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Results for “ALKALINE EARTH ISOTOPES”

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At least 19 records

Isotope fractionation in surface ionization ion source of alkaline-earth iodides

The relationship between the isotope fractionation of alkaline-earth elements in the surface ionization ion source and the evaporation filament current, i.e., filament temperature, was studied. It was confirmed that the isotope fractionation depends on the evaporation filament temperature; the isotope fractionation in the case of higher temperature of filament becomes larger. The ionization and evaporation process in the surface ionization ion source was discussed, and it was concluded that the isotope fractionation is suppressed by setting at the lower temperature of evaporation filament because the dissociations are inhibited on the evaporation filament.

07 ISOTOPE AND RADIATION SOURCES↗

Signatures of structural changes in neutron-rich Sr, Zr and Mo isotopes

The evolution of the ground-state nuclear shapes in neutron-rich Sr, Zr, and Mo isotopes, including both even-even and odd-A nuclei, is discussed within the mean-field approximation based on the Gogny-D1S Gogny Energy Density Functional. Calculations for neutron separation energies and charge radii are presented and compared with available data. A correlation between a shape transition and a discontinuity in those observables is found within our microscopic framework. It is shown that, while in Sr and Zr isotopes the steep behavior observed in the isotopic dependence of the charge radii is a consequence of a sharp prolate-oblate transition, the smooth behavior found in Mo isotopes has its origin in an emergent region of triaxiality.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Quasifree (e,e{sup '}p) reactions on nuclei with neutron excess

We study the evolution of the (e,e{sup '}p) cross section on nuclei with increasing asymmetry between the number of neutrons and protons. The calculations are done within the framework of the distorted-wave impulse approximation, by adopting nonrelativistic and relativistic models. We compare the results obtained with three different approaches based on the mean-field description for the proton bound-state wave function. In the nonrelativistic model phenomenological Woods-Saxon and Hartree-Fock wave functions are used; in the relativistic model the wave functions are solutions of Dirac-Hartree equations. The models are first tested against experimental data on {sup 16}O, {sup 40}Ca, and {sup 48}Ca nuclei, and then they are applied to calculate (e,e{sup '}p) cross sections for a set of spherical calcium and oxygen isotopes. From the comparison of the results obtained for the various isotopes we can infer information about the dependence of the various ingredients of the models on the neutron to proton asymmetry.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

{sup 58}Fe AND {sup 54}Cr IN EARLY SOLAR SYSTEM MATERIALS

Stepwise dissolution of primitive meteorites exhibits large {sup 54}Cr anomalies but no collateral effects on {sup 58}Fe and {sup 48}Ca, two other neutron-rich nuclides from the iron peak. These results suggest that {sup 54}Cr must have been produced in particular zones of the rare Type Ia supernovae or that {sup 48}Ca and/or {sup 58}Fe were produced together in Type II supernovae and were chemically separated into some mineral phase that favors Cr over Ca and Fe, and it is the dissolution properties of that phase that is driving the isotopic effect in leaching. The recent findings of nanometer-size oxide grains with very large {sup 54}Cr excesses favored the latter scenario for the origin of the mono-isotopic Cr isotopic effect. In addition, the absence of isotopic variations in the {sup 58}Fe/{sup 54}Fe ratio at the mineral scale confirms that the short-lived nuclide {sup 60}Fe (T {sub 1/2} = 2.62 Myr) was homogeneously distributed to a less than 15% dispersion in the early solar nebula.

79 ASTRONOMY AND ASTROPHYSICS↗

Transfer reactions using a low-energy {sup 11}Be beam

A series of experiments have been performed to investigate neutron rich beryllium isotopes. Scattering as well as one neutron transfer reactions have been studied using a {sup 11}Be beam on deuteron targets. Bound states of {sup 10,11,12}Be have been studied and reaction cross sections have been calculated. The elastic scattering cross section has shown remarkable structure due to the halo structure of {sup 11}Be.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Elastic scattering of Beryllium isotopes near the Coulomb barrier

In this contribution, results of experiments performed with the three Beryllium isotopes {sup 9,10,11}Be on a medium mass {sup 64}Zn target, at a center of mass energy of {approx_equal}1.4 the Coulomb barrier, will be discussed. Elastic scattering angular distributions have been measured for the {sup 9,10}Be reactions. In the {sup 11}Be case the quasielastic scattering angular distribution was obtained. In the halo nucleus case, the angular distribution exhibit a non-Fresnel-type pattern with a strong damping of the Coulomb-nuclear interference peak. Moreover, it is found that the total reaction cross-section for the halo nucleus induced collision is more than double the ones extracted in the collisions induced by the non-halo Beryllium isotopes. A large contribution to the total-reaction cross-section in the {sup 11}Be case could be attributed to transfer and/or break-up events.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Laser spectroscopy-present and future at ISOLDE

Laser spectroscopy experiments at the ISOLDE facility have a venerable history which now spans more than 30 years. This period has seen the development of a remarkable variety of laser techniques in order to study rare isotopes far from stability, which include in-source, collinear and {beta}-NMR/{beta}-NQR spectroscopy. The propensity for innovation in laser spectroscopy at ISOLDE has continued in the last three years, helped in part by synergies with laboratories across Europe. Highlights of this work include bunched-beam spectroscopy of the neutron-rich copper and gallium isotope chains and collinear-anticollinear spectroscopy of the Be isotope chain. New ionization schemes have been developed for the Po atom crucial for the successful in-source laser spectroscopy campaign. The future HIE-ISOLDE facility will provide experimentalists with improved ion-beam quality, increased yields and a larger number of accessible elements. Several new experiments are now in preparation to maximise the reach of laser spectroscopy at HIE-ISOLDE, which include collinear resonance ionization spectroscopy and in-cooler optical pumping.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ISOTOPIC COMPOSITION OF LIGHT NUCLEI IN COSMIC RAYS: RESULTS FROM AMS-01

The variety of isotopes in cosmic rays allows us to study different aspects of the processes that cosmic rays undergo between the time they are produced and the time of their arrival in the heliosphere. In this paper, we present measurements of the isotopic ratios {sup 2}H/{sup 4}He, {sup 3}He/{sup 4}He, {sup 6}Li/{sup 7}Li, {sup 7}Be/({sup 9}Be+{sup 10}Be), and {sup 10}B/{sup 11}B in the range 0.2-1.4 GeV of kinetic energy per nucleon. The measurements are based on the data collected by the Alpha Magnetic Spectrometer, AMS-01, during the STS-91 flight in 1998 June.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Be-{alpha} correlations in the linear-chain structure of C isotopes

We investigate the linear-chain structures in highly excited states of {sup 14}C using a generalized molecular-orbital model, by which we incorporate an asymmetric configuration of three {alpha} clusters in the linear-chain states. By applying this model to the {sup 14}C system, we study the {sup 10}Be+{alpha} correlation in the linear-chain state of {sup 14}C. To clarify the origin of the {sup 10}Be+{alpha} correlation in the {sup 14}C linear-chain state, we analyze linear 3 {alpha} and 3{alpha} + n systems in a similar way. We find that a linear 3{alpha} system prefers the asymmetric 2{alpha} + {alpha} configuration, whose origin is the many-body correlation incorporated by the parity projection. This configuration causes an asymmetric mean field for two valence neutrons, which induces the concentration of valence neutron wave functions around the correlating 2{alpha}. A linear-chain structure of {sup 16}C is also discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Structure of Neutron-rich Calcium Isotopes and Roles of Three-body Interaction

Structure of neutron-rich calcium isotopes are studied by shell model calculations with the inclusion of three-body interactions. The three-body force induces repulsive contributions to the monopole terms of the valence neutron-neutron interaction Ground state energies of the isotopes, which have deviations from the experimental values near drip-lines only with the microscopic two-body interaction, are found to be well reproduced up to the observed ones when the three-body interaction is included. The excitation energies of the 2{sub 1}{sup +} state in {sup 48}Ca and {sup 54}Ca are found to be enhanced with the inclusion of the three-body interaction. The three-body force thus plays a key role for the magicity of {sup 48}Ca and {sup 54}Ca. The magnetic dipole (M1) strength in {sup 48}Ca, which is fragmented in case with the microscopic two-body interaction only, is found to be concentrated and pushed up to higher excitation energy when the three-body interarction is included. An important role of the multipole components is pointed out for the concentration of the strength.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

RAPID TIMESCALES FOR MAGMA OCEAN CRYSTALLIZATION ON THE HOWARDITE-EUCRITE-DIOGENITE PARENT BODY

Asteroid 4 Vesta has long been postulated as the source for the howardite-eucrite-diogenite (HED) achondrite meteorites. Here we show that Al-free diogenite meteorites record variability in the mass-independent abundance of {sup 26}Mg ({sup 26}Mg*) that is correlated with their mineral chemistry. This suggests that these meteorites captured the Mg-isotopic evolution of a large-scale differentiating magma body with increasing {sup 27}Al/{sup 24}Mg during the lifespan of the short-lived {sup 26}Al nuclide (t {sub 1/2} {approx} 730,000 yr). Thus, diogenites and eucrites represent crystallization products of a large-scale magma ocean associated with the differentiation and magmatic evolution of the HED parent body. The {sup 26}Mg* composition of the most primitive diogenites requires onset of the magma ocean crystallization within 0.6{sup -0.4} {sub +0.5} Myr of solar system formation. Moreover, {sup 26}Mg* variations among diogenites and eucrites imply that near complete solidification of the HED parent body occurred within the following 2-3 Myr. Thermal models predict that such rapid cooling and magma ocean crystallization could only occur on small asteroids (<100 km), implying that 4 Vesta is not the source of the HED meteorites.

58 GEOSCIENCES↗

{sup 7,9,10}Be elastic scattering and total reaction cross sections on a {sup 12}C target

Elastic scattering angular distributions for {sup 7}Be, {sup 9}Be, and {sup 10}Be isotopes on {sup 12}C target were measured at laboratory energies of 18.8, 26.0, and 23.2 MeV, respectively. The analysis was performed in terms of optical model potentials using Woods-Saxon and double-folding form factors. Also, continuum discretized coupled-channels calculations were performed for {sup 7}Be and {sup 9}Be + {sup 12}C systems to infer the role of breakup in the elastic scattering. For the {sup 10}Be + {sup 12}C system, bound states coupled-channels calculations were considered. Moreover, total reaction cross sections were deduced from the elastic scattering analysis and compared with published data on other weakly and tightly bound projectiles elastically scattered on the {sup 12}C target, as a function of energy.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Microscopic self-energy calculations and dispersive optical-model potentials

Nucleon self-energies for {sup 40,48,60}Ca isotopes are generated with the microscopic Faddeev-random-phase approximation (FRPA). These self-energies are compared with potentials from the dispersive optical model (DOM) that were obtained from fitting elastic-scattering and bound-state data for {sup 40,48}Ca. The ab initio FRPA is capable of explaining many features of the empirical DOM potentials including their nucleon asymmetry dependence. The comparison furthermore provides several suggestions to improve the functional form of the DOM potentials, including among others the exploration of parity and angular momentum dependence. The nonlocality of the FRPA imaginary self-energy, illustrated by a substantial orbital angular momentum dependence, suggests that future DOM fits should consider this feature explicitly. The roles of the nucleon-nucleon tensor force and charge-exchange component in generating the asymmetry dependence of the FRPA self-energies are explored. The global features of the FRPA self-energies are not strongly dependent on the choice of realistic nucleon-nucleon interactions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Asymptotic normalization of mirror states and the effect of couplings

Assuming that the ratio between asymptotic normalization coefficients of mirror states is model independent, charge symmetry can be used to indirectly extract astrophysically relevant proton capture reactions on proton-rich nuclei based on information on stable isotopes. The assumption has been tested for light nuclei within the microscopic cluster model. In this work we explore the Hamiltonian independence of the ratio between asymptotic normalization coefficients of mirror states when deformation and core excitation is introduced in the system. For this purpose we consider a phenomenological rotor+N model where the valence nucleon is subject to a deformed mean field and the core is allowed to excite. We apply the model to {sup 8}Li/{sup 8}B, {sup 13}C/{sup 13}N, {sup 17}O/{sup 17}F, {sup 23}Ne/{sup 23}Al, and {sup 27}Mg/{sup 27}P. Our results show that, for most studied cases, the ratio between asymptotic normalization coefficients of mirror states is independent of the strength and multipolarity of the couplings induced. The exception is for cases in which there is an s-wave coupled to the ground state of the core, the proton system is loosely bound, and the states have large admixture with other configurations. We discuss the implications of our results for novae.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Low-lying dipole response in the stable {sup 40,48}Ca nuclei with the second random-phase approximation

Low-energy dipole excitations are analyzed for the stable isotopes {sup 40}Ca and {sup 48}Ca in the framework of the Skyrme-second random-phase approximation. The corresponding random-phase approximation calculations provide a negligible strength distribution for both nuclei in the energy region from 5 to 10 MeV. The inclusion and the coupling of 2 particle-2 hole configurations in the second random-phase approximation lead to an appreciable dipole response at low energies for the neutron-rich nucleus {sup 48}Ca. The presence of a neutron skin in the nucleus {sup 48}Ca would suggest the interpretation of the low-lying response in terms of a pygmy excitation. The composition of the excitation modes (content of 1 particle-1 hole and 2 particle-2 hole configurations), their transition densities and their collectivity (number and coherence of the different contributions) are analyzed. This analysis indicates that, in general, these excitations cannot be clearly interpreted in terms of oscillations of the neutron skin against the core with the exception of the peak with the largest B(E1) value, which is located at 9.09 MeV. For this peak the neutron transition density dominates and the neutron and proton transition densities oscillate out of phase in the internal part of the nucleus leading to a strong mixing of isoscalar and isovector components. Therefore, this state shows some features usually associated to pygmy resonances.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Onset of collectivity in Neutron-Rich iron isotopes: Toward a new island of inversion?

The lifetimes of the first excited 2{sup +} states in {sup 62}Fe and {sup 64}Fe have been measured for the first time using the recoil-distance Doppler shift technique, at GANIL. A {sup 238}U beam of 6.5 AMeV impinged on {sup 64}Ni target, and the target like products were slowed down by a degrader foil positioned at micrometer distance downstream of the target and identified in the VAMOS spectrometer on an event-by-event basis. The lifetimes were then determined from the intensities of the degraded and fully Doppler shifted components of the 2{sup +}{yields}0{sup +} transition detected in EXOGAM detectors positioned at backward angles.The resulting lifetimes show a steep increase of the B(E2) values of the first excited 2{sup +} state from {sup 62}Fe to {sup 64}Fe. A comparison with shell model calculations shows that the onset of collectivity is related to the occupation of neutron intruder orbitals. The large B(E2) value for {sup 64}Fe is only reproduced if the valence space includes both the neutron g{sub 9/2} and d{sub 5/2} orbitals. The transition from spherical {sup 68}Ni to more proton-deficient N 40 isotones has some similarity with the island of inversion around {sup 32}Mg. The developing quadrupole collectivity can in both cases be related to the occupation of neutron intruder orbitals which are at the same time quasi-SU(3) partners: (f{sub 7/2}, p{sub 3/2}) for {sup 32}Mg and (g{sub 9/2}, d{sub 5/2}) for the neutron-rich Fe.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

TYPE Ia SUPERNOVAE AS SITES OF THE p-PROCESS: TWO-DIMENSIONAL MODELS COUPLED TO NUCLEOSYNTHESIS

Beyond Fe, there is a class of 35 proton-rich nuclides, between {sup 74}Se and {sup 196}Hg, called p-nuclei. They are bypassed by the s and r neutron capture processes and are typically 10-1000 times less abundant than the s- and/or r-isotopes in the solar system. The bulk of p-isotopes is created in the 'gamma processes' by sequences of photodisintegrations and beta decays in explosive conditions in both core collapse supernovae (SNe II) and in Type Ia supernovae (SNe Ia). SNe II contribute to the production of p-nuclei through explosive neon and oxygen burning. However, the major problem in SN II ejecta is a general underproduction of the light p-nuclei for A < 120. We explore SNe Ia as p-process sites in the framework of a two-dimensional SN Ia delayed detonation model as well as pure deflagration models. The white dwarf precursor is assumed to have reached the Chandrasekhar mass in a binary system by mass accretion from a giant/main-sequence companion. We use enhanced s-seed distributions, with seeds directly obtained from a sequence of thermal pulse instabilities both in the asymptotic giant branch phase and in the accreted material. We apply the tracer-particle method to reconstruct the nucleosynthesis by the thermal histories of Lagrangian particles, passively advected in the hydrodynamic calculations. For each particle, we follow the explosive nucleosynthesis with a detailed nuclear reaction network for all isotopes up to {sup 209}Bi. We select tracers within the typical temperature range for p-process production, (1.5-3.7) x 10{sup 9} K, and analyze in detail their behavior, exploring the influence of different s-process distributions on the p-process nucleosynthesis. In addition, we discuss the sensitivity of p-process production to parameters of the explosion mechanism, taking into account the consequences on Fe and alpha elements. We find that SNe Ia can produce a large amount of p-nuclei, both the light p-nuclei below A = 120 and the heavy-p nuclei, at quite flat average production factors, tightly related to the s-process seed distribution. For the first time, we find a stellar source able to produce both light and heavy p-nuclei almost at the same level as {sup 56}Fe, including the debated neutron magic {sup 92,} {sup 94}Mo and {sup 96,} {sup 98}Ru. We also find that there is an important contribution from the p-process nucleosynthesis to the s-only nuclei {sup 80}Kr, {sup 86}Sr, to the neutron magic {sup 90}Zr, and to the neutron-rich {sup 96}Zr. Finally, we investigate the metallicity effect on p-process production in our models. Starting with different s-process seed distributions for two metallicities Z = 0.02 and Z = 0.001, running two-dimensional SN Ia models with different initial composition, we estimate that SNe Ia can contribute to at least 50% of the solar p-process composition. A more detailed analysis of the role of SNe Ia in Galactic chemical evolution of p-nuclei is in preparation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Nuclear Data Sheets for A = 27

Evaluated spectroscopic data and level schemes from radioactive decay and nuclear reaction studies are presented for {sup 27}F, {sup 27}Ne, {sup 27}Na, {sup 27}Mg, {sup 27}Al, {sup 27}Si, {sup 27}P, and {sup 27}S. This evaluation for A=27 supersedes the earlier evaluation by P.M. Endt (1998En04 and 1990En08).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗