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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records

Retrieval of the molecular orientation distribution from atom-pair angular distributions

Imaging laser-induced rotational dynamics is an important and active field due to its applications in capturing reactions in the molecular frame and in molecular imaging. Experimental measurement of the molecular orientation distribution, as a function of the Euler angles, has only been demonstrated for special cases when the detectable signal is generated along the molecular symmetry axis. Here we developed the general theory that maps the probability density distribution of the molecular orientation to the atom-pair angular distributions for nonlinear molecules. With the theory, the molecular orientation distribution can be retrieved from the measured atom-pair angular distribution, which we demonstrate experimentally using ultrafast electron diffractive imaging of impulsively aligned trifluoro-iodomethane molecules. Here, the retrieved molecular orientation distribution is in good agreement with direct numerical simulations of the time-dependent Schrodinger equation using the experimental conditions. Unlike the existing retrieval methods, the retrieval method does not require solving Schrodinger equation, works for any alignment method, and is in principle applicable to asymmetric top molecules.

74 ATOMIC AND MOLECULAR PHYSICS↗

Measurement of the asymmetry in angular distributions of leptons produced in dilepton t t ¯ final states in p p ¯ collisions at s = 1.96 TeV

We present measurements of asymmetries in angular distributions of leptons produced in ttbar events in proton-antiproton collisions at the Fermilab Tevatron Collider. We consider final states where the W bosons from top quark and antiquark decays both decay into l nu (l=e, mu) resulting in oppositely charged dilepton final states with accompanying jets. Using 9.7 fb -1 of integrated luminosity collected with the D0 detector, we find the asymmetries in lepton pseudorapidity compatible with predictions based on the standard model.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Angular Distribution of Dimuons from Drell-Yan Production in p+Fe Interactions at 120 GeV Beam Energy

In the E906/SeaQuest Fermilab experiment, we report a measurement of the angular distributions by measuring the angular parameters $\lambda$, $\mu$, and $\nu$ of Drell-Yan dimuons produced using a 120 GeV proton beam incident on an iron target. The angular distribution in the naive Drell-Yan model does not show any $\cos2\phi$ dependency, where $\phi$ denotes the azimuthal angle of dimuons in the Collins-Soper frame. However, pion-induced Drell-Yan experiments, such as NA10 and E615, have observed a significant dependence on $\cos2\phi$. The Boer–Mulders function, a transverse momentum-dependent distribution function, represents the correlation between the transverse spin and the transverse momentum of the quark. A non-zero Boer-Mulders function or an improved higher-order Drell-Yan model considering QCD effects can produce a $\cos 2\phi$ modulation in the Drell-Yan angular distribution. To measure the angular distributions, we have used an event mixing method to construct the combin atorial background, which was then subtracted from the data to isolate the Drell-Yan signal. Following this, we corrected the detector, trigger, and reconstruction efficiencies using a doubly-iterative Bayesian Unfolding method. This iterative unfolding technique improves the response matrix based on the results of the previous unfolding step, ensuring robust convergence without exaggeration of uncertainties. The angular distributions of the dimuons were measured over the invariant mass range $5.0 < M_{\mu^+ \mu^-} < 8.0$ $GeV/c^2$, with dimuon transverse momentum $P_T < 2$ GeV/c and Feynman-x $-0.18 < x_F < 0.9$. The measured angular distributions are then compared with the QCD calculations for $p + \text{Fe}$ interactions, and proton-induced angular distribution measurements from other experiments. We have observed weak $\cos 2\phi$ modulations as a function of $P_T$. For $P_T > 1.0 \, \text{GeV}/c$, the predicted NNLO perturbative QCD value of $\nu$ is larger than what we have me asured at E906/SeaQuest. Moreover, we have not observed a strong dependence of $\nu$ on the kinematic variables, such as dimuon mass $M_{\mu^+ \mu^-}$ and Bjorken-$x$. The spin alignment of the virtual photon, $\lambda$, measured from the SeaQuest Drell-Yan $p+\text{Fe}$ data, is found to be strongly dependent on $P_T$, decreasing as $P_T$ increases. $\lambda$ also holds to the upper bound condition $\lambda < 1.0$ within the statistical uncertainty, showing a trend similar to that predicted by NNLO perturbative QCD. However, for $1.0 < P_T < 2.0 \, \text{GeV}/c$, the extracted $\lambda$ value from SeaQuest is smaller than that predicted by perturbative QCD at NNLO.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Effects of anisotropic electron-ion interactions in atomic photoelectron angular distributions

A summary of the angular momentum transfer formulation of the differential photoionization cross section is presented and photoionization amplitudes in LS coupling are considered. The application of the theoretical concepts and relations developed is illustrated with the aid of an example involving the calculation of the angular distribution of photoelectrons ionized from atomic sulfur according to a certain reaction. The investigation shows that anisotropic electron-ion interactions in atomic sulfur lead to measurable differences between photoelectron angular distribution asymmetry parameters corresponding to alternative ionic term levels.

Dill, D.↗

Photoelectron angular distributions from rotationally resolved autoionizing states of N 2

The single-photon, photoelectron-photoion coincidence spectrum of N 2 has been recorded at high (~1.5 cm -1 ) resolution in the region between the N 2 + X 2 Σ g + , v + = 0 and 1 ionization thresholds by using a double imaging spectrometer and intense vacuum-ultraviolet light from the Synchrotron SOLEIL. This approach provides the relative photoionization cross section, the photoelectron energy distribution, and the photoelectron angular distribution as a function of photon energy. The region of interest contains autoionizing valence states, vibrationally autoionizing Rydberg states converging to vibrationally excited levels of the N 2 + X 2 Σ g + ground state, and electronically autoionizing states converging to the N 2 + A 2 Π and B 2 Σ u + states. The wavelength resolution is sufficient to resolve rotational structure in the autoionizing states, but the electron energy resolution is insufficient to resolve rotational structure in the photoion spectrum. Here, a simplified approach based on multichannel quantum defect theory is used to predict the photoelectron angular distribution parameters, β, and the results are in reasonably good agreement with experiment.

74 ATOMIC AND MOLECULAR PHYSICS↗

Recent findings on angular distributions of dayside ring current energetic ions

The angular distributions observed in the equatorial region for energetic protons, helium ions, and carbon-nitrogen-oxygen ions are investigated. The anisotropy index for the ions in the equatorial magnetosphere between L shells is examined, and a variety of angular distributions different from simple pancake distributions are presented. The survey reveals unusual angular distributions which suggest for the first time a net field-aligned transport of energetic ring current ions and a sharp intensity enhancement over a pitch angle range centered at 90 deg. The latter reflects a sharp boundary of ring curent energetic ions at L of roughly 3 and 4, plausibly due to the addition of a newly injected population.

Lui, A. T. Y.↗

SU-E-I-44: Some Preliminary Analysis of Angular Distribution of X-Ray Scattered On Soft Tissues

Purpose: The angular distribution of x-radiation scattered at small angles (up to 16 degrees) from several different animal soft tissue (skin, fat, muscle, retina, etc) were measured using standard equipment devoted to study of crystal structure which provides excellent geometry conditions of measurements. showed measurable differences for different tissues. In the simplest possible case when measured samples do not differ in structure (different concentration solutions) it can be seen that intensity of scattered radiation is decreasing function of the concentration and the peak of the maximum of scattering distribution depends on the concentration as well. Methods: An x-ray scattering profile usually consists of sharp diffraction peak; however some properties of the spatial profiles of scattered radiation as intensity, the peak position, height, area, FWHM, the ratio of peak heights, etc. Results: The data contained measurable differences for different tissues. In the simplest possible case when measured samples do not differ in structure (different concentration solutions) it can be seen that intensity of scattered radiation is decreasing function of the concentration and the peak of the maximum of scattering distribution depends on the concentration as well. Measurements of different samples in the very preliminary phase showed that simple biological material used in study showed slightly different scattering pattern, especially at higher angles (around 10degrees). Intensity of radiation scattered from same tissue type is very dependent on water content and several more parameters. Conclusion: This preliminary study using animal soft tissues on the angular distributions of scattered x-rays suggests that angular distributions of X-rays scattered off of soft tissues might be useful in distinguishing healthy tissue from malignant soft tissue.

60 APPLIED LIFE SCIENCES↗

Evolution of the angular distribution of laser-generated fast electrons due to resistive self-collimation

The evolution of the angular distribution of laser-generated fast electrons propagating in dense plasmas is studied by 3D numerical simulations. As resistively generated magnetic fields can strongly influence and even pinch the fast electron beam, the question of the effect on the angular distribution is of considerable interest. It was conjectured that in the limit of strong collimation, there will only be minimal changes to the angular distribution, whereas the largest reduction in the angular distribution will occur where there is only modest pinching of the fast electron beam and the beam is able to expand considerably. The results of the numerical simulations indicate this conjecture.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Scattering Angular Distributions in the ENDF/B Nuclear Data Library

Nuclear reactors function by controlling the chain reaction of fission events in a fissile material. Understanding the gain and loss of neutrons is crucial for controlling this chain reaction. The role of fission in liberating neutrons from nuclei is well known. The fact that neutrons can scatter out of a reactor and therefore be lost is less well appreciated. Scattering can happen within fissile fuel or off of any number of the non-fissile structural components holding a reactor together. The scattering angular distributions for reactor material are the quantity that give the probability for a particle (usually a neutron) to scatter off a nucleus into a given angle. The Evaluated Nuclear Data File/B (ENDF/B) nuclear data library is the most complete and authoritative reference for neutron scattering data, containing reaction cross sections and outgoing particle distributions (including scattering angular distributions). In this project, we will compare the scattering angular distributions given in these ENDF/B data sets with those that can be derived using the Blatt-Biedenharn formalism and the resolved resonance data also in the ENDF/B files. More comparisons between the scattering angular distributions of relevant isotopes will help identify and correct any errors in the ENDF/B files. The results of this study will be an important component of the next major release of the ENDF/B library.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Probing light quark Yukawa couplings through angularity distributions in Higgs boson decay

We propose to utilize angularity distributions in Higgs boson decay to probe light quark Yukawa couplings at e + e - colliders. Angularities $τ$ a are a class of 2-jet event shapes with variable and tunable sensitivity to the distribution of radiation in hadronic jets in the final state. Using soft-collinear effective theory (SCET), we present a prediction of angularity distributions from Higgs decaying to quark and gluon states at e + e - colliders to NNLL + $\mathcal{O}$(α s ) accuracy. Due to the different color structures in quark and gluon jets, the angularity distributions from H → $q\overline{q}$ and H → gg show different behaviors and can be used to constrain the light quark Yukawa couplings. We show that the upper limit of light quark Yukawa couplings could be probed to the level of ~ 15% of the bottom quark Yukawa coupling in the Standard Model in a conservative analysis window far away from nonperturbative effects and other uncertainties; the limit can be pushed to ≲ 7 – 9% with better control of the nonperturbative effects especially on gluon angularity distributions and/or with multiple angularities.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Ion and electron angular distributions in the Io torus region of the Jovian magnetosphere

Angular distributions are presented of ion (about 0.5-2 MeV) and electron (greater than 10 MeV) fluxes measured during the Voyager 1 spacecraft passage through the inner regions of the Jovian magnetosphere. In the regions of peak flux intensities, just outside the orbit of Io, the ion angular distributions are most sharply peaked at 90 deg local pitch angle, a configuration consistent with diffusion of the particles inward from large radial distances. Inside the orbit of Io the lower-energy ions exhibit angular distributions depleted at 90 deg local pitch angles, suggesting the possibility of charge-exchange scattering loss of these particles. In the vicinity of the Io flux tube, no significant effect is observed in the flux or pitch angle distributions of the ions. The relativistic electrons are depleted in the flux tube region and exhibit an asymmetrical pitch angle distribution, with more electrons appearing to arrive from the equatorial region (the direction of Io) than from the low-altitude mirror point.

Lanzerotti, L. J.↗

Constructing angular distributions of neutrinos in core-collapse supernovae from zeroth and first moments calibrated by full Boltzmann neutrino transport

Two-moment neutrino transport methods have been widely used for developing theoretical models of core-collapse supernovae (CCSN), since they substantially reduce the computational burden inherent in the multidimensional neutrino-radiation hydrodynamical simulations. The approximation, however, comes at a price; the detailed structure of angular distribution of neutrinos is sacrificed, that is the main drawback of this approach. In this paper, we develop a novel method by which to construct angular distributions of neutrinos from the zeroth and first angular moments. In our method, the angular distribution is expressed with two quadratic functions of the neutrino angle in a piecewise fashion. We determine the best parameters in the fitting function by comparing to the neutrino data in a spherically symmetric CCSN model with full Boltzmann neutrino transport. We demonstrate the capability of our method by using our recent 2D CCSN model. In this work, we find that the essential features of the angular distributions can be well reconstructed, whereas the angular distributions of incoming neutrinos tend to have large errors that increase with flux factor ($\textit{κ}$). This issue originates from the insensitiveness of incoming neutrinos to $\textit{κ}$, that is an intrinsic limitation in moment methods. Based on the results of the demonstration, we assess the reliability of electron- neutrinos lepton number (ELN)-crossing searches with the two-moment neutrino transport. This analysis is complementary to our [L. Johns and H. Nagakura arXiv:2104.04106] that scrutinizes the limitation of crossing searches with a few moments. We find that the systematic errors of angular distributions for incoming neutrinos lead to misjudgements of the crossing at $\textit{κ}$ ≳ 0.5. This casts doubt on the results of ELN-crossing searches based on two-moment methods in some previous studies.

79 ASTRONOMY AND ASTROPHYSICS↗

Application of Simplified Pn Approximation to Angular Distribution of Neutron Source in MOC Calculations

Concept of the simplified Pn approximation is applied to represent angular distribution of anisotropic scattering source in order to decrease number of angular flux moments stored during transport sweeps. In practical design calculations, anisotropic scattering is usually taken into account through transport correction. Though the transport correction yields a reasonable result for many cases, detail treatment of anisotropic scattering is desirable in high fidelity neutronics calculations, e.g., a direct heterogeneous transport calculation in three dimensional geometry. Direct treatment of anisotropic scattering has been established, which commonly utilizes the series expansion by the spherical harmonics functions. The expansion by the spherical harmonics functions requires (L + 1){sup 2} angular flux moments when up to L-th order anisotropy is taken into account. The previous studies suggested that consideration up to P3 anisotropic scattering yields converged results in many neutronics analysis for LWR. In this case, (3 + 1){sup 2} = 16 angular flux moments should be stored and retained in each flux region of each energy group. This storage requirement would be significant in a large scale calculation with many flux regions and energy groups. Chao et al. proposed an explicit angular flux representation based on the simplified Pn (SPn) method. Number of angular flux moments required in a SPn calculation is (L + 1) when L-th order angular distribution is considered. Since the SPn method adopts the physical picture of 'locally 1D system' along particular direction, required number of angular flux moments is much smaller than that based on the spherical harmonics functions. In the present study, concept of the SPn method is applied to describe angular distribution of anisotropic scattering source. By adopting the SPn approximation, as described above, number of angular flux moments can be significantly reduced. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Anisotropy in fission fragment and prompt neutron angular distributions

Several physics mechanisms can lead to the deviation from an isotropic angular distribution for both fission fragments and the neutrons that are emitted during the fission event. Two of these effects have recently been implemented into CGMF, the Monte Carlo fission event generator developed at Los Alamos National Laboratory: angular distribution sampling for fission fragments and pre-equilibrium neutrons (those emitted before the compound nucleus forms). Using these new developments, we show that the anisotropy of the neutrons reflects the anisotropy of the fission fragments, in particular as the outgoing energy of neutrons increases. Correlations between the fission fragment and neutron anisotropies could be used to extract the fission fragment anisotropy from the neutron angular distributions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Neutron angular distribution in plutonium-240 spontaneous fission

Nuclear safeguards applications require accurate fission models that exhibit prompt neutron anisotropy. We observed an anisotropic neutron angular distribution, in the laboratory reference frame, because prompt fission neutrons carry momentum from fully accelerated fission fragments. Furthermore, a liquid organic scintillation detector array was used with pulse shape discrimination techniques to produce neutron-neutron cross-correlation time distributions and angular distributions from spontaneous fission in a 252 Cf, a 0.84 g 240 Pu eff metal, and a 1.63 g 240 Pu eff metal sample. The effect of cross-talk, estimated with MCNPX-PoliMi simulations, is removed from neutron-neutron coincidences as a function of the angle between detector pairs. Fewer coincidences were observed at detector angles near 90°, relative to higher and lower detector angles. As light output threshold increases, the observed anisotropy increases due to spectral effects arising from fission fragment momentum transfer to emitted neutrons. Stronger anisotropy was observed in Cf-252 spontaneous fission prompt neutrons than in Pu-240 neutrons.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Off-resonance photoemission dynamics studied by recoil frame F1s and C1s photoelectron angular distributions of CH{sub 3}F

F1s and C1s photoelectron angular distributions are considered for CH{sub 3}F, a molecule which does not support any shape resonance. In spite of the absence of features in the photoionization cross section profile, the recoil frame photoelectron angular distributions (RFPADs) exhibits dramatic changes depending on both the photoelectron energy and polarization geometry. Time-dependent density functional theory calculations are also given to rationalize the photoionization dynamics. The RFPADs have been compared with the theoretical calculations, in order to assess the accuracy of the theoretical method and rationalize the experimental findings. The effect of finite acceptance angles for both ionic fragments and photoelectrons has been included in the calculations, as well as the effect of rotational averaging around the fragmentation axis. Excellent agreement between theory and experiment is obtained, confirming the good quality of the calculated dynamical quantities (dipole moments and phase shifts)

74 ATOMIC AND MOLECULAR PHYSICS↗