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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Sequential Infiltration Synthesis (SIS) of In 2 O 3 -Based Porous Photoelectrodes for Molecular Sensitization

High-surface-area photoelectrodes are highly desirable for solar energy conversion applications, particularly in systems where surface-bound molecular chromophores are responsible for light absorption. To this end, porous Indium-Zinc-Oxide (IZO) frameworks are fabricated via Sequential Infiltration Synthesis (SIS) into poly(methyl methacrylate) (PMMA) films followed by air annealing. A more complete understanding of the multimetal infiltration process conditions and postannealing temperature allows for precise control of zinc (Zn) incorporation to afford porous, conductive, transparent, and amorphous photoelectrodes. Uniform incorporation of both indium (In) and Zn is found to require extended diethylzinc (DEZ) exposures to compensate for remarkably slow precursor diffusion in the presence of indium oxyhydroxide nuclei. SIS-fabricated IZO photoelectrodes are structurally robust, electrochemically active, and exhibit dye adsorption that suggest practical surface area enhancements greater than 100×. In conclusion, these attributes establish SIS as a rapid, scalable, and reproducible route to photoelectrodes for solar energy conversion and hybrid interface characterization.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1987

Calculations of the displacement damage and short-circuit current degradation in proton irradiated (AlGa)As-GaAs solar cells

A theoretical model for computing the displacement damage defect density and the short-circuit current (I sub sc) degradation in proton-irradiated (AlGa)As-GaAs p-n junction solar cells is presented. Assumptions were made with justification that the radiation induced displacement defects form an effective recombination center which controls the electron and hole lifetimes in the junction space charge region and in the n-GaAs active layer of the irradiated GaAs p-n junction cells. The degradation of I sub sc in the (AlGa)As layer was found to be negligible compared to the total degradation. In order to determine the I sub sc degradation, the displacement defect density, path length, range, reduced energy after penetrating a distance x, and the average number of displacements formed by one proton scattering event were first calculated. The I sub sc degradation was calculated by using the electron capture cross section in the p-diffused layer and the hole capture cross section in the n-base layer as well as the wavelength dependent absorption coefficients. Excellent agreement was found between the researchers calculated values and the measured I sub sc in the proton irradiated GaAs solar cells for proton energies of 100 KeV to 10 MeV and fluences from 10 to the 10th power p/square cm to 10 to the 12th power p/square cm.

Yeh, C. S.↗
DOE OSTI2025

Low-energy pathways lead to self-healing defects in CsPbBr 3

Self-regulation of free charge carriers in perovskites via Schottky defect formation has been posited as the origin of the well-known defect-tolerance of metal halide perovskite materials. Understanding the mechanisms of self-regulation promises to lead to the fabrication of better performing solar cell materials with higher efficiencies. We investigate many such mechanisms here for CsPbBr 3 , a popular representative of a more commercially viable all-inorganic metal halide perovskite. We investigate different atomic-level mechanisms and pathways of the diffusion and recombination of neutral and charged interstitials and vacancies (Schottky pairs) in CsPbBr 3 . We use nudged elastic band calculations and ab initio-derived pseudopotentials within quantum ESPRESSO to determine energies of formation and migration and hence the activation energies for these defects. While halide vacancies are known to exhibit low formation energies, the migration of interstitials is less studied. Our calculations uncover interstitial defect pathways capable of producing an activation energy at, or below, the single experimental value of 0.53 eV observed for the slow, temperature-dependent recovery of light-induced conductivity in bulk CsPbBr 3 . Our work reveals the existence of a low-energy diffusion pathway involving a concerted “domino effect” of interstitials, with the net result that interstitials can diffuse more readily over longer distances than expected. This observation suggests that defect self-healing can be promoted if the “domino effect” strategy can be engaged.

14 SOLAR ENERGY↗
DOE OSTI2018

Evaluation of Alternative Designs for a High Temperature Particle-to-SCO2 Heat Exchanger

This paper presents an evaluation of alternative particle heat-exchanger designs, including moving packed-bed and fluidized-bed designs, for high-temperature heating of a solar-driven supercritical CO2 (sCO2) Brayton power cycle. The design requirements for high pressure (= 20 MPa) and high temperature (= 700 degrees C) operation associated with sCO2 posed several challenges requiring high-strength materials for piping and/or diffusion bonding for plates. Designs from several vendors for a 100 kW-thermal particle-to-sCO2 heat exchanger were evaluated as part of this project. Cost, heat-transfer coefficient, structural reliability, manufacturability, parasitics and heat losses, scalability, compatibility, erosion and corrosion, transient operation, and inspection ease were considered in the evaluation. An analytical hierarchy process was used to weight and compare the criteria for the different design options. The fluidized-bed design fared the best on heat transfer coefficient, structural reliability, scalability and inspection ease, while the moving packed-bed designs fared the best on cost, parasitics and heat losses, manufacturability, compatibility, erosion and corrosion, and transient operation. A 100 kWt shell-and-plate design was ultimately selected for construction and integration with Sandia's falling particle receiver system.

14 SOLAR ENERGY↗
NASA NTRS1993

Diffuse X-ray emission from the NGC 2300 group of galaxies - Implications for dark matter and galaxy evolution in small groups

The discovery of diffuse X-ray emission from the NGC 2300 group of galaxies using the ROSAT Position Sensitive Proportional Counter is reported. The gas distributions is roughly symmetric and extends to a radius of at least 0.2/h(50) Mpc. A Raymond-Smith hot plasma model provides an excellent fit the X-ray spectrum with a best-fit value temperature of 0.9 + -/15 or - 0.14 keV and abundance 0.06 + 0/.12 or - 0.05 solar. The assumption of gravitational confinement leads to a total mass of the group of 3.0 + 0.4 or - 0.5 x 10 exp 13 solar. Baryons can reasonably account for 4 percent of this mass, and errors could push this number not higher than 10-15 percent. This is one of the strongest pieces of evidence that dark matter dominates small groups such as this one. The intragroup medium in this system has the lowest metal abundance yet found in diffuse gas in a group or cluster.

Mulchaey, John S.↗
DOE OSTI2019

Quantifying Resolution Implications for Agent-based Distributed Energy Resource Customer Adoption Models

In this report we explore tradeoffs of top-down and bottom-up methods in their precision and computational burden using NREL's dGen model, an agent-based model of residential and non-residential distributed PV adoption. In particular, we assess the role of agent resolution in instantiating statistically-representative populations in the model--and the resulting variance of model projections at the state, sector and county levels. Running the model for a single state with fixed macroeconomic assumptions, we vary both the number of agents instantiated and the number of unique simulations. Notably, in each run we introduce sources of uncertainty in cumulative DPV adoption results during agent instantiation as we stochastically sample agent attributes from localized building characteristic and solar resource distributions. We find three key trends which guide what can be expected of results. First, precision of the model projections, as measured by the variance of the unique simulations increased as a function of the number of agents sampled, though with diminishing returns to scale. The result is expected given the Law of Large Numbers. Second, the mean or expected value of projections decreased as the number of agents instantiated increased. Empirically, aggregate DPV capacities projected by dGen are 7% lower on average at a 10-agent resolution compared to 1-agent resolutions, and up to 10% lower in the non-residential sector. We attribute this outcome to a system sizing scheme that biases lower cumulative installed capacity as agent resolution increases when roof size and load are not positively correlated. Finally, the variance of model projections differed by sector, where variance was substantially larger in the commercial sector, largely due to differences in parameterization by sector. We explain the larger variance in the non-residential sector as an outcome of the greater variance in building uses and load shapes as compared to the residential sector, and we find that a resolution on the order of 100-agents per county would be necessary to bring non-residential variance in line with residential variance at a 2-agent resolution. We propose that further research explore increasing precision and agent resolution in the non-residential sector. Moreover, given that days of intensive computing may be required to resolve a suitable estimate even at the extent of a single state within acceptable levels of precision, to promote computational efficiency we also suggest more clearly quantifying sources of variability at the county level such that resolution can by dynamically increased where county level results are least precise.

14 SOLAR ENERGY↗
NASA NTRS1976

Silicon solar cells from transition metal doped Czochralski and web crystals

The influence of metallic impurities on solar cell characteristics has been examined to establish the cost sensitive purity versus performance trade-offs. Solar cells were fabricated on 2 to 4 ohm-cm p-type substrates obtained by Czochralski and dendritic web growth processes. Controlled amounts of metallic impurities were introduced into the melt during growth and included Fe, Cr, Mn, Ni, Cu, Ti, V, Zr, Mg, Zn, and Al. Impurity concentrations in the crystals were determined using emission and mass spectrographic techniques and in some cases by neutron activation analysis. The solar cells were characterized by means of a computer program to curve-fit measured voltage-current data. The principal effect of the added impurities is a degradation of lifetime and diffusion length.

Davis, J. R.↗
NASA NTRS1978

The interplanetary modulation and transport of Jovian electrons

Based on simultaneous measurements by Pioneer 11 of the 3-6 MeV Jovian electron flux, interplanetary magnetic field magnitude, and solar wind speed, the interplanetary transport of energetic particles is studied. It is found that corotating interaction regions (CIR's) greatly inhibit electron transport across the average field direction. Cross-field transport is also influenced by the degree of compression of the solar wind since CIR's are areas of compressed solar wind plasma. The propagation of Jovian electrons is studied by a model that includes the effects of CIR's. The model tests whether or not the three-dimensional convection-diffusion theory adequately describes the cross-field transport of electrons. The model is also valid for Jovian electron observations from earth-orbiting satellites. The model may be further applied to 1 AU from the sun where it is found that the cross-field diffusion of electrons explains why Jovian electrons are detected at the earth even during periods when the interplanetary magnetic field does not connect the earth directly to Jupiter.

Conlon, T. F.↗
NASA NTRS1978

Evaporation of ice in planetary atmospheres: Ice-covered rivers on Mars

The evaporation rate of water ice on the surface of a planet with an atmosphere involves an equilibrium between solar heating and radiative and evaporative cooling of the ice layer. The thickness of the ice is governed principally by the solar flux which penetrates the ice layer and then is conducted back to the surface. Evaporation from the surface is governed by wind and free convection. In the absence of wind, eddy diffusion is caused by the lower density of water vapor in comparison to the density of the Martian atmosphere. For mean martian insolations, the evaporation rate above the ice is approximately 10 to the minus 8th power gm/sq cm/s. Evaporation rates are calculated for a wide range of frictional velocities, atmospheric pressures, and insolations and it seems clear that at least some subset of observed Martian channels may have formed as ice-chocked rivers. Typical equilibrium thicknesses of such ice covers are approximately 10m to 30 m; typical surface temperatures are 210 to 235 K.

Wallace, D.↗
NASA NTRS1982

Supernovae, young remnants, and nucleosynthesis

Chemical abundance data from extragalactic supernovae and from supernova remnants (SNR) less than 1000 yrs old are employed to show that nuclear burning beyond helium synthesis actually occurs. Supernova (SN) are classified into types I or II, having no hydrogen lines or featuring hydrogen lines, respectively. The SN I's have been observed as having a preponderance of Fe lines, and emitting from a source at around 12,000 K with a center continuum of approximately 10 AU. Decay chains which could account for detected luminosities and spectra are presented, noting a good fit of Fe II spectrum with observed SN spectra. SNR pass through younger and older stages, going from the outpouring of material to diffusion in the interstellar medium. Expanding flocculi from young SNR show oxygen abundances as well as lines from sulfur, calcium, and argon, with a corresponding necessity of an explosive source of 15 solar masses.

Kirshner, R. P.↗
NASA NTRS1985

Laboratory simulation of meteoritic noble gases. II - Sorption of xenon on carbon: Etching and heating experiments

The release of trapped Xe from amorphous-C phases of meteorites is simulated experimentally by HNO3 etching of carbon-black and pyrolyzed polyvinylidene chloride samples exposed to Xe-127 for 0.5-240 h at 100-1000 C and then degassed for 9 h or more at the same temperatures, as reported by Wacker et al. (1985). The results are presented in tables and graphs and characterized in detail. Samples exposed at 100-200 C are found to lose most of their Xe after etching to a depth of only about 20 pm, while those exposed at 800-1000 C exhibit a second more tightly bound component extending to a depth of 3 nm, indicative of diffusion of Xe during exposure and resembling planetary Xe. The higher noble-gas concentrations measured in meteorites are attributed to rate-controlled Xe uptake over a long period in the solar nebula.

Zadnik, M. G.↗
NASA NTRS1986

Modulation of galactic cosmic rays in the heliosphere

Observations of the intensity of galactic cosmic rays and anomalous components near earth and in the outer heliosphere are providing important tests for theories of solar modulation. The most recent observations show effects that seem to require that models for modulation include gradient and curvature drifts as well as the conventional processes of convection, adiabatic deceleration, and diffusion. New observations are required to define the interplay of these processes in the three-dimensional heliosphere.

Mckibben, R. B.↗
NASA NTRS1990

Cosmic-ray streaming in the Born approximation

The present work invokes the Born approximation to derive a more accurate expression for the streaming of cosmic rays parallel to the mean magnetic field. While all prior results pertaining to the helicity dependence of the diffusion coefficient and convection speed can be recovered as special cases from this streaming equation, it is concluded that a new set of transport parameters presented here is more appropriate for the solar modulation of galactic cosmic rays. In addition, a new parameter related to time variability, which may be a dominant cause of charge sign-dependent transport of solar particles, is introduced.

Bieber, J. W.↗
NASA NTRS1991

COBE ground segment gyro calibration

Discussed here is the calibration of the scale factors and rate biases for the Cosmic Background Explorer (COBE) spacecraft gyroscopes, with the emphasis on the adaptation for COBE of an algorithm previously developed for the Solar Maximum Mission. Detailed choice of parameters, convergence, verification, and use of the algorithm in an environment where the reference attitudes are determined form the Sun, Earth, and star observations (via the Diffuse Infrared Background Experiment (DIRBE) are considered. Results of some recent experiments are given. These include tests where the gyro rate data are corrected for the effect of the gyro baseplate temperature on the spacecraft electronics.

Freedman, I.↗
NASA NTRS1995

Long-term variation of Saturn H2 emission

The goal of this research effort was to analyze the long-term IUE database of Saturn images for the possible presence of diffuse H2 emissions, using techniques originally developed for analysis of Jupiter images. The poor S/N ratio in many of the Saturn images proved to be a significant limitation to the possible detection of H2 emission. The creation of a satisfactory background atmosphere model was also limited by difficulties in reproducing the observed C2H2 band structure at long wavelengths. The results currently available suggest that diffuse H2 emission is present on Saturn on some occasions. However, the IUE data are not able to indicate whether H2 emission is present at all times with a magnitude proportional to solar activity, as was shown for Jupiter.

DeLand, Matthew T.↗
NASA NTRS2009

Sources of Sodium in the Lunar Exosphere: Modeling Using Ground-Based Observations of Sodium Emission and Spacecraft Data of the Plasma

Observations of the equatorial lunar sodium emission are examined to quantify the effect of precipitating ions on source rates for the Moon's exospheric volatile species. Using a model of exospheric sodium transport under lunar gravity forces, the measured emission intensity is normalized to a constant lunar phase angle to minimize the effect of different viewing geometries. Daily averages of the solar Lyman alpha flux and ion flux are used as the input variables for photon-stimulated desorption (PSD) and ion sputtering, respectively, while impact vaporization due to the micrometeoritic influx is assumed constant. Additionally, a proxy term proportional to both the Lyman alpha and to the ion flux is introduced to assess the importance of ion-enhanced diffusion and/or chemical sputtering. The combination of particle transport and constrained regression models demonstrates that, assuming sputtering yields that are typical of protons incident on lunar soils, the primary effect of ion impact on the surface of the Moon is not direct sputtering but rather an enhancement of the PSD efficiency. It is inferred that the ion-induced effects must double the PSD efficiency for flux typical of the solar wind at 1 AU. The enhancement in relative efficiency of PSD due to the bombardment of the lunar surface by the plasma sheet ions during passages through the Earth's magnetotail is shown to be approximately two times higher than when it is due to solar wind ions. This leads to the conclusion that the priming of the surface is more efficiently carried out by the energetic plasma sheet ions.

Sarantos, Menelaos↗
NASA NTRS1977

Perturbations of a close-earth satellite due to sunlight diffusely reflected from the earth. II - Variable albedo

A semianalytical method has been developed to calculate the radiation-pressure perturbations of a close-earth satellite due to sunlight reflected from the earth. It is assumed that the satellite is spherically symmetric and that the solar radiation is reflected from the earth according to Lambert's law. To account for the increasing reflectivity of the earth toward the poles, its albedo is assumed to have a latitudinal dependence. The effect of the terminator on the perturbations has been neglected. The perturbations within a particular revolution are given analytically, while the long-range perturbations are obtained by accumulation.

Lautman, D. A.↗
NASA NTRS1978

Development of Low Cost Contacts to Silicon Solar Cells

Commercial electroless Cu solutions were used. Satisfactory adhesion (and fairly good cell performance) resulted from the use of thin layers of barrier metals such as Au, Cr or Pd. In these tests, photoresist masks were used to contact silicon P-type slices with diffused N+ and alloyed P+ surfaces; and electrolytic Cu solution was used to build up the contact thickness to provide good cell behavior. In addition some cells with evaporated Cr-Cu contacts were also made (along with evaporated Ti-Pd-Ag contacts as controls), with the intention of subjecting cells to gradually increasing heat-treatments, to determine whether Cu causes the cells to be inherently unstable.

Iles, P. A.↗