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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,783 records · Page 99
All sourcesNASA NTRSDOE OSTI
DOE OSTI2014

Quantum Hamiltonian Physics with Supercomputers

The vision of solving the nuclear many-body problem in a Hamiltonian framework with fundamental interactions tied to QCD via Chiral Perturbation Theory is gaining support. The goals are to preserve the predictive power of the underlying theory, to test fundamental symmetries with the nucleus as laboratory and to develop new understandings of the full range of complex quantum phenomena. Advances in theoretical frameworks (renormalization and many-body methods) as well as in computational resources (new algorithms and leadership-class parallel computers) signal a new generation of theory and simulations that will yield profound insights into the origins of nuclear shell structure, collective phenomena and complex reaction dynamics. Fundamental discovery opportunities also exist in such areas as physics beyond the Standard Model of Elementary Particles, the transition between hadronic and quark–gluon dominated dynamics in nuclei and signals that characterize dark matter. I will review some recent achievements and present ambitious consensus plans along with their challenges for a coming decade of research that will build new links between theory, simulations and experiment. Opportunities for graduate students to embark upon careers in the fast developing field of supercomputer simulations is also discussed.

Physics↗
DOE OSTI2020

Divertor heat flux challenge and mitigation in SPARC

Owing to its high magnetic field, high power, and compact size, the SPARC experiment will operate with divertor conditions at or above those expected in reactor-class tokamaks. Power exhaust at this scale remains one of the key challenges for practical fusion energy. Based on empirical scalings, the peak unmitigated divertor parallel heat flux is projected to be greater than 10 GW m -2 . This is nearly an order of magnitude higher than has been demonstrated to date. Furthermore, the divertor parallel Edge-Localized Mode (ELM) energy fluence projections (~11–34 MJ m -2 ) are comparable with those for ITER. However, the relatively short pulse length (~25 s pulse, with a ~10 s flat top) provides the opportunity to consider mitigation schemes unsuited to long-pulse devices including ITER and reactors. The baseline scenario for SPARC employs a ~1 Hz strike point sweep to spread the heat flux over a large divertor target surface area to keep tile surface temperatures within tolerable levels without the use of active divertor cooling systems. In addition, SPARC operation presents a unique opportunity to study divertor heat exhaust mitigation at reactor-level plasma densities and power fluxes. Not only will SPARC test the limits of current experimental scalings and serve for benchmarking theoretical models in reactor regimes, it is also being designed to enable the assessment of long-legged and X-point target advanced divertor magnetic configurations. Experimental results from SPARC will be crucial to reducing risk for a fusion pilot plant divertor design.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Quantitative Proteomics and Quantitative PCR as Predictors of cis -1,2-Dichlorethene and Vinyl Chloride Reductive Dechlorination Rates in Bioaugmented Aquifer Microcosms

Quantitative measurement of process-specific biomarker genes of Dehalococcoides mccartyi (Dhc) supports monitoring at chlorinated ethene contaminated sites. In this study, we varied Dhc cell abundances from ~103 to 108 cells/mL in aquifer microcosms and correlated the corresponding reductive dehalogenase (RDase) gene and RDase protein abundances with measured reductive dechlorination (RD) rates of cis-1,2-dichloroethene (cDCE) and vinyl chloride (VC). An additional set of microcosms tested the RD rate-predictive power of the regression analyses. These efforts revealed (1) that targeted proteomics quantifies Dhc biomarker proteins (e.g., TceA and VcrA, OmeA) over a relevant range of Dhc cell densities, and (2) that protein and gene abundances can predict RD rates. Protein detection limits translated to a rate coefficient of 10 –4 day –1 (0.04 year –1 ) for both k cDCE and k vc , which is within the range observed at sites undergoing monitored natural attenuation (MNA) (i.e., without the implementation of enhanced bioremediation treatment). Rates predicted using a combination of quantitative biomarker gene and protein measurements generally resulted in the best match with experimentally determined rate constants. These new findings provide evidence that quantitative biomarker measurements may be useful predictors of in situ RD rates, which would constitute a major advance for the cost-effective management of contaminated sites.

42 ENGINEERING↗
DOE OSTI2020

Development of an autothermal formate-based hydrogen generator: From optimization of formate dehydrogenation conditions to thermal integration with Fuel Cells

Formate received significant attention for storing H2 in chemical bonds using the concept of H2 carriers. In this report, hydrogen generation from formate was optimized systematically by varying reaction variables. Initial mass activity with a turnover frequency of 3200 molH2 molPd–1 h–1 and 92% H2 yield were obtained in sodium formate (7 M 2.0 mL) dehydrogenation over Pd(3 wt %)/C at 80 °C. Influence of formate cations (Na, K, and NH4) on dehydrogenation was also elucidated, presenting that the fastest initial reaction kinetics was achieved with ammonium formate, whereas the highest H2 yield was obtained with potassium formate (PF) in multiple catalyst recycle tests. Finally, an on-site power generation system was integrated, where a proton exchange membrane fuel cell (PEMFC) was operated in conjunction with H2 produced from the custom developed semibatch dehydrogenation reactors. The system operation was demonstrated with continuous feeding of PF to generate H2 and power on demand without an external heat source by utilizing waste heat produced from the PEMFC in a highly efficient manner.

formate dehydrogenation, optimization of reaction ↗
DOE OSTI2026

Rational design of high-performance low-loading oxygen reduction catalysts for alkaline fuel cells

The lack of mechanistic understanding and catalyst design principles for alkaline electrolytes, especially for the sluggish oxygen reduction reaction, has impeded the advancement of alkaline fuel cells. Here, in this study, we propose a modified volcano plot and apply this rationale to strategically design Pt nanosheets with PdH x nanosheets substrates. This catalyst exhibited high stability with a specific activity of 1.71 mA cm −2 at 0.95 V versus the reversible hydrogen electrode, surpassing the benchmark of Pt/C by 49-fold. Spectroscopic, electrochemical and electron microscopic characterizations revealed that such performance enhancement originated from tensile-strained Pt{111} facets, improving oxidative stability and suppressing carbon corrosion. In fuel cell testing, the catalyst enabled a peak power density of 1.67 W cm −2 with a loading of 10 µg PGM Cathode cm −2 . Further optimization delivered a peak power density of 21.7 W mg −1 PGM Cathode+Anode with a total specific catalyst cost US$\$$1.27 kW −1 , surpassing the US Department of Energy’s Pt group metal loading and cost targets. This study provides valuable insights into catalyst design for the alkaline oxygen reduction reaction.

36 MATERIALS SCIENCE↗
DOE OSTI2011

Soft magnetic properties of (Ni{sub 80}Fe{sub 20}){sub 1-x}(Ni{sub 0.5}Zn{sub 0.5}Fe{sub 2}O{sub 4}){sub x} films for high frequency applications

A series of (Ni{sub 80}Fe{sub 20}){sub 1-x}(Ni{sub 0.5}Zn{sub 0.5}Fe{sub 2}O{sub 4}){sub x} films were fabricated on Si substrates by means of radio frequency magnetron sputtering and the electrical and magnetic properties were studied. Optimal films with the desired properties of low coercivity H{sub c} {approx} 4 Oe, high saturation magnetization 4{pi}Ms {approx} 14.5 kG, and high electrical resistivity {rho} {approx} 1500 {mu}{Omega} cm were obtained. The permeability spectra measured shows that its natural ferromagnetic resonant frequency was about 3.4 GHz. The tested results shown that the sputtering power had an important effect on the films properties and that it can be convenient to adjust the natural ferromagnetic resonant frequency of the films.

36 MATERIALS SCIENCE↗
DOE OSTI2012

Incorporation of the stress concentration slots into the flexures for a high-performance microaccelerometer

Presented in this paper is a development of a high-performance piezoresistive microaccelerometer based on the slot etching in the quad flexures for the vibration detection of high speed spindle. The proposed structure consists of a proof mass supported by four thin flexures with slots etched in the middle. Boron diffused piezoresistors located near the stress concentration regions are used for sensing the localized stress resulting from the incorporation of the slots into the flexures. Theoretical analysis and finite element analysis show satisfactory results of an improved sensitivity and favorable natural frequency higher than 10 kHz, conforming to the initial design requirements. The microfabrication techniques are described to prototype the two accelerometer chips, one with slots and the other one without slots. The tested microaccelerometers with 3 V DC power supply show an average sensitivity of 0.424 mV/g normal to the proof mass plane, increased by 60.6% than the ones without slots. An average transverse sensitivity is found to be 9.2 {mu}V/g along X axis and 14.2 {mu}V/g along Y axis, either of which is less than 3.5% of prime-axis sensitivity. Concerning the resonant frequency, dynamic experiment shows about 12.46 kHz and is available for the proposed design with a tiny loss of 3.5% compared with the quad-beam design. When taking the product of sensitivity and natural frequency as judgment criteria, an inspiring increase by 28.6% of the figure of merit is accomplished for the proposed accelerometer. Overall, the findings of this study confirm the feasibility of incorporating slots into the conventional configurations to improve the sensor sensitivity while maintaining a comparatively high natural frequency.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2016

GMI in the reentrant spin-glass Fe 90 Zr 10 alloy: Investigation of the spin dynamics in the MHz frequency regime

Giant magnetoimpedance (GMI) in the reentrant spin-glass (SG) phase of ferromagnetic Fe 90 Zr 10 is reported. The temperature (T) dependence of the GMI allows the investigation of the spin dynamics in the SG phase in the MHz frequency regime and thus very short relaxation times τ (~10 -8 s). The GMI shows a broad maximum around 150 K and diminishes with decreasing T below the glass temperature T g of 15 K. The magnetic permeability data obtained from the GMI data show the general features observed in the ac magnetic susceptibility measured at lower frequencies (10 ≤ f ≤ 10 4 Hz), yielding values of T f (=T g (f)) that allow testing the validity of the power-law scaling used for describing the dynamics of SG-phases up to 15 MHz. A log-log plot of τ (=1/f) versus the reduced critical temperature shows two distinct regimes in the time-domain: (1) a critical slowing-down is observed for values τ > 3 × 10 -3 s; and (2) for 7 × 10 -8 ≤ τ ≤ 3 × 10 -3 s. In the latter case a fitting to the power-law yields the value 7.4 for the product of the critical exponents zν, and 1.6 × 10 -7 s for the microscopic relaxation time τ 0 . In conclusion, the product of the exponents is appropriate for an Ising spin glass.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Quantifying CTFE content in FK-800 using ATR-FTIR and time to peak crystallization

The chlorotrifluoroethylene (CTFE) content in vinylidene fluoride (VDF)-CTFE copolymers greatly influences the chemical and physical properties and ultimately determines the application. The copolymer known as FK-800 has a VDF:CTFE ratio of ~1:3 and is used almost exclusively as the binder in the insensitive high explosive (HE) formulation PBX 9502. Due to the dangerous nature of HE work and the effect CTFE content variations have, the ability to quickly and easily quantify CTFE content is of interest. Two techniques, attenuated total reflectance-Fourier transform infrared spectroscopy (ATR-FTIR) and time to peak crystallization measured by heat flow calorimetry, were evaluated here as potential means for quantifying CTFE content. Based on the certificate of analyses (COAs), FK-800 lots with varied CTFE content encompassing the range historically used in HE applications were used as standards for both methodologies. For FTIR, a linear regression was performed on the peak area of the C-Cl IR stretch and the CTFE content; the methodology was then demonstrated on four samples, two lots of unadulterated material and material recovered from two HE samples. The calculated CTFE content and COAs were in good agreement for all four samples. Heat flow calorimetry revealed the relationship between time to peak crystallization and CTFE content was best fit by a power regression; the methodology was then tested on two different FK-800 lots. Only one sample showed good agreement between the calculated CTFE content and the COA. This discrepancy indicates the method developed is not suitable for quantifying CTFE, but provides valuable insight regarding the crystallization behavior of VDF-CTFE copolymers.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2018

Supervised classification of electric power transmission line nominal voltage from high-resolution aerial imagery

For many researchers, government agencies, and emergency responders, access to the geospatial data of US electric power infrastructure is invaluable for analysis, planning, and disaster recovery. Historically, however, access to high quality geospatial energy data has been limited to few agencies because of commercial licenses restrictions, and those resources which are widely accessible have been of poor quality, particularly with respect to reliability. Recent efforts to develop a highly reliable and publicly accessible alternative to the existing datasets were met with numerous challenges – not the least of which was filling the gaps in power transmission line voltage ratings. To address the line voltage rating problem, we developed and tested a basic methodology that fuses knowledge and techniques from power systems, geography, and machine learning domains. Specifically, we identified predictors of nominal voltage that could be extracted from aerial imagery and developed a tree-based classifier to classify nominal line voltage ratings. Overall, we found that line support height, support span, and conductor spacing are the best predictors of voltage ratings, and that the classifier built with these predictors had a reliable predictive accuracy (that is, within one voltage class for four out of the five classes sampled). In conclusion, we applied our approach to a study area in Minnesota.

24 POWER TRANSMISSION AND DISTRIBUTION↗
DOE OSTI2011

THE DIFFERENT NATURE OF SEYFERT 2 GALAXIES WITH AND WITHOUT HIDDEN BROAD-LINE REGIONS

We compile a large sample of 120 Seyfert 2 galaxies (Sy2s) which contains 49 hidden broad-line region (HBLR) Sy2s and 71 non-HBLR Sy2s. From the difference in the power sources between two groups, we test whether HBLR Sy2s are dominated by active galactic nuclei (AGNs) and whether non-HBLR Sy2s are dominated by starbursts. We show that (1) HBLR Sy2s have larger accretion rates than non-HBLR Sy2s; (2) HBLR Sy2s have larger [Ne V] {lambda}14.32/[Ne II] {lambda}12.81 and [O IV] {lambda}25.89/[Ne II] {lambda}12.81 line ratios than non-HBLR Sy2s; and (3) HBLR Sy2s have smaller IRAS f{sub 60}/f{sub 25} flux ratios, which show the relative strength of the host galaxy and nuclear emission, than non-HBLR Sy2s. Consequently, we suggest that HBLR Sy2s and non-HBLR Sy2s are AGN dominated and starburst dominated, respectively. In addition, non-HBLR Sy2s can be classified into luminous (L{sub [OIII]}>10{sup 41} erg s{sup -1}) and less luminous (L{sub [OIII]} < 10{sup 41} erg s{sup -1}) samples, when considering only their obscuration. We suggest that (1) the invisibility of polarized broad lines (PBLs) in the luminous non-HBLR Sy2s depends on the obscuration and (2) the invisibility of PBLs in the less luminous non-HBLR Sy2s depends on the very low Eddington ratio rather than the obscuration.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

Decaying dark matter and the tension in σ{sub 8}

We consider decaying dark matter (DDM) as a resolution to the possible tension between cosmic microwave background (CMB) and weak lensing (WL) based determinations of the amplitude of matter fluctuations, σ{sub 8}. We perform N-body simulations in a model where dark matter decays into dark radiation and develop an accurate fitting formula for the non-linear matter power spectrum, which enables us to test the DDM model by the combined measurements of CMB, WL and the baryon acoustic oscillation (BAO). We employ a Markov chain Monte Carlo analysis to examine the overlap of posterior distributions of the cosmological parameters, comparing CMB alone with WL+BAO. We find an overlap that is significantly larger in the DDM model than in the standard CDM model. This may be hinting at DDM, although current data is not constraining enough to unambiguously favour a non-zero dark matter decay rate Γ. From the combined CMB+WL data, we obtain a lower bound Γ{sup −1}≥ 97 Gyr at 95 % C.L, which is less tight than the constraint from CMB alone.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

Prototyping high-gradient mm-wave accelerating structures

We present single-cell accelerating structures designed for high-gradient testing at 110 GHz. The purpose of this work is to study the basic physics of ultrahigh vacuum RF breakdown in high-gradient RF accelerators. The accelerating structures are π-mode standing-wave cavities fed with a TM 01 circular waveguide. The structures are fabricated using precision milling out of two metal blocks, and the blocks are joined with diffusion bonding and brazing. The impact of fabrication and joining techniques on the cell geometry and RF performance will be discussed. First prototypes had a measured Q 0 of 2800, approaching the theoretical design value of 3300. The geometry of these accelerating structures are as close as practical to singlecell standing-wave X-band accelerating structures more than 40 of which were tested at SLAC. This wealth of X-band data will serve as a baseline for these 110 GHz tests. Furthermore, the structures will be powered with short pulses from a MW gyrotron oscillator. RF power of 1 MW may allow an accelerating gradient of 400 MeV/m to be reached.

43 PARTICLE ACCELERATORS↗
DOE OSTI2011

EXTENDED SCALING LAWS IN NUMERICAL SIMULATIONS OF MAGNETOHYDRODYNAMIC TURBULENCE

Magnetized turbulence is ubiquitous in astrophysical systems, where it notoriously spans a broad range of spatial scales. Phenomenological theories of MHD turbulence describe the self-similar dynamics of turbulent fluctuations in the inertial range of scales. Numerical simulations serve to guide and test these theories. However, the computational power that is currently available restricts the simulations to Reynolds numbers that are significantly smaller than those in astrophysical settings. In order to increase computational efficiency and, therefore, probe a larger range of scales, one often takes into account the fundamental anisotropy of field-guided MHD turbulence, with gradients being much slower in the field-parallel direction. The simulations are then optimized by employing the reduced MHD equations and relaxing the field-parallel numerical resolution. In this work we explore a different possibility. We propose that there exist certain quantities that are remarkably stable with respect to the Reynolds number. As an illustration, we study the alignment angle between the magnetic and velocity fluctuations in MHD turbulence, measured as the ratio of two specially constructed structure functions. We find that the scaling of this ratio can be extended surprisingly well into the regime of relatively low Reynolds number. However, the extended scaling easily becomes spoiled when the dissipation range in the simulations is underresolved. Thus, taking the numerical optimization methods too far can lead to spurious numerical effects and erroneous representation of the physics of MHD turbulence, which in turn can affect our ability to identify correctly the physical mechanisms that are operating in astrophysical systems.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2012

A METHOD FOR LOCALIZING ENERGY DISSIPATION IN BLAZARS USING FERMI VARIABILITY

The distance of a Fermi-detected blazar {gamma}-ray emission site from a supermassive black hole is a matter of active debate. Here we present a method for testing if the GeV emission of powerful blazars is produced within the subparsec-scale broad-line region (BLR) or farther out in the parsec-scale molecular torus (MT) environment. If the GeV emission takes place within the BLR, the inverse Compton (IC) scattering of the BLR ultraviolet (UV) seed photons that produces the {gamma}-rays takes place at the onset of the Klein-Nishina regime. This causes the electron cooling time to become practically energy-independent and the variation of the {gamma}-ray emission to be almost achromatic. If, on the other hand, the {gamma}-ray emission is produced farther out in the parsec-scale MT, the IC scattering of the infrared (IR) MT seed photons that produces the {gamma}-rays takes place in the Thomson regime, resulting in energy-dependent electron cooling times, manifested as faster cooling times for higher Fermi energies. We demonstrate these characteristics and discuss the applicability and limitations of our method.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

DIRECTLY IMAGING TIDALLY POWERED MIGRATING JUPITERS

Upcoming direct-imaging experiments may detect a new class of long-period, highly luminous, tidally powered extrasolar gas giants. Even though they are hosted by {approx} Gyr-'old' main-sequence stars, they can be as 'hot' as young Jupiters at {approx}100 Myr, the prime targets of direct-imaging surveys. They are on years-long orbits and presently migrating to 'feed' the 'hot Jupiters'. They are expected from 'high-e' migration mechanisms, in which Jupiters are excited to highly eccentric orbits and then shrink semimajor axis by a factor of {approx}10-100 due to tidal dissipation at close periastron passages. The dissipated orbital energy is converted to heat, and if it is deposited deep enough into the atmosphere, the planet likely radiates steadily at luminosity L {approx} 100-1000 L{sub Jup}(2 Multiplication-Sign 10{sup -7}-2 Multiplication-Sign 10{sup -6} L{sub Sun }) during a typical {approx} Gyr migration timescale. Their large orbital separations and expected high planet-to-star flux ratios in IR make them potentially accessible to high-contrast imaging instruments on 10 m class telescopes. {approx}10 such planets are expected to exist around FGK dwarfs within {approx}50 pc. Long-period radial velocity planets are viable candidates, and the highly eccentric planet HD 20782b at maximum angular separation {approx}0.''08 is a promising candidate. Directly imaging these tidally powered Jupiters would enable a direct test of high-e migration mechanisms. Once detected, the luminosity would provide a direct measurement of the migration rate, and together with mass (and possibly radius) estimate, they would serve as a laboratory to study planetary spectral formation and tidal physics.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

QUIJOTE scientific results – IV. A northern sky survey in intensity and polarization at 10–20 GHz with the multifrequency instrument

ABSTRACT We present QUIJOTE intensity and polarization maps in four frequency bands centred around 11, 13, 17, and 19 GHz, and covering approximately 29 000 deg2, including most of the northern sky region. These maps result from 9000 h of observations taken between May 2013 and June 2018 with the first QUIJOTE multifrequency instrument (MFI), and have angular resolutions of around 1°, and sensitivities in polarization within the range 35–40 µK per 1° beam, being a factor ∼2–4 worse in intensity. We discuss the data processing pipeline employed, and the basic characteristics of the maps in terms of real space statistics and angular power spectra. A number of validation tests have been applied to characterize the accuracy of the calibration and the residual level of systematic effects, finding a conservative overall calibration uncertainty of 5 per cent. We also discuss flux densities for four bright celestial sources (Tau A, Cas A, Cyg A, and 3C274), which are often used as calibrators at microwave frequencies. The polarization signal in our maps is dominated by synchrotron emission. The distribution of spectral index values between the 11 GHz and WMAP 23 GHz map peaks at β = −3.09 with a standard deviation of 0.14. The measured BB/EE ratio at scales of ℓ = 80 is 0.26 ± 0.07 for a Galactic cut |b| > 10°. We find a positive TE correlation for 11 GHz at large angular scales (ℓ ≲ 50), while the EB and TB signals are consistent with zero in the multipole range 30 ≲ ℓ ≲ 150. The maps discussed in this paper are publicly available.

Astronomy & Astrophysics↗
DOE OSTI2017

Lens covariance effects on likelihood analyses of CMB power spectra

Non-Gaussian correlations induced in CMB power spectra by gravitational lensing needs to be included in likelihood analyses for future CMB experiments. We present a simple but accurate likelihood model which includes these correlations and use it for Markov Chain Monte Carlo parameter estimation from simulated lensed CMB maps in the context of ΛCDM and extensions which include the sum of neutrino masses or the dark energy equation of state w. If lensing-induced covariance is not taken into account for a CMB-S4 type experiment, the errors for one combination of parameters in each case would be underestimated by more then a factor of two and lower limits on w could be misestimated substantially. The frequency of falsely ruling out the true model or finding tension with other data sets would also substantially increase. Our analysis also enables a separation of lens and unlensed information from CMB power spectra, which provides for consistency tests of the model and, if combined with other such measurements, a nearly lens-sample-variance free test for systematics and new physics in the unlensed spectrum. This parameterization also leads to a simple effective likelihood that can be used to assist model building in case consistency tests of ΛCDM fail.

79 ASTRONOMY AND ASTROPHYSICS↗