Elevated nitrogenous organics in aloft atmospheric particles across the United States
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Atmospheric particles play critical roles in climate. However, significant knowledge gaps remain regarding the vertically resolved organic molecular-level composition of atmospheric particles due to aloft sampling challenges. To address this, we use a tethered balloon system at the Southern Great Plains Observatory and high-resolution mass spectrometry to, respectively, collect and characterize organic molecular formulas (MF) in the ground level and aloft (up to 750 m) samples. We show that organic MF uniquely detected aloft were dominated by organonitrates (139 MF; 54% of all uniquely detected aloft MF). Organonitrates that were uniquely detected aloft featured elevated O/C ratios (0.73 ± 0.23) compared to aloft organonitrates that were commonly observed at the ground level (0.63 ± 0.22). Unique aloft organic molecular composition was positively associated with increased cloud coverage, increased aloft relative humidity (~40% increase compared to ground level), and decreased vertical wind variance. Furthermore, 29% of extremely low volatility organic compounds in the aloft sample were truly unique to the aloft sample compared to the ground level, emphasizing potential oligomer formation at higher altitudes. Overall, this study highlights the importance of considering vertically resolved organic molecular composition (particularly for organonitrates) and hypothesizes that aqueous phase transformations and vertical wind variance may be key variables affecting the molecular composition of aloft organic aerosol.
Direct current measurements are available near the attachment point from both natural cloud-to-ground lightning and rocket-triggered lightning, but little is known about the rise time and peak amplitude of return-stroke currents aloft. We present, as functions of height, current amplitudes, rise times, and effective propagation velocities that have been estimated with a novel remote-sensing technique from data on 24 subsequent return strokes in six different lightning flashes that were triggering at the NASA Kennedy Space Center, FL, during 1987. The unique feature of this data set is the stereo pairs of still photographs, from which three-dimensional channel geometries were determined previously. This has permitted us to calculate the fine structure of the electric-field-change (E) waveforms produced by these strokes, using the current waveforms measured at the channel base together with physically reasonable assumptions about the current distributions aloft. The computed waveforms have been compared with observed E waveforms from the same strokes, and our assumptions have been adjusted to maximize agreement. In spite of the non-uniqueness of solutions derived by this technique, several conclusions seem inescapable: 1) The effective propagation speed of the current up the channel is usually significantly (but not unreasonably) faster than the two-dimensional velocity measured by a streak camera for 14 of these strokes. 2) Given the deduced propagation speed, the peak amplitude of the current waveform often must decrease dramatically with height to prevent the electric field from being over-predicted. 3) The rise time of the current wave front must always increase rapidly with height in order to keep the fine structure of the calculated field consistent with the observations.
The ALOFT campaign is a unique suborbital campaign to advance the science of highenergy radiation emissions from thunderstorms, validate existing spaceborne lightning mappers and evaluate design concepts for next-generation mappers, and study convection from a suborbital platform. ALOFT is a collaboration between NASA, the University of Bergen, and other institutions that will fly the ER-2 aircraft over tropical thunderstorms around the Gulf of Mexico, Central America, and the Caribbean. The payload will consist of lightning detectors, gamma-ray scintillators, and a mixture of passive and/or active microwave sensors. Supporting the flights will be a diverse groundbased network of lightning instruments spread across the region of interest.
The ALOFT1 campaign took place during July 2023. The NASA ER-2 high-altitude aircraft was based in Tampa, Florida, and flew approximately 60 hours sampling tropical and sub-tropical thunderstorms that were mostly contained within the common fields of view of GLM4-16 and GLM-18. In addition, multiple underflights of the ISS LIS5 instrument occurred. The FEGS2 and LIP6 instrument suite on the ER-2 provided a combination of multispectral optical, slow and fast electric field change, and three-dimensional electric field measurements of lightning and thunderstorms. Notably, in addition to the 777-nm band used by GLM and LIS, FEGS also observed at 337 nm, 500 nm, 868 nm, wideband visible-to-infrared, and shortwave infrared. A spectrometer that spanned most major lightning bands from the ultraviolet to infrared was included. Observations of gamma-ray production by thunderstorms were also collected during ALOFT. Thus, the lightning-observing suite on the ER-2 during ALOFT provides an unprecedented suborbital dataset for direct optical-to-optical and indirect radio-to-optical validation of existing spaceborne lightning sensors like GLM and LIS. In addition, the multispectral observations from FEGS enables evaluation of current and future spaceborne lightning-observing concepts. For example, the 337-nm channel is relevant to both existing missions like ASIM7 as well as future concepts like the CubeSpark mission currently being formulated by NASA. Complementary to LIS, the ISS also carries the STP-H88 payload, which features microwave radiometers covering 18-182 GHz, while the ER-2 carried radiometers covering 10-684 GHz, enabling evaluation of spaceborne passive microwave measurements that are complementary to the lightning observations. 1. Airborne Lightning Observatory for FEGS2 and TGFs3 2. Fly’s Eye GLM4 Simulator 3. Terrestrial Gamma-ray Flashes 4. Geostationary Lightning Mapper 5. International Space Station Lightning Imaging Sensor 6. Lightning Instrument Package 7. Atmosphere-Space Interactions Monitor 8. 8th Space Test Program – Houston mission
Laser radar observations of clear tropopause compared to other data on atmospheric winds aloft
Statistical sampling procedure for jimsphere winds aloft population
Lidar observations of visually clear troposphere compared with simultaneous rawinsonde data for relationship between lidar echoes and atmospheric winds aloft
In connection with the development of the Meteorological Interactive Data Display System (MIDDS) for utilization by the Launch Systems Evaluation Advisory Team (LSEAT), requirements have been established to expand the pre-launch analysis of winds aloft for the Space Shuttle. Statistical analyses developed for the system include: comparison of pre-launch wind component profiles to wind component extremes at each altitude calculated from launch site historical data; conditional probability ellipses for wind vectors at a future time given the wind vector at an initial time; comparison of observed extreme wind shear and associated wind speed with launch site historical data utilizing the bivariate extreme value (Gumbel) distribution; estimation of extremes of wind speed or wind shear at a future time given the extremes of either variable at an initial time, utilizing the conditional extreme value distribution; power spectrum analysis for tracking wind perturbation energy in sequential pre-launch Jimsphere wind profiles.
NASA and the U.S. Army Cold Regions Research and Engineering Laboratory (CRREL) have an on-going activity to develop remote sensing technologies for the detection and measurement of icing conditions aloft. Radar has been identified as a strong tool for this work. However, since the remote detection of icing conditions with the intent to identify areas of icing hazard is a new and evolving capability, there are no set requirements for radar sensitivity. This work is an initial attempt to quantify, through analysis, the sensitivity requirements for an icing remote sensing radar. The primary radar of interest for cloud measurements is Ka-band, however, since NASA is currently using an X-band unit, this frequency is also examined. Several aspects of radar signal analysis were examined. Cloud reflectivity was calculated for several forms of cloud using two different techniques. The Air Force Geophysical Laboratory (AFGL) cloud models, with different drop spectra represented by a modified gamma distribution, were utilized to examine several categories of cloud formation. Also a fundamental methods approach was used to allow manipulation of the cloud droplet size spectra. And an analytical icing radar simulator was developed to examine the complete radar system response to a configurable multi-layer cloud environment. Also discussed is the NASA vertical pointing X-band radar. The radar and its data system are described, and several summer weather events are reviewed.
The Natural Environments Branch at the National Aeronautics and Space Administration s Marshall Space Flight Center monitors the winds aloft at Kennedy Space Center in support of the Space Shuttle Program day of launch operations. High resolution wind profiles are derived from radar tracked Jimsphere balloons, which are launched at predetermined times preceding the launch, for evaluation. The spatial (shear) and temporal (persistence) wind characteristics are assessed against a design wind database to ensure wind change does not violate wind change criteria. Evaluations of wind profies are reported to personnel at Johnson Space Center.
ALOFT is a collaborative field campaign that used the NASA ER-2 in July 2023 to hunt for gamma-rays and lightning in tropical thunderstorms
A high level description of the lightning sensors provided by MSFC for the 2023 ALOFT campaign.
Low-level clouds in the Arctic affect the surface energy budget and vertical transport of heat and moisture. The limited availability of cloud-droplet-forming aerosol particles strongly impacts cloud properties and lifetime. Vertical particle distributions are required to study aerosol–cloud interaction over sea ice comprehensively. This article presents vertically resolved measurements of aerosol particle number concentrations and sizes using tethered balloons. The data were collected during the Multidisciplinary drifting Observatory for the Study of Arctic Climate expedition in the summer of 2020. Thirty-four profiles of aerosol particle number concentration were observed in 2 particle size ranges: 12–150 nm (N 12−150 ) and above 150 nm (N >150 ). Concurrent balloon-borne meteorological measurements provided context for the continuous profiles through the cloudy atmospheric boundary layer. Radiosoundings, cloud remote sensing data, and 5-day back trajectories supplemented the analysis. The majority of aerosol profiles showed more particles above the lowest temperature inversion, on average, double the number concentration compared to below. Increased N 12−150 up to 3,000 cm −3 were observed in the free troposphere above low-level clouds related to secondary particle formation. Long-range transport of pollution increased N >150 to 310 cm −3 in a warm, moist air mass. Droplet activation inside clouds caused reductions of N >150 by up to 100%, while the decrease in N 12−150 was less than 50%. When low-level clouds were thermodynamically coupled with the surface, profiles showed 5 times higher values of N 12−150 in the free troposphere than below the cloud-capping temperature inversion. Enhanced N 12−150 and N >150 interacting with clouds were advected above the lowest inversion from beyond the sea ice edge when clouds were decoupled from the surface. Vertically discontinuous aerosol profiles below decoupled clouds suggest that particles emitted at the surface are not transported to clouds in these conditions. It is concluded that the cloud-surface coupling state and free tropospheric particle abundance are crucial when assessing the aerosol budget for Arctic low-level clouds over sea ice.
Ascent rate of jimsphere balloons indicating vertical air currents
Wind vector change with respect to time at Cape Kennedy, Florida, is examined according to the theory of multivariate normality. The joint distribution of the four variables represented by the components of the wind vector at an initial time and after a specified elapsed time is hypothesized to be quadravariate normal; the fourteen statistics of this distribution, calculated from fifteen years of twice daily Rawinsonde data are presented by monthly reference periods for each month from 0 to 27 km. The hypotheses that the wind component changes with respect to time is univariate normal, the joint distribution of wind component changes is bivariate normal, and the modulus of vector wind change is Rayleigh, has been tested by comparison with observed distributions. Statistics of the conditional bivariate normal distributions of vector wind at a future time given the vector wind at an initial time are derived. Wind changes over time periods from one to five hours, calculated from Jimsphere data, are presented.
Ground level runway wind statistics cover crosswind, tailwind, and headwind reversal percentage frequencies with respect to month and hour for the two major runways. Also presented are bivariate normal wind statistics for a 90 degree flight azimuth for altitudes 0 through 27 km. Wind probability distributions, synthetic vector wind profiles, and statistics for any rotation of axes are computed from five given parameters.
Ground level runway wind statistics for the Edwards AFB, California area are presented. Crosswind, headwind, tailwind, and headwind reversal percentage frequencies are given with respect to month and hour for the two major Edwards AFB runways. Also presented are Edwards AFB bivariate normal wind statistics for a 90 degree flight azimuth for altitudes 0 through 27 km. Wind probability distributions and statistics for any rotation of axes can be computed from the five given parameters.