. A model of the ground hydrology, involving the liquid, ice and snow states of water, is included. A short summary is given of the scheme for computing solar and infrared radiation transfers through clear and cloudy air.
Arakawa, A.↗
Rain scavenging of solid rocket exhaust clouds
An explicit model for cloud microphysics was developed for application to the problem of co-condensation/vaporization of HCl and H2O in the presence of Al2O3 particulate nuclei. Validity of the explicit model relative to the implicit model, which has been customarily applied to atmospheric cloud studies, was demonstrated by parallel computations of H2O condensation upon (NH4)2 SO4 nuclei. A mesoscale predictive model designed to account for the impact of wet processes on atmospheric dynamics is also under development. Input data specifying the equilibrium state of HC1 and H2O vapors in contact with aqueous HC1 solutions were found to be limited, particularly in respect to temperature range.
Dingle, A. N.↗
Uranus atmospheric dynamics and circulation
The observations, models, and theories relevant to the atmospheric dynamics and meteorology of Uranus are discussed. The available models for the large-scale heat transport and atmospheric dynamics as well as diagnostic interpretations of the Voyager data are reviewed. Some pertinent ideas and questions regarding the global circulation balance are considered, partly in comparison with other planetary atmospheres. The available data indicate atmospheric rotation at midlatitudes nearly 200 m/s faster than that of the planetary magnetic field. Analysis of the dynamical deformation of the shape and size of isobaric surfaces measured by the Voyager radio-occultation experiment suggests a subrotating equator at comparable altitudes. Infrared temperature retrievals above the cloud deck indicate a smaller equator-to-pole contrast than expected for purely radiative-convective equilibrium, but show local variations implying a latitudinally correlated decrease with altitude in the cloud-tracked wind.
Allison, Michael↗
Incremental triangulation by way of edge swapping and local optimization
This document is intended to serve as an installation, usage, and basic theory guide for the two dimensional triangulation software 'HARLEY' written for the Silicon Graphics IRIS workstation. This code consists of an incremental triangulation algorithm based on point insertion and local edge swapping. Using this basic strategy, several types of triangulations can be produced depending on user selected options. For example, local edge swapping criteria can be chosen which minimizes the maximum interior angle (a MinMax triangulation) or which maximizes the minimum interior angle (a MaxMin or Delaunay triangulation). It should be noted that the MinMax triangulation is generally only locally optical (not globally optimal) in this measure. The MaxMin triangulation, however, is both locally and globally optical. In addition, Steiner triangulations can be constructed by inserting new sites at triangle circumcenters followed by edge swapping based on the MaxMin criteria. Incremental insertion of sites also provides flexibility in choosing cell refinement criteria. A dynamic heap structure has been implemented in the code so that once a refinement measure is specified (i.e., maximum aspect ratio or some measure of a solution gradient for the solution adaptive grid generation) the cell with the largest value of this measure is continually removed from the top of the heap and refined. The heap refinement strategy allows the user to specify either the number of cells desired or refine the mesh until all cell refinement measures satisfy a user specified tolerance level. Since the dynamic heap structure is constantly updated, the algorithm always refines the particular cell in the mesh with the largest refinement criteria value. The code allows the user to: triangulate a cloud of prespecified points (sites), triangulate a set of prespecified interior points constrained by prespecified boundary curve(s), Steiner triangulate the interior/exterior of prespecified boundary curve(s), refine existing triangulations based on solution error measures, and partition meshes based on the Cuthill-McKee, spectral, and coordinate bisection strategies.
Wiltberger, N. Lyn↗
Evaluation of Cloud Physical Properties of ECMWF Analysis and Re-Analysis (ERA-40 and ERA Interim) against CERES Tropical Deep Convective Cloud Object Observations
This study presents an approach that converts the vertical profiles of grid-averaged cloud properties from large-scale models to probability density functions (pdfs) of subgrid-cell cloud physical properties measured at satellite footprints. Cloud physical and radiative properties, rather than just cloud and precipitation occurrences, of assimilated cloud systems by the European Center for Medium-range Weather Forecasts (ECMWF) operational analysis (EOA) and ECMWF Re-Analyses (ERA-40 and ERA Interim) are validated against those obtained from Earth Observing System satellite cloud object data for January-August 1998 and March 2000 periods. These properties include ice water path (IWP), cloud-top height and temperature, cloud optical depth and solar and infrared radiative fluxes. Each cloud object, a contiguous region with similar cloud physical properties, is temporally and spatially matched with EOA and ERA-40 data. Results indicate that most pdfs of EOA and ERA-40 cloud physical and radiative properties agree with those of satellite observations of the tropical deep convective cloud-object type for the January-August 1998 period. There are, however, significant discrepancies in selected ranges of the cloud property pdfs such as the upper range of EOA cloud top height. A major discrepancy is that the dependence of the pdfs on the cloud object size for both EOA and ERA-40 is not as strong as in the observations. Modifications to the cloud parameterization in ECMWF that occurred in October 1999 eliminate the clouds near the tropopause but shift power of the pdf to lower cloud-top heights and greatly reduce the ranges of IWP and cloud optical depth pdfs. These features persist in ERA-40 due to the use of the same cloud parameterizations. The downgrade of data assimilation technique and the lack of snow water content information in ERA-40, not the coarser horizontal grid resolution, are also responsible for the disagreements with observed pdfs of cloud physical properties although the detection rates of cloud object occurrence are improved for small size categories. A possible improvement to the convective parameterization is to introduce a stronger dependence of updraft penetration heights with grid-cell dynamics. These conclusions will be rechecked using the ERA Interim data, due to recent changes in the ECMWF convective parameterization (Bechtold et al. 2004, 2008). Results from the ERA Interim will be presented at the meeting.
Xu, Kuan-Man↗
Leveraging CSPP: Building a cloud based direct broadcast processing system
Reducing the time that it takes to have useful satellite information is very important because timely access allows for more informed decision making. This is especially true in time critical situations like disaster response and financial market analysis. One way to achieve reductions in the overall time between information capture and delivery to use the direct broadcast from weather satellites. In this work, we describe a state driven satellite information system that captures a satellite’s direct broadcast signal and uses cloud-based resources to provide end-user controlled processing. The system takes advantage of the reliability and customizability of Amazon Web Services to provide fast and reliable access to a system that takes the direct broadcast signal and leverages the CSPP software as well as dynamically supplied end-user processing modules to produce a user desired information product. Finally, we describe the development process and how a flexible design allowed for changes as the capabilities of the processing platform evolved and the lessons we learned from the process.
CSPP↗
Variational Assimilation of Global Microwave Rainfall Retrievals: Physical and Dynamical Impact on GEOS Analyses and Forecasts
Global microwave rainfall retrievals from a 5-satellite constellation, including TMI from TRMM, SSWI from DMSP F13, F14 and F15, and AMSR-E from EOS-AQUA, are assimilated into the NASA Goddard Earth Observing System (GEOS) Data Assimilation System (DAS) using a 1-D variational continuous assimilation (VCA) algorithm. The physical and dynamical impact of rainfall assimilation on GEOS analyses and forecasts is examined at various temporal and spatial scales. This study demonstrates that the 1-D VCA algorithm, which was originally developed and evaluated for rainfall assimilations over tropical oceans, can effectively assimilate satellite microwave rainfall retrievals and improve GEOS analyses over both the Tropics and the extratropics where the atmospheric processes are dominated by different large-scale dynamics and moist physics, and also over the land, where rainfall estimates from passive microwave radiometers are believed to be less accurate. Results show that rainfall assimilation renders the GEOS analysis physically and dynamically more consistent with the observed precipitation at the monthly-mean and 6-hour time scales. Over regions where the model precipitation tends to misbehave in distinctly different rainy regimes, the 1-D VCA algorithm, by compensating for errors in the model s moist time-tendency in a 6-h analysis window, is able to bring the rainfall analysis closer to the observed. The radiation and cloud fields also tend to be in better agreement with independent satellite observations in the rainfall-assimilation m especially over regions where rainfall analyses indicate large improvements. Assimilation experiments with and without rainfall data for a midlatitude frontal system clearly indicates that the GEOS analysis is improved through changes in the thermodynamic and dynamic fields that respond to the rainfall assimilation. The synoptic structures of temperature, moisture, winds, divergence, and vertical motion, as well as vorticity are more realistically captured across the front. Short-term forecasts using initial conditions assimilated with rainfall data also show slight improvements. 1
Lin, Xin↗
Calculations of the radiative and dynamical state of the Venus atmosphere
Results are reported for accurate multiple-scattering calculations to determine the solar-energy deposition profile in the atmosphere of Venus. It is found that most of the absorbed energy is deposited in the main cloud-layer region, located at altitudes above 35 km, and that the ground receives approximately 3% of the energy absorbed in toto by Venus. Using these results, vertical temperature profiles are computed under conditions of pure radiative equilibrium and radiative-convective equilibrium. Since the latter results satisfactorily match the temperature structure determined from various spacecraft observations, it is inferred that the greenhouse effect can account for the high surface temperature. Aerosols make an important contribution to the infrared opacity in these calculations. Preliminary three-dimensional calculations of the general circulation of the atmosphere are discussed which incorporate the results of the radiative calculations.
Pollack, J. B.↗
Thermal structure and dynamics of Saturn and Jupiter
High resolution Voyager IRIS measurements for Saturn and Jupiter are assembled in meridional cross sections of the retrieved upper tropospheric temperatures. The calculated thermal wind shear in the upper troposphere is highly correlated on both planets with the cloud top winds derived from imaging data. In contrast, temperatures below approximately 300 mbar are not simply related to the zonal jet structure. The upper tropospheric temperatures seem to have been more consistently correlated with cloud top winds than with major albedo features at the time of the Voyager encounters.
Pirraglia, J. A.↗
New Empirical Formulation for the Sublimational Breakup of Graupel and Dendritic Snow
Abstract Ice fragments are generated by sublimation of ice particles in subsaturated conditions in natural clouds. Conceivably, such sublimational breakup would be expected to cause ice multiplication in natural clouds. Any fragment that survives will grow to become ice precipitation that may sublimate and fragment further. As a first step toward assessing this overlooked process, a formulation is proposed for the number of ice fragments from sublimation of ice particles for an atmospheric model. This is done by amalgamating laboratory observations from previously published studies. The concept of a “sublimated mass activity spectrum” for the breakup is applied to the dataset. The number of ice fragments is determined by the relative humidity over ice and the initial size of the parent ice particles. The new formulation applies to dendritic crystals and heavily rimed particles only. Finally, a thought experiment is performed for an idealized scenario of subsaturation with in-cloud descent. Scaling analysis yields an estimate of an ice enhancement ratio of about 5 (10) within a weak deep convective downdraft of about 2 m s −1 , for an initial monodisperse population of dendritic snow (graupel) particles of 3 L −1 and 2 mm. During descent, there is a dynamic equilibrium between continual emission of fragments and their depletion by sublimation. A simplified bin microphysics parcel model exhibits this dynamical quasi equilibrium, consistent with the thought experiment. The fragments have average lifetimes of around 90 and 70 s for dendrites and graupel, respectively. Sublimational breakup is predicted to cause significant secondary ice production.
54 ENVIRONMENTAL SCIENCES↗
Statistical Theory on the Functional Form of Cloud Particle Size Distributions
Abstract Several functional forms of cloud particle size distributions (PSDs) have been used in numerical modeling and remote sensing retrieval studies of clouds and precipitation, including exponential, gamma, lognormal, and Weibull distributions. However, there is no satisfying theoretical explanation as to why certain distribution forms preferentially occur instead of others. Intuitively, the analytical form of a PSD can be derived by directly solving the general dynamic equation, but no analytical solutions have been found yet. Instead of a process-level approach, the use of the principle of maximum entropy (MaxEnt) for determining the theoretical form of PSDs from the perspective of system is examined here. MaxEnt theory states that the probability density function with the largest information entropy among a group satisfying the given properties of the variable should be chosen. Here, the issue of variability under coordinate transformations that arises using the Gibbs–Shannon definition of entropy is identified, and the use of the concept of relative entropy to avoid these problems is discussed. Focusing on cloud physics, the four-parameter generalized gamma distribution is proposed as the analytical form of a PSD using the principle of maximum (relative) entropy with assumptions on power-law relations among state variables, scale invariance, and a further constraint on the expectation of one state variable (e.g., bulk water mass). The four-parameter generalized gamma distribution is very flexible to accommodate various type of constraints that could be assumed for cloud PSDs.
54 ENVIRONMENTAL SCIENCES↗
Fast Molecular Cloud Destruction Requires Fast Cloud Formation
A large fraction of the gas in the Galaxy is cold, dense, and molecular. If all this gas collapsed under the influence of gravity and formed stars in a local free-fall time, the star formation rate in the Galaxy would exceed that observed by more than an order of magnitude. Other star-forming galaxies behave similarly. Yet, observations and simulations both suggest that the molecular gas is indeed gravitationally collapsing, albeit hierarchically. Prompt stellar feedback offers a potential solution to the low observed star formation rate if it quickly disrupts star-forming clouds during gravitational collapse. However, this requires that molecular clouds must be short-lived objects, raising the question of how so much gas can be observed in the molecular phase. This can occur only if molecular clouds form as quickly as they are destroyed, maintaining a global equilibrium fraction of dense gas. We therefore examine cloud formation timescales. We first demonstrate that supernova and superbubble sweeping cannot produce dense gas at the rate required to match the cloud destruction rate. On the other hand, Toomre gravitational instability can reach the required production rate. We thus argue that, although dense, star-forming gas may last only around a single global free-fall time; the dense gas in star-forming galaxies can globally exist in a state of dynamic equilibrium between formation by gravitational instability and disruption by stellar feedback. At redshift z ≳ 2, the Toomre instability timescale decreases, resulting in a prediction of higher molecular gas fractions at early times, in agreement with the observations.
79 ASTRONOMY AND ASTROPHYSICS↗
RICH KOZAI–LIDOV DYNAMICS IN AN INITIALLY THIN AND ECCENTRIC STELLAR DISK AROUND A SUPERMASSIVE BLACK HOLE
There is growing evidence of star formation in the vicinity of supermassive black holes (SMBHs) in galactic nuclei. A viable scenario for this process assumes infall of a massive gas cloud toward the SMBH and subsequent formation of a dense accretion disk, which gives birth to the young stars. Numerical hydrodynamical models indicate that this star formation process is rather fast and precedes full circularization of the accretion flow, i.e., the new stars are born on elliptic orbits. By means of direct numerical N -body modeling, we show in this paper that the nonzero eccentricity of the stellar disks around the SMBH leads to an onset of various types of the Kozai–Lidov oscillations of a non-negligible subset of individual orbits in the disk, showing a remarkable robustness of this classical mechanism. Among others, we demonstrate that under certain circumstances, the presence of an additional spherical cluster (which is generally known to damp Kozai–Lidov oscillations) may trigger such oscillations as a result of affecting the internal flow of the angular momentum through the disk. We conclude that the Kozai–Lidov oscillations are capable of substantially modifying the initial structure of the disk (its thickness and distribution of eccentricities, in particular).
79 ASTRONOMY AND ASTROPHYSICS↗
Temperature structure and dynamics of the middle atmosphere of Venus
Data obtained by the Pioneer Venus Orbiter Infrared Radiometer in late 1978 and early 1979 are presented in tabular form, including, in particular, the mean temperature structure, with complete latitudinal and longitudinal coverage, and zonal-mean cloud properties. The mean thermal and cloud structures can be interpreted in terms of general circulation of the middle atmosphere. The interim results indicate that (1) the zonal winds on Venus fall to very low values above 90 km, (2) there is a strong midlatitude jet which circles the planet approximately every two days, and (3) the observed solar tides are dominated by the semidiurnal component.
Taylor, F. W.↗