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At least 1,783 records · Page 99

Fast Z Z free entangling gates for superconducting qubits assisted by a driven resonator

Engineering high-fidelity two-qubit gates is an indispensable step toward practical quantum computing. For superconducting quantum platforms, one important setback is the stray interaction between qubits, which causes significant coherent errors. For transmon qubits, protocols for mitigating such errors usually involve fine-tuning the hardware parameters or introducing usually noisy flux-tunable couplers. In this work, we propose a simple scheme to cancel these stray interactions. The coupler used for such cancelation is a driven high-coherence resonator, where the amplitude and frequency of the drive serve as control knobs. Through the resonator-induced-phase interaction, the static Z Z coupling can be entirely neutralized. We numerically show that such a scheme can enable short and high-fidelity entangling gates, including cross-resonance controlled-not (cnot) gates within 40 ns and adiabatic controlled- Z gates within 140 ns. Our architecture is not only Z Z -free, but also contains no extra noisy components, such that it preserves the coherence times of fixed-frequency transmon qubits. With the state-of-the-art coherence times, the error of our cross-resonance cnot gate can be reduced to below 10 − 4 .

Huang, Ziwen↗

Rethinking CO adsorption on transition-metal surfaces: Effect of density-driven self-interaction errors

Adsorption of the molecule CO on metallic surfaces is an important unsolved problem in Kohn-Sham density functional theory (KS-DFT). We present a detailed study of carbon monoxide adsorption on fcc (111) surfaces of 3d, 4d, and 5d metals using nonempirical semilocal density functionals for the exchange-correlation energy: the local-density approximation (LDA), two generalized gradient approximations or GGAs [Perdew-Burke-Ernzerhof (PBE) and PBE for solids (PBEsol)], and a meta-GGA [strongly constrained and appropriately normed (SCAN) functional]. The typical error pattern (as found earlier for free molecules and for free transition-metal surfaces), in which results improve from LDA to PBE or PBEsol to SCAN, due to the satisfaction of more exact constraints, is not found here. Instead, for CO adsorption on transition-metal surfaces, we find that, while SCAN overbinds much less than LDA, it overbinds slightly more than PBE. Moreover, the tested functionals often predict the wrong adsorption site, as first pointed out for LDA and GGA in the CO/Pt (111) puzzle. This abnormal pattern leads us to suspect that the errors of PBE and SCAN for this problem are density-driven self-interaction errors associated with incorrect charge transfer between molecule and metal surface. We point out that, by the variational principle, overbinding by an approximate functional would be reduced if that functional were applied not to its self-consistent density for the adsorbed system but to an exact or more correct density for that system. Finally, we show for CO on Pt(111) that the site preference is corrected and the adsorption energy is improved for the PBE functional by using not the self-consistent PBE density but a PBE+U density. The resulting correction to the PBE total energy is much larger for the adsorbed system than for its desorbed components, showing that the error is in the density of the adsorbed system. Furthermore, this seems to solve the Feibelman 2001 CO/Pt(111) puzzle, in principle if not fully in practice.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

The antiferromagnetic phase of the Floquet-driven Hubbard model

A saddle point plus fluctuation analysis of the periodically driven half-filled two-dimensional Hubbard model is performed. For drive frequencies below the equilibrium gap, we find discontinuous transitions to time-dependent solutions. Furthermore, a highly excited, generically nonthermal distribution of magnons occurs even for drive frequencies far above the gap. Above a critical drive amplitude, the low-energy magnon distribution diverges as the frequency tends to zero and antiferromagnetism is destroyed, revealing the generic importance of collective mode excitations arising from a nonequilibrium drive.

2-dimensional systems↗

Chiral edge currents for ac-driven skyrmions in confined pinning geometries

In this work, we show that ac-driven skyrmion lattices in a weak pinning channel confined by regions of strong pinning exhibit edge transport carried by skipping orbits while skyrmions in the bulk of the channel undergo localized orbits with no net transport. The magnitude of the edge currents can be controlled by varying the amplitude and frequency of the ac drive or by changing the ratio of the Magnus force to the damping term. We identify a localized phase in which the orbits are small and edge transport is absent, an edge transport regime, and a fluctuating regime that appears when the ac drive is strong enough to dynamically disorder the skyrmion lattice. We also find that in some cases, multiple rows of skyrmions participate in the transport due to a drag effect from the skyrmion-skyrmion interactions. The edge currents are robust for finite disorder and should be a general feature of skyrmions interacting with confined geometries or inhomogeneous disorder under an ac drive. We show that similar effects can occur for skyrmion lattices at interfaces or along domain boundaries for multiple coexisting skyrmion species. The edge current effect provides a new method to control skyrmion motion, and we discuss the connection of these results with recent studies on the emergence of edge currents in chiral active matter systems and gyroscopic metamaterials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Time- and momentum-resolved tunneling spectroscopy of pump-driven nonthermal excitations in Mott insulators

We present a computational technique to calculate time- and momentum-resolved nonequilibrium spectral density of correlated systems using a tunneling approach akin to scanning tunneling spectroscopy. The important difference is that our probe is extended, basically a copy of the sample, allowing one to extract the momentum information of the excitations. We illustrate the method by measuring the spectrum of a Mott-insulating extended Hubbard chain after a sudden quench with the aid of time-dependent density-matrix renormalization-group calculations. In this work, we demonstrate that the system realizes a nonthermal state that is an admixture of spin and charge density wave states, with corresponding signatures that are recognizable as in-gap subbands. In particular, we identify a band of excitons and one of stable antibound states at high energies that gains enhanced visibility after the pump. We do not appreciate noticeable relaxation within the time scales considered, which is attributed to the lack of decay channels due to spin-charge separation. These ideas can be readily applied to study transient dynamics and spectral signatures of correlation-driven nonequilibrium processes.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Pressure-driven valence increase and metallization in the Kondo insulator Ce 3 Bi 4 Pt 3

We report the results of high-pressure x-ray diffraction, x-ray absorption, and electrical transport measurements of the Kondo insulator (KI) Ce 3 Bi 4 Pt 3 up to 42 GPa, the highest pressure reached in the study of any Ce-based KI. Here, we observe a smooth decrease in volume and movement toward intermediate Ce valence with pressure, both of which point to increased electron correlations. Despite this, temperature-dependent resistance data show the suppression of the interaction-driven ambient pressure insulating ground state. We also discuss potential ramifications of these results for the predicted topological KI state.

36 MATERIALS SCIENCE↗

Lifetime renormalization of driven weakly anharmonic superconducting qubits. II. The readout problem

Recent experiments in superconducting qubit systems have shown an unexpectedly strong dependence of the qubit relaxation rate on the readout drive power. This phenomenon limits the maximum measurement strength and thus the achievable readout speed and fidelity. We address this problem here and provide a plausible mechanism for drive-power dependence of relaxation rates. To this end we introduce a two-parameter perturbative expansion in qubit anharmonicity and the drive amplitude through a unitary transformation technique introduced in Part I. This approach naturally reveals number-nonconserving terms in the Josephson potential as a fundamental mechanism through which applied microwave drives can activate additional relaxation mechanisms. Here, we present our results in terms of an effective master equation with renormalized state- and drive-dependent transition frequency and relaxation rates. Comparison of numerical results from this effective master equation to those obtained from a Lindblad master equation which only includes number-conserving terms (i.e., Kerr interactions) shows that number-nonconserving terms can lead to significant drive-power dependence of the relaxation rates. The systematic expansion technique introduced here is of general applicability to obtaining effective master equations for driven-dissipative quantum systems that contain weakly nonlinear degrees of freedom.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Current-driven transverse domain wall oscillations in perpendicular spin-valve structures

Spin-transfer-driven oscillations of a transverse domain wall confined to a perpendicular spin-valve structure are investigated using a one-dimensional model. The stack consists of a polarizer, nonmagnetic spacer, soft free layer, and pinned magnetic layer. It is found that the domain-wall oscillation frequency is a nonmonotonic, highly asymmetrical function of applied electric current, showing a strong dependence on the current direction and the relative strengths of the interfacial and bulk spin-transfer torques. Micromagnetic analysis reveals that the surprising and atypical oscillator response is due to an interplay between the interfacial spin-transfer torque, the bulk spin-transfer torque, the exchange torque, and the damping torque. The underlying physical and material responses are examined, including the important role of the domain-wall twist. The competitions between the involved torques under different operating conditions suggest that the oscillator could serve as a model system to investigate magnetic and spintronic phenomena at the nanoscale. Finally, the observed current-dependent twisting of the free-layer magnetization about the axis of precession may further be found interesting for investigations of the interaction between spin-polarized current and chiral spin structures.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Temperature-driven BCS-BEC crossover and Cooper-paired metallic phase in coupled boson-fermion systems

Motivated by strongly correlated and frustrated systems, in this work we propose an effective model that describes the dynamics of pairs of opposite spin fermions scattering from localized bosons. Integrating out one of the degrees, either the bosons or fermions, generates temperature-dependent long-range effective interactions between the entities that we investigate using Monte Carlo techniques. The behavior of bosons is dominated by vortex-antivortex unbinding, with effective interboson interactions beyond the nearest-neighbor Josephson coupling of phases. Remarkably, in the fermion sector we observe a temperature-driven phase transition from a SC phase with a “BCS” spectral function that shows a gap minimum on the underlying Fermi surface to a conducting phase of pairs but with a “BEC” spectral function with a gap minimum at k = 0. Tunneling and angle-resolved photoemission spectroscopy on Bose-Fermi mixtures in cold atomic systems and superconducting islands on graphene are some of the promising experimental platforms to test our predictions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Laser pulse driven control of charge and spin order in the two-dimensional Kondo lattice

Fast and dynamical control of quantum phases is highly desired in the application of quantum phenomena in devices. On the experimental side, ultrafast laser pulses provide an ideal platform to induce femtosecond dynamics in a variety of materials. Here we show that a laser pulse driven heavy fermion system can be tuned to dynamically evolve into a phase, which is not present in equilibrium. Using the state-of-the-art time-dependent variational Monte Carlo method, we perform numerical simulations of realistic laser pulses applied to the Kondo lattice model. By tracking spin and charge degrees of freedom we identify a dynamical phase transition, within the partially Kondo screened phase, from a charge ordered into a metallic state, while preserving the spin order of the system. Furthermore, we propose using high-harmonic generation and nonequilibrium optical conductivity to identify the dynamical phase transition in an ultrafast experiment.

36 MATERIALS SCIENCE↗

Defect-driven ferrimagnetism and hidden magnetization in MnBi 2 Te 4

MnBi 2 Te 4 (MBT) materials are promising antiferromagnetic topological insulators in which field-driven ferromagnetism is predicted to cause a transition between axion insulator and Weyl semimetallic states. However, the presence of antiferromagnetic coupling between Mn/Bi antisite defects and the main Mn layer can reduce the low-field magnetization, and it has been shown that such defects are more prevalent in the structurally identical magnetic insulator MnSb 2 Te 4 (MST). We use high-field magnetization measurements to show that the magnetization of MBT and MST occur in stages and full saturation requires fields of ~60 T. As a consequence, the low-field magnetization plateau state in MBT, where many determinations of the quantum anomalous Hall state are studied, actually consists of ferrimagnetic septuple blocks containing both uniform and staggered magnetization components.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Direct observation of the quantum fluctuation driven amplitude mode in a microcavity polariton condensate

The Higgs amplitude mode is a collective excitation studied and observed in a broad class of matter, including superconductors, charge density waves, antiferromagnets, 3He p-wave superfluid, and ultracold atomic condensates. In all the observations reported thus far, the amplitude mode was excited by perturbing the condensate out of equilibrium. Studying an exciton-polariton condensate, here, we report the observation of this amplitude mode purely driven by intrinsic quantum fluctuations without such perturbations. By using an ultrahigh quality microcavity and a Raman spectrometer to maximally reject photoluminescence (PL) from the condensate, we observe weak but distinct PL at energies below the condensate emission. We identify this as the so-called ghost branches of the amplitude mode arising from quantum depletion of the condensate into this mode. These energies, as well as the overall structure of the PL spectra, are in good agreement with our theoretical analysis.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Ultrafast laser-driven many-body dynamics and Kondo coherence collapse

Ultrafast laser pulse has provided a systematic way to inspect the dynamics of electrons in condensed matter systems. In this paper, by means of time-dependent density matrix renormalization group, we study an ultrafast laser-driven Kondo lattice model, in which conduction electrons are strongly coupled with magnetically local moments. The single-particle spectral function due to strong correlation effects and photon emission in the nonequilibrium states under laser driving are calculated. We find laser field excited collective doublon-hole pairs and an associated transient melting of Kondo coherence phase, signifying the collapse of Kondo energy gap. Moreover, we show that the photon emission, induced by a strong laser field, exhibits a different intensity characteristics than in the equilibrium Kondo insulator, which could be explained by the Kondo collapse and related suppression of both intraband and interband contribution in Kondo melting liquid. This theoretical insight is accessible with time- and angle-resolved photoemission spectroscopy and high-harmonic generation spectroscopy and will stimulate the investigation of nonequilibrium dynamics and nonlinear phenomenon in heavy fermion systems.

36 MATERIALS SCIENCE↗

Dynamics and nonmonotonic drag for individually driven skyrmions

Here, we examine the motion of an individual skyrmion driven through an assembly of other skyrmions in the absence of quenched disorder. The skyrmion behavior is determined by the ratio of the damping and Magnus terms, known as the intrinsic skyrmion Hall angle. For fixed drive in the damping dominated regime, the effective viscosity decreases monotonically with increasing skyrmion density. In contrast, in the Magnus dominated regime, the velocity varies nonmonotonically with density, and there is a regime in which the skyrmion moves faster with increasing density, as well as a pronounced speed-up effect in which a skyrmion traveling through a dense medium moves more rapidly than for low densities or the single-particle limit. The velocity-force curves in the Magnus-dominated regime exhibit an overshoot effect and other differences from the damping-dominated regime. We find a finite threshold force for skyrmion motion which increases with density as well as a drive-dependent skyrmion Hall angle. We map dynamic phase diagrams showing the threshold for motion, nonlinear flow, speed-up, and saturation regimes. In some cases, increasing the density can reduce the skyrmion Hall angle while producing a velocity boost, which could be valuable for applications.

36 MATERIALS SCIENCE↗

Magnetization reversal driven by electron localization-delocalization crossover in the inverse spinel Co 2 VO 4

Neutron diffraction, magnetization, and muon spin relaxation measurements, supplemented by density functional theory (DFT) calculations are employed to unravel temperature-driven magnetization reversal in inverse spinel Co 2 VO 4 . All measurements show a second-order magnetic phase transition at T C = 168 K to a collinear ferrimagnetic phase. Neutron diffraction measurements reveal two antiparallel ferromagnetic (FM) sublattices, belonging to magnetic ions on two distinct crystal lattice sites, where the relative balance between the two sublattices determine the net FM moment in the unit cell. As the evolution of the ordered moment with temperature differs between the two sublattices, the net magnetic moment reaches a maximum at T NC = 138 K and reverses its sign at T MR = 65 K. The DFT results suggest that the underlying microscopic mechanism for the reversal is a delocalization of the unfilled 3d -shell electrons on one sublattice just below T C , followed by a gradual localization as the temperature is lowered. Furthermore, this delocalized-localized crossover is supported by muon spectroscopy results, as strong T 1 relaxation observed below T C indicates fluctuating internal fields.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Possible quadrupole-order-driven commensurate-incommensurate phase transition in B20 CoGe

For this study, the B20-type cobalt germanide CoGe was investigated by measuring the specific heat, resistivity, and 59 Co nuclear magnetic resonance (NMR). We observed a phase transition at T Q = 13.7 K, evidenced by a very narrow peak of the specific heat and sharp changes of the nuclear spin-spin (T 2 –1 ) and spin-lattice ( T 1 – 1 ) relaxation rates. The fact that the entropy release is extremely small and the Knight shift is almost independent of temperature down to low temperatures as anticipated in a paramagnetic metal indicates that the T Q transition is of nonmagnetic origin. In addition, we detected a crossover scale T 0 ~ 30 K below which the resistivity and the NMR linewidth increase, and T 1 –1 is progressively distributed in space, that is, a static and dynamical spatial inhomogeneity develops. While the order parameter for the T Q transition remains an open question, a group-theoretical analysis suggests that the finite electric quadrupole density arising from the low local site symmetry at cobalt sites could drive the crystal symmetry lowering from the P2 1 3 symmetry that is commensurate to the R3 symmetry with an incommensurate wave vector, which fairly well accounts for the T Q transition. The quadrupole-order-driven commensurate-incommensurate phase transition may be another remarkable phenomenon arising from the structural chirality inherent in the noncentrosymmetric B20 family.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Temperature-driven changes in the Fermi surface of graphite

Here we report on temperature-dependent size and anisotropy of the Fermi pockets in graphite revealed by magnetotransport measurements. The magnetoresistances (MRs) obtained in fields along the c axis obey an extended Kohler's rule, with the carrier density following the prediction of a temperature-dependent Fermi energy, indicating a change in the Fermi pocket size with temperature. The angle-dependent magnetoresistivities at a given temperature exhibit a scaling behavior. The scaling factor that reflects the anisotropy of the Fermi surface is also found to vary with temperature. Our results demonstrate that temperature-driven changes in Fermi surface can be ubiquitous and need to be considered in understanding the temperature-dependent carrier density and MR anisotropy in semimetals.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Magnetic order driven ultrafast phase transition in NdNiO 3

Ultrashort x-ray pulses can be used to disentangle magnetic and structural dynamics and are accordingly utilized here to study the photoexcitation of NdNiO 3 (NNO), a model nickelate exhibiting structural and magnetic dynamics that conspire to induce an insulator-to-metal transition (IMT). Here, during the course of the photoinduced IMT with above-gap excitation, we observe an ultrafast (< 180 fs) quenching of magnetic order followed by a time delayed collapse of the insulating phase probed by x-ray absorption and THz transmission (450 fs) that correlates with the slowest optical phonon mode involved in the structural transition. A simultaneous order-disorder response at the Ni site and displacive response at the Nd site coexist in the ultrafast magnetic response. Crucially, we observe the optical phonon through its coherent coupling with Nd magnetic order, demonstrating that the magnetic and structural degrees of freedom both contribute in driving the IMT. Density functional theory calculations reveal a consistent scenario where optically driven intersite charge transfer drives a collapse of antiferromagnetic order that in turn destabilizes the charge-ordered phase resulting in an IMT. These experiments provide different modalities for the control of electronic phase transitions in quantum materials based on the ultrafast interplay between structural and magnetic orders created by femtosecond photoexcitation.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗