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At least 1,765 records · Page 98

FLOWERS AEP: An Analytical Model for Wind Farm Layout Optimization

Annual energy production (AEP) is commonly used in objective functions for wind farm layout optimization. AEP is proportional to wind farm power production integrated over an annual distribution of free-stream wind conditions. Physics-based estimates of wind farm power production typically rely on low-fidelity engineering wake models that approximate the steady-state wind farm flow field. AEP estimates are then obtained by performing independent simulations for discrete wind conditions and using rectangular quadrature to account for each condition's expected frequency of occurrence. Depending on the number of simulated discrete wind conditions, this numerical integral could be hampered by poor accuracy or high computational costs. The FLOWERS AEP model instead poses an analytical integral of the engineering wake model over the variable wind conditions, yielding a closed-form, analytical function for wind farm AEP. This paper derives the analytical functions for FLOWERS AEP and its derivatives with respect to turbine position, which are useful for gradient-based wind farm layout optimization, in nondimensional form. We then analyze the benefits of the FLOWERS AEP model over conventional reference models, focusing on its low cost, adequate wake loss predictions, and smooth design space. Although the FLOWERS approach is found to predict the exact value of AEP with some error relative to the reference model (within 14% on average), it dramatically reduces computation time by an order of magnitude, produces a qualitatively similar design space at relatively low resolution, and yields comparable optimal layouts. This significant speed improvement is critical in layout optimization applications, where determining an optimal layout in an efficient manner is more important than precise AEP prediction.

17 WIND ENERGY↗

Optimally configuring a measurement system to detect diversions from a nuclear fuel cycle

The civilian nuclear fuel cycle is an industrial process that produces electrical power from the nuclear fission of uranium. Using a measurement system to accurately account for nuclear material, such as uranium, in a fuel cycle is important because of the possible loss or diversion of this potentially dangerous material. A measurement system is defined by a set of measurement methods, or “devices,” used to account for material flows and inventory values at specific locations in the fuel cycle. Here, we develop a simulation-optimization algorithm and an integer-programming model to find the best, or near-best, resource-limited measurement system with a high degree of confidence. The simulation-optimization algorithm minimizes a weighted sum of false positive and false negative diversion-detection probabilities while accounting for material quantities and measurement errors across a finite, discrete time horizon in hypothetical non-diversion and diversion contexts. In each time period, the estimated cumulative material unaccounted for is compared to a fixed or an optimized threshold value to assess if a “significant amount of material” is lost from a measurement system. The integer-programming model minimizes the population variance of the estimated material loss, i.e., material unaccounted for, in a measurement system. We analyze three potential problems in nuclear fuel cycle measurement systems: (i) given location-dependent device precisions, find the configuration of n devices at n locations ( n = 3) that gives the lowest corresponding objective values using the simulation-optimization algorithm and integer-programming model, (ii) find the location at which improving device precision reduces objective values the most using the simulation-optimization algorithm, and determine the effect of measurement frequency on measurement system configurations and objective values using the simulation-optimization algorithm. We obtain comparable results for each problem at least an order of magnitude faster than existing methods do. Using an optimized, rather than fixed, detection threshold in the simulation-optimization algorithm reduces the weighted sum of false positive and false negative probabilities.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Status on the Development of a Modeling and Simulation Framework for the Economic Assessment of Nuclear Hybrid Energy

Continued effort to design and build a modeling and simulation framework to assess the economic viability of Nuclear Hybrid Energy Systems (NHES) was undertaken in fiscal year (FY) 2016. The purpose of this report is to document the various tasks associated with the development of such a framework and to provide a status of their progress. Several tasks have been accomplished. First, a synthetic time history generator has been developed in RAVEN, which consists of Fourier series and autoregressive moving average model. The former is used to capture the seasonal trend in historical data, while the latter is to characterize the autocorrelation in residue time series (e.g., measurements with seasonal trends subtracted). As demonstration, both synthetic wind speed and grid demand are generated, showing matching statistics with database. In order to build a design and operations optimizer in RAVEN, a new type of sampler has been developed with highly object-oriented design. In particular, simultaneous perturbation stochastic approximation algorithm is implemented. The optimizer is capable to drive the model to optimize a scalar objective function without constraint in the input space, while the constraints handling is a work in progress and will be implemented to improve the optimization capability. Furthermore, a simplified cash flow model of the performance of an NHES in the electric market has been developed in Python and used as external model in RAVEN to confirm expectations on the analysis capability of RAVEN to provide insight into system economics and to test the capability of RAVEN to identify limit surfaces. Finally, an example calculation is performed that shows the integration and proper data passing in RAVEN of the synthetic time history generator, the cash flow model and the optimizer. It has been shown that the developed Python models external to RAVEN are able to communicate with RAVEN and each other through the newly developed RAVEN capability called “EnsembleModel”.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Advanced Fluid Reduced Order Models for Compressible Flow.

This report summarizes fiscal year (FY) 2017 progress towards developing and implementing within the SPARC in-house finite volume flow solver advanced fluid reduced order models (ROMs) for compressible captive-carriage flow problems of interest to Sandia National Laboratories for the design and qualification of nuclear weapons components. The proposed projection-based model order reduction (MOR) approach, known as the Proper Orthogonal Decomposition (POD)/Least- Squares Petrov-Galerkin (LSPG) method, can substantially reduce the CPU-time requirement for these simulations, thereby enabling advanced analyses such as uncertainty quantification and de- sign optimization. Following a description of the project objectives and FY17 targets, we overview briefly the POD/LSPG approach to model reduction implemented within SPARC . We then study the viability of these ROMs for long-time predictive simulations in the context of a two-dimensional viscous laminar cavity problem, and describe some FY17 enhancements to the proposed model reduction methodology that led to ROMs with improved predictive capabilities. Also described in this report are some FY17 efforts pursued in parallel to the primary objective of determining whether the ROMs in SPARC are viable for the targeted application. These include the implemen- tation and verification of some higher-order finite volume discretization methods within SPARC (towards using the code to study the viability of ROMs on three-dimensional cavity problems) and a novel structure-preserving constrained POD/LSPG formulation that can improve the accuracy of projection-based reduced order models. We conclude the report by summarizing the key takeaways from our FY17 findings, and providing some perspectives for future work.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Characterizing convective cold pools

Abstract Cold pools produced by convective storms play an important role in Earth's climate system. However, a common framework does not exist for objectively identifying convective cold pools in observations and models. The present study investigates convective cold pools within a simulation of tropical continental convection that uses a cloud‐resolving model with a coupled land‐surface model. Multiple variables are assessed for their potential in identifying convective cold pool boundaries, and a novel technique is developed and tested for identifying and tracking cold pools in numerical model simulations. This algorithm is based on surface rainfall rates and radial gradients in the density potential temperature field. The algorithm successfully identifies near‐surface cold pool boundaries and is able to distinguish between connected cold pools. Once cold pools have been identified and tracked, composites of cold pool evolution are then constructed, and average cold pool properties are investigated. Wet patches are found to develop within the centers of cold pools where the ground has been soaked with rainwater. These wet patches help to maintain cool surface temperatures and reduce cold pool dissipation, which has implications for the development of subsequent convection.

54 ENVIRONMENTAL SCIENCES↗

Fabricating 3D Structures by Combining 2D Printing and Relaxation of Strain

This article describes the fabrication of elastomeric three-dimensional (3D) structures starting from two-dimensional (2D) sheets using a combination of direct-ink printing and relaxation of strain. These structures are fabricated in a two-step process: first, elastomeric inks are deposited as 2D structures on a stretched elastomeric sheet, and second, after curing of the elastomeric inks, relaxation of strain in the 2D sheet causes it to deform into a 3D shape. To predict bending of elastomeric objects fabricated with this technique, a simple mechanical model is developed. The strategy of using initially 2D materials to fabricate 3D structures offers four new features that complement digital fabrication techniques. (i) It provides a simple route to create shapes with complex curves, suspended features, and internal cavities. (ii) It is a faster method of fabricating some types of shapes than “conventional” 3D printing, because the features are printed in 2D. (iii) It forms surfaces that can be both smoother, and structured in a way that is not compatible with layer-by-layer processing. (iv) It forms structures that can be deformed reversibly after fabrication by reapplying strain. This paper demonstrates these features by fabrication of helices, structures inspired by cubes and tables, “pop-up” structures, and soft grippers.

36 MATERIALS SCIENCE↗

Reconstructing porous media using generative flow networks

One area of intense scientific interest for the study of sandstones, carbonates, and shale at the pore scale is the use of limited image and petrophysical data to generate multiple realizations of a rock’s pore structure. Such images aid efforts to quantify uncertainty in petrophysical properties, including porosity–permeability transforms. We develop and evaluate a deep learning-based method to synthesize porous media volumes using a so-called generative flow model trained on x-ray microscope images of rock texture and pore structure. These models are optimized on a log-likelihood objective and they synthesize large and realistic three-dimensional images. Further, we demonstrate the rapid generation of sandstone image volumes that display realism as gauged by quantitative comparison of topological features using Minkowski functionals of porosity, specific surface area, and the Euler–Poincaré characteristic (i.e., pore connectivity). We also evaluate the single-phase permeability using Navier–Stokes and lattice Boltzmann methods and show that transport properties of the generated samples match measured trends.

58 GEOSCIENCES↗

A signal compensation based cascaded PI control for an industrial heat exchange system

Since the characteristics of the industrial heat exchange system (HES) are drastically affected by variations of the steam pressure, ambient temperature and water quality, it is difficult for the classical cascade PI control system to meet the desirable control objectives. Therefore, in this paper, a deterministic linear model with unmodeled dynamics is used to describe the dynamic characteristics of the HES. It should be noted that the unmodeled dynamics at the previously sampled instant can be calculated using actual measurements and that the tracking error, which includes effects of the rate of changes of unmodeled dynamics on the controlled model, can be accurately determined. An additional compensating signal is obtained with the feedforward control together with a one-step optimal control law. Consequently, the cascade PI control strategy with the signal compensation is established. Furthermore, the simulation and industrial application show that the proposed method can effectively improve the performance of the cascade PI control system, especially when the unmodeled dynamics is subjected to unknown variations.

42 ENGINEERING↗

Molecular-Level Insights into Photocatalysis from Scanning Probe Microscopy Studies on TiO2(110)

The field of heterogeneous photocatalysis has grown considerably in the decades since Fujishima and Honda's ground-breaking publications of photoelectrochemistry on TiO2. Numerous review articles continue to point to both progress made in the use of heterogeneous materials (such as TiO2) to perform photoconversion processes, and the many opportunities and challenges in heterogeneous photocatalysis research such as solar energy conversion and environmental remediation. The past decade has also seen an increase in the use of molecular-level approaches applied to model single crystal surfaces in an effort to obtain new insights into photocatalytic phenomena. In particular, scanning probe techniques (SPM) have enabled researchers to take a ‘nanoscale’ approach to photocatalysis that includes interrogation of the reactivities of specific sites and adsorbates on a model photocatalyst surface. The rutile TiO2(110) surface has become the prototypical oxide single crystal surface for fundamental studies of many interfacial phenomena. In particular, TiO2(110) has become an excellent model surface for probing photochemical and photocatalytic reactions at the molecular level. A variety of experimental approaches have emerged as being ideally suited for studying photochemical reactions on TiO2(110), including desorption-oriented approaches and electronic spectroscopies, but perhaps the most promising techniques for evaluating site-specific properties are those of SPM. In this review, we highlight the growing use of SPM techniques in providing molecular-level insights into surface photochemistry on the model photocatalyst surface of rutile TiO2(110). Our objective is to both illustrate the unique knowledge that scanning probe techniques have already provided the field of photocatalysis, and also to motivate a new generation of effort into the use of such approaches to obtain new insights into the molecular level details of photochemical events occurring at interfaces. Discussion will start with an examination of how scanning probe techniques are being used to characterize the TiO2(110) surface in ways that are relevant to photocatalysis. We will then discuss specific classes of photochemical reaction on TiO2(110) for which SPM has proven indispensible in providing unique molecular-level insights, and conclude with discussion of future areas in which SPM studies may prove valuable to photocatalysis on TiO2. This work was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. I.L. was partially supported by a Pacific Northwest National Laboratory (PNNL) Chemical Imaging Initiative project. PNNL is a multiprogram national laboratory operated for DOE by Battelle.

photocatalysis↗

Autonomous reinforcement learning agent for chemical vapor deposition synthesis of quantum materials

Abstract Predictive materials synthesis is the primary bottleneck in realizing functional and quantum materials. Strategies for synthesis of promising materials are currently identified by time-consuming trial and error and there are no known predictive schemes to design synthesis parameters for materials. We use offline reinforcement learning (RL) to predict optimal synthesis schedules, i.e., a time-sequence of reaction conditions like temperatures and concentrations, for the synthesis of semiconducting monolayer MoS 2 using chemical vapor deposition. The RL agent, trained on 10,000 computational synthesis simulations, learned threshold temperatures and chemical potentials for onset of chemical reactions and predicted previously unknown synthesis schedules that produce well-sulfidized crystalline, phase-pure MoS 2 . The model can be extended to multi-task objectives such as predicting profiles for synthesis of complex structures including multi-phase heterostructures and can predict long-time behavior of reacting systems, far beyond the domain of molecular dynamics simulations, making these predictions directly relevant to experimental synthesis.

36 MATERIALS SCIENCE↗

Astrometric microlensing probes of the isolated neutron star population with Roman

Notoriously hard to detect and study, isolated neutron stars (NSs) might provide valuable answers to fundamental questions about stellar evolution and explosion physics. With the upcoming Roman Space Telescope, scheduled for launch in 2026, a new and powerful channel for their detection will become available: astrometric microlensing. We set out to create a realistic sample of simulated gravitational microlensing events as observed by Roman with the Galactic Bulge Time Domain Survey. We focus in particular on the population of NS lenses, which has until now been largely understudied. We used dedicated Galactic models tailored for application to microlensing by compact objects. In addition to populations of stars, white dwarfs, and black holes, we simulated four different NS populations with Maxwellian natal kick distributions: v = (150, 250, 350, 450) km/s. For each simulation, we applied projected Roman precision, cadence, and detectability criteria. We found that the parameter space log10 t E –log 10 θ E , which will be accessible to Roman observations, is efficient for the classification of stellar remnants. We found a feature in this space that is characteristic of NSs; using this feature, optimal samples of NS candidates can be constructed from Roman -like datasets. We describe the dependence of the observable parameter distributions on the assumed mean kick velocities. As the effects of natal kicks are very complex and mutually counteracting, we suggest that more detailed studies focused on the dynamics of NSs are needed in anticipation of Roman and future surveys. We estimate that Roman will observe approximately 11 000 microlensing events, including ~100 with NS lenses, whose photometric and astrometric signals are detectable; the event yield decreases by 38% when gap-filling low-cadence observations are not included. We make all simulated microlensing event datasets publicly available in preparation for Roman data.

79 ASTRONOMY AND ASTROPHYSICS↗

Automated Fitting of a Semi-empirical Multiphase Equation of State for Carbon

The equation of state (EOS) of carbon is important in high explosive, geophysical, and inertial confinement fusion applications. Within the semi-empirical Sesame framework, the EOS of each phase is represented by a sum of cold, vibrational, and thermal electronic Helmholtz free energy contributions. Each phase has ~5-10 independent parameters that are adjusted to reproduce single-phase data (e.g., thermal expansion, isothermal compression) as well as experimentally- and computationally- derived phase boundaries. Manual calibration of the full multiphase EOS is arduous. We present our progress in development of automated EOS parameterization based on minimization of an objective function. Here, this function encodes deviation of model EOS results from experimental/computational benchmarks. Optimization is implemented as a combination of global (particle swarm) and local optimization techniques.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

TWO SNe Ia AT REDSHIFT ∼2: IMPROVED CLASSIFICATION AND REDSHIFT DETERMINATION WITH MEDIUM-BAND INFRARED IMAGING

We present two supernovae (SNe) discovered with the Hubble Space Telescope (HST) in the Cosmic Assembly Near-infrared Deep Extragalactic Legacy Survey, an HST multi-cycle treasury program. We classify both objects as SNe Ia and find redshifts of z = 1.80 ± 0.02 and 2.26{sup +0.02}{sub −0.10}, the latter of which is the highest redshift SN Ia yet seen. Using light curve fitting we determine luminosity distances and find that both objects are consistent with a standard ΛCDM cosmological model. These SNe were observed using the HST Wide Field Camera 3 infrared detector, with imaging in both wide- and medium-band filters. We demonstrate that the classification and redshift estimates are significantly improved by the inclusion of single-epoch medium-band observations. This medium-band imaging approximates a very low resolution spectrum (λ/Δλ ≲ 100) which can isolate broad spectral absorption features that differentiate SNe Ia from their most common core collapse cousins. This medium-band method is also insensitive to dust extinction and (unlike grism spectroscopy) it is not affected by contamination from the SN host galaxy or other nearby sources. As such, it can provide a more efficient—though less precise—alternative to IR spectroscopy for high-z SNe.

79 ASTRONOMY AND ASTROPHYSICS↗

Signatures of young star formation activity within two parsecs of Sgr A*

We present radio and infrared observations indicating ongoing star formation activity inside the ∼2–5 pc circumnuclear ring at the Galactic center. Collectively these measurements suggest a continued disk-based mode of ongoing star formation has taken place near Sgr A* over the last few million years. First, Very Large Array observations with spatial resolution 2.″17 × 0.″81 reveal 13 water masers, several of which have multiple velocity components. The presence of interstellar water masers suggests gas densities that are sufficient for self-gravity to overcome the tidal shear of the 4×10{sup 6} M{sub ⊙} black hole. Second, spectral energy distribution modeling of stellar sources indicates massive young stellar object (YSO) candidates interior to the molecular ring, supporting in situ star formation near Sgr A* and appear to show a distribution similar to that of the counter-rotating disks of ∼100 OB stars orbiting Sgr A*. Some YSO candidates (e.g., IRS 5) have bow shock structures, suggesting that they have gaseous disks that are phototoevaporated and photoionized by the strong radiation field. Third, we detect clumps of SiO (2-1) and (5-4) line emission in the ring based on Combined Array for Research in Millimeter-wave Astronomy and Sub-Millimeter Array observations. The FWHM and luminosity of the SiO emission is consistent with shocked protostellar outflows. Fourth, two linear ionized features with an extent of ∼0.8 pc show blue and redshifted velocities between +50 and −40 km s{sup −1}, suggesting protostellar jet driven outflows with mass-loss rates of ∼5×10{sup −5} M{sub ⊙} yr{sup −1}. Finally, we present the imprint of radio dark clouds at 44 GHz, representing a reservoir of molecular gas that feeds star formation activity close to Sgr A*.

79 ASTRONOMY AND ASTROPHYSICS↗

ON THE EVOLUTION OF MAGNETIC WHITE DWARFS

We present the first radiation magnetohydrodynamic simulations of the atmosphere of white dwarf stars. We demonstrate that convective energy transfer is seriously impeded by magnetic fields when the plasma-β parameter, the thermal-to-magnetic-pressure ratio, becomes smaller than unity. The critical field strength that inhibits convection in the photosphere of white dwarfs is in the range B = 1–50 kG, which is much smaller than the typical 1–1000 MG field strengths observed in magnetic white dwarfs, implying that these objects have radiative atmospheres. We have employed evolutionary models to study the cooling process of high-field magnetic white dwarfs, where convection is entirely suppressed during the full evolution (B ≳ 10 MG). We find that the inhibition of convection has no effect on cooling rates until the effective temperature (T{sub eff}) reaches a value of around 5500 K. In this regime, the standard convective sequences start to deviate from the ones without convection due to the convective coupling between the outer layers and the degenerate reservoir of thermal energy. Since no magnetic white dwarfs are currently known at the low temperatures where this coupling significantly changes the evolution, the effects of magnetism on cooling rates are not expected to be observed. This result contrasts with a recent suggestion that magnetic white dwarfs with T{sub eff} ≲ 10,000 K cool significantly slower than non-magnetic degenerates.

79 ASTRONOMY AND ASTROPHYSICS↗

ALMA OBSERVATIONS OF THE GALACTIC CENTER: SiO OUTFLOWS AND HIGH-MASS STAR FORMATION NEAR Sgr A*

ALMA observations of the Galactic center with a spatial resolution of 2.''61 Multiplication-Sign 0.''97 resulted in the detection of 11 SiO (5-4) clumps of molecular gas within 0.6 pc (15'') of Sgr A*, interior to the 2 pc circumnuclear molecular ring. The three SiO (5-4) clumps closest to Sgr A* show the largest central velocities, {approx}150 km s{sup -1}, and the broadest asymmetric line widths with full width zero intensity (FWZI) {approx}110-147 km s{sup -1}. The remaining clumps, distributed mainly to the NE of the ionized mini-spiral, have narrow FWZI ({approx}18-56 km s{sup -1}). Using CARMA SiO (2-1) data, Large Velocity Gradient modeling of the SiO line ratios for the broad velocity clumps constrains the column density N(SiO) {approx}10{sup 14} cm{sup -2}, and the H{sub 2} gas density n{sub H{sub 2}} = (3-9) x 10{sup 5} cm{sup -3} for an assumed kinetic temperature 100-200 K. The SiO clumps are interpreted as highly embedded protostellar outflows, signifying an early stage of massive star formation near Sgr A* in the last 10{sup 4}-10{sup 5} yr. Support for this interpretation is provided by the SiO (5-4) line luminosities and velocity widths which lie in the range measured for protostellar outflows in star-forming regions in the Galaxy. Furthermore, spectral energy distribution modeling of stellar sources shows two young stellar object candidates near SiO clumps, supporting in situ star formation near Sgr A*. We discuss the nature of star formation where the gravitational potential of the black hole dominates. In particular, we suggest that external radiative pressure exerted on self-shielded molecular clouds enhances the gas density, before the gas cloud becomes gravitationally unstable near Sgr A*. Alternatively, collisions between clumps in the ring may trigger gravitational collapse.

79 ASTRONOMY AND ASTROPHYSICS↗

Large binocular telescope observations of new six compact star-forming galaxies with [Ne v ] λ3426 Å emission

ABSTRACT We report the discovery of [Ne v] λ3426 emission, in addition to He ii λ4686 emission, in six compact star-forming galaxies. These observations considerably increase the sample of eight such galaxies discovered earlier by our group. For four of the new galaxies, the optical observations are supplemented by near-infrared spectra. All galaxies, but one, have H ii regions that are dense, with electron number densities of ∼ 300–700 cm−3. They are all characterized by high H β equivalent widths EW(H β) ∼ 190–520 Å and high O32 = [O iii] λ5007/[O ii] λ3727 ratios of 10–30, indicating young starburst ages and the presence of high ionization radiation. All are low-metallicity objects with 12 + logO/H = 7.46–7.88. The spectra of all galaxies show a low-intensity broad component of the H α line and five of six objects show Wolf–Rayet features. Comparison with photoionization models shows that pure stellar ionization radiation from massive stars is not hard enough to produce such strong [Ne v] and He ii emission in our galaxies. The [Ne v] λ3426/He ii λ4686 flux ratio of ∼1.2 in J1222+3602 is consistent with some contribution of active galactic nucleus ionizing radiation. However, in the remaining five galaxies, this ratio is considerably lower, $\lesssim$ 0.4. The most plausible models are likely to be non-uniform in density, where He ii and [Ne v] lines are emitted in low-density channels made by outflows and illuminated by harder ionizing radiation from radiative shocks propagating through these channels, whereas [O iii] emission originates in denser regions exposed to softer stellar ionizing sources.

79 ASTRONOMY AND ASTROPHYSICS↗

Statistical Uncertainty of Inhalation Dose Coefficients: Impact of Particle Deposition in ICRP 66 Human Respiratory Tract Model

Inhaled radioactive materials can pose a long-term health concern, as the material can be incorporated into the body’s metabolic pathways and remain in organs and tissues for extended durations. During the retention period, the radioactive material may localize in a source organ and irradiate adjacent target organs and tissues. Distribution of these materials changes over time, requiring biokinetic modeling to evaluate their movement through various tissues and organs. The evolving distribution depends on multiple inputs characterizing the inhaled material, such as particle size and size distribution, particle density, aspect ratio, specific radionuclide, the chemical form, and solubility. In addition, biological parameters such as breathing rate, breathing type (nasal or nasal/oral), respiratory system morphometry, tidal volume, functional residual capacity, and anatomical dead space all influence material transport. These aerosol properties and physiological characteristics of the respiratory tract jointly define a range of initial conditions that influence the time-dependent distribution of radioactive material. To evaluate both uncertainty in the initial conditions of inhalation exposure and the final output (committed effective dose) from biokinetic models, a Python-based software tool, Radiological Exposure Dose Calculator (REDCAL), was developed to propagate uncertainty within the human respiratory tract model. Focusing on deposition fraction uncertainty, the primary objective was to characterize the initial activity distribution across respiratory regions as a function of anticipated particle sizes and distributions. The impact of the deposition fraction uncertainty was propagated to committed effective dose coefficients for selected radionuclides in a companion publication. For each particle size, a lognormal distribution, characterized by its geometric mean as defined within ICRP Publication 66, serves as the basis for introducing uncertainty into the physical processes governing deposition in various lung regions. Finally, this study addresses the deposition process and examines how uncertainty in deposition mechanisms affects activity distribution in the airways, ultimately presenting the expected range and standard deviation of deposited activity as a function of particle size.

International Commission on Radiological Protectio↗